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Development of a distributed and integratable manufacturing execution system framework 被引量:4
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作者 杨浩 周娜 +1 位作者 朱剑英 罗翔 《Journal of Southeast University(English Edition)》 EI CAS 2003年第1期64-69,共6页
Using remote method invocation (RMI) and a distributed object-oriented technique, this paper presents a systematic approach to developing a manufacturing execution system (MES) framework, which is open, modularized, d... Using remote method invocation (RMI) and a distributed object-oriented technique, this paper presents a systematic approach to developing a manufacturing execution system (MES) framework, which is open, modularized, distributed, configurable, interoperable and maintainable. Moreover, the design patterns for the framework .are developed and a variety of functional components are designed by inheriting appropriate patterns. And then an application is constructed by invoking corresponding methods of related components. An MES system implementing the framework and design patterns can be facilely integrated with other manufacturing applications, such as enterprise resource planning (ERP) and floor control system (FCS) . 展开更多
关键词 manufacturing execution system framework design pattern distributed object-oriented remote method invocation
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Framework of Distributed Coupled Atmosphere-Ocean-Wave Modeling System 被引量:3
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作者 文元桥 黄立文 +3 位作者 邓健 张进峰 王思思 王立军 《Advances in Atmospheric Sciences》 SCIE CAS CSCD 2006年第3期442-448,共7页
In order to research the interactions between the atmosphere and ocean as well as their important role in the intensive weather systems of coastal areas, and to improve the forecasting ability of the hazardous weather... In order to research the interactions between the atmosphere and ocean as well as their important role in the intensive weather systems of coastal areas, and to improve the forecasting ability of the hazardous weather processes of coastal areas, a coupled atmosphere-ocean-wave modeling system has been developed. The agent-based environment framework for linking models allows flexible and dynamic information exchange between models. For the purpose of flexibility, portability and scalability, the framework of the whole system takes a multi-layer architecture that includes a user interface layer, computational layer and service-enabling layer. The numerical experiment presented in this paper demonstrates the performance of the distributed coupled modeling system. 展开更多
关键词 system framework mesoscale models distributed coupled modeling
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Distributed adaptive direct position determination based on diffusion framework 被引量:2
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作者 Wei Xia Wei Liu Lingfeng Zhu 《Journal of Systems Engineering and Electronics》 SCIE EI CSCD 2016年第1期28-38,共11页
The conventional direct position determination(DPD) algorithm processes all received signals on a single sensor.When sensors have limited computational capabilities or energy storage,it is desirable to distribute th... The conventional direct position determination(DPD) algorithm processes all received signals on a single sensor.When sensors have limited computational capabilities or energy storage,it is desirable to distribute the computation among other sensors.A distributed adaptive DPD(DADPD)algorithm based on diffusion framework is proposed for emitter localization.Unlike the corresponding centralized adaptive DPD(CADPD) algorithm,all but one sensor in the proposed algorithm participate in processing the received signals and estimating the common emitter position,respectively.The computational load and energy consumption on a single sensor in the CADPD algorithm is distributed among other computing sensors in a balanced manner.Exactly the same iterative localization algorithm is carried out in each computing sensor,respectively,and the algorithm in each computing sensor exhibits quite similar convergence behavior.The difference of the localization and tracking performance between the proposed distributed algorithm and the corresponding CADPD algorithm is negligible through simulation evaluations. 展开更多
关键词 emitter localization time difference of arrival(TDOA) direct position determination(DPD) distributed adaptive DPD(DADPD) diffusion framework.
