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Carbon Emission Effects Driven by Evolution of Chinese Dietary Structure from 1987 to 2020 被引量:1
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作者 ZHU Yuanyuan ZHANG Yan ZHU Xiaohua 《Chinese Geographical Science》 SCIE CSCD 2024年第1期181-194,共14页
Exploring carbon emission effects based on the evolution of residents’ dietary structure to achieve the carbon neutrality goal and mitigate climate change is an important task.This study took China as the research ob... Exploring carbon emission effects based on the evolution of residents’ dietary structure to achieve the carbon neutrality goal and mitigate climate change is an important task.This study took China as the research object(data excluding Hong Kong,Macao and Taiwan) and used the carbon emission coefficient method to quantitatively measure the food carbon emissions from 1987–2020,then analyzed the carbon emission effects under the evolution of dietary structure.The results showed that during the study period,the Chinese dietary structure gradually changed to a high-carbon consumption pattern.The dietary structure of urban residents developed to a balanced one,while that of rural residents developed to a high-quality one.During the study period,the per capita food carbon emissions and total food consumption of Chinese showed an increasing trend.The per capita food carbon emissions of residents in urban and rural showed an overall upward trend.The total food carbon emissions in urban increased significantly,while that in rural increased first and then decreased.The influence of beef and mutton on carbon emissions is the highest in dietary structure.Compared with the balanced dietary pattern,the food carbon emissions of Chinese residents had not yet reached the peak,but were evolving to a high-carbon consumption pattern. 展开更多
关键词 dietary structure structural evolution carbon emission effects carbon neutrality China
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Poverty Reduction in China: Experiences and Measurement of Effects
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作者 Zhan Wang 《China Economist》 2024年第1期103-126,共24页
This study employs the generalized method of moments(GMM)and panel vector autoregression(PVAR)models for a multi-factor quantitative dissection of China’s poverty reduction process across multiple stages,using provin... This study employs the generalized method of moments(GMM)and panel vector autoregression(PVAR)models for a multi-factor quantitative dissection of China’s poverty reduction process across multiple stages,using provincial panel data from 2000 to 2019.According to our research,economic growth and social development are the key drivers of poverty reduction in China,but the trickle-down effect of economic growth is diminishing and marketization is having a lesser pro-poor effect.Public expenditure has failed to provide social protection and income redistribution benefits due to issues such as targeting error and elite capture.Increasing the efficiency of the poverty reduction system calls for adaptive adjustments.Finally,this study highlights China’s poverty reduction experiences and analyzes current challenges,which serve as inspiration for consolidating poverty-reduction achievements,combating relative poverty,and attaining countryside vitalization. 展开更多
关键词 Poverty reduction governance measurement of effects countryside vitalization common prosperity
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Clinical effects of nonconvulsive electrotherapy combined with mindfulness-based stress reduction and changes of serum inflammatory factors in depression
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作者 Zhi-Wen Gu Chun-Ping Zhang +1 位作者 Li-Ping Chen Xiong Huang 《World Journal of Psychiatry》 SCIE 2024年第5期653-660,共8页
BACKGROUND Depression is a common and serious psychological condition,which seriously affects individual well-being and functional ability.Traditional treatment methods include drug therapy and psychological counselin... BACKGROUND Depression is a common and serious psychological condition,which seriously affects individual well-being and functional ability.Traditional treatment methods include drug therapy and psychological counseling;however,these methods have different degrees of side effects and limitations.In recent years,nonconvulsive electrotherapy(NET)has attracted increasing attention as a noninvasive treatment method.However,the clinical efficacy and potential mechanism of NET on depression are still unclear.We hypothesized that NET has a positive clinical effect in the treatment of depression,and may have a regulatory effect on serum inflammatory factors during treatment.AIM To assess the effects of NET on depression and analyze changes in serum inflammatory factors.METHODS This retrospective study enrolled 140 patients undergoing treatment for depression between May 2017 and June 2022,the observation group that received a combination of mindfulness-based stress reduction(MBSR)and NET treatment(n=70)and the control group that only received MBSR therapy(n=70).The clinical effectiveness of the treatment was evaluated by assessing various