Parity–time(PT) and quasi-anti-parity–time(quasi-APT) symmetric optical gyroscopes have been proposed recently which enhance Sagnac frequency splitting. However, the operation of gyroscopes at the exceptional point(...Parity–time(PT) and quasi-anti-parity–time(quasi-APT) symmetric optical gyroscopes have been proposed recently which enhance Sagnac frequency splitting. However, the operation of gyroscopes at the exceptional point(EP) is challenging due to strict fabrication requirements and experimental uncertainties. We propose a new quasi-APT-symmetric micro-optical gyroscope which can be operated at the EP by easily shifting the Kerr nonlinearity. A single resonator is used as the core sensitive component of the quasi-APT-symmetric optical gyroscope to reduce the size, overcome the strict structural requirements and detect small rotation rates. Moreover, the proposed scheme also has an easy readout method for the frequency splitting. As a result, the device achieves a frequency splitting 10~5 times higher than that of a classical resonant optical gyroscope with the Earth's rotation. This proposal paves the way for a new and valuable method for the engineering of micro-optical gyroscopes.展开更多
Thin transparent oxide conducting films(TCOFs)of titanium and gallium substituted zinc oxide(TGZO)were fabricated via radio frequency(RF)magnetron sputtering technique.The effects of RF power on electrical,linear and ...Thin transparent oxide conducting films(TCOFs)of titanium and gallium substituted zinc oxide(TGZO)were fabricated via radio frequency(RF)magnetron sputtering technique.The effects of RF power on electrical,linear and nonlinear optical characteristics were investigated by Hall tester,Ultraviolet(UV)-visible spectrophotometer and optical characterization method.The results indicate that RF power significantly influences the electrical and optical properties of the deposited films.As RF power raises,the resistivity and Urbach energy fall initially and then rise,while the figure of merit,mean visible transmittance and optical bandgap show the reverse variation trend.At RF power of 190 W,the TGZO sample exhibits the highest electro-optical properties,with the maximum figure of merit(1.14×10^(4)Ω^(-1)∙cm^(-1)),mean visible transmittance(86.9%)and optical bandgap(3.50 eV),the minimum resistivity(6.26×10^(-4)Ω∙cm)and Urbach energy(174.23 meV).In addition,the optical constants of the deposited films were determined by the optical spectrum fitting method,and the RF power dependence of nonlinear optical properties was studied.It is observed that all the thin films exhibit normal dispersion characteristics in the visible region,and the nonlinear optical parameters are greatly affected by the RF power in the ultraviolet region.展开更多
The study of nonlinear optical responses in the mid-infrared(mid-IR)regime is essential for advancing ultrafast mid-IR laser applications.However,nonlinear optical effects under mid-IR excitation are rarely reported d...The study of nonlinear optical responses in the mid-infrared(mid-IR)regime is essential for advancing ultrafast mid-IR laser applications.However,nonlinear optical effects under mid-IR excitation are rarely reported due to the lack of suitable nonlinear optical materials.The natural van derWaals heterostructure franckeite,known for its narrow bandgap and stability in air,shows great potential for developing mid-IR nonlinear optical devices.We have experimentally demonstrated that layered franckeite exhibits a broadband wavelength-dependent nonlinear optical response in the mid-IR spectral region.Franckeite nanosheets were prepared using a liquid-phase exfoliation method,and their nonlinear optical response was characterized in the spectral range of 3000 nm to 5000 nm.The franckeite nanosheets exhibit broadband wavelengthdependent third-order nonlinearities,with nonlinear absorption and refraction coefficients estimated to be about 10^(-7)cm/W and 10^(-11)cm^(2)/W,respectively.Additionally,a passively Q-switched fluoride fiber laser operating around a wavelength of 2800 nm was achieved,delivering nanosecond pulses with a signal-to-noise ratio of 43.6 dB,based on the nonlinear response of franckeite.These findings indicate that layered franckeite possesses broadband nonlinear optical characteristics in the mid-IR region,potentially enabling new possibilities for mid-IR photonic devices.展开更多
The ultrashort lasers working in pulse-burst mode reveal great machining performance in recent years. The number of pulses in bursts effects greatly on the removal rate and roughness. To generate a more equal amplitud...The ultrashort lasers working in pulse-burst mode reveal great machining performance in recent years. The number of pulses in bursts effects greatly on the removal rate and roughness. To generate a more equal amplitude of pulses in burst with linear polarization output and time gap adjustable, we propose a new method by the harmonic beam combining(HBC).The beam combining is commonly used in adding pulses into the output beam while maintaining the pulse waveform and beam quality. In the HBC, dichroic mirrors are used to combine laser pulses of fundamental wave(FW) into harmonic wave(HW), and nonlinear crystals are used to convert the FW into HW. Therefore, HBC can add arbitrarily more HW pulses to generate pulse-burst in linear polarization with simple structure. The amplitude of each pulse in bursts can be adjusted the same to increase the stability of the burst, the time gap of each pulse can be adjusted precisely by proper time delay. Because HBC adds pulses sequentially, the peak power density of the burst is the same as each pulse, pulses can be combined without concern of back-conversion which often occurs in high peak power density. In the demonstration, the extendibility of HBC was verified by combining two beams with a third beam. The combined efficiency rates were larger than 99%, and the beam quality of each beam was maintained at M^(2)≈1.4.展开更多
