Reconfigurable and polarization-dependent optical filtering for transflective full-color generation utilizing low-loss phase-change materials

All-dielectric metasurface, which features low optical absorptance and high resolution, is becoming a promising candidate for full-color generation. However, the optical response of current metamaterials is fixed and lacks active tuning. In this work, we demonstrate a reconfigurable and polarization-dependent active color generation technique by incorporating low-loss phase change materials(PCMs) and CaF_2 all-dielectric substrate. Based on the strong Mie resonance effect and low optical absorption structure, a transflective, full-color with high color purity and gamut value is achieved. The spectrum can be dynamically manipulated by changing either the polarization of incident light or the PCM state. High transmittance and reflectance can be simultaneously achieved by using low-loss PCMs and substrate. The novel active metasurfaces can bring new inspiration in the areas of optical encryption, anti-counterfeiting, and display technologies.

High‑Entropy Electrode Materials:Synthesis,Properties and Outlook

High-entropy materials represent a new category of high-performance materials,first proposed in 2004 and extensively investigated by researchers over the past two decades.The definition of high-entropy materials has continuously evolved.In the last ten years,the discovery of an increasing number of high-entropy materials has led to significant advancements in their utilization in energy storage,electrocatalysis,and related domains,accompanied by a rise in techniques for fabricating high-entropy electrode materials.Recently,the research emphasis has shifted from solely improving the performance of high-entropy materials toward exploring their reaction mechanisms and adopting cleaner preparation approaches.However,the current definition of high-entropy materials remains relatively vague,and the preparation method of high-entropy materials is based on the preparation method of single metal/low-or medium-entropy materials.It should be noted that not all methods applicable to single metal/low-or medium-entropy materials can be directly applied to high-entropy materials.In this review,the definition and development of high-entropy materials are briefly reviewed.Subsequently,the classification of high-entropy electrode materials is presented,followed by a discussion of their applications in energy storage and catalysis from the perspective of synthesis methods.Finally,an evaluation of the advantages and disadvantages of various synthesis methods in the production process of different high-entropy materials is provided,along with a proposal for potential future development directions for high-entropy materials.

Research status and prospects of the fractal analysis of metal material surfaces and interfaces

As a mathematical analysis method,fractal analysis can be used to quantitatively describe irregular shapes with self-similar or self-affine properties.Fractal analysis has been used to characterize the shapes of metal materials at various scales and dimensions.Conventional methods make it difficult to quantitatively describe the relationship between the regular characteristics and properties of metal material surfaces and interfaces.However,fractal analysis can be used to quantitatively describe the shape characteristics of metal materials and to establish the quantitative relationships between the shape characteristics and various properties of metal materials.From the perspective of two-dimensional planes and three-dimensional curved surfaces,this paper reviews the current research status of the fractal analysis of metal precipitate interfaces,metal grain boundary interfaces,metal-deposited film surfaces,metal fracture surfaces,metal machined surfaces,and metal wear surfaces.The relationship between the fractal dimensions and properties of metal material surfaces and interfaces is summarized.Starting from three perspectives of fractal analysis,namely,research scope,image acquisition methods,and calculation methods,this paper identifies the direction of research on fractal analysis of metal material surfaces and interfaces that need to be developed.It is believed that revealing the deep influence mechanism between the fractal dimensions and properties of metal material surfaces and interfaces will be the key research direction of the fractal analysis of metal materials in the future.

Advanced Functional Electromagnetic Shielding Materials:A Review Based on Micro‑Nano Structure Interface Control of Biomass Cell Walls

Research efforts on electromagnetic interference(EMI)shielding materials have begun to converge on green and sustainable biomass materials.These materials offer numerous advantages such as being lightweight,porous,and hierarchical.Due to their porous nature,interfacial compatibility,and electrical conductivity,biomass materials hold significant potential as EMI shielding materials.Despite concerted efforts on the EMI shielding of biomass materials have been reported,this research area is still relatively new compared to traditional EMI shielding materials.In particular,a more comprehensive study and summary of the factors influencing biomass EMI shielding materials including the pore structure adjustment,preparation process,and micro-control would be valuable.The preparation methods and characteristics of wood,bamboo,cellulose and lignin in EMI shielding field are critically discussed in this paper,and similar biomass EMI materials are summarized and analyzed.The composite methods and fillers of various biomass materials were reviewed.this paper also highlights the mechanism of EMI shielding as well as existing prospects and challenges for development trends in this field.

