The traditional standard wet sieving method uses steel sieves with aperture?0.063 mm and can only determine the particle size distribution(PSD)of gravel and sand in general soil.This paper extends the traditional meth...The traditional standard wet sieving method uses steel sieves with aperture?0.063 mm and can only determine the particle size distribution(PSD)of gravel and sand in general soil.This paper extends the traditional method and presents an extended wet sieving method.The extended method uses both the steel sieves and the nylon filter cloth sieves.The apertures of the cloth sieves are smaller than 0.063 mm and equal 0.048 mm,0.038 mm,0.014 mm,0.012 mm,0.0063 mm,0.004 mm,0.003 mm,0.002 mm,and 0.001 mm,respectively.The extended method uses five steps to separate the general soil into many material sub-groups of gravel,sand,silt and clay with known particle size ranges.The complete PSD of the general soil is then calculated from the dry masses of the individual material sub-groups.The extended method is demonstrated with a general soil of completely decomposed granite(CDG)in Hong Kong,China.The silt and clay materials with different particle size ranges are further examined,checked and verified using stereomicroscopic observation,physical and chemical property tests.The results further confirm the correctness of the extended wet sieving method.展开更多
Ten rock samples consisting of one pyroclastic density current(PDC1)deposit,seven lava flows(LF1–7),and two summit lava domes(LD1,2)were studied to understand the petrogenesis and magma dynamics at Mt.Sumbing.The str...Ten rock samples consisting of one pyroclastic density current(PDC1)deposit,seven lava flows(LF1–7),and two summit lava domes(LD1,2)were studied to understand the petrogenesis and magma dynamics at Mt.Sumbing.The stratigraphy is arranged as LF1,PDC1,LF2,LF3,LF4,LF5,LF6,LF7,LD1,and LD2;furthermore,these rocks were divided into two types.TypeⅠ,observed in the oldest(LF1)sample,has poor MgO and high Ba/Nb,Th/Yb and Sr.The remaining samples(PDC1–LD2)represent typeⅡ,characterized by high MgO and low Ba/Nb,Th/Yb and Sr values.We suggest that type I is derived from AOC(altered oceanic crust)-rich melts that underwent significant crustal assimilation,while typeⅡoriginates from mantle-rich melts with less significant crustal assimilation.The early stage of typeⅡmagma(PDC1–LF3)was considered a closed system,evolving basaltic andesite into andesite(55.0–60.2 wt%SiO_(2))with a progressively increasing phenocryst(0.30–0.48φ_(PC))and decreasing crystal size distribution(CSD)slope(from-3.9 to-2.9).The evidence of fluctuating silica and phenocryst contents(between 55.9–59.7 wt%and 0.25–0.41φ_(PC),respectively),coupled with the kinked and steep(from-5.0 to-3.3)CSD curves imply the interchanging condition between open(i.e.,magma mixing)and closed magmatic systems during the middle stage(LF4–LF6).Finally,it underwent to closed system again during the final stage(LF7–LD2)because the magma reached dacitic composition(at most 68.9 wt%SiO_(2))with abundant phenocryst(0.38–0.45φ_(PC))and gentle CSD slope(from-4.1 to-1.2).展开更多
Sea salt aerosols play a critical role in regulating the global climate through their interactions with solar radiation.The size distribution of these particles is crucial in determining their bulk optical properties....Sea salt aerosols play a critical role in regulating the global climate through their interactions with solar radiation.The size distribution of these particles is crucial in determining their bulk optical properties.In this study,we analyzed in situ measured size distributions of sea salt aerosols from four field campaigns and used multi-mode lognormal size distributions to fit the data.We employed super-spheroids and coated super-spheroids to account for the particles’non-sphericity,inhomogeneity,and hysteresis effect during the deliquescence and crystallization processes.To compute the singlescattering properties of sea salt aerosols,we used the state-of-the-art invariant imbedding T-matrix method,which allows us to obtain accurate optical properties for sea salt aerosols with a maximum volume-equivalent diameter of 12μm at a wavelength of 532 nm.Our results demonstrated that the particle models developed in this study were successful in replicating both the measured depolarization and lidar ratios at various relative humidity(RH)levels.Importantly,we observed that large-size particles with diameters larger than 4μm had a substantial impact on the optical properties of sea salt aerosols,which has not been accounted for in previous studies.Specifically,excluding particles with diameters larger than 4μm led to underestimating the scattering and backscattering coefficients by 27%−38%and 43%−60%,respectively,for the ACE-Asia field campaign.Additionally,the depolarization ratios were underestimated by 0.15 within the 50%−70%RH range.These findings emphasize the necessity of considering large particle sizes for optical modeling of sea salt aerosols.展开更多
The particle composition and spatial distribution of landslide-induced dam bodies are critical geotechnical parameters for studying the hazards of dam-break floods.However,current research often neglects the influence...The particle composition and spatial distribution of landslide-induced dam bodies are critical geotechnical parameters for studying the hazards of dam-break floods.However,current research often neglects the influence of the initial particle composition and spatial distribution of the landslide on the particle composition and spatial distribution of the landslide dam.This study investigated the impact of initial particle size distribution,volume,and sliding length on the energy and velocity changes of characteristic particles during the sliding process and the spatial distribution of particle sizes in the landslide dam body.Numerical simulations and physical models were employed to examine the effects of sequential gradient arrangements(where particle sizes decrease from top to bottom)and four other different initial particle arrangements on the energy and velocity changes of particles and the spatial distribution of particle sizes in the dam body.The study reveals the characteristics of translational and rotational energy of different particles and the laws of mechanical energy conversion,obtaining the spatial distribution patterns of particle sizes in landslide-induced dams.The results show that under the sequential gradient arrangement,the energy dissipation of the landslide movement is lower,with larger particles mainly distributed at the distal end and smaller particles at the proximal end of the landslide dam.In contrast,under the reverse gradient arrangement,the energy dissipation of the landslide movement is higher,and the distribution pattern of the dam particles is opposite to that of the sequential gradient arrangement.For the other arrangement modes,the spatial distribution of dam particles falls between the aforementioned two.There is a positive correlation between particle size and translational kinetic energy within the particle flow during the landslide process,and rotational motion increases energy dissipation.Under constant slope conditions,sliding length does not affect the movement pattern of the particle flow or the spatial distribution of particles in the dam body.The findings of this study provide a scientific basis for the accurate simulation and prediction of dam-break flood processes.展开更多
Meroplankton play a crucial role in both benthic and pelagic ecosystems.Existing quantitative research on estimating the quantities of meroplankton groups is both underrepresented and inaccurate.To investigate and eva...Meroplankton play a crucial role in both benthic and pelagic ecosystems.Existing quantitative research on estimating the quantities of meroplankton groups is both underrepresented and inaccurate.To investigate and evaluate the influence of varying mesh sizes(505 and 160μm)on the sampling efficiency of meroplankton,we conducted an examination using two commonly used plankton nets during the spring season in the Southern Yellow Sea(SYS).Our study revealed a total of 12 meroplankton groups,with 9 groups identified in the 505-μm mesh nets and 11 groups in the 160-μm mesh nets.The results demonstrated the superior collection efficiency of the 160-μm net compared to the 505-μm net across the majority of meroplankton groups.Furthermore,we focused on exploring the abundance,distribution patterns,and realized niches of meroplankton collected by the two mesh size nets,and observed that the distribution of meroplankton closely resembled the distribution of possible benthic adults in the SYS.Correlation analysis of the six dominant groups collected in the 160-μm mesh nets revealed that seawater temperature and salinity emerged as the key environmental factors driving variations in meroplankton abundance within the SYS.This study also found that a smaller mesh size net does not necessarily capture meroplankton more comprehensively.A comprehensive understanding of the ecological characteristics of meroplankton requires the combination of two types of nets for research.Our research significantly advances our understanding of the quantification,abundance,and distribution of meroplankton,serving as a valuable contribution to the broader landscape of detailed quantitative meroplankton studies.展开更多
