Extensive experimental work on hysteresis in a c℃urrent gas-liquid upflow packed bed was carried out with three kinds of packings and the air-water system. However, only when packed with small glass beads ((1.4 mm) w...Extensive experimental work on hysteresis in a c℃urrent gas-liquid upflow packed bed was carried out with three kinds of packings and the air-water system. However, only when packed with small glass beads ((1.4 mm) was the bed pressure drop hysteresis observed. Two more liquids with different liquid properties were employed to further examine the influence of parameters on pressure drop hysteresis. The similarity of pressure drop hysteresis in packed beds was concluded in combination of experimental evidence reported in literature.展开更多
In recent years, antibiotic pollution has become a serious threat to human health. In this study, a gas-liquid discharge plasma is developed to degrade ciprofloxacin hydrochloride in a multiphase mixed system containi...In recent years, antibiotic pollution has become a serious threat to human health. In this study, a gas-liquid discharge plasma is developed to degrade ciprofloxacin hydrochloride in a multiphase mixed system containing inorganic and organic impurities. The discharge characteristics are analyzed by diagnosing the applied voltage and discharge current waveforms, as well as the optical emission spectra. The work investigates how degradation efficiency is affected by applied voltage, gas flow rate, treatment time, initial concentration as well as the addition of γ-Al_(2)O_(3) pellets and peanut straw. After 70 min, the degradation efficiency of ciprofloxacin hydrochloride in the multiphase mixed system reached 99.6%. Its removal efficiency increases as the initial concentration decreases and the applied voltage increases. Besides, there is still a good degradation efficiency of ciprofloxacin hydrochloride with the addition of peanut straw.The degradation mechanism of ciprofloxacin hydrochloride is investigated through the analysis of degraded intermediates and reactive species.展开更多
Conventional conductivity methods for measuring the void fraction in gas-liquid multiphase systems are typically affected by accuracy problems due to the presence of fluid flow and salinity.This study presents a novel...Conventional conductivity methods for measuring the void fraction in gas-liquid multiphase systems are typically affected by accuracy problems due to the presence of fluid flow and salinity.This study presents a novel approach for determining the void fraction based on a reciprocating dynamic conductivity probe used to measure the liquid film thickness under forced annular-flow conditions.The measurement system comprises a cyclone,a conductivity probe,a probe reciprocating device,and a data acquisition and processing system.This method ensures that the flow pattern is adjusted to a forced annular flow,thereby minimizing the influence of complex and variable gas-liquid flow patterns on the measurement results;Moreover,it determines the liquid film thickness solely according to circuit connectivity rather than specific conductivity values,thereby mitigating the impact of salinity.The reliability of the measurement system is demonstrated through laboratory experiments.The experimental results indicate that,in a range of gas phase superficial velocities 5–20 m/s and liquid phase superficial velocities 0.079–0.48 m/s,the maximum measurement deviation for the void fraction is 4.23%.展开更多
A new measurement device,consisting of swirling blades and capsule-shaped throttling elements,is proposed in this study to eliminate typical measurement errors caused by complex flow patterns in gas-liquid flow.The sw...A new measurement device,consisting of swirling blades and capsule-shaped throttling elements,is proposed in this study to eliminate typical measurement errors caused by complex flow patterns in gas-liquid flow.The swirling blades are used to transform the complex flow pattern into a forced annular flow.Drawing on the research of existing blockage flow meters and also exploiting the single-phase flow measurement theory,a formula is introduced to measure the phase-separated flow of gas and liquid.The formula requires the pressure ratio,Lockhart-Martinelli number(L-M number),and the gas phase Froude number.The unknown parameters appearing in the formula are fitted through numerical simulation using computational fluid dynamics(CFD),which involves a comprehensive analysis of the flow field inside the device from multiple perspectives,and takes into account the influence of pressure fluctuations.Finally,the measurement model is validated through an experimental error analysis.The results demonstrate that the measurement error can be maintained within±8%for various flow patterns,including stratified flow,bubble flow,and wave flow.展开更多
