In the framework of the Hartree-Fock approach the proton spin-orbital splittings of the 1p orbits and the shell gaps in the oxygen isotopes are investigated with the interactions SLy5+T,SLy5+Tw,SGII+Te1,SGII+Te2,SGII+...In the framework of the Hartree-Fock approach the proton spin-orbital splittings of the 1p orbits and the shell gaps in the oxygen isotopes are investigated with the interactions SLy5+T,SLy5+Tw,SGII+Te1,SGII+Te2,SGII+Te3 and many sets of the TIJ interactions.All of the interactions are the Skyrme interactions and contain a tensor component(tensor force).It is shown that the evolution of the single-proton levels for the oxygen isotopes is sensitive to a parameterβTwhich is associated with the tensor force strength of the Skyrme interactions.To understand this phenomenon,we systematically analyze the dependence of the spin-orbit splittings and shell gaps on the parameterβTin terms of the spin-orbit potential and the corresponding wave function.We find that the Skyrme interactions can be classified into two groups:(a)T21,T32,T43,T54,SLy5+T,SLy5+Tw,SGII+Te1 and SGII+Te2,which can roughly reproduce the experimental shell gaps of the oxygen isotopes;(b)T1J and SGII+Te3,which can not reproduce the experimental shell gaps.展开更多
A nuclear mass formula based on the macroscopic microscopic approach is proposed,in which the number of model parameters is reduced compared with other macroscopic microscopic models.The root mean square(RMS)deviation...A nuclear mass formula based on the macroscopic microscopic approach is proposed,in which the number of model parameters is reduced compared with other macroscopic microscopic models.The root mean square(RMS)deviation with respect to 2314 training sets(measured nuclear masses)is reduced to 0.447 MeV,and the calculated value of each nucleus is no more than 0.8%different from the experimental value.The single and two nucleon separation energies and the shell gaps are calculated to test the model.The shell corrections and double magic number of superheavy nuclei are also analyzed.展开更多
A simple polyol and sol–gel Stober process were employed for synthesis of YF_3:Tb~+(core), YF_3:Tb~+@LaF_3(core/shell) and YF_3:Tb~+@LaF_3@SiO_2(core/shell/SiO_2) nanoparticles(NPs). The phase purity, c...A simple polyol and sol–gel Stober process were employed for synthesis of YF_3:Tb~+(core), YF_3:Tb~+@LaF_3(core/shell) and YF_3:Tb~+@LaF_3@SiO_2(core/shell/SiO_2) nanoparticles(NPs). The phase purity, crystalinity,morphology, optical and photoluminescence properties were investigated and discussed with the help of various analytical techniques including X-ray diffraction pattern,FE-transmission electron microscopy(TEM),FTIR, UV/vis absorption, energy band gap and emission spectra. XRD andFE-TEM studies indicate the formation of core/shell nanostructure and ~10 nm thick amorphous silica surface coating surrounding the core-NPs, which is also confirmed byFTIR spectral results. The surface modifications of core-NPs significantly affect the optical features in the form of energy band gap, which were correlated with particle size of the nanomaterials. The comparative emission spectral results show that after inert layer coating the luminescent core-NPs display stronger emission intensity in respect to core and silica coated core/shell/SiO_2-NPs. The solubility character along with colloidal stability was improved after silica surface modification, whereas luminescent intensity was suppressed causing the surface functionalized with high energy silanol(Si-OH) molecules. These novel luminescent nanomaterials with enhanced emission intensity and excellent solubility in aqueous solvents would be potentially useful for fluorescence bioimaging/optical bio-probe etc.展开更多
基金supported by the Fundamental Research Funds for the Central Universities(Grant No.13QN59)the National Natural Science Foundation of China(Grant Nos.11275271 and 11305109)+1 种基金the Funds for Creative Research Groups of China(Grant No.11021504)the Natural Science Foundation of Guizhou Province of China(Grant No.2013GZ62432)
文摘In the framework of the Hartree-Fock approach the proton spin-orbital splittings of the 1p orbits and the shell gaps in the oxygen isotopes are investigated with the interactions SLy5+T,SLy5+Tw,SGII+Te1,SGII+Te2,SGII+Te3 and many sets of the TIJ interactions.All of the interactions are the Skyrme interactions and contain a tensor component(tensor force).It is shown that the evolution of the single-proton levels for the oxygen isotopes is sensitive to a parameterβTwhich is associated with the tensor force strength of the Skyrme interactions.To understand this phenomenon,we systematically analyze the dependence of the spin-orbit splittings and shell gaps on the parameterβTin terms of the spin-orbit potential and the corresponding wave function.We find that the Skyrme interactions can be classified into two groups:(a)T21,T32,T43,T54,SLy5+T,SLy5+Tw,SGII+Te1 and SGII+Te2,which can roughly reproduce the experimental shell gaps of the oxygen isotopes;(b)T1J and SGII+Te3,which can not reproduce the experimental shell gaps.
文摘A nuclear mass formula based on the macroscopic microscopic approach is proposed,in which the number of model parameters is reduced compared with other macroscopic microscopic models.The root mean square(RMS)deviation with respect to 2314 training sets(measured nuclear masses)is reduced to 0.447 MeV,and the calculated value of each nucleus is no more than 0.8%different from the experimental value.The single and two nucleon separation energies and the shell gaps are calculated to test the model.The shell corrections and double magic number of superheavy nuclei are also analyzed.
基金funded byNational Plan for Science,Technology and Innovation(MAARIFAH)King Abdulaziz City for Science and Technology,Kingdom of Saudi Arabia,award number(No.13-Bio1246-02)
文摘A simple polyol and sol–gel Stober process were employed for synthesis of YF_3:Tb~+(core), YF_3:Tb~+@LaF_3(core/shell) and YF_3:Tb~+@LaF_3@SiO_2(core/shell/SiO_2) nanoparticles(NPs). The phase purity, crystalinity,morphology, optical and photoluminescence properties were investigated and discussed with the help of various analytical techniques including X-ray diffraction pattern,FE-transmission electron microscopy(TEM),FTIR, UV/vis absorption, energy band gap and emission spectra. XRD andFE-TEM studies indicate the formation of core/shell nanostructure and ~10 nm thick amorphous silica surface coating surrounding the core-NPs, which is also confirmed byFTIR spectral results. The surface modifications of core-NPs significantly affect the optical features in the form of energy band gap, which were correlated with particle size of the nanomaterials. The comparative emission spectral results show that after inert layer coating the luminescent core-NPs display stronger emission intensity in respect to core and silica coated core/shell/SiO_2-NPs. The solubility character along with colloidal stability was improved after silica surface modification, whereas luminescent intensity was suppressed causing the surface functionalized with high energy silanol(Si-OH) molecules. These novel luminescent nanomaterials with enhanced emission intensity and excellent solubility in aqueous solvents would be potentially useful for fluorescence bioimaging/optical bio-probe etc.