Near-infrared H_(2)O_(2)production via dual pathways of O_(2)reduction and H_(2)O oxidation

Hydrogen peroxide(H_(2)O_(2))is a chemical that is widely of interest in both environmental and energy fields.On the one hand,as a clean oxidant,H_(2)O_(2)has been commonly used in the field of bleaching,disinfection,and advanced oxidation processes.On the other hand,H_(2)O_(2)has also been explored as a liquid fuel alternative to H_(2)or fossil fuels in fuel cells due to its high energy density.However,the current industrial production of H_(2)O_(2)relies on the anthraquinone(AO)method that involves palladium-catalyzed hydrogenation-oxidation steps.

DYNAMIC MODELING FOR AIRSHIP EQUIPPED WITH BALLONETS AND BALLAST

Total dynamics of an airship is modeled. The body of an airship is taken as a submerged rigid body with neutral buoyancy, i. e. , buoyancy with value equal to that of gravity, and the coupled dynamics between the body with ballonets and ballast is considered. The total dynamics of the airship is firstly derived by Newton-Euler laws and Kirchhoff＇ s equations. Furthermore, by using Hamiltonian and Lagrangian semidirect product reduction theories, the dynamics is formulated as a Lie-Poisson system, or also an Euler-Poincare system. These two formulations can be exploited for the control design using energy-based methods for Hamiltonian or Lagrangian system.

The Role of Forced Oscillators of Coupled Circuits in Radiation Physics: New Linear Accelerator Design Improving Tomo-Scanning Technology (Radiotherapy and CT), Heisenberg-Euler Scatter, and Extension to Bremsstrahlung with GeV Electrons

The quantization of circuits has received to be rather attractive in domains of solid state—molecular—and biophysics, since the quanta referred to as Q-bits play a significant role in the design of the quantum computer and entangled structures. Quantized circuits cannot be applied without modifications, since the energy differences are not equidistant and the polarization of the excited states has to be accounted for having particular importance for the creation of virtual states. Applications of the presented theory are scanning methods in radiotherapy without multi-leaf collimators, which may be realized in tomo-scanning radiotherapy and in the keV domain, which provides a new design of CT. The problem of lateral scatter in the target and energy storage by heat production is significantly reduced by a multilayer system with focusing the impinging electrons at the walls and by a magnetic field. The verification of the Heisenberg-Euler scatter of crossing beams of 9 MV is a central problem of photon physics and can be solved by the new bremsstrahlung technique. A comparison with GEANT 4 Monte-Carlo data indicates that the presented method also works in the GeV domain, and a multi-target can improve the bremsstrahlung yield. GEANT 4 provides the spatial distribution, whereas the virtual oscillator states only show the created energy spectrum. In every case, the exploitation yield can be drastically improved by the superiority of the focused multitarget system compared to a single standard target, and the door to new technologies is opened.

Effects of operating conditions on iron(hydr)oxides evolution and ciprofloxacin degradation in potassium ferrate-ozone stepwise oxidation system

In this study,a stepwise oxidation system of potassium ferrate(K_(2)FeO_(4))combined with ozone(O+3)was used to degrade ciprofloxacin(CIP).The effects of pH and pre-oxidation time of K_(2)FeO_(4) on the evolution of K_(2)FeO_(4) reduction products(iron(hydr)oxides)and CIP degradation were investigated.It was found that in addition to its own oxidation capacity,K_(2)FeO_(4) can also influence the treatment effect of CIP by changing the catalyst content.The presence of iron(hydr)oxides effectively enhanced the mineralization rate of CIP by catalyzing ozonation.The pH value can influence the content and types of the components with catalytic ozonation effect in iron(hydr)oxides.The K_(2)FeO_(4) pre-oxidation stage can produce more iron(hydr)oxides with catalytic components for subsequent ozonation,but the evolution of iron(hydr)oxides components was influenced by O_(3) treatment.It can also avoid the waste of oxidation capacity owing to the oxidation of iron(hydr)oxides by O_(3) and free radicals.The intermediate degradation products were identified by Fourier transform ion cyclotron resonance mass spectrometry(FT-ICR-MS).Besides,the degradation pathways were proposed.Among the degradation products of CIP,the product with broken quinolone ring structure only appeared in the stepwise oxidation system.

