A multi-anabranch river with three braid bars is a typical river pattern in nature, but no studies have been conducted to describe mixing characteristics of pollutants in the river. In this study, a physical model of ...A multi-anabranch river with three braid bars is a typical river pattern in nature, but no studies have been conducted to describe mixing characteristics of pollutants in the river. In this study, a physical model of a typical multi-anabranch river with three braid bars was established to explore the pollutant mixing characteristics in different branches. The multi-anabranch reach was separated into seven branches, B1, B2, B3, B4, B5, B6, and BT, by three braid bars. Five tracer release positions located 2.9 m upstream from the inlet section of the multi-anabranch reach were adopted, and the distances from the five positions to the left bank of the upstream main channel were 1/6B, 1/3B, 1/2B, 2/3B, and 5/6B (B is the width of the upstream main channel), respectively. The longitudinal velocities and pollutant concentrations in the seven branches were measured. The planar flow field and mixing characteristics of pollutants from the bottom to the surface in the multi-anabranch river were obtained and analyzed. The results show that the pollutant release positions are the main influencing factors in the pollutant transport process, and the diversion points and pollutant release positions jointly influence the percentage ratios of the pollutant fluxes in branches B 1, B2, and B3 to the pollutant flux in the upstream main channel.展开更多
Objective To study the possibility of removing nitrogen, phosphorus, and organic pollutants using seeding type immobilized microorganisms. Methods Lakes P and M in Wuhan were chosen as the objects to study the removal...Objective To study the possibility of removing nitrogen, phosphorus, and organic pollutants using seeding type immobilized microorganisms. Methods Lakes P and M in Wuhan were chosen as the objects to study the removal of nitrogen, phosphorus, and organic pollutants with the seeding type immobilized microorganisms. Correlations between the quantity of heterotrophic bacteria and the total nitrogen (TN), total phosphorus (TP), and total organic carbon (TOC) in the two lakes were studied. The dominant bacteria were detected, inoculated to the sludge and acclimated by increasing nitrogen, phosphorus and decreasing carbon source in an intermittent, time-controlled and fixed-quantity way. The bacteria were then used to prepare the seeding type immobilized microorganisms, selecting diatomite as the adsorbent cartier. The ability and influence factors of removing nitrogen, phosphorus, and organic pollutant from water samples by the seeding type immobilized microorganisms were studied. Results The coefficients of the heterotrophic bacterial quantity correlated with TOC, TP, and TN were 0.9143, 0.8229, 0.7954 in Lake P and 0.9168, 0.7187, 0.6022 in Lake M. Ten strains of dominant heterotrophic bacteria belonging to Pseudomonas, Coccus, Aeromonas, Bacillus, and Enterobateriaceae, separately, were isolated. The appropriate conditions for the seeding type immobilized microorgansims in purifying the water sample were exposure time=24 h, pH=7.0-8.0, and quantity of the immobilized microorganisms=0.75-1g/50 mL. The removal rates of TOC, TP, and TN under the above conditions were 80.2%, 81.6%, and 86.8%, respectively. Conclusion The amount of heterotrophic bacteria in the two lakes was correlated with TOC, TP, and TN. These bacteria could be acclimatized and prepared for the immobilized microorganisms which could effectively remove nitrogen, phosphorus, and mixed organic pollutants in the water sample.展开更多
Numerical simulations are carried out to investigate the effect of cloud condensation nuclei(CCN) concentrations on microphysical processes and precipitation characteristics of hailstorms. Two hailstorm cases are si...Numerical simulations are carried out to investigate the effect of cloud condensation nuclei(CCN) concentrations on microphysical processes and precipitation characteristics of hailstorms. Two hailstorm cases are simulated, a spring case and a summer case, in a semiarid region of northern China, with the Regional Atmospheric Modeling System. The results are used to investigate the differences and similarities of the CCN effects between spring and summer hailstorms. The similarities are:(1) The total hydrometeor mixing ratio decreases, while the total ice-phase mixing ratio enhances, with increasing CCN concentration;(2) Enhancement of the CCN concentration