Plasma-catalysis is considered as one of the most promising technologies for antibiotic degradation in water.In the plasma-catalytic system,one of the factors affecting the degradation effect is the performance of the...Plasma-catalysis is considered as one of the most promising technologies for antibiotic degradation in water.In the plasma-catalytic system,one of the factors affecting the degradation effect is the performance of the photocatalyst,which is usually restricted by the rapid recombination of electrons and holes as well as narrow light absorption range.In this research,a photocatalyst g-C_(3)N_(4)/TiO_(2) was prepared and coupled with gas-liquid discharge(GLD)to degrade tetracycline(TC).The performance was examined,and the degradation pathways and mechanisms were studied.Results show that a 90%degradation rate is achieved in the GLD with g-C_(3)N_(4)/TiO_(2) over a 10 min treatment.Increasing the pulse voltage is conducive to increasing the degradation rate,whereas the addition of excessive g-C_(3)N_(4)/TiO_(2) tends to precipitate agglomerates,resulting in a poor degradation efficiency.The redox properties of the g-C_(3)N_(4)/TiO_(2) surface promote the generation of oxidizing active species(H2O2,O3)in solution.Radical quenching experiments showed that·OH,hole(h^(+)),play important roles in the TC degradation by the discharge with g-C_(3)N_(4)/TiO_(2).Two potential degradation pathways were proposed based on the intermediates.The toxicity of tetracycline was reduced by treatment in the system.Furthermore,the g-C_(3)N_(4)/TiO_(2) composites exhibited excellent recoverability and stability.展开更多
The wall wettability of microchannels plays an important role in the gas-liquid mass transfer dynamics under Taylor flow.In this study,we regulated the contact angle of the wall surface through surface chemical grafti...The wall wettability of microchannels plays an important role in the gas-liquid mass transfer dynamics under Taylor flow.In this study,we regulated the contact angle of the wall surface through surface chemical grafting polymerization under controlled experimental conditions.The dynamic changes of CO_(2)bubbles flowing along the microchannel were captured by a high-speed video camera mounted on a stereo microscope,whilst a unit cell model was employed to theoretically investigate the gas-liquid mass transfer dynamics.We quantitatively characterized the effects of wall wettability,specifically the contact angle,on the formation mechanism of gas bubbles and mass transfer process experimentally.The results revealed that the gas bubble velocity,the overall volumetric liquid phase mass transfer coefficients(kLa),and the specific interfacial area(a)all increased with the increase of the contact angle.Conversely,gas bubble length and leakage flow decreased.Furthermore,we proposed a new modified model to predict the gas-liquid two-phase mass transfer performance,based on van Baten’s and Yao’s models.Our proposed model was observed to agree reasonably well with experimental observations.展开更多
Accurate prediction of the frictional pressure drop is important for the design and operation of subsea oil and gas transporting system considering the length of the pipeline. The applicability of the correlations to ...Accurate prediction of the frictional pressure drop is important for the design and operation of subsea oil and gas transporting system considering the length of the pipeline. The applicability of the correlations to pipeline-riser flow needs evaluation since the flow condition in pipeline-riser is quite different from the original data where they were derived from. In the present study, a comprehensive evaluation of 24prevailing correlation in predicting frictional pressure drop is carried out based on experimentally measured data of air-water and air-oil two-phase flows in pipeline-riser. Experiments are performed in a system having different configuration of pipeline-riser with the inclination of the downcomer varied from-2°to-5°to investigated the effect of the elbow on the frictional pressure drop in the riser. The inlet gas velocity ranges from 0.03 to 6.2 m/s, and liquid velocity varies from 0.02 to 1.3 m/s. A total of885 experimental data points including 782 on air-water flows and 103 on air-oil flows are obtained and used to access the prediction ability of the correlations. Comparison of the predicted results with the measured data indicate that a majority of the investigated correlations under-predict the pressure drop on severe slugging. The result of this study highlights the requirement of new method considering the effect of pipe layout on the frictional pressure drop.展开更多
