A review of data-driven whole-life state of health prediction for lithium-ion batteries:Data preprocessing,aging characteristics,algorithms,and future challenges

Lithium-ion batteries are the preferred green energy storage method and are equipped with intelligent battery management systems(BMSs)that efficiently manage the batteries.This not only ensures the safety performance of the batteries but also significantly improves their efficiency and reduces their damage rate.Throughout their whole life cycle,lithium-ion batteries undergo aging and performance degradation due to diverse external environments and irregular degradation of internal materials.This degradation is reflected in the state of health(SOH)assessment.Therefore,this review offers the first comprehensive analysis of battery SOH estimation strategies across the entire lifecycle over the past five years,highlighting common research focuses rooted in data-driven methods.It delves into various dimensions such as dataset integration and preprocessing,health feature parameter extraction,and the construction of SOH estimation models.These approaches unearth hidden insights within data,addressing the inherent tension between computational complexity and estimation accuracy.To enha nce support for in-vehicle implementation,cloud computing,and the echelon technologies of battery recycling,remanufacturing,and reuse,as well as to offer insights into these technologies,a segmented management approach will be introduced in the future.This will encompass source domain data processing,multi-feature factor reconfiguration,hybrid drive modeling,parameter correction mechanisms,and fulltime health management.Based on the best SOH estimation outcomes,health strategies tailored to different stages can be devised in the future,leading to the establishment of a comprehensive SOH assessment framework.This will mitigate cross-domain distribution disparities and facilitate adaptation to a broader array of dynamic operation protocols.This article reviews the current research landscape from four perspectives and discusses the challenges that lie ahead.Researchers and practitioners can gain a comprehensive understanding of battery SOH estimation methods,offering valuable insights for the development of advanced battery management systems and embedded application research.

Accuracy comparison and improvement for state of health estimation of lithium-ion battery based on random partial recharges and feature engineering

State of health(SOH)estimation of e-mobilities operated in real and dynamic conditions is essential and challenging.Most of existing estimations are based on a fixed constant current charging and discharging aging profiles,which overlooked the fact that the charging and discharging profiles are random and not complete in real application.This work investigates the influence of feature engineering on the accuracy of different machine learning(ML)-based SOH estimations acting on different recharging sub-profiles where a realistic battery mission profile is considered.Fifteen features were extracted from the battery partial recharging profiles,considering different factors such as starting voltage values,charge amount,and charging sliding windows.Then,features were selected based on a feature selection pipeline consisting of filtering and supervised ML-based subset selection.Multiple linear regression(MLR),Gaussian process regression(GPR),and support vector regression(SVR)were applied to estimate SOH,and root mean square error(RMSE)was used to evaluate and compare the estimation performance.The results showed that the feature selection pipeline can improve SOH estimation accuracy by 55.05%,2.57%,and 2.82%for MLR,GPR and SVR respectively.It was demonstrated that the estimation based on partial charging profiles with lower starting voltage,large charge,and large sliding window size is more likely to achieve higher accuracy.This work hopes to give some insights into the supervised ML-based feature engineering acting on random partial recharges on SOH estimation performance and tries to fill the gap of effective SOH estimation between theoretical study and real dynamic application.

State of health prediction for lithium-ion batteries based on ensemble Gaussian process regression

The performance of lithium-ion batteries(LIBs)gradually declines over time,making it critical to predict the battery’s state of health(SOH)in real-time.This paper presents a model that incorporates health indicators and ensemble Gaussian process regression(EGPR)to predict the SOH of LIBs.Firstly,the degradation process of an LIB is analyzed through indirect health indicators(HIs)derived from voltage and temperature during discharge.Next,the parameters in the EGPR model are optimized using the gannet optimization algorithm(GOA),and the EGPR is employed to estimate the SOH of LIBs.Finally,the proposed model is tested under various experimental scenarios and compared with other machine learning models.The effectiveness of EGPR model is demonstrated using the National Aeronautics and Space Administration(NASA)LIB.The root mean square error(RMSE)is maintained within 0.20%,and the mean absolute error(MAE)is below 0.16%,illustrating the proposed approach’s excellent predictive accuracy and wide applicability.

