A pore-array intensified tube-in-tube microchannel(PA-TMC),which is characterized by high throughput and low pressure drop,was developed as a gas–liquid contactor.The sulfite oxidation method was used to determine th...A pore-array intensified tube-in-tube microchannel(PA-TMC),which is characterized by high throughput and low pressure drop,was developed as a gas–liquid contactor.The sulfite oxidation method was used to determine the oxygen efficiency(φ)and volumetric mass transfer coefficient(k_(L)a)of PA-TMC,and the mass transfer amount per unit energy(ε)was calculated by using the pressure drop.The effects of structural and operating parameters were investigated systematically,and the twophase flow behavior was monitored by using a charge-coupled device imaging system.The results indicated that the gas absorption efficiency and mass transfer performance of the PA-TMC were improved with increasing pore number,flow rate,and number of helical coil turns and decreasing pore size,row number,annular size,annular length,and surface tension.Theφ,εand k La of PA-TMC could reach 31.3%,1.73×10^(-4) mol/J,and 7.0 s-1,respectively.The Sherwood number was correlated with the investigated parameters to guide the design of PA-TMC in gas absorption and mass transfer processes.展开更多
基金supported by National Key Research and Development Program(No.2016YFD0501402-04)National Natural Science Foundation of China(Nos.21776179,21621004)the Program for Changjiang Scholars and Innovative Research Team in University(No.IRT_15R46)。
文摘A pore-array intensified tube-in-tube microchannel(PA-TMC),which is characterized by high throughput and low pressure drop,was developed as a gas–liquid contactor.The sulfite oxidation method was used to determine the oxygen efficiency(φ)and volumetric mass transfer coefficient(k_(L)a)of PA-TMC,and the mass transfer amount per unit energy(ε)was calculated by using the pressure drop.The effects of structural and operating parameters were investigated systematically,and the twophase flow behavior was monitored by using a charge-coupled device imaging system.The results indicated that the gas absorption efficiency and mass transfer performance of the PA-TMC were improved with increasing pore number,flow rate,and number of helical coil turns and decreasing pore size,row number,annular size,annular length,and surface tension.Theφ,εand k La of PA-TMC could reach 31.3%,1.73×10^(-4) mol/J,and 7.0 s-1,respectively.The Sherwood number was correlated with the investigated parameters to guide the design of PA-TMC in gas absorption and mass transfer processes.
