The presence of light-absorbing aerosols (LAA) in snow profoundly influence the surface energy balance and water budget. However, most snow-process schemes in land-surface and climate models currently do not take th...The presence of light-absorbing aerosols (LAA) in snow profoundly influence the surface energy balance and water budget. However, most snow-process schemes in land-surface and climate models currently do not take this into consider- ation. To better represent the snow process and to evaluate the impacts of LAA on snow, this study presents an improved snow albedo parameterization in the Snow-Atmosphere-Soil on snow. Specifically, the Snow, Ice and Aerosol Radiation Transfer (SAST) model, which includes the impacts of LAA (SNICAR) model is incorporated into the SAST model with an LAA mass stratigraphy scheme. The new coupled model is validated against in-situ measurements at the Swamp Angel Study Plot (SASP), Colorado, USA. Results show that the snow albedo and snow depth are better reproduced than those in the original SAST, particularly during the period of snow ablation. Furthermore, the impacts of LAA on snow are esti- mated in the coupled model through case comparisons of the snowpack, with or without LAA. The LAA particles directly absorb extra solar radiation, which accelerates the growth rate of the snow grain size. Meanwhile, these larger snow particles favor more radiative absorption. The average total radiative forcing of the LAA at the SASP is 47.5 W m-2. This extra radiative absorption enhances the snowmelt rate. As a result, the peak runoff time and "snow all gone" day have shifted 18 and 19.5 days earlier, respectively, which could further impose substantial impacts on the hydrologic cycle and atmospheric processes.展开更多
In this study the authors apply the chemistry version of the Weather Research and Forecasting model (WRF-Chem) to examine the impacts of black carbon (BC)-induced changes in snow albedo on simulated tem-perature and p...In this study the authors apply the chemistry version of the Weather Research and Forecasting model (WRF-Chem) to examine the impacts of black carbon (BC)-induced changes in snow albedo on simulated tem-perature and precipitation during the severe snowstorm that occurred in southern China during 0800 26 January to 0800 29 January 2008 (Note that all times are local time except when otherwise stated).Black carbon aerosol was simulated online within the WRF-Chem.The model re-sults showed that surface-albedo,averaged over 27 28 January,can be reduced by up to 10% by the deposition of BC.As a result,relative to a simulation that does not con-sider deposition of BC on snow/ice,the authors predicted surface air temperatures during 27 28 January can differ by 1.95 to 2.70 K,and the authors predicted accumu-lated precipitation over 27 28 January can differ by 2.91 to 3.10 mm over Areas A and B with large BC deposition.Different signs of changes are determined by the feedback of clouds and by the availability of water vapor in the atmosphere.展开更多
Since snow cover is one of the fastest modifications to the land surface albedo, the treatment of snow-covered surface albedo is important for the simulation of land processes in weather and climate models. A simple f...Since snow cover is one of the fastest modifications to the land surface albedo, the treatment of snow-covered surface albedo is important for the simulation of land processes in weather and climate models. A simple formulation is developed here to represent the solar zenith angle (SZA) dependence of albedo under maximum snow cover condition on the basis of Moderate Resolution Imaging Spectroradiometer (MODIS) Bidirectional Reflectance Distribution Function (BRDF) algorithm. The SZA dependence of black-sky (or direct) albedo is weaker under snow condition than that under snow-free condition, and it does not differ much among different vegetation types. The blue-sky albedo (or combined albedo from direct and diffuse radiations) based on the above formulation and in situ diffuse ratio of solar radiation is consistent with in situ data from two Canadian sites (grassland and evergreen needleleaf forest) and one U.S. grassland site. In particular, the SZA dependence of bluesky snow albedo is almost always weak because of high diffuse ratios for high SZA in winter. With the snow albedo formulation from this study and snow-free albedo formulations from the authors' previous studies, albedos with partial snow cover can be obtained as the snow frac- tion-weighted average of snow and snow-free albedos.展开更多
An 18-year long(1993–2011) comprehensive dataset of snow and meteorological variables from Col de Porte, France is used to analyze the variation of shortwave broadband albedo with elapsed time after snowfalls(snow ag...An 18-year long(1993–2011) comprehensive dataset of snow and meteorological variables from Col de Porte, France is used to analyze the variation of shortwave broadband albedo with elapsed time after snowfalls(snow aging) during each snow season. The effects of air temperature, snow surface temperature and snow depth on snow albedo are investigated. An index based on the accumulation of air temperature over several consecutive days with daily mean higher than 2.5 °C is proposed to divide each snow-covered period into a dry and the following wet snow season when this index reaches 18 °C.The results indicate that snow surface albedo decreases exponentially with time in both dry and wet snow seasons.Snow albedo reduction with snow aging is small at low surface temperature and the reduction rate increases with the rise of surface temperature. However, the reduction rate is widely scattered within the observed range of temperature, implying a loose relationship between snow albedo and snow surface temperature. Snow albedo in wet snowseason is generally smaller and decreases faster than in dry snow season. For Col de Porte site, snow depths to effectively mask the underlying surface are 21 and 33 cm in dry and wet snow season respectively.展开更多
