Based on the dynamics of ABS-equipped vehicles during cornering braking, the electronic brake- force distribution (EBD) control methods of ABS-equipped vehicles during cornering braking are proposed. According to th...Based on the dynamics of ABS-equipped vehicles during cornering braking, the electronic brake- force distribution (EBD) control methods of ABS-equipped vehicles during cornering braking are proposed. According to the dynamics and the tire model under tire adhesion limit, the stability acceptance criteria of vehicles during cornering braking are proposed. According to the stability acceptance criteria and the ABS control, the EBD control methods of ABS-equipped vehicles during cornering braking are implemented by adjusting the threshold values of tires slip independently. The vehicle states during cornering braking at two typical initial velocities of the vehicle are analyzed by the EBD control methods, whose results indicate the EBD control methods can improve the braking performances of the vehicle during cornering braking comparing with the ABS control.展开更多
In general,as the radio frequency(RF)power increases in a capacitively coupled plasma(CCP),the power transfer efficiency decreases because the resistance of the CCP decreases.In this work,a parallel resonance circuit ...In general,as the radio frequency(RF)power increases in a capacitively coupled plasma(CCP),the power transfer efficiency decreases because the resistance of the CCP decreases.In this work,a parallel resonance circuit is applied to improve the power transfer efficiency at high RF power,and the effect of the parallel resonance on the electron energy distribution function(EEDF)is investigated in a 60 MHz CCP.The CCP consists of a power feed line,the electrodes,and plasma.The reactance of the CCP is positive at 60 MHz and acts like an inductive load.A vacuum variable capacitor(VVC)is connected in parallel with the inductive load,and then the parallel resonance between the VVC and the inductive load can be achieved.As the capacitance of the VVC approaches the parallel resonance condition,the equivalent resistance of the parallel circuit is considerably larger than that without the VVC,and the current flowing through the matching network is greatly reduced.Therefore,the power transfer efficiency of the discharge is improved from 76%,70%,and 68%to 81%,77%,and 76%at RF powers of 100 W,150 W,and 200 W,respectively.At parallel resonance conditions,the electron heating in bulk plasma is enhanced,which cannot be achieved without the VVC even at the higher RF powers.This enhancement of electron heating results in the evolution of the shape of the EEDF from a biMaxwellian distribution to a distribution with the smaller temperature difference between high-energy electrons and low-energy electrons.Due to the parallel resonance effect,the electron density increases by approximately 4%,18%,and 21%at RF powers of 100 W,150 W,and 200 W,respectively.展开更多
This article presents the 2D simulation results of a nanosecond pulsed hollow cathode discharge obtained through a combination of fluid and kinetic models.The spatio-temporal evolution of the electron energy distribut...This article presents the 2D simulation results of a nanosecond pulsed hollow cathode discharge obtained through a combination of fluid and kinetic models.The spatio-temporal evolution of the electron energy distribution function(EEDF)of the plasma column and electrical characteristics of the nanosecond pulsed hollow cathode discharge at a gas pressure of 5 Torr are studied.The results show that the discharge development starts with the formation of an ionization front at the anode surface.The ionization front splits into two parts in the cathode cavity while propagating along its lateral surfaces.The ionization front formation leads to an increase in the fast isotropic EEDF component at its front,as well as in the anisotropic EEDF component.The accelerated electrons enter the cathode cavity,which significantly contributes to the formation of the highenergy EEDF component and EEDF anisotropy.展开更多
Ultrashort and powerful laser interactions with a target generate intense wideband electromagnetic pulses(EMPs).In this study,we report EMPs generated by the interactions between petawatt(30 fs,1.4×10^(20) W/cm^(...Ultrashort and powerful laser interactions with a target generate intense wideband electromagnetic pulses(EMPs).In this study,we report EMPs generated by the interactions between petawatt(30 fs,1.4×10^(20) W/cm^(2))femtosecond(fs)lasers with metal flat,plastic flat,and plastic nanowire-array(NWA)targets.Detailed analyses are conducted on the EMPs in terms of their spatial distribution,time and frequency domains,radiation energy,and protection.The results indicate that EMPs from metal targets exhibit larger amplitudes at varying angles than those generated by other types of targets and are enhanced significantly for NWA targets.Using a plastic target holder and increasing the laser focal spot can significantly decrease the radiation energy of the EMPs.Moreover,the composite shielding materials indicate an effective shielding effect against EMPs.The simulation results show that the NWA targets exert a collimating effect on thermal electrons,which directly affects the distribution of EMPs.This study provides guidance for regulating EMPs by controlling the laser focal spot,target parameters,and target rod material and is beneficial for electromagnetic-shielding design.展开更多
