Emission Inventories of Carbon-containing Greenhouse Gases in China and Technological Measures for Their Abatement

The report summarizes surveys on carbon inventories and initiatives on sustainable carbon cycling taken by the Research Center for Eco-Environmental Sciences, where the authors work/worked. The first part of the report, which appeared in the preceding issue of this journal, deals with the concept of sustainable carbon cycling, the historic evolution of carbon cycling processes in China, carbon pool enhancement, value addition, carbon sequestration and carbon balance. This very paper, as the second part of the report, covers the results of carbon dynamics modeling, emission inventories of various carbon-containing greenhouse gases and their potential abatement measures.

Analysis of China's Production- and Consumption-Based CO_2 Emission Inventories

China, as the biggest GHG emitter and the largest developing country, has been urged by international society to take responsibilities for reducing GHG, especially in the post-Kyoto commitment period. Currently, the United Nations Framework Convention on Climate Change （UNFCCC） assigns the responsibility to parties who produce the pollution, using the production-based GHG emissions inventories. In this article, we analyze the difference between China＇s production- and consumption- based emission inventories and conclude that consumption-based GHG emission inventories are preferred; as it is fair that whoever consumes the emission should pay for their consumption. In addition, in order to consider environmental justice, policy-makers should take both economic and administrative measures to support poor provinces for reducing C02 emissions.

Anthropogenic Direct Radiative Forcing of Tropospheric Ozone and Aerosols in 1850 and 2000 Estimated with IPCC AR5 Emissions Inventories

This study estimates direct radiative forcing by tropospheric ozone and all aerosols between the years 1850 and 2000, using the new IPCC AR5 （the Intergovernmental Panel on Climate Change Fifth Assessment Report） emissions inventories and a fully coupled chemistry-aerosol general circulation model. As compared to the previous Global Emissions Inventory Activity （GEIA） data, that have been commonly used for forcing estimates since 1990, the IPCC AR5 emissions inventories report lower anthropogenic emissions of organic carbon and black carbon aerosols and higher sulfur and NOx emissions. The simulated global and annual mean burdens of sulfate, nitrate, black carbon （BC）, primary organic aerosol （POA）, secondary organic aerosol （SOA）, and ozone were 0.79, 0.35, 0.05, 0.49, 0.34, and 269 Tg, respectively, in the year 1850, and 1.90, 0.90, 0.11, 0.71, 0.32, and 377 Tg, respectively, in the year 2000. The estimated annual mean top of the atmosphere （TOA） direct radiative forcing of all anthropogenic aerosols based on the AR5 emissions inventories is -0.60 W m^-2 on a global mean basis from 1850 to 2000. However, this is -2.40 W m-2 when forcing values are averaged over eastern China （18-45°N and 95-125°E）. The value for tropospheric ozone is 0.17 W m^-1 on a global mean basis and 0.24 W m^-2 over eastern China. Forcing values indicate that the climatic effect of aerosols over eastern China is much more significant than the globally averaged effect.

Recent advances and perspectives towards emission inventories of mobile sources:Compilation approaches,data acquisition methods,and case studies

In recent years,great efforts have been devoted to reducing emissions from mobile sources with the dramatic growth of motor vehicle and nonroad mobile source populations.Compilation of a mobile source emission inventory is conducive to the analysis of pollution emission characteristics and the formulation of emission reduction policies.This study summarizes the latest compilation approaches and data acquisition methods for mobile source emission inventories.For motor vehicles,a high-resolution emission inventory can be developed based on a bottom-up approach with a refined traffic flow model and real-world speed-coupled emission factors.The top-down approach has advantages when dealing with macroscale vehicle emission estimation without substantial traffic flow infrastructure.For nonroad mobile sources,nonroad machinery,inland river ships,locomotives,and civil aviation aircraft,a top-down approach based on fuel consumption or power is adopted.For ocean-going ships,a bottom-up approach based on automatic identification system(AIS)data is adopted.Three typical cases are studied,including emission reduction potential,a cost-benefit model,and marine shipping emission control.Outlooks and suggestions are given on future research directions for emission inventories for mobile sources:building localized emission models and factor databases,improving the dynamic updating capability of emission inventories,establishing a database of emission factors of unconventional pollutants and greenhouse gas from mobile sources,and establishing an urban high temporalspatial resolution volatile organic compound(VOC)evaporation emission inventory.