Surface albedo over typical types of surfaces in the North China Plain was observed using a Multi-field Albedo Observation System before and after several snowfalls from 13 to 27 February 2005. Dramatic variations of ...Surface albedo over typical types of surfaces in the North China Plain was observed using a Multi-field Albedo Observation System before and after several snowfalls from 13 to 27 February 2005. Dramatic variations of the surface albedos of bare land, a frozen pond, and withered grassland during that period were analyzed. Under cloudy sky, the mean surface albedo of bare land was about 0.23, but it immediately rose to 0.85 when the surface was covered by fresh snow. The albedo decreased gradually to normal levels afterwards. The melting processes were different depending on the characteristics of the underlying surfaces. For example, over grassland the surface albedo was relatively lower after snowfall, and as a result, more solar energy could be absorbed and consequently the snow melting process was accelerated. Significant variations of surface albedo cannot be easily captured by satellite observations; therefore, detailed measurements of surface albedo and related parameters are essential for determining the impact of snow on the energy budget of the Earth.展开更多
Recent decline of cryosphere typified by retreat of glaciers is often explained by temperature rise due to global warming. However, the existence of glaciers shrinking since before 1950s warming accelerated suggested ...Recent decline of cryosphere typified by retreat of glaciers is often explained by temperature rise due to global warming. However, the existence of glaciers shrinking since before 1950s warming accelerated suggested that decline of cryosphere may be due to not only temperature rise, but also another possibility. As a possible cause of snow and ice melting, it has been pointed out that the surface albedo reduction due to increase of snow impurity, aeolian dust and anthropogenic pollutant, for example. To clarify the quantitative relationship between albedo and impurity in snow surface, we investigated the correlativity of turbidity and metal concentration in snow to the snow surface albedo from the simultaneous observations on the snow-covered area in Yamagata, Japan. The observed albedo shows a tendency of decrease with the turbidity increase in snow surface, we could find strong correlation between the albedo and the turbidity in 76% of contribution factor using logarithmic regression analysis. The relationship of albedo to total concentration of Fe and Al in snow surface shows the similar tendency to turbidity, we could model the relationship using logarithmic equation with high value of contribution ratio, 74% and 66%, respectively. The concentration ratio of Fe/Al is nearly constant with about 0.75, which is close to mean crustal ratio of both elements, therefore, it can be said there is a strong correlation between the albedo and the concentration of mineral particle in snow surface. We cannot find a significant correlation between the albedo and total concentration of Na in snow surface. It can be considered that Na existed as dissolved ion has not significant effect to the albedo in snow surface. These results indicate that the snow albedo correlates strongly with the particulate matter in snow surface, which is typified by mineral particle.展开更多
Estimation of the influence of snow grain size and black carbon on albedo is essential in obtaining the accurate albedo. In this paper, field measurement data, including snow grain size, snow depth and density was obt...Estimation of the influence of snow grain size and black carbon on albedo is essential in obtaining the accurate albedo. In this paper, field measurement data, including snow grain size, snow depth and density was obtained. Black carbon samples were collected from the snow surface. A simultaneous observation using Analytical Spectral Devices was employed in the Qiyi Glacier located in the Qilian Mountain. Analytical Spectral Devices spectrum data were used to analyze spectral re- flectance of snow for different grain size and black carbon content. The measurements were compared with the results obtained from the Snow, Ice, and Aerosol Radiation model, and the simulation was found to correlate well with the ob- served data. However, the simulated albedo was near to 0.98 times of the measured albedo, so the other factors were as- sumed to be constant using the corrected Snow, Ice, and Aerosol Radiation model to estimate the influence of measured snow grain size and black carbon on albedo. Field measurements were controlled to fit the relationship between the snow grain size and black carbon in order to estimate the influence of these factors on the snow albedo.展开更多
