This paper is concerned with three-dimensional numerical simulation of a plunging liquid jet. The transient processes of forming an air cavity around the jet, capturing an initially large air bubble, and the break-up ...This paper is concerned with three-dimensional numerical simulation of a plunging liquid jet. The transient processes of forming an air cavity around the jet, capturing an initially large air bubble, and the break-up of this large toroidal-shaped bubble into smaller bubbles were analyzed. A stabilized finite element method (FEM) was employed under parallel numerical simulations based on adaptive, unstructured grid and coupled with a level-set method to track the interface between air and liquid. These simulations show that the inertia of the liquid jet initially depresses the pool's surface, forming an annular air cavity which surrounds the liquid jet. A toroidal liquid eddy which is subse- quently formed in the liquid pool results in air cavity collapse, and in turn entrains air into the liquid pool from the unstable annular air gap region around the liquid jet.展开更多
For the design and optimization of a tubular gas-liquid atomization mixer,the atomization and mixing characteristics of liquid jet breakup in the limited tube space is a key problem.In this study,the primary breakup p...For the design and optimization of a tubular gas-liquid atomization mixer,the atomization and mixing characteristics of liquid jet breakup in the limited tube space is a key problem.In this study,the primary breakup process of liquid jet columnwas analyzed by high-speed camera,then the droplet size and velocity distribution of atomized droplets were measured by Phase-Doppler anemometry(PDA).The hydrodynamic characteristics of gas flow in tubular gas-liquid atomization mixer were analyzed by computational fluid dynamics(CFD)numerical simulation.The results indicate that the liquid flow rate has little effect on the atomization droplet size and atomization pressure drop,and the gas flowrate is themain influence parameter.Under all experimental gas flowconditions,the liquid jet column undergoes a primary breakup process,forming larger liquid blocks and droplets.When the gas flow rate(Qg)is less than 127 m^(3)·h^(−1),the secondary breakup of large liquid blocks and droplets does not occur in venturi throat region.The Sauter mean diameter(SMD)of droplets measured at the outlet is more than 140μm,and the distribution is uneven.When Qg>127 m^(3)·h^(−1),the large liquid blocks and droplets have secondary breakup process at the throat region.The SMD of droplets measured at the outlet is less than 140μm,and the distribution is uniform.When 127<Qg<162m^(3)·h^(−1),the secondary breakup mode of droplets is bag breakup or pouch breakup.When 181<Qg<216m^(3)·h^(−1),the secondary breakup mode of droplets is shear breakup or catastrophic breakup.In order to ensure efficient atomization and mixing,the throat gas velocity of the tubular atomization mixer should be designed to be about 51 m·s^(−1) under the lowest operating flow rate.The pressure drop of the tubular atomization mixer increases linearly with the square of gas velocity,and the resistance coefficient is about 2.55 in single-phase flow condition and 2.73 in gas-liquid atomization condition.展开更多
This paper shows that a turned trochoidal function disturbance may lead to peripheral drops production. The resulting model is used to describe that a turned trochoidal disturbance leads to peripheral drops production...This paper shows that a turned trochoidal function disturbance may lead to peripheral drops production. The resulting model is used to describe that a turned trochoidal disturbance leads to peripheral drops production on the liquid jet surface without the necessity for superimposed disturbances. The trochoid is a non-unique parametric function. Only non-unique parametric functions disturbances may lead to peripheral drops production. The trochoidal function disturbance is decomposed to Fourier series. Every Fourier element receives an amplification factor in accordance to the Rayleigh inviscid jet model. Peripheral drops are received on the jet surface. The paper shows that all trochoidal disturbance functions, prolate cycloid, cycloid and curtate cycloid have a capability of peripheral drops producing. A limited capability of peripheral drops production is introduced for the trochoidal curtate cycloid. Produced drops size are reduced for increasing the jet velocity and wave number. Smaller drops are also received by transition from the prolate cycloid to curtate cycloid disturbance.展开更多
The skin friction and heat transfer occurring in the laminar boundary layerwhich caused by a vertical liquid jet impinging on a continuously moving horizontal plate werestudied. Similarity solutions for shear stress a...The skin friction and heat transfer occurring in the laminar boundary layerwhich caused by a vertical liquid jet impinging on a continuously moving horizontal plate werestudied. Similarity solutions for shear stress and heat distribution were obtained by using thehooting technique. The results show that the skin friction decreases with an increase of velocityparameter, the evolving of thermal boundary decrease with increasing in Prandtl number, but increasewith increasing of velocity parameter.展开更多