A Weyl node is characterized by its chirality and tilt.We develop a theory of how nth-order nonlinear optical conductivity behaves under transformations of anisotropic tensor and tilt, which clarifies how chirality-de...A Weyl node is characterized by its chirality and tilt.We develop a theory of how nth-order nonlinear optical conductivity behaves under transformations of anisotropic tensor and tilt, which clarifies how chirality-dependent and-independent parts of optical conductivity transform under the reversal of tilt and chirality.Built on this theory, we propose ferromagnetic Mn Bi2Te4as a magnetoelectrically regulated, terahertz optical device, by magnetoelectrically switching the chiralitydependent and-independent DC photocurrents.These results are useful for creating nonlinear optical devices based on the topological Weyl semimetals.展开更多
Cyclo[18]carbon has received considerable attention thanks to its novel geometric configuration and special electronic structure.Superalkalis have low ionization energy.Doping a superalkali in cyclo[18]carbon is an ef...Cyclo[18]carbon has received considerable attention thanks to its novel geometric configuration and special electronic structure.Superalkalis have low ionization energy.Doping a superalkali in cyclo[18]carbon is an effective method to improve the optical properties of the system because considerable electron transfer occurs.In this paper,the geometry,bonding properties,electronic structure,absorption spectrum,and nonlinear optical(NLO)properties of superalkaline M_(3)O(M=Li,Na)-doped cyclo[18]carbon were studied by using density functional theory.M_(3)O and the C_(18) rings are not coplanar.The C_(18) ring still exhibits alternating long and short bonds.The charge transfer between M_(3)O and C_(18) forms stable[M_(3)O]+[C_(18)]-ionic complexes.C_(18)M_(3)O(M=Li,Na)shows striking optical nonlinearity,i.e.,their first-and second-order hyperpolarizability(βvec andγ||)increase considerably atλ=1907 nm and 1460 nm.展开更多
We propose a novel all-optical sampling method using nonlinear polarization rotation in a semiconductor optical amplifier. A rate-equation model capable of describing the all-optical sampling mechanism is presented in...We propose a novel all-optical sampling method using nonlinear polarization rotation in a semiconductor optical amplifier. A rate-equation model capable of describing the all-optical sampling mechanism is presented in this paper. Based on this model, we investigate the optimized operating parameters of the proposed system by simulating the output intensity of the probe light as functions of the input polarization angle, the phase induced by the polarization controller, and the ori- entation of the polarization beam splitter. The simulated results show that we can obtain a good linear slope and a large linear dynamic range,which is suitable for all-optical sampling. The operating power of the pump light can be less than lmW. The presented all-optical sampling method can potentially operate at a sampling rate up to hundreds GS/s and needs low optical power.展开更多
Nonlinear optical imaging is a versatile tool that has been proven to be exceptionally useful in various research fields.However,due to the use of photomultiplier tubes(PMTs),the wide application of nonlinear optical ...Nonlinear optical imaging is a versatile tool that has been proven to be exceptionally useful in various research fields.However,due to the use of photomultiplier tubes(PMTs),the wide application of nonlinear optical imaging is limited by the incapability of imaging under am-bient light.In this paper,we propose and demonstrate a new optical imaging detection method based on optical parametric amplification(OPA).As a nonlinear optical process,OPA in-trinsically rejects ambient light photons by coherence gating.Periodical poled lithium niobate(PPLN)crystals are used in this study as the media for OPA.Compared to bulk nonlinear optical crystals,PPLN crystals support the generation of OPA signal with lower pump power.Therefore,this characteristic of PPLN crystals is particularly beneficial when using high-repetition-rate lasers,which facilitate high-speed optical signal detection,such as in spec-troscopy and imaging.A PPLN-based OPA system was built to amplify the emitted imaging signal from second harmonic generation(SHG)and coherent anti-Stokes Raman scattering(CARS)microscopy imaging,and the amplified optical signal was strong enough to be detected by a biased photodiode under ordinary room light conditions.With OPA detection,ambient-light-on SHG and CARS imaging becomes possible,and achieves a similar result as PMT detection under strictly dark environments.These results demonstrate that OPA can be used as a substitute for PMTs in nonlinear optical imaging to adapt it to various applications with complex.light ing conditions.展开更多
In this paper,we study the time-asymptotically nonlinear stability of rarefaction waves for the Cauchy problem of the compressible Navier-Stokes equations for a reacting mixture with zero heat conductivity in one dime...In this paper,we study the time-asymptotically nonlinear stability of rarefaction waves for the Cauchy problem of the compressible Navier-Stokes equations for a reacting mixture with zero heat conductivity in one dimension.If the corresponding Riemann problem for the compressible Euler system admits the solutions consisting of rarefaction waves only,it is shown that its Cauchy problem has a unique global solution which tends time-asymptotically towards the rarefaction waves,while the initial perturbation and the strength of rarefaction waves are suitably small.展开更多
