Self-assembly has been extensively studied in chemistry,physics,biology,and materials engineering and has become an important“bottom-up”approach in creating intriguing structures for different applications.Using dis...Self-assembly has been extensively studied in chemistry,physics,biology,and materials engineering and has become an important“bottom-up”approach in creating intriguing structures for different applications.Using dissipative self-assembly to construct fuel-dependent,energy-consuming,and dynamic nonequilibrium systems is important for developing intelligent life-like materials.Furthermore,dissipative self-assembly has become a research hotspot in materials chemistry,biomedical science,environmental chemistry,and physical chemistry.An in-depth understanding of the process and mechanism provides useful insights to the researchers for devel-oping materials using dissipative self-assembly and also helps guide future innovation in material fabrication.This critical review comprehensively analyzes various chemical fuel input and energy consumption mechanisms,supported by numerous illustrative examples.Versatile transient assemblies,including gels,vesicles,micelles,and nanoparticle aggregates,have been systematically studied in our and other laboratories.The relationship between the molecular structure of precursors and temporal assemblies in dissipative self-assemblies is discussed from the perspective of physical chemistry.Using dissipative self-assembly methods to construct functional assemblies provides important implications for constructing high-energy,nonequilibrium,and intelligent functional materials.展开更多
Subject Code:C05 With the support by the National Natural Science Foundation of China,the research team led by Dr.Li Qing(李晴)at the State Key Laboratory of Protein and Plant Gene Research,School of Life Sciences and...Subject Code:C05 With the support by the National Natural Science Foundation of China,the research team led by Dr.Li Qing(李晴)at the State Key Laboratory of Protein and Plant Gene Research,School of Life Sciences and Peking-Tsinghua Center for Life Sciences,Peking University,Beijing,recently reported that展开更多
基金the National Natural Science Foundation of China(Grant Nos.22032003 and 22072073).
文摘Self-assembly has been extensively studied in chemistry,physics,biology,and materials engineering and has become an important“bottom-up”approach in creating intriguing structures for different applications.Using dissipative self-assembly to construct fuel-dependent,energy-consuming,and dynamic nonequilibrium systems is important for developing intelligent life-like materials.Furthermore,dissipative self-assembly has become a research hotspot in materials chemistry,biomedical science,environmental chemistry,and physical chemistry.An in-depth understanding of the process and mechanism provides useful insights to the researchers for devel-oping materials using dissipative self-assembly and also helps guide future innovation in material fabrication.This critical review comprehensively analyzes various chemical fuel input and energy consumption mechanisms,supported by numerous illustrative examples.Versatile transient assemblies,including gels,vesicles,micelles,and nanoparticle aggregates,have been systematically studied in our and other laboratories.The relationship between the molecular structure of precursors and temporal assemblies in dissipative self-assemblies is discussed from the perspective of physical chemistry.Using dissipative self-assembly methods to construct functional assemblies provides important implications for constructing high-energy,nonequilibrium,and intelligent functional materials.
文摘Subject Code:C05 With the support by the National Natural Science Foundation of China,the research team led by Dr.Li Qing(李晴)at the State Key Laboratory of Protein and Plant Gene Research,School of Life Sciences and Peking-Tsinghua Center for Life Sciences,Peking University,Beijing,recently reported that