These experimental investigations are designed to study shock wave characteristics and spray structure. Supersonic liq- uid jets injected into ambient fields are empirically studied using projectile impacts in a two-s...These experimental investigations are designed to study shock wave characteristics and spray structure. Supersonic liq- uid jets injected into ambient fields are empirically studied using projectile impacts in a two-stage light gas gun. This study looks primarily at the design of the nozzle assembly, the tip velocity of the high speed jet, the structure of the spray jet and the shock wave generation process. The supersonic liquid jets were visualized using an ultra high-speed camera and the schlieren system for visualization to quantitatively analyze the shock wave angle. The experimental re- sults with straight cone nozzle types and various non-Newtonian fluid viscosities are presented in this paper. The effects of nozzle geometry on the jet behavior are described. The characteristics of the shock wave generation and spray jet structure were found to be significantly related to the nozzle geometry. The expansion gases accelerated the projectile, which had a mass of 6 grams, from 250 m/s. As a result, it was found that the maximum jet velocity appeared in the liquid jet with high viscosity properties. Supersonic liquid jets, which occurred at the leading edge the shock waves and the compression waves in front of the jets, were observed. Also, the shock waves significantly affected the atomization process for each spray droplet.展开更多
The hydrodynamic and mass transfer characteristics of a downflow liquid jet loop reactor (D-JLR) were studied experimentally with water/air and CMC (carboxymethyl cellulose) solution/air systems. The effects of the ge...The hydrodynamic and mass transfer characteristics of a downflow liquid jet loop reactor (D-JLR) were studied experimentally with water/air and CMC (carboxymethyl cellulose) solution/air systems. The effects of the geometry, the operating parameters and the physical properties of the liquid phase on gas hold-up and mass transfer coefficient were measuered. Compared with other types of gas-liquid reactor, D-JLR shows higher mass transfer coefficient and lower energy dissipation rate, the optimum diameter ratio was found to be about 0.42-0.6. A model for gas hold-up in D-JLR with Newtonian and non-Newtonian fluids has been developed on the basis of the equation of motion and the concept of average mixing length. The prediction of gas hold-up with the model agreed with the experimental results of this work.展开更多
Numerical simulations using volume of fluid(VOF)method are performed to study the impact of liquid-to-gas density ratio on the trajectory of nonturbulent liquid jets in gaseous crossflows.In this paper,large eddy simu...Numerical simulations using volume of fluid(VOF)method are performed to study the impact of liquid-to-gas density ratio on the trajectory of nonturbulent liquid jets in gaseous crossflows.In this paper,large eddy simulation(LES)turbulence model is coupled with the VOF method to describe the turbulence effects accurately.In addition,dynamic adaptive mesh refinement method with two refinement levels is applied to refine the size of the cells located at gas-liquid interface.Density ratio is changed from 10 to 5000 while other nondimensional numbers are kept constant.Large density ratios are considered in this paper since they are common in many practical applications such as solution precursor/suspension plasma sprays.Our simulations show that the penetration height,especially in the farfield,increases as the density ratio increases.A general correlation for the jet trajectory,which can be used for a wide range of density ratios,is developed based on our simulation results.展开更多
The capture,regeneration,and conversion of CO_(2) from ambient air and flue gas streams are critical aspects of mitigating global warming.Solid sorbents for CO_(2) absorption are very promising as they have high mass ...The capture,regeneration,and conversion of CO_(2) from ambient air and flue gas streams are critical aspects of mitigating global warming.Solid sorbents for CO_(2) absorption are very promising as they have high mass transfer areas without energy input and reduce emissions and minimize corrosion as compared to liquid sorbents.However,precisely tunable solid CO_(2) sorbents are difficult to produce.Here,we demonstrate the high-throughput production of hydrogel-based CO_(2)-absorbing particles via liquid jetting.By wrapping a liquid jet consisting of an aqueous solution of cross-linkable branched polyethylenimine(PEI)with a layer of suspension containing hydrophobic silica nanoparticles,monodisperse droplets with a silica nanoparticle coating layer was formed in the air.A stable Pickering emulsion containing PEI droplets was obtained after these ejected droplets were collected in a heated oil bath.The droplets turn into mm-sized particles after thermal curing in the bath.The diameter,PEI content,and silica content of the particles were systematically varied,and their CO_(2) absorption was measured as a function of time.Steam regeneration of the particles enabled cyclic testing,revealing a CO_(2) absorption capacity of 6.5±0.5 mol kg^(−1)solid PEI in pure CO_(2) environments and 0.7±0.3 mol kg^(−1)solid PEI for direct air capture.Several thousands of particles were produced per second at a rate of around 0.5 kg per hour,with a single nozzle.This process can be further scaled by parallelization.The complete toolbox for the design,fabrication,testing,and regeneration of functional hydrogel particles provides a powerful route toward novel solid sorbents for regenerative CO_(2) capture.展开更多
