With ensured network connectivity in quantum channels, the issue of distributing entangled particles in wireless quantum communication mesh networks can be equivalently regarded as a problem of quantum backbone nodes ...With ensured network connectivity in quantum channels, the issue of distributing entangled particles in wireless quantum communication mesh networks can be equivalently regarded as a problem of quantum backbone nodes selection in order to save cost and reduce complexity. A minimum spanning tree( MST)-based quantum distribution algorithm( QDMST) is presented to construct the mesh backbone network. First, the articulation points are found,and for each connected block uncovered by the articulation points, the general centers are solved. Then, both articulation points and general centers are classified as backbone nodes and an M ST is formed. The quantum path between every two neighbor nodes on the MST is calculated. The nodes on these paths are also classified as backbone nodes. Simulation results validate the advantages of QDMST in the average backbone nodes number and average quantum channel distance compared to the existing random selection algorithm under multiple network scenarios.展开更多
In this paper, a solution to the Fokker-Planck equation is presented, which is extended to the field particles' high-energy-tail non-Maxwellian velocity distribution function in transport theory. Based on the correct...In this paper, a solution to the Fokker-Planck equation is presented, which is extended to the field particles' high-energy-tail non-Maxwellian velocity distribution function in transport theory. Based on the correct physical concept of collision intensity, introduced by CHANG and LI, the electrical conductivities for like-particles collisions are obtained in different conditions. The modified Fokker-Planck coefficients for non-Maxwellian scattering are applied in the study. It is found that the parallel part of the collision operator plays an important role. The non-Maxwellian scattering will stimulate the transport processes in various degrees with mutative deviation parameters.展开更多
The laminar boundary layer behind a constant-speed shock wave moving through a dusty gas along a solid surface is studied.The Saffman lift force acting on a spherical particle in a gas boundary layer is taken into acc...The laminar boundary layer behind a constant-speed shock wave moving through a dusty gas along a solid surface is studied.The Saffman lift force acting on a spherical particle in a gas boundary layer is taken into account.A method for calculating the density profile of dispersed phase near the wall is pro- posed and some numerical results are given.It is shown that behind the shock wave,there exists a curved thin layer where the density of particles is many times higher than the original one.This dust collection effect may be of essential importance to the problem of dust explosion in industry.展开更多
In the context of unified hydrodynamics, we discuss the pseudorapidity distributions of the charged particles produced in Au-Au and Cu-Cu collisions at the low RHIC energies of √SNN = 19.6 and 22.4 GeV, respectively....In the context of unified hydrodynamics, we discuss the pseudorapidity distributions of the charged particles produced in Au-Au and Cu-Cu collisions at the low RHIC energies of √SNN = 19.6 and 22.4 GeV, respectively. It is found that the unified hydrodynamics alone can give a good description to the experimental measurements. This is different from the collisions at the maximum RHIC energy of √SNN = 200 GeV or at LHC energy of √SNN= 2.76 TeV, in which the leading particles must be taken into account so that we can properly explain the experimental observations.展开更多
We present how the luminescence of europium RR-2-P-oxides complexes can be increased by interaction of electronic levels of the complex with the radiation field of silver nanoparticles (NPs). The procedure by which ...We present how the luminescence of europium RR-2-P-oxides complexes can be increased by interaction of electronic levels of the complex with the radiation field of silver nanoparticles (NPs). The procedure by which silver NPs are formed in a sol-gel polyurethane matrix precursor was elaborated. The formed Ag NPs were combined with Eu complex incorporated in ormocer matrix. The emission spectra of the complexes without silver NPs were compared with spectra of the same complexes with addition of silver NPs. As the result of the interaction of the electronic levels of lanthaaide ligands with silver plasmons, dramatic increase of luminescence was observed.展开更多
The road subgrade and road surface in collapsible loess area are prone to many engineering diseases such as uneven subgrade settlement,insufficient bearing capacity of soaked foundation,collapse and instability of sub...The road subgrade and road surface in collapsible loess area are prone to many engineering diseases such as uneven subgrade settlement,insufficient bearing capacity of soaked foundation,collapse and instability of sub-grade side slope due to the special properties of loess.As an environment-friendly,low-cost soil modifier with good adhesion and chelation properties,lignin has been considered to be used in highway subgrade construction.In order to explore the effect of lignin on loess,the compressive and collapsible properties of modified loess with different lignin contents were analyzed based on consolidation compression test.The improvement mechanism of lignin on loess collapsibility was studied by means of infiltration test and SEM test.The results show that lignin fibers can promote the agglomeration of loose particles and form a network structure in the soil particle pores,enhance the cementation strength between particles and soil skeleton,and reduce the permeability of loess.With the increase of lignin fiber content,the improvement degree of loess collaps ility shows a trend of first increasing and then decreasing.When the lignin fiber content is 2%,the effect is the best,and the improved loess ollapsi-bility is eliminated.展开更多
