In the application of the physical iterative method to retrieve millimeter-wave radar liquid water content(LWC)and liquid water path(LWP),particle parameter scheme is the main factor affecting retrieval performance.In...In the application of the physical iterative method to retrieve millimeter-wave radar liquid water content(LWC)and liquid water path(LWP),particle parameter scheme is the main factor affecting retrieval performance.In this paper,synchronous measurements of an airborne millimeter-wave radar and a hot-wire probe in stratus cloud are used to compare the LWC retrievals of the oceanic and continental particle parameter scheme with diameter less than 50μm and the particle parameter scheme with diameter less than 500μm and 1500μm(scheme 1,scheme 2,scheme 3,and scheme4,respectively).The results show that the particle parameter scheme needs to be selected according to the reflectivity factor when using the physical iterative method to retrieve the LWC and LWP.When the reflectivity factor is less than-30 d BZ,the retrieval error of scheme 1 is the minimum.When the reflectivity factor is greater than-30 d BZ,the retrieval error of scheme 4 is the minimum.Based on the reflectance factor value,the LWP retrievals of scheme 4 are closer to the measurements,the average relative bias is 5.2%,and the minimum relative bias is 4.4%.Compared with other schemes,scheme 4 seems to be more useful for the LWC and LWP retrieval of stratus cloud in China.展开更多
On March 16–17, 2008, a sea fog occurred in Dianbai in the west of Guangdong Province and was accompanied by a high-pressure synoptic system. Using comprehensive observation datasets, this study analyzes the evolutio...On March 16–17, 2008, a sea fog occurred in Dianbai in the west of Guangdong Province and was accompanied by a high-pressure synoptic system. Using comprehensive observation datasets, this study analyzes the evolution of liquid water content during this sea fog and investigates the relationships between liquid water content and the average diameters and count densities of fog droplets, air temperature, wind speed and turbulence exchanges. The main results are presented as follows. (1) The sea fog showed a quasi-periodic oscillation characteristic, i.e., it developed, disappeared and then developed again. (2) During the sea fog, the number of fog droplets changed significantly while the changes in average diameter of the fog droplets were relatively small. The development and disappearance of the sea fog correlated significantly with the fog droplet numbers. (3) The air-cooling mechanism played a significant role in sea fog formation and development. However, the influences of this mechanism were not evident during fog persistence. (4) During sea fog formation, weak turbulence exchanges were helpful for fog formation. During sea fog development and persistence, liquid water content increased when turbulence exchanges weakened, and vice versa. The changes in turbulence exchanges were closely related to the quasi-periodic oscillations observed in sea fog presence.展开更多
In order to research the influence of liquid water content ( LWC ) on blade icing of wind turbine, a numerical simulation method for blade icing was established. The numerical simulation was based on low speed viscous...In order to research the influence of liquid water content ( LWC ) on blade icing of wind turbine, a numerical simulation method for blade icing was established. The numerical simulation was based on low speed viscous N-S equation. The trajectory equation of water droplets was established by Lagrangian method. The mass and energy conservation equations of the water droplets impacting on the surface of the blade were solved based on control body theory. Three sections along blade span wise of a 1.5 MW wind turbine were decided to simulate icing. Five kinds of LWC were selected for simulation including 0.2,0.4,0.6,0.8 and 1.0 g/m^3 under two ambient temperatures of -10 ℃ and -20 ℃. The medium volume droplet diameter ( MVD ) was 30μm. The simulations included icing shape on blade surface, dimensionless icing area and dimensionless maximum stagnation thickness. Furthermore, the flow fields around both the iced blade airfoil and the original one were simulated and analyzed. Accor-ding to the results, the typical icing characteristics of icing shape, icing area and thickness were greatly affected by the difference of LWCs. This study can provide theoretical reference for the research on antiicing and deicing of wind turbine blade.展开更多
In this paper, some features of cloud liquid water content with respect to rain and water vapor are presented. Cloud liquid water density profile is obtained from radiosonde observation with Salonen's model and Ka...In this paper, some features of cloud liquid water content with respect to rain and water vapor are presented. Cloud liquid water density profile is obtained from radiosonde observation with Salonen's model and Karsten's model at Kolkata, a tropical location in the Indian region. Cloud liquid water contents (LWC) are obtained from these profiles which show a prominent seasonal variation. The monsoon months exhibit much higher values of LWC than in other months. However Salonen's model yields higher LWC values than that obtained with Karsten's model. The variation of daily total rainfall with LWC shows a positive relationship indicating the role of LWC in controlling the rainfall. Also the variation pattern of LWC with integrated water vapor (IWV) content of the atmosphere indicates that a threshold value of water vapor is required for cloud to form and once cloud is formed LWC increases with IWV.展开更多