The distribution of adsorbent particle sizes typically has a significant impact on adsorption performance.Most fixed-bed adsorption studies adopt the assumption of average particle size to simplify the adsorption mode...The distribution of adsorbent particle sizes typically has a significant impact on adsorption performance.Most fixed-bed adsorption studies adopt the assumption of average particle size to simplify the adsorption model,but this does not eliminate the deviation between experiments and simulations caused by particle size distribution in practice.In this study,the population balance equation(PBE)and fixed-bed adsorption kinetics model were combined to simulate the adsorption process in a fixed-bed reactor,modeling the distribution of adsorbate uptake over time on adsorbent particles of different sizes.We integrated and optimized the PBE and fixed-bed mass transfer model in the algorithm,and the resulting combined model adopts a variable time step size,which can achieve a balance between computational efficiency and error while ensuring computational convergence.By slicing the model in the spatial dimension,multiple sets of PBE can be calculated in parallel,improving computational efficiency.The adsorption process of single-component and multi-component CO_(2)/CH_(4)/N_(2)on 4A zeolite without binder was simulated,and the influence of adsorbent particle size distribution was analyzed.Simulation results show that the assumption of average adsorbent particle size,which was commonly made in published work,will underestimate the time required for adsorbates to break through the fixed bed compared with the assumption of uniform adsorbent particle size.This model helps to consider the impact of adsorbent particle size distribution on the adsorption process,thereby improving the prediction accuracy of adsorbent performance.展开更多
Pore size analysis plays a pivotal role in unraveling reservoir behavior and its intricate relationship with confined fluids.Traditional methods for predicting pore size distribution(PSD),relying on drilling cores or ...Pore size analysis plays a pivotal role in unraveling reservoir behavior and its intricate relationship with confined fluids.Traditional methods for predicting pore size distribution(PSD),relying on drilling cores or thin sections,face limitations associated with depth specificity.In this study,we introduce an innovative framework that leverages nuclear magnetic resonance(NMR)log data,encompassing clay-bound water(CBW),bound volume irreducible(BVI),and free fluid volume(FFV),to determine three PSDs(micropores,mesopores,and macropores).Moreover,we establish a robust pore size classification(PSC)system utilizing ternary plots,derived from the PSDs.Within the three studied wells,NMR log data is exclusive to one well(well-A),while conventional well logs are accessible for all three wells(well-A,well-B,and well-C).This distinction enables PSD predictions for the remaining two wells(B and C).To prognosticate NMR outputs(CBW,BVI,FFV)for these wells,a two-step deep learning(DL)algorithm is implemented.Initially,three feature selection algorithms(f-classif,f-regression,and mutual-info-regression)identify the conventional well logs most correlated to NMR outputs in well-A.The three feature selection algorithms utilize statistical computations.These algorithms are utilized to systematically identify and optimize pertinent input features,thereby augmenting model interpretability and predictive efficacy within intricate data-driven endeavors.So,all three feature selection algorithms introduced the number of 4 logs as the most optimal number of inputs to the DL algorithm with different combinations of logs for each of the three desired outputs.Subsequently,the CUDA Deep Neural Network Long Short-Term Memory algorithm(CUDNNLSTM),belonging to the category of DL algorithms and harnessing the computational power of GPUs,is employed for the prediction of CBW,BVI,and FFV logs.This prediction leverages the optimal logs identified in the preceding step.Estimation of NMR outputs was done first in well-A(80%of data as training and 20%as testing).The correlation coefficient(CC)between the actual and estimated data for the three outputs CBW,BVI and FFV are 95%,94%,and 97%,respectively,as well as root mean square error(RMSE)was obtained 0.0081,0.098,and 0.0089,respectively.To assess the effectiveness of the proposed algorithm,we compared it with two traditional methods for log estimation:multiple regression and multi-resolution graph-based clustering methods.The results demonstrate the superior accuracy of our algorithm in comparison to these conventional approaches.This DL-driven approach facilitates PSD prediction grounded in fluid saturation for wells B and C.Ternary plots are then employed for PSCs.Seven distinct PSCs within well-A employing actual NMR logs(CBW,BVI,FFV),in conjunction with an equivalent count within wells B and C utilizing three predicted logs,are harmoniously categorized leading to the identification of seven distinct pore size classification facies(PSCF).this research introduces an advanced approach to pore size classification and prediction,fusing NMR logs with deep learning techniques and extending their application to nearby wells without NMR log.The resulting PSCFs offer valuable insights into generating precise and detailed reservoir 3D models.展开更多
Characterizing soil particle-size distribution is a key measure towards soil property.The purpose of this study was to evaluate the multifractal characteristics of soil particle-size distribution among different land-...Characterizing soil particle-size distribution is a key measure towards soil property.The purpose of this study was to evaluate the multifractal characteristics of soil particle-size distribution among different land-use from a purple soil catchment and to generalize the spatial variation trend of multifractal parameters across the catchment.A total of 84 soil samples were collected from four kinds of land use patterns(dry land,orchard,paddy,and forest)in an agricultural catchment in the Three Gorges Reservoir Region,China.The multifractal analysis method was applied to quantitatively characterize the soil particle size distribution.Six soil particle size distribution(PSD)multifractal parameters(D(0),D(1),D(2),(35)a(q),(35)f[a(q)],α(0))were computed.Additionally,a geostatistical analysis was employed to reveal the spatial differentiation and map the spatial distribution of these parameters.Evident multifractal characteristics were found.The trend of generalized dimension spectrum of four land use patterns was basically consistent with the range of 0.8 to 2.0.However,orchard showed the largest monotonic decline,while the forest demonstrated the smallest decrease.D(0)of the four land use patterns were ranked as:dry land<orchard<forest<paddy,the order of D(1)was:dry land<paddy<orchard<forest,D(2)presented a rand-size relationship as dry land<forest<paddy<orchard.Furthermore,all land-use patterns presented asΔf[α(q)]<0.The rand-size relationship ofα(0)was same as D(0).The best-fitting model for D(0),D(1),D(2)andΔf[α(q)]was spherical model,forΔα(q)was gaussian model,and forα(0)was exponential model with structure variance ratio was 1.03%,49.83%,0.84%,1.48%,22.20%and 10.60%,respectively.The results showed that soil particles of each land use pattern were distributed unevenly.The multifractal parameters under different land use have significant differences,except forΔα(q).Differences in the composition of soil particles lead to differences in the multifractal properties even though they belong to the same soil texture.Farming behavior may refine particles and enhance the heterogeneity of soil particle distribution.Our results provide an effective reference for quantifying the impact of human activities on soil system in the Three Gorges Reservoir region.展开更多
Application of particle image velocity (PIV) techniques for measuringparticle size distribution and total number in an activation chamber of desulfurization system isintroduced. Watersheld algorithm is used to choose ...Application of particle image velocity (PIV) techniques for measuringparticle size distribution and total number in an activation chamber of desulfurization system isintroduced. Watersheld algorithm is used to choose the suitable initial gray level threshold whichis used to change the gray level images taken by PIV to black and white ones, then every particle inan image is isolated totally. For every isolating particle, its contour is tracked by the edgeenhancement filter function and kept by Freeman s chain code. Based on a set of particle s chincode, its size and size distribution are calculated and sorted. Finally, the experimental data ofcalcium particles and water drops, separately injected into the activation chamber, and the erroranalysis of data are given out.展开更多