results in the production of a greater amount of small-sized hydrometeor particles, but a lessening of large-sized hydrometeor particles;(3) As the CCN concentration increases, the supercooled cloud water and rainwater make a lesser contribution to hail, while the ice-phase hydrometeors take on active roles in the growth of hail;(4) When the CCN concentration increases, the amount of total precipitation lessens,while the role played by liquid-phase rainfall in the amount of total precipitation reduces, relatively, compared to that of icephase precipitation. The differences between the two storms include:(1) An increase in the CCN concentration tends to reduce pristine ice mixing ratios in the spring case but enhance them in the summer case;(2) Ice-phase hydrometeor particles contribute more to hail growth in the spring case, while liquid water contributes more in the summer case;(3) An increase in the CCN concentration has different effects on surface hail precipitation in different seasons.展开更多
To investigate the composition and possible sources of particles, especially during heavy haze pollution, a single particle aerosol mass spectrometer(SPAMS) was deployed to measure the changes of single particle spe...To investigate the composition and possible sources of particles, especially during heavy haze pollution, a single particle aerosol mass spectrometer(SPAMS) was deployed to measure the changes of single particle species and sizes during October of 2014, in Beijing. A total of 2,871,431 particles with both positive and negative spectra were collected and characterized in combination with the adaptive resonance theory neural network algorithm(ART-2a). Eight types of particles were classified: dust particles(dust, 8.1%), elemental carbon(EC, 29.0%), organic carbon(OC, 18.0%), EC and OC combined particles(ECOC, 9.5%),Na-K containing particles(Na K, 7.9%), K-containing particles(K, 21.8%), organic nitrogen and potassium containing particles(KCN, 2.3%), and metal-containing particles(metal,3.6%). Three haze pollution events(P1, P2, P3) and one clean period(clean) were analyzed,based on the mass and number concentration of PM_(2.5)and the back trajectory results from the hybrid single particle Lagrangian integrated trajectory model(Hysplit-4 model). Results showed that EC, OC and K were the major components of single particles during the three haze pollution periods, which showed clearly increased ratios compared with those in the clean period. Results from the mixing state of secondary species of different types of particles showed that sulfate and nitrate were more readily mixed with carbon-containing particles during haze pollution episodes than in clean periods.展开更多
There are multiple contaminants in practical wastewater;and the photodegradation of mixed pollutants is a challenge in the field of photocatalysis.Herein,we design a mesoporous 2D/2D TiO_(2)(B)-BiOBr heterojunction ph...There are multiple contaminants in practical wastewater;and the photodegradation of mixed pollutants is a challenge in the field of photocatalysis.Herein,we design a mesoporous 2D/2D TiO_(2)(B)-BiOBr heterojunction photocatalyst for the photodegradation of mixed pollutants.Such a coupling structure results in an enhancement in the disconnection of photoexcited carriers,and the increase of absorption and reaction sites.The 2D/2D TiO_(2)(B)-BiOBr demonstrates outstanding photocatalytic activity for photodegrading rhodamine B(RhB),methyl orange(MO),tetracycline hydrochloride(TCH),and bisphenol A(BPA)simultaneously under visible light,which is 4.7,1.4,23 and 16.4 times as high as that of original BiOBr,respectively.Our work represents a possible solution to devise promising and efficient photocatalysts for the treatment of practical wastewater in the near future.展开更多
This study explored different methodologiesusing a C-band RADARSAT-2 quad-polarized SyntheticAperture Radar (SAR) image located over China's YellowSea to investigate polarization decomposition parametersfor identif...This study explored different methodologiesusing a C-band RADARSAT-2 quad-polarized SyntheticAperture Radar (SAR) image located over China's YellowSea to investigate polarization decomposition parametersfor identifying mixed floating pollutants from a complexocean background. It was found that solitary polarizationdecomposition did not meet the demand for detecting andclassifying multiple floating pollutants, even after applyinga polarized SAR image. Furthermore, considering thatYamaguchi decomposition is sensitive to vegetation andthe algal variety