In this paper, some distinctive features of the vertical profile of precipitable liquid water content (LWC) with considerable respect to rain rates (R) and radar reflectivity (Z) obtained in a tropical location are pr...In this paper, some distinctive features of the vertical profile of precipitable liquid water content (LWC) with considerable respect to rain rates (R) and radar reflectivity (Z) obtained in a tropical location are presented. Assessment of LWC allows applications in the specific area of flight icing severity, aviation safety as well as signals traversing through the atmosphere. The parameters were typically measured using vertically-pointing Micro Rain Radar (MRR) over a period of 2 years (2011-2012) at Akure, a tropical location of Nigeria. The radar scanned at every 10 seconds and integrated over one minute samples to reduce event logging error associated with the instrument. The vertical profile of the LWC typically reveals a prominent seasonal variation. However, majority of the LWC profiles has low LWC, less than 0.1 gm?3 while the maximum observed LWC is about 3.18 gm?3. A strong like hood relation was observed between the melting layer height and the LWC, with the LWC reaches peak at the considerable height of about 4160 m which coincides precisely with the freezing height level (rain height of ~4520 m) of the study location. Good correlation was also observed between the LWC and R in most of the heights considered. The results obtained will assist system engineers to assess the level of absorption, reflection and attenuation of electromagnetic signals as a result of precipitable LWC along the transmitting paths. The novelty of the present work is in the area of linking LWC and Z as against usual relation between Z and R.展开更多
A retrieval method of microwave(MW)space-borne remote sensing of cloud liquid water content by the combined radar-radiometer is suggested.A three-layer cloud model is chosen to represent the typical stratified precipi...A retrieval method of microwave(MW)space-borne remote sensing of cloud liquid water content by the combined radar-radiometer is suggested.A three-layer cloud model is chosen to represent the typical stratified precipitating cloud.The retrieval method mainly follows our previously suggested scheme with some modifications.Numerical comparative study shows that in space-borne remote sensing of cloud liquid water content by the combined method is much better than by radar only;Also the retrieval accuracy of cloud liquid water content may be improved when using the three-layer cloud model in the combined method.展开更多
Water in room temperature ionic liquids(RTILs) could impose significant effects on their interfacial properties at a charged surface. Although the interfaces between RTILs and mica surfaces exhibit rich microstructure...Water in room temperature ionic liquids(RTILs) could impose significant effects on their interfacial properties at a charged surface. Although the interfaces between RTILs and mica surfaces exhibit rich microstructure, the influence of water content on such interfaces is little understood,in particular, considering the fact that RTILs are always associated with water due to their hygroscopicity. In this work, we studied how different types of RTILs and different amounts of water molecules affect the RTIL-mica interfaces, especially the water distribution at mica surfaces,using molecular dynamics(MD) simulation. MD results showed that(1) there is more water and a thicker water layer adsorbed on the mica surface as the water content increases, and correspondingly the average location of K^+ ions is farther from mica surface;(2) more water accumulated at the interface with the hydrophobic [Emim][TFSI] than in case of the hydrophilic [Emim][BF4] due to the respective RTIL hydrophobicity and ion size. A similar trend was also observed in the hydrogen bonds formed between water molecules. Moreover, the 2D number density map of adsorbed water revealed that the high-density areas of water seem to be related to K^+ ions and silicon/aluminum atoms on mica surface. These results are of great importance to understand the effects of hydrophobicity/hydrophicility of RTIL and water on the interfacial microstructure at electrified surfaces.展开更多
