An experiment for measuring the hyperon-related fission rate was carried out with the reaction 209^Bi(e, e'K^+)209^hPb at the Thomas Jefferson National Laboratory (Jlab). In the experiment, the performance of th...An experiment for measuring the hyperon-related fission rate was carried out with the reaction 209^Bi(e, e'K^+)209^hPb at the Thomas Jefferson National Laboratory (Jlab). In the experiment, the performance of the fission fragment detector (FFD) was dramaticlly crashed by the background particles in comparison with that during the test without beam. The scattering of the high intensity (500 nA) primary electrons was the dominant cause. Using the GEANT4 toolkit, this report simulates the experimental situation of the target chamber in which the FFD was located. The simulation results indicate that the background particles were dominantly (~ electrons, and protons and alpha particles were the important heavy background particles. The performance of the multi-wire proportional chambers (MWPCs) depends not only on the background-particle intensity but also the current density, which was also given by the simulation code. Furthermore, the measures to suppress the background particles were also investigated with the simulation code.展开更多
In this paper, a home-made code was designed to calculate the decay heat emitted by fission fragments as a result of successive radioactive emissions after a fission burst. The nuclear data necessary for the calculati...In this paper, a home-made code was designed to calculate the decay heat emitted by fission fragments as a result of successive radioactive emissions after a fission burst. The nuclear data necessary for the calculations was extracted from the latest version of the Evaluated Nuclear Data Library ENDF/B-VIII.0. The code can calculate the decay heat of thermal and fast neutron-induced fission reactions on the isotopes of Thorium, Protactinium, Uranium, Neptunium, Plutonium, Americium, Curium, California, Einsteinium, and Fermium. A numerical method was used in this work to calculate the decay heat of all fission fragments due to the individual thermal or fast fissions of the isotopes of the previous ten actinides. The most influential nuclei in the decay heat were also identified at different times after the fission event. Moreover, the code showed high capability in calculating the fission fragments inventories and decay heats due to the decay of fission fragments of 31 fissionable nuclei.展开更多
A new statistical method for systematizing the nuclei fission fragments, investigation of their mass and charge spectra and neutron fission parameters has been suggested. In proposed method, the mass and charge yields...A new statistical method for systematizing the nuclei fission fragments, investigation of their mass and charge spectra and neutron fission parameters has been suggested. In proposed method, the mass and charge yields of nucleons are determined from the equilibrium conditions of the nuclear fragments post-fission ensemble. Here we consider protons and neutrons of different fragments as statistically non-equivalent. The abilities of the proposed statistical method for explanation of the U, Pa, Th, Ac and Ra post-fission fragments ordering and neutron emission function calculation have been demonstrated.展开更多
Using the Skyrme density functional theory,potential energy surfaces of^(240)Pu with constraints on the axial quadrupole and octupole deformations(q_(20)and q_(30))were calculated.The volume-like and surface-like pair...Using the Skyrme density functional theory,potential energy surfaces of^(240)Pu with constraints on the axial quadrupole and octupole deformations(q_(20)and q_(30))were calculated.The volume-like and surface-like pairing forces,as well as a combination of these two forces,were used for the Hartree–Fock–Bogoliubov approximation.Variations in the least-energy fission path,fission barrier,pairing energy,total kinetic energy,scission line,and mass distribution of the fission fragments based on the different forms of the pairing forces were analyzed and discussed.The fission dynamics were studied based on the timedependent generator coordinate method plus the Gaussian overlap approximation.The results demonstrated a sensitivity of the mass and charge distributions of the fission fragments on the form of the pairing force.Based on the investigation of the neutron-induced fission of^(239)Pu,among the volume,mixed,and surface pairing forces,the mixed pairing force presented a good reproduction of the experimental data.展开更多
