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Seasonal response of nitrogen exchange fluxes to crab disturbance at sediment-water interface in coastal tidal wetlands
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作者 Guo-fen Hua Shang-qing Liu +4 位作者 Xiang-dong Liu Jin-li Li Yue Fang Wen-ting Xie Xiang Xu 《Water Science and Engineering》 EI CAS CSCD 2024年第2期129-138,共10页
Coastal wetlands are hotspots for nitrogen(N)cycling,and crab burrowing is known to transform N in intertidal marsh soils.However,the underlying mechanisms remain unclear.This study conducted field experiments and use... Coastal wetlands are hotspots for nitrogen(N)cycling,and crab burrowing is known to transform N in intertidal marsh soils.However,the underlying mechanisms remain unclear.This study conducted field experiments and used indoor control test devices to investigate the seasonal response of nitrogen to crab disturbance at the sediment-water interface in coastal tidal flat wetlands.The results showed that crab disturbance exhibited significant seasonality with large seasonal differences in cave density and depth.Due to crab disturbance,nitrogen fuxes at the sediment-water interface were much greater in the box with crabs than in the box without crabs.In summer,NH-N showed a positive flux from the sediment to the overlying water,but NO2-N and NOg-N showed positive fluxes from the sediment to the overlying water only in early stages.In winter,NH-N showed a positive flux from the sediment to the overlying water,but NO-N and NO,-N both exhibited positive and negative fluxes.These results indicated that the presence of crab burrows can cause the aerobic layer to move downward by approximately 8-15 cm in summer and directly promote nitrification at the sediment surface. 展开更多
关键词 Coastal tidal flat wetland Crab disturbance Nitrogen flux NITRIFICATION DENITRIFICATION Sediment-water interface
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Boundary Conditions for Momentum and Vorticity at an Interface between Two Fluids
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作者 Korekazu Ueyama 《Journal of Applied Mathematics and Physics》 2024年第1期16-33,共18页
Boundary conditions for momentum and vorticity have been precisely derived, paying attention to the physical meaning of each mathematical expression of terms rigorously obtained from the basic equations: Navier-Stokes... Boundary conditions for momentum and vorticity have been precisely derived, paying attention to the physical meaning of each mathematical expression of terms rigorously obtained from the basic equations: Navier-Stokes equation and the equation of vorticity transport. It has been shown first that a contribution of fluid molecules crossing over a conceptual surface moving with fluid velocity due to their fluctuating motion is essentially important to understanding transport phenomena of momentum and vorticity. A notion of surface layers, which are thin layers at both sides of an interface, has been introduced next to elucidate the transporting mechanism of momentum and vorticity from one phase to the other at an interface through which no fluid molecules are crossing over. A fact that a size of  δV, in which reliable values of density, momentum, and velocity of fluid are respectively defined as a volume-averaged mass of fluid molecules, a volume-averaged momentum of fluid molecules and a mass-averaged velocity of fluid molecules, is not infinitesimal but finite has been one of the key factors leading to the boundary conditions for vorticity at an interface between two fluids. The most distinguished characteristics of the boundary conditions derived here are the zero-value conditions for a normal component of momentum flux and tangential components of vorticity flux, at an interface. 展开更多