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A Fully Distributed Hybrid Control Framework For Non-Differentiable Multi-Agent Optimization
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作者 Xia Jiang Xianlin Zeng +2 位作者 Jian Sun Jie Chen Yue Wei 《IEEE/CAA Journal of Automatica Sinica》 SCIE EI CSCD 2022年第10期1792-1800,共9页
This paper develops a fully distributed hybrid control framework for distributed constrained optimization problems.The individual cost functions are non-differentiable and convex.Based on hybrid dynamical systems,we p... This paper develops a fully distributed hybrid control framework for distributed constrained optimization problems.The individual cost functions are non-differentiable and convex.Based on hybrid dynamical systems,we present a distributed state-dependent hybrid design to improve the transient performance of distributed primal-dual first-order optimization methods.The proposed framework consists of a distributed constrained continuous-time mapping in the form of a differential inclusion and a distributed discrete-time mapping triggered by the satisfaction of local jump set.With the semistability theory of hybrid dynamical systems,the paper proves that the hybrid control algorithm converges to one optimal solution instead of oscillating among different solutions.Numerical simulations illustrate better transient performance of the proposed hybrid algorithm compared with the results of the existing continuous-time algorithms. 展开更多
关键词 distributed algorithm hybrid framework multiagent network non-differentiable optimization
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Formalized Description of Distributed Denial of Service Attack 被引量:1
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作者 杜彦辉 马锐 刘玉树 《Journal of Beijing Institute of Technology》 EI CAS 2004年第4期360-364,共5页
The distributed denial of service (DDoS) attack is one of the dangers in intrusion modes. It's difficult to defense and can cause serious damage to the system. Based on a careful study of the attack principles and... The distributed denial of service (DDoS) attack is one of the dangers in intrusion modes. It's difficult to defense and can cause serious damage to the system. Based on a careful study of the attack principles and characteristics, an object-oriented formalized description is presented, which contains a three-level framework and offers full specifications of all kinds of DDoS modes and their features and the relations between one another. Its greatest merit lies in that it contributes to analyzing, checking and judging DDoS. Now this formalized description has been used in a special IDS and it works very effectively.( 展开更多
关键词 distributed) denial of service(DDoS) attack formalized description framework knowledge (expression)
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Power loss reduction of distribution systems using BFO based optimal reconfiguration along with DG and shunt capacitor placement simultaneously in fuzzy framework 被引量:1
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作者 M.Mohammadi A.Mohammadi Rozbahani S.Bahmanyar 《Journal of Central South University》 SCIE EI CAS CSCD 2017年第1期90-103,共14页