Size distribution characteristics of intercity bus hubs in China from 1997 to 2(104 were analyzed regarding highway passenger volume as a size index of intercity bus hubs. Yearly fractal dimensions of intercity bus h...Size distribution characteristics of intercity bus hubs in China from 1997 to 2(104 were analyzed regarding highway passenger volume as a size index of intercity bus hubs. Yearly fractal dimensions of intercity bus hub sizes were exactly calculated by a novel model. Fractal dimensions of the 200 biggest intercity bus hubs from 2000 to 2004 were 1. 486 2 to 1. 511 8, and that is consistent with fractal dimensions of Chinese urban system sizes. It showed that the size distribution of intercity bus hubs had fractal structure. Fractal dimensions from 1997 to 2004 indicated that intercity bus hub size distribution grew from bi-fractal to single fractal. It is concluded that the intercity bus hub system is in evolutionary progress, and the Central Government should support large intercity bus hubs more to optimize system structure.展开更多
The characteristics of raindrop size distribution (DSD) over the Tibetan Plateau and southern China are studied in this paper, using the DSD data from April to August 2014 collected by HSC-PS32 disdrometers in Nagqu...The characteristics of raindrop size distribution (DSD) over the Tibetan Plateau and southern China are studied in this paper, using the DSD data from April to August 2014 collected by HSC-PS32 disdrometers in Nagqu and Yangjiang, com- prising a total of 9430 and 63661-rain raindrop spectra, respectively. The raindrop spectra, characteristics of parameter variations with rainfall rate, and the relationships between reflectivity factor (Z) and rainfall rate (R) are analyzed, as well as their DSD changes with precipitation type and rainfall rate. The results show that the average raindrop spectra appear to be one-peak curves, the number concentration for larger drops increase significantly with rainfall rate, and its value over southern China is much higher, especially in convective rain larger drops, especially for convective rain in southern China. Standardized Gamma distributions better describe DSD for All three Gamma parameters for stratiform precipitation over the Tibetan Plateau are much higher, while its shape parameter (,u) and mass-weighted mean diameter (Dm), for convective precipitation, are less. In terms of parameter variation with rainfall rate, the normalized intercept parameter (Nw) over the Tibetan Plateau for stratiform rain increases with rainfall rate, which is opposite to the situation in convective rain. The/1 over the Tibetan Plateau for stratiform and convective precipitation types decreases with an increase in rainfall rate, which is opposite to the case for Dm variation. In Z-R relationships, like "Z = ARb'', the coefficient A over the Tibetan Plateau is smaller, while its b is higher, when the rain type transfers from stratiform to convective ones. Furthermore, with an increase in rainfall rate, parameters A and b over southern China increase gradually, while A over the Tibetan Plateau decreases sub- stantially, which differs from the findings of previous studies. In terms of geographic location and climate over the Tibetan Plateau and southern China, the precipitation in the pre-flood seasons is dominated by strong convective rain, while weak convective rain occurs frequently in northern Tibet with lower humidity and higher altitude.展开更多
The aerosol number concentration and size distribution were measured with the newly developed Wide-range Particle Spectrometer in summer and winter of 2006 at the urban site of Jinan City. Here reported the characteri...The aerosol number concentration and size distribution were measured with the newly developed Wide-range Particle Spectrometer in summer and winter of 2006 at the urban site of Jinan City. Here reported the characteristics of fine particles of the different observation seasons. Relative high number concentrations for the particles in the diameter range of 10-500 nm were observed in both seasons. It was found that the dominant number distributed in particle diameter smaller than 100 nm and the percentage over the number concentration of all air particles is much higher than what has been measured in other urban sites over the world. The number mean diameter in summer was much smaller than in winter, strongly suggesting the different origin of ultrafine particles in different seasons. That is, particles in ultrafine mode mainly came from nucleation and new particle formation in summer while from traffic emission in winter. The diurnal variation also supported this point. Number concentration in the diameter range of 10-200 um got their peak values at noontime, well correlated with the mixing ratio of SO2 and the intensity of solar radiation in summer. While in winter, those in the same diameter range showed the main peaks during the traffic hours happened in the morning and evening.展开更多
Seasonal variations of rainfall microphysics in East China are investigated using data from the observations of a twodimensional video disdrometer and a vertically pointing micro rain radar. The precipitation and rain...Seasonal variations of rainfall microphysics in East China are investigated using data from the observations of a twodimensional video disdrometer and a vertically pointing micro rain radar. The precipitation and rain drop size distribution(DSD) characteristics are revealed for different rain types and seasons. Summer rainfall is dominated by convective rain,while during the other seasons the contribution of stratiform rain to rainfall amount is equal to or even larger than that of convective rain. The mean mass-weighted diameter versus the generalized intercept parameter pairs of convective rain are plotted roughly around the "maritime" cluster, indicating a maritime nature of convective precipitation throughout the year in East China. The localized rainfall estimators, i.e., rainfall kinetic energy–rain rate, shape–slope, and radar reflectivity–rain rate relations are further derived. DSD variability is believed to be a major source of diversity of the aforementioned derived estimators. These newly derived relations would certainly improve the accuracy of rainfall kinetic energy estimation, DSD retrieval, and quantitative precipitation estimation in this specific region.展开更多
Microphysical characteristics of the raindrop size distribution(RSD)in Typhoon Morakot(2009) have been studied through the PARSIVEL disdrometer measurements at one site in Fujian province,China during the passage of t...Microphysical characteristics of the raindrop size distribution(RSD)in Typhoon Morakot(2009) have been studied through the PARSIVEL disdrometer measurements at one site in Fujian province,China during the passage of the storm from 7 to 10 August 2009.The time evolution of the RSD reveals different segments of the storm.Significant difference was observed in the microphysical characteristics between the outer rainband and the eyewall;the eyewall precipitation had a broader size distribution(a smaller slope) than the outer rainband and eye region.The outer rainband and the eye region produced stratiform rains while the eyewall precipitation was convective or mixed stratiform-convective.The RSD was typically characterized by a single peak distribution and well represented by the gamma distribution.The relations between the shape(μ)and slope(Λ)of the gamma distribution and between the reflectivity(Z)and rainfall rate(R)have been investigated.Based on the NW-Dm relationships,we suggest that the stratiform rain for the outer rainband and the eye region was formed by the melting of graupel or rimed ice particles,which likely originated from the eyewall clouds.展开更多
Particles of dust washed off streets by stormwater are an important pathway of polyaromatic hydrocarbons (PAHs) into urban streams. This article presented a comprehensive assessment of the size distribution of PAHs ...Particles of dust washed off streets by stormwater are an important pathway of polyaromatic hydrocarbons (PAHs) into urban streams. This article presented a comprehensive assessment of the size distribution of PAHs in street dust particles, the potential risks of the particles in urban streams, and the sources and sinks of PAHs in the stream network. This assessment was based on measurements of 16 PAHs from the USEPA priority list in street dust particles and river sediments in Xincheng, China. The content of total PAHs ranged from 1629 to 8986 Dg/kg in street dust particles, where smaller particles have a higher concentrations. Approximately 55% of the total PAHs were associated with particles less than 250 μm which accounted for 40% of the total mass of street dust. The PAH quantities increased from 2.41 to 46.86 μg/m2 in the sequence of new residential, rising through main roads, old town residential, commercial and industrial areas. The sediments in stream reaches in town were found to be sinks for street dust particle PAHs. The research findings suggested that particle size, land use and the hydrological conditions in the stream network were the factors which most influenced the total loads of PAH in the receiving water bodies.展开更多
