The influences of climate change on the velocity of dry matter accumulation of spring wheat and numerical simulation in arid and semi-arid regions under the condition of rainfalled agriculture or irrigated agriculture...The influences of climate change on the velocity of dry matter accumulation of spring wheat and numerical simulation in arid and semi-arid regions under the condition of rainfalled agriculture or irrigated agriculture were quantitatively analysed by using the field experimental data. The results showed that the velocity of dry matter accumulation of spring wheat was declined with the temperature rising. The accumulating velocity would be declined 4.9 - 14.0% in irrigated agriculture area when air temperature rose in 0.5-4.0℃ ; but in rainfalled agriculture regions, the velocity of dry matter accumulation would be increased with the soil moisture increasing when air temperature rose in 0.5-1.0℃ and decreased when the air temperature rose in 3.0-4.0 ℃ .展开更多
A two-year study in a typical red soil region of Southern China was conductedto determine 1) the dry deposition velocity (V_d) for SO_2 and particulate SO_4^(2-) above abroadleaf forest, and 2) atmospheric sulfur flux...A two-year study in a typical red soil region of Southern China was conductedto determine 1) the dry deposition velocity (V_d) for SO_2 and particulate SO_4^(2-) above abroadleaf forest, and 2) atmospheric sulfur fluxes so as to estimate the contribution of variousfractions in the total. Using a resistance model based on continuous hourly meteorological data,atmospheric dry sulfur deposition in a forest was estimated according to V_d and concentrations ofboth atmospheric SO_2 and particulate SO_4^(2-). Meanwhile, wet S deposition was estimated based onrainfall and sulfate concentrations in the rainwater. Results showed that about 99% of the drysulfur deposition flux in the forest resulted from SO_2 dry deposition. In addition, the observeddry S deposition was greater in 2002 than in 2000 because of a higher average concentration of SO_2in 2002 than in 2000 and not because of the average dry deposition velocity which was lower for SO_2in 2002. Also, dry SO_2 deposition was the dominant fraction of deposited atmospheric sulfur inforests, contributing over 69% of the total annual sulfur deposition. Thus, dry SO_2 depositionshould be considered when estimating sulfur balance in forest ecological systems.展开更多
Aerosol nonsphericity causes great uncertainty in radiative forcing assessments and climate simulations.Although considerable studies have attempted to quantify this uncertainty,the relationship between aerosol nonsph...Aerosol nonsphericity causes great uncertainty in radiative forcing assessments and climate simulations.Although considerable studies have attempted to quantify this uncertainty,the relationship between aerosol nonsphericity and particle size is usually not considered,thus reducing the accuracy of the results.In this study,a coupled inversion algorithm combining an improved stochastic particle swarm optimization algorithm and angular light scattering is used for the nonparametric estimation of aerosol nonsphericity variation with particle size,and the optimal sample selection method is employed to screen the data.Based on the verification of inversion accuracy,the variation of aerosol aspect ratio with particle size based on the ellipsoidal model in global regions has been obtained from Aerosol Robotic Network(AERONET)data,and the effect of nonsphericity on radiative forcing and dry deposition has been studied.The results show that the aspect ratio increases with particle size in all regions,with the maximum ranging from 1.4 to 1.8 in the desert,reflecting the differences in aerosol composition at different particle sizes.In radiation calculations,considering aerosol nonsphericity makes the aerosol cooling effect weaker and surface radiative fluxes increase,but hardly changes the aerosol absorption,with maximum differences of 9.22%and 22.12%at the bottom and top of the atmosphere,respectively.Meanwhile,the differences in radiative forcing between aspect ratios as a function of particle size and not varying with particle size are not significant,averaging less than 2%.Besides,the aspect ratio not varying with particle size underestimates the deposition velocity of small particles and overestimates that of large particles compared to that as a function of particle size,with maximum differences of 7%and 4%,respectively.展开更多
Dry deposition velocity of total suspended particles (TSP) is an effective parameter that describes the speed of atmospheric particulate matter deposit to the natural surface. It is also an important indicator to th...Dry deposition velocity of total suspended particles (TSP) is an effective parameter that describes the speed of atmospheric particulate matter deposit to the natural surface. It is also an important indicator to the capacity of atmosphere self-depuration. However, the spatial and temporal variations in dry deposition velocity of TSP at different urban landscapes and the relationship between dry deposition velocity and the meteorological parameters are subject to large uncertainties. We concurrently investigated this relationship at four different landscapes of Guangzhou, from October to December of 2009. The result of the average dry deposition velocity is (1.49 ± 0.77), (1.44 ± 0.77), (1.13 ±0.53) and (1.82± 0.82) cm/sec