The purpose of this study is two-fold： firstly, the development of a cheap, easy-to-construct and effective nanoparticle generator for testing nanoparticle sensors; secondly, the use of such a generator to test the e...The purpose of this study is two-fold： firstly, the development of a cheap, easy-to-construct and effective nanoparticle generator for testing nanoparticle sensors; secondly, the use of such a generator to test the effectiveness of a sensor device in trapping aerosolised nanoparticles. In this study, we have constructed an effective aerosol generator platform, based on aerosol-assisted chemical vapour deposition technology. Under well-controlled experimental conditions, this platform is capable of depositing aerosolised sodium chloride particles homogeneously on a substrate very effectively. Deposited aerosol droplets were subsequently dried and shown to form nanosized cubic crystals that are free from impurities. This platform was employed to test the effectiveness of a MEMS comb device in the electrostatic trapping of nanoparticles. Upon applying a DC bias （0.5 V） to the MEMS device, results showed an increase in nanoparticle deposition on the surface of the device, due to electrostatic precipitation. The presence of an electric field was shown to affect crystal formation upon drying of the aerosol droplets on the substrate; this caused a blotchy appearance on the SEM image, which was not observed in the absence of electric field.展开更多
The tapered element oscillating microbalance with filter dynamics measurement system （TEOM-FDMS） is an instrument commonly employed by the French air quality monitoring network. This instrument is currently calibrat...The tapered element oscillating microbalance with filter dynamics measurement system （TEOM-FDMS） is an instrument commonly employed by the French air quality monitoring network. This instrument is currently calibrated with calibration weights traceable to SI but having value and mass differences between each of them that are not representative of real atmospheric particle mass measurements. Moreover, these calibration weights do not allow detection of any technical problems associated with either the TEOM-FDMS sampling system upstream of the mass measurement or the intrinsic TEOM-FDMS filtration system. Therefore, a calibration method was developed using a portable reference aerosol generator （PRAG） that produces known and stable particle mass concentrations over time. Here, we present the characterization of the PRAG system in terms of a reference range of particle masses between 30 - 10 and 3456 ± 83 μg at three sampling times. Its coupling with the TEOM-FDMS and a global comparison between the defined reference range of particle masses and the measured masses obtained with each TEOM-FDMS implicated in this study are also presented.展开更多
文摘The purpose of this study is two-fold： firstly, the development of a cheap, easy-to-construct and effective nanoparticle generator for testing nanoparticle sensors; secondly, the use of such a generator to test the effectiveness of a sensor device in trapping aerosolised nanoparticles. In this study, we have constructed an effective aerosol generator platform, based on aerosol-assisted chemical vapour deposition technology. Under well-controlled experimental conditions, this platform is capable of depositing aerosolised sodium chloride particles homogeneously on a substrate very effectively. Deposited aerosol droplets were subsequently dried and shown to form nanosized cubic crystals that are free from impurities. This platform was employed to test the effectiveness of a MEMS comb device in the electrostatic trapping of nanoparticles. Upon applying a DC bias （0.5 V） to the MEMS device, results showed an increase in nanoparticle deposition on the surface of the device, due to electrostatic precipitation. The presence of an electric field was shown to affect crystal formation upon drying of the aerosol droplets on the substrate; this caused a blotchy appearance on the SEM image, which was not observed in the absence of electric field.
文摘The tapered element oscillating microbalance with filter dynamics measurement system （TEOM-FDMS） is an instrument commonly employed by the French air quality monitoring network. This instrument is currently calibrated with calibration weights traceable to SI but having value and mass differences between each of them that are not representative of real atmospheric particle mass measurements. Moreover, these calibration weights do not allow detection of any technical problems associated with either the TEOM-FDMS sampling system upstream of the mass measurement or the intrinsic TEOM-FDMS filtration system. Therefore, a calibration method was developed using a portable reference aerosol generator （PRAG） that produces known and stable particle mass concentrations over time. Here, we present the characterization of the PRAG system in terms of a reference range of particle masses between 30 - 10 and 3456 ± 83 μg at three sampling times. Its coupling with the TEOM-FDMS and a global comparison between the defined reference range of particle masses and the measured masses obtained with each TEOM-FDMS implicated in this study are also presented.
