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Numerical Study on Dry Deposition Processes in Canopy Layer
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作者 雷孝恩 Julius S.Chang 《Advances in Atmospheric Sciences》 SCIE CAS CSCD 1992年第4期491-500,共10页
A coupling model between the canopy layer(CL) and atmospheric boundary layer (ABL) for the study of dry deposition velocity is developed. The model consists of six parts: chemical species conservation equation includi... A coupling model between the canopy layer(CL) and atmospheric boundary layer (ABL) for the study of dry deposition velocity is developed. The model consists of six parts: chemical species conservation equation including absorptive factor; the species uptake action including detailed vertical variation of absorptive element in CL; momentum exchange in CL which is represented by a first-order closure momentum equation with an additional larger-scale diffusive term; momentum exchange in ABL which is described by a complete set of the ABL turbulent statistic parameters; absorptivity (or solubility or reflection) at the surface including effects of the physical and chemical characters of the species, land type, seasonal and diurnal variations of the meteorological variables; and deposition velocity derived by distributions of the species with height in CL. Variational rules of the concentration and deposition velocity with both height and time are simulated with the model for both corn and forest canopies. Results predicted with the bulk deposition velocity derived in the paper consist well with experimental data. 展开更多
关键词 Numerical Study on dry deposition Processes in Canopy Layer
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A database of modeled gridded dry deposition velocities for 45 gaseous species and three particle size ranges across North America
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作者 Leiming Zhang Zhuanshi He +3 位作者 Zhiyong Wu Anne Marie Macdonald Jeffrey R.Brook Shailesh Kharol 《Journal of Environmental Sciences》 SCIE EI CAS CSCD 2023年第5期264-272,共9页
The dry deposition process refers to the flux loss of an atmospheric pollutant due to uptake of the pollutant by the earth’s surfaces.Dry deposition flux of a chemical species is typically calculated as the product o... The dry deposition process refers to the flux loss of an atmospheric pollutant due to uptake of the pollutant by the earth’s surfaces.Dry deposition flux of a chemical species is typically calculated as the product of its surface-layer concentration and its dry deposition velocity(V_(d)).Field measurement based V_(d) data are very scarce or do not exist for many chemical species considered in chemistry transport models.In the present study,gaseous and particulate dry deposition schemes were applied to generate a database of hourly V_(d) for 45 gaseous species and three particle size ranges for two years(2016–2017)at a 15 kmby 15 km horizontal resolution across North America.Hourly V_(d) of the 45 gaseous species ranged from<0.001 to 4.6 cm/sec across the whole domain,with chemical species-dependentmedian(mean)values being in the range of 0.018–1.37 cm/sec(0.05–1.43 cm/sec).The spatial distributions of the two-year average V_(d) showed values higher than 1–3 cm/sec for those soluble and reactive species over certain land types.Soluble species have the highest V_(d) over water surfaces,while insoluble but reactive species have the highest V_(d) over forests.Hourly V_(d) of PM_(2.5) across the whole domain ranged from 0.039 to 0.75 cm/sec with median(mean)value of 0.18(0.20)cm s^(−1),while the mean V_(d) for PM_(2.5)–10 is twice that of PM_(2.5).Uncertainties in the modeled V_(d) are typically on the order of a factor of 2.0 or larger,which needs to be considered when applying the dataset in other studies. 展开更多
关键词 Air quality modeling Atmospheric pollutant Atmospheric deposition dry deposition velocity Spatiotemporal distribution
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SEASONAL CHARACTERIZATION OF DUST DAYS,MASS CONCENTRATION AND DRY DEPOSITION OF ATMOSPHERIC AEROSOLS OVER QINGDAO, CHINA 被引量:15
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作者 RenjianZhang MingxingWang +2 位作者 LifangSheng YutakaKanai AtsuyukiOhta 《China Particuology》 SCIE EI CAS CSCD 2004年第5期196-199,共4页
The seasonal characterization of dust days, mass concentration and dry deposition of atmospheric aero-sols were investigated using the historical data of dust days observed over Qingdao during the period from 1961 to ... The seasonal characterization of dust days, mass concentration and dry deposition of atmospheric aero-sols were investigated using the historical data of dust days observed over Qingdao during the period from 1961 to 2001 and ground-based aerosol sampling data collected in the period from May 2001 to November 2002. In Qingdao most of the dust days occurred in spring and in winter and no dust days existed in summer. The seasonal variation of the uplifting dust day over Qingdao was in phase with that analyzed over North China. The mean mass concentration of the total suspended particles (TSP) in spring, summer, autumn and winter was respectively 300, 110, 113 and 185 mg.m-3. The values and phase of the seasonal oscillation for fine particles were very similar to those for coarse particles except for the month March, during which the concentration of the coarse particles was about 4 times as high as that of the fine parti-cles. Comparison between seasonal variation of mass concentration of aerosols and dust days indicated that high frequency of uplifting dust day was accompanied by high TSP mass concentration. The TSP mass concentration meas-ured by the low-volume instrument was about 30% lower than that measured by high-volume instrument, though the two data sets are highly correlated (correlation coefficient=0.89). The dry deposition flux during the observation period from May 2001 to November 2002 ranged from 0.06 to 0.2 g.m-2.d-1 with a mean value of 0.13 g.m-2.d-1, which was about 1/3 as that over Beijing. 展开更多