As is well known to mineral processing scientists and engineers, fine and ultrafine particles are difficult to float mainly due to the low bubble-particle collision efficiencies. Though many efforts have been made to ...As is well known to mineral processing scientists and engineers, fine and ultrafine particles are difficult to float mainly due to the low bubble-particle collision efficiencies. Though many efforts have been made to improve flotation performance of fine and ultrafine particles, there is still much more to be done. In this paper, the effects of nano-microbubbles (nanobuhbles and microbubbles) on the flotation of fine (-38 + 14.36 μm) and ultrafine (-14.36 + 5μm) chalcopyrite particles were investigated in a laboratory scale Denver flotation cell. Nano-microbubbles were generated using a specially-designed nano- microbubble generator based on the cavitation phenomenon in Venturi tubes. In order to better under- stand the mechanisms of nano-microbubble enhanced froth flotation of fine and ultrafine chalcopyrite particles, the nano-microbubble size distribution, stability and the effect of frother concentration on nano- bubble size were also studied by a laser diffraction method. Comparative flotation tests were performed in the presence and absence of nano-microbubbles to evaluate their impact on the fine and ultrafine chalcopyrite particle flotation recovery. According to the results, the mean size of nano-microbubbles increased over time, and decreased with increase of frother concentration. The laboratory-scale flotation test results indicated that flotation recovery of chalcopyrite fine and ultrafine particles increased by approximately 16-21% in the presence of nano-microbubbles, depending on operating conditions of the process. The presence of nano-microbubbles increased the recovery of ultrafine particles (-14.36 + 5 μm) more than that of fine particles (-38 + 14.36 μm). Another major advantage is that the use of nano-microbubbles reduced the collector and frother consumptions by up to 75% and 50%, respectively.展开更多
Al-7graphite composite was processed using Al-7graphite mushy prepared by electromagnetic-mechanical stirring method, and the influence of solid fraction on the distributing of graphite particles in ingot was studied....Al-7graphite composite was processed using Al-7graphite mushy prepared by electromagnetic-mechanical stirring method, and the influence of solid fraction on the distributing of graphite particles in ingot was studied. The results shows that the relationship between solid fraction and stirring temperature of mushy is: f(s) = 591.5-0.897 t (where f(s) is the solid fraction, t is the stirring temperature). For Al-7graphite composite, with the increasing of solid fraction, the aggregation extent of graphite particles reduced gradually, and when solid fraction was larger than 30%, graphite particles could distribute evenly in ingot.展开更多
As anode materials of electrochemical energy storage system,metal sulfides with high theoretical capacities suffer from issues of materials smashing and deactivation due to huge volume change,resulting in the inferior...As anode materials of electrochemical energy storage system,metal sulfides with high theoretical capacities suffer from issues of materials smashing and deactivation due to huge volume change,resulting in the inferior cycle stability.In this paper,a new strategy of adding sulfur powder into the electrospinning precursor instead of employing sulfur powder during the sulfurizing treatment is proposed to prepare Fe_(9)S_(10)composites(CNF@G-Fe_(9)S_(10)-1).In those composites,most of Fe_(9)S_(10)particles are embedded in the graphene-carbon fibers with multiple protection.As anodes for potassium-ion batteries,CNF@G-Fe_(9)S_(10)-1 display higher rate capacities and more excellent stability(103.2 mAh·g^(-1)at 1000 mA·g^(-1)after 892 cycles)than Fe_(9)S_(10)composites synthesized by the traditional method.In addition,as anodes for potassiumion hybrid capacitors,they also deliver high capacities of102.8 mAh·g^(-1)at 1000 mA·g^(-1)after 100 cycles.The morphology characterization evidences indicate that the surface and integrity of CNF@G-Fe_(9)S_(10)-1 are more smooth and complete than the Fe_(9)S_(10)composites fabricated using a common method without sulfur power in electrospinning precursor.The excellent stability and high capacity of CNF@G-Fe_(9)S_(10)-1 can be attributed to nearly full-wrapped structure of Fe_(9)S_(10)in the carbon matrix arising from the new strategy.Owing to the formation of the structure,Fe_(9)S_(10)particles are protected from the pulverization,and the structure stability of hybrid carbon fibers is enhanced.This study may provide a new strategy for the controllable synthesis of metal sulfide-CNFs and their application for high stability energy storage.展开更多
In this paper, a new method to derive the Fokker-Planck coefficients defined by a non-Maxwellian velocity distribution function for the field particles is presented. The three- fold integral and the new Debye cutoff p...In this paper, a new method to derive the Fokker-Planck coefficients defined by a non-Maxwellian velocity distribution function for the field particles is presented. The three- fold integral and the new Debye cutoff parameter, which were introduced by CHANG and LI, are applied. Therefore, divergence difficulties and the customary replacement of relative velocity g by thermal velocity vth are naturally avoided. The probability function P(v, Av) for non- Maxwellian scattering is derived by the method of choosing velocity transfer Av, which is a true measure of collision intensity, as an independent variable. The method enables the difference between small-angle scattering and small-momentum-transfer collisions of the inverse-square force to be well clarified. With the help of the probability function, the Fokker-Planck coefficients are obtained by a normal original Fokker-Planck approach. The friction and diffusion coefficients of the Fokker-Planck equation are modified for non-Maxwellian scattering and are used to investigate the relaxation processes for the weakly coupled plasma. The profiles of the relaxation rates show that the slowing down and deflection processes are weakened in the conditions of non-Maxwellian scattering.展开更多
