A three-way catalyst comprised novel oxygen storage components for emission control in natural gas powered engines was prepared. The addition of novel oxygen storage components to the Pd/γ-Al2O3 catalysts resulted ...A three-way catalyst comprised novel oxygen storage components for emission control in natural gas powered engines was prepared. The addition of novel oxygen storage components to the Pd/γ-Al2O3 catalysts resulted in improved activities of the fresh and aged catalyst by lowering the light-off temperature for methane in natural gas engines exhaust.展开更多
Energy efficiency and environmental impact have become dominant topics in internal combustion engines development. Among many strategies to improve power and emissions outputs from diesel engines is the partial mix of...Energy efficiency and environmental impact have become dominant topics in internal combustion engines development. Among many strategies to improve power and emissions outputs from diesel engines is the partial mix of hydrogen and air as fresh charge components to form extremely lean and homogenous mixture, which resist the spontaneous combustion, while diesel fuel is injected directly inside combustion chamber using the conventional fuel injection systems. This contribution presents an analytical and experimental investigation for the effects of adding hydrogen on diesel engines power output and the reduction of emissions. Parametric analysis is used based on lamped parameters modeling of intake manifold to estimate in cylinder trapped charge. The fuel energy flow to engine cylinders is compared for a range of loads and concentrations to simulate relevant case studies. Diesel fuel reduction for significant range of part-load operation can be achieved by introducing hydrogen, along with power improvement emission reductions are affected positively as well. This is achievable without compromising the engine maximum efficiency, given that most engines are operated at small and part-load during normal driving conditions, which allow for introducing more hydrogen instead of large quantities of excess air during such operation conditions that also can be further improved by charge boosting.展开更多
China has published a stricter emission standard for thermal power plants in order to help reduce the power industry's sulfur dioxide emissions by over six
According to statistics, the average dust collection efficiency of flue gas emission in the large and medium- sized power plants in Zhejiang Province at present has attained higher than 97% which surpasses the 95% sta...According to statistics, the average dust collection efficiency of flue gas emission in the large and medium- sized power plants in Zhejiang Province at present has attained higher than 97% which surpasses the 95% standard as stipulated by the Ministry of Electric Power. The dust collection efficiency of the Beilungang Power Plant has already attained 99.92%. In recent years, Zhejiang Electric Power Corporation has stipulated that all the newly constructed generating units shall be equipped with high efficiency electrostatic precipitator (ESP) while the existing power plants shall speed up their renovation work for their dust collectors. In combination with the fourth stage project of the Taizhou Power Plant, the improvement work of the dust展开更多
In response to the lack of global quantitative research on the potential and scale prediction of CO_(2) capture,utilization and storage(CCUS)in China under the background of carbon peak and carbon neutrality goals,thi...In response to the lack of global quantitative research on the potential and scale prediction of CO_(2) capture,utilization and storage(CCUS)in China under the background of carbon peak and carbon neutrality goals,this study predicts the future economic costs of different links of ccUS technologies and the carbon capture needs of different industries in the scenario of fossil energy continuation.Based on the CO_(2) utilization and storage potential and spatial distribution in China,a cost-scale calculation model for different regions in China in 206o is constructed to predict the whole-process economic cost and its corresponding scale potential of CCUs.The results show that a local+remote storage mode is preferred,together with a local utilization mode,to meet China's 27×10^(8)t/a CO_(2) emission reduction demand under the scenario of fossil energy continuation.Specifically,about 5×10^(8) t CO_(2) emission is reduced by capture utilization,and the whole-process cost is about-1400-200 RMB/t;about 22×10^(8) t CO_(2) emission is reduced by capture storage,and the whole-process cost is about 200-450 RMB/t.According to the model results,it is recommended to develop the chemical utilization industry based on P2X(Power to X,where X is raw material)technology,construct the CcUs industrial cluster,and explore a multi-party win-win cooperation mode.A scheme of national trunk pipeline network connecting areas connecting intensive emission reduction demand areas and target storage areas is suggested.The emission reduction cost of thermal power based on CCUS is calculated to be 0.16 RMB/(kW.h).展开更多