关键词 AEROSOL physical characteristics TSP dry deposition
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Dry deposition velocity of total suspended particles and meteorological influence in four locations in Guangzhou,China 被引量:10
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作者 Leifu Chen Shaolin Peng +1 位作者 Jingang Liu Qianqian Hou 《Journal of Environmental Sciences》 SCIE EI CAS CSCD 2012年第4期632-639,共8页
Dry deposition velocity of total suspended particles (TSP) is an effective parameter that describes the speed of atmospheric particulate matter deposit to the natural surface. It is also an important indicator to th... Dry deposition velocity of total suspended particles (TSP) is an effective parameter that describes the speed of atmospheric particulate matter deposit to the natural surface. It is also an important indicator to the capacity of atmosphere self-depuration. However, the spatial and temporal variations in dry deposition velocity of TSP at different urban landscapes and the relationship between dry deposition velocity and the meteorological parameters are subject to large uncertainties. We concurrently investigated this relationship at four different landscapes of Guangzhou, from October to December of 2009. The result of the average dry deposition velocity is (1.49 ± 0.77), (1.44 ± 0.77), (1.13 ±0.53) and (1.82± 0.82) cm/sec for urban commercial landscape, urban forest landscape, urban residential landscape and country landscape, respectively. This spatial variation can be explained by the difference of both particle size composition of TSP and meteorological parameters of sampling sites. Dry deposition velocity of TSP has a positive correlation with wind speed, and a negative correlation with temperature and relative humidity. Wind speed is the strongest factor that affects the magnitude of TSP dry deposition velocity, and the temperature is another considerable strong meteorological factor. We also find out that the relative humidity brings less impact, especially during the dry season. It is thus implied that the current global warming and urban heat island effect may lead to correlative changes in TSP dry deposition velocity, especially in the urban areas. 展开更多
关键词 dry deposition velocity total suspended particles urban landscapes meteorological parameters
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Atmospheric wet and dry deposition of dissolved inorganic nitrogen to the South China Sea 被引量:2
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作者 Ying GAO Lifang WANG +2 位作者 Xianghui GUO Yi XU Li LUO 《Science China Earth Sciences》 SCIE EI CAS CSCD 2020年第9期1339-1352,共14页
At the global scale,atmospheric inputs of nitrogen are an important source of the new nitrogen that supports new marine production,especially in oligotrophic open oceans and marginal seas.This study reports quantities... At the global scale,atmospheric inputs of nitrogen are an important source of the new nitrogen that supports new marine production,especially in oligotrophic open oceans and marginal seas.This study reports quantities of atmospheric deposition of dissolved inorganic nitrogen(DIN)to the largest marginal sea in the North Pacific(the oligotrophic South China Sea,SCS)based primarily on rainwater sampling in the open northwestern region(Yongxing Island)from 2013 to 2015,and aerosol sampling from the SCS basin in June 2017.Atmospheric wet and dry deposition of DIN and their potential contributions to productivity were estimated.The volume-weighted mean rainwater concentrations during the wet and dry seasons were 4.9 and 18.1μmol L-1 for N+N(NO3-+NO2-),and 5.7 and 4.0μmol L-1 for NH4+,respectively.Rainwater concentrations of DIN were lower in the marginal seas than in the open ocean.The aerosol NO3-concentration was 1.15±1.18μg m-3 during the wet season,which is slightly lower than reported for the East China Sea and East Sea,but higher than in the Arabian Sea.Monthly wet and dry deposition rates ranged from 0.4-3.9 and 0.4-1.2 mmol m-2 mon-1 for NO3-,and 0.2-1.3 and 0.01-0.02 mmol m-2 mon-1 for NH4+,respectively.The annual wet and dry deposition fluxes of DIN were estimated to be 16.8 and 10.1 mmol m-2yr-1,respectively.Compared to other marginal seas,the SCS receives less atmospheric NO3-inputs than the Yellow Sea,East China Sea,East Sea,and northeastern Mediterranean Sea.The total atmospheric DIN deposition may account for 1.8-11.1%of the nitrogen supporting new production and 0.7-1.8%of the nitrogen supporting primary production. 展开更多
关键词 South China Sea Atmospheric deposition Wet deposition dry deposition NITRATE NO3- AMMONIUM NH4+