The electromagnetic-mechanical stirring technology was employed for preparing QTi4.3-4 graghite composite slurry,and QTi4.3-4 graghite composite with uniform distribution of graphite particles was prepared uring the ...The electromagnetic-mechanical stirring technology was employed for preparing QTi4.3-4 graghite composite slurry,and QTi4.3-4 graghite composite with uniform distribution of graphite particles was prepared uring the semi-solid casting technology successfully.The structure of this QTi4.3-4graphite composite was studied and the condition for uniform distribution of graphite particles was got.The experimental results show that there exists a linear relationship between the solid fraction and the stirring temperature of QTi4.3-4graphite slurry.With the decreasing of stirring temperature,the solid fraction of QTi4.3-4 graghite slurry increases constantly.In casting,with the increasing of solid fraction of QTi4.3-4 graphite slurry.the agglomeration of graphite particles is removed gradually.When the solid fraction is higher than 40%,graphite particles can distribute evenly in QTi4.3-4 graghite composite.展开更多
In this work,particulate matter(PM) emissions from a large two-stroke,low-speed marine diesel engine were investigated when the engine was operated with low-sulfur heavy fuel oil(HFO) at various loads.Particle samples...In this work,particulate matter(PM) emissions from a large two-stroke,low-speed marine diesel engine were investigated when the engine was operated with low-sulfur heavy fuel oil(HFO) at various loads.Particle samples were collected in situ from the engine exhaust to determine the detailed physical and chemical properties.The nanostructure and morphology of the nanoparticles were analyzed using transmission electron microscopy images(TEM).The results show that volatile organic carbon(OC) accounts for more than 80% in the HFO particles and leads to an increase in particle size.The thermodynamic conditions of a low-speed engine favor the behavior of capturing the soluble organic components.A large number of spherical char HFO particles with aerodynamic diameters of 0.2 μm-0.5 μm and a suspected inner metal core were detected.The two peak aerodynamic diameters of the HFO nanoparticles are 15 nm and 86 nm.The morphological differences among the HFO nanoparticles in varied engine conditions represent the formation process from primary nascent particles to mature graphitized particles caused by thermodynamics.The above study will be valuable for understanding the characteristics of PM emissions from low-sulfur HFO to achieve the ship PM emissions reduction target.展开更多
In recent years, Asia became the region with the highest increase in rate of urbanization and economic development in the world. According to recent estimates from the United Nations, the world population will increas...In recent years, Asia became the region with the highest increase in rate of urbanization and economic development in the world. According to recent estimates from the United Nations, the world population will increase 36% between 2000 and 2030, leading to a doubling of the number of urban dwellers in less developed regions, like Asia. Such rapid economic development has many associated environmental problems, including development of heavy aerosol pollution over Asia.展开更多
In this paper, the impact of the viaduct on flow and traffic exhausting particles dispersion within urban street canyons was numerically simulated using a computational fluid dynamics (CFD) model. Two-dimensional fl...In this paper, the impact of the viaduct on flow and traffic exhausting particles dispersion within urban street canyons was numerically simulated using a computational fluid dynamics (CFD) model. Two-dimensional flow and dispersion of particles from traffic exhausts were modeled using the standard k-e turbulence model. The street canyons with a viaduct at different widths and different heights above the ground are simulated. The results show that the airflow in street canyon is evidently in- fluenced by the viaduct: The position of the main vortex center is changed, especially there are two strong vortexes when the viaduct is placed at 10 m height above the ground. It is found based on the study of the particles number concentrations (PNCs) that the viaduct may mitigate the pollution level in the street canyon sometimes. The impact of the viaduct width on PNCs is stronger than that of the height. The study of PNDs reveals that the mean PNCs at the wall of upwind building increase when a viaduct is placed in street canyon. In addition, it is found based on the study of mean particles residence time (PRT) that the removal of the particles strongly correlates to the mean PNCs. The results indicate that the viaduct is an important factor to influence the flow patterns and particles dispersion in street canyons.展开更多
