Optimal and robust control of population transfer in asymmetric quantum-dot molecules

We present an optimal and robust quantum control method for efficient population transfer in asymmetric double quantum-dot molecules.We derive a long-duration control scheme that allows for highly efficient population transfer by accurately controlling the amplitude of a narrow-bandwidth pulse.To overcome fluctuations in control field parameters,we employ a frequency-domain quantum optimal control theory method to optimize the spectral phase of a single pulse with broad bandwidth while preserving the spectral amplitude.It is shown that this spectral-phase-only optimization approach can successfully identify robust and optimal control fields,leading to efficient population transfer to the target state while concurrently suppressing population transfer to undesired states.The method demonstrates resilience to fluctuations in control field parameters,making it a promising approach for reliable and efficient population transfer in practical applications.

Enhancing performance of inverted quantum-dot light-emitting diodes based on a solution-processed hole transport layer via ligand treatment

The performance of inverted quantum-dot light-emitting diodes(QLEDs)based on solution-processed hole transport layers(HTLs)has been limited by the solvent-induced damage to the quantum dot(QD)layer during the spin-coating of the HTL.The lack of compatibility between the HTL’s solvent and the QD layer results in an uneven surface,which negatively impacts the overall device performance.In this work,we develop a novel method to solve this problem by modifying the QD film with 1,8-diaminooctane to improve the resistance of the QD layer for the HTL’s solvent.The uniform QD layer leads the inverted red QLED device to achieve a low turn-on voltage of 1.8 V,a high maximum luminance of 105500 cd/m2,and a remarkable maximum external quantum efficiency of 13.34%.This approach releases the considerable potential of HTL materials selection and offers a promising avenue for the development of high-performance inverted QLEDs.

Analytical method for cell displacement defect quantum-dot cellular automata primitive

Quantum-dot cellular automata(QCA)is an emerging computational paradigm which can overcome scaling limitations of the existing complementary metal oxide semiconductor(CMOS)technology.The existence of defects cannot be ignored,considering the fabrication of QCA devices at the molecular level where it could alter the functionality.Therefore,defects in QCA devices need to be analyzed.So far,the simulation-based displacement defect analysis has been presented in the literature,which results in an increased demand in the corresponding mathematical model.In this paper,the displacement defect analysis of the QCA main primitive,majority voter(MV),is presented and carried out both in simulation and mathematics,where the kink energy based mathematical model is applied.The results demonstrate that this model is valid for the displacement defect in QCA MV.

Wide color gamut switchable autostereoscopic 3D display based on directional quantum-dot backlight

A switchable autostereoscopic 3-dimensional(3D) display device with wide color gamut is introduced in this paper. In conjunction with a novel directional quantum-dot(QD) backlight, the precise scanning control strategy, and the eye-tracking system, this spatial-sequential solution enables our autostereoscopic display to combine all the advantages of full resolution,wide color gamut, low crosstalk, and switchable 2D/3D. And also, we fabricated an autostereoscopic display prototype and demonstrated its performances effectively. The results indicate that our system can both break the limitation of viewing position and provide high-quality 3D images. We present two working modes in this system. In the spatial-sequential mode,the crosstalk is about 6%. In the time-multiplexed mode, the viewer should wear auxiliary and the crosstalk is about 1%,just next to that of a commercial 3D display(BENQ XL2707-B and View Sonic VX2268 WM). Additionally, our system is also completely compatible with active shutter glasses and its 3D resolution is same as its 2D resolution. Because of the excellent properties of the QD material, the color gamut can be widely extended to 77.98% according to the ITU-R recommendation BT.2020(Rec.2020).

