Active learning(AL)trains a high-precision predictor model from small numbers of labeled data by iteratively annotating the most valuable data sample from an unlabeled data pool with a class label throughout the learn...Active learning(AL)trains a high-precision predictor model from small numbers of labeled data by iteratively annotating the most valuable data sample from an unlabeled data pool with a class label throughout the learning process.However,most current AL methods start with the premise that the labels queried at AL rounds must be free of ambiguity,which may be unrealistic in some real-world applications where only a set of candidate labels can be obtained for selected data.Besides,most of the existing AL algorithms only consider the case of centralized processing,which necessitates gathering together all the unlabeled data in one fusion center for selection.Considering that data are collected/stored at different nodes over a network in many real-world scenarios,distributed processing is chosen here.In this paper,the issue of distributed classification of partially labeled(PL)data obtained by a fully decentralized AL method is focused on,and a distributed active partial label learning(dAPLL)algorithm is proposed.Our proposed algorithm is composed of a fully decentralized sample selection strategy and a distributed partial label learning(PLL)algorithm.During the sample selection process,both the uncertainty and representativeness of the data are measured based on the global cluster centers obtained by a distributed clustering method,and the valuable samples are chosen in turn.Meanwhile,using the disambiguation-free strategy,a series of binary classification problems can be constructed,and the corresponding cost-sensitive classifiers can be cooperatively trained in a distributed manner.The experiment results conducted on several datasets demonstrate that the performance of the dAPLL algorithm is comparable to that of the corresponding centralized method and is superior to the existing active PLL(APLL)method in different parameter configurations.Besides,our proposed algorithm outperforms several current PLL methods using the random selection strategy,especially when only small amounts of data are selected to be assigned with the candidate labels.展开更多
Mechanical degradation, especially fractures in active particles in an electrode, is a major reason why the capacity of lithiumion batteries fades. This paper proposes a model that couples Li-ion diffusion, stress evo...Mechanical degradation, especially fractures in active particles in an electrode, is a major reason why the capacity of lithiumion batteries fades. This paper proposes a model that couples Li-ion diffusion, stress evolution, and damage mechanics to simulate the growth of central cracks in cathode particles(Li Mn_2 O_4) by an extended finite element method by considering the influence of multiple factors. The simulation shows that particles are likely to crack at a high discharge rate, when the particle radius is large, or when the initial central crack is longer. It also shows that the maximum principal tensile stress decreases and cracking becomes more difficult when the influence of crack surface diffusion is considered. The fracturing process occurs according to the following stages: no crack growth, stable crack growth, and unstable crack growth. Changing the charge/discharge strategy before unstable crack growth sets in is beneficial to prevent further capacity fading during electrochemical cycling.展开更多
Transport of passive particles induced by chiral-active particles in microchannel is investigated by using the overdamped Langevin dynamics simulation in a two-dimensional model system. Due to the chirality of active ...Transport of passive particles induced by chiral-active particles in microchannel is investigated by using the overdamped Langevin dynamics simulation in a two-dimensional model system. Due to the chirality of active particles and special structure of microchannel, effective ratchet transport of passive particles is achieved. Effective transport of passive particles depends on the width of microchannel(d), the density(ρ), and the angular velocity(ω) of chiral-active particles.There exist optimal parameters for d and ω at which the transport efficiency for passive particles takes its maximal value.This investigation can help us understand the necessity of active motion for living systems to maintain a number of vital processes such as materials transport inside cells and the foraging dynamics of mobile organisms.展开更多
The dynamics of two-dimensional rigid circles filled with chiral active particles are investigated by employing the overdamped Langevin dynamics simulations. Unidirectional rotation of rigid circles is observed, and t...The dynamics of two-dimensional rigid circles filled with chiral active particles are investigated by employing the overdamped Langevin dynamics simulations. Unidirectional rotation of rigid circles is observed, and the rotational angular velocity(ω) relies mainly on the length(l), the number(nB), and tilt angle(γ) of boards, and the angular velocity(ω)and area fraction(ρ) of chiral active particles. There are optimum values for these parameters at which the average angular velocity of circle reaches its maximum. The center-of-mass mean square displacement for circles drops by about two orders of magnitude for large angular velocity ω of chiral active particles with oscillations in the short-time regime. Our work demonstrates that nanofabricated objects with suitable designs immersed in a bath of chiral active particles can extract and rectify energy in a unidirectional motion.展开更多
Collective motion of active particles with polar alignment is investigated on a sphere.We discussed the factors that affect particle swarm motion and define an order parameter that can show the degree of particle swar...Collective motion of active particles with polar alignment is investigated on a sphere.We discussed the factors that affect particle swarm motion and define an order parameter that can show the degree of particle swarm motion.In the model,we added a polar alignment strength,along with Gaussian curvature,affecting particles swarm motion.We find that when the force exceeds a certain limit,the order parameter will decrease with the increase of the force.Combined with our definition of order parameter and observation of the model,the reason is that particles begin to move side by side under the influence of polar forces.In addition,the effects of velocity,rotational diffusion coefficient,and packing fraction on particle swarm motion are discussed.It is found that the rotational diffusion coefficient and the packing fraction have a great influence on the clustering motion of particles,while the velocity has little influence on the clustering motion of particles.展开更多