Aerosol liquid water content(ALWC)plays an important role in secondary aerosol formation.In this study,a whole year field campaign was conducted at Shanxi in north Zhejiang Province during 2021.ALWC estimated by ISORR...Aerosol liquid water content(ALWC)plays an important role in secondary aerosol formation.In this study,a whole year field campaign was conducted at Shanxi in north Zhejiang Province during 2021.ALWC estimated by ISORROPIA-Ⅱ was then investigated to explore its characteristics and relationship with secondary aerosols.ALWC exhibited a highest value in spring(66.38μg/m^(3)),followed by winter(45.08μg/m^(3)),summer(41.64μg/m^(3)),and autumn(35.01μg/m^(3)),respectively.It was supposed that the secondary inorganic aerosols(SIA)were facilitated under higher ALWC conditions(RH>80%),while the secondary organic species tended to form under lower ALWC levels.Higher RH(>80%)promoted the NO_(3)^(-)formation via gas-particle partitioning,while SO_(4)^(2-)was generated at a relative lower RH(>50%).The ALWC was more sensitive to NO_(3)^(-)(R=0.94)than SO_(4)^(2-)(R=0.90).Thus,the self-amplifying processes between the ALWC and SIA enhanced the particle mass growth.The sensitivity of ALWC and OX(NO_(2)+O_(3))to secondary organic carbon(SOC)varied in different seasons at Shanxi,more sensitive to aqueous-phase reactions(daytime R=0.84;nighttime R=0.54)than photochemical oxidation(daytime R=0.23;nighttime R=0.41)in wintertime with a high level of OX(daytime:130-140μg/m^(3);nighttime:100-140μg/m^(3)).The self-amplifying process of ALWC and SIA and the aqueous-phase formation of SOC will enhance aerosol formation,contributing to air pollution and reduction of visibility.展开更多
ABSTRACT This paper reports airborne measurements of midlatitude altostratus clouds observed over Zhengzhou, Henan Province, China on 3 March 2007. The case demonstrates mixed-phase conditions at altitudes from 3200 ...ABSTRACT This paper reports airborne measurements of midlatitude altostratus clouds observed over Zhengzhou, Henan Province, China on 3 March 2007. The case demonstrates mixed-phase conditions at altitudes from 3200 to 4600 m (0°C to -7.6°C), with liquid water content ranging from 0.01 to 0.09 g m-3. In the observed mixed-phase cloud, liquid water content exhibited a bimodal distribution, whereas the maximum ice particle concentration was located in the middle part of the cloud. The liquid and ice particle data showed significant horizontal variability on the scale of a few hundred meters. The cloud droplet concentration varied greatly over the horizontal sampling area. There was an inverse relationship between the cloud droplet concentration and ice particle concentration. A gamma distribution provided the best description of the cloud droplet spectra. The liquid droplet distributions were found to increase in both size and concentration with altitude. It was inferred from the profile of the spectra parameters that the cloud droplet sizes tend to form a quasi-monodisperse distribution. Ice particle spectra in the cloud were fitted well by an exponential distribution. Finally, a remarkable power law relationship was found between the slope (λ) and intercept (No) parameters of the exponential size distribution.展开更多
Leaching is widely applied in the exploitation of depleted ores. In order to discover the law of leachant movement in the leaching process and calculating volumes and time intervals of spraying leachant,experiments an...Leaching is widely applied in the exploitation of depleted ores. In order to discover the law of leachant movement in the leaching process and calculating volumes and time intervals of spraying leachant,experiments and numerical simulation with the TOUGH2/EOS3 module were carried out in order to find out the principle of water movement in unsaturated copper ore. The results show that water volume increases at the same location over time,that copper ore tends to become saturated and that liquid velocity decreases at the same time as the distance from top in-creases. On the other hand,a comparison and analysis of our experimental and simulated results indicate that the EOS3 module could accurately simulate the water movement in an unsaturated state.展开更多
基金National Natural Science Foundation of China(41575031,41175089)China Postdoctoral Science Foundation(2015M580124)Key Laboratory of Geo-Information Engineering(S18701)
文摘In the application of the physical iterative method to retrieve millimeter-wave radar liquid water content(LWC)and liquid water path(LWP),particle parameter scheme is the main factor affecting retrieval performance.In this paper,synchronous measurements of an airborne millimeter-wave radar and a hot-wire probe in stratus cloud are used to compare the LWC retrievals of the oceanic and continental particle parameter scheme with diameter less than 50μm and the particle parameter scheme with diameter less than 500μm and 1500μm(scheme 1,scheme 2,scheme 3,and scheme4,respectively).The results show that the particle parameter scheme needs to be selected according to the reflectivity factor when using the physical iterative method to retrieve the LWC and LWP.When the reflectivity factor is less than-30 d BZ,the retrieval error of scheme 1 is the minimum.When the reflectivity factor is greater than-30 d BZ,the retrieval error of scheme 4 is the minimum.Based on the reflectance factor value,the LWP retrievals of scheme 4 are closer to the measurements,the average relative bias is 5.2%,and the minimum relative bias is 4.4%.Compared with other schemes,scheme 4 seems to be more useful for the LWC and LWP retrieval of stratus cloud in China.