Broadband chirped InAs quantum-dot superluminescent diodes with a small spectral dip of 0.2 dB

We report on the fabrication and characterization of InAs/GaAs chirped multilayer quantum-dot superluminescent diodes(CMQD-SLDs)with and without direct Si doping in QDs.It was found that both the output power and the spectral width of the CMQD-SLDs were significantly enhanced by direct Si doping in the QDs.The output power and spectral width have been increased by approximately 18.3%and 40%,respectively.Moreover,we shortened the cavity length of the doped CMQD-SLD and obtained a spectral width of 106 nm.In addition,the maximum output power and spectral width of the CMQD-SLD doped directly with Si can be further increased to 16.6 mW and 114 nm,respectively,through anti-reflection coating and device packaging.The device exhibited the smallest spectral dip of 0.2 dB when the spectrum was widest.The improved performances of the doped CMQD-SLD can be attributed to the direct doping of Si in the QDs,optimization of device structure and device packaging.

Quantum-dot Semiconductor Optical Amplifiers in State Space Model

A state space model(SSM) is derived for quantum-dot semiconductor optical amplifiers(QD-SOAs).Rate equations of QD-SOA are formulated in the form of state update equations,where average occupation probabilities along QD-SOA cavity are considered as state variables of the system.Simulations show that SSM calculates QD-SOA′s static and dynamic characteristics with high accuracy.

Phase Control of Transient Optical Properties of Double Coupled Quantum-Dot Nanostructure via Gaussian Laser Beams

We theoretically analyze the transient properties of a probe field absorption and dispersion in a coupled semiconductor double-quantum-dot nanostructure.We show that in the presence of the Gaussian laser beams,absorption and dispersion of the probe field can be dramatically influenced by the relative phase between applied fields and intensity of the Gaussian laser beams.Transient and steady-state behaviors of the probe field absorption and dispersion are discussed to estimate the required switching time.The estimated range is between 5-8 ps for subluminal to superluminal light propagation.

Effect of Intra-Dot Coulomb Interaction on Andreev Reflection in Normal-Metal/Quantum-Dot/Superconductor System

We investigate the effect of intra-dot Coulomb interaction on the Andreev reflection in a normalmetal/quantum-dot/superconductor (N-QD-S) system with multiple levels in the quantum dot, in the regime where the intra-dot interacting constant is comparable to the energy gap of superconducting lead. By using nonequilibrium Green function method, the averaged occupation of electrons in the quantum dot and the Andreev reflection (AR) current are studied. Comparing to the case of non-interacting quantum dot, the system shows significant changes for the a two-step-like behavior; and the I-Vg shows two groups of peaks, separated by U and with equal heights, where Vg is the gate voltage and U denotes the intra-dot Coulomb interaction constant. (ii) For finite bias voltage, dips, superposed V ≥ U/2, extra AR current peaks occur between the two groups of the peaks. Besides, the properties of the heights of the AR current peaks are more complicated.

Quantum-Dot Spin-Based Secret Sharing in an Optical Microcavity

Two schemes of quantum secret sharing are proposed via single electron spin confined in charged QDs inside a single-sided microcavity and a double-sided microcavity, respectively. Both schemes rely on coherent photonspin interaction. The two schemes axe both deterministic and can be extended to multipartite secret sharing.

Andreev Tunneling Through a Ferromagnet/Quantum-Dot/Superconductor System

We study Andreev tunneling through a ferromagnet/quantum-dot (QD)/superconductor system. By usingnonequilibrum Green function method, the averaged occupation of electrons in QD and the Andreev tunneling currentare studied. Comparing to the norma-metal/quantum-dot/superconductor, the system shows significant changes: (i)The averaged occupations of spin-up and spin-down electrons are not equal. (ii) With the increase of the polarizationof ferromagnetic lead, the Andreev reflection current decreases. (iii) However, even the ferromagnetic lead reaches fullpolarization, the averaged occupation of spin-down electrons is not zero. The physics of these changes is discussed.