Penetration depth,spray dispersion angle,droplet sizes in breakup processes and atomization processes are very important parameters in combustor of air-breathing engine.These processes will enhance air/fuel mixing ins...Penetration depth,spray dispersion angle,droplet sizes in breakup processes and atomization processes are very important parameters in combustor of air-breathing engine.These processes will enhance air/fuel mixing inside the combustor.Experimental results from the pulsed air-assist liquid jet injected into a cross-flow are investigated.And experiments were conducted to a range of cross-flow velocities from 42~136 m/s.Air is injected with 0~300kPa,with air-assist pulsation frequency of 0~20Hz.Pulsation frequency was modulated by solenoid valve.Phase Doppler Particle Analyzer(PDPA) was utilized to quantitatively measuring droplet characteristics.High-speed CCD camera was used to obtain injected spray structure.Pulsed air-assist liquid jet will offer rapid mixing and good liquid jet penetration.Air-assist makes a very fine droplet which generated mist-like spray.Pulsed air-assist liquid jet will introduce additional supplementary turbulent mixing and control of penetration depth into a cross-flow field.The results show that pulsation frequency has an effect on penetration,transverse velocities and droplet sizes.The experimental data generated in these studies are used for a development of active control strategies to optimize the liquid jet penetration in subsonic cross-flow conditions and predict combustion low frequency instability.展开更多
The fluid mechanics in the generation of hyper veloeity water jets, light oiljets and glycerin jets was studied. Framing high-speed photography and single-shot photography wereused to observe the jets directly. The pu...The fluid mechanics in the generation of hyper veloeity water jets, light oiljets and glycerin jets was studied. Framing high-speed photography and single-shot photography wereused to observe the jets directly. The purposes of this study is to investigate the disintegrationand atomization processes at the velocity of 2km/s-3km/s as well as the auto-ignition andself-combustion of the light oil jets. Therefore, in the jet velocity measurement in addition to thehigh-speed photography, the results by other methods such as the laser beams cutting method and theshock wave detection using pressure transducers were also given. In the observation of the jetsevents, the illumination phenomenon was found, which may be regarded as the result of theauto-ignition and combustion of the light oil jets. Finally, the Munroe jet was studied.展开更多
A thin circular liquid sheet can be formed by impinging two identical round jets against each other. The liquid sheet expands to a certain critical radial distance and breaks. The unsteady process of the formation and...A thin circular liquid sheet can be formed by impinging two identical round jets against each other. The liquid sheet expands to a certain critical radial distance and breaks. The unsteady process of the formation and breakup of the liquid sheet in the ambient gas is simulated numerically. Both liquid and gas are treated as incompressible Newtonian fluids. The flow considered is axisymmetric. The liquid-gas interface is modeled with a level set function. A finite difference scheme is used to solve the governing Navier-Stokes equations with physical boundary conditions. The numerical results show how a thin circular sheet can be formed and break at its circular edge in slow motion. The sheet continues to thin as it expands radially. Hence, the Weber number decreases radially. The Weber number is defined as ρu 2 h/σ, where ρ and σ are, respectively, the liquid density and the surface tension, and u and h are, respectively, the average velocity and the half sheet thickness at a local radial location in the liquid sheet. The numerical results show that the sheet indeed terminates at a radial location, where the Weber number reaches one as observed in experiments. The spatio-temporal linear theory predicts that the breakup is initiated by the sinuous mode at the critical Weber number We c =1, below which the absolute instability occurs. The other independent mode called the varicose mode grows more slowly than the sinuous mode according to the linear theory. However, our numerical results show that the varicose mode actually overtakes the sinuous mode during the nonlinear evolution, and is responsible for the final breakup. The linear theory predicts the nature of disturbance waves correctly only at the onset of the instability, but cannot predict the exact consequence of the instability.展开更多