factors,including the Hamilton Depression Scale(HAMD)-17,self-rating idea of suicide scale(SSIOS),Pittsburgh Sleep Quality Index(PSQI),and levels of serum inflammatory factors before and after 8 wk of treatment.The quality of life scores between the two groups were compared.Comparisons were made using t and χ^(2) tests.RESULTS After 8 wk of treatment,the observation group exhibited a 91.43%overall effectiveness rate which was higher than that of the control group which was 74.29%(64 vs 52,χ^(2)=7.241;P<0.05).The HAMD,SSIOS,and PSQI scores showed a significant decrease in both groups.Moreover,the observation group had lower scores than the control group(10.37±2.04 vs 14.02±2.16,t=10.280;1.67±0.28 vs 0.87±0.12,t=21.970;5.29±1.33 vs 7.94±1.35,t=11.700;P both<0.001).Additionally,there was a notable decrease in the IL-2,IL-1β,and IL-6 in both groups after treatment.Furthermore,the observation group exhibited superior serum inflammatory factors compared to the control group(70.12±10.32 vs 102.24±20.21,t=11.840;19.35±2.46 vs 22.27±2.13,t=7.508;32.25±4.6 vs 39.42±4.23,t=9.565;P both<0.001).Moreover,the observation group exhibited significantly improved quality of life scores compared to the control group(Social function:19.25±2.76 vs 16.23±2.34;Emotions:18.54±2.83 vs 12.28±2.16;Environment:18.49±2.48 vs 16.56±3.44;Physical health:19.53±2.39 vs 16.62±3.46;P both<0.001)after treatment.CONCLUSION MBSR combined with NET effectively alleviates depression,lowers inflammation(IL-2,IL-1β,and IL-6),reduces suicidal thoughts,enhances sleep,and improves the quality of life of individuals with depression. 展开更多
关键词 DEPRESSION Nonconvulsive electrotherapy Mindfulness-based stress reduction Serum inflammatory factors Clinical effect Hamilton Depression Scale
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Effect of Photovoltaic Power Generation on Carbon Dioxide Emission Reduction under Double Carbon Background
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作者 Zhao Xinrui Hao Lei +2 位作者 Wu Yiling Xu Hong Dong Jinxiang 《China Petroleum Processing & Petrochemical Technology》 SCIE CAS CSCD 2023年第4期151-163,共13页
Increasing the efficiency and proportion of photovoltaic power generation installations is one of the best ways to reduce both CO_(2) emissions and reliance on fossil-fuel-based power supplies.Solar energy is a clean ... Increasing the efficiency and proportion of photovoltaic power generation installations is one of the best ways to reduce both CO_(2) emissions and reliance on fossil-fuel-based power supplies.Solar energy is a clean and renewable power source with excellent potential for further development and utilization.In 2021,the global solar installed capacity was about 749.7 GW.Establishing correlations between solar power generation,standard coal equivalent,carbon sinks,and green sinks is crucial.However,there have been few reports about correlations between the efficiency of tracking solar photovoltaic panels and the above parameters.This paper calculates the increased power generation achievable through the use of tracking photovoltaic panels compared with traditional fixed panels and establishes relationships between power generation,standard coal equivalent,and carbon sinks,providing a basis for attempts to reduce reliance on carbon-based fuels.The calculations show that power generation efficiency can be improved by about 26.12%by enabling solar panels to track the sun's rays during the day and from season to season.Through the use of this improved technology,global CO_(2) emissions can be reduced by 183.63 Mt,and the standard coal equivalent can be reduced by 73.67 Mt yearly.Carbon capture is worth approximately EUR 15.48 billion,and carbon accounting analysis plays a vital role in carbon trading. 展开更多
关键词 photovoltaic power generation carbon accounting carbon sink emission reduction
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A cobalt(Ⅱ)porphyrin with a tethered imidazole for efficient oxygen reduction and evolution electrocatalysis 被引量:1
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作者 Xialiang Li Ping Li +10 位作者 Jindou Yang Lisi Xie Ni Wang Haitao Lei Chaochao Zhang Wei Zhang Yong-Min Lee Weiqiang Zhang Shunichi Fukuzumi Wonwoo Nam Rui Cao 《Journal of Energy Chemistry》 SCIE EI CAS CSCD 2023年第1期617-621,I0015,共6页
Electrocatalytic oxygen reduction and evolution reactions are involved in new energy conversion and storage technologies,such as various fuel cells and metal-air batteries and also water splitting devices[1,2].However... Electrocatalytic oxygen reduction and evolution reactions are involved in new energy conversion and storage technologies,such as various fuel cells and metal-air batteries and also water splitting devices[1,2].However,both reactions are very slow in kinetics,and thus catalysts are required[3,4]. 展开更多
关键词 Molecular electrocatalysis Cobalt porphyrin Axial ligand effect Oxygen reduction reaction Oxygen evolution reaction
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Effective groundwater level recovery from mining reduction: Case study of Baoding and Shijiazhuang Plain area 被引量:1