Snow albedo is an important factor influencing the snow surface energy budget and snow melting, yet uncertainties remain in the calculation of spectrally resolved snow surface albedo because the spectral composition ...Snow albedo is an important factor influencing the snow surface energy budget and snow melting, yet uncertainties remain in the calculation of spectrally resolved snow surface albedo because the spectral composition (visible versus near infrared) of the incident solar radiation is seldom available. The influence of the spectral composition of the incoming solar radiation on the snow surface albedo, snow surface energy budget, and final snow ablation is investigated through sensitivity experiments of four snow seasons at two open sites in the Alps by using a multi-layer Snow-Atmosphere-Soil-Transfer scheme (SAST). Since the snow albedo in the near infrared (NIR) spectral band is significantly lower than that in the visible (VIS) band, and almost the entire NIR part of the solar radiation is absorbed in the top layer of the snow pack, given a fixed amount of incoming solar radiation, a lower VIS/NIR ratio implies that more NIR radiation is reaching the ground surface and more is absorbed by the top layer of the snow pack, therefore, speeding up the snow melting and increasing the surface runoff, although a lesser part of the solar radiation in the visible band is transmitted into and trapped by the sub-layer of the snow pack. The above VIS/NIR ratio effect of the incoming solar radiation can result in a couple of days difference in the timing of snow ablation and it becomes more significant in late spring when the total solar radiation is intensified with seasonal evolution. Snow aging also slightly intensifies this VIS/NIR ratio effect.展开更多
Light-absorbing impurities on glaciers are important factors that influence glacial surface albedo and accelerate glacier melt. In this study, the quantity of light-absorbing impurities on Keqikaer Glacier in western ...Light-absorbing impurities on glaciers are important factors that influence glacial surface albedo and accelerate glacier melt. In this study, the quantity of light-absorbing impurities on Keqikaer Glacier in western Tien Shan, Central Asia, was measured. We found that the average concentrations of black carbon was 2,180 ng/g, with a range from 250 ng/g to more than 10,000 ng/g. The average concentrations of organic carbon and mineral dust were 1,738 ng/g and 194 μg/g, respectively. Based on simulations performed with the Snow Ice Aerosol Radiative model simulations, black carbon and dust are responsible for approximately 64% and 9%, respectively, of the albedo reduction, and are associated with instantaneous radiative forcing of 323.18 W/m2(ranging from 142.16 to 619.25 W/m2) and 24.05 W/m2(ranging from 0.15 to69.77 W/m2), respectively. For different scenarios, the albedo and radiative forcing effect of black carbon is considerably greater than that of dust. The estimated radiative forcing at Keqikaer Glacier is higher than most similar values estimated by previous studies on the Tibetan Plateau, perhaps as a result of black carbon enrichment by melt scavenging. Light-absorbing impurities deposited on Keqikaer Glacier appear to mainly originate from central Asia, Siberia, western China(including the Taklimakan Desert) and parts of South Asia in summer, and from the Middle East and Central Asia in winter.A footprint analysis indicates that a large fraction(>60%) of the black carbon contributions on Keqikaer Glacier comes from anthropogenic sources. These results provide a scientific basis for regional mitigation efforts to reduce black carbon.展开更多
Light absorbing particles(LAP, e.g., black carbon, brown carbon, and dust) influence water and energy budgets of the atmosphere and snowpack in multiple ways. In addition to their effects associated with atmospheric...Light absorbing particles(LAP, e.g., black carbon, brown carbon, and dust) influence water and energy budgets of the atmosphere and snowpack in multiple ways. In addition to their effects associated with atmospheric heating by absorption of solar radiation and interactions with clouds, LAP in snow on land and ice can reduce the surface reflectance(a.k.a., surface darkening), which is likely to accelerate the snow aging process and further reduces snow albedo and increases the speed of snowpack melt. LAP in snow and ice(LAPSI) has been identified as one of major forcings affecting climate change, e.g.in the fourth and fifth assessment reports of IPCC. However, the uncertainty level in quantifying this effect remains very high. In this review paper, we document various technical methods of measuring LAPSI and review the progress made in measuring the LAPSI in Arctic, Tibetan Plateau and other mid-latitude regions. We also report the progress in modeling the mass concentrations, albedo reduction, radiative forcing, and climatic and hydrological impact of LAPSI at global and regional scales. Finally we identify some research needs for reducing the uncertainties in the impact of LAPSI on global and regional climate and the hydrological cycle.展开更多
基金supported jointly by projects from the National Natural Science Foundation of China (Grant No.41275003)the National Key Basic Research and Development Projects of China (Grant No.2014CB953903)