Local PM_(10) and PM_(2.5) emission inventories from agricultural tillage and harvest in northeastern China

Mineral particles or particulate matters（PMs） emitted during agricultural activities are major recurring sources of atmospheric aerosol loading.However,precise PM inventory from agricultural tillage and harvest in agricultural regions is challenged by infrequent local emission factor（EF） measurements.To understand PM emissions from these practices in northeastern China,we measured EFs of PM_（10） and PM_（2.5） from three field operations（i.e.,tilling,planting and harvesting） in major crop production（i.e.,corn and soybean）,using portable real-time PM analyzers and weather station data.County-level PM_（10） and PM_（2.5） emissions from agricultural tillage and harvest were estimated,based on local EFs,crop areas and crop calendars.The EFs averaged（107 ± 27）,（17 ± 5） and 26 mg/m^2 for field tilling,planting and harvesting under relatively dry conditions（i.e.,soil moisture 〈15%）,respectively.The EFs of PM from field tillage and planting operations were negatively affected by topsoil moisture.The magnitude of PM_（10） and PM_（2.5） emissions from these three activities were estimated to be 35.1 and 9.8 kilotons/yr in northeastern China,respectively,of which Heilongjiang Province accounted for approximately45%.Spatiotemporal distribution showed that most PM_（10） emission occurred in April,May and October and were concentrated in the central regions of the northeastern plain,which is dominated by dryland crops.Further work is needed to estimate the contribution of agricultural dust emissions to regional air quality in northeastern China.

Development of National Greenhouse Gas Emissions Inventories in the Context of International Climate Negotiations

Based on the principle of common but differentiated responsibilities, the UNFCCC has different requirements on national GHG inventories submitted by Annex I and non-Annex I parties. Since 2007, the transparency of mitigation actions by developing countries, the submission frequency of national communications cored on national inventory and the relevant international consultation and analysis have become the key issues in climate negotiations. Relevant responsibilities of developing countries showed an increasing trend. Through the analysis of these different requirements, particularly on technical review system of national inventories on developed countries and of the current situation of China's inventory development, the challenges faced by China are identified and the corresponding countermeasures are also put forward, including improving institutional arrangements and statistic system, building country-specific and comprehensive database and preparing for time-series inventory development.

Atmospheric Emission Sources in the Po-Basin from the LIFE-IP PREPAIR Project

This paper presents the focus on emission estimates in the Italian Regions of the Po-basin obtained by the development of a common air pollutant emission dataset on the Po-basin and Slovenia foreseen in the project LIFE PREPAIR (https://www.lifeprepair.eu/). The objective is to update emission inventories developed by the environmental protection agencies and regions of Lombardy, Emilia-Romagna, Piedmont, Veneto, Friuli Venezia Giulia, Valle d’Aosta, the province of Bolzano (participating as stakeholder) and the province of Trento. A data flux is defined considering the activities on emission estimates by the different administrations according to the current Italian legislation. This activity has allowed the completion of two different datasets on the area for 2013 and 2017. The estimates of primary emissions of the main atmospheric pollutants have a high spatial resolution defined at the municipal level. The non-industrial combustion of biomass in small domestic appliances is the main source of primary PM10 in the Po-basin. NOx primary emissions are determined for quite of a half by road transport. Manure management and fertilization in the agriculture sector are the sources of NH3. The ensemble of the collected data shows a very good comparability even if all local compilers perform independently the estimates, thanks to a good alignment in using reference methodologies and to projects of common methodological development, as reported by the INEMAR project (https://www.inemar.eu/). The estimates of PM10, NOx and NH3 are comparable with data reported by the European Environment Agency EEA for the European Member States EU-28 (until 1 February 2020) and for Italy, reported under the UNECE Convention on Long-range Transboundary Air Pollution and European Union National Emission Ceiling Directive.