This paper describes the generation of pulsed, high-speed liquid jets usingthe cumulation method. This work mainly includes (1) the design of the nozzle assembly, (2) themeasurement of the jet velocity and (3) flow vi...This paper describes the generation of pulsed, high-speed liquid jets usingthe cumulation method. This work mainly includes (1) the design of the nozzle assembly, (2) themeasurement of the jet velocity and (3) flow visualization of the injection sequences. Thecumulation method can be briefly described as the liquid being accelerated first by the impact of amoving projectile and then further after it enters a converging section. The experimental resultsshow that the cumulation method is useful in obtaining a liquid jet with high velocity. The flowvisulization shows the roles of the Rayleigh-Tay-lor and Kelvin-Helmholtz instabilities in thebreakup of the liquid depend on the jet diameter and the downstream distance. When the liquid jetfront is far downstream from the nozzle exit, the jet is decelerated by air drag. Meanwhile, largecoherent vortex structures are formed surrounding the jet. The liquid will break up totally by theaction of these vortices. Experimental results showing the effect of the liquid volume on the jetvelocity are also included in this paper. Finally, a method for measuring the jet velocity bycutting two carbon rods is examined.展开更多
A high-resolution testing technique named liquid crystal thermography is used for the experimental study on jet array impingement to map out the distribution of heat transfer coefficients on the cooling surface. Effec...A high-resolution testing technique named liquid crystal thermography is used for the experimental study on jet array impingement to map out the distribution of heat transfer coefficients on the cooling surface. Effects of the impingement distance, the impinging hole arrangement and the initial crossflow on heat transfer characteristics are investigated. The thermal images show truly the features of local heat transfer for each jet impingement cooling. The applications of thermochromic liquid crystal are successful in the qualitative and quantitative measurement for heat transfer coefficients distribution.展开更多
To address the high rock strength and low drilling rate issues in deep oil/gas and geothermal exploitation, we performed mechanical property tests on three kinds of rock samples(granite, shale and sandstone) subjected...To address the high rock strength and low drilling rate issues in deep oil/gas and geothermal exploitation, we performed mechanical property tests on three kinds of rock samples(granite, shale and sandstone) subjected to liquid nitrogen(LN2) cooling and conducted rock-breaking experiments using LN2 jet. Rock-breaking characteristics and mechanisms of LN2 jet, heat transfer features between LN2 and rock and thermal stress evolution in rock were analyzed. A novel high-pressure LN2 jet assisted drilling method was proposed accordingly. The study results show that LN2 thermal shock can significantly reduce uniaxial compression strength and elastic modulus of rock. Rock damage and corresponding mechanical deterioration become more pronounced with increasing rock temperature. The LN2 jet has merits of high rock-breaking efficiency and low threshold rock-breaking pressure. Rock failure under LN2 jet impact is characterized by large volume breakage and the rock-breaking performance becomes more significant with increase of rock temperature. Under the impact of LN2 jet, the damage of granite is the most remarkable among the three rock samples. Thus, this method works better for high temperature granite formations. It has a good application prospect in speeding up drilling rate in deep hot dry rock geothermal reservoirs.展开更多
Both experimental and numerical studies were presented on the flow field characteristics in the process of gaseous jet impinging on liquid–water column. The effects of the impinging process on the working performance...Both experimental and numerical studies were presented on the flow field characteristics in the process of gaseous jet impinging on liquid–water column. The effects of the impinging process on the working performance of rocket engine were also analyzed. The experimental results showed that the liquid–water had better flame and smoke dissipation effect in the process of gaseous jet impinging on liquid–water column. However, the interaction between the gaseous jet and the liquid–water column resulted in two pressure oscillations with large amplitude appearing in the combustion chamber of the rocket engine with instantaneous pressure increased by 17.73% and 17.93%, respectively. To analyze the phenomena, a new computational method was proposed by coupling the governing equations of the MIXTURE model with the phase change equations of water and the combustion equation of propellant. Numerical simulations were carried out on the generation of gas, the accelerate gas flow, and the mutual interaction between gaseous jet and liquid–water column.Numerical simulations showed that a cavity would be formed in the liquid–water column when gaseous jet impinged on the liquid–water column. The development speed of the cavity increased obviously after each pressure oscillation. In the initial stage of impingement, the gaseous jet was blocked due to the inertia effect of high-density water, and a large amount of gas gathered in the area between the nozzle throat and the gas–liquid interface. The shock wave was formed in the nozzle expansion section. Under the dual action of the reverse pressure wave and the continuously ejected high-temperature gas upstream, the shock wave moved repeatedly in the nozzle expansion section, which led to the flow of gas in the combustion chamber being blocked, released, re-blocked, and re-released. This was also the main reason for the pressure oscillations in the combustion chamber.展开更多