Two-dimensional(2D)nonlinear optical mediums with high and tunable light modulation capability can significantly stimulate the development of ultrathin,compact,and integrated optoelectronics devices and photonic eleme...Two-dimensional(2D)nonlinear optical mediums with high and tunable light modulation capability can significantly stimulate the development of ultrathin,compact,and integrated optoelectronics devices and photonic elements.2D carbides and nitrides of transition metals(MXenes)are a new class of 2D materials with excellent intrinsic and strong light-matter interaction characteristics.However,the current understanding of their photo-physical properties and strategies for improving optical performance is insufficient.To address this issue,we rationally designed and in situ synthesized a 2D Nb_(2)C/MoS_(2) heterostructure that outperforms pristine Nb2C in both linear and nonlinear optical performance.Excellent agreement between experimental and theoretical results demonstrated that the Nb_(2)C/MoS_(2) inherited the preponderance of Nb_(2)C and MoS_(2) in absorption at different wavelengths,resulting in the broadband enhanced optical absorption characteristics.In addition to linear optical modulation,we also achieved stronger near infrared nonlinear optical modulation,with a nonlinear absorption coefficient of Nb_(2)C/MoS_(2) being more than two times that of the pristine Nb_(2)C.These results were supported by the band alinement model which was determined by the X-ray photoelectron spectroscopy(XPS)experiment and first-principal theory calculation.The presented facile synthesis approach and robust light modulation strategy pave the way for broadband optoelectronic devices and optical modulators.展开更多
In nonlinear optical systems,optical solitons have the transmission properties of reducing error rate,improving system security and stability,and have important research significance in future research on all optical ...In nonlinear optical systems,optical solitons have the transmission properties of reducing error rate,improving system security and stability,and have important research significance in future research on all optical communication.This paper uses the bilinear method to obtain the two-soliton solutions of the nonlinear Schrödinger equation.By analyzing the relevant physical parameters in the obtained solutions,the interaction between optical solitons is optimized.The influence of the initial conditions on the interactions of the optical solitons is analyzed in detail,the reason why the interaction of the optical solitons is sensitive to the initial condition is discussed,and the interactions of the optical solitons are effectively weakened.The relevant results are beneficial for reducing the error rate and promoting the communication quality of the system.展开更多
We investigate the nonlinear optical rectification(NOR) of spherical quantum dots(QDs) under Hulthén plus Hellmann confining potential with the external tuning elements. Energy and wavefunction are determined by ...We investigate the nonlinear optical rectification(NOR) of spherical quantum dots(QDs) under Hulthén plus Hellmann confining potential with the external tuning elements. Energy and wavefunction are determined by using the Nikiforov–Uvarov method. Expression for the NOR coefficient is derived by the density matrix theory. The results show that the applied external elements and internal parameters of this system have a strong influence on intraband nonlinear optical properties. It is hopeful that this tuning of the nonlinear optical properties of GaAs/Ga_(1-x)Al_(x)As QDs can make a greater contribution to preparation of new functional optical devices.展开更多
Four phenoxysilicon networks for nonlinear optical (NLO) applications were designed and prepared by an extended sol-gel process without additional H2O and catalyst. All poled polymer network films possess high second-...Four phenoxysilicon networks for nonlinear optical (NLO) applications were designed and prepared by an extended sol-gel process without additional H2O and catalyst. All poled polymer network films possess high second-order nonlinear optical coefficients (d(33)) Of 10(-7)similar to 10(-8) esu. The investigation of NLO temporal stability at room temperature and elevated temperature (120 degreesC) indicated that these films exhibit high d(33) stability because the orientation of the chromophores are locked in the phenoxysilicon organic/inorganic networks.展开更多
Optical dispersive nonlinearities in Er-doped optical fiber are discussed and measured at the third window wavelength 1.55 μm for optical communications firstly. The experimental method, which is developed by us, is ...Optical dispersive nonlinearities in Er-doped optical fiber are discussed and measured at the third window wavelength 1.55 μm for optical communications firstly. The experimental method, which is developed by us, is based on dynamic scanning for fixed-point-interference (DSFPI) of two fiber beams. The real part and complex value of the third-order susceptibility at the wavelength are also obtained from the measured Kerr coefficient and nonlinear-absorption coefficient reported elsewhere.展开更多
Taking into account ultra-fast carrier dynamics, this paper models 640 Gbit/s wavelength conversion scheme based on nonlinear polarization rotation (NPR) in a single semiconductor optical amplifier (SOA) and inves...Taking into account ultra-fast carrier dynamics, this paper models 640 Gbit/s wavelength conversion scheme based on nonlinear polarization rotation (NPR) in a single semiconductor optical amplifier (SOA) and investigates the performance of this kind of wavelength conversion scheme in detail. In this model, two carrier temperature equations are introduced to substitute two energy density equations, which reduce the complexity of calculation in comparison with the previous model. The temporary gain and phase shift dynamics induced by ultra-short optical pulses are numerically simulated and the simulated results are qualitatively in good agreement with reported experimental results. Simulated results show that non-inverted and inverted 640 Gbit/s wavelength conversions based on NPR are achieved with clear open eye diagrams. To further investigate the performance of the non-inverted wavelength conversion scheme, the dependence of output extinction ratio (ER) on some key parameters used in simulation is illustrated. Furthermore, simulated analyses show that high performance non-inverted wavelength conversion based on NPR can be achieved by using a red-shifted filtering scheme.展开更多
