A two-dimensional photonic crystal with a one-dimensional periodic dielectric background is proposed. The photonic band modulation effects due to the periodic background are investigated based on the plane wave expans...A two-dimensional photonic crystal with a one-dimensional periodic dielectric background is proposed. The photonic band modulation effects due to the periodic background are investigated based on the plane wave expansion method. We find that periodic modulation of the dielectric background greatly alters photonic band structures, especially for the E-polarization modes. The number, width and position of the photonic band gaps (PBGs) sensitively depend on the structure parameters (the layer thicknesses and dielectric constants) of the one-dimensional periodic background,展开更多
We describe in this paper the fabrication of two- and one-dimensional nanostructures with organic molecular beam epitaxy (OMBE) principle based on controlled selfassembly by using adsorbate-substrate and intennolecu...We describe in this paper the fabrication of two- and one-dimensional nanostructures with organic molecular beam epitaxy (OMBE) principle based on controlled selfassembly by using adsorbate-substrate and intennolecular interactions that are important in molecular fabrication. Cu(100) single crystal was used as substrate in fabricating molecular nanostructures. Scanning tunneling microscopy (STM) experiments confirmed that Zn-tetra- [3,5-di-t-butylphenyl]porphyrin-molecules can be used to fabricate both monolayer and molecular wire on Cu(100) surface simultaneously, and the latter is arranged on the terrace edges. We herein briefly discuss the selectivity in terms of a mechanism in which the highest occupied and lowest unoccupied molecular orbitals (HOMO and LUMO) of the molecules interact with the surface.展开更多
Direct-write atom lithography,one of the potential nanofabrication techniques,is restricted by some difficulties in producing optical masks for the deposition of complex structures.In order to make further progress,a ...Direct-write atom lithography,one of the potential nanofabrication techniques,is restricted by some difficulties in producing optical masks for the deposition of complex structures.In order to make further progress,a structured mirror array is developed to transversely collimate the chromium atomic beam in two dimensions.The best collimation is obtained when the laser red detunes by natural line-width of transition 7S3 → 7P40 of the chromium atom.The collimation ratio is 0.45 vertically(in x axis),and it is 0.55 horizontally(in y axis).The theoretical model is also simulated,and success of our structured mirror array is achieved.展开更多
The Ga N high electron mobility transistor(HEMT)has been considered as a potential terahertz(THz)radiation source,yet the low radiation power level restricts their applications.The HEMT array is thought to improve the...The Ga N high electron mobility transistor(HEMT)has been considered as a potential terahertz(THz)radiation source,yet the low radiation power level restricts their applications.The HEMT array is thought to improve the coupling efficiency between two-dimensional(2D)plasmons and THz radiation.In this work,we investigate the plasma oscillation,electromagnetic radiation,and the integration characteristics of Ga N HEMT targeting at a high THz radiation power source.The quantitative radiation power and directivity are obtained for integrated Ga N HEMT array with different array periods and element numbers.With the same initial plasma oscillation phase among the HEMT units,the radiation power of the two-element HEMT array can achieve 4 times as the single HEMT radiation power when the array period is shorter than 1/8electromagnetic wavelength.In addition,the radiation power of the HEMT array varies almost linearly with the element number,the smaller array period can lead to the greater radiation power.It shows that increasing the array period could narrow the main radiated lobe width while weaken the radiation power.Increasing the element number can improve both the radiation directivity and power.We also synchronize the plasma wave phases in the HEMT array by adopting an external Gaussian plane wave with central frequency the same as the plasmon resonant frequency,which solves the problem of the radiation power reduction caused by the asynchronous plasma oscillation phases among the elements.The study of the radiation power amplification of the one-dimensional(1D)Ga N HEMT array provides useful guidance for the research of compact high-power solid-state terahertz sources.展开更多
An experimental investigation was performed to investigate two-dimensional axial velocity field at downstream of the 90°double bend pipe with and without inlet swirling condition. The main objectives are to fi...An experimental investigation was performed to investigate two-dimensional axial velocity field at downstream of the 90°double bend pipe with and without inlet swirling condition. The main objectives are to find separation region and observe the influence of inlet swirling flow on the velocity fluctuation using ultrasound technique. The experiments were carried out in the pipe at Reynolds number Re = 1 × 104. In case of inlet swirling flow condition, a rotary swirler was used as swirling generator, and the swirl number was setup S = 1. The ultrasonic measurements were taken at four downstream locations of the second bend pipe. Phased Array Ultrasonic Velocity Profiler (Phased Array UVP) technique was applied to obtain the two-dimensional velocity of the fluid and the axial and tangential velocity fluctuation. It was found that the secondary reverse flow became smaller at the downstream from the bend when the inlet condition on the first bend was swirling flow. In addition, inlet swirling condition influenced mainly on the tangential velocity fluctuation, and its maximum turbulence intensity was 40%.展开更多