The demand on low-carbon emission fabrication technologies for energy storage materials is increasing dramatically with the global interest on carbon neutrality.As a promising active material for metal-sulfur batterie...The demand on low-carbon emission fabrication technologies for energy storage materials is increasing dramatically with the global interest on carbon neutrality.As a promising active material for metal-sulfur batteries,sulfur is of great interest due to its high-energy-density and abundance.However,there is a lack of industry-friendly and low-carbon fabrication strategies for high-performance sulfur-based active particles,which,however,is in critical need by their practical success.Herein,based on a hail-inspired sulfur nano-storm(HSN)technology developed in our lab,we report an energy-saving,solvent-free strategy for producing core-shell sulfur/carbon electrode particles(CNT@AC-S)in minutes.The fabrication of the CNT@AC-S electrode particles only involves low-cost sulfur blocks,commercial carbon nanotubes(CNT)and activated carbon(AC)micro-particles with high specific surface area.Based on the above core-shell CNT@AC-S particles,sulfur cathode with a high sulfur-loading of 9.2 mg cm^(-2) delivers a stable area capacity of 6.6 mAh cm^(-2) over 100 cycles.Furthermore,even for sulfur cathode with a super-high sulfur content(72 wt%over the whole electrode),it still delivers a high area capacity of 9 mAh cm^(-2) over50 cycles in a quasi-lean electrolyte condition.In a nutshell,this study brings a green and industryfriendly fabrication strategy for cost-effective production of rationally designed S-rich electrode particles.展开更多
The pharmacodynamic active parts of protecting liver of Peristrope japonica (thunb.)Bremek were identified. Rat acute liver injury model was induced by D-galactosamine (D-GlaN). The active parts were identified on the...The pharmacodynamic active parts of protecting liver of Peristrope japonica (thunb.)Bremek were identified. Rat acute liver injury model was induced by D-galactosamine (D-GlaN). The active parts were identified on the whole extraction and 4 fractions. The results showed that the pharmacodynamic active parts of Peristrope japonica were the n-BuOH fraction.展开更多
The experience of the mankind in studying the planet of our own, is long and the progress is accelerated. From the numerous geographic adventures organized in the past thousand years came only the brief knowledge of t...The experience of the mankind in studying the planet of our own, is long and the progress is accelerated. From the numerous geographic adventures organized in the past thousand years came only the brief knowledge of the outline of the land and ocean; with the scientific explorations and topographic mapping activities done in the 300-plus years that followed, only about 30% of the land got mapped. But things have been changed greatly since the beginning of the century, when the air planes were put into use for mapping: up to 1950’s, the mapped areas had gone up to 70%; From 1957, a series of resource and environment satellites have been launched one after another,observing the globe, giving coverage of it and providing endlessly varieties of information about the seas and the lands day and night.展开更多
This is a progress report of a major project that Institute of Astronomy & Astrophysics is actively engaged. The two 6m sub millimeter telescopes are being built in Taiwan. The construction of the antennas, which ...This is a progress report of a major project that Institute of Astronomy & Astrophysics is actively engaged. The two 6m sub millimeter telescopes are being built in Taiwan. The construction of the antennas, which has been contracted to Aeronautic Research Laboratory, has made good progress lately. The first reflector is completed. The mounts are also nearly finished. The antennas are expected to be completed and tested in late 1999. Our receiver lab has been built up from scratch. It is finishing the assembly of the first SMA receiver. It is also fabricating its first Nb AlO x Nb junction of 230 GHz. Our two telescopes are scheduled to join the two SAO telescopes presently at Mauna Kea in the spring of year 2000.展开更多
We simulate a two-dimensional model of a round soft boundary enclosed with self-propelled particles. Persistent motion drives these particles to accumulate near the boundary, thereby dramatically deforming the boundar...We simulate a two-dimensional model of a round soft boundary enclosed with self-propelled particles. Persistent motion drives these particles to accumulate near the boundary, thereby dramatically deforming the boundary shape through collisions. Quantitative analyses of the boundary shape and the particle distribution show that there are two typical regimes in the variation of the morphology with the increase of self-propulsion of particles. One is under small forces, characterized by the radially inhomogeneous distribution of particles and the suppression of local fluctuations of the almost round boundary, and the other is under large forces, featured by the angularly inhomogeneous distribution of particles and the global shape deformation of the boundary. These two features are strongly cooperative. We also find different mechanisms in the particle relocation at low and high particle concentrations.展开更多
We study the collective motion of active particles in environmental noise, where the environmental noise is caused by noise particles randomly diffusing in two-dimensional space. We show that active particles in a noi...We study the collective motion of active particles in environmental noise, where the environmental noise is caused by noise particles randomly diffusing in two-dimensional space. We show that active particles in a noisy environment can self organize into three typical phases: polar liquid, band, and disordered gas states. In our model, the transition between band and disordered gas states is discontinuous. Giant number fluctuation is observed in the polar liquid phase. We also compare our results with the Vicsek model and show that the interaction with noise particles can stabilize the band state to very low noise condition. This band structure could recruit most of the active particles in the system, which greatly enhances the coherence of the system. Our findings of complex collective behaviors in environmental noise help us to understand how individuals modify their self-organization by environmental factors, which may further contribute to improving the design of collective migration and navigation strategies.展开更多