By calculating the energy distribution of electrons reaching the photocathode surface and solving the Schrodinger equation that describes the behavior of an electron tunneling through the surface potential barrier,we ...By calculating the energy distribution of electrons reaching the photocathode surface and solving the Schrodinger equation that describes the behavior of an electron tunneling through the surface potential barrier,we obtain an equation to calculate the emitted electron energy distribution of transmission-mode NEA GaAs photocathodes. Accord- ing to the equation,we study the effect of cathode surface potential barrier on the electron energy distribution and find a significant effect of the barrier-Ⅰ thickness or end height,especially the thickness,on the quantum efficiency of the cath- ode. Barrier Ⅱ has an effect on the electron energy spread, and an increase in the vacuum level will lead to a narrower electron energy spread while sacrificing a certain amount of cathode quantum efficiency. The equation is also used to fit the measured electron energy distribution curve of the transmission-mode cathode and the parameters of the surface barri- er are obtained from the fitting. The theoretical curve is in good agreement with the experimental curve.展开更多
Using the semiclassical ensemble model,the dependence of relative amplitude for the recollision dynamics in nonsequential double ionization(NSDI)of neon atom driven by the orthogonally polarized two-color field(OTC)la...Using the semiclassical ensemble model,the dependence of relative amplitude for the recollision dynamics in nonsequential double ionization(NSDI)of neon atom driven by the orthogonally polarized two-color field(OTC)laser field is theoretically studied.And the dynamics in two typical collision pathways,recollision-impact-ionization(RII)and recollisionexcitation with subsequent ionization(RESI),is systematically explored.Our results reveal that the V-shaped structure in the correlated momentum distribution is mainly caused by the RII mechanism when the relative amplitude of the OTC laser field is zero,and the first ionized electrons will quickly skim through the nucleus and share few energy with the second electron.As the relative amplitude increases,the V-shaped structure gradually disappears and electrons are concentrated on the diagonal in the electron correlation spectrum,indicating that the energy sharing after electrons collision is symmetric for OTC laser fields with large relative amplitudes.Our studies show that changing the relative amplitude of the OTC laser field can efficiently control the electron–electron collisions and energy exchange efficiency in the NSDI process.展开更多
The spatial distributions of the electron density and the mean electron energy of argon radio frequency (rf) glow discharge plasma in a plasma-enhanced chemical vapour deposition (PECVD) system have been investiga...The spatial distributions of the electron density and the mean electron energy of argon radio frequency (rf) glow discharge plasma in a plasma-enhanced chemical vapour deposition (PECVD) system have been investigated using an established movable Langmuir probe. The results indicate that in the axial direction the electron density tends to peak at midway between the two electrodes while the axial variation trend of mean electron energy is different from that of the electron density, the mean electron energy is high near the electrodes. And the mean electron energy near the cathode is much higher than that near the anode. This article focuses on the radial distribution of electron density and mean electron energy. A proposed theoretical model distribution agrees well with the experimental one: the electron density and the mean electron energy both increase from the centre of the glow to the edge of electrodes. This is useful for better understanding the discharge mechanism and searching for a better deposition condition to improve thin film quality.展开更多
Electron density plays an important role in determining the properties of functional materials.Revealing the electron density distribution experimentally in real space can help to tune the properties of materials.Spin...Electron density plays an important role in determining the properties of functional materials.Revealing the electron density distribution experimentally in real space can help to tune the properties of materials.Spinel Li Mn2 O4 is one of the most promising cathode candidates because of its high voltage,low cost,and non-toxicity,but suffers severe capacity fading during electrochemical cycling due to the Mn dissolution.Real-space measurement of electron distribution of Li Mn2 O4 experimentally can provide direct evaluation on the strength of Mn–O bond and give an explanation of the structure stability.Here,through high energy synchrotron powder x-ray diffraction(SPXRD),accurate electron density distribution in spinel Li Mn2 O4 has been investigated based on the multipole model.The electron accumulation between Mn and O atoms in deformation density map indicates the shared interaction of Mn–O bond.The quantitative topological analysis at bond critical points shows that the Mn–O bond is relatively weak covalent interaction due to the oxygen loss.These findings suggest that oxygen stoichiometry is the key factor for preventing the Mn dissolution and capacity fading.展开更多