关键词 Boundary Condition for Vorticity Surface Layer interface Momentum flux Vorticity flux
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The Relationship of Sulfate-methane Interface,the Methane Flux and the Underlying Gas Hydrate 被引量:3
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作者 方银霞 初凤友 《Marine Science Bulletin》 CAS 2008年第1期28-37,共10页
The sulfate-methane interface is an important biogeochemical identification interface for the areas with high methane flux and containing gas hydrate. Above the sulfate-methane interface, the sulfate concentration in ... The sulfate-methane interface is an important biogeochemical identification interface for the areas with high methane flux and containing gas hydrate. Above the sulfate-methane interface, the sulfate concentration in the sediment is consumed progressively for the decomposition of the organic matter and anaerobic methane oxidation. Below the sulfate-methane interface, the methane concentration increases continuously with the depth. Based on the variation characters of the sulfate and methane concentration around the sulfate-methane interface, it is feasible to estimate the intensity of the methane flux, and thereafter to infer the possible occurrence of gas hydrate. The geochemical data of the pore water taken from the northern slope of the South China Sea show the sulfate-methane interface is relatively shallow, which indicates that this area has the high methane flux. It is considered that the high methane flux is most probably caused by the occurrence of underlying gas hydrate in the northern slope of the South China Sea. 展开更多
关键词 gas hydrate. methane flux sulfate-methane interface
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Analysis of heat pulse signals determination for sediment-water interface fluxes
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作者 朱腾义 Rajendra Prasad Singh 傅大放 《Journal of Southeast University(English Edition)》 EI CAS 2014年第2期192-196,共5页
The heat pulse signal is analyzed in a new way with the goals of clarifying the relationships between the variables in the heat transfer problem and simplifying the procedure for calculating sediment-water interface f... The heat pulse signal is analyzed in a new way with the goals of clarifying the relationships between the variables in the heat transfer problem and simplifying the procedure for calculating sediment-water interface fluxes J. Only three parameters x0 λand pc l are needed to calculate J by the heat pulse data for this analysis method.The results show that there is a curvilinear relationship between the peak temperature arrival time and sediment-water interface fluxes and there exists a simple linear relationship between sediment-water interface fluxes and the natural log of the ratio of the temperature increase downstream from the line heat source to the temperature increase upstream from the heat source.The simplicity of this relationship makes the heat pulse sensors an attractive option for measuring soil water fluxes. 展开更多
关键词 sediment-water interface flux seepage meter heat pulse peak arrival time
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The Effect of Bioturbation Activity of the Ark Clam Scapharca subcrenata on the Fluxes of Nutrient Exchange at the Sediment–Water Interface 被引量:5
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作者 ZHANG Shuo FANG Xin +4 位作者 ZHANG Junbo YIN Fang ZHANG Hu WU Lizhen KITAZAWA Daisuke 《Journal of Ocean University of China》 SCIE CAS CSCD 2020年第1期232-240,共9页