In distribution systems,network reconfiguration and capacitor placement are commonly used to diminish power losses and keep voltage profiles within acceptable limits.Moreover,the problem of DG allocation and sizing is... In distribution systems,network reconfiguration and capacitor placement are commonly used to diminish power losses and keep voltage profiles within acceptable limits.Moreover,the problem of DG allocation and sizing is great important.In this work,a combination of a fuzzy multi-objective approach and bacterial foraging optimization(BFO) as a meta-heuristic algorithm is used to solve the simultaneous reconfiguration and optimal sizing of DGs and shunt capacitors in a distribution system.Each objective is transferred into fuzzy domain using its membership function.Then,the overall fuzzy satisfaction function is formed and considered a fitness function inasmuch as the value of this function has to be maximized to gain the optimal solution.The numerical results show that the presented algorithm improves the performance much more than other meta-heuristic algorithms.Simulation results found that simultaneous reconfiguration with DG and shunt capacitors allocation(case 5) has 77.41%,42.15%,and 56.14%improvements in power loss reduction,load balancing,and voltage profile indices,respectively in 33-bus test system.This result found 87.27%,35.82%,and 54.34%improvements of mentioned indices respectively for 69-bus system. 展开更多
关键词 network reconfiguration distributed generation (DG) capacitor banks fuzzy framework bacterial foragingoptimization
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A Novel Approach to Design Distribution Preserving Framework for Big Data 被引量:1
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作者 Mini Prince P.M.Joe Prathap 《Intelligent Automation & Soft Computing》 SCIE 2023年第3期2789-2803,共15页
In several fields like financial dealing,industry,business,medicine,et cetera,Big Data(BD)has been utilized extensively,which is nothing but a collection of a huge amount of data.However,it is highly complicated alon... In several fields like financial dealing,industry,business,medicine,et cetera,Big Data(BD)has been utilized extensively,which is nothing but a collection of a huge amount of data.However,it is highly complicated along with time-consuming to process a massive amount of data.Thus,to design the Distribution Preserving Framework for BD,a novel methodology has been proposed utilizing Manhattan Distance(MD)-centered Partition Around Medoid(MD–PAM)along with Conjugate Gradient Artificial Neural Network(CG-ANN),which undergoes various steps to reduce the complications of BD.Firstly,the data are processed in the pre-processing phase by mitigating the data repetition utilizing the map-reduce function;subsequently,the missing data are handled by substituting or by ignoring the missed values.After that,the data are transmuted into a normalized form.Next,to enhance the classification performance,the data’s dimensionalities are minimized by employing Gaussian Kernel(GK)-Fisher Discriminant Analysis(GK-FDA).Afterwards,the processed data is submitted to the partitioning phase after transmuting it into a structured format.In the partition phase,by utilizing the MD-PAM,the data are partitioned along with grouped into a cluster.Lastly,by employing CG-ANN,the data are classified in the classification phase so that the needed data can be effortlessly retrieved by the user.To analogize the outcomes of the CG-ANN with the prevailing methodologies,the NSL-KDD openly accessible datasets are utilized.The experiential outcomes displayed that an efficient result along with a reduced computation cost was shown by the proposed CG-ANN.The proposed work outperforms well in terms of accuracy,sensitivity and specificity than the existing systems. 展开更多