The influence of optical nonlinearity on combining efficiency in ultrashort pulse fiber laser coherent combining system is investigated theoretically and experimentally.In the theoretical work,a new theoretical algori...The influence of optical nonlinearity on combining efficiency in ultrashort pulse fiber laser coherent combining system is investigated theoretically and experimentally.In the theoretical work,a new theoretical algorithm is presented for the coherent combining efficiency,which can be used to quantify the spectral coherence decay induced by optical nonlinearity imbalance between the sub-beams.The spectral information of the sub-beam is obtained by numerically solving the nonlinear Schrödinger equation(NLSE)in this algorithm to ensure an accurate prediction.In the experimental work,the coherent combining of two all-fiber picosecond lasers is achieved,and the influence of imbalanced optical nonlinearity on the combining efficiency is studied,which agrees with the theoretical prediction.This paper reveals the physical mechanism for the influence of optical nonlinearity on the combining efficiency,which is valuable for the coherent combining of ultrashort pulse fiber laser beams.展开更多
For multi-photon processed with the linear dispersion in the high-intensity terahertz(THz) field,we have systematically investigated the temperature-dependent nonlinear optical response of graphene-based systems, incl...For multi-photon processed with the linear dispersion in the high-intensity terahertz(THz) field,we have systematically investigated the temperature-dependent nonlinear optical response of graphene-based systems, including single layer graphene, graphene superlattice and gapped graphene. In the intrinsic single layer graphene system, it demonstrates that, at low temperature, nonlinear optical conductivities of the thirdand fifth-order are respectively five and ten orders of magnitude larger than the universal conductivity with high-intensity and low frequency THz wave.In the graphene superlattice and gapped graphene systems, the optical responses enhanced because of the anisotropic massless and massive Dirac fermions.展开更多
Utilizing the linear-stability analysis, this paper analytically investigates and calculates the condition and gain spectra of cross-phase modulation instability in optical fibres in the ease of exponential saturable ...Utilizing the linear-stability analysis, this paper analytically investigates and calculates the condition and gain spectra of cross-phase modulation instability in optical fibres in the ease of exponential saturable nonlinearity and high-order dispersion. The results show that, the modulation instability characteristics here are similar to those of conventional saturable nonlinearity and Kerr nonlinearity. That is to say, when the fourth-order dispersion has the same sign as that of the second-order one, a new gain spectral region called the second one which is far away from the zero point may appear. The existence of the exponential saturable nonlinearity will make the spectral width as well as the peak gain of every spectral region increase with the input powers before decrease. Namely, for every spectral regime, this may lead to a unique value of peak gain and spectral width for two different input powers. In comparison with the case of conventional saturable nonlinearity, however, when the other parameters are the same, the variations of the spectral width and the peak gain with the input powers will be faster in case of exponential saturable nonlinearity.展开更多
This paper introduces a joint nonlinearity and chromatic dispersion pre-compensation method for coherent optical orthogonal frequency-division multiplexing systems. The research results show that this method can reduc...This paper introduces a joint nonlinearity and chromatic dispersion pre-compensation method for coherent optical orthogonal frequency-division multiplexing systems. The research results show that this method can reduce the walk- off effect and can therefore equalize the nonlinear impairments effectively. Compared with the only other existing nonlinearity pre-compensation method, the joint nonlinearity and chromatic dispersion pre-compensation method is not only suitable for low-dispersion optical orthogonal frequency-division multiplexing system, but also effective for high- dispersion optical orthogonal frequency-division multiplexing transmission system with higher input power but without optical dispersion compensation. The suggested solution does not increase computation complexity compared with only nonlinearity pre-compensation method. For 40 Gbit/s coherent optical orthogonal frequency-division multiplexing 20 × 80 km standard single-mode fibre system, the suggested method can improve the nonlinear threshold (for Q 〉 10 dB) about 2.7, 1.2 and 1.0 dB, and the maximum Q factor about 1.2, 0.4 and 0.3 dB, for 2, 8 and 16 ps/(nm.km) dispersion coefficients.展开更多
Chalcogenide glasses (ChGs) are a promising candidate for applications in nonlinear photonic devices. In this paper, we review the research progress of the third-order optical nonlinearity (TONL) of ChGs from the ...Chalcogenide glasses (ChGs) are a promising candidate for applications in nonlinear photonic devices. In this paper, we review the research progress of the third-order optical nonlinearity (TONL) of ChGs from the following three aspects: chemical composition, excitation condition, and post processing. The deficiencies in previous studies and further research of the TONL property of ChGs are also discussed.展开更多
基金Project supported by the National Natural Science Foundation of China (Grant Nos.62273115,62173105)the Fundamental Research Funds for the Central Universities (Grant No.3072022FSC0401)。
文摘Parity–time(PT) and quasi-anti-parity–time(quasi-APT) symmetric optical gyroscopes have been proposed recently which enhance Sagnac frequency splitting. However, the operation of gyroscopes at the exceptional point(EP) is challenging due to strict fabrication requirements and experimental uncertainties. We propose a new quasi-APT-symmetric micro-optical gyroscope which can be operated at the EP by easily shifting the Kerr nonlinearity. A single resonator is used as the core sensitive component of the quasi-APT-symmetric optical gyroscope to reduce the size, overcome the strict structural requirements and detect small rotation rates. Moreover, the proposed scheme also has an easy readout method for the frequency splitting. As a result, the device achieves a frequency splitting 10~5 times higher than that of a classical resonant optical gyroscope with the Earth's rotation. This proposal paves the way for a new and valuable method for the engineering of micro-optical gyroscopes.