The Kubelka-Munk revised theory was adopted to derive the mix design theory of high solar reflectance and high emissivity coatings.When the concentration of each colorant is within 20%,and the width of the coating is ...The Kubelka-Munk revised theory was adopted to derive the mix design theory of high solar reflectance and high emissivity coatings.When the concentration of each colorant is within 20%,and the width of the coating is more than 200 μm,each colorant has enough covering power in visible and near-infrared spectral range.It can be assumed that the addition of colorants in coatings can only change the solar spectral absorption ratio rather than solar spectral scattering coefficient.The spectral scattering coefficient of coatings tends to a constant.The spectral absorption-scattering property of each colorant can be characterized through one parameter.The spectral absorption-scattering coefficient of coatings can be calculated with the multivariate linear relationship of each pigment.Moreover,the results can be expanded for high solar reflectivity and high long-wave emissivity coating preparation.The accuracy of Kubelka-Munk revised theory has been tested and verified through comparison between the calculated value and tested value of coating reflectance.展开更多
Feedback is said to exist in any amplifier when the fraction of output power in fed back as an input.Similarly,in gaseous discharge ions that incident on the cathode act as a natural feedback element to stabilize and ...Feedback is said to exist in any amplifier when the fraction of output power in fed back as an input.Similarly,in gaseous discharge ions that incident on the cathode act as a natural feedback element to stabilize and self sustain the discharge.The present investigation is intended to emphasize the feedback nature of ions that emits secondary electrons(SEs)from the cathode surface in DC gas discharges.The average number of SEs emitted per incident ion and non ionic species(energetic neutrals,metastables and photons)which results from ion is defined as effective secondary electronemission coefficient(ESEEC,Eg).In this study,we derive an analytic expression that corroborates the relation betweenEg and power influx by ion to the cathode based on the feedback theory of an amplifier.In addition,experimentally,we confirmed the typical positive feedback nature of SEEfrom the cathode in argon DC glow discharges.The experiment is done for three different cathode material of same dimension(tungsten(W),copper(Cu)and brass)under identical discharge conditions(pressure:0.45 mbar,cathode bias:-600 V,discharge gab:15 cm and operating gas:argon).Further,we found that theEg value of these cathode material controls the amount of feedback power given by ions.The difference in feedback leads different final output i.e the power carried by ion at cathode(Pi C¢∣).The experimentally obtained value of Pi C¢∣is 4.28 W,6.87 W and9.26 W respectively for W,Cu and brass.In addition,the present investigation reveals that the amount of feedback power in a DC gas discharges not only affect the fraction of power fed back to the cathode but also the entire characteristics of the discharge.展开更多
Prticle-in-cell(PIC) simulations demonstrated that,when the relativistic magnetron with diffraction output(MDO) is applied with a 410 kV voltage pulse,or when the relativistic magnetron with radial output is appli...Prticle-in-cell(PIC) simulations demonstrated that,when the relativistic magnetron with diffraction output(MDO) is applied with a 410 kV voltage pulse,or when the relativistic magnetron with radial output is applied with a 350 kV voltage pulse,electrons emitted from the cathode with high energy will strike the anode block wall.The emitted secondary electrons and backscattered electrons affect the interaction between electrons and RF fields induced by the operating modes,which decreases the output power in the radial output relativistic magnetron by about 15%(10%for the axial output relativistic magnetron),decreases the anode current by about 5%(5%for the axial output relativistic magnetron),and leads to a decrease of electronic efficiency by 8%(6%for the axial output relativistic magnetron).The peak value of the current formed by secondary and backscattered current equals nearly half of the amplitude of the anode current,which may help the growth of parasitic modes when the applied magnetic field is near the critical magnetic field separating neighboring modes.Thus,mode competition becomes more serious.展开更多
