A unified analysis is presented to calculate the incoherent spontaneous power of cooperative radiations based on self-amplified spontaneous emission. Using quantum mechanical tools, we derive analytical expressions fo...A unified analysis is presented to calculate the incoherent spontaneous power of cooperative radiations based on self-amplified spontaneous emission. Using quantum mechanical tools, we derive analytical expressions for the incoherent spontaneous power of undulator and Cherenkov free-electron lasers (FELs). The undulator and Cherenkov FELs are considered as two different examples for the radiation that accumulate cooperatively. In the case of the undulator FEL, we show an excellent agreement between an expression for the incoherent radiation power derived in the present work and that obtained using a completely different approach [Phys. Ftev. E 65 (2002) 026501]. For the Cherenkov radiation, we demonstrate a satisfactory agreement between the incoherent power predicted in our analysis and previous experimental results.展开更多
The requirements that a business needs to consider when building a wood panels manufacturing plant are much the same as they have been for decades, but today there is also the need for multiple environmental studies a...The requirements that a business needs to consider when building a wood panels manufacturing plant are much the same as they have been for decades, but today there is also the need for multiple environmental studies and permits. These are costly and time consuming additional expenses that often are the longest lead-time items on any project. Most industrialized countries have legislation in place to limit and control the negative impact that emission of pollutants may have on the environment. This paper discusses what is actually happening inside wood drying plants, and the prerequisite conditions for genesis of pyrolytic products relative to the operational parameters, such as choice of input raw materials, driers design and operational regime, choice of fuels for the heat generation and how these factors influence production of stack emission. The characterization of emission condensate by analytical methods is described, and survey of emission control system in use worldwide is described, and means of investigating what may be the optimum design for the control of emission is discussed. Alternate uses of utilizing the condensate, other than burning, are presented for consideration.展开更多
In this paper,acoustic emission(AE) and digital image correlation methods were applied to monitor interface cracking in thermal barrier coatings under compression.The interface failure process can be identifie via i...In this paper,acoustic emission(AE) and digital image correlation methods were applied to monitor interface cracking in thermal barrier coatings under compression.The interface failure process can be identifie via its AE features,including buckling,delamination incubation and spallation.According to the Fourier transformation of AE signals,there arefourdifferentfailuremodes:surfaceverticalcracks,opening and sliding interface cracks,and substrate deformation.The characteristic frequency of AE signals from surface vertical cracks is 0.21 MHz,whilst that of the two types of interface cracks are 0.43 and 0.29 MHz,respectively.The energy released of the two types of interface cracks are 0.43 and 0.29 MHz,respectively.Based on the energy released from cracking and the AE signals,a relationship is established between the interface crack length and AE parameters,which is in good agreement with experimental results.展开更多
On account of the background of China's "new normal" characterized by slower economic growth, this paper analyses the low-carbon economy status quo in the Beijing-Tianjin-Hebei region and empirically inv...On account of the background of China's "new normal" characterized by slower economic growth, this paper analyses the low-carbon economy status quo in the Beijing-Tianjin-Hebei region and empirically investigates the relationship between carbon dioxide(CO_2) emissions and its various factors for China's Beijing-Tianjin-Hebei region using panel data econometric technique. We find evidence of existence of Environmental Kuznets Curve. Results also show that economic scale, industrial structure, and urbanization rate are crucial factors to promote CO_2emissions. However, technological progress, especially the domestic independent research and development, plays a key role in C0_2 emissions abatement. Next, we further analyze the correlation between each subregion and various factors according to Grey Relation Analysis. Thereby,our findings provide important implications for policymakers in air pollution control and C0_2 emissions reduction for this region.展开更多