Estimation of vegetative mercury emissions in China

Vegetative mercury emissions were estimated within the framework of Biogenic Emission Inventory System (BEIS3 V3.11). In this estimation, the 19 categories of U.S. Geological Survey landcover data were incorporated to generate the vegetation-specific mercury emissions in a 81-km Lambert Conformal model grid covering the total Chinese continent. The surface temperature and cloud-corrected solar radiation from a Mesoscale Meteorological model (MM5) were retrieved and used for calculating the diurnal variation...

A biogenic volatile organic compounds emission inventory for Yunnan Province

The first detailed inventory for volatile organic compounds(VOC) emissions from vegetation over Yunnan Province, China was presented. The spatially and temporally resolved inventory was developed based on a geographic information system(GIS), remote sensing(RS) data and field measurement data, such as digitized land-use data, normalized difference vegetation index(NDVI) and temperature data from direct real-time measurement. The inventory has a spatial resolution of 5 km×5 km and a time resolution of 1 h. Urban, agriculture, and natural land-use distributions in Yunnan Province were combined with biomass factors for each land-use category to produce a spatially resolved biomass inventory. A biogenic emission inventory was developed by combining the biomass inventory with hourly emission rates for tree, shrub and ground cover species of the study area. Correcting for environmental factors, including light intensity and temperature, a value of 1.1×10 12 gC for total annual biogenic VOC emissions from Yunnan Province, including 6.1×10 11 gC for isoprene, 2.1×10 11 gC for monoterpenes, and 2.6×10 11 gC for OVOC was obtained. The highest VOC emissions occurred in the northwestern, southwestern and north region of Yunnan Province. Some uncertainties were also discussed in this study.

Air pollutants and greenhouse gases emission inventory for power plants in the Antarctic

Emissions of air pollutants and greenhouse gases into the atmosphere in Antarctica from power plants with diesel generators(the main sources of energy at Antarctic research stations and the main stationary sources of anthropogenic emissions in the Antarctic)were assessed.A bottom-up approach was used to compile an emission inventory for the Antarctic.This involved estimating emissions at various spatial levels by sequentially aggregating estimate emissions from point emission sources.This is the first time this approach has been proposed and used.Emissions of CO2,NOx,particulate matter(PM10),and CO in the modern period were estimated at the research station,geographic region,natural domain,biogeographic region,continent section,and whole continent scales.Yearly emissions are presented here,but the approach allows emissions at different averaging periods to be estimated.This means mean or maximum yearly,monthly,daily,or hourly emissions can be estimated.The estimates could be used to model pollutant transmission and dispersion,assess the impacts of pollutants,and develop emission forecasts for various scenarios.

Compilation of Emission Inventory of Air Pollution Sources in Beijing and Suggestions on Emission Reduction Policies

By establishing emission inventory of air pollution sources in Beijing,and classifying and compiling the pollutant types and corresponding pollution source data in more detail,it could provide the reference for studying causes of haze and related policy impact assessment in Beijing.In this paper,selecting relevant data published in the Beijing Statistical Yearbook,referring to emission coefficients in the technical guidelines for the preparation of various pollution sources,and combining characteristics of energy consumption in Beijing,emission inventory of air pollution sources in six parts is established:thermal power plant,industrial combustion source(by industry),technological process source(by product variety),motor vehicle,building construction and residents life,and the contribution rate of each part to air pollutants is given.Finally,policy suggestions for haze control in Beijing are put forward.

