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Studies on the Characteristics of Nitrogen and Phosphorus Pollution of Natural Outcrop Springs in Wudalianchi
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作者 魏晓雪 李月兴 +4 位作者 王菁华 方振兴 潘虹 曾颖 杨臣 《Agricultural Science & Technology》 CAS 2015年第5期1019-1022,共4页
Objective] The research aimed to study the characteristics of nitrogen and phosphorus pollution of 30 natural outcrop springs in Wudalianchi, which provides a theoretical basis for the sustainable development and util... Objective] The research aimed to study the characteristics of nitrogen and phosphorus pollution of 30 natural outcrop springs in Wudalianchi, which provides a theoretical basis for the sustainable development and utilization and protection of Wudalianchi natural mineral resources. [Method] Choosing the 30 natural outcrop spring representatives in different regions, samples were collected in low water period, normal water period, wet period respectively, and the content of nitrogen, phosphorus and other contaminants in the samples were determined. Besides, the pollution characteristics of nitrogen and phosphorus in Wudalianchi natural outcrop spring were analyzed. [Result] The 30 natural outcrop spring in Wudalianchi area were seriously polluted by nitrogen. Total nitrogen and nitrate nitrogen were the main forms of nitrogen pollution. The content of total phosphorus and ammonia nitrogen were low. [Conclusion] The natural outcrop spring is mainly caused by agricultural non-point source pollution. 展开更多
关键词 WUDALIANCHI SPRINGS nitrogen and phosphorus pollution
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Removal of Nitrogen, Phosphorus, and Organic Pollutants From Water Using Seeding Type Immobilized Microorganisms 被引量:6
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作者 LIN WANG LI-JING HUANG LUO-JIA YUN FEI TANG JING-HUI ZHAO YAN-QUN LIU XIN ZENG QI-FANG LUO 《Biomedical and Environmental Sciences》 SCIE CAS CSCD 2008年第2期150-156,共7页
Objective To study the possibility of removing nitrogen, phosphorus, and organic pollutants using seeding type immobilized microorganisms. Methods Lakes P and M in Wuhan were chosen as the objects to study the removal... Objective To study the possibility of removing nitrogen, phosphorus, and organic pollutants using seeding type immobilized microorganisms. Methods Lakes P and M in Wuhan were chosen as the objects to study the removal of nitrogen, phosphorus, and organic pollutants with the seeding type immobilized microorganisms. Correlations between the quantity of heterotrophic bacteria and the total nitrogen (TN), total phosphorus (TP), and total organic carbon (TOC) in the two lakes were studied. The dominant bacteria were detected, inoculated to the sludge and acclimated by increasing nitrogen, phosphorus and decreasing carbon source in an intermittent, time-controlled and fixed-quantity way. The bacteria were then used to prepare the seeding type immobilized microorganisms, selecting diatomite as the adsorbent cartier. The ability and influence factors of removing nitrogen, phosphorus, and organic pollutant from water samples by the seeding type immobilized microorganisms were studied. Results The coefficients of the heterotrophic bacterial quantity correlated with TOC, TP, and TN were 0.9143, 0.8229, 0.7954 in Lake P and 0.9168, 0.7187, 0.6022 in Lake M. Ten strains of dominant heterotrophic bacteria belonging to Pseudomonas, Coccus, Aeromonas, Bacillus, and Enterobateriaceae, separately, were isolated. The appropriate conditions for the seeding type immobilized microorgansims in purifying the water sample were exposure time=24 h, pH=7.0-8.0, and quantity of the immobilized microorganisms=0.75-1g/50 mL. The removal rates of TOC, TP, and TN under the above conditions were 80.2%, 81.6%, and 86.8%, respectively. Conclusion The amount of heterotrophic bacteria in the two lakes was correlated with TOC, TP, and TN. These bacteria could be acclimatized and prepared for the immobilized microorganisms which could effectively remove nitrogen, phosphorus, and mixed organic pollutants in the water sample. 展开更多
关键词 Heterotrophic bacteria ACCLIMATION Immobilized microorganisms nitrogen phosphorus Mixed organic pollutants