The aim of the work was the assessment of capability for the change control in the structure of a compact material of pelletized heatproof nickel alloy grade EP741NP using the atomic emission method. The proposed meth...The aim of the work was the assessment of capability for the change control in the structure of a compact material of pelletized heatproof nickel alloy grade EP741NP using the atomic emission method. The proposed method of evaluation is based on the statistical significance of the analytical response differences during atomic emission spectroscopy of solid specimens taken from one sample before and after heat treatment using the instruments AtomComp 81 and ARL 4460 with a high-voltage spark excitation. For calculations, the ratio of the line intensity of the analyzed element to the line intensity of the main sample component (in our case Ni<sub>2254</sub>) was used. The difference confidence estimation was made by the averages comparison method in a variance analysis. The study results are presented on the effect of material structure on analytical response during atomic emission spectroscopy of solid specimens. It was proved that the samples before and after heat treatment give statistically differing results while analyzed.展开更多
Synapses are essential units for the flow of information in the brain.Over the last 70 years,synapses have been widely studied in multiple animal models including worms,fruit flies,and rodents.In comparison,the study ...Synapses are essential units for the flow of information in the brain.Over the last 70 years,synapses have been widely studied in multiple animal models including worms,fruit flies,and rodents.In comparison,the study of human synapses has evolved significantly slower,mainly because of technical limitations.However,three novel methods allowing the analysis of molecular,morphological,and functional properties of human synapses may expand our knowledge of the human brain.Here,we briefly describe these methods,and evaluate how the information provided by each unique approach may contribute to the functional and anatomical analysis of the synaptic component of human brain circuitries.In particular,using tissue from cryopreserved human brains,synaptic plasticity can be studied in isolated synaptosomes by fluorescence analysis of single-synapse long-term potentiation(FASS-LTP),and subpopulations of synapses can be thoroughly assessed in the ribbons of brain tissue by array tomography(AT).Currently,it is also possible to quantify synaptic density in the living human brain by positron emission tomography(PET),using a novel synaptic radio-ligand.Overall,data provided by FASS-LTP,AT,and PET may significantly contribute to the global understanding of synaptic structure and function in both healthy and diseased human brains,thus directly impacting translational research.展开更多
The increasing demand for high-strength,corrosion-resistant magnesium alloys in transportation has led to the development of new processing techniques.In this work,cast and extruded ZK60 magnesium alloys were processe...The increasing demand for high-strength,corrosion-resistant magnesium alloys in transportation has led to the development of new processing techniques.In this work,cast and extruded ZK60 magnesium alloys were processed using the innovative solid-phase process,Friction Extrusion(FE).The microstructure was analyzed using Scanning Electron Microscopy(SEM),and Energy Dispersive Spectroscopy(EDS),showing a marked reduction in grain size,uniform solute distribution(Zn and Zr),and second phases after FE processing.Moreover,optical micrographs and Electron Backscatter Diffraction(EBSD)were employed to further evaluate the alloy microstructure.The corro-sion resistance and electrochemical behavior were analyzed using potentiodynamic polarization,Scanning Electrochemical Cell Impedance Microscopy(SECCIM),and atomic emission spectroelectrochemistry analysis(AESEC).Time evolution surface imaging and post-corrosion microstructures were also analyzed to support the understanding of underlying corrosion mechanisms.Corrosion initiation and propagation in FE-processed samples followed grain boundary patterns,differing from cast and extruded ZK60 behaviors.Electrochemical measurements and in-situ time-dependent optical imaging demonstrated that FE processing enhanced corrosion potential,reduced corrosion current,and increased cathodic activity.Additionally,FE processing reduced the disparity in pitting potential between cast and extruded samples,resulting in intermediate pitting potentials.Higher Mg and lower Zn dissolution was observed in the lower anodic currents for FE-processed samples.During aggravated anodic current cycles,Mg dissolution equalized,but the Zn/Mg dissolution ratio increased for FE-processed extruded samples,suggesting less cathodic activation and better resistance to further pitting.展开更多
The safety of rail is very important for the development of high speed railway, and it is necessary to investigate the features of inner cracks in rail. In order to obtain the features of Acoustic Emission (AE) sour...The safety of rail is very important for the development of high speed railway, and it is necessary to investigate the features of inner cracks in rail. In order to obtain the features of Acoustic Emission (AE) sources of inner cracks in rail, AE sources with different types, depths and propagation distances are examined for crack in rail. The finite element method is utilized to model the rail with cracks and the results of experiment demonstrate the effectiveness of this model. Wavelet transform and Rayleigh-Lamb equations are utilized to extract the features of crack AE sources. The results illustrate that the intensity ratio among AE modes can identify the AE source types and the AE sources with different frequencies in rail. There are uniform AE mode features existing in the AE signals from AE sources in rail web, however AE signals from AE sources in rail head and rail base have the complex and unstable AE modes. Different AE source types have the different propagation features in rail. It is helpful to understand the rail cracks and detect the rail cracks based on the AE technique.展开更多