文摘Thin transparent oxide conducting films(TCOFs)of titanium and gallium substituted zinc oxide(TGZO)were fabricated via radio frequency(RF)magnetron sputtering technique.The effects of RF power on electrical,linear and nonlinear optical characteristics were investigated by Hall tester,Ultraviolet(UV)-visible spectrophotometer and optical characterization method.The results indicate that RF power significantly influences the electrical and optical properties of the deposited films.As RF power raises,the resistivity and Urbach energy fall initially and then rise,while the figure of merit,mean visible transmittance and optical bandgap show the reverse variation trend.At RF power of 190 W,the TGZO sample exhibits the highest electro-optical properties,with the maximum figure of merit(1.14×10^(4)Ω^(-1)∙cm^(-1)),mean visible transmittance(86.9%)and optical bandgap(3.50 eV),the minimum resistivity(6.26×10^(-4)Ω∙cm)and Urbach energy(174.23 meV).In addition,the optical constants of the deposited films were determined by the optical spectrum fitting method,and the RF power dependence of nonlinear optical properties was studied.It is observed that all the thin films exhibit normal dispersion characteristics in the visible region,and the nonlinear optical parameters are greatly affected by the RF power in the ultraviolet region.
基金supported by the National Natural Science Foundation of China(Grant No.61975055)the Natural Science Foundation of Hunan Province,China(Grant No.2023JJ30165)+1 种基金the Natural Science Foundation of Shandong Province,China(Grant No.ZR2022QF005)the Doctoral Fund of University of Heze(Grant No.XY22BS14).
文摘The study of nonlinear optical responses in the mid-infrared(mid-IR)regime is essential for advancing ultrafast mid-IR laser applications.However,nonlinear optical effects under mid-IR excitation are rarely reported due to the lack of suitable nonlinear optical materials.The natural van derWaals heterostructure franckeite,known for its narrow bandgap and stability in air,shows great potential for developing mid-IR nonlinear optical devices.We have experimentally demonstrated that layered franckeite exhibits a broadband wavelength-dependent nonlinear optical response in the mid-IR spectral region.Franckeite nanosheets were prepared using a liquid-phase exfoliation method,and their nonlinear optical response was characterized in the spectral range of 3000 nm to 5000 nm.The franckeite nanosheets exhibit broadband wavelengthdependent third-order nonlinearities,with nonlinear absorption and refraction coefficients estimated to be about 10^(-7)cm/W and 10^(-11)cm^(2)/W,respectively.Additionally,a passively Q-switched fluoride fiber laser operating around a wavelength of 2800 nm was achieved,delivering nanosecond pulses with a signal-to-noise ratio of 43.6 dB,based on the nonlinear response of franckeite.These findings indicate that layered franckeite possesses broadband nonlinear optical characteristics in the mid-IR region,potentially enabling new possibilities for mid-IR photonic devices.
基金Project supported by Youth Innovation Promotion Association of the Chinese Academy of Sciences (Grant No.2020029)。
文摘The ultrashort lasers working in pulse-burst mode reveal great machining performance in recent years. The number of pulses in bursts effects greatly on the removal rate and roughness. To generate a more equal amplitude of pulses in burst with linear polarization output and time gap adjustable, we propose a new method by the harmonic beam combining(HBC).The beam combining is commonly used in adding pulses into the output beam while maintaining the pulse waveform and beam quality. In the HBC, dichroic mirrors are used to combine laser pulses of fundamental wave(FW) into harmonic wave(HW), and nonlinear crystals are used to convert the FW into HW. Therefore, HBC can add arbitrarily more HW pulses to generate pulse-burst in linear polarization with simple structure. The amplitude of each pulse in bursts can be adjusted the same to increase the stability of the burst, the time gap of each pulse can be adjusted precisely by proper time delay. Because HBC adds pulses sequentially, the peak power density of the burst is the same as each pulse, pulses can be combined without concern of back-conversion which often occurs in high peak power density. In the demonstration, the extendibility of HBC was verified by combining two beams with a third beam. The combined efficiency rates were larger than 99%, and the beam quality of each beam was maintained at M^(2)≈1.4.