This article reports the morphology, size, and distribution evolution of MnS inclusions in non-quenched and tempered steel during heat treatment. The variation of single large-sized MnS inclusions at high temperature ...This article reports the morphology, size, and distribution evolution of MnS inclusions in non-quenched and tempered steel during heat treatment. The variation of single large-sized MnS inclusions at high temperature was observed in situ using a confocal scanning laser microscope (CSLM). The slender MnS inclusions first changed to pearl-like slrings. These small-sized pearls subsequently coalesced and became closer together as the temperature increased. Large-sized MnS inclusions in non-quenched and tempered steel samples with different thermal histories were investigated with respect to the evolution of their morphology, size, and distribution. After 30 min of ovulation at 1573 K, the percentage of MnS inclusions larger than 3 μm decreased from 50.5% to 3.0%. After a 3 h making period, Ostwald ripening occurred. Most MnS inclusions moved from the grain bounda- ries to the interior. The present study demonstrates that heat treatment is an effective method of changing the morphology, size, and distribution of MnS inclusions, especially large-sized ones.展开更多
Nanobubble flotation technology is an important research topic in the field of fine mineral particle separation.The basic characteristics of nanobubbles,including their size,concentration,surface zeta potential,and st...Nanobubble flotation technology is an important research topic in the field of fine mineral particle separation.The basic characteristics of nanobubbles,including their size,concentration,surface zeta potential,and stability have a significant impact on the nanobubble flotation performance.In this paper,bulk nanobubbles generated based on the principle of hydrodynamic cavitation were investigated to determine the effects of different parameters(e.g.,surfactant(frother)dosage,air flow,air pressure,liquid flow rate,and solution pH value)on their size distribution and zeta potential,as measured using a nanoparticle analyzer.The results demonstrated that the nanobubble size decreased with increasing pH value,surfactant concentration,and cavitation-tube liquid flow rate but increased with increasing air pressure and increasing air flow rate.The magnitude of the negative surface charge of the nanobubbles was positively correlated with the pH value,and a certain relationship was observed between the zeta potential of the nanobubbles and their size.The structural parameters of the cavitation tube also strongly affected the characteristics of the nanobubbles.The results of this study offer certain guidance for optimizing the nanobubble flotation technology.展开更多
Total suspended particulates (TSP) samples were collected using low pressure impactors (Andersen Series 20-800, USA) on typical clear, hazy and foggy days in Beijing in order to investigate the characteristics of ...Total suspended particulates (TSP) samples were collected using low pressure impactors (Andersen Series 20-800, USA) on typical clear, hazy and foggy days in Beijing in order to investigate the characteristics of size distributions and elemental compositions of particulate matter (PM) in different weather conditions. The concentrations of sixteen elements, including Na, Mg, Al, K, Ca, Mn, Fe, Ni, Cu, Zn, As, Se, Cd, Ba, T1 and Pb were detected using inductively coupled plasma mass spectrometry (ICP-MS). The results showed that Ca, A1, Fe, Mg and Ba on foggy days were 2.0 2.6 times higher than on clear days, and 2.3-2.9 times higher than on hazy days. Concentrations of Cu, Zn, As, Se and Pb on foggy days were 163.5, 1186.7, 65.9, 32.0 and 708.2 ng m-3, respectively, in fine particles, and 68.1, 289.5, 19.8, 1.6 and 103.8 ng m-3, respectively, in coarse particles. This was 1.0~8.4 times higher and 1.4-7.4 times higher than on clear and hazy days, respectively. It is then shown that Mg, A1, Fe, Ca and Ba were mainly associated with coarse particles, peaking at 4.7~5.8 μm; that Cd, Se, Zn, As, T1 and Pb were most dominant in fine particles, peaking at 0.43-1.1 μm; and that Na, K, Ni, Cu and Mn had a multi-mode distribution, with peaks at 0.43-1.1 μm and 4.7-5.8 μm. The enrichment factors indicated that coal combustion along with vehicle and industry emissions may be the main sources of pollution elements.展开更多
For the 2008 Olympic Games, drastic control measures were implemented on industrial and urban emissions of sulfur dioxide (SO2), nitrogen oxides (NOx) and other pollutants to address the issues of poor air quality...For the 2008 Olympic Games, drastic control measures were implemented on industrial and urban emissions of sulfur dioxide (SO2), nitrogen oxides (NOx) and other pollutants to address the issues of poor air quality in Beijing. To investigate the effects of SO2 and NOx reductions on the particulate sulfate and nitrate concentrations as well as their size distributions, size-segregated aerosol samples were collected using micro-orifice uniform deposit impactors (MOUDIs) at urban and downwind rural sites in Beijing before and after full-scale controls. During the sampling period, the mass concentrations of fine particles (PMI.s) at the urban and rural sites were 94.0 and 85.9 p.g m-3, respectively. More than 90% of the sulfates and 60% of nitrates formed as fine particles. Benefiting from the advantageous meteorological conditions and the source controls, sulfates were observed in rather low concentrations and primarily in condensation mode during the Olympics. The effects of the control measures were separately analyzed for the northerly and the southerly air-mass-dominated days to account for any bias. After the control measures were implemented, PM, sulfates, and nitrates were significantly reduced when the northerly air masses prevailed, with a higher percentage of reduction in larger particles. The droplet mode particles, which dominated the sulfates and nitrates before the controls were implemented, were remarkably reduced in mass concentration after the control measures were implemented. Nevertheless, when the polluted southerly air masses prevailed, the local source control measures in Beijing did not effectively reduce the ambient sulfate concentration due to the enormous regional contribution from the North China Plain.展开更多
Granule size distribution of wheat starch is an important characteristic that can affect its chemical composition and the functionality of wheat products. Two high-yield winter wheat cultivars were used to evaluate th...Granule size distribution of wheat starch is an important characteristic that can affect its chemical composition and the functionality of wheat products. Two high-yield winter wheat cultivars were used to evaluate the effects of the application of exogenous ABA or GA during the reproductive phase of the initial grain filling on starch granule size distribution and starch components in grains at maturity. The results indicated that a bimodal curve was found in the volume and surface area distribution of grain starch granules, and a unimodal curve was observed for the number distribution under all treatments. The exogenous ABA resulted in a significant increase in the proportions (both by volume and by surface area) of B-type (〈9.9 Ixm in diameter) starch granules, with a reduction in those of A-type (〉9.9 ~tm) starch granules, while, the exogenous GA3 led to converse effects on size distribution of those starch granules. The exogenous ABA also increased starch, amylose and amylopectin contents at maturity but significantly reduced the ratio of amylose to amylopectin. Application of GA3 significantly reduced starch content, amylopectin content but increased the ratio of amylose to amylopectin. The ratio of amylose to amylopectin showed a significant and negative relationship with the volume proportion of granules 〈9.9 μm, but was positively related to the volume proportion of granules 22.8-42.8 μm.展开更多
基金The work described in this paper was partially supported by grants from the Research Grant Council of the Hong Kong Special Administrative Region,China(Project Nos.HKU 17207518 and R5037-18).