The Large Sky-Area Multi-Object Spectroscopic Telescope (LAMOST) under construction by the National Astronomical Observatories will yield up to four thousand multi-fiber spectra of stars and galaxies per field. The pr...The Large Sky-Area Multi-Object Spectroscopic Telescope (LAMOST) under construction by the National Astronomical Observatories will yield up to four thousand multi-fiber spectra of stars and galaxies per field. The present series of papers describes the automated data-reduction pipeline currently being designed in order to cope with the anticipated flood of spectrographic data. In this preliminary paper, we present an automated method for estimating the continuum level, the positions of strong lines and the 4000 A break in galaxy spectra. In order to obtain detailed information on the continuum, we use a wavelet filter bank. After continuum fitting, our software searches for a 4000 A break and distinguishes between emission-line galaxies (ELGs) and non-ELGs according to whether the break is small or large. It then searches for strong lines and measures the intensities of emission lines and the equivalent widths of absorption lines. For non-ELGs, the absorption lines are identified automatically yielding redshift measurements.展开更多
Analyzing determinants that influence polychlorinated dibenzo-p-dioxin and polychlorinated dibenzofuran(PCDD/F) emissions is helpful for decision-makers to find effective and efficient ways to mitigate PCDD/F emissi...Analyzing determinants that influence polychlorinated dibenzo-p-dioxin and polychlorinated dibenzofuran(PCDD/F) emissions is helpful for decision-makers to find effective and efficient ways to mitigate PCDD/F emissions. The PCDD/F emissions and the contributions of the scale effect, structure effect and technology effect to emissions from eight main industrial sectors in2006, 2008 and 2010 in Shandong Province, were calculated in this article. Total PCDD/F emissions in Shandong increased by 52.8% in 2008(614.1 g I-TEQ) and 49.7% in 2010(601.8 g I-TEQ) based on 2006(401.9 g I-TEQ). According to the decomposition method, the largest influencing factor on PCDD/F emission changes was the composition effect(contributed 43.4%in 2008 and 120.6% in 2010 based on 2006), which was also an emission-increasing factor.In this case, the present industrial restructuring policy should be adjusted to control the proportion of production capacities with high emission factors, such as iron ore sintering and steelmaking and the secondary non-ferrous metal sector. The scale effect increased the emissions in 2008(contributed 21.9%) and decreased the emissions in 2010(contributed-28.0%). However, as a source control measure, the excess capacity control policy indeed had a significant role in emission reduction. The main reason for the technology effect(contributed 34.7% in 2008 and 7.4% in 2010 based on 2006) having an emission-increasing role was the weakness in implementing policies for restricting industries with outdated facilities. Some specific suggestions were proposed on PCDD/F reduction for local administrators at the end.展开更多
Research on carbon cycling has attracted attention from both scientists and policy-makers. Based on material flow analysis, this study systematically budgets the carbon inputs, outputs and balance from 1980 to 2013 fo...Research on carbon cycling has attracted attention from both scientists and policy-makers. Based on material flow analysis, this study systematically budgets the carbon inputs, outputs and balance from 1980 to 2013 for China's agro-ecosystem and its sub-systems, including agricultural land use, livestock breeding and rural life. The results show that from 1980 to 2013, both the carbon input and output were growing gradually, with the carbon input doubling from 1.6 Pg C/year in 1980 to 3.4 Pg C/year in 2013, while carbon output grew from 2.2 Pg C/year in 1980 to 3.8 Pg C/year in 2013. From 1980 to 2013, the crop production system in China has remained a carbon source, and the agricultural land uses were also almost all carbon sources instead of carbon sinks. As soil carbon stock plays a very important role in deciding the function of China's agro-ecosystem as a carbon sink or source, practices that can promote carbon storage and sequestration will be an essential component of low carbon agriculture development in China.展开更多