Enteromorpha prolifera, while H/A/alphadecomposition is sensitive to oil spills, a combination ofparameters which was deduced from these two decom-positions was proposed for marine environmental mon-itoring of mixed floating sea surface pollutants. Acombination of volume scattering, surface scattering, andscattering entropy was the best indicator for classifyingmixed floating pollutants from a complex ocean back-ground. The Kappa coefficients for Enteromorpha pro-lifera and oil spills were 0.7514 and 0.8470, respectively,evidence that the composite polarized parameters based onquad-polarized SAR imagery proposed in this research isan effective monitoring method for complex marinepollution.展开更多
基金supported by the National Basic Research Program of China (973 Program, Grant No.2008CB418202)the National Natural Science Foundation of China (Grants No. 50979026 and 51179052)+3 种基金the National Key Technologies R&D Program of China (Grant No. 2012BAB03B04) the Special Fund for Public Welfare Industry of the Ministry of Water Resources of China (Grant No. 201001028)the "Six Talent Peak" Project of Jiangsu Province (Grant No. 08-C) the Fundamental Research Funds for the Central Universities (Grant No. 2010B15514)
文摘A multi-anabranch river with three braid bars is a typical river pattern in nature, but no studies have been conducted to describe mixing characteristics of pollutants in the river. In this study, a physical model of a typical multi-anabranch river with three braid bars was established to explore the pollutant mixing characteristics in different branches. The multi-anabranch reach was separated into seven branches, B1, B2, B3, B4, B5, B6, and BT, by three braid bars. Five tracer release positions located 2.9 m upstream from the inlet section of the multi-anabranch reach were adopted, and the distances from the five positions to the left bank of the upstream main channel were 1/6B, 1/3B, 1/2B, 2/3B, and 5/6B (B is the width of the upstream main channel), respectively. The longitudinal velocities and pollutant concentrations in the seven branches were measured. The planar flow field and mixing characteristics of pollutants from the bottom to the surface in the multi-anabranch river were obtained and analyzed. The results show that the pollutant release positions are the main influencing factors in the pollutant transport process, and the diversion points and pollutant release positions jointly influence the percentage ratios of the pollutant fluxes in branches B 1, B2, and B3 to the pollutant flux in the upstream main channel.
基金This work was supported by the National Natural Science Foundation of China (No. 30400346)
文摘Objective To study the possibility of removing nitrogen, phosphorus, and organic pollutants using seeding type immobilized microorganisms. Methods Lakes P and M in Wuhan were chosen as the objects to study the removal of nitrogen, phosphorus, and organic pollutants with the seeding type immobilized microorganisms. Correlations between the quantity of heterotrophic bacteria and the total nitrogen (TN), total phosphorus (TP), and total organic carbon (TOC) in the two lakes were studied. The dominant bacteria were detected, inoculated to the sludge and acclimated by increasing nitrogen, phosphorus and decreasing carbon source in an intermittent, time-controlled and fixed-quantity way. The bacteria were then used to prepare the seeding type immobilized microorganisms, selecting diatomite as the adsorbent cartier. The ability and influence factors of removing nitrogen, phosphorus, and organic pollutant from water samples by the seeding type immobilized microorganisms were studied. Results The coefficients of the heterotrophic bacterial quantity correlated with TOC, TP, and TN were 0.9143, 0.8229, 0.7954 in Lake P and 0.9168, 0.7187, 0.6022 in Lake M. Ten strains of dominant heterotrophic bacteria belonging to Pseudomonas, Coccus, Aeromonas, Bacillus, and Enterobateriaceae, separately, were isolated. The appropriate conditions for the seeding type immobilized microorgansims in purifying the water sample were exposure time=24 h, pH=7.0-8.0, and quantity of the immobilized microorganisms=0.75-1g/50 mL. The removal rates of TOC, TP, and TN under the above conditions were 80.2%, 81.6%, and 86.8%, respectively. Conclusion The amount of heterotrophic bacteria in the two lakes was correlated with TOC, TP, and TN. These bacteria could be acclimatized and prepared for the immobilized microorganisms which could effectively remove nitrogen, phosphorus, and mixed organic pollutants in the water sample.
