In this study,the theory of minimum detectable activity concentration(MDAC)for airborne gamma-ray spectrometry(AGS)was derived,and the relationship between the MDAC and the intrinsic effi-ciency of a scintillation cou...In this study,the theory of minimum detectable activity concentration(MDAC)for airborne gamma-ray spectrometry(AGS)was derived,and the relationship between the MDAC and the intrinsic effi-ciency of a scintillation counter,volume,and energy res-olution of scintillation crystals,and flight altitude of an aircraft was investigated.To verify this theory,experi-mental devices based on NaI and CeBr 3 scintillation counters were prepared,and the potassium,uranium,and thorium contents in calibration pads obtained via the stripping ratio method and theory were compared.The MDACs of AGS under different conditions were calculated and analyzed using the proposed theory and the Monte Carlo method.The relative errors found via a comparison of the experimental and theoretical results were less than 4%.The theory of MDAC can guide the work of AGS in probing areas with low radioactivity.展开更多
The determination of the effective minimum detectable activity (MDA) of radionuclides by a detection system plays an im- portant role in environmental radiation monitoring. In this study, the responses of an NaI(TI...The determination of the effective minimum detectable activity (MDA) of radionuclides by a detection system plays an im- portant role in environmental radiation monitoring. In this study, the responses of an NaI(TI) airborne γ ray spectrometry (AGRS) system to different radionuclides (137Cs and 131I) were investigated using the Monte Carlo technique. The MDA values were determined under different conditions according to the counting spectra obtained from the Monte Carlo simulation. The equivalent mass thickness method was applied to the Monte Carlo modeling for monitoring ground radiation to reduce sta- tistical uncertainty. The secondary source method was used to monitor both air and ground radiation. A quadratic relationship was found between the MDA and activity concentration. An exponential relationship was found between the MDA and altitude The MDA of a specific radionuclide from external detectors was found to be superior to that obtained from internal detectors under the same conditions. The MDA values in an NaI(Tl) AGRS system under different conditions can be estimated based on the results of this study.展开更多
To detect radioactive substances with low activity levels,an anticoincidence detector and a high-purity germanium(HPGe)detector are typically used simultaneously to suppress Compton scattering background,thereby resul...To detect radioactive substances with low activity levels,an anticoincidence detector and a high-purity germanium(HPGe)detector are typically used simultaneously to suppress Compton scattering background,thereby resulting in an extremely low detection limit and improving the measurement accuracy.However,the complex and expensive hardware required does not facilitate the application or promotion of this method.Thus,a method is proposed in this study to discriminate the digital waveform of pulse signals output using an HPGe detector,whereby Compton scattering background is suppressed and a low minimum detectable activity(MDA)is achieved without using an expensive and complex anticoincidence detector and device.The electric-field-strength and energy-deposition distributions of the detector are simulated to determine the relationship between pulse shape and energy-deposition location,as well as the characteristics of energy-deposition distributions for fulland partial-energy deposition events.This relationship is used to develop a pulse-shape-discrimination algorithm based on an artificial neural network for pulse-feature identification.To accurately determine the relationship between the deposited energy of gamma(γ)rays in the detector and the deposition location,we extract four shape parameters from the pulse signals output by the detector.Machine learning is used to input the four shape parameters into the detector.Subsequently,the pulse signals are identified and classified to discriminate between partial-and full-energy deposition events.Some partial-energy deposition events are removed to suppress Compton scattering.The proposed method effectively decreases the MDA of an HPGeγ-energy dispersive spectrometer.Test results show that the Compton suppression factors for energy spectra obtained from measurements on ^(152)Eu,^(137)Cs,and ^(60)Co radioactive sources are 1.13(344 keV),1.11(662 keV),and 1.08(1332 keV),respectively,and that the corresponding MDAs are 1.4%,5.3%,and 21.6%lower,respectively.展开更多
基金This work was supported by the Sichuan Science and Technology Program(No.2020JDRC0108)the National Science Foundation of China(Nos.41774147 and 41774190).
文摘In this study,the theory of minimum detectable activity concentration(MDAC)for airborne gamma-ray spectrometry(AGS)was derived,and the relationship between the MDAC and the intrinsic effi-ciency of a scintillation counter,volume,and energy res-olution of scintillation crystals,and flight altitude of an aircraft was investigated.To verify this theory,experi-mental devices based on NaI and CeBr 3 scintillation counters were prepared,and the potassium,uranium,and thorium contents in calibration pads obtained via the stripping ratio method and theory were compared.The MDACs of AGS under different conditions were calculated and analyzed using the proposed theory and the Monte Carlo method.The relative errors found via a comparison of the experimental and theoretical results were less than 4%.The theory of MDAC can guide the work of AGS in probing areas with low radioactivity.
基金supported by the National Defense Basic Scientific Research Project(Grant No.B2520133077)National High-tech R&D Program of China("863"Program)(Grant No.2012AA061803)
文摘The determination of the effective minimum detectable activity (MDA) of radionuclides by a detection system plays an im- portant role in environmental radiation monitoring. In this study, the responses of an NaI(TI) airborne γ ray spectrometry (AGRS) system to different radionuclides (137Cs and 131I) were investigated using the Monte Carlo technique. The MDA values were determined under different conditions according to the counting spectra obtained from the Monte Carlo simulation. The equivalent mass thickness method was applied to the Monte Carlo modeling for monitoring ground radiation to reduce sta- tistical uncertainty. The secondary source method was used to monitor both air and ground radiation. A quadratic relationship was found between the MDA and activity concentration. An exponential relationship was found between the MDA and altitude The MDA of a specific radionuclide from external detectors was found to be superior to that obtained from internal detectors under the same conditions. The MDA values in an NaI(Tl) AGRS system under different conditions can be estimated based on the results of this study.
基金This work was supported by the National Key R&D Program of China(Nos.2022YFF0709503,2022YFB1902700,2017YFC0602101)the Key Research and Development Program of Sichuan province(No.2023YFG0347)the Key Research and Development Program of Sichuan province(No.2020ZDZX0007).
文摘To detect radioactive substances with low activity levels,an anticoincidence detector and a high-purity germanium(HPGe)detector are typically used simultaneously to suppress Compton scattering background,thereby resulting in an extremely low detection limit and improving the measurement accuracy.However,the complex and expensive hardware required does not facilitate the application or promotion of this method.Thus,a method is proposed in this study to discriminate the digital waveform of pulse signals output using an HPGe detector,whereby Compton scattering background is suppressed and a low minimum detectable activity(MDA)is achieved without using an expensive and complex anticoincidence detector and device.The electric-field-strength and energy-deposition distributions of the detector are simulated to determine the relationship between pulse shape and energy-deposition location,as well as the characteristics of energy-deposition distributions for fulland partial-energy deposition events.This relationship is used to develop a pulse-shape-discrimination algorithm based on an artificial neural network for pulse-feature identification.To accurately determine the relationship between the deposited energy of gamma(γ)rays in the detector and the deposition location,we extract four shape parameters from the pulse signals output by the detector.Machine learning is used to input the four shape parameters into the detector.Subsequently,the pulse signals are identified and classified to discriminate between partial-and full-energy deposition events.Some partial-energy deposition events are removed to suppress Compton scattering.The proposed method effectively decreases the MDA of an HPGeγ-energy dispersive spectrometer.Test results show that the Compton suppression factors for energy spectra obtained from measurements on ^(152)Eu,^(137)Cs,and ^(60)Co radioactive sources are 1.13(344 keV),1.11(662 keV),and 1.08(1332 keV),respectively,and that the corresponding MDAs are 1.4%,5.3%,and 21.6%lower,respectively.