文摘The traditional standard wet sieving method uses steel sieves with aperture?0.063 mm and can only determine the particle size distribution(PSD)of gravel and sand in general soil.This paper extends the traditional method and presents an extended wet sieving method.The extended method uses both the steel sieves and the nylon filter cloth sieves.The apertures of the cloth sieves are smaller than 0.063 mm and equal 0.048 mm,0.038 mm,0.014 mm,0.012 mm,0.0063 mm,0.004 mm,0.003 mm,0.002 mm,and 0.001 mm,respectively.The extended method uses five steps to separate the general soil into many material sub-groups of gravel,sand,silt and clay with known particle size ranges.The complete PSD of the general soil is then calculated from the dry masses of the individual material sub-groups.The extended method is demonstrated with a general soil of completely decomposed granite(CDG)in Hong Kong,China.The silt and clay materials with different particle size ranges are further examined,checked and verified using stereomicroscopic observation,physical and chemical property tests.The results further confirm the correctness of the extended wet sieving method.
基金funded by the Faculty of Geography under the scheme of“Dana Hibah Penelitian Mandiri Dosen Tahun 2023 Tahap 1”。
文摘Ten rock samples consisting of one pyroclastic density current(PDC1)deposit,seven lava flows(LF1–7),and two summit lava domes(LD1,2)were studied to understand the petrogenesis and magma dynamics at Mt.Sumbing.The stratigraphy is arranged as LF1,PDC1,LF2,LF3,LF4,LF5,LF6,LF7,LD1,and LD2;furthermore,these rocks were divided into two types.TypeⅠ,observed in the oldest(LF1)sample,has poor MgO and high Ba/Nb,Th/Yb and Sr.The remaining samples(PDC1–LD2)represent typeⅡ,characterized by high MgO and low Ba/Nb,Th/Yb and Sr values.We suggest that type I is derived from AOC(altered oceanic crust)-rich melts that underwent significant crustal assimilation,while typeⅡoriginates from mantle-rich melts with less significant crustal assimilation.The early stage of typeⅡmagma(PDC1–LF3)was considered a closed system,evolving basaltic andesite into andesite(55.0–60.2 wt%SiO_(2))with a progressively increasing phenocryst(0.30–0.48φ_(PC))and decreasing crystal size distribution(CSD)slope(from-3.9 to-2.9).The evidence of fluctuating silica and phenocryst contents(between 55.9–59.7 wt%and 0.25–0.41φ_(PC),respectively),coupled with the kinked and steep(from-5.0 to-3.3)CSD curves imply the interchanging condition between open(i.e.,magma mixing)and closed magmatic systems during the middle stage(LF4–LF6).Finally,it underwent to closed system again during the final stage(LF7–LD2)because the magma reached dacitic composition(at most 68.9 wt%SiO_(2))with abundant phenocryst(0.38–0.45φ_(PC))and gentle CSD slope(from-4.1 to-1.2).
基金supported by the National Natural Science Foundation of China(Grant Nos.42022038,and 42090030).
文摘Sea salt aerosols play a critical role in regulating the global climate through their interactions with solar radiation.The size distribution of these particles is crucial in determining their bulk optical properties.In this study,we analyzed in situ measured size distributions of sea salt aerosols from four field campaigns and used multi-mode lognormal size distributions to fit the data.We employed super-spheroids and coated super-spheroids to account for the particles’non-sphericity,inhomogeneity,and hysteresis effect during the deliquescence and crystallization processes.To compute the singlescattering properties of sea salt aerosols,we used the state-of-the-art invariant imbedding T-matrix method,which allows us to obtain accurate optical properties for sea salt aerosols with a maximum volume-equivalent diameter of 12μm at a wavelength of 532 nm.Our results demonstrated that the particle models developed in this study were successful in replicating both the measured depolarization and lidar ratios at various relative humidity(RH)levels.Importantly,we observed that large-size particles with diameters larger than 4μm had a substantial impact on the optical properties of sea salt aerosols,which has not been accounted for in previous studies.Specifically,excluding particles with diameters larger than 4μm led to underestimating the scattering and backscattering coefficients by 27%−38%and 43%−60%,respectively,for the ACE-Asia field campaign.Additionally,the depolarization ratios were underestimated by 0.15 within the 50%−70%RH range.These findings emphasize the necessity of considering large particle sizes for optical modeling of sea salt aerosols.
基金reported in this manuscript is funded by the National Natural Science Foundation of China(Grant No.52130904).
文摘The particle composition and spatial distribution of landslide-induced dam bodies are critical geotechnical parameters for studying the hazards of dam-break floods.However,current research often neglects the influence of the initial particle composition and spatial distribution of the landslide on the particle composition and spatial distribution of the landslide dam.This study investigated the impact of initial particle size distribution,volume,and sliding length on the energy and velocity changes of characteristic particles during the sliding process and the spatial distribution of particle sizes in the landslide dam body.Numerical simulations and physical models were employed to examine the effects of sequential gradient arrangements(where particle sizes decrease from top to bottom)and four other different initial particle arrangements on the energy and velocity changes of particles and the spatial distribution of particle sizes in the dam body.The study reveals the characteristics of translational and rotational energy of different particles and the laws of mechanical energy conversion,obtaining the spatial distribution patterns of particle sizes in landslide-induced dams.The results show that under the sequential gradient arrangement,the energy dissipation of the landslide movement is lower,with larger particles mainly distributed at the distal end and smaller particles at the proximal end of the landslide dam.In contrast,under the reverse gradient arrangement,the energy dissipation of the landslide movement is higher,and the distribution pattern of the dam particles is opposite to that of the sequential gradient arrangement.For the other arrangement modes,the spatial distribution of dam particles falls between the aforementioned two.There is a positive correlation between particle size and translational kinetic energy within the particle flow during the landslide process,and rotational motion increases energy dissipation.Under constant slope conditions,sliding length does not affect the movement pattern of the particle flow or the spatial distribution of particles in the dam body.The findings of this study provide a scientific basis for the accurate simulation and prediction of dam-break flood processes.