Gaseous phases of carbon-containing and metastable oxides will be resulted from the carbonization of phenolic resin binders and the reduced reactions between C and oxides at high temperatures in carbon-containing refr...Gaseous phases of carbon-containing and metastable oxides will be resulted from the carbonization of phenolic resin binders and the reduced reactions between C and oxides at high temperatures in carbon-containing refractories. With the in-situ catalysis technique, these gaseous phases can be transformed to one-or two-dimensional bonding phases by deposition,which is favorable for the improvement on strength and toughness of carboncontaining refractories,especially low carbon refractories. The research results reveal that:( 1) the amorphous carbon resulted from phenolic resin can be transformed to carbon nanotubes,thus,the oxidation peak temperature is raised from 506 to 664. 6 ℃;( 2) onedimensional whiskers of MgO or Mg Al2 O4 can be in-situ formed in MgO-C refractories, and their CMOR,CCS,rupture displacement and residual CCS( two water quenching cycles,1 100 ℃) are increased by 66%,47%,13% and 26%,respectively;( 3) two-dimensional array structure of flake β-SiAlON can be in-situ formed in Al2 O3-C refractories,which improves the material strength by 60% and decreases the residual strength after thermal shock by only 4. 5 MPa. It is believed that the in-situ formation of one-or two-dimensional bonding phases at high temperatures can improvethe comprehensive thermal physical properties of carboncontaining refractories,and will be the developing trend of the strengthening and toughening of low carbon-containing refractories.展开更多
A new zinc polymer, {Zn(O2CC12H8CO2)(H2O)}, or {Zn(DPHA)(H2O)}n (O2CC12H8CO2, DPHA = 1,1′ -biphenyl-2,2′-dicarboxylate dianion) has been synthesized under hydrothermal conditions. The crystal is of monocli...A new zinc polymer, {Zn(O2CC12H8CO2)(H2O)}, or {Zn(DPHA)(H2O)}n (O2CC12H8CO2, DPHA = 1,1′ -biphenyl-2,2′-dicarboxylate dianion) has been synthesized under hydrothermal conditions. The crystal is of monoclinic, space group P21/c with a = 12.8418(5), b = 5.9505(2), c = 17.2989(5) A, β = 104.020(2)°, V = 1282.52(8) A^3, C14H10O5Zn, Mr= 323.61, Z = 4, Dc = 1.676 g/cm^3,μ = 1.930 mm^-1, F(000) = 656, R = 0.0766 and wR = 0.1871 for 1775 observed reflections (I 〉 2σ(I)). It consists of Zn2(DPHA)2(H2O)2 units, which are further extended into a one-dimensional double helical-chain polymer via Zn-O bonding. The hydrogen bonding interactions extend the helical chains into a two-dimensional layer structure.展开更多
Research on flexible or wearable electronics has been grown remarkably due to the advent of nanomaterials,such as metal nanowires,graphene,or transition metal dichalcogenides.Although each nanomaterial has mechanical ...Research on flexible or wearable electronics has been grown remarkably due to the advent of nanomaterials,such as metal nanowires,graphene,or transition metal dichalcogenides.Although each nanomaterial has mechanical and electrical characteristics that can be applied into flexible electronics,the limitations of each nanomaterial are also clear.In order to overcome the limitations of these nanomaterials,research on the hybrid structures of nanomaterials has been extensively conducted.In this study,we introduce the properties of one-dimensional nanomaterials,twodimensional nanomaterials,and their hybrid nanomaterials.And then,we provide information concerning various flexible electronics based on these nanomaterials.展开更多
Flexible electronics technology is considered as a revolutionary technology to unlock the bottleneck of traditional rigid electronics that prevalent for decades,thereby fueling the next-generation electronics.In the p...Flexible electronics technology is considered as a revolutionary technology to unlock the bottleneck of traditional rigid electronics that prevalent for decades,thereby fueling the next-generation electronics.In the past few decades,the research on flexible electronic devices based on organic materials has witnessed rapid development and substantial achievements,and inorganic semiconductors are also now beginning to shine in the field of flexible electronics.As validated by the latest research,some of the inorganic semiconductors,particularly those at low dimension,unexpectedly exhibited excellent mechanical flexibility on top of superior electrical properties.Herein,we bring together a comprehensive analysis on the recently burgeoning low-dimension inorganic semiconductor materials in flexible electronics,including one-dimensional(1D)inorganic semiconductor nanowires(NWs)and two-dimensional(2D)transition metal dichalcogenides(TMDs).The fundamental electrical properties,optical properties,mechanical properties and strain engineering of materials,and their performance in flexible device applications are discussed in detail.We also propose current challenges and predict future development directions including material synthesis and device fabrication and integration.展开更多
This article reviews the recent developments in the fabrication and properties of one-dimensional (1D) Bi-based nanostructures, including Bi, Sb, BixSb1-x and Bi2Te3 nanowire arrays, and Bi-Bi and Bi-Sb nanojunction...This article reviews the recent developments in the fabrication and properties of one-dimensional (1D) Bi-based nanostructures, including Bi, Sb, BixSb1-x and Bi2Te3 nanowire arrays, and Bi-Bi and Bi-Sb nanojunction arrays. In this article, we present an efiective method to fabricate Bi nanowire arrays with difierent diameters in anodic alumina membrane (AAM) with a single pore size by the pulsed electrodeposition. The fabrication of the high-filling and ordered Bi1-xSbx and Bi2Te3 single crystalline nanowire arrays, the Bi nanowire metalsemiconductor homojunction and Bi-Sb nanowire metal-semiconductor heterojunction arrays by the pulsed electrodeposition are reported. The factors controlling the composition, diameter, growth rate and orientation of the nanowires are analyzed, and the growth mechanism of the nanowire and nanojunction arrays are discussed together with the study of the electrical and thermal properties of Bi-based nanowires and nanojunctions.Finally, this review is concluded with some perspectives on the research directions and focuses in the Bi-based nanomaterials fields.展开更多