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Characteristics of diffuse pollution of nitrogen and phosphorous from a small town in the hilly area of the central Sichuan Basin,China 被引量:1
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作者 YANG Xiao-lin SHEN Xi ZHU Bo 《Journal of Mountain Science》 SCIE CSCD 2016年第2期292-301,共10页
Hydrological and hydro-chemical monitoring of nitrogen(N) and phosphorus(P) in a small urbanized catchment was conducted in the hilly area of the central Sichuan Basin,China,from 2010 through 2011.The diffuse N and P ... Hydrological and hydro-chemical monitoring of nitrogen(N) and phosphorus(P) in a small urbanized catchment was conducted in the hilly area of the central Sichuan Basin,China,from 2010 through 2011.The diffuse N and P loadings in different forms of total nitrogen(TN) and phosphorus(TP),dissolved nitrogen(DN) and phosphorus(DP),as well as particulate nitrogen(PN) and phosphorus(PP) were calculated based on runoff discharges and chemical analyses.The results revealed that the diffuse pollution concentrations of TN,DN,PN,TP,DP and PP exhibited large variations during rainfall events,with peak concentrations occurring during the initial period.For all of the measured parameters,the event mean concentrations(EMCs) were observed to clearly vary among rainfall events.The EMCs of TN,DN,PN,TP,DP and PP(for all of the observed rainfall events) were 10.04,6.62,3.42,1.30,0.47 and0.83 mg/L,respectively.The losses of diffuse N and P exhibited clear seasonal patterns and mainly occurred during the period from July through September,when the losses totaled 99.3 and 9.6 kg/ha for TN and TP,respectively,accounting for 75% and 74% of the total annual loadings.The mean annual loadings of TN and TP were 124.6 and 12.9 kg/ha,respectively.The results indicate that residential areas in the hilly areaof the central Sichuan Basin are subject to high diffuse N and P loadings,posing a serious risk to the receiving water quality.Ecological buffering belts are recommended to incorporate into the urbanized catchment to reduce diffuse pollution. 展开更多
关键词 nitrogen transport phosphorus transport Event mean concentration pollution loading pollution sources Non-point-source pollution Yanting Agro-ecological Station
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Controlling effects of forest belts on non-point source pollution of agricultural lands in Taihu Lake area, China 被引量:1
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作者 陈金林 侍璐璐 张爱国 《Journal of Forestry Research》 SCIE CAS CSCD 2002年第3期213-216,251,共4页
Taihu Lake area is one of the most developed areas in agricultural production. Application of fertilizers and pesticides in large quantities greatly aggravate environmental pollution of this area, and water pollution ... Taihu Lake area is one of the most developed areas in agricultural production. Application of fertilizers and pesticides in large quantities greatly aggravate environmental pollution of this area, and water pollution has worsened to an unbearable condition. Two sampling farms (respectively 1 hm2) under rape-rice rotation and wheat-rice rotation were selected as studied ecosystem and a 5-yr-old Poplar forest and 8-yr-old Metasequoia forest were chosen in the selected areas. By collecting samples of Nitrogen, Phosphorus in water, crops and underground of forest, the transfer and loss of N and P (main water pollutants) in faming ecosystem were studied, and the effects of forest belts on non-point source pollution of agricultural lands was analyzed. The results indicated that the transfer and loss of N and P vary with means of rotation, types of crops and the amount of fertilizer application. Buffering forest belts betweens farmlands and ditches can effectively stop and purify such elements as N and P in soil runoffs, thus controlling non-point source pollution of agricultural lands. When the width ratio of farmland to forest belt is 100 to 40, 50.05% losing N, 29.37% losing P can be absorbed by forest under rape-rice rotation and 30.98% N, 86.73% P can be absorbed by forest under wheat-rice rotation. When the width ratio of farmland to forest belt is 150 to 40, 33.37% losing N, 19.58% losing P can be absorbed by the forest under rape-rice rotation, and under wheat-rice rotation 20.65% lost N and 57.82% lost P can be absorbed. There is only some purification effect when the width ration of farmland to forest belt is 200 to 40. Based on model of buffering forest belts, the width ratio of farmland to forest is determined between 100 to 40 and 150 to 40, because it not only can purify water, but also occupy less farmland. It is suggested that Poplars, with the characteristics of fast-growing and high value, are suitable to be planted as shelter-forest in Taihu Lake Watershed. 展开更多