Wave-particle interactions triggered by whistler-mode chorus waves are an important contributor to the Jovian radiation belt electron dynamics. While the sensitivity of chorus-driven electron scattering to the ambient...Wave-particle interactions triggered by whistler-mode chorus waves are an important contributor to the Jovian radiation belt electron dynamics. While the sensitivity of chorus-driven electron scattering to the ambient magnetospheric and wave parameters has been investigated, there is rather limited understanding regarding the extent to which the dynamic evolution of Jovian radiation belt electrons, under the impact of chorus wave scattering, depends on the electron distribution profiles. We adopt a group of reasonable initial conditions based upon the available observations and models for quantitative analyses. We find that inclusion of pitch angle variation in initial conditions can result in increased electron losses at lower pitch angles and substantially modify the pitch angle evolution profiles of > ~500 keV electrons, while variations of electron energy spectrum tend to modify the evolution primarily of 1 MeV and 5 MeV electrons. Our results explicitly demonstrate the importance to the radiation belt electron dynamics in the Jovian magnetosphere of the initial shape of the electron phase space density, and indicate the extent to which variations in electron energy spectrum and pitch angle distribution can contribute to the evolution of Jovian radiation belt electrons caused by chorus wave scattering.展开更多
In the present paper, we shall rigorously re-establish the result of the single-particle function of a quantum dot system at finite temperature. Unlike the proof given in our previous work (Phys. Rev. B 74 195414 (2...In the present paper, we shall rigorously re-establish the result of the single-particle function of a quantum dot system at finite temperature. Unlike the proof given in our previous work (Phys. Rev. B 74 195414 (2006)), we take a different approach, which does not exploit the explicit expression of the Gibbs distribution function. Instead, we only assume that the statistical distribution function of the quantum dot system is thermodynamically stable. As a result, we are able to show clearly that the electronic structure in the quantum dot system is completely determined by its thermodynamic stability. Furthermore, the weaker requirements on the statistical distribution function also make it possible to apply the same method to the quantum dot systems in non-equilibrium states.展开更多
Electron momentum distributions for 4a1 orbitals of serial freon molecules CFaC1, CF2Cl2, and CFCl3 (CFxC14-x, x=1-3) have been reanalyzed due to the severe discrepancies between theory and experiment in low momentu...Electron momentum distributions for 4a1 orbitals of serial freon molecules CFaC1, CF2Cl2, and CFCl3 (CFxC14-x, x=1-3) have been reanalyzed due to the severe discrepancies between theory and experiment in low momentum region. The tentative calculations using equilibrium geometries of molecular ions have exhibited a great improvement in agreement with the experimental data, which suggests that the molecular geometry distortion may be responsible for the observed high intensities at p〈0.5 a.u.. Further analyses show that the severe discrepancies at low momentum region mainly arise from the influence of molecular geometry distortion on C-Cl bonding electron density distributions.展开更多
The electron energy distribution function (EEDF) for a magnetically filtered dusty plasma is studied in a dusty double plasma device where the electron energy can be varied from 0.15 eV to ~ 2.8 eV and plasma densi...The electron energy distribution function (EEDF) for a magnetically filtered dusty plasma is studied in a dusty double plasma device where the electron energy can be varied from 0.15 eV to ~ 2.8 eV and plasma density from 10 6 cm-3 to 10 9cm-3 . The characteristics of EEDF for these ranges of plasma parameters are investigated in a pristine plasma as well as in a dusty plasma. The results show that in the presence of dust, there is a drastic modification in EEDF patterns in a plasma with higher electron temperature and density than those in a low temperature and low density plasma produced by the magnetic filter.展开更多
X-ray laser based on OFI is a promising way to realize the table-top X-ray laser.A simple model to describe the electron energy distribution in plasma produced by circularly polarized optical-field-induced ionization ...X-ray laser based on OFI is a promising way to realize the table-top X-ray laser.A simple model to describe the electron energy distribution in plasma produced by circularly polarized optical-field-induced ionization is constructed on the basis of ADK tunneling ionization theory.The ionization rate,threshold intensity,residual energy and electron energy distribution of Pd-like Xe system based on optical-field-induced ionization are calculated.The results are useful to further experments on X-ray laser of Pa-like Xe system.展开更多
In order to calculate the electron energy distribution in the fuel rod gap of a VVER- 1000 nuclear reactor, the Fokker-Planck equation (FPE) governing the non-equilibrium behavior of electrons passing through the fu...In order to calculate the electron energy distribution in the fuel rod gap of a VVER- 1000 nuclear reactor, the Fokker-Planck equation (FPE) governing the non-equilibrium behavior of electrons passing through the fuel-rod gap as an absorber has been solved in this paper. Besides, the Monte Carlo Geant4 code was employed to simulate the electron migration in the fuel-rod gap and the energy distribution of electrons was found. As for the results, the accuracy of the FPE was compared to the Geant4 code outcomes and a satisfactory agreement was found. Also, different percentage of the volatile and noble gas fission fragments produced in fission reactions in fuel rod, i.e. Krypton, Xenon, Iodine, Bromine, Rubidium and Cesium were employed so as to investigate their effects on the electrons' energy distribution. The present results show that most of the electrons in the fuel rod's gap were within the thermal energy limitation and the tail of the electron energy distribution was far from a Maxwellian distribution. The interesting outcome was that the electron energy distribution is slightly increased due to the accumulation of fission fragments in the gap. It should be noted that solving the FPE for the energy straggling electrons that are penetrating into the fuel-rod gap in the VVER-1000 nuclear reactor has been carried out for the first time using an analytical approach.展开更多