基金Supported by the Laoshan Laboratory(Nos.LSKJ 202203700,LSKJ 202203704,LSKJ 202204005)the National Natural Science Foundation of China(NSFC)(Nos.42076166,42130411)the NSFC Ship Time Sharing Project(No.42149901)。
文摘Meroplankton play a crucial role in both benthic and pelagic ecosystems.Existing quantitative research on estimating the quantities of meroplankton groups is both underrepresented and inaccurate.To investigate and evaluate the influence of varying mesh sizes(505 and 160μm)on the sampling efficiency of meroplankton,we conducted an examination using two commonly used plankton nets during the spring season in the Southern Yellow Sea(SYS).Our study revealed a total of 12 meroplankton groups,with 9 groups identified in the 505-μm mesh nets and 11 groups in the 160-μm mesh nets.The results demonstrated the superior collection efficiency of the 160-μm net compared to the 505-μm net across the majority of meroplankton groups.Furthermore,we focused on exploring the abundance,distribution patterns,and realized niches of meroplankton collected by the two mesh size nets,and observed that the distribution of meroplankton closely resembled the distribution of possible benthic adults in the SYS.Correlation analysis of the six dominant groups collected in the 160-μm mesh nets revealed that seawater temperature and salinity emerged as the key environmental factors driving variations in meroplankton abundance within the SYS.This study also found that a smaller mesh size net does not necessarily capture meroplankton more comprehensively.A comprehensive understanding of the ecological characteristics of meroplankton requires the combination of two types of nets for research.Our research significantly advances our understanding of the quantification,abundance,and distribution of meroplankton,serving as a valuable contribution to the broader landscape of detailed quantitative meroplankton studies.
基金the National Natural Science Foundation of China (21706075)Guangzhou Municipal Science and Technology Project (202201011269)
文摘The distribution of adsorbent particle sizes typically has a significant impact on adsorption performance.Most fixed-bed adsorption studies adopt the assumption of average particle size to simplify the adsorption model,but this does not eliminate the deviation between experiments and simulations caused by particle size distribution in practice.In this study,the population balance equation(PBE)and fixed-bed adsorption kinetics model were combined to simulate the adsorption process in a fixed-bed reactor,modeling the distribution of adsorbate uptake over time on adsorbent particles of different sizes.We integrated and optimized the PBE and fixed-bed mass transfer model in the algorithm,and the resulting combined model adopts a variable time step size,which can achieve a balance between computational efficiency and error while ensuring computational convergence.By slicing the model in the spatial dimension,multiple sets of PBE can be calculated in parallel,improving computational efficiency.The adsorption process of single-component and multi-component CO_(2)/CH_(4)/N_(2)on 4A zeolite without binder was simulated,and the influence of adsorbent particle size distribution was analyzed.Simulation results show that the assumption of average adsorbent particle size,which was commonly made in published work,will underestimate the time required for adsorbates to break through the fixed bed compared with the assumption of uniform adsorbent particle size.This model helps to consider the impact of adsorbent particle size distribution on the adsorption process,thereby improving the prediction accuracy of adsorbent performance.
文摘Pore size analysis plays a pivotal role in unraveling reservoir behavior and its intricate relationship with confined fluids.Traditional methods for predicting pore size distribution(PSD),relying on drilling cores or thin sections,face limitations associated with depth specificity.In this study,we introduce an innovative framework that leverages nuclear magnetic resonance(NMR)log data,encompassing clay-bound water(CBW),bound volume irreducible(BVI),and free fluid volume(FFV),to determine three PSDs(micropores,mesopores,and macropores).Moreover,we establish a robust pore size classification(PSC)system utilizing ternary plots,derived from the PSDs.Within the three studied wells,NMR log data is exclusive to one well(well-A),while conventional well logs are accessible for all three wells(well-A,well-B,and well-C).This distinction enables PSD predictions for the remaining two wells(B and C).To prognosticate NMR outputs(CBW,BVI,FFV)for these wells,a two-step deep learning(DL)algorithm is implemented.Initially,three feature selection algorithms(f-classif,f-regression,and mutual-info-regression)identify the conventional well logs most correlated to NMR outputs in well-A.The three feature selection algorithms utilize statistical computations.These algorithms are utilized to systematically identify and optimize pertinent input features,thereby augmenting model interpretability and predictive efficacy within intricate data-driven endeavors.So,all three feature selection algorithms introduced the number of 4 logs as the most optimal number of inputs to the DL algorithm with different combinations of logs for each of the three desired outputs.Subsequently,the CUDA Deep Neural Network Long Short-Term Memory algorithm(CUDNNLSTM),belonging to the category of DL algorithms and harnessing the computational power of GPUs,is employed for the prediction of CBW,BVI,and FFV logs.This prediction leverages the optimal logs identified in the preceding step.Estimation of NMR outputs was done first in well-A(80%of data as training and 20%as testing).The correlation coefficient(CC)between the actual and estimated data for the three outputs CBW,BVI and FFV are 95%,94%,and 97%,respectively,as well as root mean square error(RMSE)was obtained 0.0081,0.098,and 0.0089,respectively.To assess the effectiveness of the proposed algorithm,we compared it with two traditional methods for log estimation:multiple regression and multi-resolution graph-based clustering methods.The results demonstrate the superior accuracy of our algorithm in comparison to these conventional approaches.This DL-driven approach facilitates PSD prediction grounded in fluid saturation for wells B and C.Ternary plots are then employed for PSCs.Seven distinct PSCs within well-A employing actual NMR logs(CBW,BVI,FFV),in conjunction with an equivalent count within wells B and C utilizing three predicted logs,are harmoniously categorized leading to the identification of seven distinct pore size classification facies(PSCF).this research introduces an advanced approach to pore size classification and prediction,fusing NMR logs with deep learning techniques and extending their application to nearby wells without NMR log.The resulting PSCFs offer valuable insights into generating precise and detailed reservoir 3D models.
基金funded by the National Key R&D Program of China(2017YFD0800505)Chongqing Key R&D Project of Technology Innovation and Application(NO.cstc2018jscxmszd X0055)。
文摘Characterizing soil particle-size distribution is a key measure towards soil property.The purpose of this study was to evaluate the multifractal characteristics of soil particle-size distribution among different land-use from a purple soil catchment and to generalize the spatial variation trend of multifractal parameters across the catchment.A total of 84 soil samples were collected from four kinds of land use patterns(dry land,orchard,paddy,and forest)in an agricultural catchment in the Three Gorges Reservoir Region,China.The multifractal analysis method was applied to quantitatively characterize the soil particle size distribution.Six soil particle size distribution(PSD)multifractal parameters(D(0),D(1),D(2),(35)a(q),(35)f[a(q)],α(0))were computed.Additionally,a geostatistical analysis was employed to reveal the spatial differentiation and map the spatial distribution of these parameters.Evident multifractal characteristics were found.The trend of generalized dimension spectrum of four land use patterns was basically consistent with the range of 0.8 to 2.0.However,orchard showed the largest monotonic decline,while the forest demonstrated the smallest decrease.D(0)of the four land use patterns were ranked as:dry land<orchard<forest<paddy,the order of D(1)was:dry land<paddy<orchard<forest,D(2)presented a rand-size relationship as dry land<forest<paddy<orchard.Furthermore,all land-use patterns presented asΔf[α(q)]<0.The rand-size relationship ofα(0)was same as D(0).The best-fitting model for D(0),D(1),D(2)andΔf[α(q)]was spherical model,forΔα(q)was gaussian model,and forα(0)was exponential model with structure variance ratio was 1.03%,49.83%,0.84%,1.48%,22.20%and 10.60%,respectively.The results showed that soil particles of each land use pattern were distributed unevenly.The multifractal parameters under different land use have significant differences,except forΔα(q).Differences in the composition of soil particles lead to differences in the multifractal properties even though they belong to the same soil texture.Farming behavior may refine particles and enhance the heterogeneity of soil particle distribution.Our results provide an effective reference for quantifying the impact of human activities on soil system in the Three Gorges Reservoir region.
基金The Special Funds for State Key Projects for Fun- damental Research (G1999022201-04).