The water-air and Wood’s metal-air systems are modeled by means of Computational Fluid Dynamics to study the interaction between a liquid surface and an impinging air jet under the near field blowing conditions. The ...The water-air and Wood’s metal-air systems are modeled by means of Computational Fluid Dynamics to study the interaction between a liquid surface and an impinging air jet under the near field blowing conditions. The effect of the air jet velocity, the height of the injection lance, and the density of the liquid on the depth of the formed cavity is numerically studied. The CFD results of the cavity depth are compared with results previously reported by other authors. The emergence of the splashing phenomenon is predicted in terms of the critical velocity for each liquid-air system. Besides, the blowing number indicates that the drop generation rate is not significant for jet velocities below the critical velocity, and therefore neither the splashing is significant.展开更多
基金supported by the Office of Naval Research(Grant ONRDC14292111)
文摘This paper is concerned with three-dimensional numerical simulation of a plunging liquid jet. The transient processes of forming an air cavity around the jet, capturing an initially large air bubble, and the break-up of this large toroidal-shaped bubble into smaller bubbles were analyzed. A stabilized finite element method (FEM) was employed under parallel numerical simulations based on adaptive, unstructured grid and coupled with a level-set method to track the interface between air and liquid. These simulations show that the inertia of the liquid jet initially depresses the pool's surface, forming an annular air cavity which surrounds the liquid jet. A toroidal liquid eddy which is subse- quently formed in the liquid pool results in air cavity collapse, and in turn entrains air into the liquid pool from the unstable annular air gap region around the liquid jet.
基金The financial supports from the National Natural Science Foundation of China(21808015)the Project of Construction of Innovative Teams and Teacher Career Development for Universities and Colleges under Beijing Municipality(IDHT20170507)。
文摘For the design and optimization of a tubular gas-liquid atomization mixer,the atomization and mixing characteristics of liquid jet breakup in the limited tube space is a key problem.In this study,the primary breakup process of liquid jet columnwas analyzed by high-speed camera,then the droplet size and velocity distribution of atomized droplets were measured by Phase-Doppler anemometry(PDA).The hydrodynamic characteristics of gas flow in tubular gas-liquid atomization mixer were analyzed by computational fluid dynamics(CFD)numerical simulation.The results indicate that the liquid flow rate has little effect on the atomization droplet size and atomization pressure drop,and the gas flowrate is themain influence parameter.Under all experimental gas flowconditions,the liquid jet column undergoes a primary breakup process,forming larger liquid blocks and droplets.When the gas flow rate(Qg)is less than 127 m^(3)·h^(−1),the secondary breakup of large liquid blocks and droplets does not occur in venturi throat region.The Sauter mean diameter(SMD)of droplets measured at the outlet is more than 140μm,and the distribution is uneven.When Qg>127 m^(3)·h^(−1),the large liquid blocks and droplets have secondary breakup process at the throat region.The SMD of droplets measured at the outlet is less than 140μm,and the distribution is uniform.When 127<Qg<162m^(3)·h^(−1),the secondary breakup mode of droplets is bag breakup or pouch breakup.When 181<Qg<216m^(3)·h^(−1),the secondary breakup mode of droplets is shear breakup or catastrophic breakup.In order to ensure efficient atomization and mixing,the throat gas velocity of the tubular atomization mixer should be designed to be about 51 m·s^(−1) under the lowest operating flow rate.The pressure drop of the tubular atomization mixer increases linearly with the square of gas velocity,and the resistance coefficient is about 2.55 in single-phase flow condition and 2.73 in gas-liquid atomization condition.
文摘This paper shows that a turned trochoidal function disturbance may lead to peripheral drops production. The resulting model is used to describe that a turned trochoidal disturbance leads to peripheral drops production on the liquid jet surface without the necessity for superimposed disturbances. The trochoid is a non-unique parametric function. Only non-unique parametric functions disturbances may lead to peripheral drops production. The trochoidal function disturbance is decomposed to Fourier series. Every Fourier element receives an amplification factor in accordance to the Rayleigh inviscid jet model. Peripheral drops are received on the jet surface. The paper shows that all trochoidal disturbance functions, prolate cycloid, cycloid and curtate cycloid have a capability of peripheral drops producing. A limited capability of peripheral drops production is introduced for the trochoidal curtate cycloid. Produced drops size are reduced for increasing the jet velocity and wave number. Smaller drops are also received by transition from the prolate cycloid to curtate cycloid disturbance.