The distributions of traps and electron density in the interfaces between polyimide (PI) matrix and Al2O3 nanoparticles are researched using the isothermal decay current and the small-angle x-ray scattering (SAXS)...The distributions of traps and electron density in the interfaces between polyimide (PI) matrix and Al2O3 nanoparticles are researched using the isothermal decay current and the small-angle x-ray scattering (SAXS) tests. According to the electron density distribution for quasi two-phase mixture doped by spherical nanoparticles, the electron densities in the interfaces of PI/Al2O3 nanocomposite films are evaluated. The trap level density and carrier mobility in the interface are studied. The experimental results show that the distribution and the change rate of the electron density in the three layers of interface are different, indicating different trap distributions in the interface layers. There is a maximum trap level density in the second layer, where the maximum trap level density for the nanocomposite film doped by 25 wt% is 1.054 × 10^22 eV·m^-3 at 1.324eV, resulting in the carrier mobility reducing. In addition, both the thickness and the electron density of the nanocomposite film interface increase with the addition of the doped Al2O3 contents. Through the study on the trap level distribution in the interface, it is possible to further analyze the insulation mechanism and to improve the performance of nano-dielectric materials.展开更多
A conservative transport operator in space (v//,r) and moment equations are used to describe the combined effects of a stochastic magnetic field and a radial ambipolar electric field on the electrons. The transport o...A conservative transport operator in space (v//,r) and moment equations are used to describe the combined effects of a stochastic magnetic field and a radial ambipolar electric field on the electrons. The transport operator is coupled with Fokker-planck and Ohmic heating terms to compute the electron distribution function. A physical picture exhibits the possible importance of the turbulent magnetic field on the suprathermal electrons, which may be concerned with plasma confinement.展开更多
The relativistic and distorted wave effects are investigated for the electron momentum distributions of Xe 4d electrons.The theoretical results show good agreements with the experimental data measured previously with ...The relativistic and distorted wave effects are investigated for the electron momentum distributions of Xe 4d electrons.The theoretical results show good agreements with the experimental data measured previously with electron momentum spectroscopy. The distorted wave effect and the relativistic effect are found to play important roles in the low and high momentum regions, respectively.展开更多
Resonance lines are extensively used to diagnose electronic temperature Te and ions distribution. However, the analysis of the x-ray spectroscopy emitted from plasmas produced by a ns laser Jsually needs the help of a...Resonance lines are extensively used to diagnose electronic temperature Te and ions distribution. However, the analysis of the x-ray spectroscopy emitted from plasmas produced by a ns laser Jsually needs the help of a code or some assumptions. In this paper, a diagnostic idea of using line-pairs emitted from a doubly-excited state is proposed. By using the method presented in this paper, Te and the fractional population ratio of bare nuclei and H-like ions are directly obtained from the emission intensity ratios.展开更多
The numerical calculation of the energy distribution of electrons emitted by the tungsten, for a triangular barrier and given reflection images, has been carried out. It is shown that the numerical solution of Schrodi...The numerical calculation of the energy distribution of electrons emitted by the tungsten, for a triangular barrier and given reflection images, has been carried out. It is shown that the numerical solution of Schrodinger equation is the most effective method of calculation of the transparency of potential barrier among those used in work. I-V characteristics, which were calculated by the application of this method under different conditions, match the experimental data the best. The application of the numerical solution of Schrodinger equation for the calculation of transparency of the potential barrier enables the in-depth analysis of the tunnels phenomena and allows forecasting the effects which can not be received by application of Wentzel-Kramers-Brillouin approximation.展开更多
基金the National Natural Science Foundation of China (50122155)
文摘Based on the dynamics of ABS-equipped vehicles during cornering braking, the electronic brake- force distribution (EBD) control methods of ABS-equipped vehicles during cornering braking are proposed. According to the dynamics and the tire model under tire adhesion limit, the stability acceptance criteria of vehicles during cornering braking are proposed. According to the stability acceptance criteria and the ABS control, the EBD control methods of ABS-equipped vehicles during cornering braking are implemented by adjusting the threshold values of tires slip independently. The vehicle states during cornering braking at two typical initial velocities of the vehicle are analyzed by the EBD control methods, whose results indicate the EBD control methods can improve the braking performances of the vehicle during cornering braking comparing with the ABS control.