Defect Engineering:Can it Mitigate Strong Coulomb Effect of Mg^(2+)in Cathode Materials for Rechargeable Magnesium Batteries?

Rechargeable magnesium batteries(RMBs)have been considered a promising“post lithium-ion battery”system to meet the rapidly increasing demand of the emerging electric vehicle and grid energy storage market.However,the sluggish diffusion kinetics of bivalent Mg^(2+)in the host material,related to the strong Coulomb effect between Mg^(2+)and host anion lattices,hinders their further development toward practical applications.Defect engineering,regarded as an effective strategy to break through the slow migration puzzle,has been validated in various cathode materials for RMBs.In this review,we first thoroughly understand the intrinsic mechanism of Mg^(2+)diffusion in cathode materials,from which the key factors affecting ion diffusion are further presented.Then,the positive effects of purposely introduced defects,including vacancy and doping,and the corresponding strategies for introducing various defects are discussed.The applications of defect engineering in cathode materials for RMBs with advanced electrochemical properties are also summarized.Finally,the existing challenges and future perspectives of defect engineering in cathode materials for the overall high-performance RMBs are described.

Electrically triggered dual-band tunable terahertz metamaterial band-pass filter based on Si_3N_4–VO_2–Si_3N_4 sandwich

We experimentally demonstrate an electrically triggered terahertz(THz) dual-band tunable band-pass filter based on Si_3 N_4–VO_2–Si_3 N_4 sandwich-structured hybrid metamaterials. The insulator–metal phase transition of VO_2 film is induced by the Joule thermal effect of the top metal layer. The finite-integration-time-domain(FITD) method and finite element method(FEM) are used for numerical simulations. The sample is fabricated using a surface micromachining process,and characterized by a THz time-domain-spectrometer(TDS). When the bias current is 0.225 A, the intensity modulation depths at two central frequencies of 0.56 THz and 0.91 THz are about 81.7% and 81.3%, respectively. This novel design can achieve dynamically electric–thermo–optic modulation in the THz region, and has potential applications in the fields of THz communications, imaging, sensing, and astronomy exploration.

Design and theoretical study of a polarization-insensitive multiband terahertz metamaterial bandpass filter

We report the design of a novel multiband metamaterial bandpass filter （BPF） in the terahertz （THz）-wave region. The designed BPF is composed of a metal-dielectric-metal sandwiched structure with three nested rings on the top surface and a cross structure on the bottom surface. Full-wave simulation results show that the designed BPF has three transmission peaks at frequencies of 0.42, 1.27, and 1.86 THz with transmission rates of-0.87,-1.85, and-1.83 dB, respectively. Multi-reflection interference theory is introduced to explain the transmission mechanism of the designed triple-band BPF. The theoretical transmission spectrum is in good agreement with the full-wave simulated results. The designed BPF can maintain a stable performance as the incident angle varies from 0 to 30 for both transverse electric and transverse magnetic polarizations of the incident wave. The designed BPF can be potentially used in THz devices due to its multiband transmissions, polarization insensitivity, and stable wide-angle response in the THz region.

Ultra-narrow bandwidth optical filters consisting of one-dimensional photonic crystals with anomalous dispersion materials

We present a new type of optical filter with an ultra-narrow bandwidth and a wide field-of-view （FOV）. This kind of optical filter consists of one-dimensional photonic crystal （PC） incorporating an anomalous-dispersion-material （ADM） with, for instance, an anomalous dispersion of 6P3/2←6S1/2 hyperfine structure transition of a caesium atom. The transmission spectra of optical filters are calculated by using the transfer-matrix method. The simulation results show that the designed optical filter has a bandwidth narrower than 0.33GHz and a wide FOV of ±30°as well. The response of transmission spectrum to an external magnetic field is also investigated.