基金[This work was financially supported by "973" key foundation of China (No.G 1998061510).]
文摘The skin friction and heat transfer occurring in the laminar boundary layerwhich caused by a vertical liquid jet impinging on a continuously moving horizontal plate werestudied. Similarity solutions for shear stress and heat distribution were obtained by using thehooting technique. The results show that the skin friction decreases with an increase of velocityparameter, the evolving of thermal boundary decrease with increasing in Prandtl number, but increasewith increasing of velocity parameter.
文摘These experimental investigations are designed to study shock wave characteristics and spray structure. Supersonic liq- uid jets injected into ambient fields are empirically studied using projectile impacts in a two-stage light gas gun. This study looks primarily at the design of the nozzle assembly, the tip velocity of the high speed jet, the structure of the spray jet and the shock wave generation process. The supersonic liquid jets were visualized using an ultra high-speed camera and the schlieren system for visualization to quantitatively analyze the shock wave angle. The experimental re- sults with straight cone nozzle types and various non-Newtonian fluid viscosities are presented in this paper. The effects of nozzle geometry on the jet behavior are described. The characteristics of the shock wave generation and spray jet structure were found to be significantly related to the nozzle geometry. The expansion gases accelerated the projectile, which had a mass of 6 grams, from 250 m/s. As a result, it was found that the maximum jet velocity appeared in the liquid jet with high viscosity properties. Supersonic liquid jets, which occurred at the leading edge the shock waves and the compression waves in front of the jets, were observed. Also, the shock waves significantly affected the atomization process for each spray droplet.
文摘The hydrodynamic and mass transfer characteristics of a downflow liquid jet loop reactor (D-JLR) were studied experimentally with water/air and CMC (carboxymethyl cellulose) solution/air systems. The effects of the geometry, the operating parameters and the physical properties of the liquid phase on gas hold-up and mass transfer coefficient were measuered. Compared with other types of gas-liquid reactor, D-JLR shows higher mass transfer coefficient and lower energy dissipation rate, the optimum diameter ratio was found to be about 0.42-0.6. A model for gas hold-up in D-JLR with Newtonian and non-Newtonian fluids has been developed on the basis of the equation of motion and the concept of average mixing length. The prediction of gas hold-up with the model agreed with the experimental results of this work.
文摘Numerical simulations using volume of fluid(VOF)method are performed to study the impact of liquid-to-gas density ratio on the trajectory of nonturbulent liquid jets in gaseous crossflows.In this paper,large eddy simulation(LES)turbulence model is coupled with the VOF method to describe the turbulence effects accurately.In addition,dynamic adaptive mesh refinement method with two refinement levels is applied to refine the size of the cells located at gas-liquid interface.Density ratio is changed from 10 to 5000 while other nondimensional numbers are kept constant.Large density ratios are considered in this paper since they are common in many practical applications such as solution precursor/suspension plasma sprays.Our simulations show that the penetration height,especially in the farfield,increases as the density ratio increases.A general correlation for the jet trajectory,which can be used for a wide range of density ratios,is developed based on our simulation results.
基金supported by the European Regional Development Fund(CONTROL,EFRO#00943).
文摘The capture,regeneration,and conversion of CO_(2) from ambient air and flue gas streams are critical aspects of mitigating global warming.Solid sorbents for CO_(2) absorption are very promising as they have high mass transfer areas without energy input and reduce emissions and minimize corrosion as compared to liquid sorbents.However,precisely tunable solid CO_(2) sorbents are difficult to produce.Here,we demonstrate the high-throughput production of hydrogel-based CO_(2)-absorbing particles via liquid jetting.By wrapping a liquid jet consisting of an aqueous solution of cross-linkable branched polyethylenimine(PEI)with a layer of suspension containing hydrophobic silica nanoparticles,monodisperse droplets with a silica nanoparticle coating layer was formed in the air.A stable Pickering emulsion containing PEI droplets was obtained after these ejected droplets were collected in a heated oil bath.The droplets turn into mm-sized particles after thermal curing in the bath.The diameter,PEI content,and silica content of the particles were systematically varied,and their CO_(2) absorption was measured as a function of time.Steam regeneration of the particles enabled cyclic testing,revealing a CO_(2) absorption capacity of 6.5±0.5 mol kg^(−1)solid PEI in pure CO_(2) environments and 0.7±0.3 mol kg^(−1)solid PEI for direct air capture.Several thousands of particles were produced per second at a rate of around 0.5 kg per hour,with a single nozzle.This process can be further scaled by parallelization.The complete toolbox for the design,fabrication,testing,and regeneration of functional hydrogel particles provides a powerful route toward novel solid sorbents for regenerative CO_(2) capture.