7 YSZ coating was prepared by plasma sprayphysical vapor deposition(PS-PVD) technique based on a specific experimental design.The microstructure and deposition properties of 7 YSZ coating along the radius of plasma je...7 YSZ coating was prepared by plasma sprayphysical vapor deposition(PS-PVD) technique based on a specific experimental design.The microstructure and deposition properties of 7 YSZ coating along the radius of plasma jet were investigated in detail.Results show that the coating presents regional characteristic in the radial direction,which could be divided into three typical zones:In Zone Ⅰ,the coating is all composed of columnar structures with cauliflower structure,and the coating properties including the surface roughness and deposition efficiency(DE) are almost stable;in Zone Ⅲ,the coating is made up of solid particles,droplet and gas phase mixed without columnar structures;Zone Ⅱ is between Zone Ⅰ and ZoneⅢ, in which there are columns with domed top and small particles.Based on experiment results,a model on the state and distribution of particles in plasma jet was proposed to clarify the regional characteristic.This study is helpful to comprehend and control coatings deposition by PS-PVD technique.展开更多
The present article provides an overview of the chemical and physical features of haze in China, focusing on the relationship between haze and atmospheric fine particles, and the formation mechanism of haze. It also s...The present article provides an overview of the chemical and physical features of haze in China, focusing on the relationship between haze and atmospheric fine particles, and the formation mechanism of haze. It also summarizes several of control technologies and strategies to mitigate the occurrence of haze. The development of instruments and the analysis of measurements of ambient particles and precursor concentrations have provided important information about haze formation. Indeed, the use of new instruments has greatly facilitated current haze research in China. Examples of insightful results include the relationship between fine particles and haze, the chemical compositions and sources of particles, the impacts of the aging process on haze formation, and the application of technologies that control the formation of haze. Based on these results, two relevant issues need to be addressed: understanding the relationship between haze and fine particles and understanding how to control PM2.5.展开更多
The evolution equations of moments for the Brownian coagulation of nanoparticles in both continuum and free molecule regimes are analytically studied. These equations are derived using a Taylor-expansion technique. Th...The evolution equations of moments for the Brownian coagulation of nanoparticles in both continuum and free molecule regimes are analytically studied. These equations are derived using a Taylor-expansion technique. The self-preserving size distribution is investigated using a newly defined dimensionless parameter, and the asymptotic values for this parameter are theoretically determined. The dimensionless time required for an initial size distribution to achieve self-preservation is also derived in both regimes. Once the size distribution becomes self-preserving, the time evolution of the zeroth and second moments can be theoretically obtained, and it is found that the second moment varies linearly with time in the continuum regime. Equivalent equations, rather than the original ones from which they are derived, can be employed to improve the accuracy of the results and reduce the computational cost for Brownian coagulation in the continuum regime as well as the free molecule regime.展开更多
Size distributions of ambient aerosols at the Fresno Supersite were measured with four commercially available scanning mobility particle sizers (SMPS). TSI nano, TSI standard, Grimm, and MSP instruments were colloca...Size distributions of ambient aerosols at the Fresno Supersite were measured with four commercially available scanning mobility particle sizers (SMPS). TSI nano, TSI standard, Grimm, and MSP instruments were collocated at the Fresno Supersite and particle size distributions were measured continuously from August 18 through September 18, 2005. For particles with diameters between 10 and 200 nm, differences among hourly-average ambient particle concentrations ranged from 0% between the TSI nano and Grimm in the 30-50 nm size range to 39% between the Grimm and MSP in the 10-30 nm size range. MSP concentrations were 10-33% lower than those measured with the TSI standard for particles smaller than 200 nm. The TSI nano and TSI standard agreed to within 5% in their overlapping size range (10-84 nm). The TSI nano and Grimm agreed to within 40% for 5-10 nm particles.展开更多
The parton and hadron cascade model PACIAE is used to investigate strange particle production in Au + Au collisions at √s = 62.4 GeV in different centralities and at √s =39, 11.5 and 7.7 GeV in the most central col...The parton and hadron cascade model PACIAE is used to investigate strange particle production in Au + Au collisions at √s = 62.4 GeV in different centralities and at √s =39, 11.5 and 7.7 GeV in the most central collision, respectively. It is shown that the transverse momentum distributions of strange particles by the PACIAE model fit the RHIC Beam Energy Scan experimental results well.展开更多
基金Prospective Research Project on Future Networks of Jiangsu Province,China(No.BY2013095-1-18)
文摘With ensured network connectivity in quantum channels, the issue of distributing entangled particles in wireless quantum communication mesh networks can be equivalently regarded as a problem of quantum backbone nodes selection in order to save cost and reduce complexity. A minimum spanning tree( MST)-based quantum distribution algorithm( QDMST) is presented to construct the mesh backbone network. First, the articulation points are found,and for each connected block uncovered by the articulation points, the general centers are solved. Then, both articulation points and general centers are classified as backbone nodes and an M ST is formed. The quantum path between every two neighbor nodes on the MST is calculated. The nodes on these paths are also classified as backbone nodes. Simulation results validate the advantages of QDMST in the average backbone nodes number and average quantum channel distance compared to the existing random selection algorithm under multiple network scenarios.