A self-priming pump is a centrifugal pump that has the ability to prime itself. Typically, its performance dependson the configuration of its reflux hole. In this study, the ANSYS FLUENT software is used to investigat...A self-priming pump is a centrifugal pump that has the ability to prime itself. Typically, its performance dependson the configuration of its reflux hole. In this study, the ANSYS FLUENT software is used to investigate the effectsof three different radial positions of the reflux hole on gas-liquid two-phase distribution, pressure pulsation, andimp during self-priming. The research results indicate that: (1) The effective channel size for the reflux liquid toenter the volute varies depending on the location of the reflux hole. The effect of the impeller rotation on thereflux liquid becomes more obvious as the setting distance of the reflux aperture decreases. (2) The position ofthe reflux hole significantly affects the gas phase mass fraction inside the impeller, resulting in a significant reductionin the time it takes for the mass fraction to exceed 80%. (3) The position of the reflux hole significantly affectsthe average pressure on each monitoring surface. (4) Placing the reflux hole at a excessively distant radial distancecan result in an excessive vertical component. (5) The self-priming performance of the pump can be improved tosome extent by placing the return hole at a small radial distance.展开更多
A new approach and a new related distribution system are proposed to address the issue of uneven steam injection caused by the different suction capacities of the used wells during the application of steam“stimulatio...A new approach and a new related distribution system are proposed to address the issue of uneven steam injection caused by the different suction capacities of the used wells during the application of steam“stimulation”methods for enhanced oil recovery.The new distribution system consists of a swirler,spiral dividing baffles,and critical flow nozzles.Numerical simulations are used to analyze the flow-field and degree of steam homogeneity obtained with such an approach.The results indicate that a higher inlet pressure leads to better results.Additionally,the internal flow field becomes more stable,and the deviation from an even distribution reduces to±4.0%even when the resistance of each branch is inconsistent.Furthermore,field tests have yielded satisfactory results.展开更多
Anammox was successfully transited from heterotrophic denitrification and autotrophic denitrification in two upflow biofilm reactors, respectively. The results showed that the volumetric loading rate and nitrogen remo...Anammox was successfully transited from heterotrophic denitrification and autotrophic denitrification in two upflow biofilm reactors, respectively. The results showed that the volumetric loading rate and nitrogen removal efficiency in the reactor transited from heterotrophic denitrification were higher than that in its counterpart. When the hydraulic retention time was 12 h or so, the total nitrogen loading rate was about 0.609 kg N/(m3·d), and the effluent ammonia and nitrite concentrations were less than 8.5 mg/L and 2.5 mg/L, respectively. The upflow anammox biofilm reactor was capable of keeping and accumulating the slow-growing bacteria efficiently. During operation of the reactor, the biomass color was gradually turned from brownish to red, and the ratio of ammonia consumption, nitrite consumption and nitrate production approached the theoretical one. These changes could be used as an indicator for working state of the reactor.展开更多
基金Supported by the National Natural Science Foundation of China (No.: 29676042)
文摘Extensive experimental work on hysteresis in a c℃urrent gas-liquid upflow packed bed was carried out with three kinds of packings and the air-water system. However, only when packed with small glass beads ((1.4 mm) was the bed pressure drop hysteresis observed. Two more liquids with different liquid properties were employed to further examine the influence of parameters on pressure drop hysteresis. The similarity of pressure drop hysteresis in packed beds was concluded in combination of experimental evidence reported in literature.
基金supported by National Natural Science Foundations of China (Nos. 52307163 and 12305279)the China Postdoctoral Science Foundation (Nos. 2023M740498 and 2022M710590)Postdoctoral Fellowship Program of CPSF (No. GZC20230348)。
文摘In recent years, antibiotic pollution has become a serious threat to human health. In this study, a gas-liquid discharge plasma is developed to degrade ciprofloxacin hydrochloride in a multiphase mixed system containing inorganic and organic impurities. The discharge characteristics are analyzed by diagnosing the applied voltage and discharge current waveforms, as well as the optical emission spectra. The work investigates how degradation efficiency is affected by applied voltage, gas flow rate, treatment time, initial concentration as well as the addition of γ-Al_(2)O_(3) pellets and peanut straw. After 70 min, the degradation efficiency of ciprofloxacin hydrochloride in the multiphase mixed system reached 99.6%. Its removal efficiency increases as the initial concentration decreases and the applied voltage increases. Besides, there is still a good degradation efficiency of ciprofloxacin hydrochloride with the addition of peanut straw.The degradation mechanism of ciprofloxacin hydrochloride is investigated through the analysis of degraded intermediates and reactive species.
基金the National Natural Science Foundation of China(No.62173049)the Open Fund of the Hubei Key Laboratory of Oil and Gas Drilling and Production Engineering(Yangtze University),YQZC202309.
