High-performance wearable electronics are highly desirable for the development of body warming and human health monitoring devices.In the present study,high electrically conductive and photothermal cotton yarns(CYs)wi...High-performance wearable electronics are highly desirable for the development of body warming and human health monitoring devices.In the present study,high electrically conductive and photothermal cotton yarns(CYs)with long-term stability were prepared as wearable electronics.The process contains back-to-back decoration of the fiber surface by Ti_(3)C_(2)T_(x)(MXene)nanosheets,and the poly(3,4-ethylenedioxythiophene)polystyrene sulfonate(PEDOT:PSS)composite,to form a core–shell structure(MP@CY).The addition of a small amount of PEDOT:PSS plays a dual role of protecting the MXene from oxidation and increasing the electrical conductivity.The resulting yarn exhibits excellent electrical conductivity(21.8Ωcm^(−1)),rapid electrothermal response,and superb photothermal conversion capability,supporting its application as an optical/electrical dual-drive heater.A three-dimensional(3D)honeycomb-like textile wearable heater based on MP@CY as weft yarn demonstrates outstanding electrical thermal properties(0–2.5 V,30–196.8°C)and exceptional photothermal conversion(130 mW cm^(−2),64.2°C).Using an Internet of Things(IoT)microcontroller and Espressif(ESP)electronics chip,which are combined with wireless fidelity(Wi-Fi)and smartphone,real-time visualization and precise control of the temperature interface can be achieved.Furthermore,MP@CY-based knitted sensors,obtained by hand-knitting,are utilized for monitoring human movement and health,exhibiting high sensitivity and long-term cycling stability.展开更多
Graphene composite yarns have demonstrated significant potential in the development of multifunctional wearable elec-tronics,showcasing exceptional conductivity,mechanical properties,flexibility,and lightweight design...Graphene composite yarns have demonstrated significant potential in the development of multifunctional wearable elec-tronics,showcasing exceptional conductivity,mechanical properties,flexibility,and lightweight design.However,their performance is limited by the weak interfacial interaction between the fibers and graphene.Herein,a polydopamine-reduced graphene oxide(PDA-RGO)interfacial modulation strategy is proposed to prepare graphene-coated cotton yarns with high electrical conductivity and strength.PDA-RGO serves as an interfacial bonding molecule that interacts with the cotton yarn(CY)substrate to establish a hydrogen interface,while interconnecting with highly conductive graphene throughπ-πinterac-tions.The developed interface-designed graphene-coated yarn demonstrates an impressive average electrical conductivity of(856.27±7.02)S/m(i.e.,average resistance of(57.57±5.35)Ω).Simultaneously,the obtained conductive yarn demonstrates an exceptional average tensile strength of(172.03±8.03)MPa,surpassing that of primitive CY by approximately 1.59 times.The conductive yarns can be further used as low-voltage flexible wearable heaters and high-sensitivity pressure sensors,thus showcasing their remarkable potential for high-performance and multifunctional wearable devices in real-world applications.展开更多
Fiber supercapacitors(FSs)based on transition metal oxides(TMOs)have garnered considerable attention as energy stor-age solutions for wearable electronics owing to their exceptional characteristics,including superior ...Fiber supercapacitors(FSs)based on transition metal oxides(TMOs)have garnered considerable attention as energy stor-age solutions for wearable electronics owing to their exceptional characteristics,including superior comfortability and low weights.These materials are known to exhibit high energy densities,high specific capacitances,and fast redox reactions.However,current fabrication methods for these structures primarily rely on chemical deposition,often resulting in undesir-able material structures and necessitating the use of additives,which can degrade the electrochemical performance of such structures.Herein,physically deposited TMO nanoribbon yarns generated via delamination engineering of nanopatterned TMO/metal/TMO trilayer arrays are proposed as potential high-performance FSs.To prepare these arrays,the target materials were initially deposited using a nanoline mold,and subsequently,the nanoribbon was suspended through selective plasma etching to obtain the desired twisted yarn structures.Because of the direct formation of TMOs on Ni electrodes,a high energy/power density and excellent electrochemical stability were achieved in asymmetric FS devices incorporating CoNixOy nanoribbon yarns and graphene fibers.Furthermore,a triboelectric nanogenerator,pressure sensor,and flexible light-emitting diode were synergistically combined with the FS.The integration of wearable electronic components,encompassing energy harvesting,energy storage,and powering sensing/display devices,is promising for the development of future smart textiles.展开更多