基金supported by National High-Tech ICF Committee in ChinaNational Natural Science Foundation of China(Nos.10475076,10505021,40336052,and 10175065)
文摘In this paper, a solution to the Fokker-Planck equation is presented, which is extended to the field particles' high-energy-tail non-Maxwellian velocity distribution function in transport theory. Based on the correct physical concept of collision intensity, introduced by CHANG and LI, the electrical conductivities for like-particles collisions are obtained in different conditions. The modified Fokker-Planck coefficients for non-Maxwellian scattering are applied in the study. It is found that the parallel part of the collision operator plays an important role. The non-Maxwellian scattering will stimulate the transport processes in various degrees with mutative deviation parameters.
文摘The laminar boundary layer behind a constant-speed shock wave moving through a dusty gas along a solid surface is studied.The Saffman lift force acting on a spherical particle in a gas boundary layer is taken into account.A method for calculating the density profile of dispersed phase near the wall is pro- posed and some numerical results are given.It is shown that behind the shock wave,there exists a curved thin layer where the density of particles is many times higher than the original one.This dust collection effect may be of essential importance to the problem of dust explosion in industry.
基金Supported by the Shanghai Key Lab of Modern Optical System
文摘In the context of unified hydrodynamics, we discuss the pseudorapidity distributions of the charged particles produced in Au-Au and Cu-Cu collisions at the low RHIC energies of √SNN = 19.6 and 22.4 GeV, respectively. It is found that the unified hydrodynamics alone can give a good description to the experimental measurements. This is different from the collisions at the maximum RHIC energy of √SNN = 200 GeV or at LHC energy of √SNN= 2.76 TeV, in which the leading particles must be taken into account so that we can properly explain the experimental observations.
基金supported by the Institute of Physical Chemistry of the Polish Academy of Sciences
文摘We present how the luminescence of europium RR-2-P-oxides complexes can be increased by interaction of electronic levels of the complex with the radiation field of silver nanoparticles (NPs). The procedure by which silver NPs are formed in a sol-gel polyurethane matrix precursor was elaborated. The formed Ag NPs were combined with Eu complex incorporated in ormocer matrix. The emission spectra of the complexes without silver NPs were compared with spectra of the same complexes with addition of silver NPs. As the result of the interaction of the electronic levels of lanthaaide ligands with silver plasmons, dramatic increase of luminescence was observed.
基金This work was funded under Funding of Science for Earthquake Resilience(Grant No.XH21034)the Special Fund for Innovation Team,Gansu Earthquake Agency(Grant No.2020TD-01-01)+1 种基金the grant of the National Natural Science Foundation of China(Nos.51778590,51408567)the Fundamental Research Funding for the Institute of Earthquake Forecasting,China Earthquake Administration(Grant Nos.2021IESLZ03,2018IESLZ06).
文摘The road subgrade and road surface in collapsible loess area are prone to many engineering diseases such as uneven subgrade settlement,insufficient bearing capacity of soaked foundation,collapse and instability of sub-grade side slope due to the special properties of loess.As an environment-friendly,low-cost soil modifier with good adhesion and chelation properties,lignin has been considered to be used in highway subgrade construction.In order to explore the effect of lignin on loess,the compressive and collapsible properties of modified loess with different lignin contents were analyzed based on consolidation compression test.The improvement mechanism of lignin on loess collapsibility was studied by means of infiltration test and SEM test.The results show that lignin fibers can promote the agglomeration of loose particles and form a network structure in the soil particle pores,enhance the cementation strength between particles and soil skeleton,and reduce the permeability of loess.With the increase of lignin fiber content,the improvement degree of loess collaps ility shows a trend of first increasing and then decreasing.When the lignin fiber content is 2%,the effect is the best,and the improved loess ollapsi-bility is eliminated.