文摘The presence of light-absorbing aerosols (LAA) in snow profoundly influence the surface energy balance and water budget. However, most snow-process schemes in land-surface and climate models currently do not take this into consider- ation. To better represent the snow process and to evaluate the impacts of LAA on snow, this study presents an improved snow albedo parameterization in the Snow-Atmosphere-Soil on snow. Specifically, the Snow, Ice and Aerosol Radiation Transfer (SAST) model, which includes the impacts of LAA (SNICAR) model is incorporated into the SAST model with an LAA mass stratigraphy scheme. The new coupled model is validated against in-situ measurements at the Swamp Angel Study Plot (SASP), Colorado, USA. Results show that the snow albedo and snow depth are better reproduced than those in the original SAST, particularly during the period of snow ablation. Furthermore, the impacts of LAA on snow are esti- mated in the coupled model through case comparisons of the snowpack, with or without LAA. The LAA particles directly absorb extra solar radiation, which accelerates the growth rate of the snow grain size. Meanwhile, these larger snow particles favor more radiative absorption. The average total radiative forcing of the LAA at the SASP is 47.5 W m-2. This extra radiative absorption enhances the snowmelt rate. As a result, the peak runoff time and "snow all gone" day have shifted 18 and 19.5 days earlier, respectively, which could further impose substantial impacts on the hydrologic cycle and atmospheric processes.
基金supported by the Knowledge Innovation Program of the Chinese Academy of Sciences (Grant KZCX2-YW-205)the National Natural Science Foundation of China (Grant Nos.40825016,90711004,and 40775083)
文摘In this study the authors apply the chemistry version of the Weather Research and Forecasting model (WRF-Chem) to examine the impacts of black carbon (BC)-induced changes in snow albedo on simulated tem-perature and precipitation during the severe snowstorm that occurred in southern China during 0800 26 January to 0800 29 January 2008 (Note that all times are local time except when otherwise stated).Black carbon aerosol was simulated online within the WRF-Chem.The model re-sults showed that surface-albedo,averaged over 27 28 January,can be reduced by up to 10% by the deposition of BC.As a result,relative to a simulation that does not con-sider deposition of BC on snow/ice,the authors predicted surface air temperatures during 27 28 January can differ by 1.95 to 2.70 K,and the authors predicted accumu-lated precipitation over 27 28 January can differ by 2.91 to 3.10 mm over Areas A and B with large BC deposition.Different signs of changes are determined by the feedback of clouds and by the availability of water vapor in the atmosphere.
基金supported by NOAA (NA07NES4400002)NASA (NNG06GA24G)
文摘Since snow cover is one of the fastest modifications to the land surface albedo, the treatment of snow-covered surface albedo is important for the simulation of land processes in weather and climate models. A simple formulation is developed here to represent the solar zenith angle (SZA) dependence of albedo under maximum snow cover condition on the basis of Moderate Resolution Imaging Spectroradiometer (MODIS) Bidirectional Reflectance Distribution Function (BRDF) algorithm. The SZA dependence of black-sky (or direct) albedo is weaker under snow condition than that under snow-free condition, and it does not differ much among different vegetation types. The blue-sky albedo (or combined albedo from direct and diffuse radiations) based on the above formulation and in situ diffuse ratio of solar radiation is consistent with in situ data from two Canadian sites (grassland and evergreen needleleaf forest) and one U.S. grassland site. In particular, the SZA dependence of bluesky snow albedo is almost always weak because of high diffuse ratios for high SZA in winter. With the snow albedo formulation from this study and snow-free albedo formulations from the authors' previous studies, albedos with partial snow cover can be obtained as the snow frac- tion-weighted average of snow and snow-free albedos.
基金supported by the Major National Scientific Research Project on Global Changes(2010CB951902)the National Natural Science Foundation of China(40975042 and41175005)
文摘An 18-year long(1993–2011) comprehensive dataset of snow and meteorological variables from Col de Porte, France is used to analyze the variation of shortwave broadband albedo with elapsed time after snowfalls(snow aging) during each snow season. The effects of air temperature, snow surface temperature and snow depth on snow albedo are investigated. An index based on the accumulation of air temperature over several consecutive days with daily mean higher than 2.5 °C is proposed to divide each snow-covered period into a dry and the following wet snow season when this index reaches 18 °C.The results indicate that snow surface albedo decreases exponentially with time in both dry and wet snow seasons.Snow albedo reduction with snow aging is small at low surface temperature and the reduction rate increases with the rise of surface temperature. However, the reduction rate is widely scattered within the observed range of temperature, implying a loose relationship between snow albedo and snow surface temperature. Snow albedo in wet snowseason is generally smaller and decreases faster than in dry snow season. For Col de Porte site, snow depths to effectively mask the underlying surface are 21 and 33 cm in dry and wet snow season respectively.