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作者 Tian Nan Chen Yue +4 位作者 Wen-geng Cao En-lin Mu Yang Ou Zhen-sheng Lin Wei Kang 《Journal of Groundwater Science and Engineering》 2023年第3期278-293,共16页
The effective recovery of water level is a crucial measure of the success of comprehensive groundwater over-exploitation management actions in North China.However,traditional evaluation method do not directly capture ... The effective recovery of water level is a crucial measure of the success of comprehensive groundwater over-exploitation management actions in North China.However,traditional evaluation method do not directly capture the relationship between mining and other equilibrium elements.This study presents an innovative evaluation method to assess the water level recovery resulting from mining reduction based on the relationship between variation in exploitation and recharge.Firstly,the recharge variability of source and sink terms for both the base year and evaluation year is calculated and the coefficient of recharge variationβis introduced,which is then used to calculate the effective mining reduction and solve the water level recovery value caused by the effective mining reduction,and finally the water level recovery contribution by mining reduction is calculated by combining with the actual volume of mining reduction in the evaluation area.This research focuses on Baoding and Shijiazhuang Plain area,which share similar hydrogeological conditions but vary in groundwater exploitation and utilization.As the effect of groundwater level recovery with mining reduction was evaluated in these two areas as case study.In 2018,the results showed an effective water level recovery of 0.17 m and 0.13 m in the shallow groundwater of Shijiazhuang and Baoding Plain areas,respectively.The contributions of recovery from mining reduction were 76%and 57.98%for these two areas,respectively.It was notable that the water level recovery was most prominent in the foothill plain regions.From the evaluation results,it is evident that water level recovery depends not only on the intensity of groundwater mining reduction,but also on its effectiveness.The value of water level recovery alone cannot accurately indicate the intensity of mining reduction,as recharge variation significantly influences water level changes.Therefore,in practice,it is crucial to comprehensively assess the impact of mining reduction on water level recovery by combining the coefficient of recharge variation with the contribution of water level recovery from mining reduction.This integrated approach provide a more reasonable and scientifically supported basis,offering essential data support for groundwater management and conservation.To improve the accuracy and reliability of evaluation results,future work will focus on the standardizing and normalizing raw data processing. 展开更多
关键词 Water level recovery Water balance effective mining reduction Coefficient of recharge variation Water level recovery contribution
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Pollutant emission reduction effect through effluent tax,concentration-based effluent standard,or both 被引量:2
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作者 Kunyu Niu Zhongshan Tian Jie Xue 《Chinese Journal of Population,Resources and Environment》 2016年第2期68-80,共13页
There are numerous studies comparing different kinds of environmental taxes and standards.However,forms of environmental standards focused by former researchers are usually quantitybased limits/standards(e.g.pounds pe... There are numerous studies comparing different kinds of environmental taxes and standards.However,forms of environmental standards focused by former researchers are usually quantitybased limits/standards(e.g.pounds per day or pounds per unit of output).Concentration-based emission standard(e.g.milligrams per liter of wastewater) as one important form of environmental standard has not been given much attention.In this article,comparable estimates of their probable effect on enterprise pollution reduction will be developed for concentrationbased effluent standards,effluent taxes,and a combination of both.A linear simulation model is used to clearly and obviously compare the effects of effluent taxes and concentration-based standards within the same figure.With one detailed application to the paper industry,some enlightenment and conclusions-as well as the general applicability of these principles-are then provided:Under the same effluent tax rate,enterprises,groups,and industries that are cleaner will reduce more pollutants than those that have higher pollutant abatement costs.It is recommended that effluent taxes are set by avoiding cutting it even at one stroke and considering the feasibility of pollution-reducing technology in various industries.It is necessary to reduce MAC of enterprises to better stimulate enterprises' or industries' emission reduction by preferential measures,such as high tax rate coordinated by speeding up the depreciation of environmental protection equipment. 展开更多
关键词 Concentration-based effluent standard effluent tax emission reduction effect(ere) marginal abatement cost(MAC)
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“Buckets effect”in the kinetics of electrocatalytic reactions 被引量:1
