In this study,the enhanced mineralization of p-fluoronitrobenzene(p-FNB)was achieved in a methane-based hollow-fiber membrane biofilm reactor(CH4-MBfR).A TOC removal of 73.2%was gained in CH4-MBfR with an influent p-F...In this study,the enhanced mineralization of p-fluoronitrobenzene(p-FNB)was achieved in a methane-based hollow-fiber membrane biofilm reactor(CH4-MBfR).A TOC removal of 73.2%was gained in CH4-MBfR with an influent p-FNB loading of 42―84 mg/L·d,while only 40.6%of TOC was removed in the corresponding control biological reactor(BR).Moreover,the reaction rate constant for TOC removal in CH4-MBfR was 2.48 times that of the BR.VFAs was only detected in CH4-MBfR,although oxidation elimination was the first step for p-FNB removal in both systems.Methylococcus and Methylononas were dominant strains in the CH4-MBfR,which may play an important role in converting CH4 to VFAs and then further enhancing the mineralization efficiency of p-FNB.展开更多
基金This research was supported by the National Natural Science Foundation of China(No.21307160)the Natural Science Foundation of Shandong Province(ZR2019MEE038)the Fundamental Research Funds for the Central Universities(19CX02038A).
文摘In this study,the enhanced mineralization of p-fluoronitrobenzene(p-FNB)was achieved in a methane-based hollow-fiber membrane biofilm reactor(CH4-MBfR).A TOC removal of 73.2%was gained in CH4-MBfR with an influent p-FNB loading of 42―84 mg/L·d,while only 40.6%of TOC was removed in the corresponding control biological reactor(BR).Moreover,the reaction rate constant for TOC removal in CH4-MBfR was 2.48 times that of the BR.VFAs was only detected in CH4-MBfR,although oxidation elimination was the first step for p-FNB removal in both systems.Methylococcus and Methylononas were dominant strains in the CH4-MBfR,which may play an important role in converting CH4 to VFAs and then further enhancing the mineralization efficiency of p-FNB.