基金supported by the Korea Research Foundation Grant funded by the Korean Government (MOEHRD,Basic Research Promotion Fund) (KRF-2007-D00084)
文摘Penetration depth,spray dispersion angle,droplet sizes in breakup processes and atomization processes are very important parameters in combustor of air-breathing engine.These processes will enhance air/fuel mixing inside the combustor.Experimental results from the pulsed air-assist liquid jet injected into a cross-flow are investigated.And experiments were conducted to a range of cross-flow velocities from 42~136 m/s.Air is injected with 0~300kPa,with air-assist pulsation frequency of 0~20Hz.Pulsation frequency was modulated by solenoid valve.Phase Doppler Particle Analyzer(PDPA) was utilized to quantitatively measuring droplet characteristics.High-speed CCD camera was used to obtain injected spray structure.Pulsed air-assist liquid jet will offer rapid mixing and good liquid jet penetration.Air-assist makes a very fine droplet which generated mist-like spray.Pulsed air-assist liquid jet will introduce additional supplementary turbulent mixing and control of penetration depth into a cross-flow field.The results show that pulsation frequency has an effect on penetration,transverse velocities and droplet sizes.The experimental data generated in these studies are used for a development of active control strategies to optimize the liquid jet penetration in subsonic cross-flow conditions and predict combustion low frequency instability.
基金Project partly supported by the "Bairen" Plan of Chinese Academy of Sciences. (Grant No: 11442301301)
文摘The fluid mechanics in the generation of hyper veloeity water jets, light oiljets and glycerin jets was studied. Framing high-speed photography and single-shot photography wereused to observe the jets directly. The purposes of this study is to investigate the disintegrationand atomization processes at the velocity of 2km/s-3km/s as well as the auto-ignition andself-combustion of the light oil jets. Therefore, in the jet velocity measurement in addition to thehigh-speed photography, the results by other methods such as the laser beams cutting method and theshock wave detection using pressure transducers were also given. In the observation of the jetsevents, the illumination phenomenon was found, which may be regarded as the result of theauto-ignition and combustion of the light oil jets. Finally, the Munroe jet was studied.
基金Project supported by the National Natural Science Foundation of China (Nos. 10702038 and10772107)the National Science Foundation of USA (No. CTS-0138057)+1 种基金the Foundation of Science and Technology Commission of Shanghai Municipality (No. 09DZ1141502)the ShanghaiLeading Academic Discipline Project (No. Y0103)
文摘A thin circular liquid sheet can be formed by impinging two identical round jets against each other. The liquid sheet expands to a certain critical radial distance and breaks. The unsteady process of the formation and breakup of the liquid sheet in the ambient gas is simulated numerically. Both liquid and gas are treated as incompressible Newtonian fluids. The flow considered is axisymmetric. The liquid-gas interface is modeled with a level set function. A finite difference scheme is used to solve the governing Navier-Stokes equations with physical boundary conditions. The numerical results show how a thin circular sheet can be formed and break at its circular edge in slow motion. The sheet continues to thin as it expands radially. Hence, the Weber number decreases radially. The Weber number is defined as ρu 2 h/σ, where ρ and σ are, respectively, the liquid density and the surface tension, and u and h are, respectively, the average velocity and the half sheet thickness at a local radial location in the liquid sheet. The numerical results show that the sheet indeed terminates at a radial location, where the Weber number reaches one as observed in experiments. The spatio-temporal linear theory predicts that the breakup is initiated by the sinuous mode at the critical Weber number We c =1, below which the absolute instability occurs. The other independent mode called the varicose mode grows more slowly than the sinuous mode according to the linear theory. However, our numerical results show that the varicose mode actually overtakes the sinuous mode during the nonlinear evolution, and is responsible for the final breakup. The linear theory predicts the nature of disturbance waves correctly only at the onset of the instability, but cannot predict the exact consequence of the instability.