for urban commercial landscape, urban forest landscape, urban residential landscape and country landscape, respectively. This spatial variation can be explained by the difference of both particle size composition of TSP and meteorological parameters of sampling sites. Dry deposition velocity of TSP has a positive correlation with wind speed, and a negative correlation with temperature and relative humidity. Wind speed is the strongest factor that affects the magnitude of TSP dry deposition velocity, and the temperature is another considerable strong meteorological factor. We also find out that the relative humidity brings less impact, especially during the dry season. It is thus implied that the current global warming and urban heat island effect may lead to correlative changes in TSP dry deposition velocity, especially in the urban areas.展开更多
A new dry deposition velocity pattern (NDDVP) for the study of region-scale dry deposition processes is developed. The mean ratio between NDDVP and 1022 experimental data of dry deposi- tion velocity V_d is 1. 06±...A new dry deposition velocity pattern (NDDVP) for the study of region-scale dry deposition processes is developed. The mean ratio between NDDVP and 1022 experimental data of dry deposi- tion velocity V_d is 1. 06±0.82. The result shows that NDDVP is well consistent with experimental data. Practical cases are forecasted by the high resolution regional acid deposition model (EM3) with both NDDVP and old V_d pattern. The maximum ratio between the central concentrations for SO4 can reach 2.4 only due to different V_d patterns. 3-D distributions of species concentrations and dry depositions forecasted by NDDVP are better than those by the old V_d pattern.展开更多
The dry deposition process refers to the flux loss of an atmospheric pollutant due to uptake of the pollutant by the earth’s surfaces.Dry deposition flux of a chemical species is typically calculated as the product o...The dry deposition process refers to the flux loss of an atmospheric pollutant due to uptake of the pollutant by the earth’s surfaces.Dry deposition flux of a chemical species is typically calculated as the product of its surface-layer concentration and its dry deposition velocity(V_(d)).Field measurement based V_(d) data are very scarce or do not exist for many chemical species considered in chemistry transport models.In the present study,gaseous and particulate dry deposition schemes were applied to generate a database of hourly V_(d) for 45 gaseous species and three particle size ranges for two years(2016–2017)at a 15 kmby 15 km horizontal resolution across North America.Hourly V_(d) of the 45 gaseous species ranged from<0.001 to 4.6 cm/sec across the whole domain,with chemical species-dependentmedian(mean)values being in the range of 0.018–1.37 cm/sec(0.05–1.43 cm/sec).The spatial distributions of the two-year average V_(d) showed values higher than 1–3 cm/sec for those soluble and reactive species over certain land types.Soluble species have the highest V_(d) over water surfaces,while insoluble but reactive species have the highest V_(d) over forests.Hourly V_(d) of PM_(2.5) across the whole domain ranged from 0.039 to 0.75 cm/sec with median(mean)value of 0.18(0.20)cm s^(−1),while the mean V_(d) for PM_(2.5)–10 is twice that of PM_(2.5).Uncertainties in the modeled V_(d) are typically on the order of a factor of 2.0 or larger,which needs to be considered when applying the dataset in other studies.展开更多
Based on the regional acid deposition model(RADM),a high resolution model for species exchange in the troposphere(EM3)is designed.EM3 differs considerably in the following 5 aspects from RADM.First,the vertical grid l...Based on the regional acid deposition model(RADM),a high resolution model for species exchange in the troposphere(EM3)is designed.EM3 differs considerably in the following 5 aspects from RADM.First,the vertical grid levels in the planetary boundary layer(PBL)are increased.Second,layered vertical eddy diffusivity patterns in the troposphere(TL)are considered.Third,layered horizontal eddy diffusivity patterns within TL is used.Fourth,new dry deposition velocity pattern including the effect of plant canopy layer(CL)vertical structure is adopted.Fifth,advective scheme of second-order moment conservation with less numerical diffusion is used.OSCAR 4 case is comparatively simulated with both EM3 and RADM.The results show that 3-D distribution laws of chemical species in whole TL are forecasted by EM3 better than by RADM.Under the same conditions,all ratios of the central concentrations simulated with both models in lower PBL are more than 1.8,the maximum can be more than 3.展开更多
文摘The influences of climate change on the velocity of dry matter accumulation of spring wheat and numerical simulation in arid and semi-arid regions under the condition of rainfalled agriculture or irrigated agriculture were quantitatively analysed by using the field experimental data. The results showed that the velocity of dry matter accumulation of spring wheat was declined with the temperature rising. The accumulating velocity would be declined 4.9 - 14.0% in irrigated agriculture area when air temperature rose in 0.5-4.0℃ ; but in rainfalled agriculture regions, the velocity of dry matter accumulation would be increased with the soil moisture increasing when air temperature rose in 0.5-1.0℃ and decreased when the air temperature rose in 3.0-4.0 ℃ .
