Anisotropic Magnon–Magnon Coupling in Synthetic Antiferromagnets

Magnon-magnon coupling in synthetic antiferromagnets advances it as hybrid magnonic systems to explore the quantum information technologies.To induce magnon-magnon coupling,the parity symmetry between two magnetization needs to be broken.Here we experimentally demonstrate a convenient method to break the parity symmetry by the asymmetric structure.We successfully introduce a magnon-magnon coupling in Ir-based synthetic antiferromagnets CoFeB(10 nm)/Ir(t_(Ir)=0.6 nm,1.2 nm)/CoFeB(13 nm).Remarkably,we find that the weakly uniaxial anisotropy field(-20 Oe)makes the magnon-magnon coupling anisotropic.The coupling strength presented by a characteristic anticrossing gap varies in the range between 0.54 GHz and 0.90 GHz for t_(Ir)=0.6 nm,and between 0.09 GHz and 1.4 GHz for t_(Ir)=1.2 nm.Our results demonstrate a feasible way to induce magnon-magnon coupling by an asymmetric structure and tune the coupling strength by varying the direction of in-plane magnetic field.The magnon-magnon coupling in this highly tunable material system could open exciting perspectives for exploring quantum-mechanical coupling phenomena.

Oscillation of coercivity between positive and negative in Mn_xGe_(1-x):H ferromagnetic semiconductor films

Amorphous MnxGe1-x：H ferromagnetic semiconductor films prepared in mixed Ar with 20% H2 by magnetron co- sputtering show global ferromagnetism with positive coercivity at low temperatures. With increasing temperature, the coercivity of MnxGe1-x：H films first changes from positive to negative, and then back to positive again, which was not found in the corresponding MnxGe1-x and other ferromagnetic semiconductors before. For Mn0.4Ge0.6：H film, the inverted Hall loop is also observed at 30 K, which is consistent with the negative coercivity. The negative coercivity is explained by the antiferromagnetic exchange coupling between the H-rich ferromagnetic regions separated by the H-poor non-ferromagnetic spacers. Hydrogenation is a useful method to tune the magnetic properties of MnxGe1-x films for the application in spintronics.

Two New Coordination Complexes Based on Eosin Y Dye Ligand：Syntheses,Crystal Structures and Magnetic Properties

Two novel coordination compounds formulated as [Co2（EY）2（L1）]·2C2H5OH（1） and [Mn2（EY）2（L1）]·2C2H5OH（2）（EY = Eosin Y dianion, L1 = 4,4＇-bipyridine） based on Eosin Y dye ligand have been prepared by solvothermal reactions and structurally characterized. Single-crystal X-ray diffraction studies reveal that compounds 1 and 2 are isostructural. They show weak antiferromagnetic coupling between the adjacent Co^Ⅱ and Mn^Ⅱ ions, respectively.

Performance of switch between exchange bias and coercivity:Influences of antiferromagnetic anisotropy and exchange coupling

The study on temperature dependence of exchange bias field and coercivity is crucial to solving the writing/reading dilemma in magnetic recording.Motivated by recent experimental findings,a complete switch between exchange bias field and coercivity with temperature is proposed,and the performance,characterized by average switching temperature(T_(S))and switching temperature width(T_(W)),controlled by antiferromagnetic anisotropy(KAF)and exchange coupling(J_(AF))constants is studied based on a MonteCarlo simulation.The results show that a linear relationship between T_(S)and KAFis established when KAFis above a critical value,while T_(S)is weakly influenced by J_(AF).On the contrary,T_(W)is insensitive to KAF,while strongly depends on J_(AF).Besides overcoming thermal energy,the increase of KAFfor a small J_(AF)guarantees the completely frozen states in the antiferromagnetic layers during magnetizing at higher temperature,below which the exchange bias field exists with a negligible coercivity.Otherwise,for a large J_(AF),the uncompensated antiferromagnetic magnetization behavior during the ferromagnetic magnetization reversal becomes complicated,and the switching process in the low temperature range depends on the irreversibility of uncompensated antiferromagnetic magnetization reversal during magnetizing,while in the high temperature range mainly influenced by the field-cooling process,resulting in a large T_(W).This work provides an opportunity to control/optimize the performance of the temperatureinduced switch between unidirectional and uniaxial symmetries through precisely tuning KAFand/or J_(AF)to meet different application demands in the next generation information technology.

MAGNETORESISTANCE EFFECT OBSERVED IN Fe/Mo MULTILAYERS PREPARED BY ELECTRON BEAM EVAPORATION

The Fe/Mo multilayers were prepared by electron beam evaporation, the micro structure and magnetic properties of the multilayers were studied by X-ray diffraction, vibrating-sample magnetometer (VSM) et al. The experimental results revealed that the Fe/Mo multilayers in our experimental conditions behaved magnetoresistance effect with a sharp peak on magnetoresistance (MR) ratio curve, and magnetoresistance is easily saturated at low applied magnetic fields. For [Fe(1.5nm)/Mo(1.0nm)]4,2 multilayers, MR ratio could arrive to 0.1%. The antiferromagnetic interlayer coupling could be observed in some films at room temperature. The strength of the antiferromagnetic interlayer coupling J in the films is low because of the low saturation field Hs. The relationship between magnetic properties and micro structure was also discussed in this paper.

Al-doping-induced magnetocapacitance in the multiferroic CuCrS_2

In this paper,magnetic and dielectric properties of the quasi-two-dimensional triangular-lattice system CuCrS2 and its B-site-diluted analogs CuAl1-xCrxS2（x = 0.01 and x = 0.02） are investigated.Antiferromagnetic phase transition is observed at about 38.5 K by magnetization measurement without shift induced by a small amount of doping Al.Magnetodielectric effect is found near TN in each of the three compounds.The dielectric constant decreases and the magnetocapacitance increases with the increase of substitution of nonmagnetic Al3＋ ions for the magnetic Cr^3＋ ions.The negative magnetocapacitive effect reaches ～ 13% for CuAl0.02Cr0.98S2.

Al-doping-induced magnetocapacitance in the multiferroic AgCrS_2

In this paper, multiferroics and magnetocapacitive effect of triangular-lattice antiferromagnet Ag Al0.02Cr0.98S2 are investigated by magnetic, ferroelectric, pyroelectric current and dielectric measurement. We find that it is a multiferroic material and the magnetocapacitive effect reaches a factor of up to 90 in an external field of 7 T. The results imply the further possibility of synthesizing the magnetocapacitive materials by modifying the frustrated spin structure in terms of a few B-site doping nonmagnetic ions.

Synthesis, Crystal Structure and Magnetic Properties of a New 3D Cobalt Vanadate

A new cobalt vanadate compound 1 [CoII(H2O)2V2VO6] has been hydrothermally synthesized and characterized by the elemental analyses and the single crystal X-ray diffraction analysis. Compound 1 crystallizes in the orthorhombic system, space group Pmna, with a=0.55646, b=1.06900, c=1.18452 nm, and Z=4. The magnetic susceptibility of the cobalt vanadate has been measured and indicates possible antiferromagnetic coupling between adjacent cobalt (II) (0.54320.5697 nm) through bond or space.