基金Project supported by the National Key R&D Program of China (Grant Nos.2018YFA, 0305601, and 2021YFA1400100)the National Natural Science Foundation of China (Grant Nos.12274003, 11725415, and 11934001)the Innovation Program for Quantum Science and Technology (Grant No.2021ZD0302600)。
文摘A Weyl node is characterized by its chirality and tilt.We develop a theory of how nth-order nonlinear optical conductivity behaves under transformations of anisotropic tensor and tilt, which clarifies how chirality-dependent and-independent parts of optical conductivity transform under the reversal of tilt and chirality.Built on this theory, we propose ferromagnetic Mn Bi2Te4as a magnetoelectrically regulated, terahertz optical device, by magnetoelectrically switching the chiralitydependent and-independent DC photocurrents.These results are useful for creating nonlinear optical devices based on the topological Weyl semimetals.
基金Project supported by the Natural Science Foundation of Anhui Province(Grant No.1908085MA12)the National Natural Science Foundation of China(Grant No.21703222)。
文摘Cyclo[18]carbon has received considerable attention thanks to its novel geometric configuration and special electronic structure.Superalkalis have low ionization energy.Doping a superalkali in cyclo[18]carbon is an effective method to improve the optical properties of the system because considerable electron transfer occurs.In this paper,the geometry,bonding properties,electronic structure,absorption spectrum,and nonlinear optical(NLO)properties of superalkaline M_(3)O(M=Li,Na)-doped cyclo[18]carbon were studied by using density functional theory.M_(3)O and the C_(18) rings are not coplanar.The C_(18) ring still exhibits alternating long and short bonds.The charge transfer between M_(3)O and C_(18) forms stable[M_(3)O]+[C_(18)]-ionic complexes.C_(18)M_(3)O(M=Li,Na)shows striking optical nonlinearity,i.e.,their first-and second-order hyperpolarizability(βvec andγ||)increase considerably atλ=1907 nm and 1460 nm.
文摘We propose a novel all-optical sampling method using nonlinear polarization rotation in a semiconductor optical amplifier. A rate-equation model capable of describing the all-optical sampling mechanism is presented in this paper. Based on this model, we investigate the optimized operating parameters of the proposed system by simulating the output intensity of the probe light as functions of the input polarization angle, the phase induced by the polarization controller, and the ori- entation of the polarization beam splitter. The simulated results show that we can obtain a good linear slope and a large linear dynamic range,which is suitable for all-optical sampling. The operating power of the pump light can be less than lmW. The presented all-optical sampling method can potentially operate at a sampling rate up to hundreds GS/s and needs low optical power.
基金supported in part by grants from the National Institutes of Health (R01CA213149,R01CA241618).
文摘Nonlinear optical imaging is a versatile tool that has been proven to be exceptionally useful in various research fields.However,due to the use of photomultiplier tubes(PMTs),the wide application of nonlinear optical imaging is limited by the incapability of imaging under am-bient light.In this paper,we propose and demonstrate a new optical imaging detection method based on optical parametric amplification(OPA).As a nonlinear optical process,OPA in-trinsically rejects ambient light photons by coherence gating.Periodical poled lithium niobate(PPLN)crystals are used in this study as the media for OPA.Compared to bulk nonlinear optical crystals,PPLN crystals support the generation of OPA signal with lower pump power.Therefore,this characteristic of PPLN crystals is particularly beneficial when using high-repetition-rate lasers,which facilitate high-speed optical signal detection,such as in spec-troscopy and imaging.A PPLN-based OPA system was built to amplify the emitted imaging signal from second harmonic generation(SHG)and coherent anti-Stokes Raman scattering(CARS)microscopy imaging,and the amplified optical signal was strong enough to be detected by a biased photodiode under ordinary room light conditions.With OPA detection,ambient-light-on SHG and CARS imaging becomes possible,and achieves a similar result as PMT detection under strictly dark environments.These results demonstrate that OPA can be used as a substitute for PMTs in nonlinear optical imaging to adapt it to various applications with complex.light ing conditions.
基金supported by the Beijing Natural Science Foundation(1182004,Z180007,1192001).
文摘In this paper,we study the time-asymptotically nonlinear stability of rarefaction waves for the Cauchy problem of the compressible Navier-Stokes equations for a reacting mixture with zero heat conductivity in one dimension.If the corresponding Riemann problem for the compressible Euler system admits the solutions consisting of rarefaction waves only,it is shown that its Cauchy problem has a unique global solution which tends time-asymptotically towards the rarefaction waves,while the initial perturbation and the strength of rarefaction waves are suitably small.