The complexity of biological samples determines that the detection of a single biomolecule is unable to satisfy actual needs. Moreover, the "false positives" results caused by a single biomolecule detections...The complexity of biological samples determines that the detection of a single biomolecule is unable to satisfy actual needs. Moreover, the "false positives" results caused by a single biomolecule detections easily leads to erroneous clinical diagnosis and treatment. Thus, it is important for the homogenous quantification of multiple biomolecules in not only basic research but also practical application. As a consequent, a large number of literatures have been exploited to monitor multiple biomolecules in homogenous solution, enabling facilitating the development of the disease diagnosis, treatment as well as drug discovery. One-dimensional nanomaterials and two-dimensional nanomaterials have special physical and chemical properties, such as good electrochemical properties, stable structure, large specific surface area, and biocompatibility, which are widely used in electrochemical and fluorescent detection of biomolecules. This tutorial review highlights the recent development for the detection of multiple biomolecules by using nanomaterials including one-dimensional materials(1DMs) as well as twodimensional materials(2DMs).展开更多
Tomonaga-Luttinger liquid(TLL),a peculiar one-dimensional(1D)electronic behavior due to strong correlation,was first studied in 1D nanostructures and has attracted significant attention over the last several decades.W...Tomonaga-Luttinger liquid(TLL),a peculiar one-dimensional(1D)electronic behavior due to strong correlation,was first studied in 1D nanostructures and has attracted significant attention over the last several decades.With the rise of new two-dimensional(2D)quantum materials,1D nanostructures in 2D materials have provided a new platform with a well-defined configuration at the atomic scale for studying TLL electronic behavior.In this paper,we review the recent progress of TLL electronic features in emerging 2D materials embedded with various 1D nanostructures,including island edges,domain walls,and 1D moirépatterns.Specifically,novel physical phenomena,such as 1D edge states in 2D transition metal dichalcogenides(TMDs),helical TLL in 2D topological insulators(2DTI),and chiral TLL in 2D quantum Hall systems,are described and discussed at the nanoscale.We also analyze challenges and opportunities at the frontier of this research area.展开更多
The concept of difference and sum co-array(DSCA)has become a new design idea for planar sparse arrays.Inspired by the shifting invariance property of DSCA,a specific configuration named here as the improved L-shaped a...The concept of difference and sum co-array(DSCA)has become a new design idea for planar sparse arrays.Inspired by the shifting invariance property of DSCA,a specific configuration named here as the improved L-shaped array is proposed.Compared to other traditional 2D sparse array configurations such as 2D nested arrays and hourglass arrays,the proposed configuration has larger central consecutive ranges in its DSCA,thus increasing the DOF.At the same time,the mutual coupling effect is also reduced due to the enlarged spacing between the adjacent sensors.Simulations further demonstrate the superiority of the proposed arrays in terms of detection performance and estimation accuracy.展开更多
It is an important theme in nanoscience to control the interval of the ordered array of nanoparticles through modifying the chain length of the passivating molecules of the nanoparticles. The theme runs through most o...It is an important theme in nanoscience to control the interval of the ordered array of nanoparticles through modifying the chain length of the passivating molecules of the nanoparticles. The theme runs through most of the applications of the ordered array of nanoparticles. Though the Langmuir-Blodgett (LB) technique is one of the most important ways to prepare the two-dimensional ordered array of nanoparticles, it has only been used in case that the passivating molecules are short enough (【C12). When the passivating molecules become longer, it is difficult to obtain the ordered array of the particles simply by compressing them on the surface of water. The present work focused on the formation of the two-dimensional array of the octadecyl-amine-passivated gold nanoparticles at the air/water interface. By properly modifying the ordinary LB technique, the long-term two-dimensional ordered array of nanoparticles was successfully achieved. The surface pressure-area isotherms and the electron microscopy展开更多
A two-dimensional(2D) optical true-time delay(TTD) beam-forming system using a compact fiber grating prism(FGP) for a planar phased array antenna(PAA) is proposed. The optical beam-forming system mainly consists of a ...A two-dimensional(2D) optical true-time delay(TTD) beam-forming system using a compact fiber grating prism(FGP) for a planar phased array antenna(PAA) is proposed. The optical beam-forming system mainly consists of a TTD unit based on the same compact FGP, one tunable laser for elevation beam steering, and a controlled wavelength converter for azimuth beam steering. A planar PAA using such 2D optical TTD unit has advantages such as compactness, low bandwidth requirement for tunable laser sources, and potential for large-scale system implementations. The proof-of-concept experiment results demonstrate the feasibility of the proposed scheme.展开更多
Kronecker sequences constructed from short sequences are good sequences for spread spectrum communication systems. In this paper we study a similar problem for two-dimensional arrays, and we determine the linear compl...Kronecker sequences constructed from short sequences are good sequences for spread spectrum communication systems. In this paper we study a similar problem for two-dimensional arrays, and we determine the linear complexity of the Kronecker product of two arrays, Our result shows that similar good property on linear complexity holds for Kronecker product of arrays.展开更多
As the basis of machine vision,the biomimetic image sensing devices are the eyes of artificial intelligence.In recent years,with the development of two-dimensional(2D)materials,many new optoelectronic devices are deve...As the basis of machine vision,the biomimetic image sensing devices are the eyes of artificial intelligence.In recent years,with the development of two-dimensional(2D)materials,many new optoelectronic devices are developed for their outstanding performance.However,there are still little sensing arrays based on 2D materials with high imaging quality,due to the poor uniformity of pixels caused by material defects and fabrication technique.Here,we propose a 2D MoS_(2)sensing array based on artificial neural network(ANN)learning.By equipping the MoS_(2)sensing array with a“brain”(ANN),the imaging quality can be effectively improved.In the test,the relative standard deviation(RSD)between pixels decreased from about 34.3%to 6.2%and 5.49%after adjustment by the back propagation(BP)and Elman neural networks,respectively.The peak signal to noise ratio(PSNR)and structural similarity(SSIM)of the image are improved by about 2.5 times,which realizes the re-recognition of the distorted image.This provides a feasible approach for the application of 2D sensing array by integrating ANN to achieve high quality imaging.展开更多