Wearable fiber-based lithium-ion batteries(LiBs)made with textile-like functional electrode materials are key to realizing smart energy options for powering wearable electronics.However,the process of attenuating the ...Wearable fiber-based lithium-ion batteries(LiBs)made with textile-like functional electrode materials are key to realizing smart energy options for powering wearable electronics.However,the process of attenuating the existing functional materials commonly used in planar and solid-state batteries to functional fiber or yarn electrodes tends to deteriorate the material performance when assembled into textile-based electrodes.In this work,we focus on understanding and enabling layered Ni-rich cathode material into a wearable cathode yarn.Layered Ni-rich cathode materials typically contain a higher proportion of Ni compared to other metals like Co and Mn,with a Li[Ni_(1−x)M_(x)]O_(2)(M=transition metal element,such as Mn,Al,Co,and so on)typical structure.They are increasingly gaining popularity in the research and development of LiBs as they offer several advantages,including higher energy density,improved cycle life,and reduced cost compared to many commercial cathode materials.Our fabricated flexible Ni-rich cathode yarn with an overall diameter of~360μm and a coating thickness of~80μm exhibited textile properties with promising mechanical strength and the ability to conform to any shape.When tested in a half-cell arrangement with Li metal as the counter electrode,the Ni-rich cathode yarn electrode showed stable cyclic performance with a discharge areal capacity of~3 mAh/cm^(2) and an average coulombic efficiency of 99.5%at a 0.2 mA/cm^(2) current density.Overall,the results show that Ni-rich cathode materials,despite their layered structure,are integrateable into usable wearable textile LiBs.展开更多
The increasing demand for sustainable and environmentally friendly materials has driven research towards the development of green composites.In this work,the flax/polylactic acid(PLA)braided yarns were fabricated by b...The increasing demand for sustainable and environmentally friendly materials has driven research towards the development of green composites.In this work,the flax/polylactic acid(PLA)braided yarns were fabricated by braiding PLA filaments with 4 to 24 spindles on flax yarns.After curing at different temperatures(180℃and 190℃),the core/sheath structural flax/PLA composite yarns were manufactured.According to the results of the tensile test,the flax/PLA composite yarn with 4-spindle PLA yarns as a sheath layer and at a curing temperature of 180℃reached the maximum elastic modulus of about(5.79±0.65)GPa and the maximum tensile strength of about(162.17±18.18)MPa.This flax/PLA composite yarn with good mechanical properties would be suitable for green composites in the automobile manufacturing industry and building materials.展开更多
Nanofiber core-spun yarn(NCSY)combines the advantages of traditional fibers and nanofibers to be widely used in smart wearable textiles,biomedical textiles,and functional textiles.Here,for the first time,the forming p...Nanofiber core-spun yarn(NCSY)combines the advantages of traditional fibers and nanofibers to be widely used in smart wearable textiles,biomedical textiles,and functional textiles.Here,for the first time,the forming process of NCSY and its shape regulation mechanism were explored via finite element analysis and response surface analysis method to obtain mathematical model for predicting the various forms of yarn.As proof-of-concept applications,shape-controllable nanofiber core-spun yarns were prepared for thermal–moisture management and solar steam generation,respectively.The as-obtained shape-controllable PAN nanofiber/cotton composite yarns could achieve an interval control of average water transfer velocity in the horizontal(0.17–0.24 cm min^(-1))and vertical(0.24–0.33 cm min^(-1))directions within 30 min due to the arrangement of PAN nanofibers causes microchannels and hydrophilicity,matching the sweat secretion of human bodies under dynamic or static conditions and realizing the purpose of thermal and moisture comfort.Furthermore,PAN nanofiber wrapped CNTs/cotton composite yarn-based(PAN@CNTs-NCSY)evaporator was designed,which shows a fast water evaporation rate of 1.40 kg m^(-2)h^(-1),exceeding in most fabric-based evaporators reported to date.These findings have guiding significance for preparing rich style NCSY according to demand and designing functional and intelligent textiles via adjusting the type of core and shell fibers.展开更多