Statistical Models for Condition Monitoring and State of Health Estimation of Lithium-Ion Batteries for Ships

Battery systems are increasingly being used for powering ocean going ships,and the number of fully electric or hybrid ships relying on battery power for propulsion is growing.To ensure the safety of such ships,it is important to monitor the available energy that can be stored in the batteries,and classification societies typically require the state of health(SOH)to be verified by independent tests.This paper addresses statistical modeling of SOH for maritime lithium-ion batteries based on operational sensor data.Various methods for sensor-based,data-driven degradation monitoring will be presented,and advantages and challenges with the different approaches will be discussed.The different approaches include cumulative degradation models and snapshot models,models that need to be trained and models that need no prior training,and pure data-driven models and physics-informed models.Some of the methods only rely on measured data,such as current,voltage,and temperature,whereas others rely on derived quantities such as state of charge.Models include simple statistical models and more complicated machine learning techniques.Insight from this exploration will be important in establishing a framework for data-driven diagnostics and prognostics of maritime battery systems within the scope of classification societies.

A review of deep learning approach to predicting the state of health and state of charge of lithium-ion batteries

In the field of energy storage,it is very important to predict the state of charge and the state of health of lithium-ion batteries.In this paper,we review the current widely used equivalent circuit and electrochemical models for battery state predictions.The review demonstrates that machine learning and deep learning approaches can be used to construct fast and accurate data-driven models for the prediction of battery performance.The details,advantages,and limitations of these approaches are presented,compared,and summarized.Finally,future key challenges and opportunities are discussed.

End-cloud collaboration method enables accurate state of health and remaining useful life online estimation in lithium-ion batteries

Though the lithium-ion battery is universally applied,the reliability of lithium-ion batteries remains a challenge due to various physicochemical reactions,electrode material degradation,and even thermal runaway.Accurate estimation and prediction of battery health conditions are crucial for battery safety management.In this paper,an end-cloud collaboration method is proposed to approach the track of battery degradation process,integrating end-side empirical model with cloud-side data-driven model.Based on ensemble learning methods,the data-driven model is constructed by three base models to obtain cloud-side highly accurate results.The double exponential decay model is utilized as an empirical model to output highly real-time prediction results.With Kalman filter,the prediction results of end-side empirical model can be periodically updated by highly accurate results of cloud-side data-driven model to obtain highly accurate and real-time results.Subsequently,the whole framework can give an accurate prediction and tracking of battery degradation,with the mean absolute error maintained below 2%.And the execution time on the end side can reach 261μs.The proposed end-cloud collaboration method has the potential to approach highly accurate and highly real-time estimation for battery health conditions during battery full life cycle in architecture of cyber hierarchy and interactional network.

Boosting battery state of health estimation based on self-supervised learning

State of health(SoH) estimation plays a key role in smart battery health prognostic and management.However,poor generalization,lack of labeled data,and unused measurements during aging are still major challenges to accurate SoH estimation.Toward this end,this paper proposes a self-supervised learning framework to boost the performance of battery SoH estimation.Different from traditional data-driven methods which rely on a considerable training dataset obtained from numerous battery cells,the proposed method achieves accurate and robust estimations using limited labeled data.A filter-based data preprocessing technique,which enables the extraction of partial capacity-voltage curves under dynamic charging profiles,is applied at first.Unsupervised learning is then used to learn the aging characteristics from the unlabeled data through an auto-encoder-decoder.The learned network parameters are transferred to the downstream SoH estimation task and are fine-tuned with very few sparsely labeled data,which boosts the performance of the estimation framework.The proposed method has been validated under different battery chemistries,formats,operating conditions,and ambient.The estimation accuracy can be guaranteed by using only three labeled data from the initial 20% life cycles,with overall errors less than 1.14% and error distribution of all testing scenarios maintaining less than 4%,and robustness increases with aging.Comparisons with other pure supervised machine learning methods demonstrate the superiority of the proposed method.This simple and data-efficient estimation framework is promising in real-world applications under a variety of scenarios.

Estimating the State of Health for Lithium-ion Batteries:A Particle Swarm Optimization-Assisted Deep Domain Adaptation Approach

The state of health(SOH)is a critical factor in evaluating the performance of the lithium-ion batteries(LIBs).Due to various end-user behaviors,the LIBs exhibit different degradation modes,which makes it challenging to estimate the SOHs in a personalized way.In this article,we present a novel particle swarm optimization-assisted deep domain adaptation(PSO-DDA)method to estimate the SOH of LIBs in a personalized manner,where a new domain adaptation strategy is put forward to reduce cross-domain distribution discrepancy.The standard PSO algorithm is exploited to automatically adjust the chosen hyperparameters of developed DDA-based method.The proposed PSODDA method is validated by extensive experiments on two LIB datasets with different battery chemistry materials,ambient temperatures and charge-discharge configurations.Experimental results indicate that the proposed PSO-DDA method surpasses the convolutional neural network-based method and the standard DDA-based method.The Py Torch implementation of the proposed PSO-DDA method is available at https://github.com/mxt0607/PSO-DDA.