基金Natural Science Foundation of China (40675013)Foundation project of Nanjing University of Information Science & TechnologyProject on natural science for universities and colleges in Jiangsu province
文摘On March 16–17, 2008, a sea fog occurred in Dianbai in the west of Guangdong Province and was accompanied by a high-pressure synoptic system. Using comprehensive observation datasets, this study analyzes the evolution of liquid water content during this sea fog and investigates the relationships between liquid water content and the average diameters and count densities of fog droplets, air temperature, wind speed and turbulence exchanges. The main results are presented as follows. (1) The sea fog showed a quasi-periodic oscillation characteristic, i.e., it developed, disappeared and then developed again. (2) During the sea fog, the number of fog droplets changed significantly while the changes in average diameter of the fog droplets were relatively small. The development and disappearance of the sea fog correlated significantly with the fog droplet numbers. (3) The air-cooling mechanism played a significant role in sea fog formation and development. However, the influences of this mechanism were not evident during fog persistence. (4) During sea fog formation, weak turbulence exchanges were helpful for fog formation. During sea fog development and persistence, liquid water content increased when turbulence exchanges weakened, and vice versa. The changes in turbulence exchanges were closely related to the quasi-periodic oscillations observed in sea fog presence.
基金sponsored by the projects supported by the National Natural Science Foundation of China(NSFC,No.51576037 and 11172314)the National Key Basic Research Program of China (2015CB755800)
文摘In order to research the influence of liquid water content ( LWC ) on blade icing of wind turbine, a numerical simulation method for blade icing was established. The numerical simulation was based on low speed viscous N-S equation. The trajectory equation of water droplets was established by Lagrangian method. The mass and energy conservation equations of the water droplets impacting on the surface of the blade were solved based on control body theory. Three sections along blade span wise of a 1.5 MW wind turbine were decided to simulate icing. Five kinds of LWC were selected for simulation including 0.2,0.4,0.6,0.8 and 1.0 g/m^3 under two ambient temperatures of -10 ℃ and -20 ℃. The medium volume droplet diameter ( MVD ) was 30μm. The simulations included icing shape on blade surface, dimensionless icing area and dimensionless maximum stagnation thickness. Furthermore, the flow fields around both the iced blade airfoil and the original one were simulated and analyzed. Accor-ding to the results, the typical icing characteristics of icing shape, icing area and thickness were greatly affected by the difference of LWCs. This study can provide theoretical reference for the research on antiicing and deicing of wind turbine blade.
文摘In this paper, some features of cloud liquid water content with respect to rain and water vapor are presented. Cloud liquid water density profile is obtained from radiosonde observation with Salonen's model and Karsten's model at Kolkata, a tropical location in the Indian region. Cloud liquid water contents (LWC) are obtained from these profiles which show a prominent seasonal variation. The monsoon months exhibit much higher values of LWC than in other months. However Salonen's model yields higher LWC values than that obtained with Karsten's model. The variation of daily total rainfall with LWC shows a positive relationship indicating the role of LWC in controlling the rainfall. Also the variation pattern of LWC with integrated water vapor (IWV) content of the atmosphere indicates that a threshold value of water vapor is required for cloud to form and once cloud is formed LWC increases with IWV.