This paper focuses on a beginner adult ESL classroom aiming to enhance their participation under the guidance of“taskbased teaching”method. By incorporating three strategies of priming students to elicit their prior...This paper focuses on a beginner adult ESL classroom aiming to enhance their participation under the guidance of“taskbased teaching”method. By incorporating three strategies of priming students to elicit their prior knowledge on certain topic, designing a sequence of tasks to scaffold students for the final produce and modelling with lower level students to ensure their under? standing of task instructions, the activeness could see a significant increase.展开更多
In the framework of vigorous promotion of low-carbon power system growth as well as economic globalization,multi-resource penetration in active distribution networks has been advancing fiercely.In particular,distribut...In the framework of vigorous promotion of low-carbon power system growth as well as economic globalization,multi-resource penetration in active distribution networks has been advancing fiercely.In particular,distributed generation(DG)based on renewable energy is critical for active distribution network operation enhancement.To comprehensively analyze the accessing impact of DG in distribution networks from various parts,this paper establishes an optimal DG location and sizing planning model based on active power losses,voltage profile,pollution emissions,and the economics of DG costs as well as meteorological conditions.Subsequently,multiobjective particle swarm optimization(MOPSO)is applied to obtain the optimal Pareto front.Besides,for the sake of avoiding the influence of the subjective setting of the weight coefficient,the decisionmethod based on amodified ideal point is applied to execute a Pareto front decision.Finally,simulation tests based on IEEE33 and IEEE69 nodes are designed.The experimental results show thatMOPSO can achieve wider and more uniformPareto front distribution.In the IEEE33 node test system,power loss,and voltage deviation decreased by 52.23%,and 38.89%,respectively,while taking the economy into account.In the IEEE69 test system,the three indexes decreased by 19.67%,and 58.96%,respectively.展开更多
The development of precise and sensitive electrophysiological recording platforms holds the utmost importance for research in the fields of cardiology and neuroscience.In recent years,active micro/nano-bioelectronic d...The development of precise and sensitive electrophysiological recording platforms holds the utmost importance for research in the fields of cardiology and neuroscience.In recent years,active micro/nano-bioelectronic devices have undergone significant advancements,thereby facilitating the study of electrophysiology.The distinctive configuration and exceptional functionality of these active micro-nano-collaborative bioelectronic devices offer the potential for the recording of high-fidelity action potential signals on a large scale.In this paper,we review three-dimensional active nano-transistors and planar active micro-transistors in terms of their applications in electroexcitable cells,focusing on the evaluation of the effects of active micro/nano-bioelectronic devices on electrophysiological signals.Looking forward to the possibilities,challenges,and wide prospects of active micro-nano-devices,we expect to advance their progress to satisfy the demands of theoretical investigations and medical implementations within the domains of cardiology and neuroscience research.展开更多
The efficient separation and collection of ammonia(NH_(3))during NH_(3) synthesis process is essential to improve the economic efficiency and protect the environment.In this work,ethanolammonium hydrochloride(EtOHACl)...The efficient separation and collection of ammonia(NH_(3))during NH_(3) synthesis process is essential to improve the economic efficiency and protect the environment.In this work,ethanolammonium hydrochloride(EtOHACl)and phenol(PhOH)were used to prepare a novel class of deep eutectic solvents(DESs)with multiple active sites and low viscosities.The NH_(3) separation performance of EtOHACl+PhOH DESs was analyzed completely.It is figured out that the NH_(3) absorption rates in EtOHACl+PhOH DESs are very fast.The NH_(3) absorption capacities are very high and reach up to 5.52 and 10.74 mol·kg1 at 11.2 and 100.4 kPa under 298.2 K,respectively.In addition,the EtOHACl+PhOH DESs present highly selective absorption of NH_(3) over N_(2) and H_(2) and good regenerative properties after seven cycles of absorption/desorption.The intrinsic separation mechanism of NH_(3) by EtOHACl+PhOH DESs was further revealed by spectroscopic analysis and quantum chemistry calculations.展开更多
Phosphate removal is crucial for eutrophication control and water quality improvement.Electro-assisted adsorption,an eco-friendly elec-trosorption process,exhibited a promising potential for wastewater treatment.Howev...Phosphate removal is crucial for eutrophication control and water quality improvement.Electro-assisted adsorption,an eco-friendly elec-trosorption process,exhibited a promising potential for wastewater treatment.However,there are few works focused on phosphate electro-sorption,and reported electrodes cannot attach satisfactory removal capacities and rates.Herein,electro-assisted adsorption of phosphate via in-situ construction of La active centers on hierarchically porous carbon(LaPC)has been originally demonstrated.The resulted LaPC composite not only possessed a hierarchically porous structure with uniformly dispersed La active sites,but also provided good conductivity for interfacial electron transfer.The LaPC electrode achieved an ultrahigh phosphate electrosorption capability of 462.01 mg g^(-1) at 1 V,outperforming most existing electrodes.The superior phosphate removal performance originates from abundant active centers formed by the coupling of electricfield and capture sites.Besides,the stability and selectivity toward phosphate capture were maintained well even under comprehensive conditions.Moreover,a series of kinetics and isotherms models were employed to validate the electrosorption process.This work demonstrates a deep understanding and promotes a new level of phosphate electrosorption.展开更多