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作者 Haowen Cui Yan-Xia Chen 《Journal of Energy Chemistry》 SCIE EI CAS CSCD 2024年第2期388-396,I0010,共10页
In this study,we systematically investigated the effect of proton concentration on the kinetics of the oxygen reduction reaction(ORR)on Pt(111)in acidic solutions.Experimental results demonstrate a rectangular hyperbo... In this study,we systematically investigated the effect of proton concentration on the kinetics of the oxygen reduction reaction(ORR)on Pt(111)in acidic solutions.Experimental results demonstrate a rectangular hyperbolic relationship,i.e.,the ORR current excluding the effect of other variables increases with proton concentration and then tends to a constant value.We consider that this is caused by the limitation of ORR kinetics by the trace oxygen concentration in the solution,which determines the upper limit of ORR kinetics.A model of effective concentration is further proposed for rectangular hyperbolic relationships:when the reactant concentration is high enough to reach a critical saturation concentration,the effective reactant concentration will become a constant value.This could be due to the limited concentration of a certain reactant for reactions involving more than one reactant or the limited number of active sites available on the catalyst.Our study provides new insights into the kinetics of electrocatalytic reactions,and it is important for the proper evaluation of catalyst activity and the study of structureperformance relationships. 展开更多
关键词 Oxygen reduction reaction KINETICS Zero order Rectangular hyperbolic relationship pH effect
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Research on the effects of command-and-control and market-oriented policy tools on China's energy conservation and emissions reduction innovation 被引量:2
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作者 Qin Ye Shaoqing Dai Gang Zeng 《Chinese Journal of Population,Resources and Environment》 2018年第1期1-11,共11页
The impact of environmental regulation on technology innovation is a hot spot in current research where a large number of empirical studies are based on Porter Hypothesis(PH). However, there are still controversies in... The impact of environmental regulation on technology innovation is a hot spot in current research where a large number of empirical studies are based on Porter Hypothesis(PH). However, there are still controversies in academia about the establishment of "weak" and "narrow" versions of PH. Based on the panel data of application for patent of energy conservation and emission reduction(ECER) technology of Chinese city scale during 2008-2014, comprehensive energy price, pollutant emission, etc., mixed regression model and systematic generalized method of moments method were adopted, respectively,to study the impact of market-oriented and command-and-control policy tool on China's ECER technology innovation. The results show that the environmental regulation hindered the technological innovation in the immediate phase; however, it turned out to be positive in the first-lag phase. Hence, the establishment of "weak" PH is time-bounded. The command-and-control policy tool played a more positive role in promoting technological innovation in the first-lag phase than market-oriented policy tool. Therefore, "narrow" PH is not tenable. The reason is that the main participants of China's ECER technology innovation are state-owned companies and public institutions. Regionally speaking, the impact which command-and-control policy tool has on technological innovation at sight was nonsignificant in the eastern, the central, and the western regions of China whilst market-oriented policy tool had a negative effect. And market-oriented policy tool in the central region had strongest negative effect, which would diminish in the eastern region and become weakest in the western region. This was related to regional energy consumption level and the market economic vitality. 展开更多
关键词 Environmental regulation command-and-control policy tools market-oriented policy tools emissions reduction INNOVATION
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Spatial emission reduction effects of China’s carbon emissions trading:quasi-natural experiments and policy spillovers 被引量:2
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作者 Zhiguo Li Jie Wang 《Chinese Journal of Population,Resources and Environment》 2021年第3期246-255,共10页