基金financial support from the National Natural Science Foundation of China(Nos.61874141,11904239)Natural Science Foundation of Hunan Province(Grant Nos.2021JJ40709,2021JJ20080,2022JJ20080)+2 种基金Postgraduate Innovative Project of Central South University(Grant No.2021zzts0056)Open Sharing Found for the Large-scale Instruments and Equipment of Central South Universitysupported in part by the High Performance Computing Center of Central South University。
文摘Two-dimensional(2D)nonlinear optical mediums with high and tunable light modulation capability can significantly stimulate the development of ultrathin,compact,and integrated optoelectronics devices and photonic elements.2D carbides and nitrides of transition metals(MXenes)are a new class of 2D materials with excellent intrinsic and strong light-matter interaction characteristics.However,the current understanding of their photo-physical properties and strategies for improving optical performance is insufficient.To address this issue,we rationally designed and in situ synthesized a 2D Nb_(2)C/MoS_(2) heterostructure that outperforms pristine Nb2C in both linear and nonlinear optical performance.Excellent agreement between experimental and theoretical results demonstrated that the Nb_(2)C/MoS_(2) inherited the preponderance of Nb_(2)C and MoS_(2) in absorption at different wavelengths,resulting in the broadband enhanced optical absorption characteristics.In addition to linear optical modulation,we also achieved stronger near infrared nonlinear optical modulation,with a nonlinear absorption coefficient of Nb_(2)C/MoS_(2) being more than two times that of the pristine Nb_(2)C.These results were supported by the band alinement model which was determined by the X-ray photoelectron spectroscopy(XPS)experiment and first-principal theory calculation.The presented facile synthesis approach and robust light modulation strategy pave the way for broadband optoelectronic devices and optical modulators.
基金Project supported by the National Natural Science Foundation of China(Grant No.11875005).
文摘In nonlinear optical systems,optical solitons have the transmission properties of reducing error rate,improving system security and stability,and have important research significance in future research on all optical communication.This paper uses the bilinear method to obtain the two-soliton solutions of the nonlinear Schrödinger equation.By analyzing the relevant physical parameters in the obtained solutions,the interaction between optical solitons is optimized.The influence of the initial conditions on the interactions of the optical solitons is analyzed in detail,the reason why the interaction of the optical solitons is sensitive to the initial condition is discussed,and the interactions of the optical solitons are effectively weakened.The relevant results are beneficial for reducing the error rate and promoting the communication quality of the system.
基金Project supported by the National Natural Science Foundation of China (Grant Nos.51702003,61775087,11674312,52174161,and 12174161)。
文摘We investigate the nonlinear optical rectification(NOR) of spherical quantum dots(QDs) under Hulthén plus Hellmann confining potential with the external tuning elements. Energy and wavefunction are determined by using the Nikiforov–Uvarov method. Expression for the NOR coefficient is derived by the density matrix theory. The results show that the applied external elements and internal parameters of this system have a strong influence on intraband nonlinear optical properties. It is hopeful that this tuning of the nonlinear optical properties of GaAs/Ga_(1-x)Al_(x)As QDs can make a greater contribution to preparation of new functional optical devices.
文摘Four phenoxysilicon networks for nonlinear optical (NLO) applications were designed and prepared by an extended sol-gel process without additional H2O and catalyst. All poled polymer network films possess high second-order nonlinear optical coefficients (d(33)) Of 10(-7)similar to 10(-8) esu. The investigation of NLO temporal stability at room temperature and elevated temperature (120 degreesC) indicated that these films exhibit high d(33) stability because the orientation of the chromophores are locked in the phenoxysilicon organic/inorganic networks.
文摘Optical dispersive nonlinearities in Er-doped optical fiber are discussed and measured at the third window wavelength 1.55 μm for optical communications firstly. The experimental method, which is developed by us, is based on dynamic scanning for fixed-point-interference (DSFPI) of two fiber beams. The real part and complex value of the third-order susceptibility at the wavelength are also obtained from the measured Kerr coefficient and nonlinear-absorption coefficient reported elsewhere.
基金Project supported by the Ministry of Education of China(Grant Nos105036 and NCET-04-0116)
文摘Taking into account ultra-fast carrier dynamics, this paper models 640 Gbit/s wavelength conversion scheme based on nonlinear polarization rotation (NPR) in a single semiconductor optical amplifier (SOA) and investigates the performance of this kind of wavelength conversion scheme in detail. In this model, two carrier temperature equations are introduced to substitute two energy density equations, which reduce the complexity of calculation in comparison with the previous model. The temporary gain and phase shift dynamics induced by ultra-short optical pulses are numerically simulated and the simulated results are qualitatively in good agreement with reported experimental results. Simulated results show that non-inverted and inverted 640 Gbit/s wavelength conversions based on NPR are achieved with clear open eye diagrams. To further investigate the performance of the non-inverted wavelength conversion scheme, the dependence of output extinction ratio (ER) on some key parameters used in simulation is illustrated. Furthermore, simulated analyses show that high performance non-inverted wavelength conversion based on NPR can be achieved by using a red-shifted filtering scheme.