Comparison of the Anthropogenic Emission Inventory for CMIP6 Models with a Country-Level Inventory over China and the Simulations of the Aerosol Properties

Anthropogenic emission inventory for aerosols and reactive gases is crucial to the estimation of aerosol radiative forcing and climate effects.Here,the anthropogenic emission inventory for AerChemMIP,endorsed by CMIP6,is briefly introduced.The CMIP6 inventory is compared with a country-level inventory(i.e.,MEIC)over China from 1986 to 2015.Discrepancies are found in the yearly trends of the two inventories,especially after 2006.The yearly trends of the aerosol burdens simulated by CESM2 using the two inventories follow their emission trends and deviate after the mid-2000s,while the simulated aerosol optical depths(AODs)show similar trends.The difference between the simulated AODs is much smaller than the difference between model and observation.Although the simulated AODs agree with the MODIS satellite retrievals for country-wide average,the good agreement is an offset between the underestimation in eastern China and the overestimation in western China.Low-biased precursor gas of SO_(2),overly strong convergence of the wind field,overly strong dilution and transport by summer monsoon circulation,too much wet scavenging by precipitation,and overly weak aerosol swelling due to low-biased relative humidity are suggested to be responsible for the underestimated AOD in eastern China.This indicates that the influence of the emission inventory uncertainties on simulated aerosol properties can be overwhelmed by model biases of meteorology and aerosol processes.It is necessary for climate models to perform reasonably well in the dynamical,physical,and chemical processes that would influence aerosol simulations.

Inventory of unintentional POPs emission from anthropogenic sources in Antarctica

In spite of remote location and very limited human activities,Antarctica is affected by persistent organic pollutants(POPs).POPs investigation in Antarctica has a comparatively long history,but there are still large knowledge gaps in assessment of their emission into environment.In the paper the results of the first inventory of unintentional POPs emission from anthropogenic sources in Antarctica for modern period and preliminary estimate for the late 1980s are presented.Assessment of dioxin/furans(PCDD/Fs)emission in different media,as well as polychlorinated biphenyls(PCBs)and hexachlorobenzene(HCB)in air is based on methodology of emission factors and indicators of human activity.The following sources of POPs emission have been estimated:power generation and heating,waste incineration,mobile sources and open burning of waste(in the past).According to the data obtained,annual PCDD/Fs air emission for modern period comprises 60.74 mg toxic equivalent(TEQ),PCBs-5.09 mg TEQ,and HCB-457.6 mg.Additionally 2.5 mg TEQ of dioxin/furans is released to residues,so total PCDD/Fs emission is amounted 63.23 mg TEQ.Waste incineration makes the greatest contribution to POPs emission(96% of PCDD/Fs,98%of PCBs and 36% of HCB air emission).In late 1980s open burning of waste was the major source of POPs.Retrospective assessment shows that over a 30-year period air emissions of PCDD/Fs decreased about 13 times,PCBs-15 times and HCB-57 times,primarily due to the prohibition of open burning of waste in compliance with the Protocol on Environmental Protection to the Antarctic Treaty requirements.

Study on carbon emission in prefecture-level cities of china

The study on greenhouse gas inventory in urban China lags far behind the global level. The important factor that curbs the carbon inventory of cities of China is inventory methodology and scope. Given the insufficiency of Chinese cities carbon inventory, a system and accounting model （scopel＋ scope2） as well as principles and boundaries were proposed for China. The carbon emissions in scopel and scopel＋ scope2 were calculated in Chinese prefecture-level cities. The EDGAR dataset was used for the calculation of scopel carbon emissions in cities in China and the level of uncertainty was analyzed as well. The results showed that the direct carbon emission of cities in China was about 31.65% of China total emissions. The scopel＋ scope2 carbon emissions in cities of China were calculated based on the GIS and RS model. The results showed that the sum of direct （scopel） and indirect （scope2） carbon emissions of cities in China accounted for 38.80% of total China carbon emissions.