文摘In this paper, some distinctive features of the vertical profile of precipitable liquid water content (LWC) with considerable respect to rain rates (R) and radar reflectivity (Z) obtained in a tropical location are presented. Assessment of LWC allows applications in the specific area of flight icing severity, aviation safety as well as signals traversing through the atmosphere. The parameters were typically measured using vertically-pointing Micro Rain Radar (MRR) over a period of 2 years (2011-2012) at Akure, a tropical location of Nigeria. The radar scanned at every 10 seconds and integrated over one minute samples to reduce event logging error associated with the instrument. The vertical profile of the LWC typically reveals a prominent seasonal variation. However, majority of the LWC profiles has low LWC, less than 0.1 gm?3 while the maximum observed LWC is about 3.18 gm?3. A strong like hood relation was observed between the melting layer height and the LWC, with the LWC reaches peak at the considerable height of about 4160 m which coincides precisely with the freezing height level (rain height of ~4520 m) of the study location. Good correlation was also observed between the LWC and R in most of the heights considered. The results obtained will assist system engineers to assess the level of absorption, reflection and attenuation of electromagnetic signals as a result of precipitable LWC along the transmitting paths. The novelty of the present work is in the area of linking LWC and Z as against usual relation between Z and R.
基金This work is sponsored by the National Natural Science Foundation of China under the auspices of Project Contrant No.49485006.
文摘A retrieval method of microwave(MW)space-borne remote sensing of cloud liquid water content by the combined radar-radiometer is suggested.A three-layer cloud model is chosen to represent the typical stratified precipitating cloud.The retrieval method mainly follows our previously suggested scheme with some modifications.Numerical comparative study shows that in space-borne remote sensing of cloud liquid water content by the combined method is much better than by radar only;Also the retrieval accuracy of cloud liquid water content may be improved when using the three-layer cloud model in the combined method.
基金supported by the National Natural Science Foundation of China (51406060)Shenzhen Basic Research Project (JCYJ20170307171511292)the National Supercomputing Centers in Tianjin (Tianhe-1A) and Guangzhou (Tianhe Ⅱ)
文摘Water in room temperature ionic liquids(RTILs) could impose significant effects on their interfacial properties at a charged surface. Although the interfaces between RTILs and mica surfaces exhibit rich microstructure, the influence of water content on such interfaces is little understood,in particular, considering the fact that RTILs are always associated with water due to their hygroscopicity. In this work, we studied how different types of RTILs and different amounts of water molecules affect the RTIL-mica interfaces, especially the water distribution at mica surfaces,using molecular dynamics(MD) simulation. MD results showed that(1) there is more water and a thicker water layer adsorbed on the mica surface as the water content increases, and correspondingly the average location of K^+ ions is farther from mica surface;(2) more water accumulated at the interface with the hydrophobic [Emim][TFSI] than in case of the hydrophilic [Emim][BF4] due to the respective RTIL hydrophobicity and ion size. A similar trend was also observed in the hydrogen bonds formed between water molecules. Moreover, the 2D number density map of adsorbed water revealed that the high-density areas of water seem to be related to K^+ ions and silicon/aluminum atoms on mica surface. These results are of great importance to understand the effects of hydrophobicity/hydrophicility of RTIL and water on the interfacial microstructure at electrified surfaces.
基金supported by the National Natural Science Foundation of China(Nos.91844301 and 42005087)the support from State Environmental Protection Key Laboratory of Formation and Prevention of Urban Air Pollution Complex,Shanghai Academy of Environment Sciences(No.CX2020080581)。
文摘Aerosol liquid water content(ALWC)plays an important role in secondary aerosol formation.In this study,a whole year field campaign was conducted at Shanxi in north Zhejiang Province during 2021.ALWC estimated by ISORROPIA-Ⅱ was then investigated to explore its characteristics and relationship with secondary aerosols.ALWC exhibited a highest value in spring(66.38μg/m^(3)),followed by winter(45.08μg/m^(3)),summer(41.64μg/m^(3)),and autumn(35.01μg/m^(3)),respectively.It was supposed that the secondary inorganic aerosols(SIA)were facilitated under higher ALWC conditions(RH>80%),while the secondary organic species tended to form under lower ALWC levels.Higher RH(>80%)promoted the NO_(3)^(-)formation via gas-particle partitioning,while SO_(4)^(2-)was generated at a relative lower RH(>50%).The ALWC was more sensitive to NO_(3)^(-)(R=0.94)than SO_(4)^(2-)(R=0.90).Thus,the self-amplifying processes between the ALWC and SIA enhanced the particle mass growth.The sensitivity of ALWC and OX(NO_(2)+O_(3))to secondary organic carbon(SOC)varied in different seasons at Shanxi,more sensitive to aqueous-phase reactions(daytime R=0.84;nighttime R=0.54)than photochemical oxidation(daytime R=0.23;nighttime R=0.41)in wintertime with a high level of OX(daytime:130-140μg/m^(3);nighttime:100-140μg/m^(3)).The self-amplifying process of ALWC and SIA and the aqueous-phase formation of SOC will enhance aerosol formation,contributing to air pollution and reduction of visibility.