基金upported by the Key Program of Beijing Municipal Natural Science Foundation,China(Grant No.KZ201910005006)the National Natural Science Foundation of China(Grant No.62005004)+1 种基金Natural Science Foundation of Beijing Municipality,China(Grant No.4204091)National Science Foundation for Post-doctor Scientists of China(Grant No.212423)。
文摘The influence of optical nonlinearity on combining efficiency in ultrashort pulse fiber laser coherent combining system is investigated theoretically and experimentally.In the theoretical work,a new theoretical algorithm is presented for the coherent combining efficiency,which can be used to quantify the spectral coherence decay induced by optical nonlinearity imbalance between the sub-beams.The spectral information of the sub-beam is obtained by numerically solving the nonlinear Schrödinger equation(NLSE)in this algorithm to ensure an accurate prediction.In the experimental work,the coherent combining of two all-fiber picosecond lasers is achieved,and the influence of imbalanced optical nonlinearity on the combining efficiency is studied,which agrees with the theoretical prediction.This paper reveals the physical mechanism for the influence of optical nonlinearity on the combining efficiency,which is valuable for the coherent combining of ultrashort pulse fiber laser beams.
基金supported by the National Special Fund for the Development of Major Research Equipment and Instruments (project No. 2011YQ13001805)the Foundation of Beijing Educational Commission, China(Grant No. KM201010028006)
文摘For multi-photon processed with the linear dispersion in the high-intensity terahertz(THz) field,we have systematically investigated the temperature-dependent nonlinear optical response of graphene-based systems, including single layer graphene, graphene superlattice and gapped graphene. In the intrinsic single layer graphene system, it demonstrates that, at low temperature, nonlinear optical conductivities of the thirdand fifth-order are respectively five and ten orders of magnitude larger than the universal conductivity with high-intensity and low frequency THz wave.In the graphene superlattice and gapped graphene systems, the optical responses enhanced because of the anisotropic massless and massive Dirac fermions.
基金Project supported by the Key Program of the Natural Science Foundation of Sichuan Provincial Education Department (Grant No. 2006A124)the Fundamental Application Research Project of the Department of Science & Technology of Sichuan Province (Grant No. 05JY029-084)
文摘Utilizing the linear-stability analysis, this paper analytically investigates and calculates the condition and gain spectra of cross-phase modulation instability in optical fibres in the ease of exponential saturable nonlinearity and high-order dispersion. The results show that, the modulation instability characteristics here are similar to those of conventional saturable nonlinearity and Kerr nonlinearity. That is to say, when the fourth-order dispersion has the same sign as that of the second-order one, a new gain spectral region called the second one which is far away from the zero point may appear. The existence of the exponential saturable nonlinearity will make the spectral width as well as the peak gain of every spectral region increase with the input powers before decrease. Namely, for every spectral regime, this may lead to a unique value of peak gain and spectral width for two different input powers. In comparison with the case of conventional saturable nonlinearity, however, when the other parameters are the same, the variations of the spectral width and the peak gain with the input powers will be faster in case of exponential saturable nonlinearity.
基金supported by the National High Technology Research and Development Program of China(Grant No.2009AA01A345)the National Basic Research Program of China(Grant No.2011CB302702)the National Natural Science Foundation of China(Grant No.60932004)
文摘This paper introduces a joint nonlinearity and chromatic dispersion pre-compensation method for coherent optical orthogonal frequency-division multiplexing systems. The research results show that this method can reduce the walk- off effect and can therefore equalize the nonlinear impairments effectively. Compared with the only other existing nonlinearity pre-compensation method, the joint nonlinearity and chromatic dispersion pre-compensation method is not only suitable for low-dispersion optical orthogonal frequency-division multiplexing system, but also effective for high- dispersion optical orthogonal frequency-division multiplexing transmission system with higher input power but without optical dispersion compensation. The suggested solution does not increase computation complexity compared with only nonlinearity pre-compensation method. For 40 Gbit/s coherent optical orthogonal frequency-division multiplexing 20 × 80 km standard single-mode fibre system, the suggested method can improve the nonlinear threshold (for Q 〉 10 dB) about 2.7, 1.2 and 1.0 dB, and the maximum Q factor about 1.2, 0.4 and 0.3 dB, for 2, 8 and 16 ps/(nm.km) dispersion coefficients.
基金Project supported by the National Natural Science Foundation of China(Grant No.61675106)the National Key Research and Development Program of China(Grant No.2016YFB0303803)the K C Wong Magna Fund in Ningbo University
文摘Chalcogenide glasses (ChGs) are a promising candidate for applications in nonlinear photonic devices. In this paper, we review the research progress of the third-order optical nonlinearity (TONL) of ChGs from the following three aspects: chemical composition, excitation condition, and post processing. The deficiencies in previous studies and further research of the TONL property of ChGs are also discussed.