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A NEW DRY DEPOSITION VELOCITY PATTERN AND ITS PRACTICAL APPLICATION IN HIGH RESOLUTION REGIONAL ACID DEPOSITION MODEL 被引量:3
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作者 雷孝恩 《Acta meteorologica Sinica》 SCIE 1996年第1期118-128,共11页
A new dry deposition velocity pattern (NDDVP) for the study of region-scale dry deposition processes is developed. The mean ratio between NDDVP and 1022 experimental data of dry deposi- tion velocity V_d is 1. 06±... A new dry deposition velocity pattern (NDDVP) for the study of region-scale dry deposition processes is developed. The mean ratio between NDDVP and 1022 experimental data of dry deposi- tion velocity V_d is 1. 06±0.82. The result shows that NDDVP is well consistent with experimental data. Practical cases are forecasted by the high resolution regional acid deposition model (EM3) with both NDDVP and old V_d pattern. The maximum ratio between the central concentrations for SO4 can reach 2.4 only due to different V_d patterns. 3-D distributions of species concentrations and dry depositions forecasted by NDDVP are better than those by the old V_d pattern. 展开更多
关键词 new dry deposition velocity pattern (NDDVP) high resolution regional acid deposition model (EM3) canopy layer (CL) land-use
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Vegetation-related dry deposition of global PM_(2.5) from satellite observations 被引量:1
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作者 FENG Huihui DING Ying +6 位作者 ZOU Bin COHEN Jason Blake YE Shuchao YANG Zhuolin QIN Kai LIU Lei GU Xiaodong 《Journal of Geographical Sciences》 SCIE CSCD 2022年第4期589-604,共16页
Vegetation plays an important role in the dry deposition of particles with significant spatial variability,but the magnitude remains unclear at the global scale.With the aid of satellite products,this study estimated ... Vegetation plays an important role in the dry deposition of particles with significant spatial variability,but the magnitude remains unclear at the global scale.With the aid of satellite products,this study estimated the vegetation-related dry deposition of fine particulate matter(PM_(2.5)).Methodologically,dry deposition was first calculated using an empirical algorithm.Then,deposition on the leaf surface was estimated to evaluate the influence of vegetation.Our results showed that the mean deposition velocity(V_(d))of global PM_(2.5)was 0.91×10^(-3)μg·m^(-2)·s^(-1),with high velocities observed in sparsely vegetated regions because of the high friction velocity.Under the combined effect of the PM_(2.5)mass concentration and deposition velocity,the global mean dry deposition reached 0.47 g·m-^(2)·yr^(-1).Global vegetation absorbed 0.26 g·m-^(2)·yr^(-1)from PM_(2.5)pollution sources,contributing 54.98%of the total dry deposition.Spatially,vegetation-related dry deposition was high in the Amazon,Central Africa and East China due to dense vegetation coverage or serious pollution.Temporally,the increasing trends were mainly in Central Africa and India because of worsening air pollution.The results of this study helped to clarify the impact of vegetation on air pollution,which supported related land management and planning for air quality improvement. 展开更多
关键词 air pollution PM_(2.5) dry deposition vegetation change globe SATELLITE
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Dry deposition of PM_(10) over the Yellow Sea during Asian dust events from 2001 to 2007
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作者 Han Yan Xiaohuan Liu +1 位作者 Jianhua Qi Huiwang Gao 《Journal of Environmental Sciences》 SCIE EI CAS CSCD 2014年第1期54-64,共11页
Dry deposition velocities and fluxes of PM10 during Asian dust events over the Yellow Sea from 2001 to 2007 were investigated using observation data in Qingdao, China and Jeju, Korea. The dry deposition velocities of ... Dry deposition velocities and fluxes of PM10 during Asian dust events over the Yellow Sea from 2001 to 2007 were investigated using observation data in Qingdao, China and Jeju, Korea. The dry deposition velocities of PM 10 during dust events over the Yellow Sea ranged from 0.19 to 8.17 cm/sec, with an average of 3.38 cm/sec. Dry deposition fluxes of PM10 during dust events over the Yellow Sea were in the range of 68.5-2647.1 mg/(m2.day), with an average of 545.4 mg/(m2.day), which is 2-10 times higher than those reported by other studies for both dust and non-dust periods. It was estimated that 2.6× 10^11-48.7 × 10^11 g dust particles deposit to the Yellow Sea during dust events through dry deposition every year. Compared with the results in previous studies, it was found that the dry deposition of PM10 over the Yellow Sea during dust events in the years with high frequency of dust could account for a large or overwhelming fraction of the annual total dry deposition. Backward air mass trajectory analysis showed that dust events influenced Jeju mainly originated from the desert regions located in Mongolia and Inner Mongolia, China. There were 119 backward trajectories influenced both Qingdao and Jeju during 15 dust events from 2001 to 2007, accounting for 61.3% of the total trajectories of 194, indicating that Qingdao and Jeju were usually on the same pathway of dust transport downwind from source areas. 展开更多