In recent years, nuclear magnetic resonance (NMR) has been increasingly used for fluid- typing in well-logging because of the improved generations of NMR logging tools. This paper first discusses the applicable cond...In recent years, nuclear magnetic resonance (NMR) has been increasingly used for fluid- typing in well-logging because of the improved generations of NMR logging tools. This paper first discusses the applicable conditions of two one-dimensional NMR methods: the dual TW method and dual TE method. Then, the two-dimensional (T2, D) and (T2, T1) NMR methods are introduced. These different typing methods for hydrocarbon are compared and analyzed by numerical simulation. The results show that the dual TW method is not suitable for identifying a macroporous water layer. The dual TE method is not suitable for typing gas and irreducible water. (T2, T1) method is more effective in typing a gas layer. In an oil-bearing layer of movable water containing big pores, (T2, T1) method can solve the misinterpretation problem in the dual TWmethod between a water layer with big pores and an oil layer. The (T2, T1) method can distinguish irreducible water from oil of a medium viscosity, and the viscosity range of oil becomes wide in contrast with that of the dual TW method. The (T2, D) method is more effective in typing oil and water layers. In a gas layer, when the SNR is higher than a threshold, the (T2, D) method can resolve the overlapping T2 signals of irreducible water and gas that occurs due to the use of the dual TE method. Twodimensional NMR for fluid-typing is an important development of well logging technology.展开更多
In the past decade, researchers in the fields of energy production have concentrated on the improvement of new energy storage devices. Lithium-ion batteries(LIBs) and faradaic supercapacitors(FSs) have attracted speci...In the past decade, researchers in the fields of energy production have concentrated on the improvement of new energy storage devices. Lithium-ion batteries(LIBs) and faradaic supercapacitors(FSs) have attracted special attention as a result of the rapid development of new electrode nanomaterials, especially hybrid nanomaterials, which can meet the increasingly higher requirements for future energy, such as the capability to deliver high-power performance and an extremely long life cycle. In these hybrid nanostructures, a series of synergistic effects and unique properties arising from the combination of individual components are a major factor leading to improved charge/discharge capability, energy density, and system lifetime. This paper describes the most recent progress in the growth of hybrid electrode materials for LIBs and FSs systems, focusing on the combination of zero-dimensional(0 D), one-dimensional(1 D), two-dimensional(2 D), and three-dimensional(3 D) nanomaterials, respectively.展开更多
The development of pressure sensor arrays capable of distinguishing the shape and texture details of objects is of considerable interest in the emerging fields of smart robots,prostheses,human-machine interfaces,and a...The development of pressure sensor arrays capable of distinguishing the shape and texture details of objects is of considerable interest in the emerging fields of smart robots,prostheses,human-machine interfaces,and artificial intelligence(AI).Here we report an integrated pressure sensor array,by combining solution-processed two-dimensional(2D)MoS2 van der Waals(vdW)thin film transistor(TFT)active matrix and conductive micropyramidal pressure-sensitive rubber(PSR)electrodes made of polydimethylsiloxane/carbon nanotube composites,to achieve spatially revolved pressure mapping with excellent contrast and low power consumption.We demonstrate a 10×10 active matrix by using the 2D MoS2 vdW-TFTs with high on-off ratio>10^(6),minimal hysteresis,and excellent device-to-device uniformity.The combination of the vdW-TFT active matrix with the highly uniform micropyramidal PSR electrodes creates an integrated pressure sensing array for spatially resolved pressure mapping.This study demonstrates that the solution-processed 2D vdW-TFTs offer a solution for active-matrix control of pressure sensor arrays,and could be extended for other active-matrix arrays of electronic or optoelectronic devices.展开更多
基金supported by the State Key Basic Research Program of China under Grant No.2006CB921607China-Australia Special Fund for Science and Technology
文摘A two-dimensional photonic crystal with a one-dimensional periodic dielectric background is proposed. The photonic band modulation effects due to the periodic background are investigated based on the plane wave expansion method. We find that periodic modulation of the dielectric background greatly alters photonic band structures, especially for the E-polarization modes. The number, width and position of the photonic band gaps (PBGs) sensitively depend on the structure parameters (the layer thicknesses and dielectric constants) of the one-dimensional periodic background,
基金This work was supported by the Excellent Scientist Program of South China University of Technology (324-D60090), the Scientific Research Foundation for the Returned Overseas Chinese Scholars, State Education Ministry (B09-B7060040) and the National Natural Science Foundation of China (20643001)
文摘We describe in this paper the fabrication of two- and one-dimensional nanostructures with organic molecular beam epitaxy (OMBE) principle based on controlled selfassembly by using adsorbate-substrate and intennolecular interactions that are important in molecular fabrication. Cu(100) single crystal was used as substrate in fabricating molecular nanostructures. Scanning tunneling microscopy (STM) experiments confirmed that Zn-tetra- [3,5-di-t-butylphenyl]porphyrin-molecules can be used to fabricate both monolayer and molecular wire on Cu(100) surface simultaneously, and the latter is arranged on the terrace edges. We herein briefly discuss the selectivity in terms of a mechanism in which the highest occupied and lowest unoccupied molecular orbitals (HOMO and LUMO) of the molecules interact with the surface.