Filter-feeding shellfish are common benthos and significantly affect the biogeochemical cycle in the shallow coastal ecosystems.Ark clam Scapharca subcrenata is one of the widely cultured bivalve species in many coast... Filter-feeding shellfish are common benthos and significantly affect the biogeochemical cycle in the shallow coastal ecosystems.Ark clam Scapharca subcrenata is one of the widely cultured bivalve species in many coastal areas owing to its tremendous economic value.However,there is little information regarding the effects of the bioturbation of S.subcrenata on the fluxes of nutrient exchange in the sediment-water interface(SWI).In this regard,S.subcrenata was sampled during October 2016 to determine the effects of its bioturbation activity on the nutrient exchange flux of the SWI.The results showed that the biological activity of S.subcrenata could increase the diffusion depth and the rate of the nutrients exchange in the sediments.The bioturbation of S.subcrenata could allow the nutrients to permeate into the surface sediments at 6-10cm and increase the release rate of nutrients at the SWI.The releasing fluxes of DIN and PO43−-P in the culture area were found to be around three times higher than that in the non-cultured region.The culture of S.subcrenata has been proved to be an important contributor to nutrient exchange across the SWI in the farming area of Haizhou Bay.Nutrients exchange in the SWI contributes a part of 86%DIN,71%PO43−-P and 18%SiO32−-Si for the aquaculture farm. 展开更多
关键词 BIOTURBATION NUTRIENTS exchange flux ark clam sediment-water interface
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Carbon dioxide partial pressure and carbon fluxes of air-water interface in Taihu Lake, China 被引量:2
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作者 范成新 胡维平 +3 位作者 Phillip W. Ford 陈宇炜 瞿文川 张路 《Chinese Journal of Oceanology and Limnology》 SCIE CAS CSCD 2005年第1期29-38,共10页
To obtain carbon dioxide (CO2) flux between water-air interface of Taihu lake, monthly water samplers at 14 sites and the local meteorological data of the lake were collected and analyzed in 1998. Carbon dioxide par... To obtain carbon dioxide (CO2) flux between water-air interface of Taihu lake, monthly water samplers at 14 sites and the local meteorological data of the lake were collected and analyzed in 1998. Carbon dioxide partial pressures (pCO2) at air-water interface in the lake were calculated using alkalinity, pH, ionic strength, active coefficient, and water temperature. The carbon fluxes at different sublakes and areas were estimated by concentration gradient between water and air in consideration of Schmidt numbers of 600 and daily mean windspeed at 10 m above water surface. The results indicated that the mean values of pCO2 in Wuli Lake,Meiliang Bay, hydrophyte area, west littoral zone, riverine mouths, and the open lake areas were 1 807.8±1 071.4(mean±standard deviation)μatm (latm=1.013 25×10^5pa), 416.3±217.0μatm, 576.5±758.8μatm, 304.2±9.43.5μatm, 1 933.6±1 144.7 μatm, and 448.5±202.6μatm, respectively. Maximum and minimum pCO2 values were found in the hypertrophic (4 053.7μatm) and the eutrophic (3.2 μatm) areas. The riverine mouth areas have the maximum fluxes (82.0±62.8 mmol/m^2a). But there was no significant difference between eutrophic and mesotrophic areas in pCO2 and the flux of CO2. The hydrophyte area, however, has the minimum (--0.58±12.9mmol/m^2a). In respect to CO2 equilibrium, input of the rivers will obviously influence inorganic carbon distribution in the riverine estuary. For example, the annual mean CO2 flux in Zhihugang River estuary was 19 times of that in Meiliang Bay, although the former is only a part of the latter. The sites in the body of the lake show a clear seasonal cycle with pCO2 higher than atmospheric equilibrium in winter, and much lower than atmospheric in summer due to CO2 consumption by photosynthesis. The CO2 amount of the net annual evasion that enters the atmosphere is 28.42×10^4 t/a, of which those from the west littoral zone and the open lake account for 53.8% and 36.7%, respectively. 展开更多