Insufficient assessment of emission reduction effects still exists in the carbon emission rights trading system,a major environmental regulation measure in China.Based on the data from the carbon trading pilot coverin... Insufficient assessment of emission reduction effects still exists in the carbon emission rights trading system,a major environmental regulation measure in China.Based on the data from the carbon trading pilot covering the years from 2007 to 2017,this study combined the synthetic control method with dynamic spatial Durbin model to comprehensively evaluate the spatial emission reduction effects of carbon trading policies.The results showed that:①The carbon trading policies promoted carbon emission reductions in the pilot regions,among which Tianjin and Hubei responded significantly,and also helped to suppress carbon emissions in the neighboring areas.②Long-term emission reduction effect from carbon emissions trading became gradually significant,while the indirect emission reduction effect was relatively weaker.③In term of reducing carbon emissions,the economic development channel played a key role,but it had a threat to the promotion of carbon emissions in the surrounding areas.Energy consumption was the main obstacle to the growth of carbon emissions.④In the long run,technological progress tended to become the key to the effective implementation of potential emission reduction effects of carbon trading policies.Based on the above findings,we suggest that the construction of a national carbon trading market should be promoted,the balanced development and orderly advancement of regional carbon trading markets should be paid attention to,the coordinated development of green economy as well as knowledge and technology exchange and cooperation among regions should be strengthened to form a low carbon development model among regions. 展开更多
关键词 Carbon emissions trading Eemission reduction effect Synthetic control method Policy spillover
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Effect of steam spraying on a sintering bed on sinter quality and the emission of flue gas pollutants
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作者 QI Yilong WU Hongliang +3 位作者 YU Zhengwei LONG Hongming WU Zhiyong WANG Wen 《Baosteel Technical Research》 CAS 2023年第2期37-46,共10页
The technology for spraying a sintering bed and thus improving sinter quality indicators while reducing the emission of flue gas pollutants has recently become an important research topic.The impacts on sinter quality... The technology for spraying a sintering bed and thus improving sinter quality indicators while reducing the emission of flue gas pollutants has recently become an important research topic.The impacts on sinter quality and emissions when spraying the sintering surface with different amounts and flow rates of steam were investigated in this study.The sinter quality indicators were most effectively improved by spraying 180 g of steam flow continuously at a rate of 0.02 m^(3)/min for 15 min after ignition for 8 min.The optimal effect on emission reduction was obtained by spraying 90 g of steam flow continuously at a rate of 0.01 m^(3)/min for 15 min after ignition for 8 min. 展开更多
关键词 SINTERING steam spraying emission reduction flue gas pollutants
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Exploration on Key Technologies and Practical Paths for Carbon Emission Reduction in Food System
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作者 Zhenzhong BAI Yunhao LU Hongling WANG 《Agricultural Biotechnology》 CAS 2023年第2期96-104,共9页
On the basis of existing research,carbon emission reduction technologies in production,processing,packaging,transportation and storage of the food system were summarized,and their application effects were analyzed.In ... On the basis of existing research,carbon emission reduction technologies in production,processing,packaging,transportation and storage of the food system were summarized,and their application effects were analyzed.In view of the inherent inadequacy of carbon emission reduction technologies in Chinese food system,starting from carbon labeling technologies and ESG system of the food industry,the unsoundness of the carbon emission reduction evaluation system and the high cost of related technology promotion,countermeasures such as strengthening top-level design,encouraging and supporting the development of new carbon emission reduction technologies,and improving carbon emission reduction technology subsidies were proposed by drawing on domestic and international experiences. 展开更多
关键词 Food system Carbon emission reduction Key technology Practice path
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Carbon emissions reduction potentiality for railroad transportation based on life cycle assessment
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作者 Yintao Lu Tongtong Zhang +3 位作者 Shengming Qiu Xin Liu Xiaohua Yu Hong Yao 《High-Speed Railway》 2023年第3期195-203,共9页
This study addresses the comparative carbon emissions of different transportation modes within a unified evaluation framework,focusing on their carbon footprints from inception to disposal.Specifically,the entire life... This study addresses the comparative carbon emissions of different transportation modes within a unified evaluation framework,focusing on their carbon footprints from inception to disposal.Specifically,the entire life cycle carbon emissions of High-Speed Rail(HSR),battery electric vehicles,conventional internal combustion engine vehicles,battery electric buses,and conventional internal combustion engine buses are analyzed.The life cycle is segmented into vehicle manufacturing,fuel or electricity production,operational,and dismantlingrecycling stages.This analysis is applied to the Beijing-Tianjin intercity transportation system to explore emission reduction strategies.Results indicate that HSR demonstrates significant carbon emission reduction,with an intensity of only 24%-32% compared to private vehicles and 47%-89% compared to buses.Notably,HSR travel for Beijing-Tianjin intercity emits only 24% of private vehicle emissions,demonstrating the emission reduction benefits of transportation structure optimization.Additionally,predictive modeling reveals the potential for carbon emission reduction through energy structure optimization,providing a guideline for the development of effective transportation management systems. 展开更多
