Spin-dependent negative differential conductance in transport through single-molecule magnets

Transport properties are theoretically studied through an anisotropy single-molecule magnet symmetrically connected to two identical ferromagnetic leads. It is found that even though in parallel configuration of leads’ magnetizations, the total current still greatly depends on the spin polarization of leads at certain particular bias region, and thus for large polarization a prominent negative differential conductance （NDC） emerges. This originates from the joint effect of single-direction transitions and spin polarization, which removes the symmetry between spin-up and spin-down transitions. The present mechanism of NDC is remarkably different from the previously reported mechanisms. To clarify the physics of the NDC, we further monitored the shot noise spectroscopy and found that the appearance of the NDC is accompanied by the rapid decrease of Fano factor.

Low-bias negative differential conductance controlled by electrode separation

The electronic transport properties of a single thiolated arylethynylene molecule with 9,10-dihydroanthracene core, denoted as TADHA, is studied by using non-equilibrium Green＇s function formalism combined with ab initio calculations. The numerical results show that the TADHA molecule exhibits excellent negative differential conductance （NDC） behavior at lower bias regime as probed experimentally. The NDC behavior of TADHA molecule originates from the Stark effect of the applied bias voltage, by which the highest occupied molecular orbital （HOMO） and the HOMO-1 are pulled apart and become localized. The NDC behavior of TADHA molecular system is tunable by changing the electrode distance. Shortening the electrode separation can enhance the NDC effect which is attributed to the possible increase of coupling between the two branches of TADHA molecule.

Ferromagnetic barrier-induced negative differential conductance on the surface of a topological insulator

The effect of the negative differential conductance of a ferromagnetic barrier on the surface of a topological insulat（ is theoretically investigated. Due to the changes of the shape and position of the Fermi surfaces in the ferromagnetic barrie the transport processes can be divided into three kinds： the total, partial, and blockade transmission mechanisms. The bias voltage can give rise to the transition of the transport processes from partial to blockade transmission mechanisms, which results in a considerable effect of negative differential conductance. With appropriate structural parameters, the currenl voltage characteristics show that the minimum value of the current can reach to zero in a wide range of the bias voltag and then a large peak-to-valley current ratio can be obtained.

Ac response of a coupled double quantum dot

The effect of phase-breaking process on the ac response of a coupled double quantum dot is studied in this paper based on the nonequilibrium Green function formalism. A general expression is derived for the ac current in the presence of electron-phonon interaction. The ac conductance is numerically computed and the results are compared with those in [Anatram M P and Datta S 1995 Phys. Rev. B 51 7632]. Our results reveal that the inter-dot electron tunnelling interplays with that between dots and electron reservoirs, and contributes prominently to the ac current when inter-dot tunnelling coupling is much larger than the tunnelling coupling between dots and electron reservoirs. In addition, the phase-breaking process is found to have a significant effect on the ac transport through the coupled double dot.

Influence of electron–phonon interaction on the properties of transport through double quantum dot with ferromagnetic leads

Electronic transport through a vibrating double quantum dot （DQD） in contact with noncollinear ferromagnetic （FM） leads is investigated. The state transition between the two dots of the DQD is excited by an AC microwave driving field. The corresponding currents and differential conductance are calculated in the Coulomb blockade regime by means of the Born-Markov master equation. It is shown that the interplay between electrons and phonons gives rise to phonon-assisted tunneling resonances and Franck-Condon blockade under certain conditions. In noncollinear magnetic configurations, spin-blockade effects are also observed, and the angle of polarization has some influence on the transport characteristics.

Gas-sensor property of single-molecule device:F_2 adsorbing effect

The single thiolated arylethynylene molecule with 9,10-dihydroanthracene core（denoted as TADHA） possesses pronounced negative differential conductance（NDC） behavior at lower bias regime. The adsorption effects of F2 molecule on the current and NDC behavior of TADHA molecular junctions are studied by applying non-equilibrium Green＇s formalism combined with density functional theory. The numerical results show that the F2 molecule adsorbed on the benzene ring of TADHA molecule near the electrode can dramatically suppresses the current of TADHA molecular junction. When the F2 molecule adsorbed on the conjugated segment of 9,10-dihydroanthracene core of TADHA molecule, an obviously asymmetric effect on the current curves induces the molecular system showing apparent rectifier behavior. However, the current especially the NDC behavior have been significantly enlarged when F2 addition reacted with triple bond of TADHA molecule.