文摘Conventional conductivity methods for measuring the void fraction in gas-liquid multiphase systems are typically affected by accuracy problems due to the presence of fluid flow and salinity.This study presents a novel approach for determining the void fraction based on a reciprocating dynamic conductivity probe used to measure the liquid film thickness under forced annular-flow conditions.The measurement system comprises a cyclone,a conductivity probe,a probe reciprocating device,and a data acquisition and processing system.This method ensures that the flow pattern is adjusted to a forced annular flow,thereby minimizing the influence of complex and variable gas-liquid flow patterns on the measurement results;Moreover,it determines the liquid film thickness solely according to circuit connectivity rather than specific conductivity values,thereby mitigating the impact of salinity.The reliability of the measurement system is demonstrated through laboratory experiments.The experimental results indicate that,in a range of gas phase superficial velocities 5–20 m/s and liquid phase superficial velocities 0.079–0.48 m/s,the maximum measurement deviation for the void fraction is 4.23%.
基金Supported By Open Fund of Hubei Key Laboratory of Oil and Gas Drilling and Production Engineering(Yangtze University),YQZC202309.
文摘A new measurement device,consisting of swirling blades and capsule-shaped throttling elements,is proposed in this study to eliminate typical measurement errors caused by complex flow patterns in gas-liquid flow.The swirling blades are used to transform the complex flow pattern into a forced annular flow.Drawing on the research of existing blockage flow meters and also exploiting the single-phase flow measurement theory,a formula is introduced to measure the phase-separated flow of gas and liquid.The formula requires the pressure ratio,Lockhart-Martinelli number(L-M number),and the gas phase Froude number.The unknown parameters appearing in the formula are fitted through numerical simulation using computational fluid dynamics(CFD),which involves a comprehensive analysis of the flow field inside the device from multiple perspectives,and takes into account the influence of pressure fluctuations.Finally,the measurement model is validated through an experimental error analysis.The results demonstrate that the measurement error can be maintained within±8%for various flow patterns,including stratified flow,bubble flow,and wave flow.
基金supported by National Natural Science Foundation of China(Nos.52277151 and 51907088)Innovative Talents Team Project of‘Six Talent Peaks’of Jiangsu Province(No.TD-JNHB-006).
文摘Plasma-catalysis is considered as one of the most promising technologies for antibiotic degradation in water.In the plasma-catalytic system,one of the factors affecting the degradation effect is the performance of the photocatalyst,which is usually restricted by the rapid recombination of electrons and holes as well as narrow light absorption range.In this research,a photocatalyst g-C_(3)N_(4)/TiO_(2) was prepared and coupled with gas-liquid discharge(GLD)to degrade tetracycline(TC).The performance was examined,and the degradation pathways and mechanisms were studied.Results show that a 90%degradation rate is achieved in the GLD with g-C_(3)N_(4)/TiO_(2) over a 10 min treatment.Increasing the pulse voltage is conducive to increasing the degradation rate,whereas the addition of excessive g-C_(3)N_(4)/TiO_(2) tends to precipitate agglomerates,resulting in a poor degradation efficiency.The redox properties of the g-C_(3)N_(4)/TiO_(2) surface promote the generation of oxidizing active species(H2O2,O3)in solution.Radical quenching experiments showed that·OH,hole(h^(+)),play important roles in the TC degradation by the discharge with g-C_(3)N_(4)/TiO_(2).Two potential degradation pathways were proposed based on the intermediates.The toxicity of tetracycline was reduced by treatment in the system.Furthermore,the g-C_(3)N_(4)/TiO_(2) composites exhibited excellent recoverability and stability.
基金the financial supports from National Natural Science Foundation of China(21978250,22208278)Natural Science Foundation of Shandong Province(ZR2020KB013,ZR2020QE211,2019KJC012).
文摘The wall wettability of microchannels plays an important role in the gas-liquid mass transfer dynamics under Taylor flow.In this study,we regulated the contact angle of the wall surface through surface chemical grafting polymerization under controlled experimental conditions.The dynamic changes of CO_(2)bubbles flowing along the microchannel were captured by a high-speed video camera mounted on a stereo microscope,whilst a unit cell model was employed to theoretically investigate the gas-liquid mass transfer dynamics.We quantitatively characterized the effects of wall wettability,specifically the contact angle,on the formation mechanism of gas bubbles and mass transfer process experimentally.The results revealed that the gas bubble velocity,the overall volumetric liquid phase mass transfer coefficients(kLa),and the specific interfacial area(a)all increased with the increase of the contact angle.Conversely,gas bubble length and leakage flow decreased.Furthermore,we proposed a new modified model to predict the gas-liquid two-phase mass transfer performance,based on van Baten’s and Yao’s models.Our proposed model was observed to agree reasonably well with experimental observations.