基金Project supported by the National Key Basic Research Support Foundation (NKBRSF) of China (No. 1999011805)the Knowledge Innovation Program of Chinese Academy of Sciences (No.ISSASIP0205) the State Key Laboratory of Soil and Sustainable Agriculture, C
文摘A two-year study in a typical red soil region of Southern China was conductedto determine 1) the dry deposition velocity (V_d) for SO_2 and particulate SO_4^(2-) above abroadleaf forest, and 2) atmospheric sulfur fluxes so as to estimate the contribution of variousfractions in the total. Using a resistance model based on continuous hourly meteorological data,atmospheric dry sulfur deposition in a forest was estimated according to V_d and concentrations ofboth atmospheric SO_2 and particulate SO_4^(2-). Meanwhile, wet S deposition was estimated based onrainfall and sulfate concentrations in the rainwater. Results showed that about 99% of the drysulfur deposition flux in the forest resulted from SO_2 dry deposition. In addition, the observeddry S deposition was greater in 2002 than in 2000 because of a higher average concentration of SO_2in 2002 than in 2000 and not because of the average dry deposition velocity which was lower for SO_2in 2002. Also, dry SO_2 deposition was the dominant fraction of deposited atmospheric sulfur inforests, contributing over 69% of the total annual sulfur deposition. Thus, dry SO_2 depositionshould be considered when estimating sulfur balance in forest ecological systems.
基金the National Natural Science Foundation of China(grant No.52376072)。
文摘Aerosol nonsphericity causes great uncertainty in radiative forcing assessments and climate simulations.Although considerable studies have attempted to quantify this uncertainty,the relationship between aerosol nonsphericity and particle size is usually not considered,thus reducing the accuracy of the results.In this study,a coupled inversion algorithm combining an improved stochastic particle swarm optimization algorithm and angular light scattering is used for the nonparametric estimation of aerosol nonsphericity variation with particle size,and the optimal sample selection method is employed to screen the data.Based on the verification of inversion accuracy,the variation of aerosol aspect ratio with particle size based on the ellipsoidal model in global regions has been obtained from Aerosol Robotic Network(AERONET)data,and the effect of nonsphericity on radiative forcing and dry deposition has been studied.The results show that the aspect ratio increases with particle size in all regions,with the maximum ranging from 1.4 to 1.8 in the desert,reflecting the differences in aerosol composition at different particle sizes.In radiation calculations,considering aerosol nonsphericity makes the aerosol cooling effect weaker and surface radiative fluxes increase,but hardly changes the aerosol absorption,with maximum differences of 9.22%and 22.12%at the bottom and top of the atmosphere,respectively.Meanwhile,the differences in radiative forcing between aspect ratios as a function of particle size and not varying with particle size are not significant,averaging less than 2%.Besides,the aspect ratio not varying with particle size underestimates the deposition velocity of small particles and overestimates that of large particles compared to that as a function of particle size,with maximum differences of 7%and 4%,respectively.