关键词 AGRICULTURE Non-point source pollution Ultrophication nitrogen phosphorus Forest belt Sustainable development
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Non-Point-Source Nitrogen and Phosphorus Loadings from a Small Watershed in the Three Gorges Reservoir Area 被引量:25
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作者 ZHU BO WANG Zhenhua +1 位作者 WANG Tao DONG Zhixin 《Journal of Mountain Science》 SCIE CSCD 2012年第1期10-15,共6页
Non-point-source pollution has become a major threat to the water quality of the Three Gorges Reservoir(TGR);however,nutrient loadings from terrestrial sources are unclear due to a lack of in situ monitoring.A represe... Non-point-source pollution has become a major threat to the water quality of the Three Gorges Reservoir(TGR);however,nutrient loadings from terrestrial sources are unclear due to a lack of in situ monitoring.A representative small watershed in the central part of the TGR area was selected to monitor the loss of nitrogen(N) and phosphorous(P) continuously along with the runoff from 2007 through 2009 to understand the exact sources and loadings.Results show that the non-point-source nitrogen and phosphorus comes mainly from the storm runoff from residential areas,citrus orchards and sloping croplands,which contributes up to 76% of the loadings in this watershed.Thus,a crucial measure for controlling non-point-source pollution is to intercept storm runoff from the three sources.Paddy fields provide a sink for non-point-source N and P by intercepting the runoff and sediment along with their different forms of nitrogen and phosphorus.The N and P removal efficiency by paddy fields from residential areas is within the range of 56% to 98%.Paddy fields are an important land-use option for reducing the non-point-source loading of N and P in the TGR area. 展开更多
关键词 Non-point-source pollution Source and sink nitrogen phosphorus Paddy fields Three Gorges Reservoir area China
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Nitrogen and Phosphorus Loss Law and Emission Reduction Effects Under Water and Fertilizer Management Integrated Mode in Dike Paddy Field 被引量:2
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作者 GUO Longsheng ZHOU Guangtao GUO Zhongyuan 《Journal of Northeast Agricultural University(English Edition)》 CAS 2009年第4期31-37,共7页
To achieve the purpose of reducing farm non-point source pollution, we integrated site specific nitrogen management precise irrigation, controlled drainage, and wetland eco-repair system in dike area of Taihu basin. D... To achieve the purpose of reducing farm non-point source pollution, we integrated site specific nitrogen management precise irrigation, controlled drainage, and wetland eco-repair system in dike area of Taihu basin. During investigation, it had given prominence for the water and fertilizer coupling effects of precise irrigation and site specific nutrient management, the characteristics of integration on controlled irrigation, controlled drainage and wetland ecosystem non-point source pollution control. Then the water and fertilizer integrated management mode of paddy field was put forward in Taihu basin where the water production efficiency increased to 1.64 kg. m-3, water saved 37.8%, fertilizer use efficiency raised 15,4%, yield raised 10%, and N, P load decreased 26%-72%. The modern agricultural and farmland ecosystems that control and cut down the farm non-point source pollution came into being, which can be a reference by Taihu basin to control its agricultural non-point source pollution and eutrophicated water body. 展开更多
关键词 paddy field the integrated mode of water and fertilizer management non-point source pollution nitrogen and phosphorus loss
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Validation of an agricultural non-point source(AGNPS)pollution model for a catchment in the Jiulong River watershed,China 被引量:13