基金Project supported by the Shanghai Nanoscience Foundation,China (Grant Nos. 0852nm07000 and 0952nm07000)the National Natural Science Foundation of China (Grant Nos. 10804084 and 91123022)+1 种基金the National Key Technology R & D Program,China (Grant No. 2006BAF06B08)the Specialized Research Fund for the Doctoral Program of Ministry of High Education of China (Grant No. 200802471008)
文摘Direct-write atom lithography,one of the potential nanofabrication techniques,is restricted by some difficulties in producing optical masks for the deposition of complex structures.In order to make further progress,a structured mirror array is developed to transversely collimate the chromium atomic beam in two dimensions.The best collimation is obtained when the laser red detunes by natural line-width of transition 7S3 → 7P40 of the chromium atom.The collimation ratio is 0.45 vertically(in x axis),and it is 0.55 horizontally(in y axis).The theoretical model is also simulated,and success of our structured mirror array is achieved.
基金Project supported by the National Natural Science Foundation of China(Grant Nos.92163204,61921002,and 62171098)。
文摘The Ga N high electron mobility transistor(HEMT)has been considered as a potential terahertz(THz)radiation source,yet the low radiation power level restricts their applications.The HEMT array is thought to improve the coupling efficiency between two-dimensional(2D)plasmons and THz radiation.In this work,we investigate the plasma oscillation,electromagnetic radiation,and the integration characteristics of Ga N HEMT targeting at a high THz radiation power source.The quantitative radiation power and directivity are obtained for integrated Ga N HEMT array with different array periods and element numbers.With the same initial plasma oscillation phase among the HEMT units,the radiation power of the two-element HEMT array can achieve 4 times as the single HEMT radiation power when the array period is shorter than 1/8electromagnetic wavelength.In addition,the radiation power of the HEMT array varies almost linearly with the element number,the smaller array period can lead to the greater radiation power.It shows that increasing the array period could narrow the main radiated lobe width while weaken the radiation power.Increasing the element number can improve both the radiation directivity and power.We also synchronize the plasma wave phases in the HEMT array by adopting an external Gaussian plane wave with central frequency the same as the plasmon resonant frequency,which solves the problem of the radiation power reduction caused by the asynchronous plasma oscillation phases among the elements.The study of the radiation power amplification of the one-dimensional(1D)Ga N HEMT array provides useful guidance for the research of compact high-power solid-state terahertz sources.
文摘An experimental investigation was performed to investigate two-dimensional axial velocity field at downstream of the 90°double bend pipe with and without inlet swirling condition. The main objectives are to find separation region and observe the influence of inlet swirling flow on the velocity fluctuation using ultrasound technique. The experiments were carried out in the pipe at Reynolds number Re = 1 × 104. In case of inlet swirling flow condition, a rotary swirler was used as swirling generator, and the swirl number was setup S = 1. The ultrasonic measurements were taken at four downstream locations of the second bend pipe. Phased Array Ultrasonic Velocity Profiler (Phased Array UVP) technique was applied to obtain the two-dimensional velocity of the fluid and the axial and tangential velocity fluctuation. It was found that the secondary reverse flow became smaller at the downstream from the bend when the inlet condition on the first bend was swirling flow. In addition, inlet swirling condition influenced mainly on the tangential velocity fluctuation, and its maximum turbulence intensity was 40%.
文摘Gaseous phases of carbon-containing and metastable oxides will be resulted from the carbonization of phenolic resin binders and the reduced reactions between C and oxides at high temperatures in carbon-containing refractories. With the in-situ catalysis technique, these gaseous phases can be transformed to one-or two-dimensional bonding phases by deposition,which is favorable for the improvement on strength and toughness of carboncontaining refractories,especially low carbon refractories. The research results reveal that:( 1) the amorphous carbon resulted from phenolic resin can be transformed to carbon nanotubes,thus,the oxidation peak temperature is raised from 506 to 664. 6 ℃;( 2) onedimensional whiskers of MgO or Mg Al2 O4 can be in-situ formed in MgO-C refractories, and their CMOR,CCS,rupture displacement and residual CCS( two water quenching cycles,1 100 ℃) are increased by 66%,47%,13% and 26%,respectively;( 3) two-dimensional array structure of flake β-SiAlON can be in-situ formed in Al2 O3-C refractories,which improves the material strength by 60% and decreases the residual strength after thermal shock by only 4. 5 MPa. It is believed that the in-situ formation of one-or two-dimensional bonding phases at high temperatures can improvethe comprehensive thermal physical properties of carboncontaining refractories,and will be the developing trend of the strengthening and toughening of low carbon-containing refractories.