An environmentally friendly,low power consuming,sensitive and compact mercury analyzer was developed for the determination of mercury in water samples by integrating a thin film dielectric barrier discharge induced co...An environmentally friendly,low power consuming,sensitive and compact mercury analyzer was developed for the determination of mercury in water samples by integrating a thin film dielectric barrier discharge induced cold vapor reactor and a dielectric barrier discharge optical emission spectrometer into a small polymethyl methacrylate plate(10.5 cm length×8.0 cm width×1.2 cm height).Mercury cold vapor was generated when standard or sample solutions with or without formic acid were introduced to the reactor to form thin film liquid and exposed to microplasma irradiation and subsequently separated from the liquid phase for transport to the microplasma and detection of its atomic emission.Limits of detection of 0.20 μg L^-1 and 2.6 μg L^-1 were obtained for the proposed system using or not using formic acid,respectively.Compared to the conventional microplasma optical emission spectrometry used for mercury analysis,this system not only retains the good limit of detection amenable to the determination of mercury in real samples,but also reduces power consumption,eliminates the generation of hydrogen and avoids the use of toxic or unstable reductant.Method validation was demonstrated by analysis of a certified reference material of water sample and three real water samples with good spike recoveries(88-102%).展开更多
Emission characterization of particle number as well as particle mass from three diesel passenger cars equipped with diesel particulate filter(DPF), diesel oxidation catalyst(DOC)and exhaust gas recirculation(EGR...Emission characterization of particle number as well as particle mass from three diesel passenger cars equipped with diesel particulate filter(DPF), diesel oxidation catalyst(DOC)and exhaust gas recirculation(EGR) under the vehicle driving cycles and regulatory cycle.Total particle number emissions(PNEs) decreased gradually during speed-up of vehicle from 17.3 to 97.3 km/hr. As the average vehicle speed increases, the size-segregated peak of particle number concentration shifts to smaller size ranges of particles. The correlation analysis with various particulate components such as particle number concentration(PNC),ultrafine particle number concentration(UFPNC) and particulate matter(PM) mass was conducted to compare gaseous compounds(CO, CO2, HC and NOx). The UFPNC and PM were not only emitted highly in Seoul during severe traffic jam conditions, but also have good correlation with hydrocarbons and NOxinfluencing high potential on secondary aerosol generation. The effect of the dilution temperature on total PNC under the New European Driving Cycle(NEDC), was slightly higher than the dilution ratio. In addition, the nuclei mode(DP: ≤ 13 nm) was confirmed to be more sensitive to the dilution temperature rather than other particle size ranges. Comparison with particle composition between vehicle speed cycles and regulatory cycle showed that sulfate was slightly increased at regulatory cycle, while other components were relatively similar. During cold start test, semivolatile nucleation particles were increased due to effect of cold environment. Research on particle formation dependent on dilution conditions of diesel passenger cars under the NEDC is important to verify impact on vehicular traffic and secondary aerosol formation in Seoul.展开更多
基金Supported by the ASRT-INFN Joint Project between the Academy of Scientific Research and Technology in Egypt and INFN in Italy
文摘A unified analysis is presented to calculate the incoherent spontaneous power of cooperative radiations based on self-amplified spontaneous emission. Using quantum mechanical tools, we derive analytical expressions for the incoherent spontaneous power of undulator and Cherenkov free-electron lasers (FELs). The undulator and Cherenkov FELs are considered as two different examples for the radiation that accumulate cooperatively. In the case of the undulator FEL, we show an excellent agreement between an expression for the incoherent radiation power derived in the present work and that obtained using a completely different approach [Phys. Ftev. E 65 (2002) 026501]. For the Cherenkov radiation, we demonstrate a satisfactory agreement between the incoherent power predicted in our analysis and previous experimental results.
文摘The requirements that a business needs to consider when building a wood panels manufacturing plant are much the same as they have been for decades, but today there is also the need for multiple environmental studies and permits. These are costly and time consuming additional expenses that often are the longest lead-time items on any project. Most industrialized countries have legislation in place to limit and control the negative impact that emission of pollutants may have on the environment. This paper discusses what is actually happening inside wood drying plants, and the prerequisite conditions for genesis of pyrolytic products relative to the operational parameters, such as choice of input raw materials, driers design and operational regime, choice of fuels for the heat generation and how these factors influence production of stack emission. The characterization of emission condensate by analytical methods is described, and survey of emission control system in use worldwide is described, and means of investigating what may be the optimum design for the control of emission is discussed. Alternate uses of utilizing the condensate, other than burning, are presented for consideration.