文摘This paper describes the generation of pulsed, high-speed liquid jets usingthe cumulation method. This work mainly includes (1) the design of the nozzle assembly, (2) themeasurement of the jet velocity and (3) flow visualization of the injection sequences. Thecumulation method can be briefly described as the liquid being accelerated first by the impact of amoving projectile and then further after it enters a converging section. The experimental resultsshow that the cumulation method is useful in obtaining a liquid jet with high velocity. The flowvisulization shows the roles of the Rayleigh-Tay-lor and Kelvin-Helmholtz instabilities in thebreakup of the liquid depend on the jet diameter and the downstream distance. When the liquid jetfront is far downstream from the nozzle exit, the jet is decelerated by air drag. Meanwhile, largecoherent vortex structures are formed surrounding the jet. The liquid will break up totally by theaction of these vortices. Experimental results showing the effect of the liquid volume on the jetvelocity are also included in this paper. Finally, a method for measuring the jet velocity bycutting two carbon rods is examined.
文摘A high-resolution testing technique named liquid crystal thermography is used for the experimental study on jet array impingement to map out the distribution of heat transfer coefficients on the cooling surface. Effects of the impingement distance, the impinging hole arrangement and the initial crossflow on heat transfer characteristics are investigated. The thermal images show truly the features of local heat transfer for each jet impingement cooling. The applications of thermochromic liquid crystal are successful in the qualitative and quantitative measurement for heat transfer coefficients distribution.
基金Supported by National Science Fund for Distinguished Young Scholars(NO.51725404)Program of Introducing Talents of Discipline to Chinese Universities(NO.B17045)National Natural Science Foundation of China(NO.51521063)
文摘To address the high rock strength and low drilling rate issues in deep oil/gas and geothermal exploitation, we performed mechanical property tests on three kinds of rock samples(granite, shale and sandstone) subjected to liquid nitrogen(LN2) cooling and conducted rock-breaking experiments using LN2 jet. Rock-breaking characteristics and mechanisms of LN2 jet, heat transfer features between LN2 and rock and thermal stress evolution in rock were analyzed. A novel high-pressure LN2 jet assisted drilling method was proposed accordingly. The study results show that LN2 thermal shock can significantly reduce uniaxial compression strength and elastic modulus of rock. Rock damage and corresponding mechanical deterioration become more pronounced with increasing rock temperature. The LN2 jet has merits of high rock-breaking efficiency and low threshold rock-breaking pressure. Rock failure under LN2 jet impact is characterized by large volume breakage and the rock-breaking performance becomes more significant with increase of rock temperature. Under the impact of LN2 jet, the damage of granite is the most remarkable among the three rock samples. Thus, this method works better for high temperature granite formations. It has a good application prospect in speeding up drilling rate in deep hot dry rock geothermal reservoirs.
基金Project supported by the National Natural Science Foundation of China(Grant No.51305204)
文摘Both experimental and numerical studies were presented on the flow field characteristics in the process of gaseous jet impinging on liquid–water column. The effects of the impinging process on the working performance of rocket engine were also analyzed. The experimental results showed that the liquid–water had better flame and smoke dissipation effect in the process of gaseous jet impinging on liquid–water column. However, the interaction between the gaseous jet and the liquid–water column resulted in two pressure oscillations with large amplitude appearing in the combustion chamber of the rocket engine with instantaneous pressure increased by 17.73% and 17.93%, respectively. To analyze the phenomena, a new computational method was proposed by coupling the governing equations of the MIXTURE model with the phase change equations of water and the combustion equation of propellant. Numerical simulations were carried out on the generation of gas, the accelerate gas flow, and the mutual interaction between gaseous jet and liquid–water column.Numerical simulations showed that a cavity would be formed in the liquid–water column when gaseous jet impinged on the liquid–water column. The development speed of the cavity increased obviously after each pressure oscillation. In the initial stage of impingement, the gaseous jet was blocked due to the inertia effect of high-density water, and a large amount of gas gathered in the area between the nozzle throat and the gas–liquid interface. The shock wave was formed in the nozzle expansion section. Under the dual action of the reverse pressure wave and the continuously ejected high-temperature gas upstream, the shock wave moved repeatedly in the nozzle expansion section, which led to the flow of gas in the combustion chamber being blocked, released, re-blocked, and re-released. This was also the main reason for the pressure oscillations in the combustion chamber.
文摘The water-air and Wood’s metal-air systems are modeled by means of Computational Fluid Dynamics to study the interaction between a liquid surface and an impinging air jet under the near field blowing conditions. The effect of the air jet velocity, the height of the injection lance, and the density of the liquid on the depth of the formed cavity is numerically studied. The CFD results of the cavity depth are compared with results previously reported by other authors. The emergence of the splashing phenomenon is predicted in terms of the critical velocity for each liquid-air system. Besides, the blowing number indicates that the drop generation rate is not significant for jet velocities below the critical velocity, and therefore neither the splashing is significant.