基金supported by the National Natural Science Foundation of China (Grant Nos. 41205099 and 41575037)the National Science Foundation of China (Grant No. 41405128)+2 种基金the National Grand Fundamental Research 973 Programs of China (Grant Nos. 2014CB441403 and 2013CB430105)the Special Scientific Research Project of the Meteorological Public Welfare Profession of China (Grant No. GYHY201006031)the Guizhou Province Scientific Research Joint Project (Grant No. G[2013]4001)
文摘Numerical simulations are carried out to investigate the effect of cloud condensation nuclei(CCN) concentrations on microphysical processes and precipitation characteristics of hailstorms. Two hailstorm cases are simulated, a spring case and a summer case, in a semiarid region of northern China, with the Regional Atmospheric Modeling System. The results are used to investigate the differences and similarities of the CCN effects between spring and summer hailstorms. The similarities are:(1) The total hydrometeor mixing ratio decreases, while the total ice-phase mixing ratio enhances, with increasing CCN concentration;(2) Enhancement of the CCN concentration results in the production of a greater amount of small-sized hydrometeor particles, but a lessening of large-sized hydrometeor particles;(3) As the CCN concentration increases, the supercooled cloud water and rainwater make a lesser contribution to hail, while the ice-phase hydrometeors take on active roles in the growth of hail;(4) When the CCN concentration increases, the amount of total precipitation lessens,while the role played by liquid-phase rainfall in the amount of total precipitation reduces, relatively, compared to that of icephase precipitation. The differences between the two storms include:(1) An increase in the CCN concentration tends to reduce pristine ice mixing ratios in the spring case but enhance them in the summer case;(2) Ice-phase hydrometeor particles contribute more to hail growth in the spring case, while liquid water contributes more in the summer case;(3) An increase in the CCN concentration has different effects on surface hail precipitation in different seasons.
基金supported by the National Natural Science Foundation of China (No.41205115)
文摘To investigate the composition and possible sources of particles, especially during heavy haze pollution, a single particle aerosol mass spectrometer(SPAMS) was deployed to measure the changes of single particle species and sizes during October of 2014, in Beijing. A total of 2,871,431 particles with both positive and negative spectra were collected and characterized in combination with the adaptive resonance theory neural network algorithm(ART-2a). Eight types of particles were classified: dust particles(dust, 8.1%), elemental carbon(EC, 29.0%), organic carbon(OC, 18.0%), EC and OC combined particles(ECOC, 9.5%),Na-K containing particles(Na K, 7.9%), K-containing particles(K, 21.8%), organic nitrogen and potassium containing particles(KCN, 2.3%), and metal-containing particles(metal,3.6%). Three haze pollution events(P1, P2, P3) and one clean period(clean) were analyzed,based on the mass and number concentration of PM_(2.5)and the back trajectory results from the hybrid single particle Lagrangian integrated trajectory model(Hysplit-4 model). Results showed that EC, OC and K were the major components of single particles during the three haze pollution periods, which showed clearly increased ratios compared with those in the clean period. Results from the mixing state of secondary species of different types of particles showed that sulfate and nitrate were more readily mixed with carbon-containing particles during haze pollution episodes than in clean periods.
基金funding support from the National Science Foundation of China(NO.220413201)。
文摘There are multiple contaminants in practical wastewater;and the photodegradation of mixed pollutants is a challenge in the field of photocatalysis.Herein,we design a mesoporous 2D/2D TiO_(2)(B)-BiOBr heterojunction photocatalyst for the photodegradation of mixed pollutants.Such a coupling structure results in an enhancement in the disconnection of photoexcited carriers,and the increase of absorption and reaction sites.The 2D/2D TiO_(2)(B)-BiOBr demonstrates outstanding photocatalytic activity for photodegrading rhodamine B(RhB),methyl orange(MO),tetracycline hydrochloride(TCH),and bisphenol A(BPA)simultaneously under visible light,which is 4.7,1.4,23 and 16.4 times as high as that of original BiOBr,respectively.Our work represents a possible solution to devise promising and efficient photocatalysts for the treatment of practical wastewater in the near future.
文摘This study explored different methodologiesusing a C-band RADARSAT-2 quad-polarized SyntheticAperture Radar (SAR) image located over China's YellowSea to investigate polarization decomposition parametersfor identifying mixed floating pollutants from a complexocean background. It was found that solitary polarizationdecomposition did not meet the demand for detecting andclassifying multiple floating pollutants, even after applyinga polarized SAR image. Furthermore, considering thatYamaguchi decomposition is sensitive to vegetation andthe algal variety Enteromorpha prolifera, while H/A/alphadecomposition is sensitive to oil spills, a combination ofparameters which was deduced from these two decom-positions was proposed for marine environmental mon-itoring of mixed floating sea surface pollutants. Acombination of volume scattering, surface scattering, andscattering entropy was the best indicator for classifyingmixed floating pollutants from a complex ocean back-ground. The Kappa coefficients for Enteromorpha pro-lifera and oil spills were 0.7514 and 0.8470, respectively,evidence that the composite polarized parameters based onquad-polarized SAR imagery proposed in this research isan effective monitoring method for complex marinepollution.