关键词 Asian dust the Yellow Sea dry deposition fluxes backward trajectory analysis
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Wet and dry deposition fluxes of heavy metals in Pearl River Delta Region(China):Characteristics,ecological risk assessment,and source apportionment 被引量:21
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作者 Lyumeng Ye Minjuan Huang +6 位作者 Buqing Zhong Xuemei Wang Qiulan Tu Haoran Sun Chao Wang Luolin Wu Ming Chang 《Journal of Environmental Sciences》 SCIE EI CAS CSCD 2018年第8期106-123,共18页
The atmospheric deposition of heavy metals poses serious risks to the ecological system and human health. To advance our knowledge of atmospheric dry/wet heavy metal deposition in the PRD region, monthly fluxes were e... The atmospheric deposition of heavy metals poses serious risks to the ecological system and human health. To advance our knowledge of atmospheric dry/wet heavy metal deposition in the PRD region, monthly fluxes were examined based on soluble/insoluble fractions of five heavy metal elements(Cu, Pb, Cd, Cr and Zn) in samples collected from January 2014 to December 2015 at Guangzhou(urban) and Dinghushan(suburban) sites. The ratios of wet/dry deposition fluxes indicated that heavy metal deposition was governed by wet deposition rather than dry deposition in the PRD region. Affected by the shifting of the Asian monsoon, wet deposition fluxes exhibited significant seasonal variation between summer monsoon seasons(April to September) and winter monsoon seasons(October to February) in this region. Cd was classified as an extremely strong potential ecological risk based on solubility and the Hakanson ecological risk index. Source contributions to wet deposition were calculated by PMF, suggesting that dust, biomass burning, industries,vehicles, long-range transport and marine aerosol sources in Guangzhou, and Zn fertilizers,marine aerosol sources, agriculture, incense burning, biomass burning, vehicles and the ceramics industry in Dinghushan, were the potential sources of heavy metals. 展开更多
关键词 Atmospheric dry/wet deposition Heavy metals Ecological risk assessment Sources apportionment The Pearl River Delta region
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Study on the Characteristics of Atmospheric Dry and Wet Deposition in the Upper Reaches of Baiyangdian
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作者 Ye LI Hongbo LI +2 位作者 Qi ZHAO Ning LUO Xinyong CHEN 《Meteorological and Environmental Research》 CAS 2022年第1期63-66,共4页
To study the characteristics of atmospheric dry and wet deposition in the upper reaches of Baiyangdian,two sampling sites in Baoding City were monitored for 1 year from September 2018 to August 2019.The results showed... To study the characteristics of atmospheric dry and wet deposition in the upper reaches of Baiyangdian,two sampling sites in Baoding City were monitored for 1 year from September 2018 to August 2019.The results showed that the dry and wet deposition fluxes of total nitrogen(TN)during the monitoring period were 6.87 and 6.46 kg/(hm^(2)·a),respectively.The ratio of wet to dry deposition of TN was approximately 1∶1,with wet deposition being dominated by ammonium nitrogen deposition.The dry and wet deposition fluxes of total phosphorus(TP)were 0.228 and 0.125 kg/(hm^(2)·a),and it was dominated by dry deposition.The average concentration of TN in wet deposition exceeded the standard threshold for eutrophic waters,and its ecological effects on the Baiyangdian basin should be concerned.Wet deposition fluxes of nitrogen and phosphorus had a significantly positive correlation with rainfall,while their deposition concentrations were negatively correlated with rainfall.The dry deposition of atmospheric nitrogen and phosphorus was influenced by the amount of dustfall and climatic factors such as rainfall,temperature,and humidity,which mainly occurred from April to August. 展开更多
关键词 Atmospheric deposition dry and wet deposition Nitrogen deposition Phosphorus deposition deposition flux
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Annual Fluxes of Heavy Metal Elements in Atmospheric Dry and Wet Depositions in the Pearl River Delta Economic Region, Guangdong Province
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作者 Lu Lu Cen Kuang 《Journal of Geoscience and Environment Protection》 2021年第5期8-14,共7页
<div style="text-align:justify;"> There are 158 sampling points to be set up in the Pearl River delta economic region. The collecting period is mostly one year, namely, from July 2007 to July 2008. The... <div style="text-align:justify;"> There are 158 sampling points to be set up in the Pearl River delta economic region. The collecting period is mostly one year, namely, from July 2007 to July 2008. The eight heavy metal elements of Cr, Ni, Cu, Pb, Zn, As, Hg, and Cd in 474 dry and wet deposition samples were tested in terms of the standard procedures. Their average annual fluxes have no obvious difference between dry deposition and wet deposition. So these elements might be at an equilibrium or quasi-equilibrium state between dry deposition and wet deposition. </div> 展开更多
关键词 Atmospheric dry and Wet deposition Heavy Metal Element FLUX Pearl River Delta Economic Region
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Major Ions in Atmospheric Deposition in Lake Kivu Basin
