The present investigation targets minimum cost of reactors in series for the case of one single chemical reaction, considering plug flow and stirred tank reactor(s) in the sequence of flow reactors. Using Guthrie'...The present investigation targets minimum cost of reactors in series for the case of one single chemical reaction, considering plug flow and stirred tank reactor(s) in the sequence of flow reactors. Using Guthrie's cost correlations three typical cases were considered based on the profile of the reaction rate reciprocal versus conversion. Significant differences were found compared to the classical approach targeting minimum total reactor volume.展开更多
Activated carbon-supported Ru-based catalyst and A301 iron catalyst were prepared,and the influences of reaction temperature,space velocity,pressure,and H2/N2 ratio on performance of iron catalyst coupled with Ru cata...Activated carbon-supported Ru-based catalyst and A301 iron catalyst were prepared,and the influences of reaction temperature,space velocity,pressure,and H2/N2 ratio on performance of iron catalyst coupled with Ru catalyst in series for ammonia synthesis were investigated.The activity tests were also performed on the single Ru and Fe catalysts as comparison.Results showed that the activity of the Ru catalyst for ammonia synthesis was higher than that of the iron catalyst by 33.5%-37.6% under the reaction conditions：375-400 °C,10 MPa,10000 h-1,H2︰N2 3,and the Ru catalyst also had better thermal stability when treated at 475 °C for 20 h.The outlet ammonia concentration using Fe-Ru catalyst was increased by 45.6%-63.5% than that of the single-iron catalyst at low tem-perature （375-400 °C）,and the outlet ammonia concentration increased with increasing Ru catalyst loading.展开更多
The Variable Series Reactors(VSRs)can efficiently control the power flow through the adjustment of the line reactance.When they are appropriately allocated in the power network,the transmission congestion and generati...The Variable Series Reactors(VSRs)can efficiently control the power flow through the adjustment of the line reactance.When they are appropriately allocated in the power network,the transmission congestion and generation cost can be reduced.This paper proposes a planning model to optimally allocate VSRs considering AC constraints and multi-scenarios including base case and contingencies.The planning model is originally a non-convex large scale mixed integer nonlinear program(MINLP),which is generally intractable.The proposed Benders approach decomposes the MINLP model into a mixed integer linear program(MILP)master problem and a number of nonlinear subproblems.Numerical case studies based on IEEE 118-bus demonstrate the high performance of the proposed approach.展开更多
文摘The present investigation targets minimum cost of reactors in series for the case of one single chemical reaction, considering plug flow and stirred tank reactor(s) in the sequence of flow reactors. Using Guthrie's cost correlations three typical cases were considered based on the profile of the reaction rate reciprocal versus conversion. Significant differences were found compared to the classical approach targeting minimum total reactor volume.
基金Supported by the National Natural Science Foundation of China（20803064） the Natural Science Foundation of Zhejiang Province（Y409034）
文摘Activated carbon-supported Ru-based catalyst and A301 iron catalyst were prepared,and the influences of reaction temperature,space velocity,pressure,and H2/N2 ratio on performance of iron catalyst coupled with Ru catalyst in series for ammonia synthesis were investigated.The activity tests were also performed on the single Ru and Fe catalysts as comparison.Results showed that the activity of the Ru catalyst for ammonia synthesis was higher than that of the iron catalyst by 33.5%-37.6% under the reaction conditions：375-400 °C,10 MPa,10000 h-1,H2︰N2 3,and the Ru catalyst also had better thermal stability when treated at 475 °C for 20 h.The outlet ammonia concentration using Fe-Ru catalyst was increased by 45.6%-63.5% than that of the single-iron catalyst at low tem-perature （375-400 °C）,and the outlet ammonia concentration increased with increasing Ru catalyst loading.
基金This work was supported in part by the Advanced Research Projects Agency-Energy(ARPA-E)the Engineering Research Center Program of the National Science Foundation+2 种基金the Department of Energy under NSF Award Number EEC-1041877the CURENT Industry Partnership Programthe Science and Technology Project of State Grid Corporation of China(Project Analysis Techniques for Coordinated Development of New Energy,Distributed Generation,Energy Storage and Power Grid to Meet Global Energy Interconnection Demand).
文摘The Variable Series Reactors(VSRs)can efficiently control the power flow through the adjustment of the line reactance.When they are appropriately allocated in the power network,the transmission congestion and generation cost can be reduced.This paper proposes a planning model to optimally allocate VSRs considering AC constraints and multi-scenarios including base case and contingencies.The planning model is originally a non-convex large scale mixed integer nonlinear program(MINLP),which is generally intractable.The proposed Benders approach decomposes the MINLP model into a mixed integer linear program(MILP)master problem and a number of nonlinear subproblems.Numerical case studies based on IEEE 118-bus demonstrate the high performance of the proposed approach.