With one-and two-dimensional particle-in-cell(PIC)codes,we simulate the generation of high power terahertz(THz)emission from the interaction of ultrashort intense lasers with tenuous plasma and gas targets.By driving ...With one-and two-dimensional particle-in-cell(PIC)codes,we simulate the generation of high power terahertz(THz)emission from the interaction of ultrashort intense lasers with tenuous plasma and gas targets.By driving high-amplitude electron plasma waves either with a laser wakefield or the beatwave of two laser pulses,powerful THz electromagnetic pulses can be produced by linear mode conversion in inhomogeneous plasma or by the transient current induced at the surfaces of a thin plasma layer of few plasma wavelengths.Even with incident lasers at moderate intensity such as 1017W/cm2,the produced emission can be at the level of tens of MW in power and capable of affording field strengths of a few MV/cm,suitable for the studies of THz nonlinear physics.With field ionization included in the PIC codes,THz emission from laser interaction with tenuous gas targets is simulated.It is found that the transient transverse current formed during the ionization processes is responsible for the THz emission.With this mechanism,onemay also obtain THz fields ofMV/cm at lower laser intensity as compared with the schemes of plasma-wave excitation.展开更多
Concern over the health effects of fine particles in the ambient environment led the U.S. Environmental Protection Agency to develop the first standard for PM2.5 (particulate matter less than 2.5 μm) in 1997. The P...Concern over the health effects of fine particles in the ambient environment led the U.S. Environmental Protection Agency to develop the first standard for PM2.5 (particulate matter less than 2.5 μm) in 1997. The Particle Technology Laboratory at the University of Minnesota has helped to establish the PM2.5 standard by developing many instruments and samplers to perform atmospheric measurements. In this paper, we review various aspects of PM2.5, including its measurement, source apportionment, visibility and health effects, and mitigation. We focus on PM2.s studies in China and where appropriate, compare them with those obtained in the U.S. Based on accurate PM2.5 sampling, chemical analysis, and source apportionment models, the major PM2.5 sources in China have been identified to be coal combustion, motor vehicle emissions, and industrial sources. Atmospheric visibility has been found to correlate well with PM2.s concentration. Sulfate, ammonium, and nitrate carried by PM2.s, commonly found in coal burning and vehicle emissions, are the dominant contributors to regional haze in China. Short-term exposure to PM2.s is strongly associated with the increased risk of morbidity and mortality from cardiovascular and respiratory diseases in China. The strategy for PMzs mitigation must be based on reducing the pollutants from the two primary sources of coal-fired power plants and vehicle emissions. Although conventional Particulate Emission Control Devices (PECD) such as electrostatic precipitators in Chinese coal-fired power plants are generally effective for large particles, most of them may not have high collection efficiency of PM2.5. Baghouse filtration is gradually incorporated into the PECD to increase the PM2.5 collection efficiency. By adopting stringent vehicle emissions standard such as Euro 5 and 6, the emissions from vehicles can be gradually reduced over the years. An integrative approach, from collaboration among academia, government, and industries, can effectively manage and mitigate the PM2.s pollution in China.展开更多
基金the National Natural Science Foundation of China(No:20273043)the Ministry of Education of China for providing financial support for this project
文摘A three-way catalyst comprised novel oxygen storage components for emission control in natural gas powered engines was prepared. The addition of novel oxygen storage components to the Pd/γ-Al2O3 catalysts resulted in improved activities of the fresh and aged catalyst by lowering the light-off temperature for methane in natural gas engines exhaust.
文摘Energy efficiency and environmental impact have become dominant topics in internal combustion engines development. Among many strategies to improve power and emissions outputs from diesel engines is the partial mix of hydrogen and air as fresh charge components to form extremely lean and homogenous mixture, which resist the spontaneous combustion, while diesel fuel is injected directly inside combustion chamber using the conventional fuel injection systems. This contribution presents an analytical and experimental investigation for the effects of adding hydrogen on diesel engines power output and the reduction of emissions. Parametric analysis is used based on lamped parameters modeling of intake manifold to estimate in cylinder trapped charge. The fuel energy flow to engine cylinders is compared for a range of loads and concentrations to simulate relevant case studies. Diesel fuel reduction for significant range of part-load operation can be achieved by introducing hydrogen, along with power improvement emission reductions are affected positively as well. This is achievable without compromising the engine maximum efficiency, given that most engines are operated at small and part-load during normal driving conditions, which allow for introducing more hydrogen instead of large quantities of excess air during such operation conditions that also can be further improved by charge boosting.