When a A hyperon is embedded in a nucleus it can form a hypernucleus. The lifetime and its mass dependence of stable hypernuclei provide information about the AN interaction in the nuclear medium. This work will intro...When a A hyperon is embedded in a nucleus it can form a hypernucleus. The lifetime and its mass dependence of stable hypernuclei provide information about the AN interaction in the nuclear medium. This work will introduce the Jefferson Lab experiment (E02-017), which aims to study the lifetime of the heavy hypernuclei using a specially developed fission fragment detection technique: a multi-wire proportional chamber operating under low gas pressure (LPMWPC). The trajectory of the detected fragment is reconstructed and used to find the fission point on the target foil, the position resolution is less than I ram, which meets the original design, the separation of target materials and events mixture percentage in different regions are verified by Monte Carlo simulation.展开更多
Based on the neutron induced fission fragment mass distribution data up to neutron energy 20 MeV measured with the double kinetic energy method (KEM) and the radio active method (RAM), the systematics of fission f...Based on the neutron induced fission fragment mass distribution data up to neutron energy 20 MeV measured with the double kinetic energy method (KEM) and the radio active method (RAM), the systematics of fission fragment mass distribution was investigated by using 5 Gaussian model and the systematics parameters were obtained by fitting the experimental data. With the systematics, the yields of any mass A and at any energy in the region from 0 to 20 MeV of neutron energy can be calculated. The calculated results could well reproduce the experimental data measured with KEM, but show some systematical deviation from the data measured by RAM, which reflects some systematical deviations between the two kinds of measured data. The error of systematics yield was calculated in an exact error transformation way, including from the error of the experimental yield data to the error of the discrete parameters, then to the systematics parameters, and at last to the yield calculated with systematics.展开更多
According to some experimental and evaluated data,the total excitation energy partitioning way between both of the fission fragments was given with a semi-empirical method. With the calculated energy partitioning way,...According to some experimental and evaluated data,the total excitation energy partitioning way between both of the fission fragments was given with a semi-empirical method. With the calculated energy partitioning way,the prompt neutron multiplicity as a function of fragment mass,(A) ,for neutron-induced fission of 235U at En=0.0253 eV,3 MeV,and 5 MeV was calculated. The results are checked with the total average prompt neutron multiplicities and compared with the experimental and evaluated data.展开更多
We applied the four dimensional Langevin dynamical model to investigate the average spin of fission fragments. Elongation, neck thickness, asymmetry parameter, and the orientation degree of freedom(K coordinate)are ...We applied the four dimensional Langevin dynamical model to investigate the average spin of fission fragments. Elongation, neck thickness, asymmetry parameter, and the orientation degree of freedom(K coordinate)are the four dimensions of the dynamical model. We assume that the collective modes depend on the emission angle of the fragments, then different parameters related to the average spin of fission fragments are calculated dynamically.The angle dependence of average spin of fission fragments is investigated by calculating the spin at angles 90?and165?. Also, the obtained results based on the transition state model at scission point are presented. One can obtain better agreement between the results of the dynamical model and experimental data in comparison with the results of the transition state model.展开更多
The temperature dependent width of the fission fragment distributions was simulated in the Langevin equation by taking two-parameter exponential form of the fission fragment mass variance at scission point for each fi...The temperature dependent width of the fission fragment distributions was simulated in the Langevin equation by taking two-parameter exponential form of the fission fragment mass variance at scission point for each fission event. The result can reproduce experimental data well, and it permits to make reliable estimate for unmeasured product yields near symmetry fission.展开更多
The fission angular distributions and the angular dependence of fragment spins in ter-ms of preequilibrium fission model are calculated.The results show strong effects of preequil-ibrium fission on both angular distri...The fission angular distributions and the angular dependence of fragment spins in ter-ms of preequilibrium fission model are calculated.The results show strong effects of preequil-ibrium fission on both angular distributions and angular dependence of fragment spins.展开更多