基金This work was financially supported by the NNSF of China (No. 20173063), the State Key Basic Research and Development Plan of China (001CB108906) and the NSF of Fujian Province (E0020001)
文摘A new zinc polymer, {Zn(O2CC12H8CO2)(H2O)}, or {Zn(DPHA)(H2O)}n (O2CC12H8CO2, DPHA = 1,1′ -biphenyl-2,2′-dicarboxylate dianion) has been synthesized under hydrothermal conditions. The crystal is of monoclinic, space group P21/c with a = 12.8418(5), b = 5.9505(2), c = 17.2989(5) A, β = 104.020(2)°, V = 1282.52(8) A^3, C14H10O5Zn, Mr= 323.61, Z = 4, Dc = 1.676 g/cm^3,μ = 1.930 mm^-1, F(000) = 656, R = 0.0766 and wR = 0.1871 for 1775 observed reflections (I 〉 2σ(I)). It consists of Zn2(DPHA)2(H2O)2 units, which are further extended into a one-dimensional double helical-chain polymer via Zn-O bonding. The hydrogen bonding interactions extend the helical chains into a two-dimensional layer structure.
基金Bio&Medical Technology Development Program,Grant/Award Number:2018M3A9F1021649Industrial Technology Innovation Program,Grant/Award Number:10080577+3 种基金Institute for Basic Science,Grant/Award Number:IBS-R026-D1Ministry of Science&ICT(MSIT)and the Ministry of Trade,Industry and Energy(MOTIE)of Korea through the National Research Foundation,Grant/Award Numbers:2016R1A5A1009926,2019R1A2B5B03069358Nano Material Technology Development Program,Grant/Award Numbers:2015M3A7B4050308,2016M3A7B4910635Research Program funded by Yonsei University,Grant/Award Number:2018-22-0194。
文摘Research on flexible or wearable electronics has been grown remarkably due to the advent of nanomaterials,such as metal nanowires,graphene,or transition metal dichalcogenides.Although each nanomaterial has mechanical and electrical characteristics that can be applied into flexible electronics,the limitations of each nanomaterial are also clear.In order to overcome the limitations of these nanomaterials,research on the hybrid structures of nanomaterials has been extensively conducted.In this study,we introduce the properties of one-dimensional nanomaterials,twodimensional nanomaterials,and their hybrid nanomaterials.And then,we provide information concerning various flexible electronics based on these nanomaterials.
基金supported by the Natural Science Foundation of China(No.51902101)Natural Science Foundation of Jiangsu Province(No.BK20201381)+1 种基金Science Foundation of Nanjing University of Posts and Telecommunications(No.NY219144)Postgraduate Research&Practice Innovation Program of Jiangsu Province(No.SJCX22_0254).
文摘Flexible electronics technology is considered as a revolutionary technology to unlock the bottleneck of traditional rigid electronics that prevalent for decades,thereby fueling the next-generation electronics.In the past few decades,the research on flexible electronic devices based on organic materials has witnessed rapid development and substantial achievements,and inorganic semiconductors are also now beginning to shine in the field of flexible electronics.As validated by the latest research,some of the inorganic semiconductors,particularly those at low dimension,unexpectedly exhibited excellent mechanical flexibility on top of superior electrical properties.Herein,we bring together a comprehensive analysis on the recently burgeoning low-dimension inorganic semiconductor materials in flexible electronics,including one-dimensional(1D)inorganic semiconductor nanowires(NWs)and two-dimensional(2D)transition metal dichalcogenides(TMDs).The fundamental electrical properties,optical properties,mechanical properties and strain engineering of materials,and their performance in flexible device applications are discussed in detail.We also propose current challenges and predict future development directions including material synthesis and device fabrication and integration.
基金The authors acknowledge the support from the National Major Project of Fundamental Research for Nanomaterials and Nanostructures (No. 2005CB623603);National Natural Science Foundation of China (No. 10474098);Natural Science Foundation of Anhui Provinc(No. 050440902).
文摘This article reviews the recent developments in the fabrication and properties of one-dimensional (1D) Bi-based nanostructures, including Bi, Sb, BixSb1-x and Bi2Te3 nanowire arrays, and Bi-Bi and Bi-Sb nanojunction arrays. In this article, we present an efiective method to fabricate Bi nanowire arrays with difierent diameters in anodic alumina membrane (AAM) with a single pore size by the pulsed electrodeposition. The fabrication of the high-filling and ordered Bi1-xSbx and Bi2Te3 single crystalline nanowire arrays, the Bi nanowire metalsemiconductor homojunction and Bi-Sb nanowire metal-semiconductor heterojunction arrays by the pulsed electrodeposition are reported. The factors controlling the composition, diameter, growth rate and orientation of the nanowires are analyzed, and the growth mechanism of the nanowire and nanojunction arrays are discussed together with the study of the electrical and thermal properties of Bi-based nanowires and nanojunctions.Finally, this review is concluded with some perspectives on the research directions and focuses in the Bi-based nanomaterials fields.