Recovery of boron from high-boron iron concentrate using reduction roasting and magnetic separation

The comprehensive utilization of abundant high-boron iron concentrate is of particular significance to Chi- na, and the high-boron iron concentrate has not yet been utilized as a source for boron at an industrial scale due to its complex mineralogy and fine mineral dissemination. An innovative method was proposed for recovery of boron and iron from high-boron iron concentrate by reduction roasting and magnetic sepa- ration. The effects of reduction temperature and roasting time were investigated and their optimum condi- tions were determined. The mineralogical changes during roasting were characterized by X-ray diffraction （XRD） and scanning electron microscopy （SEM）. The results showed that the pyrrhotite （FeS） contained in the high-boron iron concentrate and the new-formed FeS-Fe solid solution softened or melted at high temperatures owing to their low melting points, and then decreased the metallic iron ratio and accelerated the growth of metallic iron particles. Meanwhile, the magnetite and szaibelyite were converted into metal- lic iron and suanite, respectively. Consequently, boron was readily enriched into the non-magnetic product and the metallic iron was aggregated to the magnetic concentrate by magnetic separation. Boron recovery of 88.6% with corresponding B2O3 content of 14.5% and iron recovery of 95.1% with an iron grade of 92.7% were achieved when high-boron iron concentrate was reduced at 1 125℃ for 150 min. Besides, the boron reactivity of the boron-rich non-magnetic product was up to 80.8%.

0D/3D direct Z-scheme heterojunctions hybridizing by MoS2 quantum dots and honeycomb conjugated triazine polymers (CTPs) for enhanced photocatalytic performance

Herein,a novel direct Z-scheme photocatalyst was accomplished by hybridization of 0D MoS2 quantum dots(MSQDs)and 3D honeycomb-like conjugated triazine polymers(CTP)(namely,CTP-MSQD).The unique 0D/3D hierarchical structure significantly enhanced the exposure of active sites and light harvesting property,while the formed p-n junction enabled the direct strong interface coupling without the necessity of any mediators.The optimized CTP-MSQD3 exhibited continuously increased visible-light-driven photocatalytic activity and strong durability both in Cr(VI)reduction and H2 evolution,featured a rate of 0.069 min^(-1) and 1070μmol/(hr•g),respectively,which were 8 times than those of pure 3D-CTP(0.009 min^(−1) and 129μmol/(hr•g)).We believe that this work provides a promising photocatalyst system that combines a 0D/3D hierarchical structure and a Z-scheme charge flow for efficient and stable photocatalytic conversion.

An Elastic Architecture Adaptable to Various Application Scenarios

The quantity of computer applications is increasing dramatically as the computer industry prospers. Meanwhile, even for one application, it has different requirements of performance and power in different scenarios. Although various processors with different architectures emerge to fit for the various applications in different scenarios, it is impossible to design a dedicated processor to meet all the requirements. Furthermore, dealing with uncertain processors significantly aggravates the burden of programmers and system integrators to achieve specific performance/power. In this paper, we propose elastic architecture （EA） to provide a uniform computing platform with high elasticity, i.e., the ratio of worst-case to best-case performance/power/performance-power trade-off, which can meet different requirements for different applications. It is achieved by dynamically adjusting architecture parameters （instruction set, branch predictor, data path, memory hierarchy, concurrency, status^zcontrol, and so on） on demand. The elasticity of our prototype implementation of EA, as Sim-EA, ranges from 3.31 to 14.34, with 5.41 in arithmetic average, for SPEC CPU2000 benchmark suites, which provides great flexibility to fulfill the different performance and power requirements in different scenarios. Moreover, Sim-EA can reduce the EDP （energy-delay product） for 31.14% in arithmetic average compared with a baseline fixed architecture. Besides, some subsequent experiments indicate a negative correlation between application intervals＇ lengths and their elasticities.