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作者 Mashimango Bagalwa Jackson Gilbert Mwanjalolo Majaliwa +2 位作者 Katcho Karume Sarah Akello Frank Kansiime 《Journal of Environmental Protection》 CAS 2023年第3期185-205,共21页
This study investigated the major ion composition and sources in wet and dry deposition samples collected over 15 months (December 2017 to February 2019) at four stations representing four different land use/cover typ... This study investigated the major ion composition and sources in wet and dry deposition samples collected over 15 months (December 2017 to February 2019) at four stations representing four different land use/cover types on the western side of Lake Kivu basin in D.R. Congo. The samples were collected every 13 days for dry deposition and two to three times per month for wet deposition. Samples were analyzed for major ionic components (Cl<sup>-, NO<sub>-</sub>3</sup>, SO<sub>2-</sub>4</sup>, Na<sup>+</sup>, K<sup>+</sup>, NH<sub>+</sub>4</sup>, Ca<sup>2+</sup>, CO<sub>2-</sub>3</sup>, HCO<sub>-</sub>3</sup> and Mg<sup>2+</sup>). Electrical conductivity and pH were analyzed immediately in the field while major ion measurements were in the laboratory. Results showed the pH of both the dry and the wet depositions were higher than what would have been expected based on equilibration with atmospheric CO<sub>2</sub> (pH > 5.6) at all four sites, with conductivity less than 50 μS/cm. The neutralization process in dry and wet atmospheric deposition is due to Ca<sup>2+</sup>, NH<sub>+</sub>4</sup>, HCO<sub>-</sub>3</sup> and CO<sub>2-</sub>3</sup>. The anion: cation ratio in dry deposition was close to 1 for Iko and Bukavu, and it was greater than 1.0 (1.1 - 1.2) for Lwiro and Goma in wet deposition. The dominant anions in wet deposition were SO<sub>2-</sub>4</sup> and NO<sub>-</sub>3</sup>, found around the rural area near cement factory and the urban area near active volcanoes, respectively. The most abundant cation was Na+ followed by K<sup>+</sup>. The enrichment factors and correlation analysis suggest that the main sources of Ca<sup>2+</sup>, Na<sup>+</sup> and Mg<sup>2+</sup> were disintegration of soil processes, aeolian suspension of soil and volcanic ash, biomass burning and the cement/lime factory around the Lake Kivu basin. 展开更多
关键词 dry and Wet deposition Major Ions Lake Kivu
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Atmospheric deposition of inorganic nitrogen in a semi-arid grassland of Inner Mongolia, China 被引量:5
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作者 ZHANG Yibo XU Wen +4 位作者 WEN Zhang WANG Dandan HAO Tianxiang TANG Aohan LIU Xuejun 《Journal of Arid Land》 SCIE CSCD 2017年第6期810-822,共13页
Due to increasing global demand for crop production and energy use, more and more reactive nitrogen(Nr) has been generated and emitted to the environment. As a result, global atmospheric nitrogen(N) deposition has... Due to increasing global demand for crop production and energy use, more and more reactive nitrogen(Nr) has been generated and emitted to the environment. As a result, global atmospheric nitrogen(N) deposition has tripled since the industrial revolution and the ecological environment and human health have been harmed. In this study, we measured dry and wet/bulk N deposition from July 2013 to December 2015 in a semi-arid grassland of Duolun County, Inner Mongolia, China. The samples of dry and wet/bulk N deposition were collected monthly with a DELTA(DEnuder for Long Term Atmospheric sampling) system and with Gradko passive samplers and a precipitation gauge. The measured results show that the annual mean concentrations of NH_3, NO_2, HNO_3, particulate NH_4~+(pNH_4~+) and particulate NO_3^-(pNO_3^-) in atmosphere were 2.33, 1.90, 0.18, 1.42 and 0.42 μg N/m3, respectively, and that the annual mean volume-weighted concentrations of NH_4~+-N and NO_3^--N in precipitation were 2.71 and 1.99 mg N/L, respectively. The concentrations of Nr components(including NH_3, NO_2, HNO_3, p NH_4~+, pNO_3^-, NH_4~+-N and NO_3^--N) exhibited different seasonal variations. Specifically, NO_2 and HNO_3 exhibited higher concentrations in autumn than in summer, while the other Nr components(NH_3, pNH_4~+, pNO_3^-, NH_4~+-N and NO_3^--N) showed the highest values in summer. Based on measured concentrations of Nr components and their deposition velocities estimated using the GEOS-Chem global atmospheric chemical transport model, the calculated annual mean dry deposition fluxes were 3.17, 1.13, 0.63, 0.91 and 0.36 kg N/(hm^2·a) for NH_3, NO_2, HNO_3, p NH_4~+ and pNO_3^-, respectively, and the calculated annual mean wet/bulk deposition fluxes were 5.37 and 3.15 kg N/(hm^2·a) for NH_4~+-N and NO_3^--N, respectively. The estimated annual N deposition(including dry N deposition and wet/bulk N deposition) reached 14.7 kg N/(hm^2·a) in grassland of Duolun County, approaching to the upper limit of the N critical load(10–15 kg N/(hm^2·a)). Dry and wet/bulk deposition fluxes of all Nr components(with an exception of HNO_3) showed similar seasonal variations with the maximum deposition flux in summer and the minimum in winter. Reduced Nr components(e.g., gaseous NH_3 and p NH_4~+ in atmosphere and NH_4~+-N in precipitation) dominated the total N deposition at the sampling site(accounted for 64% of the total N deposition), suggesting that the deposited atmospheric Nr mainly originated from agricultural activities. Considering the projected future increases in crop and livestock production in Inner Mongolia, the ecological and human risks to the negative effects of increased N deposition could be increased if no mitigation measures are taken. 展开更多