基金supported by the National Research Foundation of Korea(Nos.NRF-2019M1A7A1A03087579 and NRF-2021R1I1A1A01050312)the Ministry of Trade,Industry&Energy(Nos.20011226 and 20009415)。
文摘In general,as the radio frequency(RF)power increases in a capacitively coupled plasma(CCP),the power transfer efficiency decreases because the resistance of the CCP decreases.In this work,a parallel resonance circuit is applied to improve the power transfer efficiency at high RF power,and the effect of the parallel resonance on the electron energy distribution function(EEDF)is investigated in a 60 MHz CCP.The CCP consists of a power feed line,the electrodes,and plasma.The reactance of the CCP is positive at 60 MHz and acts like an inductive load.A vacuum variable capacitor(VVC)is connected in parallel with the inductive load,and then the parallel resonance between the VVC and the inductive load can be achieved.As the capacitance of the VVC approaches the parallel resonance condition,the equivalent resistance of the parallel circuit is considerably larger than that without the VVC,and the current flowing through the matching network is greatly reduced.Therefore,the power transfer efficiency of the discharge is improved from 76%,70%,and 68%to 81%,77%,and 76%at RF powers of 100 W,150 W,and 200 W,respectively.At parallel resonance conditions,the electron heating in bulk plasma is enhanced,which cannot be achieved without the VVC even at the higher RF powers.This enhancement of electron heating results in the evolution of the shape of the EEDF from a biMaxwellian distribution to a distribution with the smaller temperature difference between high-energy electrons and low-energy electrons.Due to the parallel resonance effect,the electron density increases by approximately 4%,18%,and 21%at RF powers of 100 W,150 W,and 200 W,respectively.
基金supported by the Russian Foundation for Basic Research(No.20–32–90150)by State Assignment(No.FZNZ–2020–0002)。
文摘This article presents the 2D simulation results of a nanosecond pulsed hollow cathode discharge obtained through a combination of fluid and kinetic models.The spatio-temporal evolution of the electron energy distribution function(EEDF)of the plasma column and electrical characteristics of the nanosecond pulsed hollow cathode discharge at a gas pressure of 5 Torr are studied.The results show that the discharge development starts with the formation of an ionization front at the anode surface.The ionization front splits into two parts in the cathode cavity while propagating along its lateral surfaces.The ionization front formation leads to an increase in the fast isotropic EEDF component at its front,as well as in the anisotropic EEDF component.The accelerated electrons enter the cathode cavity,which significantly contributes to the formation of the highenergy EEDF component and EEDF anisotropy.
基金This work was supported by the National Natural Science Foundation of China(Nos.12122501,11975037,61631001,and 11921006)the National Grand Instrument Project(Nos.2019YFF01014400,2019YFF01014404)the Foundation of Science and Technology on Plasma Physics Laboratory(No.6142A04220108).
文摘Ultrashort and powerful laser interactions with a target generate intense wideband electromagnetic pulses(EMPs).In this study,we report EMPs generated by the interactions between petawatt(30 fs,1.4×10^(20) W/cm^(2))femtosecond(fs)lasers with metal flat,plastic flat,and plastic nanowire-array(NWA)targets.Detailed analyses are conducted on the EMPs in terms of their spatial distribution,time and frequency domains,radiation energy,and protection.The results indicate that EMPs from metal targets exhibit larger amplitudes at varying angles than those generated by other types of targets and are enhanced significantly for NWA targets.Using a plastic target holder and increasing the laser focal spot can significantly decrease the radiation energy of the EMPs.Moreover,the composite shielding materials indicate an effective shielding effect against EMPs.The simulation results show that the NWA targets exert a collimating effect on thermal electrons,which directly affects the distribution of EMPs.This study provides guidance for regulating EMPs by controlling the laser focal spot,target parameters,and target rod material and is beneficial for electromagnetic-shielding design.