The Sichuan-Tibet transportation corridor is prone to numerous active faults and frequent strong earthquakes.While extensive studies have individually explored the effect of active faults and strong earthquakes on dif...The Sichuan-Tibet transportation corridor is prone to numerous active faults and frequent strong earthquakes.While extensive studies have individually explored the effect of active faults and strong earthquakes on different engineering structures,their combined effect remains unclear.This research employed multiple physical model tests to investigate the dynamic response of various engineering structures,including tunnels,bridges,and embankments,under the simultaneous influence of cumulative earthquakes and stick-slip misalignment of an active fault.The prototype selected for this study was the Kanding No.2 tunnel,which crosses the Yunongxi fault zone within the Sichuan-Tibet transportation corridor.The results demonstrated that the tunnel,bridge,and embankment exhibited amplification in response to the input seismic wave,with the amplification effect gradually decreasing as the input peak ground acceleration(PGA)increased.The PGAs of different engineering structures were weakened by the fault rupture zone.Nevertheless,the misalignment of the active fault may decrease the overall stiffness of the engineering structure,leading to more severe damage,with a small contribution from seismic vibration.Additionally,the seismic vibration effect might be enlarged with the height of the engineering structure,and the tunnel is supposed to have a smaller PGA and lower dynamic earth pressure compared to bridges and embankments in strong earthquake zones crossing active faults.The findings contribute valuable insights for evaluating the dynamic response of various engineering structures crossing an active fault and provide an experimental reference for secure engineering design in the challenging conditions of the Sichuan-Tibet transportation corridor.展开更多
Active tectonics in an area includes ongoing or recent geologic events.This paper investigates the tectonic influence on the subsidence,uplift and tilt of western Saurashtra through morphotectonic analysis of ten wate...Active tectonics in an area includes ongoing or recent geologic events.This paper investigates the tectonic influence on the subsidence,uplift and tilt of western Saurashtra through morphotectonic analysis of ten watersheds along with characteristics of relief and drainage orientation.Watersheds 7-9 to the north(N)are tectonically active,which can be linked with the North Kathiawar Fault System(NKFS)and followed by watersheds 6,10,1,4 and 5.Stream-length gradient index and sinuosity index indicate the effect of tectonic events along the master streams in watersheds 6-9.Higher R^(2)values of the linear curve fit for watershed 7 indicate its master stream is much more tectonically active than the others.The R^(2)curve fitting model and earthquake magnitude/depth analysis confirm the region to be active.The reactivation of the NKFS most likely led to the vertical movement of western Saurashtra.展开更多
This paper proposes a modified iterative learning control(MILC)periodical feedback-feedforward algorithm to reduce the vibration of a rotor caused by coupled unbalance and parallel misalignment.The control of the vibr...This paper proposes a modified iterative learning control(MILC)periodical feedback-feedforward algorithm to reduce the vibration of a rotor caused by coupled unbalance and parallel misalignment.The control of the vibration of the rotor is provided by an active magnetic actuator(AMA).The iterative gain of the MILC algorithm here presented has a self-adjustment based on the magnitude of the vibration.Notch filters are adopted to extract the synchronous(1×Ω)and twice rotational frequency(2×Ω)components of the rotor vibration.Both the notch frequency of the filter and the size of feedforward storage used during the experiment have a real-time adaptation to the rotational speed.The method proposed in this work can provide effective suppression of the vibration of the rotor in case of sudden changes or fluctuations of the rotor speed.Simulations and experiments using the MILC algorithm proposed here are carried out and give evidence to the feasibility and robustness of the technique proposed.展开更多
Aqueous Zn-ion batteries(AZIBs)have attracted increasing attention in next-generation energy storage systems due to their high safety and economic.Unfortunately,the side reactions,dendrites and hydrogen evolution effe...Aqueous Zn-ion batteries(AZIBs)have attracted increasing attention in next-generation energy storage systems due to their high safety and economic.Unfortunately,the side reactions,dendrites and hydrogen evolution effects at the zinc anode interface in aqueous electrolytes seriously hinder the application of aqueous zinc-ion batteries.Here,we report a critical solvation strategy to achieve reversible zinc electrochemistry by introducing a small polar molecule acetonitrile to form a“catcher”to arrest active molecules(bound water molecules).The stable solvation structure of[Zn(H_(2)O)_(6)]^(2+)is capable of maintaining and completely inhibiting free water molecules.When[Zn(H_(2)O)_(6)]^(2+)is partially desolvated in the Helmholtz outer layer,the separated active molecules will be arrested by the“catcher”formed by the strong hydrogen bond N-H bond,ensuring the stable desolvation of Zn^(2+).The Zn||Zn symmetric battery can stably cycle for 2250 h at 1 mAh cm^(-2),Zn||V_(6)O_(13) full battery achieved a capacity retention rate of 99.2%after 10,000 cycles at 10 A g^(-1).This paper proposes a novel critical solvation strategy that paves the route for the construction of high-performance AZIBs.展开更多
基金supported by the National Natural Science Foundation of China(62201398)Natural Science Foundation of Zhejiang Province(LY21F020001),Science and Technology Plan Project of Wenzhou(ZG2020026).