关键词 atmospheric reactive nitrogen dry deposition wet/bulk deposition reduced nitrogen grassland ecosystem Inner Mongolia
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Gap edge canopy buffering of throughfall deposition in a subalpine natural forest
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作者 Siyi Tan Qing Dong +3 位作者 Xiangyin Ni Kai Yue Shu Liao Fuzhong Wu 《Forest Ecosystems》 SCIE CSCD 2022年第4期503-510,共8页
Base cation loads are rarely considered in forest gap edge canopies,but they can play critical roles in capturing or buffering atmospheric deposition in forests with frequent gap disturbances,such as subalpine forests... Base cation loads are rarely considered in forest gap edge canopies,but they can play critical roles in capturing or buffering atmospheric deposition in forests with frequent gap disturbances,such as subalpine forests.We selected an expanded gap edge canopy and a closed canopy in a subalpine natural forest on the eastern Tibetan Plateau.The throughfall deposition and canopy exchange processes of common base cations(K^(+),Ca^(2+),Na^(+),and Mg^(2+))were continuously studied over two years.The results showed that the enrichment ratio and fluxes had lower levels of base cations in the gap-edge canopy than in the closed canopy,which indicated that base cations were concentrated more in the closed canopy than in the gap-edge canopy.Although Ca^(2+)in the gap-edge canopy showed a higher net throughfall flux,the annual net throughfall fluxes of K^(+),Na^(+) and Mg^(2+) within the gap-edge canopy were 1.83,6.75 and 2.95 times lower than those in the closed canopy,respectively.Moreover,dry deposition fluxes of base cations significantly decreased in the gap edge canopy compared to those in the closed canopy,and the decreasing tendency was more significant during the snowy season than during the rainy season.Overall,these results suggest that the amount of base cations in subalpine natural forest ecosystems may be overestimated when the throughfall deposition of ions in gap edge canopies is ignored. 展开更多
关键词 Canopy exchange dry deposition THROUGHFALL Subalpine forest Precipitation deposition
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Deposition of water-soluble inorganic ions in PM_(2.5) in a typical forestry system in Beijing,China
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作者 Junqi Ding Xiaoxiu Lun +4 位作者 Weifang Ma Lu Zhao Yingying Cao Fengbin Sun Renna Li 《Forest Ecosystems》 SCIE CSCD 2018年第4期486-497,共12页
Background: Rapid economic development in China has resulted in an increase in severe air pollution in city groups such as the Beijing-Tianjin-Hebei Metropolitan Region. PM2.5(fine particles with an aerodynamic equiva... Background: Rapid economic development in China has resulted in an increase in severe air pollution in city groups such as the Beijing-Tianjin-Hebei Metropolitan Region. PM2.5(fine particles with an aerodynamic equivalent diameter of 2.5 μm or less) is one of the most important pollutants. The deposition process is an important way of removing particles from the air. To evaluate the effect of an urban forest on atmospheric particle removal, a concentration gradient method was used to measure the deposition velocities of water-soluble inorganics in PM2.5 in two national forest parks in Beijing, China. The following eight water-soluble inorganic ions in PM2.5 were investigated: sodium, ammonium, potassium, magnesium, calcium, chloride, nitrate, and sulfate.Methods: Samples were taken from two sites in Beijing from the 7 th to the 15 th May, 2013. The concentrations of water-soluble inorganic ions were analyzed with ion chromatography. We used the concentration gradient technique to estimate the deposition flux and velocity. To determine the relationships between leaf traits and particle accumulation, typical leaf samples from each selected species were studied using scanning electron microscopy.Results: The total deposition flux and total deposition velocity during the daytime were higher than those at night.Sulfate showed the biggest deposition flux and velocity at both study sites, whereas the other ions showed different trends at each site. Result from higher proportion of coniferous to broadleaved trees, the total deposition flux of the eight ions measured in Jiufeng National Forest Park was greater than that in Olympic Forest Park.Conclusions: The deposition velocity was affected by meteorological conditions such as wind speed, temperature,and humidity. The deposition velocity was also influenced by tree species. The surface of plants is an important factor influencing particle deposition. The results of this study may help in assessing the effects of forestry systems on particle removal and provide evidence for urban air pollution control and afforestation of urban areas. 展开更多
关键词 Fine particle Water-soluble inorganics FOREST dry deposition deposition velocity