文摘Application of particle image velocity (PIV) techniques for measuringparticle size distribution and total number in an activation chamber of desulfurization system isintroduced. Watersheld algorithm is used to choose the suitable initial gray level threshold whichis used to change the gray level images taken by PIV to black and white ones, then every particle inan image is isolated totally. For every isolating particle, its contour is tracked by the edgeenhancement filter function and kept by Freeman s chain code. Based on a set of particle s chincode, its size and size distribution are calculated and sorted. Finally, the experimental data ofcalcium particles and water drops, separately injected into the activation chamber, and the erroranalysis of data are given out.
基金The Ph.D.Programs Foundation of Ministry of Edu-cation of China(No20050710006)
文摘Size distribution characteristics of intercity bus hubs in China from 1997 to 2(104 were analyzed regarding highway passenger volume as a size index of intercity bus hubs. Yearly fractal dimensions of intercity bus hub sizes were exactly calculated by a novel model. Fractal dimensions of the 200 biggest intercity bus hubs from 2000 to 2004 were 1. 486 2 to 1. 511 8, and that is consistent with fractal dimensions of Chinese urban system sizes. It showed that the size distribution of intercity bus hubs had fractal structure. Fractal dimensions from 1997 to 2004 indicated that intercity bus hub size distribution grew from bi-fractal to single fractal. It is concluded that the intercity bus hub system is in evolutionary progress, and the Central Government should support large intercity bus hubs more to optimize system structure.
基金supported jointly by the China Meteorological Administration Special Public Welfare Research Fund (Grant No. GYHY201406001)the National (Key) Basic Research and Development (973) Program of China (Grant No. 2012CB417202)the National Natural Science Foundation of China (Grant No. 41175038)
文摘The characteristics of raindrop size distribution (DSD) over the Tibetan Plateau and southern China are studied in this paper, using the DSD data from April to August 2014 collected by HSC-PS32 disdrometers in Nagqu and Yangjiang, com- prising a total of 9430 and 63661-rain raindrop spectra, respectively. The raindrop spectra, characteristics of parameter variations with rainfall rate, and the relationships between reflectivity factor (Z) and rainfall rate (R) are analyzed, as well as their DSD changes with precipitation type and rainfall rate. The results show that the average raindrop spectra appear to be one-peak curves, the number concentration for larger drops increase significantly with rainfall rate, and its value over southern China is much higher, especially in convective rain larger drops, especially for convective rain in southern China. Standardized Gamma distributions better describe DSD for All three Gamma parameters for stratiform precipitation over the Tibetan Plateau are much higher, while its shape parameter (,u) and mass-weighted mean diameter (Dm), for convective precipitation, are less. In terms of parameter variation with rainfall rate, the normalized intercept parameter (Nw) over the Tibetan Plateau for stratiform rain increases with rainfall rate, which is opposite to the situation in convective rain. The/1 over the Tibetan Plateau for stratiform and convective precipitation types decreases with an increase in rainfall rate, which is opposite to the case for Dm variation. In Z-R relationships, like "Z = ARb'', the coefficient A over the Tibetan Plateau is smaller, while its b is higher, when the rain type transfers from stratiform to convective ones. Furthermore, with an increase in rainfall rate, parameters A and b over southern China increase gradually, while A over the Tibetan Plateau decreases sub- stantially, which differs from the findings of previous studies. In terms of geographic location and climate over the Tibetan Plateau and southern China, the precipitation in the pre-flood seasons is dominated by strong convective rain, while weak convective rain occurs frequently in northern Tibet with lower humidity and higher altitude.
基金Project supported by the National Basic Research Project(973)of China(No.2005CB422203)the National Post-Doctor Foundation of China(No.20060390990).
文摘The aerosol number concentration and size distribution were measured with the newly developed Wide-range Particle Spectrometer in summer and winter of 2006 at the urban site of Jinan City. Here reported the characteristics of fine particles of the different observation seasons. Relative high number concentrations for the particles in the diameter range of 10-500 nm were observed in both seasons. It was found that the dominant number distributed in particle diameter smaller than 100 nm and the percentage over the number concentration of all air particles is much higher than what has been measured in other urban sites over the world. The number mean diameter in summer was much smaller than in winter, strongly suggesting the different origin of ultrafine particles in different seasons. That is, particles in ultrafine mode mainly came from nucleation and new particle formation in summer while from traffic emission in winter. The diurnal variation also supported this point. Number concentration in the diameter range of 10-200 um got their peak values at noontime, well correlated with the mixing ratio of SO2 and the intensity of solar radiation in summer. While in winter, those in the same diameter range showed the main peaks during the traffic hours happened in the morning and evening.
基金primarily supported by the National Key Research and Development Program of China(Grant No.2017YFC1501703)the National Natural Science Foundation of China(Grant Nos.41875053,41475015 and 41322032)+1 种基金the National Fundamental Research 973 Program of China(Grant Nos.2013CB430101 and 2015CB452800)collected by a National 973 Project(Grant No.2013CB430101)
文摘Seasonal variations of rainfall microphysics in East China are investigated using data from the observations of a twodimensional video disdrometer and a vertically pointing micro rain radar. The precipitation and rain drop size distribution(DSD) characteristics are revealed for different rain types and seasons. Summer rainfall is dominated by convective rain,while during the other seasons the contribution of stratiform rain to rainfall amount is equal to or even larger than that of convective rain. The mean mass-weighted diameter versus the generalized intercept parameter pairs of convective rain are plotted roughly around the "maritime" cluster, indicating a maritime nature of convective precipitation throughout the year in East China. The localized rainfall estimators, i.e., rainfall kinetic energy–rain rate, shape–slope, and radar reflectivity–rain rate relations are further derived. DSD variability is believed to be a major source of diversity of the aforementioned derived estimators. These newly derived relations would certainly improve the accuracy of rainfall kinetic energy estimation, DSD retrieval, and quantitative precipitation estimation in this specific region.
基金National Natural Science Foundation of China(40730948,40830958,40921160382)National Grand Fundamental Research 973 Program of China(2009CB421502)
文摘Microphysical characteristics of the raindrop size distribution(RSD)in Typhoon Morakot(2009) have been studied through the PARSIVEL disdrometer measurements at one site in Fujian province,China during the passage of the storm from 7 to 10 August 2009.The time evolution of the RSD reveals different segments of the storm.Significant difference was observed in the microphysical characteristics between the outer rainband and the eyewall;the eyewall precipitation had a broader size distribution(a smaller slope) than the outer rainband and eye region.The outer rainband and the eye region produced stratiform rains while the eyewall precipitation was convective or mixed stratiform-convective.The RSD was typically characterized by a single peak distribution and well represented by the gamma distribution.The relations between the shape(μ)and slope(Λ)of the gamma distribution and between the reflectivity(Z)and rainfall rate(R)have been investigated.Based on the NW-Dm relationships,we suggest that the stratiform rain for the outer rainband and the eye region was formed by the melting of graupel or rimed ice particles,which likely originated from the eyewall clouds.
基金supported by the Key Project of Zhe-jiang Province (No. 2006C13057)the CAS Program(No. KZCX1-YW-06-02)the Jiaxing City Project(No. 2005AZ3040).