Analytical Result on the Supercurrent Through a Superconductor/Quantum-Dot/Superconductor Junction

We present an analytical result for the supercurrent across a superconductor/quantum-dot/superconductor junction. By converting the current integration into a special contour integral, we can express the current as a sum of the residues of poles. These poles are real and give a natural definition of the Andreev bound states. We also use the exact result to explain some features of the supercurrent transport behavior.

A new phenomenon of quantum-dot cellular automata

If an external point charge and the movable charges of an isolated quantum-dot cellular automata (QCA) cell have the same polarity, the point charge greatly affects the polarization (P) of the cell only when it is in a narrow band with periodically changing width. The center of the band is on a radius R circle. The ratio of R to the electric charge (q) is a constant determined by the parameters of the cell. A QCA cell can be used as charge detector based on the above phenomenon.

Single-Bit Comparator in Quantum-Dot Cellular Automata (QCA) Technology Using Novel QCAXNOR Gates

To fill the continuous needs for faster processing elements with less power consumption causes large pressure on the complementary metal oxide semiconductor(CMOS)technology developers.The scaling scenario is not an option nowadays and other technologies need to be investigated.The quantum-dot cellular automata(QCA)technology is one of the important emerging nanotechnologies that have attracted much researchers’attention in recent years.This technology has many interesting features,such as high speed,low power consumption,and small size.These features make it an appropriate alternative to the CMOS technique.This paper suggests three novel structures of XNOR gates in the QCA technology.The presented structures do not follow the conventional approaches to the logic gates design but depend on the inherent capabilities of the new technology.The proposed structures are used as the main building blocks for a single-bit comparator.The resulted circuits are simulated for the verification purpose and then compared with existing counterparts in the literature.The comparison results are encouraging to append the proposed structures to the library of QCA gates.

Junction-Temperature Measurement in InAs/InP(100) Quantum-Dot Lasers

We report on the measurement of junction temperature of the InAs/InP（l00） quantum dot lasers working in the 1.55μm wavelength region. The measurement is based on analyzing the temperature induced mode shift of the Fabry-Perot cavity. Under pulsed operation mode, more than 20℃ junction temperature rise is measured for the quantum-dot （QD） laser when the duty cycle is increased from 1% to 95%. For a reference quantum well laser, the junction temperature rise is obtained as only around 3℃. The large junction temperature rise might be a crucial factor to improve the performance of QD lasers.

Defect and Temperature Effects on Complex Quantum-Dot Cellular Automata Devices

The authors present an analysis of the fault tolerant properties and the effects of temperature on an exclusive OR (XOR) gate and a full adder device implemented using quantum-dot cellular automata (QCA) structures. A Hubbard-type Hamiltonian and the Inter-cellular Hartree approximation have been used for modeling, and a uniform random distribution has been implemented for the simulated dot displacements within cells. We have shown characteristic features of all four possible input configurations for the XOR device. The device performance degrades significantly as the magnitude of defects and the temperature increase. Our results show that the fault-tolerant characteristics of an XOR device are highly dependent on the input configurations. The input signal that travels through the wire crossing (also called a crossover) in the central part of the device weakens the signal significantly. The presence of multiple wire crossings in the full adder design has a major impact on the functionality of the device. Even at absolute zero temperature, the effect of the dot displacement defect is very significant. We have observed that the breakdown characteristic is much more pronounced in the full adder than in any other devices under investigation.

Novel Adder Circuits Based On Quantum-Dot Cellular Automata (QCA)

Quantum-dot cellular automaton (QCA) is a novel nanotechnology that provides a very different computation platform than traditional CMOS, in which polarization of electrons indicates the digital information. This paper demonstrates designing combinational circuits based on quantum-dot cellular automata (QCA) nanotechnology, which offers a way to implement logic and all interconnections with only one homogeneous layer of cells. In this paper, the authors have proposed a novel design of XOR gate. This model proves designing capabilities of combinational circuits that are compatible with QCA gates within nano-scale. Novel adder circuits such as half adders, full adders, which avoid the fore, mentioned noise paths, crossovers by careful clocking organization, have been proposed. Experiment results show that the performance of proposed designs is more efficient than conventional designs. The modular layouts are verified with the freely available QCA Designer tool.