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The study on the depositional styles of major ions and the climatic effect of nssSO_4^(2-)in Princess Elizabeth Land, Antarctica
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作者 张明军 李忠勤 +3 位作者 秦大河 效存德 康建成 李军 《Chinese Journal of Polar Science》 2000年第2期107-112,共6页
Snow samples collected from a 50 m firn core and two snow pits along the route of the 1996/1997 Chinese First Antarctic Inland Traverse Expedition in Princess Elizabeth Land, East Antarctica, have been analyzed for ch... Snow samples collected from a 50 m firn core and two snow pits along the route of the 1996/1997 Chinese First Antarctic Inland Traverse Expedition in Princess Elizabeth Land, East Antarctica, have been analyzed for chemical composition and oxygen isotope ratio. Analyzing the relationship between the concentration and flux of major ions and accumulation rate can draw the following conclusions. 1) The concentrations of major ions in the atmosphere in the study region is big enough so that the concentrations of the ions do not vary with snow accumulation rate, that is to say, the concentrations of major chemical species are independent of snow accumulation rate. 2) The results of analyzing the depositional styles of major chemical species suggest that wet deposition dominates the major ions flux. In addition, there is no apparent correlation between nssSO 2- 4 fluctuations and isotope profile. This would indicate the short-term climatic effect of volcanism is not evident in the region. 展开更多
关键词 ion dry deposition wet deposition volcanic.
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Effects of a Remotely Sensed Land Cover Dataset with High Spatial Resolution on the Simulation of Secondary Air Pollutants over China Using the Nested-grid GEOS-Chem Chemical Transport Model 被引量:1
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作者 LI Mingwei WANG Yuxuan JU Weimin 《Advances in Atmospheric Sciences》 SCIE CAS CSCD 2014年第1期179-187,共9页
A number of remotely sensed land cover datasets with spatial resolutions ~〈 1 km have recently become available or are in the process of being mapped. The application of these higher resolution and more up-to-date la... A number of remotely sensed land cover datasets with spatial resolutions ~〈 1 km have recently become available or are in the process of being mapped. The application of these higher resolution and more up-to-date land cover datasets in chemical transport models (CTMs) is expected to improve the simulation of dry deposition and biogenic emissions of non-methane volatile organic compounds (NMVOCs), which affect ozone and other secondary air pollutants. In the present study, we updated the land cover dataset in the nested-grid GEOS-Chem CTM with the 1 km resolution GLC2000 land cover map and examined the resulting changes in the simulation of surface ozone and sulfate over China in July 2007. Through affecting the dry deposition velocities of ozone and its precursors, using GLC2000 in the dry deposition module can decrease the simulated surface ozone by 3% (up to 6 ppb) over China. Simulated surface sulfate shows an increase of 3% in northwestern China and a decrease of 1% in northern China. Applying GLC2000 in the biogenic emissions of the NMVOC module can lead to a 0.5--4.5 ppb increase in simulated surface ozone over East China, mainly driven by the larger cove~:age of broadleaf trees in East China in the GLC2000 dataset. Our study quantifies the large sensitivity to land cover dataset~ with different spatial resolutions and time periods of simulated secondary air pollutants over China, supporting ongoing research efforts to produce high resolution and dynamically updated land cover datasets over China, as well as for the globe. 展开更多
关键词 land cover dry deposition biogenic emissions OZONE SULFATE
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Fluxes of NH_3 and HNO_3 over heathland in the Netherlands:implications for chemical interactions
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作者 Zhang Yuanhang Center of Environmental Sciences,Peking University,Beijing 100871,China 《Journal of Environmental Sciences》 SCIE EI CAS CSCD 1997年第1期49-58,共10页
The surface exchange of NH_3 and HNO_3 gases over heathland was measured with the aerodynamic gradient method in Leende,the Netherlands during April 25 and May 9,1991.Due to reactions in the system NH_3,HNO_3 and NH_4... The surface exchange of NH_3 and HNO_3 gases over heathland was measured with the aerodynamic gradient method in Leende,the Netherlands during April 25 and May 9,1991.Due to reactions in the system NH_3,HNO_3 and NH_4NO_3,the NH_3 deposition flux is overestimated,while HNO_3 shows apparent emission fluxes mostly during the field experiment.Results reveal that NH_3 gradients are influenced slightly by HNO_3 and the HNO_3 gradients are strongly controlled by the NH_3.A clear relationship between NH_3 and HNO_3 gradient is suggested by the Leende experiment. Before the late afternoon,NH_3 deposition gradients will cause HNO_3 upward gradients,meanwhile the NH_3 gradients themselves will become smaller.After the HNO_3 upward gradient reaches maxi- mum,the NH_3 deposition gradients will be enlarged or the emission gradients depressed,while the HNO_3 upward gradients become smaller. 展开更多
关键词 dry deposition AMMONIA nitric acid equilibrium fluxes.