文摘By calculating the energy distribution of electrons reaching the photocathode surface and solving the Schrodinger equation that describes the behavior of an electron tunneling through the surface potential barrier,we obtain an equation to calculate the emitted electron energy distribution of transmission-mode NEA GaAs photocathodes. Accord- ing to the equation,we study the effect of cathode surface potential barrier on the electron energy distribution and find a significant effect of the barrier-Ⅰ thickness or end height,especially the thickness,on the quantum efficiency of the cath- ode. Barrier Ⅱ has an effect on the electron energy spread, and an increase in the vacuum level will lead to a narrower electron energy spread while sacrificing a certain amount of cathode quantum efficiency. The equation is also used to fit the measured electron energy distribution curve of the transmission-mode cathode and the parameters of the surface barri- er are obtained from the fitting. The theoretical curve is in good agreement with the experimental curve.
基金Project supported by the National Natural Science Foundation of China (Grant Nos.12204132 and 12304376)Excellent Youth Science Foundation of Shandong Province (Overseas) (Grant No.2022HWYQ-073)+1 种基金the Fundamental Research Funds for the Central Universities (Grant No.HIT.OCEF.2022042)Natural Science Foundation of Shandong Province (Grant No.ZR2023QA075)。
文摘Using the semiclassical ensemble model,the dependence of relative amplitude for the recollision dynamics in nonsequential double ionization(NSDI)of neon atom driven by the orthogonally polarized two-color field(OTC)laser field is theoretically studied.And the dynamics in two typical collision pathways,recollision-impact-ionization(RII)and recollisionexcitation with subsequent ionization(RESI),is systematically explored.Our results reveal that the V-shaped structure in the correlated momentum distribution is mainly caused by the RII mechanism when the relative amplitude of the OTC laser field is zero,and the first ionized electrons will quickly skim through the nucleus and share few energy with the second electron.As the relative amplitude increases,the V-shaped structure gradually disappears and electrons are concentrated on the diagonal in the electron correlation spectrum,indicating that the energy sharing after electrons collision is symmetric for OTC laser fields with large relative amplitudes.Our studies show that changing the relative amplitude of the OTC laser field can efficiently control the electron–electron collisions and energy exchange efficiency in the NSDI process.
文摘The spatial distributions of the electron density and the mean electron energy of argon radio frequency (rf) glow discharge plasma in a plasma-enhanced chemical vapour deposition (PECVD) system have been investigated using an established movable Langmuir probe. The results indicate that in the axial direction the electron density tends to peak at midway between the two electrodes while the axial variation trend of mean electron energy is different from that of the electron density, the mean electron energy is high near the electrodes. And the mean electron energy near the cathode is much higher than that near the anode. This article focuses on the radial distribution of electron density and mean electron energy. A proposed theoretical model distribution agrees well with the experimental one: the electron density and the mean electron energy both increase from the centre of the glow to the edge of electrodes. This is useful for better understanding the discharge mechanism and searching for a better deposition condition to improve thin film quality.
基金Beijing Natural Science Foundation,China(Grant No.Z190010)the National Key Research and Development Program of China(Grant No.2019YFA0308500)+2 种基金the Strategic Priority Research Program of Chinese Academy of Sciences(Grant No.XDB07030200)Key Research Projects of Frontier Science of Chinese Academy of Sciences(Grant No.QYZDB-SSW-JSC035)the National Natural Science Foundation of China(Grant Nos.51421002,51672307,51991344,52025025,and 52072400).
文摘Electron density plays an important role in determining the properties of functional materials.Revealing the electron density distribution experimentally in real space can help to tune the properties of materials.Spinel Li Mn2 O4 is one of the most promising cathode candidates because of its high voltage,low cost,and non-toxicity,but suffers severe capacity fading during electrochemical cycling due to the Mn dissolution.Real-space measurement of electron distribution of Li Mn2 O4 experimentally can provide direct evaluation on the strength of Mn–O bond and give an explanation of the structure stability.Here,through high energy synchrotron powder x-ray diffraction(SPXRD),accurate electron density distribution in spinel Li Mn2 O4 has been investigated based on the multipole model.The electron accumulation between Mn and O atoms in deformation density map indicates the shared interaction of Mn–O bond.The quantitative topological analysis at bond critical points shows that the Mn–O bond is relatively weak covalent interaction due to the oxygen loss.These findings suggest that oxygen stoichiometry is the key factor for preventing the Mn dissolution and capacity fading.