关键词 Life cycle assessment High-speed-rail Transportation structure Intercity transportation Carbon emission reduction potentiality
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Study on the Emission Reduction Effect of Environmental Protection Tax—An Empirical Study Based on the Change of Pollution Charge Standard in China? 被引量:2
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作者 Lixin Du Qian Zhou 《Journal of Geoscience and Environment Protection》 2022年第1期207-217,共11页
This paper reflects the actual effect of China’s environmental protection tax by empirically analyzing the environmental effect of the emission fee, in order to provide reference for China’s environmental tax reform... This paper reflects the actual effect of China’s environmental protection tax by empirically analyzing the environmental effect of the emission fee, in order to provide reference for China’s environmental tax reform. Based on the traditional environmental “Kuznets” model, the factor of environmental tax is added to verify the effect of environmental governance of environmental tax. The results show that: 1) the improvement of sulfur dioxide emission charge standard can effectively inhibit industrial sulfur dioxide emission, which verifies the existence of environmental effect of pollution levy policies</span><span style="font-family:"">.</span><span style="font-family:""> 2) The improvement of sewage charge standard has better inhibitory effect on sulfur dioxide emission per unit GDP than on sulfur dioxide emission</span><span style="font-family:"">.</span><span style="font-family:""> 3) There is regional heterogeneity in the “emission reduction” effect of sulfur dioxide emission charges in the eastern, central and western regions of China. Pollutants should be taxed differently according to regional differences</span><span style="font-family:"">.</span><span style="font-family:""> 4) Economic growth and sulfur dioxide emission show an inverted “U” shape, China is still in the stage before the inflection point of EKC. Economic growth still takes environmental damage as the cost, and the “emission reduction” effect of technological progress is not ideal, which reveals the urgency of increasing technological development in the field of green environmental protection under the current situation. 展开更多
关键词 Environmental Tax Environmental Kuznets Model emissions reduction Pollution Levy Policies
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Examining the Effects and Operational Mechanisms of Green Credit on Carbon Emissions in Chinese Regions
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作者 Qin Liu 《Proceedings of Business and Economic Studies》 2023年第5期38-48,共11页
The utilization of a green financial system,particularly through the implementation of green credit,plays a pivotal role in fostering environmentally sustainable,low-carbon economic growth and facilitating the transit... The utilization of a green financial system,particularly through the implementation of green credit,plays a pivotal role in fostering environmentally sustainable,low-carbon economic growth and facilitating the transition toward a more ecologically responsible economy.This paper employs a two-way fixed-effects model,utilizing provincial panel data spanning from 2012 to 2020,to investigate the influence of green credit on regional carbon emissions within different regions of China.The results reveal a significant reduction in carbon emissions as a consequence of the green credit program’s implementation.The analysis of the pathway indicates that green credit is instrumental in mitigating carbon emissions by instigating shifts in the energy mix,with evidence suggesting a partial mediating effect.Furthermore,a heterogeneity analysis discovered that the suppressive impact of green credit on carbon emissions is more pronounced in the eastern and western regions of China,while it is less significant in the central and northeastern areas.The implications of this study provide robust evidence in support of the role of green credit in reducing carbon emissions and can serve as a valuable resource for policymakers aiming to promote the expansion of green credit programs and,in turn,contribute to substantial reductions in carbon emissions. 展开更多
关键词 Carbon emission Green credit Intermediary effect
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Strong synergy between physical and chemical properties:Insight into optimization of atomically dispersed oxygen reduction catalysts
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作者 Yifan Zhang Linsheng Liu +4 位作者 Yuxuan Li Xueqin Mu Shichun Mu Suli Liu Zhihui Dai 《Journal of Energy Chemistry》 SCIE EI CAS CSCD 2024年第4期36-49,共14页