Estimation of state of health based on charging characteristics and back-propagation neural networks with improved atom search optimization algorithm

With the rapid development of new energy technologies, lithium batteries are widely used in the field of energy storage systems and electric vehicles. The accurate prediction for the state of health(SOH) has an important role in maintaining a safe and stable operation of lithium-ion batteries. To address the problems of uncertain battery discharge conditions and low SOH estimation accuracy in practical applications, this paper proposes a SOH estimation method based on constant-current battery charging section characteristics with a back-propagation neural network with an improved atom search optimization algorithm. A temperature characteristic, equal-time temperature variation(Dt_DT), is proposed by analyzing the temperature data of the battery charging section with the incremental capacity(IC) characteristics obtained from an IC analysis as an input to the data-driven prediction model. Testing and analysis of the proposed prediction model are carried out using publicly available datasets. Experimental results show that the maximum error of SOH estimation results for the proposed method in this paper is below 1.5%.

Lithium battery state of charge and state of health prediction based on fuzzy Kalman filtering

This paper presents a more accurate battery state of charge(SOC)and state of health(SOH)estimation method.A lithium battery is represented by a nonlinear two-order resistance-capacitance equivalent circuit model.The model parameters are estimated by searching least square error optimization algorithm.Precisely defined by this method,the model parameters allow to accurately determine the capacity of the battery,which in turn allows to specify the SOC prediction value used as a basis for the SOH value.Application of the extended Kalman filter(EKF)removes the need of prior known initial SOC,and applying the fuzzy logic helps to eliminate the measurement and process noise.Simulation results obtained during the urban dynamometer driving schedule(UDDS)test show that the maximum error in estimation of the battery SOC is 0.66%.Battery capacity is estimate by offline updated Kalman filter,and then SOH will be predicted.The maximum error in estimation of the battery capacity is 1.55%.

Estimation of Battery State of Health Using Back Propagation Neural Network

100 pieces of 26650-type Lithium iron phosphate（LiFePO4） batteries cycled with a fixed charge and discharge rate are tested, and the influence of the battery internal resistance and the instantaneous voltage drop at the start of discharge on the state of health（SOH） is discussed. A back propagation（BP） neural network model using additional momentum is built up to estimate the state of health of Li-ion batteries. The additional 10 pieces are used to verify the feasibility of the proposed method. The results show that the neural network prediction model have a higher accuracy and can be embedded into battery management system（BMS） to estimate SOH of LiFePO4 Li-ion batteries.

State of Health Estimation of LiFePO_(4) Batteries for Battery Management Systems

When considering the mechanism of the batteries,the capacity reduction at storage(when not in use)and cycling(during use)and increase of internal resistance is because of degradation in the chemical composition inside the batteries.To optimize battery usage,a battery management system(BMS)is used to estimate possible aging effects while different load profiles are requested from the grid.This is specifically seen in a case when the vehicle is connected to the net(online through BMS).During this process,the BMS chooses the optimized load profiles based on the least aging effects on the battery pack.The major focus of this paper is to design an algorithm/model for lithium iron phosphate(LiFePO4)batteries.The model of the batteries is based on the accelerated aging test data(data from the beginning of life till the end of life).The objective is to develop an algorithm based on the actual battery trend during the whole life of the battery.By the analysis of the test data,the complete trend of the battery aging and the factors on which the aging is depending on is identified,the aging model can then be recalibrated to avoid any differences in the production process during cell manufacturing.The validation of the model was carried out at the end by utilizing different driving profiles at different C-rates and different ambient temperatures.A Linear and non-linear model-based approach is used based on statistical data.The parameterization was carried out by dividing the data into small chunks and estimating the parameters for the individual chunks.Self-adaptive characteristic map using a lookup table was also used.The nonlinear model was chosen as the best candidate among all other approaches for longer validation of 8-month data with real driving data set.