Research on the Relationship between Density of States and Conducting Properties of Single-walled Carbon Nanotubes

The analytical expression of the electronic density of states (DOS) for single-walled carbon nanotubes (SWNTs) has been derived on the basis of graphene approximation of the energy E(k) near the Fermi level EF. The distinctive properties of the DOS, the normalized differential conductivity and the current us bias for SWNTs are deduced and analyzed theoretically. The singularities in the DOS (or in the normalized differential conductivity) predict that the jump structure of current (or conductance)-bias of SWNTs exists. All conclusions from the theoretical analysis are in well agreement with the experimental results of SWNT's electronic structure and electronic transport. In other words, the simple theoretical model in this paper can be applied to understand a range of spectroscopic and other measurement data related to the DOS of SWNTs.

Dynamics and Its Control in Modulation-Doped Heterostructures

A simulation model and the dynamics of the forced modulation doped heterostructure, which operates in the state far from thermodynamic equilibrium, are discussed. The numerical simulations clearly reveal that the system under an appropriate bias including DC and AC voltages exhibits expected complex dynamical behaviors. The amplitude and frequency of the externally applied microwave field are taken as the control parameters in the system. Because many nonlinear dynamical systems may have more than one possible time asympotic final state depending on the different initial conditions, the basins of attractions of both ordinary attractor and chaotic attractor are also studied respecively. Finally, as a possible application a method based on pulse driving to control chaos in semiconductor is proposed.

Different Geometries of Superheterodyne Amplification of Electromagnetic Beams in Waveguides Nitride-Dielectric

The superheterodyne amplification of electromagnetic waves is investigated when the resonant three-wave interaction of two electromagnetic waves with the space charge wave occurs in the waveguides nitride n-GaN, n-InN films-dielectric. The amplification of SCW waves due to the negative differential conductivity is investigated in nitride n-GaN, n-InN films at the frequencies f ≤ 400 GHz in the lower part of the terahertz (THz) range. The electromagnetic waves are either in the upper part of THz range or in the optical range. The superheterodyne amplification is considered in two geometries, the collinear one in which the three interacting waves travel in the same direction and the anti-collinear geometry where the second electromagnetic wave propagates in the opposite direction. The preferences and drawbacks of each geometry are pointed out. The finite width of space charge waves leads to decrease of increments of amplification.

Dry-regulated hydrogels with anisotropic mechanical performance and ionic conductivity

Nature consists of various soft tissues with well-ordered hierarchical anisotropic structures, which play essential roles in biological systems to exhibit particular functions. Mimicking bio-tissues, synthetic hydrogels with anisotropic structures have received considerable attention in recent years. However, existing approaches to fabricate anisotropic hydrogels often require complicated procedures, which are timeconsuming and labor-demanding. Inspired by the dry-induced crystallization phenomenon, we report a simple yet effective prestretching-drying-swelling method to afford anisotropic crystalline polyvinyl alcohol hydrogels. Owing to the distinct anisotropic microstructure, the hydrogels demonstrate excellent mechanical properties with noticeable directional distinction. It is revealed that both the enhancing of pre-orientation strain and the extending of heating time make the hydrogels with better mechanical properties and more remarkable anisotropicity. Owing to the anisotropically aligned structure, the hydrogels exhibit remarkably differential ionic conductivity: the difference between the parallel and vertical conductivity of the same sample can reach as high as 6.6 times, making the materials possible candidates as nano-conductive materials. We anticipate that this simple yet effective approach may become highly useful for fabricating oriented hydrogels and endow the materials with more promising application prospects in the future.

Complex dynamical behaviors in modulation-doped GaAs/Al_xGa_(1-x)As heterostructures

We study dynamics of the forced modulation-doped GaAs/AIGaAs heterostructure de-vices . The coupled differential equations governing the dynamical behaviors are numerically simulated. Biased with an appropriate dc field, the system exhibits two states: spontaneous current oscillation and fixed points. By imposing an ac driving force, the dynamical system shows frequency locking, quasiperiodicity, and chaos, which are sensitive to the amplitude and frequency of the externally ap-plied periodical microwave field. The basins of attraction of both ordinary attractors and strange attrac-tors are presented.