By solving the time-dependent Schr6dinger equation, the dependence of photoelectron energy spectra on the binding energy of targets, wavelength and the intensity of laser pulse is exhibited and a scaling law of kineti...By solving the time-dependent Schr6dinger equation, the dependence of photoelectron energy spectra on the binding energy of targets, wavelength and the intensity of laser pulse is exhibited and a scaling law of kinetic energy spectra of both the direct and the rescattered photoelectrons is concluded. The scaling law provides a convenient tool to determine the equivalent photoionization process of various atoms or molecules in various laser fields. The verification of the scaling law by independent methods provides incontestable support to the validity of the scaling law.展开更多
By developing a full quantum scattering theory of high-order above-threshold ionization,we study the energy spectra and the angular distributions of photoelectrons from atoms with intense laser fields shining on them....By developing a full quantum scattering theory of high-order above-threshold ionization,we study the energy spectra and the angular distributions of photoelectrons from atoms with intense laser fields shining on them.We find that real rescattering can occur many times,and even infinite times.The photoelectrons from the rescattering process form a broad plateau in the kinetic-energy spectrum.We further disclose a multiple-plateau structure formed by the high-energy photoelectrons,which absorb many photons during the rescattering process.Moreover,we find that both the angular distributions and the kinetic-energy spectra of photoelectrons obey the same scaling law as that for directly emitted photoelectrons.展开更多
The photoelectron energy spectra (PESs) excited by monochromatic femtosecond x-ray pulses in the presence of a femtosecond laser are investigated. APES is composed of a set of separate peaks, showing interesting com...The photoelectron energy spectra (PESs) excited by monochromatic femtosecond x-ray pulses in the presence of a femtosecond laser are investigated. APES is composed of a set of separate peaks, showing interesting comb-like structures. These structures result from the quantum interferences between photoelectron wave packets generated at different times. The width and the localization of each peak as well as the number of peaks are determined by all the laser and x-ray parameters. Most of peak heights of the PES are higher than the classical predictions.展开更多
The photoelectron energy spectra (PESs) excited by narrow bandwidth attosecond x-ray pulses in the presence of a few-cycle laser are quantum-mechanically calculated. Transfer equations are used to reconstruct the de...The photoelectron energy spectra (PESs) excited by narrow bandwidth attosecond x-ray pulses in the presence of a few-cycle laser are quantum-mechanically calculated. Transfer equations are used to reconstruct the detailed temporal structure of an attosecond x-ray pulse directly from a measured PES. Theoretical analysis shows that the temporal uncertainties of the pulse reconstruction depend on the x-ray bandwidth. The procedure of pulse reconstruction is direct and simple without making any previous pulse assumption, data fitting analysis and time-resolved measurement of PESs. The temporal measurement range is half of a laser optical cycle.展开更多
Investigations show that X-ray-boosted photoionization (XBP) has the following advantages for in-situ measurements of ultrahigh laser intensity 1 and field envelope F(t) (time t, pulse duration VL, carrier-envelo...Investigations show that X-ray-boosted photoionization (XBP) has the following advantages for in-situ measurements of ultrahigh laser intensity 1 and field envelope F(t) (time t, pulse duration VL, carrier-envelope-phase Ф): accuracy, dynamic range, and rapidness. The calculated XBP spectra resemble inversely proportional functions of the photoelectron momentum shift. The maximum momentum p and the observable value Q (defined as a double integration of a normalized photoelectron energy spectrum, PES) linearly depend on I^1/2 and τL, respectively. Ф and F(t) can be determined from the PES cut-off energy and peak positions. The measurable laser intensity can be up to and over 1018 W/cm2 by using high energy X-rays and highly charged inert gases.展开更多
基金Project supported by the National Natural Science Foundation of China (Grant Nos. 61078080 and 11174304)the National Basic Research Program of China (Grant Nos. 2010CB923203 and 2011CB808103)
文摘By solving the time-dependent Schr6dinger equation, the dependence of photoelectron energy spectra on the binding energy of targets, wavelength and the intensity of laser pulse is exhibited and a scaling law of kinetic energy spectra of both the direct and the rescattered photoelectrons is concluded. The scaling law provides a convenient tool to determine the equivalent photoionization process of various atoms or molecules in various laser fields. The verification of the scaling law by independent methods provides incontestable support to the validity of the scaling law.
基金Project supported by the National Natural Science Foundation of China (Grant Nos. 10774513,61078080,11174304,and 11104167)the National Basic Research Program of China (Grant Nos. 2010CB923203 and 2011CB808103)
文摘By developing a full quantum scattering theory of high-order above-threshold ionization,we study the energy spectra and the angular distributions of photoelectrons from atoms with intense laser fields shining on them.We find that real rescattering can occur many times,and even infinite times.The photoelectrons from the rescattering process form a broad plateau in the kinetic-energy spectrum.We further disclose a multiple-plateau structure formed by the high-energy photoelectrons,which absorb many photons during the rescattering process.Moreover,we find that both the angular distributions and the kinetic-energy spectra of photoelectrons obey the same scaling law as that for directly emitted photoelectrons.
基金Project supported by the National Natural Science Foundation of China (Grant No 10675014)
文摘The photoelectron energy spectra (PESs) excited by monochromatic femtosecond x-ray pulses in the presence of a femtosecond laser are investigated. APES is composed of a set of separate peaks, showing interesting comb-like structures. These structures result from the quantum interferences between photoelectron wave packets generated at different times. The width and the localization of each peak as well as the number of peaks are determined by all the laser and x-ray parameters. Most of peak heights of the PES are higher than the classical predictions.
基金Project supported by the National Natural Science Foundation of China (Grant No 10675014)
文摘The photoelectron energy spectra (PESs) excited by narrow bandwidth attosecond x-ray pulses in the presence of a few-cycle laser are quantum-mechanically calculated. Transfer equations are used to reconstruct the detailed temporal structure of an attosecond x-ray pulse directly from a measured PES. Theoretical analysis shows that the temporal uncertainties of the pulse reconstruction depend on the x-ray bandwidth. The procedure of pulse reconstruction is direct and simple without making any previous pulse assumption, data fitting analysis and time-resolved measurement of PESs. The temporal measurement range is half of a laser optical cycle.
基金supported by the National Natural Science Foundation of China (Grant No. 11175010)
文摘Investigations show that X-ray-boosted photoionization (XBP) has the following advantages for in-situ measurements of ultrahigh laser intensity 1 and field envelope F(t) (time t, pulse duration VL, carrier-envelope-phase Ф): accuracy, dynamic range, and rapidness. The calculated XBP spectra resemble inversely proportional functions of the photoelectron momentum shift. The maximum momentum p and the observable value Q (defined as a double integration of a normalized photoelectron energy spectrum, PES) linearly depend on I^1/2 and τL, respectively. Ф and F(t) can be determined from the PES cut-off energy and peak positions. The measurable laser intensity can be up to and over 1018 W/cm2 by using high energy X-rays and highly charged inert gases.