Automatic splicing of interrupted yarns in ring spinning has always been a problem in the industry.Factors such as low yarn strengths and environmental influence on yarn tensions make it difficult to control the yarn ...Automatic splicing of interrupted yarns in ring spinning has always been a problem in the industry.Factors such as low yarn strengths and environmental influence on yarn tensions make it difficult to control the yarn tension during the robotic splicing process.The purpose of this research is to design active disturbance rejection control(ADRC)for a third-order nonlinear tension system subject to external disturbances.Firstly,a third-order extended state observer(ESO)is designed to achieve the suppression and the compensation of the internal modeling error and the external disturbances of the system.Secondly,the adaptive gain error feedback control and the filtering process are designed to reduce the influence of sensor noise on the disturbance observation.Finally,the tension control during the splicing process is simulated and experimented,and the experiments show that the method has good robustness in the tension tracking task under a dynamic environment,which verifies the effectiveness of the method.展开更多
为解决Hadoop现有调度器调度任务时不能根据任务的紧迫程度分配资源的问题,研究YARN中的资源调度机制,改进原调度器(Capacity Scheduler),提出一种基于优先级权重的Hadoop YARN(Yet Another Resource Negotiator)调度算法(Weight Schedu...为解决Hadoop现有调度器调度任务时不能根据任务的紧迫程度分配资源的问题,研究YARN中的资源调度机制,改进原调度器(Capacity Scheduler),提出一种基于优先级权重的Hadoop YARN(Yet Another Resource Negotiator)调度算法(Weight Scheduler Based on Priority)。为叶子队列设置队列优先级,结合队列资源利用率和队列优先级选择队列;将应用程序的初始权重设置为应用程序优先级的大小,通过等待时间判断是否更新权重,根据权重对队列中的应用程序进行排序,调度时优先为权重高的应用程序分配资源。实验结果表明,与原有调度算法相比,改进算法平均任务执行时间约减少141 s,平均等待时间减少34.5%,保证了用户执行任务的相对公平,提高了用户总体满意度。展开更多
基金supported by the National Natural Science Foundation of China(No.52003131)the Major Scientific and Technological Innovation Program of Shandong(No.2019JZZY010340)+2 种基金China Postdoctoral Science Foundation(No.2023M731838)Youth Innovation Science and Technology Plan of Shandong Province(2020KJA013)Taishan Scholar Program of Shandong Province in China(tsqn202211116).
文摘High-performance wearable electronics are highly desirable for the development of body warming and human health monitoring devices.In the present study,high electrically conductive and photothermal cotton yarns(CYs)with long-term stability were prepared as wearable electronics.The process contains back-to-back decoration of the fiber surface by Ti_(3)C_(2)T_(x)(MXene)nanosheets,and the poly(3,4-ethylenedioxythiophene)polystyrene sulfonate(PEDOT:PSS)composite,to form a core–shell structure(MP@CY).The addition of a small amount of PEDOT:PSS plays a dual role of protecting the MXene from oxidation and increasing the electrical conductivity.The resulting yarn exhibits excellent electrical conductivity(21.8Ωcm^(−1)),rapid electrothermal response,and superb photothermal conversion capability,supporting its application as an optical/electrical dual-drive heater.A three-dimensional(3D)honeycomb-like textile wearable heater based on MP@CY as weft yarn demonstrates outstanding electrical thermal properties(0–2.5 V,30–196.8°C)and exceptional photothermal conversion(130 mW cm^(−2),64.2°C).Using an Internet of Things(IoT)microcontroller and Espressif(ESP)electronics chip,which are combined with wireless fidelity(Wi-Fi)and smartphone,real-time visualization and precise control of the temperature interface can be achieved.Furthermore,MP@CY-based knitted sensors,obtained by hand-knitting,are utilized for monitoring human movement and health,exhibiting high sensitivity and long-term cycling stability.
基金supported by the National Natural Science Foundation of China(No.52273074)the Central government guided local science and technology development fund project,Gansu Provincial Science and Technology Plan Project(Project Number:22ZY2QA001)Lanzhou Science and Technology Plan Project Funding(Project Number:2021-1-44).
文摘Graphene composite yarns have demonstrated significant potential in the development of multifunctional wearable elec-tronics,showcasing exceptional conductivity,mechanical properties,flexibility,and lightweight design.However,their performance is limited by the weak interfacial interaction between the fibers and graphene.Herein,a polydopamine-reduced graphene oxide(PDA-RGO)interfacial modulation strategy is proposed to prepare graphene-coated cotton yarns with high electrical conductivity and strength.PDA-RGO serves as an interfacial bonding molecule that interacts with the cotton yarn(CY)substrate to establish a hydrogen interface,while interconnecting with highly conductive graphene throughπ-πinterac-tions.The developed interface-designed graphene-coated yarn demonstrates an impressive average electrical conductivity of(856.27±7.02)S/m(i.e.,average resistance of(57.57±5.35)Ω).Simultaneously,the obtained conductive yarn demonstrates an exceptional average tensile strength of(172.03±8.03)MPa,surpassing that of primitive CY by approximately 1.59 times.The conductive yarns can be further used as low-voltage flexible wearable heaters and high-sensitivity pressure sensors,thus showcasing their remarkable potential for high-performance and multifunctional wearable devices in real-world applications.