基金supported by NSFC grants (41674163) and (41474141)by the Hubei Province Natural Science ExcellentYouth Foundation (2016CFA044)the open-fund grant by the Lunar and Planetary Science Laboratory, Macao University of Science and Technology Partner Laboratory of Key Laboratory of Lunar and Deep Space Exploration, Chinese Academy of Sciences
文摘Wave-particle interactions triggered by whistler-mode chorus waves are an important contributor to the Jovian radiation belt electron dynamics. While the sensitivity of chorus-driven electron scattering to the ambient magnetospheric and wave parameters has been investigated, there is rather limited understanding regarding the extent to which the dynamic evolution of Jovian radiation belt electrons, under the impact of chorus wave scattering, depends on the electron distribution profiles. We adopt a group of reasonable initial conditions based upon the available observations and models for quantitative analyses. We find that inclusion of pitch angle variation in initial conditions can result in increased electron losses at lower pitch angles and substantially modify the pitch angle evolution profiles of > ~500 keV electrons, while variations of electron energy spectrum tend to modify the evolution primarily of 1 MeV and 5 MeV electrons. Our results explicitly demonstrate the importance to the radiation belt electron dynamics in the Jovian magnetosphere of the initial shape of the electron phase space density, and indicate the extent to which variations in electron energy spectrum and pitch angle distribution can contribute to the evolution of Jovian radiation belt electrons caused by chorus wave scattering.
基金Project supported by the National Science Foundation of China (Grant Nos. 10874003 and 11074004)the National Basic Research Program of China (Grant No. 2009CB939901)
文摘In the present paper, we shall rigorously re-establish the result of the single-particle function of a quantum dot system at finite temperature. Unlike the proof given in our previous work (Phys. Rev. B 74 195414 (2006)), we take a different approach, which does not exploit the explicit expression of the Gibbs distribution function. Instead, we only assume that the statistical distribution function of the quantum dot system is thermodynamically stable. As a result, we are able to show clearly that the electronic structure in the quantum dot system is completely determined by its thermodynamic stability. Furthermore, the weaker requirements on the statistical distribution function also make it possible to apply the same method to the quantum dot systems in non-equilibrium states.
基金V. ACKNOWLEDGMENTS This work was supported by the National Natural Science Foundation of China (No.10734040) and the Chinese Academy of Science Knowledge Promotion Project (No.KJCXI-YW-N30). The authors also gratefully acknowledge Professor C. E. Brion from University of British Columbia (UBC) in Canada for supplying the HEMS and RESFOLD programs.
文摘Electron momentum distributions for 4a1 orbitals of serial freon molecules CFaC1, CF2Cl2, and CFCl3 (CFxC14-x, x=1-3) have been reanalyzed due to the severe discrepancies between theory and experiment in low momentum region. The tentative calculations using equilibrium geometries of molecular ions have exhibited a great improvement in agreement with the experimental data, which suggests that the molecular geometry distortion may be responsible for the observed high intensities at p〈0.5 a.u.. Further analyses show that the severe discrepancies at low momentum region mainly arise from the influence of molecular geometry distortion on C-Cl bonding electron density distributions.
文摘The electron energy distribution function (EEDF) for a magnetically filtered dusty plasma is studied in a dusty double plasma device where the electron energy can be varied from 0.15 eV to ~ 2.8 eV and plasma density from 10 6 cm-3 to 10 9cm-3 . The characteristics of EEDF for these ranges of plasma parameters are investigated in a pristine plasma as well as in a dusty plasma. The results show that in the presence of dust, there is a drastic modification in EEDF patterns in a plasma with higher electron temperature and density than those in a low temperature and low density plasma produced by the magnetic filter.
基金the National Natural Science Foundation of China,the Fundamental Research Funds for the Central Universities,the Open Project of Beijing National Laboratory for Molecular Sciences,the Program for Innovative Research Team of Guizhou Province of China,the University Development Fund of Guizhou Province,the Talent Special Fund of Guizhou Province
基金Sponsored by the National Natural Science Foundation of China(Grant No.10774033)the Harbin Science and Technology Innovation Fund(Grant No.RC2007QN017030)+1 种基金the HIT Foundation(Grant No.HIT2003.05)the Program of Excellent Team in Harbin Institute of Technology
文摘X-ray laser based on OFI is a promising way to realize the table-top X-ray laser.A simple model to describe the electron energy distribution in plasma produced by circularly polarized optical-field-induced ionization is constructed on the basis of ADK tunneling ionization theory.The ionization rate,threshold intensity,residual energy and electron energy distribution of Pd-like Xe system based on optical-field-induced ionization are calculated.The results are useful to further experments on X-ray laser of Pa-like Xe system.