文摘Active learning(AL)trains a high-precision predictor model from small numbers of labeled data by iteratively annotating the most valuable data sample from an unlabeled data pool with a class label throughout the learning process.However,most current AL methods start with the premise that the labels queried at AL rounds must be free of ambiguity,which may be unrealistic in some real-world applications where only a set of candidate labels can be obtained for selected data.Besides,most of the existing AL algorithms only consider the case of centralized processing,which necessitates gathering together all the unlabeled data in one fusion center for selection.Considering that data are collected/stored at different nodes over a network in many real-world scenarios,distributed processing is chosen here.In this paper,the issue of distributed classification of partially labeled(PL)data obtained by a fully decentralized AL method is focused on,and a distributed active partial label learning(dAPLL)algorithm is proposed.Our proposed algorithm is composed of a fully decentralized sample selection strategy and a distributed partial label learning(PLL)algorithm.During the sample selection process,both the uncertainty and representativeness of the data are measured based on the global cluster centers obtained by a distributed clustering method,and the valuable samples are chosen in turn.Meanwhile,using the disambiguation-free strategy,a series of binary classification problems can be constructed,and the corresponding cost-sensitive classifiers can be cooperatively trained in a distributed manner.The experiment results conducted on several datasets demonstrate that the performance of the dAPLL algorithm is comparable to that of the corresponding centralized method and is superior to the existing active PLL(APLL)method in different parameter configurations.Besides,our proposed algorithm outperforms several current PLL methods using the random selection strategy,especially when only small amounts of data are selected to be assigned with the candidate labels.
基金support of the National Natural Science Foundation of China (11472165 and 11332005)
文摘Mechanical degradation, especially fractures in active particles in an electrode, is a major reason why the capacity of lithiumion batteries fades. This paper proposes a model that couples Li-ion diffusion, stress evolution, and damage mechanics to simulate the growth of central cracks in cathode particles(Li Mn_2 O_4) by an extended finite element method by considering the influence of multiple factors. The simulation shows that particles are likely to crack at a high discharge rate, when the particle radius is large, or when the initial central crack is longer. It also shows that the maximum principal tensile stress decreases and cracking becomes more difficult when the influence of crack surface diffusion is considered. The fracturing process occurs according to the following stages: no crack growth, stable crack growth, and unstable crack growth. Changing the charge/discharge strategy before unstable crack growth sets in is beneficial to prevent further capacity fading during electrochemical cycling.
基金supported by the National Natural Science Foundation of China(Grant Nos.21374102,21674096,and 21674082)
文摘Transport of passive particles induced by chiral-active particles in microchannel is investigated by using the overdamped Langevin dynamics simulation in a two-dimensional model system. Due to the chirality of active particles and special structure of microchannel, effective ratchet transport of passive particles is achieved. Effective transport of passive particles depends on the width of microchannel(d), the density(ρ), and the angular velocity(ω) of chiral-active particles.There exist optimal parameters for d and ω at which the transport efficiency for passive particles takes its maximal value.This investigation can help us understand the necessity of active motion for living systems to maintain a number of vital processes such as materials transport inside cells and the foraging dynamics of mobile organisms.
基金Project supported by the National Natural Science Foundation of China(Grant Nos.21674096 and 21873082)
文摘The dynamics of two-dimensional rigid circles filled with chiral active particles are investigated by employing the overdamped Langevin dynamics simulations. Unidirectional rotation of rigid circles is observed, and the rotational angular velocity(ω) relies mainly on the length(l), the number(nB), and tilt angle(γ) of boards, and the angular velocity(ω)and area fraction(ρ) of chiral active particles. There are optimum values for these parameters at which the average angular velocity of circle reaches its maximum. The center-of-mass mean square displacement for circles drops by about two orders of magnitude for large angular velocity ω of chiral active particles with oscillations in the short-time regime. Our work demonstrates that nanofabricated objects with suitable designs immersed in a bath of chiral active particles can extract and rectify energy in a unidirectional motion.