关键词 carbon dioxide partial pressure air-water interface carbon flux trophic area river input Taihu Lake
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Nitrogen and Phosphorus Diffusive Fluxes Across the Sediment-Water Interface in Estuarine and Coastal Tidal Flats 被引量:2
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作者 刘敏 侯立军 +3 位作者 许世远 张斌亮 欧冬妮 刘巧梅 《Marine Science Bulletin》 CAS 2002年第1期34-41,共8页
Nitrogen and phosphorus contents are analyzed in the overlying waters and pore waters taken from the Changjiang Estuary and Shanghai coastal tidal flats in this study. In addition, the diffusion fluxes of nitrogen and... Nitrogen and phosphorus contents are analyzed in the overlying waters and pore waters taken from the Changjiang Estuary and Shanghai coastal tidal flats in this study. In addition, the diffusion fluxes of nitrogen and phosphorus across the sediment-water interface in tidal flats are estimated according to the nutrient concentration gradients at the interface. It has been indicated that the concentrations of ammonium, nitrite, nitrate and dissolved phosphorus in overlying waters range from 0.0082-2.56, 0.03-0.58, 0.69-5.38 and 0.035-0.53 mg/L, respectively, while 0.0025 - 1.35 mg /L for NH^-N, 0. 0055 ~0.20mg/L for NO2-N, 0.61-1.14 mg/L for NO3-N and 0.11~0.53mg/L for DP insurface pore waters.The findings have revealed that ammonium, nitrite, nitrate and dissolved phosphorus diffusionfluxes across the sediment-water interface are between -0.024~0.99, -0.39~ -0.0019, -3.09--0.12 and -0.48- 0.12 ug/ (cm.d ) respectively, showing that the sediment in tidal flats is the source of phosphorus and an important sink for nitrogen in the waters. 展开更多
关键词 Nitrogen and phosphorus diffusion fluxes pore waters sediment-water interface the Changjiang Estuary and coastal area
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Numerical Investigation on the Deformation of the Free Interface During Water Entry and Exit of a Circular Cylinder by Using the Immersed Boundary-Multiphase Lattice Boltzmann Flux Solver
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作者 Guiyong Zhang Haoran Yan +2 位作者 Hong Song Heng Wang Da Hui 《Journal of Marine Science and Application》 CSCD 2022年第3期99-113,共15页
In this work,the deformation of free interface during water entry and exit of a circular cylinder is investigated numerically by using the two-dimensional(2D)immersed boundary-multiphase lattice Boltzmann flux solver(... In this work,the deformation of free interface during water entry and exit of a circular cylinder is investigated numerically by using the two-dimensional(2D)immersed boundary-multiphase lattice Boltzmann flux solver(IB-MLBFS).The fluid domain is discretized by finite volume discretization,and the flux on the grid interface is evaluated by lattice Boltzmann equations.Both the implicit velocity correction and the surface flux correction are implemented by using the immersed boundary-method to consider the fluid-structure interaction and the contact interface between the multiphase fluids and the structure.First,the water entry of a circular cylinder is simulated and the results are compared with the experiment,which considered the length-diameter ratio of the circular cylinder.The reliability of 2D simulation is verified and the deformation of the free interface is well investigated.Afterward,the water exit of a circular cylinder with constant velocity is simulated,which is less researched.In addition,the results show the advantage of present IB-MLBFS to some extent.Finally,the water exit and re-entry of a circular cylinder are presented,and the results present the complex deformation of the free interface and the dynamic response of the moving structure.Based on the numerical results,the free interface of the multiphase fluids is well captured,and the contact interface on the boundary of the moving structure is accurately presented by the IB-MLBFS. 展开更多