基金supported by the National Natural Science Foundation of China (40675017)
文摘Surface albedo over typical types of surfaces in the North China Plain was observed using a Multi-field Albedo Observation System before and after several snowfalls from 13 to 27 February 2005. Dramatic variations of the surface albedos of bare land, a frozen pond, and withered grassland during that period were analyzed. Under cloudy sky, the mean surface albedo of bare land was about 0.23, but it immediately rose to 0.85 when the surface was covered by fresh snow. The albedo decreased gradually to normal levels afterwards. The melting processes were different depending on the characteristics of the underlying surfaces. For example, over grassland the surface albedo was relatively lower after snowfall, and as a result, more solar energy could be absorbed and consequently the snow melting process was accelerated. Significant variations of surface albedo cannot be easily captured by satellite observations; therefore, detailed measurements of surface albedo and related parameters are essential for determining the impact of snow on the energy budget of the Earth.
文摘Recent decline of cryosphere typified by retreat of glaciers is often explained by temperature rise due to global warming. However, the existence of glaciers shrinking since before 1950s warming accelerated suggested that decline of cryosphere may be due to not only temperature rise, but also another possibility. As a possible cause of snow and ice melting, it has been pointed out that the surface albedo reduction due to increase of snow impurity, aeolian dust and anthropogenic pollutant, for example. To clarify the quantitative relationship between albedo and impurity in snow surface, we investigated the correlativity of turbidity and metal concentration in snow to the snow surface albedo from the simultaneous observations on the snow-covered area in Yamagata, Japan. The observed albedo shows a tendency of decrease with the turbidity increase in snow surface, we could find strong correlation between the albedo and the turbidity in 76% of contribution factor using logarithmic regression analysis. The relationship of albedo to total concentration of Fe and Al in snow surface shows the similar tendency to turbidity, we could model the relationship using logarithmic equation with high value of contribution ratio, 74% and 66%, respectively. The concentration ratio of Fe/Al is nearly constant with about 0.75, which is close to mean crustal ratio of both elements, therefore, it can be said there is a strong correlation between the albedo and the concentration of mineral particle in snow surface. We cannot find a significant correlation between the albedo and total concentration of Na in snow surface. It can be considered that Na existed as dissolved ion has not significant effect to the albedo in snow surface. These results indicate that the snow albedo correlates strongly with the particulate matter in snow surface, which is typified by mineral particle.
基金supported by "Strategic Priority Research Program (B)" of the Chinese Academy of Sciences (Grant No. XDB03030204)SKLCS (No. SKLCS-OP-2014-03)Major Research of National Natural Science Foundation of China (Grant No. 41190084)
文摘Estimation of the influence of snow grain size and black carbon on albedo is essential in obtaining the accurate albedo. In this paper, field measurement data, including snow grain size, snow depth and density was obtained. Black carbon samples were collected from the snow surface. A simultaneous observation using Analytical Spectral Devices was employed in the Qiyi Glacier located in the Qilian Mountain. Analytical Spectral Devices spectrum data were used to analyze spectral re- flectance of snow for different grain size and black carbon content. The measurements were compared with the results obtained from the Snow, Ice, and Aerosol Radiation model, and the simulation was found to correlate well with the ob- served data. However, the simulated albedo was near to 0.98 times of the measured albedo, so the other factors were as- sumed to be constant using the corrected Snow, Ice, and Aerosol Radiation model to estimate the influence of measured snow grain size and black carbon on albedo. Field measurements were controlled to fit the relationship between the snow grain size and black carbon in order to estimate the influence of these factors on the snow albedo.