基金supported by the National Natural Science Foundation of China (No. 30670385)
文摘Dry deposition velocity of total suspended particles (TSP) is an effective parameter that describes the speed of atmospheric particulate matter deposit to the natural surface. It is also an important indicator to the capacity of atmosphere self-depuration. However, the spatial and temporal variations in dry deposition velocity of TSP at different urban landscapes and the relationship between dry deposition velocity and the meteorological parameters are subject to large uncertainties. We concurrently investigated this relationship at four different landscapes of Guangzhou, from October to December of 2009. The result of the average dry deposition velocity is (1.49 ± 0.77), (1.44 ± 0.77), (1.13 ±0.53) and (1.82± 0.82) cm/sec for urban commercial landscape, urban forest landscape, urban residential landscape and country landscape, respectively. This spatial variation can be explained by the difference of both particle size composition of TSP and meteorological parameters of sampling sites. Dry deposition velocity of TSP has a positive correlation with wind speed, and a negative correlation with temperature and relative humidity. Wind speed is the strongest factor that affects the magnitude of TSP dry deposition velocity, and the temperature is another considerable strong meteorological factor. We also find out that the relative humidity brings less impact, especially during the dry season. It is thus implied that the current global warming and urban heat island effect may lead to correlative changes in TSP dry deposition velocity, especially in the urban areas.
基金The study is supported by the National Natural Science Foundation of China,LASG and LAPC in IAP, CAS
文摘A new dry deposition velocity pattern (NDDVP) for the study of region-scale dry deposition processes is developed. The mean ratio between NDDVP and 1022 experimental data of dry deposi- tion velocity V_d is 1. 06±0.82. The result shows that NDDVP is well consistent with experimental data. Practical cases are forecasted by the high resolution regional acid deposition model (EM3) with both NDDVP and old V_d pattern. The maximum ratio between the central concentrations for SO4 can reach 2.4 only due to different V_d patterns. 3-D distributions of species concentrations and dry depositions forecasted by NDDVP are better than those by the old V_d pattern.
文摘The dry deposition process refers to the flux loss of an atmospheric pollutant due to uptake of the pollutant by the earth’s surfaces.Dry deposition flux of a chemical species is typically calculated as the product of its surface-layer concentration and its dry deposition velocity(V_(d)).Field measurement based V_(d) data are very scarce or do not exist for many chemical species considered in chemistry transport models.In the present study,gaseous and particulate dry deposition schemes were applied to generate a database of hourly V_(d) for 45 gaseous species and three particle size ranges for two years(2016–2017)at a 15 kmby 15 km horizontal resolution across North America.Hourly V_(d) of the 45 gaseous species ranged from<0.001 to 4.6 cm/sec across the whole domain,with chemical species-dependentmedian(mean)values being in the range of 0.018–1.37 cm/sec(0.05–1.43 cm/sec).The spatial distributions of the two-year average V_(d) showed values higher than 1–3 cm/sec for those soluble and reactive species over certain land types.Soluble species have the highest V_(d) over water surfaces,while insoluble but reactive species have the highest V_(d) over forests.Hourly V_(d) of PM_(2.5) across the whole domain ranged from 0.039 to 0.75 cm/sec with median(mean)value of 0.18(0.20)cm s^(−1),while the mean V_(d) for PM_(2.5)–10 is twice that of PM_(2.5).Uncertainties in the modeled V_(d) are typically on the order of a factor of 2.0 or larger,which needs to be considered when applying the dataset in other studies.
文摘Based on the regional acid deposition model(RADM),a high resolution model for species exchange in the troposphere(EM3)is designed.EM3 differs considerably in the following 5 aspects from RADM.First,the vertical grid levels in the planetary boundary layer(PBL)are increased.Second,layered vertical eddy diffusivity patterns in the troposphere(TL)are considered.Third,layered horizontal eddy diffusivity patterns within TL is used.Fourth,new dry deposition velocity pattern including the effect of plant canopy layer(CL)vertical structure is adopted.Fifth,advective scheme of second-order moment conservation with less numerical diffusion is used.OSCAR 4 case is comparatively simulated with both EM3 and RADM.The results show that 3-D distribution laws of chemical species in whole TL are forecasted by EM3 better than by RADM.Under the same conditions,all ratios of the central concentrations simulated with both models in lower PBL are more than 1.8,the maximum can be more than 3.