AC Line Filter Electrochemical Capacitors:Materials,Morphology,and Configuration

Recently,more and more supercapacitors(SCs)have been developed as AC line filter capacitors,which are generally named AC line filter electrochemical capacitors(FECs).Compared to traditional bulky aluminum electrolytic capacitors(AECs),FECs have higher capacity and lower space occupancy,which makes them a strong competitor.However,different from the common SCs for energy storage,it is necessary to consider the frequency response of the SCs for AC line filtering,where the contradiction between frequency response and specific capacitance is a challenge.The researchers have proposed different solutions from the perspective of materials,morphology,and configuration for this challenge.Based on the above background,in this review,we briefly introduce the principle and parameters of AC line filter electrochemical capacitors.We systematically summarize the state-of-the-art progresses of FECs and discuss their possible application and development in the future.The development of FECs can greatly promote the planarization,integration,and miniaturization of filter capacitors,and provide a new solution for the utilization of green and unstable energy.

Investigation of Atmospheric Pressure Plasma Discharge and Its Application to Surface Modification of Blood-Filtering Material

Melt-blown polybutylene terephthalate (PBT) nonwoven materials treated by usingplasma is regarded as one of the excellent materials to filter white blood cells (WBC) from blood.In this paper, dielectric barrier discharge (DBD) plasma source at an improved quasi-stable at-mospheric pressure is achieved when discharge voltage, discharge current, and gap between theelectrodes are carefully controlled. This plasma source has been used to modify the surface ofPBT melt-blown nonwoven materials. Experimental results indicate that both the wettablity andpermeation of treated PBT melt-blown nonwoven materials are greatly improved.

Mechanically tunable metamaterials terahertz dual-band bandstop filter

We experimentally demonstrate a mechanically tunable metamaterials terahertz（THz） dual-band bandstop filter. The unit cell of the filter contains an inner aluminum circle and an outside aluminum Ohm-ring on high resistance silicon substrate. The performance of the filter is simulated by finite-integration-time-domain（FITD） method. The sample is fabricated using a surface micromachining process and experimentally demonstrated using a THz time-domain-spectroscopy（TDS） system. The results show that, when the incident THz wave is polarized in y-axis, the filter has two intensive absorption peaks locating at 0.71 THz and 1.13 THz, respectively. The position of the high-frequency absorption peak and the amplitude of the low-frequency absorption peak can be simultaneously tuned by rotating the sample along its normal axis.The tunability of the high-frequency absorption peak is due to the shift of resonance frequency of two electrical dipoles,and that of the low-frequency absorption peak results from the effect of rotationally induced transparent. This tunable filter is very useful for switch, manipulation, and frequency selective detection of THz beam.

Efficiency characterization of ceramic filtering materials used for drinking water treatment

For ceramic filtering materials, their adsorption capacities, purification efficiencies to remove organic compounds from drinking water, and correlation between adsorption capacities and pore structures were tested and analyzed. The results show that correlation coefficient between the specific surface area and the adsorptive amount of iodine molecule is 0.99; correlation coefficient between the pore volume and the adsorptive value of tannin molecule is 0.92, and correlation coefficient between the most probable diameter and the adsorption parameter is 1.0. A new method of morphology characterization for ceramic filtering materials was developed, which offered a sort of standard for the evaluation on water purification efficiencies and selection of ceramic filtering materials.

Clean Steel Technologies Based on Interactions of Refractory Filtering Materials with Steel Melt

New carbon bonded filters with “active and reactive coatings ” for higher filtration efficiency of alumina based inclusions as well as nano-engineered filters with nano-scaled additives are explored with the aid of impingement tests and are evaluated according to their cold crushing strengths at room temperature. The combination of carbon nanotubes and alumina nanosheets additives leads to in situ formation of Al3 CON. Both the nanoscaled additives as well as the extra alumina “active”coating lead to improved mechanical performance of the carbon bonded filters and open the horizon for filter macrostructures with higher filtration capacities in means of bigger dimensions. In a further step MWCNT（ multi walled carbon nanotubes） in combination with a synthetic pitch have been used as a functional coating on the surface of alumina carbon bonded filters. These filters have then been evaluated also with uncoated filters in a special casting simulator and the interactions between steel and filtering material have been investigated.