关键词 Big data artificial neural network fisher discriminant analysis distribution preserving framework manhattan distance
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A Tutorial on Federated Learning from Theory to Practice:Foundations,Software Frameworks,Exemplary Use Cases,and Selected Trends
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作者 M.Victoria Luzón Nuria Rodríguez-Barroso +5 位作者 Alberto Argente-Garrido Daniel Jiménez-López Jose M.Moyano Javier Del Ser Weiping Ding Francisco Herrera 《IEEE/CAA Journal of Automatica Sinica》 SCIE EI CSCD 2024年第4期824-850,共27页
When data privacy is imposed as a necessity,Federated learning(FL)emerges as a relevant artificial intelligence field for developing machine learning(ML)models in a distributed and decentralized environment.FL allows ... When data privacy is imposed as a necessity,Federated learning(FL)emerges as a relevant artificial intelligence field for developing machine learning(ML)models in a distributed and decentralized environment.FL allows ML models to be trained on local devices without any need for centralized data transfer,thereby reducing both the exposure of sensitive data and the possibility of data interception by malicious third parties.This paradigm has gained momentum in the last few years,spurred by the plethora of real-world applications that have leveraged its ability to improve the efficiency of distributed learning and to accommodate numerous participants with their data sources.By virtue of FL,models can be learned from all such distributed data sources while preserving data privacy.The aim of this paper is to provide a practical tutorial on FL,including a short methodology and a systematic analysis of existing software frameworks.Furthermore,our tutorial provides exemplary cases of study from three complementary perspectives:i)Foundations of FL,describing the main components of FL,from key elements to FL categories;ii)Implementation guidelines and exemplary cases of study,by systematically examining the functionalities provided by existing software frameworks for FL deployment,devising a methodology to design a FL scenario,and providing exemplary cases of study with source code for different ML approaches;and iii)Trends,shortly reviewing a non-exhaustive list of research directions that are under active investigation in the current FL landscape.The ultimate purpose of this work is to establish itself as a referential work for researchers,developers,and data scientists willing to explore the capabilities of FL in practical applications. 展开更多
关键词 Data privacy distributed machine learning federated learning software frameworks
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Analytical Framework for Market-oriented DSR Flexibility Integration and Management 被引量:1
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作者 Shi You Junjie Hu +1 位作者 Kai Heussen Chunyu Zhang 《Energy and Power Engineering》 2013年第4期1367-1371,共5页
Integration and management of the flexibility of Demand Side Resources (DSR) in today’s energy systems plays a significant role in building up a sustainable society. However, the challenges of understanding, predicat... Integration and management of the flexibility of Demand Side Resources (DSR) in today’s energy systems plays a significant role in building up a sustainable society. However, the challenges of understanding, predicating and handling the uncertainties associated this subject to a great extent hamper its development. In this paper, an analytical framework based on a multi-portfolio setup in presence of a deregulated power market is proposed to address such challenges by adopting the thinking in modern portfolio theory (MPT). A Numerical example that targets on analyzing the risk and return for various flexibility pricing strategies are presented to illustrate some features of the framework. 展开更多