Develop an Air Emission Inventory for Potential Point Sources in Northern Key Economic Zone and Simulate Its Impacts on Air Quality in Hanoi City,Vietnam

The Northern Key Economic region of Vietnam is a dynamic economic center that is an important economic locomotive of the North and the whole of Vietnam.In this area,large industrial parks are concentrated,attracting many large FDI projects.Key industries:cement production,cars-motorcycles,electronics,...Economic development entails environmental problems.The industrial sector has been identified as the number one driving force driving the growth of Hanoi city and neighboring provinces.Therefore,industrial development is one of the main causes of environmental pollution.In addition,the growth rate of industry in neighboring provinces significantly affects the air quality in Hanoi city.Some factories in Vinh Phuc,Hung Yen,Bac Ninh and Hai Duong provinces have large sources of gas emissions,potentially affecting air quality around Hanoi city.Monitoring results show that air pollution in Hanoi city is mainly caused by dust pollution,especially PM2.5 superfine dust.This is a very harmful dust to health;it is necessary to determine the cause and control solution.Therefore,the objectives of this study are:(1)inventory of potential emissions sources for industrial activities in the northern key economic region around Hanoi;(2)Simulate air spread by AERMOD model to get an overall picture of the industrial impact of surrounding provinces in Hanoi city;(3)Propose solutions to manage air quality for the city in the coming time.Simulation results for pollutants with the highest concentration of NOx for 1 hour,24 hours and the average of the year is 7.94;1.02;0.222(μg/m3);of CO for 1 hour and 8 hours are 27.616;8.89(μg/m3);of SO2 for 1 hour,24 hours and the average of the year is 4.005;0.288;0.038(μg/m3);of PM2.5 for 1 hour,24 hours and the average of the year is 0.32;0.023;0.003(μg/m3);of PM10 in 1 hour,24 hours and year average are 1.03;0.074;0.098(μg/m3).

Estimates and Spatial Distribution of Emissions from Sugar Cane Bagasse Fired Thermal Power Plants in Brazil

Sugar cane bagasse is one of the largest fuels used for electricity generation in Brazil and its usage has continuously increased to supply the energy demand. This paper presents emission inventory based on power plants burning sugar cane bagasse. The inventory involves the spatial distribution and the estimated flows for the following major pollutants: nitrogen oxides (NOx), particulate material (PM), carbon dioxide (CO2) and total organic carbon (TOC). A total of 384 power plants were inventoried, representing a generated power of 9.9 GW, about 26% of the energy produced by thermal power plants sector. The plants are concentrated in two main poles: one of them in S?o Paulo State and nearby areas and the other one in coast of Brazilian Northeast. The limits proposed by the AP-42 Regulations of the US Environmental Protection Agency (USEPA) for the emission factors were applied. Additional emission factors identified in the scientific literature were also included in the analysis in order to assess the uncertainties associated to the estimative. The estimated emissions showed values in the range 16.0 - 20.5 Gg?year?1 for NOx, 18.0 - 267.0 Gg?year?1 for MP and 20.5 - 26.7 Tg?year?1 for CO2. The contribution of TOC showed a minor contribution around 10 - 20 Mg?year?1. PM showed to be the most representative pollutant emitted by the thermal plants burning sugar cane bagasse, but with a large range of uncertainty. There is a high level of uncertainty associated to the preparation of cane as well as the use of collectors to control particulate emissions. The adequate control over all stages could reduce the bagasse ash content in 90% or more.

赛德西港用于船舶减排的陆上可再生能源供电评估

Air pollution from shipping is becoming a critical issue,particularly in dense hub port cities.One proposed solution to minimize ship-based emissions at ports is the implementation of an Onshore Power Supply(OPS)system.OPS allows ships to shut off their auxiliary engines and instead connect to the port grid.While there have been numerous studies conducted on ports in Europe and the United States,little research has been done on Egyptian ports.Therefore,this paper aims to investigate the feasibility of implementing OPS at Port Said West Port in Egypt,aligning with Egypt Vision 2030’s goals for addressing climate change.The research primarily focuses on analyzing data collected from calling ships to generate socio-economic and cost-effectiveness analyses of OPS.To further enhance the environmental benefits of OPS,the paper proposes the use of solar energy as the OPS electricity source.The findings of the study revealed that by relying on the national grid,emissions can be reduced by 28%.Moreover,it is predicted that this reduction could reach 100%if electricity generation is solely based on solar energy.Additionally,the economic analysis demonstrates promising profitability,with a payback period of approximately two years.