An Influencing Factor - Water-Filter Ratio on Heat Resistance of Condensate Polishing Filter Material in Water

In air-cooled condenser, high temperature condensing water m summer which approaching and exceed 60＊ C, which may result in filter materials degradation and release impurities. This paper discusses an influencing factor, water-filter ratio （soaking solution and filter quality ratio）, on leachable dissolution rate and filter material degradation rate m high temperature water. The UV absorption at 254nm （A254） and the exchange capacity ware measured after heat test as composite indicators. In addition, the Wends of A254 variation with heating time were measured in different water-filter ratio. The stability is probably due to the effect of water-filter ratio. This has been further borne out that, water-filter ratio increases, leachable concentration decreases exponentially and tends to a fLxed value.

Design and experimental verification of a dual-band metamaterial filter

In this paper, we present the design, simulation, and experimental verification of a dual-band free-standing metamaterial filter operating in a frequency range of 1 THz–30 THz. The proposed structure consists of periodically arranged composite air holes, and exhibits two broad and flat transmission bands. To clarify the effects of the structural parameters on both resonant transmission bands, three sets of experiments are performed. The first resonant transmission band shows a shift towards higher frequency when the side width w;of the main air hole is increased. In contrast, the second resonant transmission band displays a shift towards lower frequency when the side width w;of the sub-holes is increased, while the first resonant transmission band is unchanged. The measured results indicate that these resonant bands can be modulated individually by simply optimizing the relevant structural parameters（w;or w;） for the required band. In addition, these resonant bands merge into a single resonant band with a bandwidth of 7.7 THz when w;and w;are optimized simultaneously. The structure proposed in this paper adopts different resonant mechanisms for transmission at different frequencies and thus offers a method to achieve a dual-band and low-loss filter.

一种基于Filter Faster R-CNN的数字PCR液滴检测技术

目的研究液滴数字聚合酶链式反应(ddPCR)液滴检测技术,去除图像中灰尘、气泡、芯片表面的划痕以及微小凹陷等因素产生的异常点对结果的影响,实现高通量、稳定和准确的ddPCR液滴的自动检测。方法提出Filter Faster R-CNN ddPCR液滴检测模型。使用Faster R-CNN生成液滴预测框,之后使用异常点过滤模块(Filter)去除阳性液滴预测框中的异常点。以诺如病毒片段的质粒为模板进行ddPCR实验,建立一个ddPCR数据集,用于模型的训练(2462例,约占78.56%)和测试(672例,约占21.44%)。对异常点过滤模块的3个过滤支路在验证集上进行消融实验,通过与其他ddPCR液滴检测模型进行比较的对比实验以及进行ddPCR的绝对定量实验。结果在少尘和多尘的环境中,Filter Faster R-CNN阳性液滴准确率为98.23%和88.35%,综合指标F1分数分别达到了99.15%和99.14%,高于其他相比较的模型。独立样本T检验的结果证明,相比未添加过滤模块的网络,添加过滤模块后能够显著提示模型在多尘环境中的阳性准确率。在ddPCR绝对定量实验中,将商业化流式检测设备的结果作为标准浓度,绘制了回归线。结果显示,回归线斜率为1.0005,截距为-0.025,决定系数达到了0.9997,二者结果高度一致。结论本文提出了一种基于Filter Faster R-CNN的ddPCR液滴检测技术,为在多种环境条件下的ddPCR实验提供了鲁棒的液滴检测方法。

Dynamically tunable terahertz passband filter based on metamaterials integrated with a graphene middle layer