关键词 Free interface Water entry Water exit Immersed boundary method Lattice Boltzmann flux solver
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DISSOLVED OXYGEN DISTRIBUTION AND O_2 FLUXES ACROSS THE SEA-AIR INTERFACE IN EAST CHINA SEA WATERS
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作者 宋金明 詹滨秋 李鹏程 《Chinese Journal of Oceanology and Limnology》 SCIE CAS CSCD 1996年第4期297-302,共6页
This study on the sectional and vertical distribution of dissolved oxygen (DO) and the O_2 fluxes acrossthe sea-air interface in East China Sea (ESC) waters shows that the waters were in steady state and thatthe diffe... This study on the sectional and vertical distribution of dissolved oxygen (DO) and the O_2 fluxes acrossthe sea-air interface in East China Sea (ESC) waters shows that the waters were in steady state and thatthe difference of DO was great in upper and bottom waters in Apr. 1994; but that seawater mixingwas strong and the difference of DO was small in upper and bettom waters in Oct. 1994. The above con-dusions were specially obvious in continental shelf waters under 100m. The DO maximum in subsurfacelayer waters appeared only at several stations and in general the DO in the waters decreased with depth.The horizontal distributions of O_2 fluxes across the sea-air interface appeared in stripes in Leg 9404 whenmost regions covend were supersaturated with O_2. seawater to air flux wn large, and that on section No.1was 1.594 L/m^2·d. The horizontal distribution of O_2 fluxes across the sea-air interface appeared lumpy inLeg 9410, when most regions covered were unsaturated with O_2. O_2 was dissolved from air to seawater,and the fluxes were 0.819 L/m^2·d on section No. 1 in Leg 9310, 0.219 L/m^2·d in Leg 9410. The mainreasons for DO change in surface layer seawater were the mixture of upper and bottom layer water, and theexchange of O_2 across the sea-air interface. The variation of DO by biological activity was only 20% of totalchange of DO. 展开更多
关键词 dissolved oxygen(Do) O_2 fluxes across the sea-air interface East China Sea waters
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Relations between Low-Frequency Modes of Climate Variability and Air-Sea Heat Flux at the Mediterranean Interface
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作者 Lamri Nacef Nour El Islam Bachari 《Journal of Earth Science and Engineering》 2014年第2期101-106,共6页
The main objective of this work is to examine statistical causality relationships between low-frequency modes of climate variability and winter (December to February) anomaly of net heat flux at the Mediterranean ai... The main objective of this work is to examine statistical causality relationships between low-frequency modes of climate variability and winter (December to February) anomaly of net heat flux at the Mediterranean air-sea interface. The introduction of the concept of Granger causality allowed us to examine the influence of these climates indices on the net heat flux anomaly and to select Mediterranean surface regions that really influenced by each index. Results show that the winter anomaly of the net heat flux in the Algerian basin south and the gulf of Lion is mainly caused by the Arctic Oscillation. El Nifio-Southern Oscillation influences much more the Algerian basin north and the northern lonian Sea. The Quasi-Biennial Oscillation affects only the Alboran and the Tyrrhenian Seas. But the Adriatic and Levantine basin are impacted by any climate index. They also show that these climate indices can increase explained variance in winter variations of air-sea net heat flux by 10% to 15%, with a lag of three seasons. These relationships are less persistent and spatially limited. 展开更多