关键词 ANALYTICAL framework distributed Energy Resources Flexiblity Deregulated Power Market Morden PORTFOLIO Theory Risk and RETURN
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Synthesis,gas adsorption and reliable pore size estimation of zeolitic imidazolate framework-7 using CO_2 and water adsorption 被引量:3
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作者 Mahdi Niknam Shahrak Morteza Niknam Shahrak +3 位作者 Akbar Shahsavand Nasser Khazeni Xiaofei Wu Shuguang Deng 《Chinese Journal of Chemical Engineering》 SCIE EI CAS CSCD 2017年第5期595-601,共7页
Reliable estimation of the pore size distribution(PSD) in porous materials such as metal–organic frameworks(MOFs) and zeolitic imidazolate frameworks(ZIFs) is crucial for accurately assessing adsorption capacity and ... Reliable estimation of the pore size distribution(PSD) in porous materials such as metal–organic frameworks(MOFs) and zeolitic imidazolate frameworks(ZIFs) is crucial for accurately assessing adsorption capacity and corresponding selectivity. In this study, the so-called zeolitic imidazolate framework-7(ZIF-7) is successfully synthesized via relatively fast and convenient microwave technique. The morphology and structure of the obtained MOF were characterized by XRD, SEM and N_2 and CO_2adsorption/desorption isotherms at 77 K and0 °C respectively. Then, to determine the PSD of the fabricated MOF, carbon dioxide isotherms are experimentally measured at various temperatures up to atmospheric pressure. Afterward, the experimental CO_2 isotherms data are utilized in two recently proposed in-house algorithms of SHN1 and SHN2 to extract the true PSD of manufactured ZIF-7. The obtained results revealed that median pore diameter of the fabricated ZIF-7 is estimated around 0.404 nm and 0.370 nm by using CO_2 isotherms at 273 K and 298 K respectively. These values are in good agreement with the real pore diameter of 0.42 nm. Moreover, experimental data of water adsorption isotherms over four different MOFs, borrowed from literature, are employed to illustrate further effectiveness of the above algorithms on successful determination of the corresponding pore size distributions. All predicted PSDs are proved to be in good agreement with those obtained from independent methods such as topology and morphology studies. 展开更多
关键词 ZIF-7 Metal–organic framework Size distribution Adsorption CO2 capture Gas
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Using the KISO's Framework to Integrate Knowledge Sources
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作者 王念滨 Xu +4 位作者 Xiaofei Sun Yuhan Deng Shengchun 《High Technology Letters》 EI CAS 2001年第1期74-78,共5页
In complicated application environment such as CIMS (Computer Integrated Manufacture System) enterprise, it will bring great benefits to integrate distributed knowledge sources. But the difficulties of knowledge shari... In complicated application environment such as CIMS (Computer Integrated Manufacture System) enterprise, it will bring great benefits to integrate distributed knowledge sources. But the difficulties of knowledge sharing and reuse seriously encumbrance the implementation of knowledge integration. In this paper, we describe how a framework of knowledge-integrated system based on ontology (KISO) can be used to support integrating distributed knowledge sources. 展开更多