基金supported by the National Natural Science Foundation of China (Nos. 21525523, 21722507, 21574048, 21874121)the National Basic Research Program of China (973 Program, No. 2015CB932600)+1 种基金the National Key R&D Program of China (Nos. 2017YFA020800, 2016YFF0100800)Natural Science Foundation of Zhejiang Province of China (No. LY18B050002)
文摘The complexity of biological samples determines that the detection of a single biomolecule is unable to satisfy actual needs. Moreover, the "false positives" results caused by a single biomolecule detections easily leads to erroneous clinical diagnosis and treatment. Thus, it is important for the homogenous quantification of multiple biomolecules in not only basic research but also practical application. As a consequent, a large number of literatures have been exploited to monitor multiple biomolecules in homogenous solution, enabling facilitating the development of the disease diagnosis, treatment as well as drug discovery. One-dimensional nanomaterials and two-dimensional nanomaterials have special physical and chemical properties, such as good electrochemical properties, stable structure, large specific surface area, and biocompatibility, which are widely used in electrochemical and fluorescent detection of biomolecules. This tutorial review highlights the recent development for the detection of multiple biomolecules by using nanomaterials including one-dimensional materials(1DMs) as well as twodimensional materials(2DMs).
基金Thanks for the financial supporting from the National Key Research and Development Program of China(Nos.2020YFA0308800 and 2019YFA0308000)the National Natural Science Foundation of China(Nos.61971035,61901038,and 61725107)+2 种基金Beijing Natural Science Foundation(Nos.Z190006 and 4192054)the Strategic Priority Research Program of Chinese Academy of Sciences(Nos.XDB30000000 and XDB28000000)the Beijing Institute of Technology Research Fund Program for Young Scholars(No.2020CX04084).
文摘Tomonaga-Luttinger liquid(TLL),a peculiar one-dimensional(1D)electronic behavior due to strong correlation,was first studied in 1D nanostructures and has attracted significant attention over the last several decades.With the rise of new two-dimensional(2D)quantum materials,1D nanostructures in 2D materials have provided a new platform with a well-defined configuration at the atomic scale for studying TLL electronic behavior.In this paper,we review the recent progress of TLL electronic features in emerging 2D materials embedded with various 1D nanostructures,including island edges,domain walls,and 1D moirépatterns.Specifically,novel physical phenomena,such as 1D edge states in 2D transition metal dichalcogenides(TMDs),helical TLL in 2D topological insulators(2DTI),and chiral TLL in 2D quantum Hall systems,are described and discussed at the nanoscale.We also analyze challenges and opportunities at the frontier of this research area.
基金Supported by the National Natural Science Foundation of China(61801024)。
文摘The concept of difference and sum co-array(DSCA)has become a new design idea for planar sparse arrays.Inspired by the shifting invariance property of DSCA,a specific configuration named here as the improved L-shaped array is proposed.Compared to other traditional 2D sparse array configurations such as 2D nested arrays and hourglass arrays,the proposed configuration has larger central consecutive ranges in its DSCA,thus increasing the DOF.At the same time,the mutual coupling effect is also reduced due to the enlarged spacing between the adjacent sensors.Simulations further demonstrate the superiority of the proposed arrays in terms of detection performance and estimation accuracy.
文摘It is an important theme in nanoscience to control the interval of the ordered array of nanoparticles through modifying the chain length of the passivating molecules of the nanoparticles. The theme runs through most of the applications of the ordered array of nanoparticles. Though the Langmuir-Blodgett (LB) technique is one of the most important ways to prepare the two-dimensional ordered array of nanoparticles, it has only been used in case that the passivating molecules are short enough (【C12). When the passivating molecules become longer, it is difficult to obtain the ordered array of the particles simply by compressing them on the surface of water. The present work focused on the formation of the two-dimensional array of the octadecyl-amine-passivated gold nanoparticles at the air/water interface. By properly modifying the ordinary LB technique, the long-term two-dimensional ordered array of nanoparticles was successfully achieved. The surface pressure-area isotherms and the electron microscopy
基金supported by the National "973" Project of China(Nos.2010CB328202,2010CB328204,and 2012CB315604)the National Natural Science Foundation of China(Nos.61271191 and 61001124)+3 种基金the National "863" Project of China(No.2012AA011302)the Program for New Century Excellent Talents in University(No.NCET-12-0793)the Beijing Nova Program(No.2011065)the Fundamental Research Funds for the Central Universities
文摘A two-dimensional(2D) optical true-time delay(TTD) beam-forming system using a compact fiber grating prism(FGP) for a planar phased array antenna(PAA) is proposed. The optical beam-forming system mainly consists of a TTD unit based on the same compact FGP, one tunable laser for elevation beam steering, and a controlled wavelength converter for azimuth beam steering. A planar PAA using such 2D optical TTD unit has advantages such as compactness, low bandwidth requirement for tunable laser sources, and potential for large-scale system implementations. The proof-of-concept experiment results demonstrate the feasibility of the proposed scheme.
基金Supported by the National Natural Science Foundation of China(No.90104034,No.60373041).