基金supported in part by the National Natural Science Foundation of China(Grant Nos.12075090 and 12005066)the Science and Technology Program of Guangzhou(Grant No.2019050001)+1 种基金the Natural Science Foundation of Guangdong Province,China(Grant No.2017A030313029)the Major Basic Research Project of Guangdong Province,China(Grant No.2017KZDXM024)。
文摘Collective motion of active particles with polar alignment is investigated on a sphere.We discussed the factors that affect particle swarm motion and define an order parameter that can show the degree of particle swarm motion.In the model,we added a polar alignment strength,along with Gaussian curvature,affecting particles swarm motion.We find that when the force exceeds a certain limit,the order parameter will decrease with the increase of the force.Combined with our definition of order parameter and observation of the model,the reason is that particles begin to move side by side under the influence of polar forces.In addition,the effects of velocity,rotational diffusion coefficient,and packing fraction on particle swarm motion are discussed.It is found that the rotational diffusion coefficient and the packing fraction have a great influence on the clustering motion of particles,while the velocity has little influence on the clustering motion of particles.
基金supported by the Double First-Class Construction Funds of Sichuan University and National Natural Science Foundation of China(NNSFC)financial support from the National Science Foundation of China(51873126,51422305,51721091)。
文摘The demand on low-carbon emission fabrication technologies for energy storage materials is increasing dramatically with the global interest on carbon neutrality.As a promising active material for metal-sulfur batteries,sulfur is of great interest due to its high-energy-density and abundance.However,there is a lack of industry-friendly and low-carbon fabrication strategies for high-performance sulfur-based active particles,which,however,is in critical need by their practical success.Herein,based on a hail-inspired sulfur nano-storm(HSN)technology developed in our lab,we report an energy-saving,solvent-free strategy for producing core-shell sulfur/carbon electrode particles(CNT@AC-S)in minutes.The fabrication of the CNT@AC-S electrode particles only involves low-cost sulfur blocks,commercial carbon nanotubes(CNT)and activated carbon(AC)micro-particles with high specific surface area.Based on the above core-shell CNT@AC-S particles,sulfur cathode with a high sulfur-loading of 9.2 mg cm^(-2) delivers a stable area capacity of 6.6 mAh cm^(-2) over 100 cycles.Furthermore,even for sulfur cathode with a super-high sulfur content(72 wt%over the whole electrode),it still delivers a high area capacity of 9 mAh cm^(-2) over50 cycles in a quasi-lean electrolyte condition.In a nutshell,this study brings a green and industryfriendly fabrication strategy for cost-effective production of rationally designed S-rich electrode particles.
文摘The pharmacodynamic active parts of protecting liver of Peristrope japonica (thunb.)Bremek were identified. Rat acute liver injury model was induced by D-galactosamine (D-GlaN). The active parts were identified on the whole extraction and 4 fractions. The results showed that the pharmacodynamic active parts of Peristrope japonica were the n-BuOH fraction.
文摘The experience of the mankind in studying the planet of our own, is long and the progress is accelerated. From the numerous geographic adventures organized in the past thousand years came only the brief knowledge of the outline of the land and ocean; with the scientific explorations and topographic mapping activities done in the 300-plus years that followed, only about 30% of the land got mapped. But things have been changed greatly since the beginning of the century, when the air planes were put into use for mapping: up to 1950’s, the mapped areas had gone up to 70%; From 1957, a series of resource and environment satellites have been launched one after another,observing the globe, giving coverage of it and providing endlessly varieties of information about the seas and the lands day and night.
文摘This is a progress report of a major project that Institute of Astronomy & Astrophysics is actively engaged. The two 6m sub millimeter telescopes are being built in Taiwan. The construction of the antennas, which has been contracted to Aeronautic Research Laboratory, has made good progress lately. The first reflector is completed. The mounts are also nearly finished. The antennas are expected to be completed and tested in late 1999. Our receiver lab has been built up from scratch. It is finishing the assembly of the first SMA receiver. It is also fabricating its first Nb AlO x Nb junction of 230 GHz. Our two telescopes are scheduled to join the two SAO telescopes presently at Mauna Kea in the spring of year 2000.
基金supported by the National Natural Science Foundation of China(Grant Nos.21474074,21674078,21374073,and 21574096)
文摘We simulate a two-dimensional model of a round soft boundary enclosed with self-propelled particles. Persistent motion drives these particles to accumulate near the boundary, thereby dramatically deforming the boundary shape through collisions. Quantitative analyses of the boundary shape and the particle distribution show that there are two typical regimes in the variation of the morphology with the increase of self-propulsion of particles. One is under small forces, characterized by the radially inhomogeneous distribution of particles and the suppression of local fluctuations of the almost round boundary, and the other is under large forces, featured by the angularly inhomogeneous distribution of particles and the global shape deformation of the boundary. These two features are strongly cooperative. We also find different mechanisms in the particle relocation at low and high particle concentrations.
基金Project supported by the National Natural Science Foundation of China(Grant Nos.91427302,91027040,and 11474155)the National Basic Research Program of China(Grant No.2012CB821500)
文摘We study the collective motion of active particles in environmental noise, where the environmental noise is caused by noise particles randomly diffusing in two-dimensional space. We show that active particles in a noisy environment can self organize into three typical phases: polar liquid, band, and disordered gas states. In our model, the transition between band and disordered gas states is discontinuous. Giant number fluctuation is observed in the polar liquid phase. We also compare our results with the Vicsek model and show that the interaction with noise particles can stabilize the band state to very low noise condition. This band structure could recruit most of the active particles in the system, which greatly enhances the coherence of the system. Our findings of complex collective behaviors in environmental noise help us to understand how individuals modify their self-organization by environmental factors, which may further contribute to improving the design of collective migration and navigation strategies.