关键词 Mediterranean Sea winter net heat flux air-sea interface climate index causality analysis.
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固液界面热阻的温度依赖特性模拟研究
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作者 王军 李海洋 夏国栋 《北京工业大学学报》 CAS CSCD 北大核心 2024年第7期864-871,共8页
基于非平衡态分子动力学模拟方法,研究了系统温度及固液结合强度对固液界面传热的影响规律。模拟结果表明,固液界面热阻随着系统温度的升高而降低,并且亲水性界面的界面热阻温度依赖性较弱。基于微观热流密度计算式的分析表明,随着系统... 基于非平衡态分子动力学模拟方法,研究了系统温度及固液结合强度对固液界面传热的影响规律。模拟结果表明,固液界面热阻随着系统温度的升高而降低,并且亲水性界面的界面热阻温度依赖性较弱。基于微观热流密度计算式的分析表明,随着系统温度升高,动能项和维里项的贡献均逐渐增大,因而固液界面传热增强,但是动能项占比逐渐增大,维里项占比逐渐降低;随着固液结合强度逐渐增大,界面吸附效应增强,维里项贡献明显增大,这是较强的固液相互作用能够强化界面传热的主要原因。 展开更多
关键词 界面热阻 分子动力学模拟 固液界面 温度依赖性 润湿性 微观热流密度
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海水多品种养殖池塘沉积物-水界面氮磷通量
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作者 陈仲 《水产科学》 CAS CSCD 北大核心 2024年第3期461-467,共7页
为探明生源要素氮、磷在沉积物与水体间的迁移过程,比较3种不同养殖模式下、不同时间养殖池塘沉积物-水界面的氮、磷通量变化,2014年6—10月,在3种综合养殖池塘:海蜇+凡纳滨对虾+菲律宾蛤仔、海蜇+凡纳滨对虾+缢蛏和海蜇+凡纳滨对虾的... 为探明生源要素氮、磷在沉积物与水体间的迁移过程,比较3种不同养殖模式下、不同时间养殖池塘沉积物-水界面的氮、磷通量变化,2014年6—10月,在3种综合养殖池塘:海蜇+凡纳滨对虾+菲律宾蛤仔、海蜇+凡纳滨对虾+缢蛏和海蜇+凡纳滨对虾的整个养殖周期内,采集检测3口池塘沉积物-水界面样品中的亚硝态氮、硝态氮、氨氮和活性磷酸盐含量,分析沉积物-水界面的亚硝态氮+硝态氮、氨氮和活性磷酸盐的通量变化。试验结果显示,6—10月,3种综合养殖池塘沉积物上覆水中亚硝态氮和硝态氮均以向沉积物中扩散为主,仅10月海蜇+凡纳滨对虾池塘沉积物中亚硝态氮和硝态氮向上覆水释放。海蜇+凡纳滨对虾+菲律宾蛤仔、海蜇+凡纳滨对虾+缢蛏池塘沉积物上覆水中氨氮向沉积物扩散,6月海蜇+凡纳滨对虾+缢蛏池塘沉积物中氨氮向上覆水扩散;与海蜇+凡纳滨对虾+菲律宾蛤仔和海蜇+凡纳滨对虾+缢蛏池塘相比,海蜇+凡纳滨对虾池塘氨氮通量变化幅度较大,6—7月上覆水中氨氮向沉积物扩散,且扩散速率逐渐降低,9—10月沉积物中氨氮向上覆水释放,释放速率逐渐上升。6、7、10月海蜇+凡纳滨对虾+菲律宾蛤仔池塘沉积物中活性磷酸盐向上覆水释放,8—9月上覆水中活性磷酸盐向沉积物扩散;6—10月,海蜇+凡纳滨对虾+缢蛏池塘沉积物中活性磷酸盐向上覆水释放;海蜇+凡纳滨对虾池塘上覆水中活性磷酸盐向沉积物扩散,10月沉积物中活性磷酸盐向上覆水释放。试验结果表明,配养底栖贝类,可以通过改变综合养殖池塘沉积物-水界面的氮、磷通量,改善池塘的底质和水质环境。 展开更多
关键词 综合养殖池塘 沉积物-水界面 营养盐通量
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夏季桑沟湾沉积物–水界面溶解氧分布和消耗的微观变化研究
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作者 康秦梓 刘毅 +3 位作者 吴文广 仲毅 王新萌 张继红 《渔业科学进展》 CSCD 北大核心 2024年第5期96-108,共13页
为探明高温条件下贝藻养殖区沉积物–水界面溶解氧(DO)分布和消耗的微观变化特性,在2022年夏季,采用微剖面法对桑沟湾贝类区、贝藻区、藻类区和外海区内沉积物DO、H2S、pH的剖面分布进行了调查,测定了沉积物中有机碳含量、粒径等因子的... 为探明高温条件下贝藻养殖区沉积物–水界面溶解氧(DO)分布和消耗的微观变化特性,在2022年夏季,采用微剖面法对桑沟湾贝类区、贝藻区、藻类区和外海区内沉积物DO、H2S、pH的剖面分布进行了调查,测定了沉积物中有机碳含量、粒径等因子的剖面分布,计算了不同养殖区域沉积物–水界面的DO交换通量和沉积物的耗氧率。研究发现,贝类区、贝藻区、藻类区和外海区沉积物扩散边界层(DBL)厚度分别为(1.5±0.3)、(1.0±0.3)、(2.0±0.8)和(1.3±0.2)mm,区域间差异不显著;氧渗透深度(OPD)分别为(12.49±1.59)、(12.17±0.09)、(15.49±0.79)和(14.87±1.27)mm,其中,贝类区和贝藻区氧渗透深度显著低于藻类区和外海区。贝类区、贝藻区、藻类区和外海区的DO扩散通量分别为(24.10±1.89)、(49.53±10.24)、(26.69±13.13)和(24.79±7.95)mmol/(m^(2)·d),贝藻区沉积物–水界面DO扩散通量显著高于其他区域。沉积物–水界面DO扩散通量受上覆水DO浓度和沉积物耗氧率的显著影响,贝类区沉积物–水界面DO扩散通量受上覆水DO、DBL厚度及水–沉积物界面处DO的共同影响,贝藻区、藻类区沉积物–水界面DO扩散通量主要影响因素为沉积物上覆水DO。研究结果为深入了解养殖活动在养殖生态系统碳循环中的作用提供了科技支撑。 展开更多
关键词 沉积物–水界面 微电极 溶解氧扩散通量 有机碳矿化
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浅水湖泊冬季温室气体浓度与通量的变化特征及影响因素
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作者 陈曦 程俊翔 +2 位作者 徐力刚 徐宪根 丁竹红 《环境科学研究》 CAS CSCD 北大核心 2024年第11期2478-2489,共12页
内陆水体是大气二氧化碳(CO_(2))、甲烷(CH_(4))、氧化亚氮(N_(2)O)的重要自然排放源。为研究浅水湖泊温室气体溶存浓度及排放通量,以太湖流域上游浅水湖泊-长荡湖为例,在冬季(2022年1-2月)利用顶空平衡-气相色谱法对其表层水体温室气... 内陆水体是大气二氧化碳(CO_(2))、甲烷(CH_(4))、氧化亚氮(N_(2)O)的重要自然排放源。为研究浅水湖泊温室气体溶存浓度及排放通量,以太湖流域上游浅水湖泊-长荡湖为例,在冬季(2022年1-2月)利用顶空平衡-气相色谱法对其表层水体温室气体溶存浓度及排放通量进行测定,综合采用方差分析、多元逐步回归分析等方法探究了长荡湖湖区及主要出入湖河口区温室气体溶存浓度与排放通量的空间分布特征及主要影响因素。结果表明:①长荡湖冬季CO_(2)、CH_(4)、N_(2)O平均溶存浓度分别为(40.49±14.18)μmol/L、(0.86±1.92)μmol/L和(18.43±8.44)nmol/L,平均排放通量分别为(49.99±69.49)μmol/(m^(2)·h)、(1.28±2.64)μmol/(m^(2)·h)和(12.01±14.37)nmol/(m^(2)·h)。②在空间分布上,湖区CO_(2)排放通量高于出入湖河口区,湖区CH_(4)、N_(2)O溶存浓度和排放通量均显著低于出入湖河口区。③CO_(2)排放主要受水温、电导率(EC)以及TN、TP和Chla浓度的影响,CH_(4)排放主要受pH、高锰酸盐指数(CODMn)、EC和DO浓度的影响,N_(2)O排放主要受pH以及DO、TN和TP浓度的影响。④长荡湖冬季CO_(2)、CH_(4)和N_(2)O累积排放通量分别为47.51、0.44和0.01 kg/hm^(2),结合水域面积估算得出温室气体排放总量为545.57 t(以CO_(2)当量计)。研究显示,长荡湖冬季温室气体排放呈现较明显的空间异质性,并受到不同区域水环境条件、外源营养输入及人类活动的共同影响。本研究强调了浅水湖泊冬季温室气体排放在内陆水体温室气体收支中的重要性,可为全球和区域湖泊温室气体排放精确估算提供重要支撑。 展开更多