关键词 ONTOLOGY distributed knowledge sources Knowledge integrated framework
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Microsoft.Net Framework及COM+技术系统开发架构及实现
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作者 陆子旭 《计算机光盘软件与应用》 2011年第16期178-179,共2页
本文针对微软公司(Microsoft Corporation)的,NetFramework技术及COM+~件技术在实际的信息管理系统开发及应用架构中的方式和实现方法进行详细论述。以Microsoft.Net Framework技术为基础实现的信息管理系统应用架构中主要包含:Mi... 本文针对微软公司(Microsoft Corporation)的,NetFramework技术及COM+~件技术在实际的信息管理系统开发及应用架构中的方式和实现方法进行详细论述。以Microsoft.Net Framework技术为基础实现的信息管理系统应用架构中主要包含:MicrosoftCOM+组件技术、Microsoft Distributed Transaction Coordinator(分布式事务协调)技术,Microsoft Remoting Service技术,webService技术等。 展开更多
关键词 COM+组件 Net framework REMOTING Service MSDTC 分布式应用 管理系统
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县域休闲农业体验产品规划技术及实证——以全国休闲农业重点县临安区为例
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作者 蔡碧凡 周嘉韵 《天津农业科学》 CAS 2024年第4期39-48,共10页
休闲农业是推进乡村产业振兴和农文旅融合的重要产业和关键业态。县域是政策制度设计与空间落地实施的重要行政单元,更是消费者休闲农业体验的重要目的地。因此,从县域尺度开展休闲农业体验产品规划是促进休闲农业转型升级的关键路径。... 休闲农业是推进乡村产业振兴和农文旅融合的重要产业和关键业态。县域是政策制度设计与空间落地实施的重要行政单元,更是消费者休闲农业体验的重要目的地。因此,从县域尺度开展休闲农业体验产品规划是促进休闲农业转型升级的关键路径。本研究引入昂谱(RMP)理论和体验经济理论,基于改进的E-RMP分析框架,构建了县域休闲农业体验产品规划技术流程,并以全国休闲农业重点县浙江省杭州市临安区为例,在资源转化评价、市场体验评价、产品创新外部环境分析的基础上,对全区休闲农业体验产品空间布局、产品谱系和游线组织等方面提出规划策略。空间布局上,全区构建了一条杭黄世界级山地特色农业景观廊道和东部都市休闲农业、中部耕织体验农业、西部山地特色农业三个组团“1+3”格局,并规划出不同主题、不同季节的休闲农业体验产品谱系和游览线路。E-RMP分析框架为县域尺度开展休闲农业体验产品规划提供技术遵循,为合理开展空间布局、产品谱系和游览线路设计提供技术支撑。本研究为未来几年地方开展县域休闲农业规划和争创全国休闲农业重点县提供经验借鉴和决策依据。 展开更多
关键词 休闲农业 E-RMP分析框架 乡村振兴 空间布局 体验产品
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长江经济带农业经济韧性的时空分布及组态影响因素——基于TOE框架的fs-QCA分析
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作者 张俊 尤赟 冯越珺 《青海师范大学学报(社会科学版)》 2024年第2期79-91,共13页
新发展格局下,增强农业经济韧性是助力农业强国建设的时代需求。从3个维度构建农业经济韧性评价体系,运用熵值法测算2012—2021长江经济带农业经济韧性。借助H-P滤波分析法、标准差椭圆模型、局域热点分析描绘农业经济韧性的时空演化格... 新发展格局下,增强农业经济韧性是助力农业强国建设的时代需求。从3个维度构建农业经济韧性评价体系,运用熵值法测算2012—2021长江经济带农业经济韧性。借助H-P滤波分析法、标准差椭圆模型、局域热点分析描绘农业经济韧性的时空演化格局。基于组态视角,采用fsQCA并依托TOE理论框架,厘清长江经济带农业经济韧性的多元提升路径。结果发现:长江经济带农业经济韧性共经历2轮周期波动,周期波动态势有所强化。长江经济带农业经济韧性重心向东南方向移动,发展日益均衡化。热点区和次热点区空间集聚范围主要分布于长三角地区。组态视角下,存在4种组态路径实现农业经济韧性的提升,分别是融智拉动型、要素提质型、技术主导产业结构支持型和全面优化型。 展开更多
关键词 农业经济韧性 时空分布 TOE框架 fsQCA 组态视角
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考虑天气特征与多变量相关性的配电网短期负荷预测 被引量:1
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作者 于越 葛磊蛟 +2 位作者 金朝阳 王玥 丁磊 《电力系统保护与控制》 EI CSCD 北大核心 2024年第6期131-141,共11页
针对配电网短期负荷预测受到众多复杂天气特征等随机不确定性因素影响,以及传统预测模型难以有效分析不同特征序列之间的相关性等问题,提出一种考虑天气特征与多变量相关性的配电网短期负荷预测方法。首先,提出多变量快速最大信息系数(m... 针对配电网短期负荷预测受到众多复杂天气特征等随机不确定性因素影响,以及传统预测模型难以有效分析不同特征序列之间的相关性等问题,提出一种考虑天气特征与多变量相关性的配电网短期负荷预测方法。首先,提出多变量快速最大信息系数(multi-variable rapid maximal information coefficient,MVRapidMIC)提取相关性高的天气特征序列。其次,引入探索性因子分析法(exploratory factor analysis,EFA),对高相关性特征序列进行降维处理。最后,将维度分段(dimension-segment-wise,DSW)机制和两阶段注意力(two-stage attention,TSA)机制与Informer模型结合,提高预测模型对不同特征序列相关性的分析能力。通过DTU 7K 47节点实际配电网的历史负荷数据开展仿真测试,验证所提方法的预测精度、鲁棒性和时效性。 展开更多
关键词 配电网 短期负荷预测 天气特征 最大信息系数 Informer框架
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基于流计算和大数据平台的实时交通流预测 被引量:1
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作者 李星辉 曾碧 魏鹏飞 《计算机工程与设计》 北大核心 2024年第2期553-561,共9页