The dynamic tunability of a terahertz（THz） passband filter was realized by changing the Fermi energy（EF） of graphene based on the sandwiched structure of metal-graphene-metal metamaterials（MGMs）. By using plane wave simulation, we demonstrated that the central frequency（ f0） of the proposed filter can shift from 5.04 THz to 5.71 THz; this shift is accompanied by a 3 dB bandwidth（ f） decrease from 1.82 THz to 0.01 THz as the EFincreases from 0 to 0.75 eV.Additionally, in order to select a suitable control equation for the proposed filter, the curves of f and f0 under different graphene EFwere fitted using five different mathematical models. The fitting results demonstrate that the Dose Resp model offers accurate predictions of the change in the 3 dB bandwidth, and the Quartic model can successfully describe the variation in the center frequency of the proposed filter. Moreover, the electric field and current density analyses show that the dynamic tuning property of the proposed filter is mainly caused by the competition of two coupling effects at different graphene EF, i.e., graphene-polyimide coupling and graphene-metal coupling. This study shows that the proposed structures are promising for realizing dynamically tunable filters in innovative THz communication systems.

The Roadmap of 2D Materials and Devices Toward Chips

Due to the constraints imposed by physical effects and performance degra certain limitations in sustaining the advancement of Moore’s law.Two-dimensional(2D)materials have emerged as highly promising candidates for the post-Moore era,offering significant potential in domains such as integrated circuits and next-generation computing.Here,in this review,the progress of 2D semiconductors in process engineering and various electronic applications are summarized.A careful introduction of material synthesis,transistor engineering focused on device configuration,dielectric engineering,contact engineering,and material integration are given first.Then 2D transistors for certain electronic applications including digital and analog circuits,heterogeneous integration chips,and sensing circuits are discussed.Moreover,several promising applications(artificial intelligence chips and quantum chips)based on specific mechanism devices are introduced.Finally,the challenges for 2D materials encountered in achieving circuit-level or system-level applications are analyzed,and potential development pathways or roadmaps are further speculated and outlooked.

Evaluation of Inocula and Packing Material for Acceleration of Start-Up in Biofilters

Several strategies with different combination of inocula and packing material were investigated to obtain the optimal start-up time and elimination capacity (EC) in toluene biofiltration. The inocula contained the activated sludge and toluene degrading bacteria, and the packing material consisted of different mixing ratios of peat and wood chips. A final toluene load of 21.2 g/(m3·h) was attained step by step in four parallel biofilters. A shortest start-up time of 15 days and a highest EC of 17.0 g/(m3·h) were observed in the biofilter B-4, which was inoculated with a special microbial consortium consisting of three strains of toluene degrading bacteria and was packed with the mixture of peat and wood chips at a ratio of 80:20 (w/w). These results indicated that inoculating pre-acclimatized microbes dramatically shortened the start-up time, and such a composition of packing material could maintain an appropriate environment (with the bed porosity and water content equating to 0.45 and 1.96, respectively) for the growth of dominant toluene degrading bacteria in the biofilter.

Structural Engineering of Anode Materials for Low-Temperature Lithium-Ion Batteries:Mechanisms,Strategies,and Prospects

The severe degradation of electrochemical performance for lithium-ion batteries(LIBs)at low temperatures poses a significant challenge to their practical applications.Consequently,extensive efforts have been contributed to explore novel anode materials with high electronic conductivity and rapid Li^(+)diffusion kinetics for achieving favorable low-temperature performance of LIBs.Herein,we try to review the recent reports on the synthesis and characterizations of low-temperature anode materials.First,we summarize the underlying mechanisms responsible for the performance degradation of anode materials at subzero temperatures.Second,detailed discussions concerning the key pathways(boosting electronic conductivity,enhancing Li^(+)diffusion kinetics,and inhibiting lithium dendrite)for improving the low-temperature performance of anode materials are presented.Third,several commonly used low-temperature anode materials are briefly introduced.Fourth,recent progress in the engineering of these low-temperature anode materials is summarized in terms of structural design,morphology control,surface&interface modifications,and multiphase materials.Finally,the challenges that remain to be solved in the field of low-temperature anode materials are discussed.This review was organized to offer valuable insights and guidance for next-generation LIBs with excellent low-temperature electrochemical performance.