关键词 浅水湖泊 温室气体 溶存浓度 水-气界面 排放通量 影响因子
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丘陵山区水库沉积物-水界面磷源汇转换机制
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作者 谭立贤 康得军 +3 位作者 刘成 朱利钊 申秋实 陈开宁 《中国环境科学》 EI CAS CSCD 北大核心 2024年第4期2137-2147,共11页
以东南丘陵山区典型深水水库对河口水库为研究对象,开展了1a的原位调研,在主要水域内采集原位柱状沉积物样品,分析了沉积物磷的含量、赋存形态、间隙水剖面特征以及沉积物-水界面交换通量的时空变化特征.结果表明:对河口水库表层沉积物... 以东南丘陵山区典型深水水库对河口水库为研究对象,开展了1a的原位调研,在主要水域内采集原位柱状沉积物样品,分析了沉积物磷的含量、赋存形态、间隙水剖面特征以及沉积物-水界面交换通量的时空变化特征.结果表明:对河口水库表层沉积物总磷(TP)含量变化范围为(470.8~1012.3)mg/kg,平均值达到(688.4±186.48)mg/kg,呈现从上游至下游逐渐增加的趋势,下游坝前区域磷污染最为严重;沉积物中各形态磷含量大小顺序依次为:铝结合态磷(352.61mg/kg)>铁结合态磷(Fe-P)(98.10mg/kg)>闭蓄态磷(88.77mg/kg)>钙结合态磷(72.42mg/kg)>有机磷(33.38mg/kg)>可交换态磷(1.64mg/kg).全库沉积物总体表现为磷的释放源,其中,秋季释放风险最高,冬季大部分区域沉积物从磷释放的源转变为汇;全年平均静态释放通量和扩散通量分别为(0.81±2.34)mg/(m^(2)·d)和(2.15±3.47)mg/(m^(2)·d),2种方法所得全年磷释放量分别为1.92和3.67t,秋季释放量最大.铁结合态磷(Fe-P)的转化可能是控制沉积物-水界面磷源-汇转换的重要原因,由氧分层导致的沉积物厌氧及铁结合态磷(Fe-P)溶解释放将增加下层水体磷浓度,并在水体逆温后增加水柱总体磷浓度.在秋季大量磷释放之后,应更加关注随后的逆温对整个水体磷浓度的影响. 展开更多
关键词 内源磷负荷 沉积物-水界面 磷通量 对河口水库 深水水库
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海洋天然气水合物发育顶界模拟——沉积物毛细管作用影响
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作者 曹运诚 周海玲 +1 位作者 郑子涵 陈多福 《沉积学报》 CAS CSCD 北大核心 2024年第4期1229-1238,共10页
【目的】海洋沉积物孔隙内部的毛细管作用可以升高水合物—水二相甲烷的溶解度,影响天然气水合物的分布。确定毛细管作用对水合物发育顶界的影响,可以为水合物的成藏演化研究及水合物勘察提供理论支撑。【方法】考虑毛细管作用,根据甲... 【目的】海洋沉积物孔隙内部的毛细管作用可以升高水合物—水二相甲烷的溶解度,影响天然气水合物的分布。确定毛细管作用对水合物发育顶界的影响,可以为水合物的成藏演化研究及水合物勘察提供理论支撑。【方法】考虑毛细管作用,根据甲烷的质量守恒,建立了基于海底沉积物孔隙水硫酸根浓度计算水合物发育顶界深度的模型,利用数值模拟方法研究布莱克海台ODP994站位沉积物孔隙毛细管作用影响下的甲烷浓度分布和水合物发育顶界。【结果与结论】模拟计算显示考虑实际孔径计算的ODP994站位水合物发育顶界为194 m,与实际的水合物发育顶界深度一致。毛细管作用可以增大水合物—水二相甲烷溶解度,使生成水合物所需甲烷浓度升高。毛细管作用升高流体溶解的甲烷浓度,有利于甲烷运移到更浅的深度,可以使水合物发育顶界更浅。水合物顶界附近的局部的最大孔径沉积层具有更小的水合物-水二相甲烷溶解度,是水合物发育顶界优先发育位置。因此,确定水合物稳定带内的沉积物孔隙特征,是评估天然气水合物顶界的重要基础。 展开更多
关键词 毛细管作用 硫酸根甲烷界面 甲烷通量 水合物发育顶界 数值模拟
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澜沧江(云南段)水-气界面氧化亚氮释放通量时空分布特征及其影响因素研究
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作者 袁茜 傅开道 +2 位作者 陶雨晨 张年 杨丽莎 《生态环境学报》 CSCD 北大核心 2024年第1期54-61,共8页
温室气体浓度上升导致全球气候变暖已成为国际社会关注的焦点。氧化亚氮(N_(2)O)作为痕量温室气体,在全球气候变暖过程中扮演着重要的角色。河流和水库被认为是N_(2)O释放的活跃区域,然而目前研究多集中在对单一河流或水库的监测,对大... 温室气体浓度上升导致全球气候变暖已成为国际社会关注的焦点。氧化亚氮(N_(2)O)作为痕量温室气体,在全球气候变暖过程中扮演着重要的角色。河流和水库被认为是N_(2)O释放的活跃区域,然而目前研究多集中在对单一河流或水库的监测,对大范围河库系统的N_(2)O研究仍相对欠缺。选取澜沧江(云南段)流域作为考察对象,在2022年4月、8月采用悬浮箱采集24个点位的水-气界面的气体样品,并于实验室通过气象色谱仪检测气样氧化亚氮浓度,探究该流域干支流N_(2)O释放通量的时空分布特征;同时,测定了水体水环境参数,解析其时空差异的环境影响因素。结果表明,1)在时间尺度上,澜沧江(云南段)旱季N_(2)O通量均值低于雨季。旱季N_(2)O通量均值为0.10 mg·m^(-2)·d^(-1),雨季为0.18 mg·m^(-2)·d^(-1),其中旱季干流均值为0.11 mg·m^(-2)·d^(-1),支流为0.05 mg·m^(-2)·d^(-1);雨季干流均值为0.18 mg·m^(-2)·d^(-1),支流为0.15 mg·m^(-2)·d^(-1)。2)在空间尺度上,N_(2)O通量沿程整体呈现释放量递增的趋势。干流N_(2)O通量均值为0.15 mg·m^(-2)·d^(-1),支流为0.10 mg·m^(-2)·d^(-1),干流N_(2)O通量高于支流。水库坝上N_(2)O通量均值为0.02 mg·m^(-2)·d^(-1),坝下为0.31 mg·m^(-2)·d^(-1),水库坝下N_(2)O通量值是坝上的15.5倍,水库发电下泄高速水流加速了水-气界面N_(2)O释放。3)澜沧江水-气界面N_(2)O通量与水温(WT)(r=0.341,P=0.009)、氨氮(NH4^(+))(r=0.384,P=0.004)和流速(r=0.283,P=0.026)呈显著正相关关系,与溶解氧(DO)(r=-0.420,P=0.001)呈显著负相关关系,表明在高WT、低DO、高NH4^(+)和高流速条件下有利于N_(2)O产生与释放。研究结果揭示澜沧江(云南段)河库系统氧化亚氮释放通量时空分布特征以及影响因素,为流域温室气体排放评估提供数据支持和科学依据。 展开更多
关键词 澜沧江 氧化亚氮(N_(2)O) 释放通量 时空分布 影响因素 水-气界面
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南四湖出湖口沉积物-水界面中营养盐分布特征分析及释放风险评估
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作者 王津 杨丽原 +1 位作者 刘恩峰 栾日坚 《济南大学学报(自然科学版)》 CAS 北大核心 2024年第1期61-67,共7页