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作者 LIU Jianchang ZHANG Luoping +2 位作者 ZHANG Yuzhen HONG Huasheng DENG Hongbing 《Journal of Environmental Sciences》 SCIE EI CAS CSCD 2008年第5期599-606,共8页
This study tested and evaluated the agricultural non-point source (AGNPS) model for the Wuchuan catchment, a typical agricultural area in the Jiulong River watershed, Fujian Province, China. The AGNPS model was cali... This study tested and evaluated the agricultural non-point source (AGNPS) model for the Wuchuan catchment, a typical agricultural area in the Jiulong River watershed, Fujian Province, China. The AGNPS model was calibrated and validated for the study area with observed data on ten storms. The data on eight storms in 2002 were used for calibration while data on two storms were used for validation of the model. Considering the lack of water quality data over a long-term series, a novel method, comparing an internal nested catchment with its surrounding catchment, was used to supplement the less long-term series data. Dual calibration and validation of the AGNPS model was obtained by this comparison. The results indicate that the correlation coefficients were 0.99 and 0.98 for runoff, 0.94 and 0.95 for the peak runoff rate of the large catchment and the small catchment, respectively, and 0.76 for the sediment of the small catchment only. Each pair of correlation coefficients is homogeneous for the same event for the two catchments. With the exception of the sediment yield and particulate phosphorus, the peak runoff rate and other nutrients were well predicted. Sensitivity analysis showed that the Soil Conservation Service curve number and rainfall quantity were the most sensitive parameters, which resulted in high output variations. Erosivity and other parameters had little influence on the hydrological and quality outputs. 展开更多
关键词 non-point source pollution agricultural non-point source (AGNPS) agriculture RUNofF nitrogen phosphorus SEDIMENT
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The land-sourced pollution in the Jiaozhou Bay 被引量:3
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作者 高振会 杨东方 +2 位作者 秦洁 相利宏 张柯 《Chinese Journal of Oceanology and Limnology》 SCIE CAS CSCD 2008年第2期229-232,共4页
In recent years, natural environment of the Jiaozhou Bay has been changed largely by fast developing industry and agriculture of the cities around, from which wastewaters were generated. The size of the bay has been c... In recent years, natural environment of the Jiaozhou Bay has been changed largely by fast developing industry and agriculture of the cities around, from which wastewaters were generated. The size of the bay has been continuously shrunk with reduced river flows, resulting in serious contamination to the marine lives in the bay. After analyzing the basic historical data, the authors put forward a suggestion of how to protect the bay ecology for sustaining the resources in the Jiaozhou Bay. 展开更多
关键词 nutrients nitrogen and phosphorus land-sourced pollution red tide Jiaozhou Bay
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Effect of groundwater on the ecological water environment of typical inland lakes in the Inner Mongolian Plateau 被引量:2
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作者 Chu Yu Li-jie Wu +3 位作者 Yi-long Zhang Xiu-ya Wang Zhan-chuan Wang Zhou Zhang 《Journal of Groundwater Science and Engineering》 2022年第4期353-366,共14页
To explore the causes of the ecological environment deterioration of lakes in the Inner Mongolia Plateau,this study took a typical inland lake Daihai as an example,and investigated the groundwater recharge in the proc... To explore the causes of the ecological environment deterioration of lakes in the Inner Mongolia Plateau,this study took a typical inland lake Daihai as an example,and investigated the groundwater recharge in the process of lake shrinkage and eutrophication.Using the radon isotope(^(222)Rn)as the main means of investigation,the ^(222)Rn mass balance equation was established to evaluate the groundwater recharge in Daihai.The spatial variability of ^(222)Rn activity in lake water and groundwater,the contribution of groundwater recharge to lake water balance and its effect on nitrogen and phosphorus pollution in lake water were discussed.The analysis showed that,mainly controlled by the fault structure,the