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Altitude-dependent distribution of 137Cs in the environment:a case study of Aragats massif, Armenia
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作者 Konstantin Pyuskyulyan Stephen P.LaMont +3 位作者 Vovik Atoyan Olga Belyaeva Nona Movsisyan Armen Saghatelyan 《Acta Geochimica》 EI CAS CSCD 2020年第1期127-138,共12页
This paper considers the distribution of technogenic 137Cs and naturally occurring radionuclides:238 U,232 Th and40 R concentrations in soils and 137Cs in atmospheric dry depositions by altitudinal belts of the Aragat... This paper considers the distribution of technogenic 137Cs and naturally occurring radionuclides:238 U,232 Th and40 R concentrations in soils and 137Cs in atmospheric dry depositions by altitudinal belts of the Aragats mountain massif,Republic of Armenia.Undisturbed soil samples were collected at altitudes from 1000 to 3200 m.For the determination of geochemical variability,two soil sampling campaigns were undertaken.Atmospheric dry depositions were sampled from five stations at1100-3200 m collected onto organic fiber filters between June and December 2016.137Cs activity was measured using a high-purity Germanium detector coupled to a multichannel analyzer(Canberra).Results indicated that specific activity of 137Cs in soils at 1000 m is495-528 Bq m^-2,andat3200 mis10,500-11,470 Bq m^-2.No correlation observed for 137Cs versus naturally occurring radionuclides,which varies in distribution by altitude.Specific activities of 137Cs in dry atmospheric depositions varies from 1.06 at 846 m to2.37 Bq m^-2 per quarter at 3200 m and increases as the altitude increases.Activities of 137Cs in soil and dry atmospheric deposition correlated significantly,and 137Cs activity in soils and atmospheric dry depositions decrease as the absolute altitude decreases.The 50-year effective dose from exposure to 137Cs fallout varies with altitude from 0.007 to 1.42 m Sv. 展开更多
关键词 137Cs Distribution by altitude Naturally occurring radionuclides TOPSOIL dry atmospheric depositions Gamma radiation Mountain regions
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Influence of specimen-reconstituting method on the undrained response of loose granular soil under static loading
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作者 Noureddine Della Ahmed Arab Mostefa Belkhatir 《Acta Mechanica Sinica》 SCIE EI CAS CSCD 2011年第5期796-802,共7页
This paper describes the results of an experimental study on the undrained shear behaviour of loose sand collected from the location close to the epicenter of the recent Chlef (Algeria) Earthquake (October 10,1980... This paper describes the results of an experimental study on the undrained shear behaviour of loose sand collected from the location close to the epicenter of the recent Chlef (Algeria) Earthquake (October 10,1980).The study focuses on the effects of the mode of the soil deposition on the liquefaction resistance of the Chlef sand.For this purpose,the results of undrained monotonic triaxial compression tests performed on samples with initial density of 0.29 under initial confining pressures ranged from 50 kPa to 200 kPa are presented.The specimens were prepared by two depositional methods namely dry funnel pluviation and wet deposition.It was found that there was a marked difference in the undrained behaviour of sand in terms of maximal deviatoric stress,peak strength,residual strength and excess pore water pressure,even though the density and stress conditions were identical.The conclusion was that the soil fabric was responsible for this result.The results indicated also that at low confining pressures,the specimens reconstituted by the wet deposition method exhibited complete static liquefaction (zero effective confining pressure and zero stress difference). 展开更多
关键词 Liquefaction · Undrained · dry funnel pluviation · Wet deposition · Residual strength
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