基金supported by the National Natural Science Foundation of China (Grants 11472237,11002122,51172192,and 11272275)
文摘In this paper,acoustic emission(AE) and digital image correlation methods were applied to monitor interface cracking in thermal barrier coatings under compression.The interface failure process can be identifie via its AE features,including buckling,delamination incubation and spallation.According to the Fourier transformation of AE signals,there arefourdifferentfailuremodes:surfaceverticalcracks,opening and sliding interface cracks,and substrate deformation.The characteristic frequency of AE signals from surface vertical cracks is 0.21 MHz,whilst that of the two types of interface cracks are 0.43 and 0.29 MHz,respectively.The energy released of the two types of interface cracks are 0.43 and 0.29 MHz,respectively.Based on the energy released from cracking and the AE signals,a relationship is established between the interface crack length and AE parameters,which is in good agreement with experimental results.
基金supported by National Social Science Foundation Project of China-A study on the Long-term Mechanism and Policy of Promoting the Construction of Ecological Civilization with Green Technological Innovation in China:[Grant Number 14AJL017]
文摘On account of the background of China's "new normal" characterized by slower economic growth, this paper analyses the low-carbon economy status quo in the Beijing-Tianjin-Hebei region and empirically investigates the relationship between carbon dioxide(CO_2) emissions and its various factors for China's Beijing-Tianjin-Hebei region using panel data econometric technique. We find evidence of existence of Environmental Kuznets Curve. Results also show that economic scale, industrial structure, and urbanization rate are crucial factors to promote CO_2emissions. However, technological progress, especially the domestic independent research and development, plays a key role in C0_2 emissions abatement. Next, we further analyze the correlation between each subregion and various factors according to Grey Relation Analysis. Thereby,our findings provide important implications for policymakers in air pollution control and C0_2 emissions reduction for this region.
文摘The aim of the work was the assessment of capability for the change control in the structure of a compact material of pelletized heatproof nickel alloy grade EP741NP using the atomic emission method. The proposed method of evaluation is based on the statistical significance of the analytical response differences during atomic emission spectroscopy of solid specimens taken from one sample before and after heat treatment using the instruments AtomComp 81 and ARL 4460 with a high-voltage spark excitation. For calculations, the ratio of the line intensity of the analyzed element to the line intensity of the main sample component (in our case Ni<sub>2254</sub>) was used. The difference confidence estimation was made by the averages comparison method in a variance analysis. The study results are presented on the effect of material structure on analytical response during atomic emission spectroscopy of solid specimens. It was proved that the samples before and after heat treatment give statistically differing results while analyzed.
基金supported by National Institutes of Health Grants R21-AG048506,P01-AG000538 and RO1-AG34667(to CWC)UC MEXUS-CONACYT Grant CN-16-170(to GAP and CWC)
文摘Synapses are essential units for the flow of information in the brain.Over the last 70 years,synapses have been widely studied in multiple animal models including worms,fruit flies,and rodents.In comparison,the study of human synapses has evolved significantly slower,mainly because of technical limitations.However,three novel methods allowing the analysis of molecular,morphological,and functional properties of human synapses may expand our knowledge of the human brain.Here,we briefly describe these methods,and evaluate how the information provided by each unique approach may contribute to the functional and anatomical analysis of the synaptic component of human brain circuitries.In particular,using tissue from cryopreserved human brains,synaptic plasticity can be studied in isolated synaptosomes by fluorescence analysis of single-synapse long-term potentiation(FASS-LTP),and subpopulations of synapses can be thoroughly assessed in the ribbons of brain tissue by array tomography(AT).Currently,it is also possible to quantify synaptic density in the living human brain by positron emission tomography(PET),using a novel synaptic radio-ligand.Overall,data provided by FASS-LTP,AT,and PET may significantly contribute to the global understanding of synaptic structure and function in both healthy and diseased human brains,thus directly impacting translational research.