基金financially supported by the National Creative Research Initiative(CRI)Center for Multi-Dimensional Directed Nanoscale Assembly(2015R1A3A2033061)a Creative Challenge research grant(RS-2023-00248902)through the National Research Foundation of Korea(NRF),funded by the Ministry of Science+2 种基金supported by the Collabo R&D between Industry,Academy,and Research Institute(RS-2024-00428937)funded by the Ministry of SMEs and Startups(MSS,Korea)This study was also supported by the Development Program of Machinery and Equipment Industrial Technology(20018235,Development of an inline nanoimprinter for nanophotonic device)funded by the Ministry of Trade,Industry,&Energy(MI,Korea),the Ministry of Culture,Sports,and Tourism,and the Korea Creative Content Agency(Project Number:R2022020033)It was also supported by a National Research Foundation of Korea(NRF)grant funded by the Korean government(MSIT)(No.2021R1A2C3008742).
文摘Fiber supercapacitors(FSs)based on transition metal oxides(TMOs)have garnered considerable attention as energy stor-age solutions for wearable electronics owing to their exceptional characteristics,including superior comfortability and low weights.These materials are known to exhibit high energy densities,high specific capacitances,and fast redox reactions.However,current fabrication methods for these structures primarily rely on chemical deposition,often resulting in undesir-able material structures and necessitating the use of additives,which can degrade the electrochemical performance of such structures.Herein,physically deposited TMO nanoribbon yarns generated via delamination engineering of nanopatterned TMO/metal/TMO trilayer arrays are proposed as potential high-performance FSs.To prepare these arrays,the target materials were initially deposited using a nanoline mold,and subsequently,the nanoribbon was suspended through selective plasma etching to obtain the desired twisted yarn structures.Because of the direct formation of TMOs on Ni electrodes,a high energy/power density and excellent electrochemical stability were achieved in asymmetric FS devices incorporating CoNixOy nanoribbon yarns and graphene fibers.Furthermore,a triboelectric nanogenerator,pressure sensor,and flexible light-emitting diode were synergistically combined with the FS.The integration of wearable electronic components,encompassing energy harvesting,energy storage,and powering sensing/display devices,is promising for the development of future smart textiles.
基金support from an ARC Discovery Project(DP180102003)are highly appreciated.
文摘Wearable fiber-based lithium-ion batteries(LiBs)made with textile-like functional electrode materials are key to realizing smart energy options for powering wearable electronics.However,the process of attenuating the existing functional materials commonly used in planar and solid-state batteries to functional fiber or yarn electrodes tends to deteriorate the material performance when assembled into textile-based electrodes.In this work,we focus on understanding and enabling layered Ni-rich cathode material into a wearable cathode yarn.Layered Ni-rich cathode materials typically contain a higher proportion of Ni compared to other metals like Co and Mn,with a Li[Ni_(1−x)M_(x)]O_(2)(M=transition metal element,such as Mn,Al,Co,and so on)typical structure.They are increasingly gaining popularity in the research and development of LiBs as they offer several advantages,including higher energy density,improved cycle life,and reduced cost compared to many commercial cathode materials.Our fabricated flexible Ni-rich cathode yarn with an overall diameter of~360μm and a coating thickness of~80μm exhibited textile properties with promising mechanical strength and the ability to conform to any shape.When tested in a half-cell arrangement with Li metal as the counter electrode,the Ni-rich cathode yarn electrode showed stable cyclic performance with a discharge areal capacity of~3 mAh/cm^(2) and an average coulombic efficiency of 99.5%at a 0.2 mA/cm^(2) current density.Overall,the results show that Ni-rich cathode materials,despite their layered structure,are integrateable into usable wearable textile LiBs.