基金supported by the Ministry of Science and Technology of China under Grant Nos.2007CB411505 and 2006CB403604the Ministry of Finance of China through Grant GYHY200706005
文摘Snow albedo is an important factor influencing the snow surface energy budget and snow melting, yet uncertainties remain in the calculation of spectrally resolved snow surface albedo because the spectral composition (visible versus near infrared) of the incident solar radiation is seldom available. The influence of the spectral composition of the incoming solar radiation on the snow surface albedo, snow surface energy budget, and final snow ablation is investigated through sensitivity experiments of four snow seasons at two open sites in the Alps by using a multi-layer Snow-Atmosphere-Soil-Transfer scheme (SAST). Since the snow albedo in the near infrared (NIR) spectral band is significantly lower than that in the visible (VIS) band, and almost the entire NIR part of the solar radiation is absorbed in the top layer of the snow pack, given a fixed amount of incoming solar radiation, a lower VIS/NIR ratio implies that more NIR radiation is reaching the ground surface and more is absorbed by the top layer of the snow pack, therefore, speeding up the snow melting and increasing the surface runoff, although a lesser part of the solar radiation in the visible band is transmitted into and trapped by the sub-layer of the snow pack. The above VIS/NIR ratio effect of the incoming solar radiation can result in a couple of days difference in the timing of snow ablation and it becomes more significant in late spring when the total solar radiation is intensified with seasonal evolution. Snow aging also slightly intensifies this VIS/NIR ratio effect.
基金supported by the National Natural Science Foundation of China (41630754, 41671067, and 41501063)the Chinese Academy of Sciences (KJZD-EW-G03-04), the State Key Laboratory of Cryosphere Science (SKLCS-ZZ-2015)the Foundation for Excellent Youth Scholars of Northwest Institute of Eco-Environment and Resources, CAS
文摘Light-absorbing impurities on glaciers are important factors that influence glacial surface albedo and accelerate glacier melt. In this study, the quantity of light-absorbing impurities on Keqikaer Glacier in western Tien Shan, Central Asia, was measured. We found that the average concentrations of black carbon was 2,180 ng/g, with a range from 250 ng/g to more than 10,000 ng/g. The average concentrations of organic carbon and mineral dust were 1,738 ng/g and 194 μg/g, respectively. Based on simulations performed with the Snow Ice Aerosol Radiative model simulations, black carbon and dust are responsible for approximately 64% and 9%, respectively, of the albedo reduction, and are associated with instantaneous radiative forcing of 323.18 W/m2(ranging from 142.16 to 619.25 W/m2) and 24.05 W/m2(ranging from 0.15 to69.77 W/m2), respectively. For different scenarios, the albedo and radiative forcing effect of black carbon is considerably greater than that of dust. The estimated radiative forcing at Keqikaer Glacier is higher than most similar values estimated by previous studies on the Tibetan Plateau, perhaps as a result of black carbon enrichment by melt scavenging. Light-absorbing impurities deposited on Keqikaer Glacier appear to mainly originate from central Asia, Siberia, western China(including the Taklimakan Desert) and parts of South Asia in summer, and from the Middle East and Central Asia in winter.A footprint analysis indicates that a large fraction(>60%) of the black carbon contributions on Keqikaer Glacier comes from anthropogenic sources. These results provide a scientific basis for regional mitigation efforts to reduce black carbon.
基金supported by the U.S.Department of Energy, Office of Science, Biological and Environmental Research, as part of the Earth System Modeling ProgramThe NASA Modeling, Analysis, and Prediction (MAP) Program by the Science Mission Directorate at NASA Headquarters supported the work contributed by Teppei J.YASUNARI and William K.M.LAU+2 种基金The NASA GEOS-5 simulation was implemented in the system for NASA Center for Climate Simulation (NCCS).M.G.Flanner was partially supported by NSF 1253154support from the China Scholarship FundThe Pacific Northwest National Laboratory is operated for DOE by Battelle Memorial Institute under contract DE-AC06-76RLO1830
文摘Light absorbing particles(LAP, e.g., black carbon, brown carbon, and dust) influence water and energy budgets of the atmosphere and snowpack in multiple ways. In addition to their effects associated with atmospheric heating by absorption of solar radiation and interactions with clouds, LAP in snow on land and ice can reduce the surface reflectance(a.k.a., surface darkening), which is likely to accelerate the snow aging process and further reduces snow albedo and increases the speed of snowpack melt. LAP in snow and ice(LAPSI) has been identified as one of major forcings affecting climate change, e.g.in the fourth and fifth assessment reports of IPCC. However, the uncertainty level in quantifying this effect remains very high. In this review paper, we document various technical methods of measuring LAPSI and review the progress made in measuring the LAPSI in Arctic, Tibetan Plateau and other mid-latitude regions. We also report the progress in modeling the mass concentrations, albedo reduction, radiative forcing, and climatic and hydrological impact of LAPSI at global and regional scales. Finally we identify some research needs for reducing the uncertainties in the impact of LAPSI on global and regional climate and the hydrological cycle.