目前交通流预测实时性差,很难满足在线分析和预测任务的需求,基于此提出一种Flink流计算框架和大数据平台结合的实时交通流预测方法。基于流计算框架实时捕捉和预处理数据,包括采用Flink的transform算子对数据进行校验和处理,将处理后... 目前交通流预测实时性差,很难满足在线分析和预测任务的需求,基于此提出一种Flink流计算框架和大数据平台结合的实时交通流预测方法。基于流计算框架实时捕捉和预处理数据,包括采用Flink的transform算子对数据进行校验和处理,将处理后的数据sink到大数据的HDFS文件系统,交由下一步的大数据并行框架进行分析建模与训练,实现基于流计算和大数据平台的实时交通流预测。实验结果表明,Flink能够实时捕捉和预处理交通流数据,把数据准时无误送入分布式文件系统中,在此基础上借助大数据框架下的并行分析和建模优势,在实时性数据分析与预测方面取得了较好的效果。 展开更多
关键词 大数据 数据并行 流计算框架 实时处理 交通流预测 分布式系统 实时性分析
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基于分布式证据学习算法的脱硫浆液品质监测模型研究
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作者 徐侠 朱万进 +2 位作者 薛钧赢 苏志刚 郝勇生 《现代化工》 CAS CSCD 北大核心 2024年第S02期348-354,共7页
基于分布式计算框架与证据学习算法,对脱硫浆液品质建立了健康品质监测模型,突破了海量脱硫系统运行数据对基于传统机器学习的浆液品质监测方法所带来的计算瓶颈,并利用该模型对江苏某1000 MW电厂的浆液品质进行了在线监测。测试表明,... 基于分布式计算框架与证据学习算法,对脱硫浆液品质建立了健康品质监测模型,突破了海量脱硫系统运行数据对基于传统机器学习的浆液品质监测方法所带来的计算瓶颈,并利用该模型对江苏某1000 MW电厂的浆液品质进行了在线监测。测试表明,所建立的监测模型能够准确监测出脱硫浆液品质的恶化,与其他3类先进监测方法对比结果说明了所建立模型能够达到最优的报警及时性。将分布式计算框架结合证据理论应用于脱硫浆液品质监测是可行的,为脱硫浆液品质监测提供了一种新方法。 展开更多
关键词 脱硫浆液 状态监测 证据理论 分布式计算框架
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考虑群体决策差异冲突解决机制的配电站房健康状态评估方法
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作者 罗昆 高伟 洪翠 《电力系统保护与控制》 EI CSCD 北大核心 2024年第10期167-178,共12页
针对配电站房缺乏健康评估机制、运维周期设置不合理的问题,提出了一种考虑群体决策差异冲突解决机制的配电站房健康状态综合评估方法。首先,建立配电站房指标体系和专家评价框架,设计了一种新型的二元冲突测量函数来量化全局冲突。然后... 针对配电站房缺乏健康评估机制、运维周期设置不合理的问题,提出了一种考虑群体决策差异冲突解决机制的配电站房健康状态综合评估方法。首先,建立配电站房指标体系和专家评价框架,设计了一种新型的二元冲突测量函数来量化全局冲突。然后,使用专家评价结果的虚假度、可信度、可用度等测度指标构造专家修正因子,以改进D-S证据理论,通过聚合不同专家的评价意见来量化评价指标的权重。接着,建立改进灰色关联度-逼近理想解法(grey relation analysis-technique for order preference by similarity to an ideal solution, GRA-TOPSIS)评估模型,引入灰色关联接近度,与距离接近度融合得到综合接近度,改善TOPSIS评价判据片面性的缺陷。最后,计算每个配电站房的评价值与理想解之间的综合接近度,反映配电站房的健康状态。实验分析表明该方法能兼容专家评价之间的冲突性、差异性、不确定性,与现有方法相比评估结果更具准确性和合理性,对运维人员制定合理的检修决策具有一定的指导价值。 展开更多
关键词 配电站房 专家评价框架 改进D-S证据理论 专家修正因子 改进GRA-TOPSIS评估方法
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毛白杨木材/MOF-5复合材料的制备及甲苯吸附性能研究
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作者 李新宇 高玉磊 +4 位作者 李世杰 杨易菲 张进 任云鹏 赵建国 《木材科学与技术》 北大核心 2024年第1期42-50,共9页
优化MOF-5的合成工艺,确定金属中心与有机配体的最佳配比,并基于最佳配比通过真空浸渍和水热作用在毛白杨木材孔隙内部原位合成MOF-5,制备毛白杨木材/MOF-5复合材料,并对毛白杨木材/MOF-5复合材料的微观形貌、结合机理、孔隙结构和甲苯... 优化MOF-5的合成工艺,确定金属中心与有机配体的最佳配比,并基于最佳配比通过真空浸渍和水热作用在毛白杨木材孔隙内部原位合成MOF-5,制备毛白杨木材/MOF-5复合材料,并对毛白杨木材/MOF-5复合材料的微观形貌、结合机理、孔隙结构和甲苯吸附性能进行表征。结果表明,当金属中心与有机配体物质的量比为1∶3时,合成的MOF-5晶体粒径较小,BET比表面积为268.729 m^(2)/g,孔容为0.136 cm^(3)/g,且具备典型的MOF-5晶体X射线特征峰。在毛白杨木材孔隙内部原位合成的MOF-5的平均负载量为22.6%;红外光谱的分析结果显示MOF-5与毛白杨木材通过氢键和静电相互作用相结合。扫描电镜、压汞法和氮气吸/脱附测试的孔隙结构表明,MOF-5填充了毛白杨木材中的部分大孔和介孔,增加了微孔的比表面积和孔容。常温常压下毛白杨木材/MOF-5复合材料对甲苯的最大吸附量为16.07 cm^(3)/g,展现了较好的甲苯吸/脱附性能。毛白杨木材/MOF-5复合材料在气体吸附与分离领域展现了较好的应用潜力,这为速生木材作为吸附材料的功能化应用提供了参考。 展开更多
关键词 毛白杨木材 金属有机框架 孔径分布 甲苯吸附 功能化改性
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数据驱动的湿地微塑料分布格局与影响因素研究
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作者 李智渊 郭兆凤 +4 位作者 罗艳 刘懂 张东 徐宇尧 徐耀阳 《生态毒理学报》 CAS CSCD 北大核心 2024年第2期75-83,共9页
湿地作为水生态系重要拦污屏障和关键缓冲带,其不断累积的微塑料污染负荷不仅破坏了其自身生态系统结构和功能,也因独特的生态位“塑料际”增加了水源性传播疾病的扩散。然而,目前尚不清楚湿地微塑料在全球范围内的分布格局及其驱动机... 湿地作为水生态系重要拦污屏障和关键缓冲带,其不断累积的微塑料污染负荷不仅破坏了其自身生态系统结构和功能,也因独特的生态位“塑料际”增加了水源性传播疾病的扩散。然而,目前尚不清楚湿地微塑料在全球范围内的分布格局及其驱动机制。鉴于此,本研究基于数据汇编、整理和统计分析框架,整合了来自19个湿地的200个微塑料样本数据,以阐释湿地微塑料赋存特征并识别其影响因素。多元统计分析结果表明,湿地类型和环境介质影响微塑料丰度差异,并且内陆湿地的微塑料丰度显著大于海岸湿地。湿地水体和沉积物中微塑料形状和颜色存在显著相似性,并且纤维状的透明微塑料是其主要赋存形态。湿地水体和沉积物中微塑料赋存格局受到微塑料分析方法,包括采样和提取方法的显著影响。此外,地理距离作为主导因素,影响了湿地微塑料的分布,并且观测到微塑料丰度随距离的增加而减少的趋势。本研究基于湿地微塑料数据特征构建的数据驱动框架,既可为更好地掌握湿地微塑料分布格局及其污染状况提供方法参考,也可为湿地甚至其他水生态系统中微塑料的污染管控提供数据支撑。 展开更多
关键词 湿地 微塑料 数据驱动框架 分布格局 影响因素
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