MIXED Oxide Nuclear fuel (MOX) contains both uranium and plutonium in oxidized form. It is important to calculate the nuclear decay heat due to the single thermal fission (fission due to 0.0235 eV neutron) for all fis...MIXED Oxide Nuclear fuel (MOX) contains both uranium and plutonium in oxidized form. It is important to calculate the nuclear decay heat due to the single thermal fission (fission due to 0.0235 eV neutron) for all fissile nuclei in the MOX fuels (U<sup>235</sup>, Pu<sup>239</sup>, and Pu<sup>241</sup>). These fissile nuclei are the main source of the decay heat in MOX fuel. Decay heat calculation of the weighted fissile material content in MOX fuel is also important. A numerical method was used in this work to calculate the concentrations of all fission products due to the individual thermal fission of the three fissile materials as a function of time N(t). The decay heat calculations for the three fissile materials are directly calculated using the summation method by knowing the different concentrations of fission products over time. The average decay heat of the MOX fuel in induced thermal fission is also concluded. The most influential nuclei in the decay heat were also identified. The method used has been validated by several comparisons before, but the new in this work is using the most recent Evaluated Nuclear Data Library ENDF/B-VIII.0. Calculations of decay heat show very common trends for a period of 10<sup>7</sup> sec after the fission burst of thermal fissions of individual fissile nuclei. Moreover, the code showed high capability in calculating the fission fragments inventories and decay heats due to the decay of fission fragments of 31 fissionable nuclei.展开更多
Photofission fragments mass yield for^(232)Th,^(234;238) U,^(237) Np, and^(239;240;242) Pu isotopes are investigated.The calculations are done using a developed approach based on Gorodisskiy's phenomenological for...Photofission fragments mass yield for^(232)Th,^(234;238) U,^(237) Np, and^(239;240;242) Pu isotopes are investigated.The calculations are done using a developed approach based on Gorodisskiy's phenomenological formalism. The Gorodisskiy's method is developed to be applied for the neutron-induced fission. Here we revised it for application to photofission. The effect of emitted neutron prior to fission on the fission fragment mass yields has also been studied. The peak-to-valley ratio is extracted for the240 Pu isotope as a function of energy. Obtained results of the present formalism are compared with the available experimental data. Satisfactory agreement is achieved between the results of present approach and the experimental data.展开更多
The fragment angular distributions of fusion-fission reactions for the systemsof <sup>16</sup>O+<sup>232</sup>Th,<sup>19</sup>F+<sup>232</sup>Th and <sup>16</su...The fragment angular distributions of fusion-fission reactions for the systemsof <sup>16</sup>O+<sup>232</sup>Th,<sup>19</sup>F+<sup>232</sup>Th and <sup>16</sup>O+<sup>238</sup>U at near-and sub-barrier energies were measured.The measured fragment anisotropies obviously deviate from the predictions ofscission-point transition-state model.We also compared the excitation energy of tiltingmode with the statistical assumption.It was found that thermal equilibrium is not estab-lished at scission for the reactions studied.展开更多
The 230Ra has been produced via multinucleon transfer and dissipative fragmentation of heavy target in the 60 MeV/u 18O ion reaction with natural thorium. The radium was radiochemically separated from irradiated thori...The 230Ra has been produced via multinucleon transfer and dissipative fragmentation of heavy target in the 60 MeV/u 18O ion reaction with natural thorium. The radium was radiochemically separated from irradiated thorium targets. 230Ac was obtained by 230Ra β-→230Ac. Thin Ra sources were prepared for observing fission fragments from β-delayed fission of 230Ac. The sources were exposed to the mica fission track detectors and measured by a HPGe γ detector. The two fission events were obtained and could been assigned to the β-delayed fission of 230Ac. The β-delayed fission probability of 230Ac was determined to be (1.19±0.85)×10-8.展开更多
基金supported by the Fundamental Research Funds for the Central Universities of China (No.HEUCF101501)the Fundamental Research Funds of Harbin Engineering University of China (No.002150260713)
文摘An experiment for measuring the hyperon-related fission rate was carried out with the reaction 209^Bi(e, e'K^+)209^hPb at the Thomas Jefferson National Laboratory (Jlab). In the experiment, the performance of the fission fragment detector (FFD) was dramaticlly crashed by the background particles in comparison with that during the test without beam. The scattering of the high intensity (500 nA) primary electrons was the dominant cause. Using the GEANT4 toolkit, this report simulates the experimental situation of the target chamber in which the FFD was located. The simulation results indicate that the background particles were dominantly (~ electrons, and protons and alpha particles were the important heavy background particles. The performance of the multi-wire proportional chambers (MWPCs) depends not only on the background-particle intensity but also the current density, which was also given by the simulation code. Furthermore, the measures to suppress the background particles were also investigated with the simulation code.