文摘China has published a stricter emission standard for thermal power plants in order to help reduce the power industry's sulfur dioxide emissions by over six
文摘According to statistics, the average dust collection efficiency of flue gas emission in the large and medium- sized power plants in Zhejiang Province at present has attained higher than 97% which surpasses the 95% standard as stipulated by the Ministry of Electric Power. The dust collection efficiency of the Beilungang Power Plant has already attained 99.92%. In recent years, Zhejiang Electric Power Corporation has stipulated that all the newly constructed generating units shall be equipped with high efficiency electrostatic precipitator (ESP) while the existing power plants shall speed up their renovation work for their dust collectors. In combination with the fourth stage project of the Taizhou Power Plant, the improvement work of the dust
基金Supported by the National Natural Science Foundation of China(72140006)GEIDCO Independent Research Project(ZY2023008).
文摘In response to the lack of global quantitative research on the potential and scale prediction of CO_(2) capture,utilization and storage(CCUS)in China under the background of carbon peak and carbon neutrality goals,this study predicts the future economic costs of different links of ccUS technologies and the carbon capture needs of different industries in the scenario of fossil energy continuation.Based on the CO_(2) utilization and storage potential and spatial distribution in China,a cost-scale calculation model for different regions in China in 206o is constructed to predict the whole-process economic cost and its corresponding scale potential of CCUs.The results show that a local+remote storage mode is preferred,together with a local utilization mode,to meet China's 27×10^(8)t/a CO_(2) emission reduction demand under the scenario of fossil energy continuation.Specifically,about 5×10^(8) t CO_(2) emission is reduced by capture utilization,and the whole-process cost is about-1400-200 RMB/t;about 22×10^(8) t CO_(2) emission is reduced by capture storage,and the whole-process cost is about 200-450 RMB/t.According to the model results,it is recommended to develop the chemical utilization industry based on P2X(Power to X,where X is raw material)technology,construct the CcUs industrial cluster,and explore a multi-party win-win cooperation mode.A scheme of national trunk pipeline network connecting areas connecting intensive emission reduction demand areas and target storage areas is suggested.The emission reduction cost of thermal power based on CCUS is calculated to be 0.16 RMB/(kW.h).
基金Supported by the 12th Five-year National Science and Technology Support Plan(No.2011BAE27B04)the Natural Science Foundation of China(No.51378391)the China Scholarship Council(award to HE Yan for studying in the University of Toronto)
文摘The Kubelka-Munk revised theory was adopted to derive the mix design theory of high solar reflectance and high emissivity coatings.When the concentration of each colorant is within 20%,and the width of the coating is more than 200 μm,each colorant has enough covering power in visible and near-infrared spectral range.It can be assumed that the addition of colorants in coatings can only change the solar spectral absorption ratio rather than solar spectral scattering coefficient.The spectral scattering coefficient of coatings tends to a constant.The spectral absorption-scattering property of each colorant can be characterized through one parameter.The spectral absorption-scattering coefficient of coatings can be calculated with the multivariate linear relationship of each pigment.Moreover,the results can be expanded for high solar reflectivity and high long-wave emissivity coating preparation.The accuracy of Kubelka-Munk revised theory has been tested and verified through comparison between the calculated value and tested value of coating reflectance.
文摘Feedback is said to exist in any amplifier when the fraction of output power in fed back as an input.Similarly,in gaseous discharge ions that incident on the cathode act as a natural feedback element to stabilize and self sustain the discharge.The present investigation is intended to emphasize the feedback nature of ions that emits secondary electrons(SEs)from the cathode surface in DC gas discharges.The average number of SEs emitted per incident ion and non ionic species(energetic neutrals,metastables and photons)which results from ion is defined as effective secondary electronemission coefficient(ESEEC,Eg).In this study,we derive an analytic expression that corroborates the relation betweenEg and power influx by ion to the cathode based on the feedback theory of an amplifier.In addition,experimentally,we confirmed the typical positive feedback nature of SEEfrom the cathode in argon DC glow discharges.The experiment is done for three different cathode material of same dimension(tungsten(W),copper(Cu)and brass)under identical discharge conditions(pressure:0.45 mbar,cathode bias:-600 V,discharge gab:15 cm and operating gas:argon).Further,we found that theEg value of these cathode material controls the amount of feedback power given by ions.The difference in feedback leads different final output i.e the power carried by ion at cathode(Pi C¢∣).The experimentally obtained value of Pi C¢∣is 4.28 W,6.87 W and9.26 W respectively for W,Cu and brass.In addition,the present investigation reveals that the amount of feedback power in a DC gas discharges not only affect the fraction of power fed back to the cathode but also the entire characteristics of the discharge.