activity of ^(222)Rn in groundwater north and south of Daihai is higher than that in the east and west,and the difference in lithology and hydraulic gradient may also be the influencing factors of this phenomenon.The ^(222)Rn activity of the middle and southeast of the underlying lake is greater,indicating that the ^(222)Rn flux of groundwater inflow is higher,and the runoff intensity is greater,which is the main groundwater recharge area for the lake.The estimated groundwater recharge in 2021 was 3017×10^(4) m^(3),which was 57%of the total recharge to the lake,or 1.6 times and 8.1 times that of precipitation and surface runoff.The TN and TP contents in Daihai have been rising continuously,and the average TN and TP concentrations in the lake water in 2021 were 4.21 mg·L^(−1) and 0.12 mg·L^(−1),respectively.The TN and TP contents entering the lake with groundwater recharge were 6.8 times and 8.7 times above those of runoff,accounting for 87%and 90%of the total input,respectively.The calculation results showed that groundwater is not only the main source of recharge for Daihai,but also the main source of exogenous nutrients.In recent years,the pressurized exploitation of groundwater in the basin is beneficial in increasing the groundwater recharge to the lake,reducing the water balance difference of the lake,and slowing down the shrinking degree of the lake surface.However,under the action of high evaporation,nitrogen and phosphorus brought by groundwater recharge would become more concentrated in the lake,leading to a continuous increase in the content of nutrients and degree of eutrophication.Therefore,the impact of changes in regional groundwater quantity and quality on Daihai is an important issue that needs further assessment. 展开更多
关键词 Groundwater recharge Radon isotopes nitrogen and phosphorus pollution Ecological environment Daihai
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Water Environment Improvement of Zhongdong River by Water Diversion and Distribution in Hangzhou
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作者 Wang Yan Duan Xuejun +1 位作者 Yang Lei Zhang Xiaohong 《Meteorological and Environmental Research》 CAS 2017年第1期61-66,共6页
As the development of city economy,Zhongdong River in Hangzhou was seriously polluted,with the worst water quality.In order to obtain the effect of water diversion and distribution from Qiantang River on the water qua... As the development of city economy,Zhongdong River in Hangzhou was seriously polluted,with the worst water quality.In order to obtain the effect of water diversion and distribution from Qiantang River on the water quality of Zhongdong River,7-year continuous monitoring was conducted,which was at the fixed stations before and after the water diversion and distribution.After the water diversion project,the dissolved oxygen concentration of the river water was one to two times higher than before,and the ammonia nitrogen and total phosphorus decreased by 60%and 65%,respectively.When increased the amount of water diversion,the dissolved oxygen concentration of the river water elevated by 13%,and the ammonia nitrogen,total phosphorus and potassium permanganate index decreased by 8%,3%and 14%,respectively.The reason for the river water pollution was contributed to the combined sewer system and riverway sludge,especially during the rainfall,the dissolved oxygen concentration of Zhongdong River sharply declined by 95%,while the ammonia nitrogen and total phosphorus increased by 90%and 87%,respectively.The research results could provide theoretic basis for sustainable improvement of Zhongdong River water quality and river management department making the related regulations and policies. 展开更多
关键词 Dissolved oxygen AMMONIA nitrogen Total phosphorus POTASSIUM PERMANGANATE index ENDOGENOUS and EXOGENOUS pollution China
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Spatio-Temporal Distribution of Agricultural Non-Point Source Pollution in Binzhou City Based on Large Computer Data
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作者 Xiaodan FEI Kun RONG Yong LI 《Asian Agricultural Research》 2017年第3期61-63,共3页