文摘This paper focuses on a beginner adult ESL classroom aiming to enhance their participation under the guidance of“taskbased teaching”method. By incorporating three strategies of priming students to elicit their prior knowledge on certain topic, designing a sequence of tasks to scaffold students for the final produce and modelling with lower level students to ensure their under? standing of task instructions, the activeness could see a significant increase.
基金The authors gratefully acknowledge the support of the Enhancement Strategy of Multi-Type Energy Integration of Active Distribution Network(YNKJXM20220113).
文摘In the framework of vigorous promotion of low-carbon power system growth as well as economic globalization,multi-resource penetration in active distribution networks has been advancing fiercely.In particular,distributed generation(DG)based on renewable energy is critical for active distribution network operation enhancement.To comprehensively analyze the accessing impact of DG in distribution networks from various parts,this paper establishes an optimal DG location and sizing planning model based on active power losses,voltage profile,pollution emissions,and the economics of DG costs as well as meteorological conditions.Subsequently,multiobjective particle swarm optimization(MOPSO)is applied to obtain the optimal Pareto front.Besides,for the sake of avoiding the influence of the subjective setting of the weight coefficient,the decisionmethod based on amodified ideal point is applied to execute a Pareto front decision.Finally,simulation tests based on IEEE33 and IEEE69 nodes are designed.The experimental results show thatMOPSO can achieve wider and more uniformPareto front distribution.In the IEEE33 node test system,power loss,and voltage deviation decreased by 52.23%,and 38.89%,respectively,while taking the economy into account.In the IEEE69 test system,the three indexes decreased by 19.67%,and 58.96%,respectively.
基金The work is supported in part by the National Natural Science Foundation of China(Grant Nos.62171483,82061148011)Zhejiang Provincial Natural Science Foundation of China(Grant No.LZ23F010004)+1 种基金Hangzhou Agricultural and Social Development Research Key Project(Grant No.20231203A08)Doctoral Initiation Program of the Tenth Affiliated Hospital,Southern Medical University(Grant No.K202308).
文摘The development of precise and sensitive electrophysiological recording platforms holds the utmost importance for research in the fields of cardiology and neuroscience.In recent years,active micro/nano-bioelectronic devices have undergone significant advancements,thereby facilitating the study of electrophysiology.The distinctive configuration and exceptional functionality of these active micro-nano-collaborative bioelectronic devices offer the potential for the recording of high-fidelity action potential signals on a large scale.In this paper,we review three-dimensional active nano-transistors and planar active micro-transistors in terms of their applications in electroexcitable cells,focusing on the evaluation of the effects of active micro/nano-bioelectronic devices on electrophysiological signals.Looking forward to the possibilities,challenges,and wide prospects of active micro-nano-devices,we expect to advance their progress to satisfy the demands of theoretical investigations and medical implementations within the domains of cardiology and neuroscience research.
基金supported by the National Natural Science Foundation of China(22221005 and 22008033).
文摘The efficient separation and collection of ammonia(NH_(3))during NH_(3) synthesis process is essential to improve the economic efficiency and protect the environment.In this work,ethanolammonium hydrochloride(EtOHACl)and phenol(PhOH)were used to prepare a novel class of deep eutectic solvents(DESs)with multiple active sites and low viscosities.The NH_(3) separation performance of EtOHACl+PhOH DESs was analyzed completely.It is figured out that the NH_(3) absorption rates in EtOHACl+PhOH DESs are very fast.The NH_(3) absorption capacities are very high and reach up to 5.52 and 10.74 mol·kg1 at 11.2 and 100.4 kPa under 298.2 K,respectively.In addition,the EtOHACl+PhOH DESs present highly selective absorption of NH_(3) over N_(2) and H_(2) and good regenerative properties after seven cycles of absorption/desorption.The intrinsic separation mechanism of NH_(3) by EtOHACl+PhOH DESs was further revealed by spectroscopic analysis and quantum chemistry calculations.
基金This work is financially supported by the National Science Foundation of Tianjin(17JCYBJC23300).
文摘Phosphate removal is crucial for eutrophication control and water quality improvement.Electro-assisted adsorption,an eco-friendly elec-trosorption process,exhibited a promising potential for wastewater treatment.However,there are few works focused on phosphate electro-sorption,and reported electrodes cannot attach satisfactory removal capacities and rates.Herein,electro-assisted adsorption of phosphate via in-situ construction of La active centers on hierarchically porous carbon(LaPC)has been originally demonstrated.The resulted LaPC composite not only possessed a hierarchically porous structure with uniformly dispersed La active sites,but also provided good conductivity for interfacial electron transfer.The LaPC electrode achieved an ultrahigh phosphate electrosorption capability of 462.01 mg g^(-1) at 1 V,outperforming most existing electrodes.The superior phosphate removal performance originates from abundant active centers formed by the coupling of electricfield and capture sites.Besides,the stability and selectivity toward phosphate capture were maintained well even under comprehensive conditions.Moreover,a series of kinetics and isotherms models were employed to validate the electrosorption process.This work demonstrates a deep understanding and promotes a new level of phosphate electrosorption.