基金supported by the National Natural Science Foundation of China (Grant No. 41175120)the Knowledge Innovation Program of the Chinese Academy of Sciences (Grant No. KZCX2-EW-203)
文摘ABSTRACT This paper reports airborne measurements of midlatitude altostratus clouds observed over Zhengzhou, Henan Province, China on 3 March 2007. The case demonstrates mixed-phase conditions at altitudes from 3200 to 4600 m (0°C to -7.6°C), with liquid water content ranging from 0.01 to 0.09 g m-3. In the observed mixed-phase cloud, liquid water content exhibited a bimodal distribution, whereas the maximum ice particle concentration was located in the middle part of the cloud. The liquid and ice particle data showed significant horizontal variability on the scale of a few hundred meters. The cloud droplet concentration varied greatly over the horizontal sampling area. There was an inverse relationship between the cloud droplet concentration and ice particle concentration. A gamma distribution provided the best description of the cloud droplet spectra. The liquid droplet distributions were found to increase in both size and concentration with altitude. It was inferred from the profile of the spectra parameters that the cloud droplet sizes tend to form a quasi-monodisperse distribution. Ice particle spectra in the cloud were fitted well by an exponential distribution. Finally, a remarkable power law relationship was found between the slope (λ) and intercept (No) parameters of the exponential size distribution.
文摘Leaching is widely applied in the exploitation of depleted ores. In order to discover the law of leachant movement in the leaching process and calculating volumes and time intervals of spraying leachant,experiments and numerical simulation with the TOUGH2/EOS3 module were carried out in order to find out the principle of water movement in unsaturated copper ore. The results show that water volume increases at the same location over time,that copper ore tends to become saturated and that liquid velocity decreases at the same time as the distance from top in-creases. On the other hand,a comparison and analysis of our experimental and simulated results indicate that the EOS3 module could accurately simulate the water movement in an unsaturated state.
文摘以大气垂直累积液态水含量的预报问题为例,使用UNet网络结构作为基础结构构建时空预报模型,对比了采用两类预报策略的模型的预报效果,预报策略包含一个迭代预报策略(Recursive Forecast Strategy,RFS)以及两个直接预报策略(Direct Forecast Strategies,DFSs)。研究结果表明,两个直接预报模型对整体预报时段的预报效果明显优于迭代预报模型,直接预报模型的RMSE比迭代预报模型低19%。随着预报时次的增加,迭代预报模型的预报误差累积速度比两个直接预报模型快。在两个直接预报模型中,多时次输出模型(Direct Forecast Model Multi-Steps,DFS-M)的预报表现更加稳健,在整体预报时段上预报效果优于单时次输出模型(Direct Forecast Model Single-Step,DFS-S),但DFS-S模型对几个前期时次的预报效果较好。本研究利用深度学习可解释性技术中的深度学习重要特征分析方法(Deep Learning Important FeaTures,DeepLIFT)分析DFS-M和DFS-S模型各个输入时次对于模型预报的相对重要性。研究结果表明,DFS-M和DFS-S模型80%的输入重要性都集中在最后两个输入时次上,较早期输入时次的重要性随着预报时次的增加而呈现上升趋势。由于各输出时次间存在一定的统计相关性,受输出时次相关性约束的DFS-M模型的输入时次重要性变化比DFS-S模型更加稳定。通过将DFS-M和DFS-S模型对于不同时次的预报进行结合,可以得到效果更加均衡的预报。本研究可以为基于深度学习的天气气候预报方法的选择提供新的思路。