Full Quantum State Resolved Scattering Dynamics of the F+H_(2)→HF+H Reaction at 5.02 kJ/mol

A crossed molecular beams, state-to-state scattering study was carried out on the F＋H2→HF＋H reaction at the collision energy of 5.02 kJ/mol, using the highly sensitive H atom Rydberg tagging time-of-flight method. All the peaks in the TOF spectra can be clearly assigned to the ro-vibrational structures of the HF product. The forward scattering of the HF product at v′=3 has been observed. The small forward scattering of the HF product at v′=2 has also been detected. Detailed theoretical analysis is required in order to fully understand the dynamical origin of these forward scattering products at this high collision energy.

Study on γ-ray source from the resonant reaction ^19F(p,αγ)^16O at Ep=340 keV

High energyγ-ray can be used in many fields,such as nuclear resonant fluorescence,nuclear medicine imaging.One of the methods to generate high-energyγ-ray is nuclear resonant reaction.The 19F(p,αγ)16O reaction was used to generate 6.13-MeVγ-ray in this work.The angular distribution of 6.13-MeVγ-ray was measured by six LaBr3 detectors.The thick-target yield curve of 6.13-MeVγ-ray had been measured.The maximum yield was determined to be(1.85±0.01)×10^-8γ/proton,which was measured by HPGe detector and LaBr3 detector.The absolute efficiency of all the detectors was calibrated using 60Co and 27Al(p,γ)^28Si reaction at Ep=992 keV.The cross section and total resonant width of the reaction were determined to be 95.1±1.0 mb(1 b=10^-24 cm^2)andΓCM=2.21±0.22 keV,respectively.

Direct measurement of the resonance strengths and branching ratios of low-energy(p,γ)reactions on Mg isotopes

Proton capture reactions on Mg isotopes are significant in the Mg-Al cycle in stellar H-burning.In particular,the resonance strengths and branching ratios of low-energy resonances in 23Mg(p,γ)26Al reactions determine the production of which is one of the most important long-lived radioactive nuclei in nuclear astrophysics.In this article,we report our first experiment using the intense proton beam of approximately 2 mA provided by the JUNA accelerator ground laboratory and a new technique that can minimize the composition change of targets under intense beam irradiation.The resonance strengths and branching ratios of E=214,304,and 326 keV resonances in the reactions of 2~4Mg(p,γ)25Al,25Mg(p,γ)26Al,and 26Mg(p,γ)27Al,respectively,were measured with high accuracy.The success of this experiment provides a good calibration for the nuclear astrophysical experiment at the Jinping underground laboratory.

THE ELECTRON SPIN RESONANCE STUDY ON PRIMARY PHOTOCHEMICAL REACTION OF HEMATOPORPHYRIN DERIVATIVE

The rate of oxygen consumption and the yield of free radical anion of hematoporphyrin derivative (HPD) in aqueous solutions of HPD and pyrocatechol were measured by the probe 2,2,6,6-tetramethyl4-piperidone-1-oxyl.It has been found that both singlet oxygen and free radical mechanisms exist simultaneously in primary photochemical reactions, and there is a competition between both mechanisms. When the oxygen concentration in solutions comes down to 12-14% of the stanting level, the predominant mechanism can be changed from the singlet oxygen to the free radical.Whether HPD exists in aggregation state is very important to photosensitization mechanisms.In the presence of the aggregation state of HPD, the predominant mechanism is the free radical,and photosensitization effects of HPD are all the better.

First result from the Jinping Underground Nuclear Astrophysics experiment JUNA:precise measurement of the 92 keV ^(25)Mg(p,γ)^(26)Al resonance

The ^(25)Mg(p,γ)^(26)Al reaction plays an important role in the study of cosmic 1.809 MeV γ-ray as a signature of ongoing nucleosynthesis in the Galaxy.At astrophysical temperature around 0.1 GK,the ^(25)Mg(p,γ)^(26)Al reaction rates are dominated by the 92 keV resonance capture process.We report a precise measurement of the 92 keV ^(25)Mg(p,γ)^(26)Al resonance in the day-one experiment at Jinping Underground Nuclear Astrophysics experiment(JUNA)facility in the China Jinping Underground Laboratory(CJPL).The resonance strength and ground state feeding factor are determined to be 3.8±0.3×10^(-10) eV and 0:660:04,respectively.The results are in agreement with those reported in the previous direct underground measurement within uncertainty,but with significantly reduced uncertainties.Consequently,we recommend new ^(25)Mg(p,γ)^(26)Al reaction rates which are by a factor of 2.4 larger than those adopted in REACLIB database at the temperature around 0.1 GK.The new results indicate higher production rates of ^(26g)Al and the cosmic 1.809 MeV γ-ray.The implication of the new rates for the understanding of other astrophysical situations is also discussed.