文摘In this paper, a home-made code was designed to calculate the decay heat emitted by fission fragments as a result of successive radioactive emissions after a fission burst. The nuclear data necessary for the calculations was extracted from the latest version of the Evaluated Nuclear Data Library ENDF/B-VIII.0. The code can calculate the decay heat of thermal and fast neutron-induced fission reactions on the isotopes of Thorium, Protactinium, Uranium, Neptunium, Plutonium, Americium, Curium, California, Einsteinium, and Fermium. A numerical method was used in this work to calculate the decay heat of all fission fragments due to the individual thermal or fast fissions of the isotopes of the previous ten actinides. The most influential nuclei in the decay heat were also identified at different times after the fission event. Moreover, the code showed high capability in calculating the fission fragments inventories and decay heats due to the decay of fission fragments of 31 fissionable nuclei.
文摘A new statistical method for systematizing the nuclei fission fragments, investigation of their mass and charge spectra and neutron fission parameters has been suggested. In proposed method, the mass and charge yields of nucleons are determined from the equilibrium conditions of the nuclear fragments post-fission ensemble. Here we consider protons and neutrons of different fragments as statistically non-equivalent. The abilities of the proposed statistical method for explanation of the U, Pa, Th, Ac and Ra post-fission fragments ordering and neutron emission function calculation have been demonstrated.
基金supported by the National Key R&D Program of China(No.2022YFA1602000)National Natural Science Foundation of China(Nos.12275081,U2067205,11790325,and U1732138)the Continuous-support Basic Scientific Research Project。
文摘Using the Skyrme density functional theory,potential energy surfaces of^(240)Pu with constraints on the axial quadrupole and octupole deformations(q_(20)and q_(30))were calculated.The volume-like and surface-like pairing forces,as well as a combination of these two forces,were used for the Hartree–Fock–Bogoliubov approximation.Variations in the least-energy fission path,fission barrier,pairing energy,total kinetic energy,scission line,and mass distribution of the fission fragments based on the different forms of the pairing forces were analyzed and discussed.The fission dynamics were studied based on the timedependent generator coordinate method plus the Gaussian overlap approximation.The results demonstrated a sensitivity of the mass and charge distributions of the fission fragments on the form of the pairing force.Based on the investigation of the neutron-induced fission of^(239)Pu,among the volume,mixed,and surface pairing forces,the mixed pairing force presented a good reproduction of the experimental data.
基金Supported by National Natural Science Foundation of China(11175075,11135002 and 91026021)supported by the State Scholarship Fund Program of the China Scholarship Council
文摘When a A hyperon is embedded in a nucleus it can form a hypernucleus. The lifetime and its mass dependence of stable hypernuclei provide information about the AN interaction in the nuclear medium. This work will introduce the Jefferson Lab experiment (E02-017), which aims to study the lifetime of the heavy hypernuclei using a specially developed fission fragment detection technique: a multi-wire proportional chamber operating under low gas pressure (LPMWPC). The trajectory of the detected fragment is reconstructed and used to find the fission point on the target foil, the position resolution is less than I ram, which meets the original design, the separation of target materials and events mixture percentage in different regions are verified by Monte Carlo simulation.
文摘Based on the neutron induced fission fragment mass distribution data up to neutron energy 20 MeV measured with the double kinetic energy method (KEM) and the radio active method (RAM), the systematics of fission fragment mass distribution was investigated by using 5 Gaussian model and the systematics parameters were obtained by fitting the experimental data. With the systematics, the yields of any mass A and at any energy in the region from 0 to 20 MeV of neutron energy can be calculated. The calculated results could well reproduce the experimental data measured with KEM, but show some systematical deviation from the data measured by RAM, which reflects some systematical deviations between the two kinds of measured data. The error of systematics yield was calculated in an exact error transformation way, including from the error of the experimental yield data to the error of the discrete parameters, then to the systematics parameters, and at last to the yield calculated with systematics.
文摘According to some experimental and evaluated data,the total excitation energy partitioning way between both of the fission fragments was given with a semi-empirical method. With the calculated energy partitioning way,the prompt neutron multiplicity as a function of fragment mass,(A) ,for neutron-induced fission of 235U at En=0.0253 eV,3 MeV,and 5 MeV was calculated. The results are checked with the total average prompt neutron multiplicities and compared with the experimental and evaluated data.