Atomically dispersed catalysts exhibit significant influence on facilitating the sluggish oxygen reduction reaction(ORR)kinetics with high atom economy,owing to remarkable attributes including nearly 100%atomic utiliz... Atomically dispersed catalysts exhibit significant influence on facilitating the sluggish oxygen reduction reaction(ORR)kinetics with high atom economy,owing to remarkable attributes including nearly 100%atomic utilization and exceptional catalytic functionality.Furthermore,accurately controlling atomic physical properties including spin,charge,orbital,and lattice degrees of atomically dispersed catalysts can realize the optimized chemical properties including maximum atom utilization efficiency,homogenous active centers,and satisfactory catalytic performance,but remains elusive.Here,through physical and chemical insight,we review and systematically summarize the strategies to optimize atomically dispersed ORR catalysts including adjusting the atomic coordination environment,adjacent electronic orbital and site density,and the choice of dual-atom sites.Then the emphasis is on the fundamental understanding of the correlation between the physical property and the catalytic behavior for atomically dispersed catalysts.Finally,an overview of the existing challenges and prospects to illustrate the current obstacles and potential opportunities for the advancement of atomically dispersed catalysts in the realm of electrocatalytic reactions is offered. 展开更多
关键词 Atomically dispersed catalysts Coordination environment Electronic orbitals Inter-site distance effect Oxygen reduction reaction
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Internal Polarization Field Induced Hydroxyl Spillover Effect for Industrial Water Splitting Electrolyzers
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作者 Jingyi Xie Fuli Wang +3 位作者 Yanan Zhou Yiwen Dong Yongming Chai Bin Dong 《Nano-Micro Letters》 SCIE EI CAS CSCD 2024年第2期438-449,共12页
The formation of multiple oxygen intermediates supporting efficient oxygen evolution reaction(OER)are affinitive with hydroxyl adsorption.However,ability of the catalyst to capture hydroxyl and maintain the continuous... The formation of multiple oxygen intermediates supporting efficient oxygen evolution reaction(OER)are affinitive with hydroxyl adsorption.However,ability of the catalyst to capture hydroxyl and maintain the continuous supply at active sits remains a tremendous challenge.Herein,an affordable Ni2P/FeP2 heterostructure is presented to form the internal polarization field(IPF),arising hydroxyl spillover(HOSo)during OER.Facilitated by IPF,the oriented HOSo from FeP2 to Ni2P can activate the Ni site with a new hydroxyl transmission channel and build the optimized reaction path of oxygen intermediates for lower adsorption energy,boosting the OER activity(242 mV vs.RHE at 100 mA cm-2)for least 100 h.More interestingly,for the anion exchange membrane water electrolyzer(AEMWE)with low concentration electrolyte,the advantage of HOSo effect is significantly amplified,delivering 1 A cm^(-2)at a low cell voltage of 1.88 V with excellent stability for over 50 h. 展开更多
关键词 Hydroxyl spillover effect Internal polarization field HETEROSTRUCTURE Oxygen reduction reaction Anion exchange membrane water electrolysis
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Competitive effect, but not competitive response, varies along a climatic gradient depending on tree species identity
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作者 Teresa Valor Lluís Coll +9 位作者 David I.Forrester Hans Pretzsch Miren del Río Kamil Bielak Bogdan Brzeziecki Franz Binder Torben Hilmers Zuzana Sitková Roberto Tognetti Aitor Ameztegui 《Forest Ecosystems》 SCIE CSCD 2024年第2期142-151,共10页
Background: Understanding the role of species identity in interactions among individuals is crucial for assessing the productivity and stability of mixed forests over time. However, there is limited knowledge concerni... Background: Understanding the role of species identity in interactions among individuals is crucial for assessing the productivity and stability of mixed forests over time. However, there is limited knowledge concerning the variation in competitive effect and response of different species along climatic gradients. In this study, we investigated the importance of climate, tree size, and competition on the growth of three tree species: spruce(Picea abies), fir(Abies alba), and beech(Fagus sylvatica), and examined their competitive response and effect along a climatic gradient.Methods: We selected 39 plots distributed across the European mountains with records of the position and growth of 5,759 individuals. For each target species, models relating tree growth to tree size, climate and competition were proposed. Competition was modelled using a neighbourhood competition index that considered the effects of inter-and intraspecific competition on target trees. Competitive responses and effects were related to climate.Likelihood methods and information theory were used to select the best model.Results: Our findings revealed that competition had a greater impact on target