基金support of the U.S. Department of Energy, Vehicle Technologies Office (DOE/VTO)
文摘The increasing demand for high-strength,corrosion-resistant magnesium alloys in transportation has led to the development of new processing techniques.In this work,cast and extruded ZK60 magnesium alloys were processed using the innovative solid-phase process,Friction Extrusion(FE).The microstructure was analyzed using Scanning Electron Microscopy(SEM),and Energy Dispersive Spectroscopy(EDS),showing a marked reduction in grain size,uniform solute distribution(Zn and Zr),and second phases after FE processing.Moreover,optical micrographs and Electron Backscatter Diffraction(EBSD)were employed to further evaluate the alloy microstructure.The corro-sion resistance and electrochemical behavior were analyzed using potentiodynamic polarization,Scanning Electrochemical Cell Impedance Microscopy(SECCIM),and atomic emission spectroelectrochemistry analysis(AESEC).Time evolution surface imaging and post-corrosion microstructures were also analyzed to support the understanding of underlying corrosion mechanisms.Corrosion initiation and propagation in FE-processed samples followed grain boundary patterns,differing from cast and extruded ZK60 behaviors.Electrochemical measurements and in-situ time-dependent optical imaging demonstrated that FE processing enhanced corrosion potential,reduced corrosion current,and increased cathodic activity.Additionally,FE processing reduced the disparity in pitting potential between cast and extruded samples,resulting in intermediate pitting potentials.Higher Mg and lower Zn dissolution was observed in the lower anodic currents for FE-processed samples.During aggravated anodic current cycles,Mg dissolution equalized,but the Zn/Mg dissolution ratio increased for FE-processed extruded samples,suggesting less cathodic activation and better resistance to further pitting.
基金supported by the China Scholarship Council,the National Natural Science Foundation of China(61171197,61201307,61371045)the Innovation Funds of Harbin Institute of Technology(Grant IDGA18102011)the Promotive Research Fund for Excellent Young and Middle-Aged Scientisits of Shandong Province(BS2010DX001)
文摘The safety of rail is very important for the development of high speed railway, and it is necessary to investigate the features of inner cracks in rail. In order to obtain the features of Acoustic Emission (AE) sources of inner cracks in rail, AE sources with different types, depths and propagation distances are examined for crack in rail. The finite element method is utilized to model the rail with cracks and the results of experiment demonstrate the effectiveness of this model. Wavelet transform and Rayleigh-Lamb equations are utilized to extract the features of crack AE sources. The results illustrate that the intensity ratio among AE modes can identify the AE source types and the AE sources with different frequencies in rail. There are uniform AE mode features existing in the AE signals from AE sources in rail web, however AE signals from AE sources in rail head and rail base have the complex and unstable AE modes. Different AE source types have the different propagation features in rail. It is helpful to understand the rail cracks and detect the rail cracks based on the AE technique.
文摘The Large Sky-Area Multi-Object Spectroscopic Telescope (LAMOST) under construction by the National Astronomical Observatories will yield up to four thousand multi-fiber spectra of stars and galaxies per field. The present series of papers describes the automated data-reduction pipeline currently being designed in order to cope with the anticipated flood of spectrographic data. In this preliminary paper, we present an automated method for estimating the continuum level, the positions of strong lines and the 4000 A break in galaxy spectra. In order to obtain detailed information on the continuum, we use a wavelet filter bank. After continuum fitting, our software searches for a 4000 A break and distinguishes between emission-line galaxies (ELGs) and non-ELGs according to whether the break is small or large. It then searches for strong lines and measures the intensities of emission lines and the equivalent widths of absorption lines. For non-ELGs, the absorption lines are identified automatically yielding redshift measurements.
基金financed primarily by the International Science & Technology Cooperation Program of China (No. 2012DFA91150)the Chinese Academy of Sciences under Grant No. KZZD-EW-TZ-12the National Natural Science Foundation of China (No. 41371488, 41171394)
文摘Analyzing determinants that influence polychlorinated dibenzo-p-dioxin and polychlorinated dibenzofuran(PCDD/F) emissions is helpful for decision-makers to find effective and efficient ways to mitigate PCDD/F emissions. The PCDD/F emissions and the contributions of the scale effect, structure effect and technology effect to emissions from eight main industrial sectors in2006, 2008 and 2010 in Shandong Province, were calculated in this article. Total PCDD/F emissions in Shandong increased by 52.8% in 2008(614.1 g I-TEQ) and 49.7% in 2010(601.8 g I-TEQ) based on 2006(401.9 g I-TEQ). According to the decomposition method, the largest influencing factor on PCDD/F emission changes was the composition effect(contributed 43.4%in 2008 and 120.6% in 2010 based on 2006), which was also an emission-increasing factor.In this case, the present industrial restructuring policy should be adjusted to control the proportion of production capacities with high emission factors, such as iron ore sintering and steelmaking and the secondary non-ferrous metal sector. The scale effect increased the emissions in 2008(contributed 21.9%) and decreased the emissions in 2010(contributed-28.0%). However, as a source control measure, the excess capacity control policy indeed had a significant role in emission reduction. The main reason for the technology effect(contributed 34.7% in 2008 and 7.4% in 2010 based on 2006) having an emission-increasing role was the weakness in implementing policies for restricting industries with outdated facilities. Some specific suggestions were proposed on PCDD/F reduction for local administrators at the end.