Based on the relevant statistics on the agricultural non-point source pollution in Binzhou City,we studied the spatio-temporal variation in agricultural non-point source nitrogen pollution and phosphorus pollution in ... Based on the relevant statistics on the agricultural non-point source pollution in Binzhou City,we studied the spatio-temporal variation in agricultural non-point source nitrogen pollution and phosphorus pollution in Binzhou City during 2008-2015. The results showed that the agricultural non-point source nitrogen pollution and phosphorus pollution in Binzhou City changed from 114400 t and 28800 t in 2008 to110600 t and 24400 t in 2015,respectively; for the non-point source nitrogen pollution sources,the proportion of chemical fertilizer,manure and domestic sewage changed from 80. 41%,10. 47% and 9. 13% in 2008 to 82. 94%,4. 77% and 12. 29% in 2015,respectively; for the non-point source phosphorus pollution sources,the proportion of chemical fertilizer,manure and domestic sewage changed from 89. 29%,8. 32% and 2. 39% in 2008 to 91. 6%,4. 78% and 3. 62% in 2015,respectively; in 2015,the non-point source nitrogen pollution was most serious in Wudi County and Huimin County and least serious in Zhanhua County; the non-point source phosphorus pollution was most serious in Zouping County and least serious in Wudi County. 展开更多
关键词 Non-point source pollution nitrogen phosphorus Spatio-temporal distribution Binzhou City
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Eutrophication Evaluation of Water Body at Huailai Section of the Yongding River 被引量:3
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作者 Zhao Jianguo Li Hongbo +4 位作者 Liu Cunqi Li Xiaoyu Chen Xinyong Yan Donghua Luo Ning 《Meteorological and Environmental Research》 CAS 2018年第6期66-72,78,共8页
In order to understand the water pollution characteristics in Huailai section of the Yongding River,the monitoring from November of 2016 to October of 2017 was conducted. 6 sampling points were selected for monitoring... In order to understand the water pollution characteristics in Huailai section of the Yongding River,the monitoring from November of 2016 to October of 2017 was conducted. 6 sampling points were selected for monitoring 6 indicators,and the temporal-spatial variation characteristics of nitrogen and phosphorus in the river were explored. Moreover,the ratio of nitrogen to phosphorus and an exponential universal formula of power function in logarithmic form were used to analyze temporal-spatial variation rules of nitrogen and phosphorus in water,assess the degree of eutrophication,and analyze eutrophication risk. The results showed that water pollution in Huailai section of the Yongding River was more serious. TN was13. 25 times of concentration limit of class III water in the dividing of surface water environment function area in the " 13 thFive-year" Development Planning" of National Environmental Protection Standard. ON and NO-3-N were the main forms of TN,while mean value of TP was 0. 64 mg/L,and each index had the characteristics of agricultural non-point source pollution. The temporal-spatial distribution characteristics of nitrogen and phosphorus in the water body was obvious. At the time scale,the concentrations of nitrogen and phosphorus in the water body showed seasonal variation; at the space scale,the distribution of nitrogen and phosphorus in the water body was similar. The annual average ratio of nitrogen and phosphorus in Huailai section of the Yongding River was 32. 78,and the phytoplankton was in the overall state of phosphorus limitation. During the flat water period,phosphorus was the limiting nutrient element,and the ratio of nitrogen and phosphorus in the dry period and the abundant water period was suitable for the growth and reproduction of algae. The temporal-spatial variation of water body in Huailai section of the Yongding River was mostly in the " eutrophication" stage. The maximum EI value was 228. 11 in dry season,and the lowest was 213. 06 in flood season,while it was218. 30 in flat water period. The fluvial dynamics process in Huailai section of the Yongding River was good,and the flow pattern of the river was continuous. The flow velocity of the main stream was 0. 43-1. 45 m/s,which was much larger than that of the algal bloom. The risk of cyanobacteria blooms in the main stream was low. 展开更多
关键词 The Yongding River nitrogen phosphorus EUTROPHICATION risk assessment
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Research on the Non-Point Pollution Loads in the Lake Uluabat Basin
