In conversion of the integrated slant column amount of atmospheric ozone(O_3)measured by the ground-based spectrometer technique during twilight to the vertical quantity,the air-mass factor(AMF)is an important paramet...In conversion of the integrated slant column amount of atmospheric ozone(O_3)measured by the ground-based spectrometer technique during twilight to the vertical quantity,the air-mass factor(AMF)is an important parameter.In this work,calculations of AMF for ozone were performed for different atmospheres.It is shown that the O_3 AMF has seasonal variations with the minimum at the beginning of spring and the maximum in summer due to the seasonal change in the vertical distributions of O_3.A parameterization relation is obtained between O_3 AMF and optical thickness of stratospheric volcanic aerosols based on the Monte-Carlo radiative transfer simulations.展开更多
A method for aerosol extinction profile retrieval using ground-based multi-axis differential optical absorption spectroscopy(MAX-DOAS)is studied,which is based on a look-up table algorithm.The algorithm uses parametri...A method for aerosol extinction profile retrieval using ground-based multi-axis differential optical absorption spectroscopy(MAX-DOAS)is studied,which is based on a look-up table algorithm.The algorithm uses parametric method to represent aerosol extinction profiles and simulate different atmospheric aerosol states through atmospheric radiation transfer model.Based on the method,aerosol extinction profile was obtained during six cloud-free days.The O4 differential air mass factor(dAMF)measured by MAX-DOAS is compared with the corresponding model results under different atmospheric conditions(R^2=0.78).The aerosol optical thickness,aerosol weight factor in boundary layer,and the height of the boundary layer are obtained after the process of minimization and look-up table method.The retrieved aerosol extinction in boundary layer is compared with PM2.5 data measured by ground point instrument.The diurnal variation trends of the two methods are in good agreement.The correlation coefficients of the two methods are 0.71 when the aerosol optical thickness is smaller than 0.5.The results show that the look-up table method can obtain the aerosol state of the troposphere and provide validation for other instrument data.展开更多
文摘In conversion of the integrated slant column amount of atmospheric ozone(O_3)measured by the ground-based spectrometer technique during twilight to the vertical quantity,the air-mass factor(AMF)is an important parameter.In this work,calculations of AMF for ozone were performed for different atmospheres.It is shown that the O_3 AMF has seasonal variations with the minimum at the beginning of spring and the maximum in summer due to the seasonal change in the vertical distributions of O_3.A parameterization relation is obtained between O_3 AMF and optical thickness of stratospheric volcanic aerosols based on the Monte-Carlo radiative transfer simulations.
基金Project supported by the National Natural Science Foundation of China(Grant Nos.41875040,41705012,and 1605013)
文摘A method for aerosol extinction profile retrieval using ground-based multi-axis differential optical absorption spectroscopy(MAX-DOAS)is studied,which is based on a look-up table algorithm.The algorithm uses parametric method to represent aerosol extinction profiles and simulate different atmospheric aerosol states through atmospheric radiation transfer model.Based on the method,aerosol extinction profile was obtained during six cloud-free days.The O4 differential air mass factor(dAMF)measured by MAX-DOAS is compared with the corresponding model results under different atmospheric conditions(R^2=0.78).The aerosol optical thickness,aerosol weight factor in boundary layer,and the height of the boundary layer are obtained after the process of minimization and look-up table method.The retrieved aerosol extinction in boundary layer is compared with PM2.5 data measured by ground point instrument.The diurnal variation trends of the two methods are in good agreement.The correlation coefficients of the two methods are 0.71 when the aerosol optical thickness is smaller than 0.5.The results show that the look-up table method can obtain the aerosol state of the troposphere and provide validation for other instrument data.