基金supported by the National Science & Technology Pillar Program during the 12th Five-year Plan Period (No. 2013BAD11B03)the National Natural Science Foundation of China (Nos. 71573260,71273153,and 71525007)the Basic Scientific Research Fund (No. BSRF201311) for National Nonprofit Institutes from Ministry of Agriculture(MoA),China
文摘Research on carbon cycling has attracted attention from both scientists and policy-makers. Based on material flow analysis, this study systematically budgets the carbon inputs, outputs and balance from 1980 to 2013 for China's agro-ecosystem and its sub-systems, including agricultural land use, livestock breeding and rural life. The results show that from 1980 to 2013, both the carbon input and output were growing gradually, with the carbon input doubling from 1.6 Pg C/year in 1980 to 3.4 Pg C/year in 2013, while carbon output grew from 2.2 Pg C/year in 1980 to 3.8 Pg C/year in 2013. From 1980 to 2013, the crop production system in China has remained a carbon source, and the agricultural land uses were also almost all carbon sources instead of carbon sinks. As soil carbon stock plays a very important role in deciding the function of China's agro-ecosystem as a carbon sink or source, practices that can promote carbon storage and sequestration will be an essential component of low carbon agriculture development in China.
基金the National Natural Science Foundation of China(No.21575092)for financial support
文摘An environmentally friendly,low power consuming,sensitive and compact mercury analyzer was developed for the determination of mercury in water samples by integrating a thin film dielectric barrier discharge induced cold vapor reactor and a dielectric barrier discharge optical emission spectrometer into a small polymethyl methacrylate plate(10.5 cm length×8.0 cm width×1.2 cm height).Mercury cold vapor was generated when standard or sample solutions with or without formic acid were introduced to the reactor to form thin film liquid and exposed to microplasma irradiation and subsequently separated from the liquid phase for transport to the microplasma and detection of its atomic emission.Limits of detection of 0.20 μg L^-1 and 2.6 μg L^-1 were obtained for the proposed system using or not using formic acid,respectively.Compared to the conventional microplasma optical emission spectrometry used for mercury analysis,this system not only retains the good limit of detection amenable to the determination of mercury in real samples,but also reduces power consumption,eliminates the generation of hydrogen and avoids the use of toxic or unstable reductant.Method validation was demonstrated by analysis of a certified reference material of water sample and three real water samples with good spike recoveries(88-102%).
基金supported by Transportation Pollution Research Center,National Institute of Environmental Research in Republic of Korea
文摘Emission characterization of particle number as well as particle mass from three diesel passenger cars equipped with diesel particulate filter(DPF), diesel oxidation catalyst(DOC)and exhaust gas recirculation(EGR) under the vehicle driving cycles and regulatory cycle.Total particle number emissions(PNEs) decreased gradually during speed-up of vehicle from 17.3 to 97.3 km/hr. As the average vehicle speed increases, the size-segregated peak of particle number concentration shifts to smaller size ranges of particles. The correlation analysis with various particulate components such as particle number concentration(PNC),ultrafine particle number concentration(UFPNC) and particulate matter(PM) mass was conducted to compare gaseous compounds(CO, CO2, HC and NOx). The UFPNC and PM were not only emitted highly in Seoul during severe traffic jam conditions, but also have good correlation with hydrocarbons and NOxinfluencing high potential on secondary aerosol generation. The effect of the dilution temperature on total PNC under the New European Driving Cycle(NEDC), was slightly higher than the dilution ratio. In addition, the nuclei mode(DP: ≤ 13 nm) was confirmed to be more sensitive to the dilution temperature rather than other particle size ranges. Comparison with particle composition between vehicle speed cycles and regulatory cycle showed that sulfate was slightly increased at regulatory cycle, while other components were relatively similar. During cold start test, semivolatile nucleation particles were increased due to effect of cold environment. Research on particle formation dependent on dilution conditions of diesel passenger cars under the NEDC is important to verify impact on vehicular traffic and secondary aerosol formation in Seoul.