为了解决南四湖出湖口沉积物-水界面中磷酸盐、氨氮和硝态氮等营养盐释放风险控制缺乏科学依据的问题,利用薄膜扩散梯度技术、高分辨率孔隙水采样技术分析南四湖出湖口沉积物-水界面中营养盐浓度的垂直剖面分布特征,并根据有效态磷、有... 为了解决南四湖出湖口沉积物-水界面中磷酸盐、氨氮和硝态氮等营养盐释放风险控制缺乏科学依据的问题,利用薄膜扩散梯度技术、高分辨率孔隙水采样技术分析南四湖出湖口沉积物-水界面中营养盐浓度的垂直剖面分布特征,并根据有效态磷、有效态氨氮和有效态硝态氮的浓度,计算三者的净扩散通量,评估三者的释放风险。结果表明:非泄洪期南四湖出湖口上覆水中的溶解态磷浓度低于孔隙水中的,表明沉积物孔隙水中的溶解态磷可能会因浓度梯度的存在而向上覆水中扩散;根据连续分级提取法,钙结合态磷是南四湖出湖口沉积物中磷元素的主要赋存形态,表层沉积物中的不稳定磷元素含量高于深层沉积物中的;有效态磷与有效态铁呈显著正相关,说明南四湖出湖口沉积物-水界面中有效态磷的释放受铁氧化物还原释放影响;有效态磷、有效态氨氮和有效态硝态氮的净扩散通量分别为17.58、1.16、-40.72 ng/(cm^(2)·d),说明有效态磷和有效态氨氮有从沉积物向上覆水中释放的潜在风险。 展开更多
关键词 环境科学 净扩散通量 薄膜扩散梯度技术 营养盐 沉积物-水界面 南四湖
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Exchange fluxes of nutrients between sediment and sea water in the Bohai Sea
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作者 Liu Sumei, Zhang Jing, Zhang Hong, Yu Jianhua 1. College of Chemistry and Chemical Engineering, Ocean University of Qingdao, Qingdao 266003, China 2. State Key Laboratory of Estuarine and Coastal Research, East China Normal University, 3663 Zhongshanbei 《Acta Oceanologica Sinica》 SCIE CAS CSCD 2001年第3期363-370,共8页
Investigations of sediment-water fluxes of nutrients in the Bohai Sea were carried out in September - October 1998 and April - May 1999. The exchange fluxes of nutrients between sediment and sea water were determined ... Investigations of sediment-water fluxes of nutrients in the Bohai Sea were carried out in September - October 1998 and April - May 1999. The exchange fluxes of nutrients between sediment and sea water were determined by incubating the core-top sediments with overlying water aerated with air. The benthic fluxes of NO3- , NO2- , NH4+ , DIN, DON and TON in the first cruise and the flux-es of NO3 , NO2- , NH4+ , DIN, DON, TDN, PO43- , DOP and TDP in the second cruise were measured. The exchange fluxes of nutrients in fall were higher than in spring. The benthic nutrient fluxes represented 15% -55% of nutrient budgets in the Bohai Sea. 展开更多
关键词 flux NUTRIENTS sediment-water interface the Bohai Sea
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In situ measurements of benthic oxygen fluxes in Hui-quan Bay of Qingdao by eddy correlation techniques:short term pattern variations in gravel beach
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作者 CUI Shanggong YU Xinsheng ZHAO Guangtao 《Marine Science Bulletin》 CAS 2020年第2期36-52,共17页
The oxygen fluxe across the sediment-water interface(SWI)in coastal region is a key measure to fully understand the regulation of biogeochemical cycles in an aquatic environment.However,studies on fluxes of dissolved ... The oxygen fluxe across the sediment-water interface(SWI)in coastal region is a key measure to fully understand the regulation of biogeochemical cycles in an aquatic environment.However,studies on fluxes of dissolved oxygen in gravel beach are limited,because of the difficulty in sample collection and instrumentations deployment.In this study,benthic oxygen fluxes across rocky substratum in an intertidal zone of Huiquan Bay was estimated by using noninvasive eddy correlation techniques.A total of 10 burst measurements were analyzed.The oxygen flux fluctuated from-5.7888±2.6 to+49.3344±2.6 mmol O2 m-2/d were observed.The cospectra analysis showed that the oxygen flux at the frequency band between 0.093 and 0.279 Hz(at a period from 3.58 to 10.75 s)contributed 50.19%to the total spectrum on average.The results showed that the major contribution band moved to the high frequency region gradually and reached a steady state with increasing tidal flood.It is demonstrated that wave movement and wave breaking interaction resulted in the change of oxygen flux between gravel beach and shallow waters at the start and the end of a rising tide period,respectively.The eddy correlation techniques offer an efficient means for flux measurement over a gravel or mixed sand and gravel beaches. 展开更多
关键词 sediment-water interface(SWI) oxygen fluxes eddy correlation gravel beaches in situ measurement
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