基金the Tarbiat Modares University (TMU), the Iran Mineral Processing Research Center (IMPRC) and the IMIDRO for the technical assistance and financial support
文摘As is well known to mineral processing scientists and engineers, fine and ultrafine particles are difficult to float mainly due to the low bubble-particle collision efficiencies. Though many efforts have been made to improve flotation performance of fine and ultrafine particles, there is still much more to be done. In this paper, the effects of nano-microbubbles (nanobuhbles and microbubbles) on the flotation of fine (-38 + 14.36 μm) and ultrafine (-14.36 + 5μm) chalcopyrite particles were investigated in a laboratory scale Denver flotation cell. Nano-microbubbles were generated using a specially-designed nano- microbubble generator based on the cavitation phenomenon in Venturi tubes. In order to better under- stand the mechanisms of nano-microbubble enhanced froth flotation of fine and ultrafine chalcopyrite particles, the nano-microbubble size distribution, stability and the effect of frother concentration on nano- bubble size were also studied by a laser diffraction method. Comparative flotation tests were performed in the presence and absence of nano-microbubbles to evaluate their impact on the fine and ultrafine chalcopyrite particle flotation recovery. According to the results, the mean size of nano-microbubbles increased over time, and decreased with increase of frother concentration. The laboratory-scale flotation test results indicated that flotation recovery of chalcopyrite fine and ultrafine particles increased by approximately 16-21% in the presence of nano-microbubbles, depending on operating conditions of the process. The presence of nano-microbubbles increased the recovery of ultrafine particles (-14.36 + 5 μm) more than that of fine particles (-38 + 14.36 μm). Another major advantage is that the use of nano-microbubbles reduced the collector and frother consumptions by up to 75% and 50%, respectively.
基金China and Tsinghua-Zhongda Postdoctoral Science Foundation.]
文摘Al-7graphite composite was processed using Al-7graphite mushy prepared by electromagnetic-mechanical stirring method, and the influence of solid fraction on the distributing of graphite particles in ingot was studied. The results shows that the relationship between solid fraction and stirring temperature of mushy is: f(s) = 591.5-0.897 t (where f(s) is the solid fraction, t is the stirring temperature). For Al-7graphite composite, with the increasing of solid fraction, the aggregation extent of graphite particles reduced gradually, and when solid fraction was larger than 30%, graphite particles could distribute evenly in ingot.
基金financially supported by the National Natural Science Foundation of China(Nos.51772082 and 51804106)the Natural Science Foundation of Hunan Province(Nos.2019JJ30002 and 2019JJ50061)。
文摘As anode materials of electrochemical energy storage system,metal sulfides with high theoretical capacities suffer from issues of materials smashing and deactivation due to huge volume change,resulting in the inferior cycle stability.In this paper,a new strategy of adding sulfur powder into the electrospinning precursor instead of employing sulfur powder during the sulfurizing treatment is proposed to prepare Fe_(9)S_(10)composites(CNF@G-Fe_(9)S_(10)-1).In those composites,most of Fe_(9)S_(10)particles are embedded in the graphene-carbon fibers with multiple protection.As anodes for potassium-ion batteries,CNF@G-Fe_(9)S_(10)-1 display higher rate capacities and more excellent stability(103.2 mAh·g^(-1)at 1000 mA·g^(-1)after 892 cycles)than Fe_(9)S_(10)composites synthesized by the traditional method.In addition,as anodes for potassiumion hybrid capacitors,they also deliver high capacities of102.8 mAh·g^(-1)at 1000 mA·g^(-1)after 100 cycles.The morphology characterization evidences indicate that the surface and integrity of CNF@G-Fe_(9)S_(10)-1 are more smooth and complete than the Fe_(9)S_(10)composites fabricated using a common method without sulfur power in electrospinning precursor.The excellent stability and high capacity of CNF@G-Fe_(9)S_(10)-1 can be attributed to nearly full-wrapped structure of Fe_(9)S_(10)in the carbon matrix arising from the new strategy.Owing to the formation of the structure,Fe_(9)S_(10)particles are protected from the pulverization,and the structure stability of hybrid carbon fibers is enhanced.This study may provide a new strategy for the controllable synthesis of metal sulfide-CNFs and their application for high stability energy storage.