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作者 Aslihan Katip Feza Karaer 《Journal of Environmental Protection》 2013年第7期29-37,共9页
Lake Uluabat, having an international significance and subject to the Ramsar Convention, is fed by the basin of Mustafakemalpasa Stream which runs through fertile lands utilized for livestock breeding and agriculture.... Lake Uluabat, having an international significance and subject to the Ramsar Convention, is fed by the basin of Mustafakemalpasa Stream which runs through fertile lands utilized for livestock breeding and agriculture. In this study, total amount of nitrogen (TN) and phosphorus (TP) loads of non-point pollutants (agriculture, livestock breeding, vegetation, surface runoff and small settlements) was calculated. It was found out that most intensive pollution load stemmed from livestock breeding which causes dispersion of 13653.57 tons·year-1 of TN and 3224.45 tons·year-1 of TP into the Lake Uluabat. Additionally, seasonal changes in concentration of TN and TP were observed during the period of 2008-2009 in Lake Uluabat. It was concluded that the rise of agricultural activities in summer months was the reason underlying the increase in pollution during the months in question. 展开更多
关键词 Lake Uluabat Basin nitrogen Non-Point pollution Loads phosphorus Transport Coefficients
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天津与上海35岁以上人群氮氧化物个体暴露水平及其影响因素
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作者 庞博 郭桐君 +13 位作者 陈曦 郭华棋 石嘉章 陈娟 王欣梅 李耀妍 单安琪 余恒意 黄婧 汤乃军 王艳 郭新彪 李国星 吴少伟 《北京大学学报(医学版)》 CAS CSCD 北大核心 2024年第4期700-707,共8页
目的:对天津和上海35岁以上人群氮氧化物(nitrogen oxides,NO_(X))与二氧化氮(nitrogen dioxide,NO_(2))个体暴露水平进行测量,并探讨研究对象基线特征、居住环境情况及日常活动模式等因素对其影响。方法:采用定组研究,在天津和上海招... 目的:对天津和上海35岁以上人群氮氧化物(nitrogen oxides,NO_(X))与二氧化氮(nitrogen dioxide,NO_(2))个体暴露水平进行测量,并探讨研究对象基线特征、居住环境情况及日常活动模式等因素对其影响。方法:采用定组研究,在天津和上海招募91名年龄35岁以上的研究对象,分别在夏季和冬季各进行3次随访(上海冬季因新型冠状病毒肺炎疫情影响只进行了1次随访),每两次随访之间间隔至少为2个星期,有27名研究对象参与了两个季节的研究。每次随访使用Ogawa被动式采样器测量个体24 h NO_(X)与NO_(2)暴露浓度,通过问卷和日志收集日常活动模式信息。采用混合线性效应模型分析不同因素对NO_(X)与NO_(2)个体暴露水平的影响。结果:两地人群共完成349人次有效的24 h内NO_(2)与NO_(X)个体暴露监测,天津夏季NO_(2)与NO_(X)个体暴露日均值(体积分数)分别为18.0×10^(-9)和26.2×10^(-9),天津冬季分别为31.0×10^(-9)和54.9×10^(-9),上海夏季分别为38.7×10^(-9)和100.0×10^(-9),上海冬季分别为45.5×10^(-9)和139.2×10^(-9)。单因素回归分析结果显示NO_(X)与NO_(2)个体暴露水平与城市、季节、性别、日均做饭次数以及监测站大气NO_(2)浓度显著相关。除以上因素外,NO_(X)个体暴露水平还与教育水平有显著关联,NO_(2)个体暴露水平还与是否被动吸烟、日均居家时间、烹饪燃料类型、住宅与交通主干道距离、是否使用抽油烟机存在显著关联。多因素回归分析显示,NO_(2)与NO_(X)个体暴露水平天津显著低于上海,夏季显著低于冬季,男性NO_(X)个体暴露水平显著高于女性。监测站NO_(2)浓度与NO_(2)和NO_(X)个体暴露水平呈显著正向关联;日均做饭次数与NO_(2)个体暴露水平之间呈显著正向关联,日均居家时间与NO_(2)个体暴露水平之间呈显著负向关联。大气NO_(2)浓度每升高1个四分位间距(interquartile range,IQR),即12.7×10^(-9),NO_(2)个体暴露水平上升27.5%[95%置信区间(confidence interval,CI):17.0%~38.9%],NO_(X)个体暴露水平上升16.1%(95%CI:7.1%~25.8%)。结论:不同季节、城市和大气NO_(2)浓度均可以影响NO_(2)与NO_(X)的个体暴露水平,同时NO_(2)个体暴露水平还受到生活习惯等因素的影响。 展开更多
关键词 空气污染 氮氧化物 个体暴露 危险因素
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黄河流域农业农村氮流时空分布特征及演化规律研究 被引量:1
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作者 张弼 庞爱萍 李春晖 《环境科学研究》 CSCD 北大核心 2024年第1期80-91,共12页
氮磷等营养元素过剩引发的面源污染问题,是黄河流域水质恶化的重要原因.为应对黄河流域氮素危机,从源头上降低面源污染负荷,本研究基于物质流和空间分析方法,刻画1949-2022年间黄河流域农业农村氮流时空格局演化规律,评估黄河流域面源... 氮磷等营养元素过剩引发的面源污染问题,是黄河流域水质恶化的重要原因.为应对黄河流域氮素危机,从源头上降低面源污染负荷,本研究基于物质流和空间分析方法,刻画1949-2022年间黄河流域农业农村氮流时空格局演化规律,评估黄河流域面源污染关键氮流和高风险区.结果表明:(1)新中国成立以来,黄河流域的作物收获量整体呈现上升的趋势,2015年之后在氮输入水平持续下降的情况下,仍然能够保持年均2%的增长,黄河流域在氮素利用水平上得到了极大的提升.(2)黄河流域农业农村依然存在严重的氮流失现象,其中存贮和反硝化是氮流失的主要部分,1962年、1992年和2022年这两部分流失量分别占耕地氮输出流的51%、47%和36%.2015开始氮素流失(存储)量逐年下降,2022年比2015年减少了15.55%,但是每年仍有30.12×10^(8)kg氮素流失到大气、水体和土壤中,是当年作物收获氮量的1.64倍,氮素损失率高达62.05%.(3)降雨和地势地形是影响氮径流的决定因素,在高风险区内约有27%~45%的氮剩余流失到附近的地表水中,主要分布在甘肃省的最南部和东南角部分地区、陕西省的最南部和山东省东部地区.研究显示:黄河流域在氮素利用提升和氮污染治理方面取得一定成效,但是仍然存在严重的氮流失现象;需要持续推进化肥减量、粪便还田和农村污水治理,同时需要在高风险区采取构建缓冲带等工程措施,才能实现面源污染等氮危机的有效控制. 展开更多
关键词 黄河流域 农业农村污染 氮流路径 时空分布 高风险区
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河南省氮素农业面源污染风险评价与关键管控区识别 被引量:1
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作者 高林林 吴用 +3 位作者 杨书涵 刘雪珂 李玲 李栋浩 《农业机械学报》 EI CAS CSCD 北大核心 2024年第3期311-320,共10页