Environmental damage costs from fossil electricity generation in China, 2000~2003

Electricity consumption increases rapidly with the rapid development of China. The environmental damage costs of electricity generation are very important for both policy analysis and the proper management of the environment. A method was developed in this work to estimate gross environmental damage costs according to emission inventory and environmental cost factors, and to extend the costs from provincial to national level with population density. In this paper, sulfur dioxide (SO2), nitrogen oxides (NOx), particulate matter less than 10 μm in diameter (PM10), and carbon dioxide (CO2) from fossil fired power plants over 6000 kW were selected as index pollutants to quantify the environmental costs of damages on human health and global warming. With the new developed method, environmental damage costs, caused by 3 types of fired power plants in 30 provinces and 6 economic sectors during the years 2000 to 2003, were evaluated and analyzed. It can be seen that the calculated total national environmental damage costs of electricity have rapidly increased from 94930.87×106 USD in 2000 to about 141041.39×106 USD in 2003, with an average annual growth rate of 14.11%. Environmental damage costs of SO2, NOx, PM10, and CO2 are 69475.69×106, 30079.29×106, 28931.84×106, and 12554.57×106 USD and account for 49.26%, 21.33%, 20.51%, and 8.90% of total environmental costs in fossil electricity generation, respectively. With regard to regional distribution, external costs caused by fossil electricity generation are mainly concentrated in the more populated and industrialized areas of China, i.e., the Eastern Central and Southeastern areas.

Determining an optimal control strategy for anthropogenic VOC emissions in China based on source emissions and reactivity

An evidence-based control strategy for emission reduction of VOC sources can effectively solve the regional PM2.5and O3compound pollution in China.We estimated the anthropogenic VOC emission inventory in China in 2018 and established a source profile database containing 129 sources based on localized detection and the latest research results.Then,the distribution of the ozone formation potential(OFP)and secondary organic aerosol formation potential(SOAFP)for emission sources was analyzed.Moreover,priority control routes for VOC emission sources were proposed for different periods.Anthropogenic VOC emissions in China reached 27,211.8 Gg in 2018,and small passenger cars,industrial protective coatings,biomass burning,heavy trucks,printing,asphalt paving,oil storage and transportation,coking,and oil refining were the main contributors.Industrial protective coatings,small passenger cars,and biomass burning all contributed significantly to OFP and SOAFP.Priority in emission reduction control should be given to industrial protective coatings,small passenger cars,heavy trucks,coking,printing,asphalt paving,chemical fibers,and basic organic chemical sources over the medium and long term in China.In addition,the priority control route for VOC emission sources should be adjusted according to the variations in VOC emission characteristics and regional differences,so as to obtain the maximum environmental benefits.

Inventory Research of Greenhouse Gas about Energy Sector Activities in Jiangsu Province and Analysis on Relevant Problems

The emission of greenhouse gas generated by energy activity had the maximum influence on total emission. We introduced research content and method of inventory for greenhouse gas generated by energy activity in Jiangsu in 2005 and 2010, and obtained finial results. According to the sum of green gas emission from various parts, greenhouse gas emission of energy activity in Jiangsu occupied 76% -79% of total emission in 2005 and 2010. Meanwhile, the problems encountering in preparation process of inventory were summed and deeply analyzed, such as data ob- taining and processing, inconsistent statistical channel and actual measurement of emission factor. Finally, some suggestions about carrying out provincial greenhouse gas inventory work of energy activity in the future were put forward.