文摘We applied the four dimensional Langevin dynamical model to investigate the average spin of fission fragments. Elongation, neck thickness, asymmetry parameter, and the orientation degree of freedom(K coordinate)are the four dimensions of the dynamical model. We assume that the collective modes depend on the emission angle of the fragments, then different parameters related to the average spin of fission fragments are calculated dynamically.The angle dependence of average spin of fission fragments is investigated by calculating the spin at angles 90?and165?. Also, the obtained results based on the transition state model at scission point are presented. One can obtain better agreement between the results of the dynamical model and experimental data in comparison with the results of the transition state model.
基金Supported by Knowledge Innovation Program of Chinese Academy of Sciences (55010701)National Support Plan of Science and Technology of China (2006BAI08B04-7)+2 种基金973 Program (2007CB815004)Shanghai Development Foundation from Science and Technology (06JC14082)National Natural Science Foundation of China (10775167)
文摘The temperature dependent width of the fission fragment distributions was simulated in the Langevin equation by taking two-parameter exponential form of the fission fragment mass variance at scission point for each fission event. The result can reproduce experimental data well, and it permits to make reliable estimate for unmeasured product yields near symmetry fission.
文摘The fission angular distributions and the angular dependence of fragment spins in ter-ms of preequilibrium fission model are calculated.The results show strong effects of preequil-ibrium fission on both angular distributions and angular dependence of fragment spins.
文摘MIXED Oxide Nuclear fuel (MOX) contains both uranium and plutonium in oxidized form. It is important to calculate the nuclear decay heat due to the single thermal fission (fission due to 0.0235 eV neutron) for all fissile nuclei in the MOX fuels (U<sup>235</sup>, Pu<sup>239</sup>, and Pu<sup>241</sup>). These fissile nuclei are the main source of the decay heat in MOX fuel. Decay heat calculation of the weighted fissile material content in MOX fuel is also important. A numerical method was used in this work to calculate the concentrations of all fission products due to the individual thermal fission of the three fissile materials as a function of time N(t). The decay heat calculations for the three fissile materials are directly calculated using the summation method by knowing the different concentrations of fission products over time. The average decay heat of the MOX fuel in induced thermal fission is also concluded. The most influential nuclei in the decay heat were also identified. The method used has been validated by several comparisons before, but the new in this work is using the most recent Evaluated Nuclear Data Library ENDF/B-VIII.0. Calculations of decay heat show very common trends for a period of 10<sup>7</sup> sec after the fission burst of thermal fissions of individual fissile nuclei. Moreover, the code showed high capability in calculating the fission fragments inventories and decay heats due to the decay of fission fragments of 31 fissionable nuclei.
文摘Photofission fragments mass yield for^(232)Th,^(234;238) U,^(237) Np, and^(239;240;242) Pu isotopes are investigated.The calculations are done using a developed approach based on Gorodisskiy's phenomenological formalism. The Gorodisskiy's method is developed to be applied for the neutron-induced fission. Here we revised it for application to photofission. The effect of emitted neutron prior to fission on the fission fragment mass yields has also been studied. The peak-to-valley ratio is extracted for the240 Pu isotope as a function of energy. Obtained results of the present formalism are compared with the available experimental data. Satisfactory agreement is achieved between the results of present approach and the experimental data.
基金The project supported by the National Natural Science Foundation of China under the contract No.19275067.
文摘The fragment angular distributions of fusion-fission reactions for the systemsof <sup>16</sup>O+<sup>232</sup>Th,<sup>19</sup>F+<sup>232</sup>Th and <sup>16</sup>O+<sup>238</sup>U at near-and sub-barrier energies were measured.The measured fragment anisotropies obviously deviate from the predictions ofscission-point transition-state model.We also compared the excitation energy of tiltingmode with the statistical assumption.It was found that thermal equilibrium is not estab-lished at scission for the reactions studied.
基金Supported by the National Natural Science Foundation of ChinaMajor State Basic Research Development Program, Chinese Aca
文摘The 230Ra has been produced via multinucleon transfer and dissipative fragmentation of heavy target in the 60 MeV/u 18O ion reaction with natural thorium. The radium was radiochemically separated from irradiated thorium targets. 230Ac was obtained by 230Ra β-→230Ac. Thin Ra sources were prepared for observing fission fragments from β-delayed fission of 230Ac. The sources were exposed to the mica fission track detectors and measured by a HPGe γ detector. The two fission events were obtained and could been assigned to the β-delayed fission of 230Ac. The β-delayed fission probability of 230Ac was determined to be (1.19±0.85)×10-8.