Controllable Tunneling of Light through a Quantum-Dot-Molecule Dielectric Film via Electromagnetically Induced Transparency

Since discrete multilevel transitions of quantum-dot molecules driven by external electromagnetic fields can exhibit quantum coherence effects, such an optical characteristic can be utilized to control propagation of electromagnetic wave through a quantum-dot molecule dielectric film. Since inner-dot tunneling in quantum-dot molecules can be controlled by a gate voltage, destructive quantum coherence among multilevel transitions in quantum-dot molecule would give rise to EIT (electromagnetically induced transparency). In this report, we shall investigate controllable on- and off-resonance tunneling effects of an incident electromagnetic wave through such a quan-tum-dot-molecule dielectric film, of which the optical response is tuned by the switchable gate voltage. We have found from the theoretical mechanism that a high gate voltage can cause the EIT phenomenon of quan-tum-dot-molecule systems, and under the condition of on-resonance light tunneling through the thin film, the probe field will propagation without loss if the probe frequency detuning is zero. By taking advantage of these effects sensitive to the tunable gate voltage, such quantum coherence would be inte-grated in certain photonic structures, and some devices such as photonic switching and transistors can be designed. Transient evolution of optical characteristics in the quantum-dot-molecule dielectric film (once the tunable gate voltage is turned on or off) is also considered in this report.

CdS和Bi_2Se_3量子点共敏化TiO_2光电极用于光解水制氢研究

采用化学气相沉积法将CdS、Bi2Se3量子点沉积在TiO2纳米棒阵列上,组装成光电极,采用XRD对CdS/TiO2、Bi2Se3/TiO2电极进行结构测试,并用SEM、TEM对3个电极进行形貌测试。Na2S/Na2SO3溶液中,测试几个光电极的光解水制氢能力,结果表明:Bi2Se3/CdS/TiO2电极产生的氢气量最大。进一步分析光电极的光电化学性能,得出Bi2Se3/CdS/TiO2电极的光电流是TiO2电极的20倍,是CdS/TiO2、Bi2Se3/TiO2电极的2倍,说明CdS量子点、Bi2Se3量子点共敏化TiO2电极表现出优良的制氢能力。

Recent progress of colloidal quantum dot based solar cells

Colloidal quantum dot （CQD） solar cells have attracted great interest due to their low cost and superior photo-electric properties. Remarkable improvements in cell performances of both quantum dot sensitized solar cells （QDSCs） and FbX （X = S, Se） based CQD solar cells have been achieved in recent years, and the power conversion efficiencies （PCEs） ex- ceeding 12% were reported so far. In this review, we will focus on the recent progress in CQD solar cells. We firstly summarize the advance of CQD sensitizer materials and the strategies for enhancing carrier collection efficiency in QD- SCs, including developing multi-component alloyed CQDs and core-shell structured CQDs, as well as various methods to suppress interfacial carrier recombination. Then, we discuss the device architecture development of PbX CQD based solar cells and surface/interface passivation methods to increase light absorption and carrier extraction efficiencies. Finally, a short summary, challenge, and perspective are given.

Fano versus Kondo Resonances in a Closed Aharonov-Bohm Interferometer Coupled to Ferromagnetic Electrodes

Using the Keldysh nonequilibrium Green function and equation-of-motion technique, we investigate Fano versus Kondo resonances in a closed Aharonov-Bohm interferometer coupled to ferromagnetic leads and study their effects on the conductance of this system. The conductance with both parallel and antiparallel lead-polarization alignments is analysed for various values of the magnetic flux. Our results show that this system can provide an excellent spin filtering property, and a large tunnelling magnetoresistance can arise by adjusting the system parameters, which indicates that this system is a possible candidate for spin valve transistors and has important applications in spintronics.