基金National High-Tech ICF(Inertial Confinement Fusion)Committee in ChinaNational Natural Science Foundation of China(Nos.10475076,10505021,40336052,and 10175065)
文摘In this paper, a new method to derive the Fokker-Planck coefficients defined by a non-Maxwellian velocity distribution function for the field particles is presented. The three- fold integral and the new Debye cutoff parameter, which were introduced by CHANG and LI, are applied. Therefore, divergence difficulties and the customary replacement of relative velocity g by thermal velocity vth are naturally avoided. The probability function P(v, Av) for non- Maxwellian scattering is derived by the method of choosing velocity transfer Av, which is a true measure of collision intensity, as an independent variable. The method enables the difference between small-angle scattering and small-momentum-transfer collisions of the inverse-square force to be well clarified. With the help of the probability function, the Fokker-Planck coefficients are obtained by a normal original Fokker-Planck approach. The friction and diffusion coefficients of the Fokker-Planck equation are modified for non-Maxwellian scattering and are used to investigate the relaxation processes for the weakly coupled plasma. The profiles of the relaxation rates show that the slowing down and deflection processes are weakened in the conditions of non-Maxwellian scattering.
文摘The electromagnetic-mechanical stirring technology was employed for preparing QTi4.3-4 graghite composite slurry,and QTi4.3-4 graghite composite with uniform distribution of graphite particles was prepared uring the semi-solid casting technology successfully.The structure of this QTi4.3-4graphite composite was studied and the condition for uniform distribution of graphite particles was got.The experimental results show that there exists a linear relationship between the solid fraction and the stirring temperature of QTi4.3-4graphite slurry.With the decreasing of stirring temperature,the solid fraction of QTi4.3-4 graghite slurry increases constantly.In casting,with the increasing of solid fraction of QTi4.3-4 graphite slurry.the agglomeration of graphite particles is removed gradually.When the solid fraction is higher than 40%,graphite particles can distribute evenly in QTi4.3-4 graghite composite.
基金supported by the Science & Technology Commission of Shanghai MunicipalityShanghai Engineering Research Center of Ship Intelligent Maintenance and Energy Efficiency under Grant 20DZ2252300。
文摘In this work,particulate matter(PM) emissions from a large two-stroke,low-speed marine diesel engine were investigated when the engine was operated with low-sulfur heavy fuel oil(HFO) at various loads.Particle samples were collected in situ from the engine exhaust to determine the detailed physical and chemical properties.The nanostructure and morphology of the nanoparticles were analyzed using transmission electron microscopy images(TEM).The results show that volatile organic carbon(OC) accounts for more than 80% in the HFO particles and leads to an increase in particle size.The thermodynamic conditions of a low-speed engine favor the behavior of capturing the soluble organic components.A large number of spherical char HFO particles with aerodynamic diameters of 0.2 μm-0.5 μm and a suspected inner metal core were detected.The two peak aerodynamic diameters of the HFO nanoparticles are 15 nm and 86 nm.The morphological differences among the HFO nanoparticles in varied engine conditions represent the formation process from primary nascent particles to mature graphitized particles caused by thermodynamics.The above study will be valuable for understanding the characteristics of PM emissions from low-sulfur HFO to achieve the ship PM emissions reduction target.
文摘In recent years, Asia became the region with the highest increase in rate of urbanization and economic development in the world. According to recent estimates from the United Nations, the world population will increase 36% between 2000 and 2030, leading to a doubling of the number of urban dwellers in less developed regions, like Asia. Such rapid economic development has many associated environmental problems, including development of heavy aerosol pollution over Asia.
基金supported by the Major Project of Knowledge Innovation Program of Chinese Academy of Sciences (Grant No.KJCX3.SYW.N3)the National Natural Science Foundation of China (Grant No.10675159)the Shanghai Natural Science Foundation (Grant No.09ZR1438200)
文摘In this paper, the impact of the viaduct on flow and traffic exhausting particles dispersion within urban street canyons was numerically simulated using a computational fluid dynamics (CFD) model. Two-dimensional flow and dispersion of particles from traffic exhausts were modeled using the standard k-e turbulence model. The street canyons with a viaduct at different widths and different heights above the ground are simulated. The results show that the airflow in street canyon is evidently in- fluenced by the viaduct: The position of the main vortex center is changed, especially there are two strong vortexes when the viaduct is placed at 10 m height above the ground. It is found based on the study of the particles number concentrations (PNCs) that the viaduct may mitigate the pollution level in the street canyon sometimes. The impact of the viaduct width on PNCs is stronger than that of the height. The study of PNDs reveals that the mean PNCs at the wall of upwind building increase when a viaduct is placed in street canyon. In addition, it is found based on the study of mean particles residence time (PRT) that the removal of the particles strongly correlates to the mean PNCs. The results indicate that the viaduct is an important factor to influence the flow patterns and particles dispersion in street canyons.