文摘Particles of dust washed off streets by stormwater are an important pathway of polyaromatic hydrocarbons (PAHs) into urban streams. This article presented a comprehensive assessment of the size distribution of PAHs in street dust particles, the potential risks of the particles in urban streams, and the sources and sinks of PAHs in the stream network. This assessment was based on measurements of 16 PAHs from the USEPA priority list in street dust particles and river sediments in Xincheng, China. The content of total PAHs ranged from 1629 to 8986 Dg/kg in street dust particles, where smaller particles have a higher concentrations. Approximately 55% of the total PAHs were associated with particles less than 250 μm which accounted for 40% of the total mass of street dust. The PAH quantities increased from 2.41 to 46.86 μg/m2 in the sequence of new residential, rising through main roads, old town residential, commercial and industrial areas. The sediments in stream reaches in town were found to be sinks for street dust particle PAHs. The research findings suggested that particle size, land use and the hydrological conditions in the stream network were the factors which most influenced the total loads of PAH in the receiving water bodies.
文摘This article reports the morphology, size, and distribution evolution of MnS inclusions in non-quenched and tempered steel during heat treatment. The variation of single large-sized MnS inclusions at high temperature was observed in situ using a confocal scanning laser microscope (CSLM). The slender MnS inclusions first changed to pearl-like slrings. These small-sized pearls subsequently coalesced and became closer together as the temperature increased. Large-sized MnS inclusions in non-quenched and tempered steel samples with different thermal histories were investigated with respect to the evolution of their morphology, size, and distribution. After 30 min of ovulation at 1573 K, the percentage of MnS inclusions larger than 3 μm decreased from 50.5% to 3.0%. After a 3 h making period, Ostwald ripening occurred. Most MnS inclusions moved from the grain bounda- ries to the interior. The present study demonstrates that heat treatment is an effective method of changing the morphology, size, and distribution of MnS inclusions, especially large-sized ones.
文摘Nanobubble flotation technology is an important research topic in the field of fine mineral particle separation.The basic characteristics of nanobubbles,including their size,concentration,surface zeta potential,and stability have a significant impact on the nanobubble flotation performance.In this paper,bulk nanobubbles generated based on the principle of hydrodynamic cavitation were investigated to determine the effects of different parameters(e.g.,surfactant(frother)dosage,air flow,air pressure,liquid flow rate,and solution pH value)on their size distribution and zeta potential,as measured using a nanoparticle analyzer.The results demonstrated that the nanobubble size decreased with increasing pH value,surfactant concentration,and cavitation-tube liquid flow rate but increased with increasing air pressure and increasing air flow rate.The magnitude of the negative surface charge of the nanobubbles was positively correlated with the pH value,and a certain relationship was observed between the zeta potential of the nanobubbles and their size.The structural parameters of the cavitation tube also strongly affected the characteristics of the nanobubbles.The results of this study offer certain guidance for optimizing the nanobubble flotation technology.
基金supported financially by the National Natural Science Foundation of China(40525016)the National Basic Research Program(2007CB407303 and 2006CB403702)
文摘Total suspended particulates (TSP) samples were collected using low pressure impactors (Andersen Series 20-800, USA) on typical clear, hazy and foggy days in Beijing in order to investigate the characteristics of size distributions and elemental compositions of particulate matter (PM) in different weather conditions. The concentrations of sixteen elements, including Na, Mg, Al, K, Ca, Mn, Fe, Ni, Cu, Zn, As, Se, Cd, Ba, T1 and Pb were detected using inductively coupled plasma mass spectrometry (ICP-MS). The results showed that Ca, A1, Fe, Mg and Ba on foggy days were 2.0 2.6 times higher than on clear days, and 2.3-2.9 times higher than on hazy days. Concentrations of Cu, Zn, As, Se and Pb on foggy days were 163.5, 1186.7, 65.9, 32.0 and 708.2 ng m-3, respectively, in fine particles, and 68.1, 289.5, 19.8, 1.6 and 103.8 ng m-3, respectively, in coarse particles. This was 1.0~8.4 times higher and 1.4-7.4 times higher than on clear and hazy days, respectively. It is then shown that Mg, A1, Fe, Ca and Ba were mainly associated with coarse particles, peaking at 4.7~5.8 μm; that Cd, Se, Zn, As, T1 and Pb were most dominant in fine particles, peaking at 0.43-1.1 μm; and that Na, K, Ni, Cu and Mn had a multi-mode distribution, with peaks at 0.43-1.1 μm and 4.7-5.8 μm. The enrichment factors indicated that coal combustion along with vehicle and industry emissions may be the main sources of pollution elements.
基金the National Key Basic Research Program of China (973program),a key project of the Shandong Provincial Environmental Protection Department,the Niche Area Development Scheme of the Hong Kong Polytechnic University,the Hong Kong Research Grants Council,the central level,scientific research institutes for basic R & D special fund business
文摘For the 2008 Olympic Games, drastic control measures were implemented on industrial and urban emissions of sulfur dioxide (SO2), nitrogen oxides (NOx) and other pollutants to address the issues of poor air quality in Beijing. To investigate the effects of SO2 and NOx reductions on the particulate sulfate and nitrate concentrations as well as their size distributions, size-segregated aerosol samples were collected using micro-orifice uniform deposit impactors (MOUDIs) at urban and downwind rural sites in Beijing before and after full-scale controls. During the sampling period, the mass concentrations of fine particles (PMI.s) at the urban and rural sites were 94.0 and 85.9 p.g m-3, respectively. More than 90% of the sulfates and 60% of nitrates formed as fine particles. Benefiting from the advantageous meteorological conditions and the source controls, sulfates were observed in rather low concentrations and primarily in condensation mode during the Olympics. The effects of the control measures were separately analyzed for the northerly and the southerly air-mass-dominated days to account for any bias. After the control measures were implemented, PM, sulfates, and nitrates were significantly reduced when the northerly air masses prevailed, with a higher percentage of reduction in larger particles. The droplet mode particles, which dominated the sulfates and nitrates before the controls were implemented, were remarkably reduced in mass concentration after the control measures were implemented. Nevertheless, when the polluted southerly air masses prevailed, the local source control measures in Beijing did not effectively reduce the ambient sulfate concentration due to the enormous regional contribution from the North China Plain.
基金supported by the National Natural Science Foundation of China (31271661, 30871477)the National Basic Program of China (2009CB118602)the Special Fund for Agro-Scientific Research in the Public Interest of China (201203100)
文摘Granule size distribution of wheat starch is an important characteristic that can affect its chemical composition and the functionality of wheat products. Two high-yield winter wheat cultivars were used to evaluate the effects of the application of exogenous ABA or GA during the reproductive phase of the initial grain filling on starch granule size distribution and starch components in grains at maturity. The results indicated that a bimodal curve was found in the volume and surface area distribution of grain starch granules, and a unimodal curve was observed for the number distribution under all treatments. The exogenous ABA resulted in a significant increase in the proportions (both by volume and by surface area) of B-type (〈9.9 Ixm in diameter) starch granules, with a reduction in those of A-type (〉9.9 ~tm) starch granules, while, the exogenous GA3 led to converse effects on size distribution of those starch granules. The exogenous ABA also increased starch, amylose and amylopectin contents at maturity but significantly reduced the ratio of amylose to amylopectin. Application of GA3 significantly reduced starch content, amylopectin content but increased the ratio of amylose to amylopectin. The ratio of amylose to amylopectin showed a significant and negative relationship with the volume proportion of granules 〈9.9 μm, but was positively related to the volume proportion of granules 22.8-42.8 μm.