农业面源污染是我国水环境保护面临的重要问题,风险评价对于农业面源污染防治具有重要意义。本研究以河南省为研究区域,采用层次分析法的分级赋值方法,基于熵值法和专家打分确定各影响因子权重,构建河南省氮素农业面源污染风险多因子综... 农业面源污染是我国水环境保护面临的重要问题,风险评价对于农业面源污染防治具有重要意义。本研究以河南省为研究区域,采用层次分析法的分级赋值方法,基于熵值法和专家打分确定各影响因子权重,构建河南省氮素农业面源污染风险多因子综合评价模型,计算河南省氮素农业面源污染风险指数并在流域尺度上进行验证,划分氮素农业面源污染的风险等级并识别关键管控区。结果表明:种植源、养殖源和生活源分别贡献河南省31.52%、38.47%和30.01%的氮素流失负荷,流失负荷呈现为西低,中、东部高的特点。河南省有39 429 km^(2)的区域存在中风险,约占河南省总面积的23.61%,有17 318 km^(2)的区域存在高风险,约占总面积的10.37%;划定距河流2 km以内的中、高风险区为一般管控区和重点管控区,面积分别为10 982 km^(2)和9 285 km^(2)。通过与同期水质自动监测数据进行相关分析,决定系数为0.82,表明模型模拟结果具有较高的精准度。综合结果表明,建立的多因子综合评价模型具有科学性和准确性,可用于氮素农业面源污染风险的识别。 展开更多
关键词 氮素农业面源污染 多因子综合评价 风险识别 管控区 河南省
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丹江口水库氮磷时空分布特征及水质安全保障对策
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作者 余启辉 林莉 +1 位作者 金海洋 陈力 《中国水利》 2024年第20期59-66,共8页
为加强丹江口水库及其上游流域水质安全保障,基于丹江口水库32个水质监测断面2017—2023年监测数据,分析丹江口水库水质及关键指标总氮和总磷的时空分布特征,核算水库氮磷的不同来源及贡献,评估水库富营养化及水华风险。结果表明:丹江... 为加强丹江口水库及其上游流域水质安全保障,基于丹江口水库32个水质监测断面2017—2023年监测数据,分析丹江口水库水质及关键指标总氮和总磷的时空分布特征,核算水库氮磷的不同来源及贡献,评估水库富营养化及水华风险。结果表明:丹江口水库水质总体良好,以Ⅰ~Ⅱ类为主,总磷浓度基本保持稳定,总氮浓度波动上升;湖北库区总磷和总氮浓度高于河南库区,上游至下游呈降低趋势;2021年汛期出现持续强降雨,总磷和总氮浓度明显升高。入库河流水质稳定向好,Ⅰ~Ⅲ类占比逐渐上升,总磷和总氮浓度下降并趋于稳定;氮磷来源以上游流域污染输入为主,消落区淹没释放次之,沉积物释放影响较小;丹江口水库总体呈中营养状态,但部分水域在特定季节呈现富营养化,支流回水区和库湾水华时有发生,富营养化及水华风险不容忽视。建议加强库区上游流域污染源治理,严格消落区管理,提高水质监测预警能力,深化水质安全保障科学研究,加强体制机制建设。 展开更多
关键词 丹江口水库 氮磷浓度 污染负荷 水质风险 富营养化
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生活垃圾填埋场内及周边地下水中氨氮污染多方法预测
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作者 王硕 熊超 韩小宾 《环境保护科学》 CAS 2024年第5期170-174,共5页
文章采用污染评价法、健康风险评估法和地下水模拟污染预测法,共同探讨了某典型填埋场及周边地区的地下水氨氮污染特性及其对周边环境的影响。研究发现,填埋场中的地下水样品存在氨氮超标的问题,并且超标情况已扩散至填埋场边界以外的... 文章采用污染评价法、健康风险评估法和地下水模拟污染预测法,共同探讨了某典型填埋场及周边地区的地下水氨氮污染特性及其对周边环境的影响。研究发现,填埋场中的地下水样品存在氨氮超标的问题,并且超标情况已扩散至填埋场边界以外的地区。通过污染评价法和健康风险评估法对调查目标污染程度和对人体健康的风险进行了评估,结果显示氨氮污染的风险水平较低且可接受。模拟预测表明,污染物在地下水中的迁移速度较慢,超过5年后的预测结果显示污染物的高浓度区域将逐渐减小。根据研究结果,在污染物迁移方向设置抽水井以控制污染扩散。 展开更多
关键词 填埋场 地下水 氨氮污染 污染评价 健康风险评估
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DITCHES AND PONDS CAN BE THE SOURCES OR SINKS OF NON-POINT SOURCE POLLUTION:OBSERVATIONS IN AN UPLAND AREA IN THE JINGLINXI CATCHMENT,CHINA
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作者 Yiwen WANG Lei CHEN +3 位作者 Kaihang ZHU Chenxi GUO Yu PU ZhenyaoSHEN 《Frontiers of Agricultural Science and Engineering》 CSCD 2023年第4期607-626,共20页
As the common features of agroecosystems,ditches and ponds benefit the irrigation and drainage,as well as intercepting non-point source pollutants.However,most ditch-pond studies have been conducted in lowland areas.T... As the common features of agroecosystems,ditches and ponds benefit the irrigation and drainage,as well as intercepting non-point source pollutants.However,most ditch-pond studies have been conducted in lowland areas.To test this source-sink assumption in upland areas,this study made observations on the ecological function of the ditch and pond system in a typical catchment in China.First,the changes in ponds in the catchment were analyzed using high-resolution remote sensing data.Then,the migration of agricultural pollutants in ditches and ponds were analyzed by field sampling and laboratory detection.The results showed that over the past 15 years the length of ditches in the catchment and the number of small ponds(<500 m2)have increased by 32%and 75%,respectively.The rate of change in nutrient concentrations in the ditches and ponds were mostly from-20%to 20%,indicating ditches and ponds can be both sources and sinks for agricultural pollutants.Lastly,the contributing factors were explored and it was found that ditches and ponds are important sinks in dry season.However,during the rainy season,ditches and ponds become sources of pollutants,with the rapid drainage of ditches and the overflow of ponds in upland areas.The results of this study revealed that the ditches and ponds could be used for ecological engineering in upland catchments to balance drainage and intercept pollutants. 展开更多
关键词 DITCHES PONDS non-point source pollution mountainous areas nitrogen phosphorus
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烟气脱硝系统还原剂由尿素代替液氨环境影响论证分析
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作者 韦宏雷 《大众科学》 2024年第5期55-57,共3页
火电厂烟气脱硝系统主要以液氨作为还原剂,液氨属于有毒气体,且易液化,与空气或氧气混合后会形成爆炸性混合物。随着国家对安全和环境保护的日益重视,烟气脱硝系统还原剂由尿素代替液氨已成为趋势,尿素替代液氨工艺已经成熟,受到许多氮... 火电厂烟气脱硝系统主要以液氨作为还原剂,液氨属于有毒气体,且易液化,与空气或氧气混合后会形成爆炸性混合物。随着国家对安全和环境保护的日益重视,烟气脱硝系统还原剂由尿素代替液氨已成为趋势,尿素替代液氨工艺已经成熟,受到许多氮氧化物产生量大的企业的青睐,不仅可大大降低企业的安全隐患,保障工作人员生命和企业财产安全,还可以降低环境污染风险。 展开更多
关键词 液氨 还原剂 氮氧化物 脱硝 环境污染 环境风险
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