文摘Kronecker sequences constructed from short sequences are good sequences for spread spectrum communication systems. In this paper we study a similar problem for two-dimensional arrays, and we determine the linear complexity of the Kronecker product of two arrays, Our result shows that similar good property on linear complexity holds for Kronecker product of arrays.
基金This project was financially supported by the Dalian Science and Technology Innovation Fund of China(No.2019J11CY011)the Science Fund for Creative Research Groups of NSFC(No.51621064).
文摘As the basis of machine vision,the biomimetic image sensing devices are the eyes of artificial intelligence.In recent years,with the development of two-dimensional(2D)materials,many new optoelectronic devices are developed for their outstanding performance.However,there are still little sensing arrays based on 2D materials with high imaging quality,due to the poor uniformity of pixels caused by material defects and fabrication technique.Here,we propose a 2D MoS_(2)sensing array based on artificial neural network(ANN)learning.By equipping the MoS_(2)sensing array with a“brain”(ANN),the imaging quality can be effectively improved.In the test,the relative standard deviation(RSD)between pixels decreased from about 34.3%to 6.2%and 5.49%after adjustment by the back propagation(BP)and Elman neural networks,respectively.The peak signal to noise ratio(PSNR)and structural similarity(SSIM)of the image are improved by about 2.5 times,which realizes the re-recognition of the distorted image.This provides a feasible approach for the application of 2D sensing array by integrating ANN to achieve high quality imaging.
基金support from PetroChina Company Limited Innovation Foundation(Grant No.07-06D-01-04-01-07)State Key Laboratory of Petroleum Resource and Prospecting,China University of Petroleum(Beijing)(Grant No.PRPDX2008-02)
文摘In recent years, nuclear magnetic resonance (NMR) has been increasingly used for fluid- typing in well-logging because of the improved generations of NMR logging tools. This paper first discusses the applicable conditions of two one-dimensional NMR methods: the dual TW method and dual TE method. Then, the two-dimensional (T2, D) and (T2, T1) NMR methods are introduced. These different typing methods for hydrocarbon are compared and analyzed by numerical simulation. The results show that the dual TW method is not suitable for identifying a macroporous water layer. The dual TE method is not suitable for typing gas and irreducible water. (T2, T1) method is more effective in typing a gas layer. In an oil-bearing layer of movable water containing big pores, (T2, T1) method can solve the misinterpretation problem in the dual TWmethod between a water layer with big pores and an oil layer. The (T2, T1) method can distinguish irreducible water from oil of a medium viscosity, and the viscosity range of oil becomes wide in contrast with that of the dual TW method. The (T2, D) method is more effective in typing oil and water layers. In a gas layer, when the SNR is higher than a threshold, the (T2, D) method can resolve the overlapping T2 signals of irreducible water and gas that occurs due to the use of the dual TE method. Twodimensional NMR for fluid-typing is an important development of well logging technology.
基金supported by the Basic Science Research Program through the National Research Foundation of Korea funded by the Ministry of Education(NRF-2017R1D1A1A09000642)by a grant from the R&D Program of the Korea Railroad Research Institute (KRRI), Republic of Korea
文摘In the past decade, researchers in the fields of energy production have concentrated on the improvement of new energy storage devices. Lithium-ion batteries(LIBs) and faradaic supercapacitors(FSs) have attracted special attention as a result of the rapid development of new electrode nanomaterials, especially hybrid nanomaterials, which can meet the increasingly higher requirements for future energy, such as the capability to deliver high-power performance and an extremely long life cycle. In these hybrid nanostructures, a series of synergistic effects and unique properties arising from the combination of individual components are a major factor leading to improved charge/discharge capability, energy density, and system lifetime. This paper describes the most recent progress in the growth of hybrid electrode materials for LIBs and FSs systems, focusing on the combination of zero-dimensional(0 D), one-dimensional(1 D), two-dimensional(2 D), and three-dimensional(3 D) nanomaterials, respectively.
基金Y.H.acknowledges the financial support from the Office of Naval Research through award N00014-18-1-2491.X.F.D.acknowledged the support from the US Department of Energy,Office of Basic Energy Sciences,Division of Materials Science and Engineering through award DE-SC0018828(material preparation).
文摘The development of pressure sensor arrays capable of distinguishing the shape and texture details of objects is of considerable interest in the emerging fields of smart robots,prostheses,human-machine interfaces,and artificial intelligence(AI).Here we report an integrated pressure sensor array,by combining solution-processed two-dimensional(2D)MoS2 van der Waals(vdW)thin film transistor(TFT)active matrix and conductive micropyramidal pressure-sensitive rubber(PSR)electrodes made of polydimethylsiloxane/carbon nanotube composites,to achieve spatially revolved pressure mapping with excellent contrast and low power consumption.We demonstrate a 10×10 active matrix by using the 2D MoS2 vdW-TFTs with high on-off ratio>10^(6),minimal hysteresis,and excellent device-to-device uniformity.The combination of the vdW-TFT active matrix with the highly uniform micropyramidal PSR electrodes creates an integrated pressure sensing array for spatially resolved pressure mapping.This study demonstrates that the solution-processed 2D vdW-TFTs offer a solution for active-matrix control of pressure sensor arrays,and could be extended for other active-matrix arrays of electronic or optoelectronic devices.