基金supported by National Natural Science Foundation of China(No.61302010)the Foundation of Science and Technology on High Power Microwave Laboratory,Central University Foundation(2013KW07)Work at the University of New Mexico in USA was supportedby ONR Grant N00014-13-1-0565
文摘Prticle-in-cell(PIC) simulations demonstrated that,when the relativistic magnetron with diffraction output(MDO) is applied with a 410 kV voltage pulse,or when the relativistic magnetron with radial output is applied with a 350 kV voltage pulse,electrons emitted from the cathode with high energy will strike the anode block wall.The emitted secondary electrons and backscattered electrons affect the interaction between electrons and RF fields induced by the operating modes,which decreases the output power in the radial output relativistic magnetron by about 15%(10%for the axial output relativistic magnetron),decreases the anode current by about 5%(5%for the axial output relativistic magnetron),and leads to a decrease of electronic efficiency by 8%(6%for the axial output relativistic magnetron).The peak value of the current formed by secondary and backscattered current equals nearly half of the amplitude of the anode current,which may help the growth of parasitic modes when the applied magnetic field is near the critical magnetic field separating neighboring modes.Thus,mode competition becomes more serious.
基金This workwas supported in part by theNationalNatural Science Foundation of China(Grants No.10425416,10335020,10674175,60621063)the National High-Tech ICF Committee in China,and the National Basic Research Program of China(Grant No.2007CB310406).
文摘With one-and two-dimensional particle-in-cell(PIC)codes,we simulate the generation of high power terahertz(THz)emission from the interaction of ultrashort intense lasers with tenuous plasma and gas targets.By driving high-amplitude electron plasma waves either with a laser wakefield or the beatwave of two laser pulses,powerful THz electromagnetic pulses can be produced by linear mode conversion in inhomogeneous plasma or by the transient current induced at the surfaces of a thin plasma layer of few plasma wavelengths.Even with incident lasers at moderate intensity such as 1017W/cm2,the produced emission can be at the level of tens of MW in power and capable of affording field strengths of a few MV/cm,suitable for the studies of THz nonlinear physics.With field ionization included in the PIC codes,THz emission from laser interaction with tenuous gas targets is simulated.It is found that the transient transverse current formed during the ionization processes is responsible for the THz emission.With this mechanism,onemay also obtain THz fields ofMV/cm at lower laser intensity as compared with the schemes of plasma-wave excitation.
文摘Concern over the health effects of fine particles in the ambient environment led the U.S. Environmental Protection Agency to develop the first standard for PM2.5 (particulate matter less than 2.5 μm) in 1997. The Particle Technology Laboratory at the University of Minnesota has helped to establish the PM2.5 standard by developing many instruments and samplers to perform atmospheric measurements. In this paper, we review various aspects of PM2.5, including its measurement, source apportionment, visibility and health effects, and mitigation. We focus on PM2.s studies in China and where appropriate, compare them with those obtained in the U.S. Based on accurate PM2.5 sampling, chemical analysis, and source apportionment models, the major PM2.5 sources in China have been identified to be coal combustion, motor vehicle emissions, and industrial sources. Atmospheric visibility has been found to correlate well with PM2.s concentration. Sulfate, ammonium, and nitrate carried by PM2.s, commonly found in coal burning and vehicle emissions, are the dominant contributors to regional haze in China. Short-term exposure to PM2.s is strongly associated with the increased risk of morbidity and mortality from cardiovascular and respiratory diseases in China. The strategy for PMzs mitigation must be based on reducing the pollutants from the two primary sources of coal-fired power plants and vehicle emissions. Although conventional Particulate Emission Control Devices (PECD) such as electrostatic precipitators in Chinese coal-fired power plants are generally effective for large particles, most of them may not have high collection efficiency of PM2.5. Baghouse filtration is gradually incorporated into the PECD to increase the PM2.5 collection efficiency. By adopting stringent vehicle emissions standard such as Euro 5 and 6, the emissions from vehicles can be gradually reduced over the years. An integrative approach, from collaboration among academia, government, and industries, can effectively manage and mitigate the PM2.s pollution in China.