基金the support of the Opening Fund of State Key Laboratory of Multiphase Flow in Power Engineering(SKLMF-KF-2102)。
文摘Accurate prediction of the frictional pressure drop is important for the design and operation of subsea oil and gas transporting system considering the length of the pipeline. The applicability of the correlations to pipeline-riser flow needs evaluation since the flow condition in pipeline-riser is quite different from the original data where they were derived from. In the present study, a comprehensive evaluation of 24prevailing correlation in predicting frictional pressure drop is carried out based on experimentally measured data of air-water and air-oil two-phase flows in pipeline-riser. Experiments are performed in a system having different configuration of pipeline-riser with the inclination of the downcomer varied from-2°to-5°to investigated the effect of the elbow on the frictional pressure drop in the riser. The inlet gas velocity ranges from 0.03 to 6.2 m/s, and liquid velocity varies from 0.02 to 1.3 m/s. A total of885 experimental data points including 782 on air-water flows and 103 on air-oil flows are obtained and used to access the prediction ability of the correlations. Comparison of the predicted results with the measured data indicate that a majority of the investigated correlations under-predict the pressure drop on severe slugging. The result of this study highlights the requirement of new method considering the effect of pipe layout on the frictional pressure drop.
基金the National Natural Science Foundation of China(Research Project No.52169018).
文摘A self-priming pump is a centrifugal pump that has the ability to prime itself. Typically, its performance dependson the configuration of its reflux hole. In this study, the ANSYS FLUENT software is used to investigate the effectsof three different radial positions of the reflux hole on gas-liquid two-phase distribution, pressure pulsation, andimp during self-priming. The research results indicate that: (1) The effective channel size for the reflux liquid toenter the volute varies depending on the location of the reflux hole. The effect of the impeller rotation on thereflux liquid becomes more obvious as the setting distance of the reflux aperture decreases. (2) The position ofthe reflux hole significantly affects the gas phase mass fraction inside the impeller, resulting in a significant reductionin the time it takes for the mass fraction to exceed 80%. (3) The position of the reflux hole significantly affectsthe average pressure on each monitoring surface. (4) Placing the reflux hole at a excessively distant radial distancecan result in an excessive vertical component. (5) The self-priming performance of the pump can be improved tosome extent by placing the return hole at a small radial distance.
基金The authors would like to acknowledge the support provided by Supported By Open Fund of Hubei Key Laboratory of Oil and Gas Drilling and Production Engineering(Yangtze University),YQZC202309.
文摘A new approach and a new related distribution system are proposed to address the issue of uneven steam injection caused by the different suction capacities of the used wells during the application of steam“stimulation”methods for enhanced oil recovery.The new distribution system consists of a swirler,spiral dividing baffles,and critical flow nozzles.Numerical simulations are used to analyze the flow-field and degree of steam homogeneity obtained with such an approach.The results indicate that a higher inlet pressure leads to better results.Additionally,the internal flow field becomes more stable,and the deviation from an even distribution reduces to±4.0%even when the resistance of each branch is inconsistent.Furthermore,field tests have yielded satisfactory results.
基金TheNationalNaturalScienceFoundationofChina (No . 30 0 70 0 1 7) theScienceandTechnologyFoundationforKeyProjectofZhejiang
文摘Anammox was successfully transited from heterotrophic denitrification and autotrophic denitrification in two upflow biofilm reactors, respectively. The results showed that the volumetric loading rate and nitrogen removal efficiency in the reactor transited from heterotrophic denitrification were higher than that in its counterpart. When the hydraulic retention time was 12 h or so, the total nitrogen loading rate was about 0.609 kg N/(m3·d), and the effluent ammonia and nitrite concentrations were less than 8.5 mg/L and 2.5 mg/L, respectively. The upflow anammox biofilm reactor was capable of keeping and accumulating the slow-growing bacteria efficiently. During operation of the reactor, the biomass color was gradually turned from brownish to red, and the ratio of ammonia consumption, nitrite consumption and nitrate production approached the theoretical one. These changes could be used as an indicator for working state of the reactor.