文摘In order to calculate the electron energy distribution in the fuel rod gap of a VVER- 1000 nuclear reactor, the Fokker-Planck equation (FPE) governing the non-equilibrium behavior of electrons passing through the fuel-rod gap as an absorber has been solved in this paper. Besides, the Monte Carlo Geant4 code was employed to simulate the electron migration in the fuel-rod gap and the energy distribution of electrons was found. As for the results, the accuracy of the FPE was compared to the Geant4 code outcomes and a satisfactory agreement was found. Also, different percentage of the volatile and noble gas fission fragments produced in fission reactions in fuel rod, i.e. Krypton, Xenon, Iodine, Bromine, Rubidium and Cesium were employed so as to investigate their effects on the electrons' energy distribution. The present results show that most of the electrons in the fuel rod's gap were within the thermal energy limitation and the tail of the electron energy distribution was far from a Maxwellian distribution. The interesting outcome was that the electron energy distribution is slightly increased due to the accumulation of fission fragments in the gap. It should be noted that solving the FPE for the energy straggling electrons that are penetrating into the fuel-rod gap in the VVER-1000 nuclear reactor has been carried out for the first time using an analytical approach.
基金Supported by the National Natural Science Foundation of China under Grant Nos 51337002,51077028,51502063 and 51307046the Foundation of Harbin Science and Technology Bureau of Heilongjiang Province under Grant No RC2014QN017034
文摘The distributions of traps and electron density in the interfaces between polyimide (PI) matrix and Al2O3 nanoparticles are researched using the isothermal decay current and the small-angle x-ray scattering (SAXS) tests. According to the electron density distribution for quasi two-phase mixture doped by spherical nanoparticles, the electron densities in the interfaces of PI/Al2O3 nanocomposite films are evaluated. The trap level density and carrier mobility in the interface are studied. The experimental results show that the distribution and the change rate of the electron density in the three layers of interface are different, indicating different trap distributions in the interface layers. There is a maximum trap level density in the second layer, where the maximum trap level density for the nanocomposite film doped by 25 wt% is 1.054 × 10^22 eV·m^-3 at 1.324eV, resulting in the carrier mobility reducing. In addition, both the thickness and the electron density of the nanocomposite film interface increase with the addition of the doped Al2O3 contents. Through the study on the trap level distribution in the interface, it is possible to further analyze the insulation mechanism and to improve the performance of nano-dielectric materials.
文摘A conservative transport operator in space (v//,r) and moment equations are used to describe the combined effects of a stochastic magnetic field and a radial ambipolar electric field on the electrons. The transport operator is coupled with Fokker-planck and Ohmic heating terms to compute the electron distribution function. A physical picture exhibits the possible importance of the turbulent magnetic field on the suprathermal electrons, which may be concerned with plasma confinement.
基金Project supported by the National Natural Science Foundation of China(Grant Nos.11327404 and U1432118)the Natural Science Research Programme of Education Department of Anhui Province,China(Grant Nos.KJ2013A260 and KJ2016A749)
文摘The relativistic and distorted wave effects are investigated for the electron momentum distributions of Xe 4d electrons.The theoretical results show good agreements with the experimental data measured previously with electron momentum spectroscopy. The distorted wave effect and the relativistic effect are found to play important roles in the low and high momentum regions, respectively.
文摘Resonance lines are extensively used to diagnose electronic temperature Te and ions distribution. However, the analysis of the x-ray spectroscopy emitted from plasmas produced by a ns laser Jsually needs the help of a code or some assumptions. In this paper, a diagnostic idea of using line-pairs emitted from a doubly-excited state is proposed. By using the method presented in this paper, Te and the fractional population ratio of bare nuclei and H-like ions are directly obtained from the emission intensity ratios.
文摘The numerical calculation of the energy distribution of electrons emitted by the tungsten, for a triangular barrier and given reflection images, has been carried out. It is shown that the numerical solution of Schrodinger equation is the most effective method of calculation of the transparency of potential barrier among those used in work. I-V characteristics, which were calculated by the application of this method under different conditions, match the experimental data the best. The application of the numerical solution of Schrodinger equation for the calculation of transparency of the potential barrier enables the in-depth analysis of the tunnels phenomena and allows forecasting the effects which can not be received by application of Wentzel-Kramers-Brillouin approximation.