基金National Natural Science Foundation of China(No.52273054)Shanghai Natural Science Foundation,China(No.20ZR1402200)。
文摘The increasing demand for sustainable and environmentally friendly materials has driven research towards the development of green composites.In this work,the flax/polylactic acid(PLA)braided yarns were fabricated by braiding PLA filaments with 4 to 24 spindles on flax yarns.After curing at different temperatures(180℃and 190℃),the core/sheath structural flax/PLA composite yarns were manufactured.According to the results of the tensile test,the flax/PLA composite yarn with 4-spindle PLA yarns as a sheath layer and at a curing temperature of 180℃reached the maximum elastic modulus of about(5.79±0.65)GPa and the maximum tensile strength of about(162.17±18.18)MPa.This flax/PLA composite yarn with good mechanical properties would be suitable for green composites in the automobile manufacturing industry and building materials.
基金supported by the Grants(52373069,52373032,51973027,and 52003044)from the National Natural Science Foundation of China,the National Key Research and Development Program of China(2023YFC3011701)the Fundamental Research Funds for the Central Universities(2232023A-05)+3 种基金International Cooperation Fund of Science and Technology Commission of Shanghai Municipality(21130750100)the Fundamental Research Funds for the Central Universities and Graduate Student Innovation Fund of Donghua University(CUSF-DH-D2022039)Major Scientific and Technological Innovation Projects of Shandong Province(2021CXGC011004,2023CXGC010610)supported by the Chang Jiang Scholars Program and the Innovation Program of Shanghai Municipal Education Commission(2019-01-07-00-03-E00023)to Prof.Xiaohong Qin.
文摘Nanofiber core-spun yarn(NCSY)combines the advantages of traditional fibers and nanofibers to be widely used in smart wearable textiles,biomedical textiles,and functional textiles.Here,for the first time,the forming process of NCSY and its shape regulation mechanism were explored via finite element analysis and response surface analysis method to obtain mathematical model for predicting the various forms of yarn.As proof-of-concept applications,shape-controllable nanofiber core-spun yarns were prepared for thermal–moisture management and solar steam generation,respectively.The as-obtained shape-controllable PAN nanofiber/cotton composite yarns could achieve an interval control of average water transfer velocity in the horizontal(0.17–0.24 cm min^(-1))and vertical(0.24–0.33 cm min^(-1))directions within 30 min due to the arrangement of PAN nanofibers causes microchannels and hydrophilicity,matching the sweat secretion of human bodies under dynamic or static conditions and realizing the purpose of thermal and moisture comfort.Furthermore,PAN nanofiber wrapped CNTs/cotton composite yarn-based(PAN@CNTs-NCSY)evaporator was designed,which shows a fast water evaporation rate of 1.40 kg m^(-2)h^(-1),exceeding in most fabric-based evaporators reported to date.These findings have guiding significance for preparing rich style NCSY according to demand and designing functional and intelligent textiles via adjusting the type of core and shell fibers.
基金National Natural Science Foundation of China(No.52275478)Fundamental Research Funds for the Central Universities,China(No.2232024Y-01)DHU Distinguished Young Professor Program,China(No.LZB2023001)。
文摘Automatic splicing of interrupted yarns in ring spinning has always been a problem in the industry.Factors such as low yarn strengths and environmental influence on yarn tensions make it difficult to control the yarn tension during the robotic splicing process.The purpose of this research is to design active disturbance rejection control(ADRC)for a third-order nonlinear tension system subject to external disturbances.Firstly,a third-order extended state observer(ESO)is designed to achieve the suppression and the compensation of the internal modeling error and the external disturbances of the system.Secondly,the adaptive gain error feedback control and the filtering process are designed to reduce the influence of sensor noise on the disturbance observation.Finally,the tension control during the splicing process is simulated and experimented,and the experiments show that the method has good robustness in the tension tracking task under a dynamic environment,which verifies the effectiveness of the method.
文摘为解决Hadoop现有调度器调度任务时不能根据任务的紧迫程度分配资源的问题,研究YARN中的资源调度机制,改进原调度器(Capacity Scheduler),提出一种基于优先级权重的Hadoop YARN(Yet Another Resource Negotiator)调度算法(Weight Scheduler Based on Priority)。为叶子队列设置队列优先级,结合队列资源利用率和队列优先级选择队列;将应用程序的初始权重设置为应用程序优先级的大小,通过等待时间判断是否更新权重,根据权重对队列中的应用程序进行排序,调度时优先为权重高的应用程序分配资源。实验结果表明,与原有调度算法相比,改进算法平均任务执行时间约减少141 s,平均等待时间减少34.5%,保证了用户执行任务的相对公平,提高了用户总体满意度。