species growth than tree size or climate. Climate did influence the competitive effects of neighbouring species, but it did not affect the target species? response to competition. The strength of competitive effects varied along the gradient, contingent on the identity of the interacting species. When the target species exhibited an intermediate competitive effect relative to neighbouring species, both higher inter-than intraspecific competitive effects and competition reduction occurred along the gradient. Notably, species competitive effects were most pronounced when the target species' growth was at its peak and weakest when growing conditions were far from their maximum.Conclusions: Climate modulates the effects of competition from neighbouring trees on the target tree and not the susceptibility of the target tree to competition. The modelling approach should be useful in future research to expand our knowledge of how competition modulates forest communities across environmental gradients. 展开更多
关键词 Competition coefficient Competition reduction Interspecific competition Intraspecific competition Mixing effects Mixed species forest Neighbourhood models Plant-plant interactions
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Effect of urban symbiosis development in China on GHG emissions reduction 被引量:1
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作者 HUANG Wei GAO Qing-Xian +3 位作者 CAO Guo-liang MA Zhan-Yun ZHANG Wei-Ding CHAO Qing-Chen 《Advances in Climate Change Research》 SCIE CSCD 2016年第4期247-252,共6页
This paper analyzes current urban symbiosis development and application in China, and then conducts a statistical analysis of the emissions reduction of CO2 and CH_4 in relation to recovery of iron and steel scraps, w... This paper analyzes current urban symbiosis development and application in China, and then conducts a statistical analysis of the emissions reduction of CO2 and CH_4 in relation to recovery of iron and steel scraps, waste paper, and waste plastics from 2011 to 2014 using the greenhouse gas(GHG) emission inventory calculation method provided by the IPCC. Results indicate that the cumulative recovery of renewable resources during China's main urban symbiosis development in 2011e2014 was 803.275 Mt, and the amount of iron and steel scraps, waste paper, and waste plastic recovery was the largest, respectively accounting for 62.2%, 18.0%, and 8.2% of total recovery in 2014. In addition, the cumulative emissions reduction of GHGs in relation to recovery of iron and steel scraps, waste paper, and waste plastics in 2011e2014 was27.962 Mt CO_2-eq, 954.695 Mt CO_2-eq, and 22.502 Mt CO_2-eq, respectively, thereby totaling 1005.159 Mt CO_2-eq. Results show a remarkable GHG emissions reduction during 2011e2014. 展开更多
关键词 城市的共生 可更新的资源的恢复 GHG 排出物减小
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Are energy conservation and emission reduction policy measures effective for industrial structure restructuring and upgrading?
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作者 Guoxing Zhang Peide Zhang +1 位作者 Jing Xiu Jian Chai 《Chinese Journal of Population,Resources and Environment》 2018年第1期12-27,共16页
The use of energy conservation emission reduction policies to promote industrial restructuring and upgrading and thus facilitate energy conservation and emission reduction is one of the 10 important strategies of envi... The use of energy conservation emission reduction policies to promote industrial restructuring and upgrading and thus facilitate energy conservation and emission reduction is one of the 10 important strategies of environmental management in China. The use of energy conservation emission reduction policies to promote industrial restructuring and upgrading and thus facilitate energy conservation and emission reduction is one of the important strategies of environmental management in China. Based on the systematic collection of 1,195 energy conservation emission reduction policies, we discuss the influence of individual measure and measure synergy of energy conservation and emission reduction policies respectively. The results show that the energy conservation and emission reduction policies have a significant effect on the overall promotion of industrial upgrading. The financial measures and guidance measures have a positive impact;the financial measures and guidance measures have significantly positive effect; however, the administrative measures, fiscal tax measures, and other economic measures do the opposite; the positive effect of the synergy of guidance measures and financial measures is greater than the negative effect of considering only the synergy of fiscal tax measures and other economic measures, and significantly greater than the negative effect of the synergy of administrative measures, fiscal tax measures, and other economic measures. We should strengthen and emphasize the use of the measure that has positive effect on industrial structure restructuring and upgrading individually and synergistically. 展开更多
关键词 Energy conservation and emission reduction policy quantification measure synergy HAC unit rootcointegration
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