Urban wastewater treatment techniques could not be applied to improve the pollutant removal efficiency,due to its characteristics of closed and quiescent conditions of the static lake water.In this study,natural zeoli...Urban wastewater treatment techniques could not be applied to improve the pollutant removal efficiency,due to its characteristics of closed and quiescent conditions of the static lake water.In this study,natural zeolite and coal cinder were chosen as filler compounds of the ecological filter.Static and dynamic experiments were carried out to study the remediation efficiency.Experimental data show that removal efficiency of ammonia nitrogen （NH ＋ 4 -N） reaches 85% in both static and dynamic patterns and its removal efficiency reaches 97% when the recycling period is 1 h in dynamic condition.The maximum removal efficiency of nitrite nitrogen （NO-2 -N） reached 98%,and the removal efficiency of total nitrogen （TN） is a maximum of 84%.The final effluent concentration of total phosphorus （TP） is 0.079 mg/L.Effluent recycling could improve the nutrient （N,P） removal efficiently.Dissolved oxygen （DO） concentration could remain high with the water cycling.The filter works efficiently on regulating pH to the standard level of healthy water.展开更多
Silicene, the silicon counterpart of graphene, has been successfully grown on metallic substrates such as Ag（111）, ZrB2（0001）, and Ir（111） surfaces. However, characterization of its electronic structure is hampe...Silicene, the silicon counterpart of graphene, has been successfully grown on metallic substrates such as Ag（111）, ZrB2（0001）, and Ir（111） surfaces. However, characterization of its electronic structure is hampered by the metallic substrate. In addition, potential applications of silicene in nanoelectronic devices will require its growth on or integration with semiconducting and insulating substrates. We herein present a review of recent theoretical works regarding the interaction of silicene with non-metallic templates, distinguishing between the weak van-der-Waals-like interactions of silicene with, for example, layered metal （di）chalcogenides, and the stronger covalent bonding between silicene and, for example, ZnS surfaces. We then present a methodology to effectively compare the stability of diverse silicene structures using thermodynamics and molecular dynamics density functional theory calculations. Recent experimental results on the growth of silicene on MoS2 are also reported and compared to the theoretical predictions.展开更多
基金supported by the National Natural Science Foundation of China (Grant Nos.50809037,40830744)the Shanghai Leading Academic Discipline Project (Grant No.S30109)the Systems Biology Research Foundation of Shanghai University
文摘Urban wastewater treatment techniques could not be applied to improve the pollutant removal efficiency,due to its characteristics of closed and quiescent conditions of the static lake water.In this study,natural zeolite and coal cinder were chosen as filler compounds of the ecological filter.Static and dynamic experiments were carried out to study the remediation efficiency.Experimental data show that removal efficiency of ammonia nitrogen （NH ＋ 4 -N） reaches 85% in both static and dynamic patterns and its removal efficiency reaches 97% when the recycling period is 1 h in dynamic condition.The maximum removal efficiency of nitrite nitrogen （NO-2 -N） reached 98%,and the removal efficiency of total nitrogen （TN） is a maximum of 84%.The final effluent concentration of total phosphorus （TP） is 0.079 mg/L.Effluent recycling could improve the nutrient （N,P） removal efficiently.Dissolved oxygen （DO） concentration could remain high with the water cycling.The filter works efficiently on regulating pH to the standard level of healthy water.
文摘Silicene, the silicon counterpart of graphene, has been successfully grown on metallic substrates such as Ag（111）, ZrB2（0001）, and Ir（111） surfaces. However, characterization of its electronic structure is hampered by the metallic substrate. In addition, potential applications of silicene in nanoelectronic devices will require its growth on or integration with semiconducting and insulating substrates. We herein present a review of recent theoretical works regarding the interaction of silicene with non-metallic templates, distinguishing between the weak van-der-Waals-like interactions of silicene with, for example, layered metal （di）chalcogenides, and the stronger covalent bonding between silicene and, for example, ZnS surfaces. We then present a methodology to effectively compare the stability of diverse silicene structures using thermodynamics and molecular dynamics density functional theory calculations. Recent experimental results on the growth of silicene on MoS2 are also reported and compared to the theoretical predictions.