基金supported by the National Natural Science Foundation of China(Grant Nos.41825018,41977248,42207219)the Second Tibetan Plateau Scientific Expedition and Research Program(STEP)(Grant No.2019QZKK0904)。
文摘The Sichuan-Tibet transportation corridor is prone to numerous active faults and frequent strong earthquakes.While extensive studies have individually explored the effect of active faults and strong earthquakes on different engineering structures,their combined effect remains unclear.This research employed multiple physical model tests to investigate the dynamic response of various engineering structures,including tunnels,bridges,and embankments,under the simultaneous influence of cumulative earthquakes and stick-slip misalignment of an active fault.The prototype selected for this study was the Kanding No.2 tunnel,which crosses the Yunongxi fault zone within the Sichuan-Tibet transportation corridor.The results demonstrated that the tunnel,bridge,and embankment exhibited amplification in response to the input seismic wave,with the amplification effect gradually decreasing as the input peak ground acceleration(PGA)increased.The PGAs of different engineering structures were weakened by the fault rupture zone.Nevertheless,the misalignment of the active fault may decrease the overall stiffness of the engineering structure,leading to more severe damage,with a small contribution from seismic vibration.Additionally,the seismic vibration effect might be enlarged with the height of the engineering structure,and the tunnel is supposed to have a smaller PGA and lower dynamic earth pressure compared to bridges and embankments in strong earthquake zones crossing active faults.The findings contribute valuable insights for evaluating the dynamic response of various engineering structures crossing an active fault and provide an experimental reference for secure engineering design in the challenging conditions of the Sichuan-Tibet transportation corridor.
基金Research Development Fund(IIT Bombay)supported SM。
文摘Active tectonics in an area includes ongoing or recent geologic events.This paper investigates the tectonic influence on the subsidence,uplift and tilt of western Saurashtra through morphotectonic analysis of ten watersheds along with characteristics of relief and drainage orientation.Watersheds 7-9 to the north(N)are tectonically active,which can be linked with the North Kathiawar Fault System(NKFS)and followed by watersheds 6,10,1,4 and 5.Stream-length gradient index and sinuosity index indicate the effect of tectonic events along the master streams in watersheds 6-9.Higher R^(2)values of the linear curve fit for watershed 7 indicate its master stream is much more tectonically active than the others.The R^(2)curve fitting model and earthquake magnitude/depth analysis confirm the region to be active.The reactivation of the NKFS most likely led to the vertical movement of western Saurashtra.
基金Supported by National Natural Science Foundation of China(Grant Nos.51975037,52375075).
文摘This paper proposes a modified iterative learning control(MILC)periodical feedback-feedforward algorithm to reduce the vibration of a rotor caused by coupled unbalance and parallel misalignment.The control of the vibration of the rotor is provided by an active magnetic actuator(AMA).The iterative gain of the MILC algorithm here presented has a self-adjustment based on the magnitude of the vibration.Notch filters are adopted to extract the synchronous(1×Ω)and twice rotational frequency(2×Ω)components of the rotor vibration.Both the notch frequency of the filter and the size of feedforward storage used during the experiment have a real-time adaptation to the rotational speed.The method proposed in this work can provide effective suppression of the vibration of the rotor in case of sudden changes or fluctuations of the rotor speed.Simulations and experiments using the MILC algorithm proposed here are carried out and give evidence to the feasibility and robustness of the technique proposed.
基金supported by the National Natural Science Foundation of China(No.52272198 and 52002122)the Project funded by China Postdoctoral Science Foundation(No.2021M690947).
文摘Aqueous Zn-ion batteries(AZIBs)have attracted increasing attention in next-generation energy storage systems due to their high safety and economic.Unfortunately,the side reactions,dendrites and hydrogen evolution effects at the zinc anode interface in aqueous electrolytes seriously hinder the application of aqueous zinc-ion batteries.Here,we report a critical solvation strategy to achieve reversible zinc electrochemistry by introducing a small polar molecule acetonitrile to form a“catcher”to arrest active molecules(bound water molecules).The stable solvation structure of[Zn(H_(2)O)_(6)]^(2+)is capable of maintaining and completely inhibiting free water molecules.When[Zn(H_(2)O)_(6)]^(2+)is partially desolvated in the Helmholtz outer layer,the separated active molecules will be arrested by the“catcher”formed by the strong hydrogen bond N-H bond,ensuring the stable desolvation of Zn^(2+).The Zn||Zn symmetric battery can stably cycle for 2250 h at 1 mAh cm^(-2),Zn||V_(6)O_(13) full battery achieved a capacity retention rate of 99.2%after 10,000 cycles at 10 A g^(-1).This paper proposes a novel critical solvation strategy that paves the route for the construction of high-performance AZIBs.