基金financially supported by Guangdong Natural Science Foundation (No.2016A030312015)the Science and Technology Cooperation Project of Guangdong Province (No.2013B050800027)the Science and Technology Cooperation Project of Guangzhou (No.201508030001)。
文摘7 YSZ coating was prepared by plasma sprayphysical vapor deposition(PS-PVD) technique based on a specific experimental design.The microstructure and deposition properties of 7 YSZ coating along the radius of plasma jet were investigated in detail.Results show that the coating presents regional characteristic in the radial direction,which could be divided into three typical zones:In Zone Ⅰ,the coating is all composed of columnar structures with cauliflower structure,and the coating properties including the surface roughness and deposition efficiency(DE) are almost stable;in Zone Ⅲ,the coating is made up of solid particles,droplet and gas phase mixed without columnar structures;Zone Ⅱ is between Zone Ⅰ and ZoneⅢ, in which there are columns with domed top and small particles.Based on experiment results,a model on the state and distribution of particles in plasma jet was proposed to clarify the regional characteristic.This study is helpful to comprehend and control coatings deposition by PS-PVD technique.
基金supported by the National Nature Science Foundation of China(No.D010504)the Strategic Priority Research Program of the Chinese Academy of Sciences(No.XDB05000000)
文摘The present article provides an overview of the chemical and physical features of haze in China, focusing on the relationship between haze and atmospheric fine particles, and the formation mechanism of haze. It also summarizes several of control technologies and strategies to mitigate the occurrence of haze. The development of instruments and the analysis of measurements of ambient particles and precursor concentrations have provided important information about haze formation. Indeed, the use of new instruments has greatly facilitated current haze research in China. Examples of insightful results include the relationship between fine particles and haze, the chemical compositions and sources of particles, the impacts of the aging process on haze formation, and the application of technologies that control the formation of haze. Based on these results, two relevant issues need to be addressed: understanding the relationship between haze and fine particles and understanding how to control PM2.5.
基金financially supported by the Major Program of National Natural Science Foundation of China(no.11132008)
文摘The evolution equations of moments for the Brownian coagulation of nanoparticles in both continuum and free molecule regimes are analytically studied. These equations are derived using a Taylor-expansion technique. The self-preserving size distribution is investigated using a newly defined dimensionless parameter, and the asymptotic values for this parameter are theoretically determined. The dimensionless time required for an initial size distribution to achieve self-preservation is also derived in both regimes. Once the size distribution becomes self-preserving, the time evolution of the zeroth and second moments can be theoretically obtained, and it is found that the second moment varies linearly with time in the continuum regime. Equivalent equations, rather than the original ones from which they are derived, can be employed to improve the accuracy of the results and reduce the computational cost for Brownian coagulation in the continuum regime as well as the free molecule regime.
基金sponsored by the California Air Resources Board (ARB) under DRI project number 04-307U.S. EPA's Supersites Program at Fresno
文摘Size distributions of ambient aerosols at the Fresno Supersite were measured with four commercially available scanning mobility particle sizers (SMPS). TSI nano, TSI standard, Grimm, and MSP instruments were collocated at the Fresno Supersite and particle size distributions were measured continuously from August 18 through September 18, 2005. For particles with diameters between 10 and 200 nm, differences among hourly-average ambient particle concentrations ranged from 0% between the TSI nano and Grimm in the 30-50 nm size range to 39% between the Grimm and MSP in the 10-30 nm size range. MSP concentrations were 10-33% lower than those measured with the TSI standard for particles smaller than 200 nm. The TSI nano and TSI standard agreed to within 5% in their overlapping size range (10-84 nm). The TSI nano and Grimm agreed to within 40% for 5-10 nm particles.
基金Supported by National Natural Science Foundation of China(11475068,11247021)Excellent Youth Foundation of Hubei Scientific Committee(2006ABB036)Key Laboratory foundation of Quark and Lepton Physics(Hua-Zhong Normal University)(QLPL2014P01)
文摘The parton and hadron cascade model PACIAE is used to investigate strange particle production in Au + Au collisions at √s = 62.4 GeV in different centralities and at √s =39, 11.5 and 7.7 GeV in the most central collision, respectively. It is shown that the transverse momentum distributions of strange particles by the PACIAE model fit the RHIC Beam Energy Scan experimental results well.