State of Health Estimation of Lithium-Ion Batteries Using Support Vector Regression and Long Short-Term Memory

Lithium-ion batteries are the most widely accepted type of battery in the electric vehicle industry because of some of their positive inherent characteristics. However, the safety problems associated with inaccurate estimation and prediction of the state of health of these batteries have attracted wide attention due to the adverse negative effect on vehicle safety. In this paper, both machine and deep learning models were used to estimate the state of health of lithium-ion batteries. The paper introduces the definition of battery health status and its importance in the electric vehicle industry. Based on the data preprocessing and visualization analysis, three features related to actual battery capacity degradation are extracted from the data. Two learning models, SVR and LSTM were employed for the state of health estimation and their respective results are compared in this paper. The mean square error and coefficient of determination were the two metrics for the performance evaluation of the models. The experimental results indicate that both models have high estimation results. However, the metrics indicated that the SVR was the overall best model.

Estimating battery state of health with 10-min relaxation voltage across various charging states of charge

Battery capacity assessment is a crucial research direction in the field of lithium-ion battery applications.In the previous research,a novel data-driven state of health(SOH)estimation method based on the voltage relaxation curve at full charging is developed.The experimental results have shown the evidence of the superiority of accurate battery SOH estimation based on physical features derived from equivalent circuit models(ECMs).However,the earlier research has limitations in estimating battery capacity with a diversity of battery charging states of charge.This study represents an extension of the previous work,aiming to investigate the feasibility of this technology for battery degradation evaluation under various charging states so that the application capability in practice is enhanced.In this study,six ECM features are extracted from 10-min voltage relaxation data across varying charging states to characterize the battery degradation evolution.Gaussian process regression(GPR)is employed to learn the relationship between the physical features and battery SOH.Experimental results under 10 different state of charge(SOC)ranges show that the developed methodology predicts accurate battery SOH,with a root mean square error being 0.9%.

A new multi-dimensional state of health evaluation method for lithium-ion batteries

Electric vehicles and battery energy storage are effective technical paths to achieve carbon neutrality,and lithium-ion batteries(LiBs)are very critical energy storage devices,which is of great significance to the goal.However,the battery’s characteristics of instant degradation seriously affect its long life and high safety applications.The aging mechanisms of LiBs are complex and multi-faceted,strongly influenced by numerous interacting factors.Currently,the degree of capacity fading is commonly used to describe the aging of the battery,and the ratio of the maximum available capacity to the rated capacity of the battery is defined as the state of health(SOH).However,the aging or health of the battery should be multifaceted.To realize the multi-dimensional comprehensive evaluation of battery health status,a novel SOH estimation method driven by multidimensional aging characteristics is proposed through the improved single-particle model.The parameter identification and sensitivity analysis of the model were carried out during the whole cycle of life in a wide temperature environment.Nine aging characteristic parameters were obtained to describe the SOH.Combined with aging mechanisms,the current health status was evaluated from four aspects:capacity level,lithium-ion dif-fusion,electrochemical reaction,and power capacity.The proposed method can more comprehensively evaluate the aging charac-teristics of batteries,and the SOH estimation error is within 2%.

Machine learning and neural network supported state of health simulation and forecasting model for lithium-ion battery

As the intersection of disciplines deepens,the field of battery modeling is increasingly employing various artificial intelligence(AI)approaches to improve the efficiency of battery management and enhance the stability and reliability of battery operation.This paper reviews the value of AI methods in lithium-ion battery health management and in particular analyses the application of machine learning(ML),one of the many branches of AI,to lithium-ion battery state of health(SOH),focusing on the advantages and strengths of neural network(NN)methods in ML for lithium-ion battery SOH simulation and prediction.NN is one of the important branches of ML,in which the application of NNs such as backpropagation NN,convolutional NN,and long short-term memory NN in SOH estimation of lithium-ion batteries has received wide attention.Reports so far have shown that the utilization of NN to model the SOH of lithium-ion batteries has the advantages of high efficiency,low energy consumption,high robustness,and scalable models.In the future,NN can make a greater contribution to lithium-ion battery management by,first,utilizing more field data to play a more practical role in health feature screening and model building,and second,by enhancing the intelligent screening and combination of battery parameters to characterize the actual lithium-ion battery SOH to a greater extent.The in-depth application of NN in lithium-ion battery SOH will certainly further enhance the science,reliability,stability,and robustness of lithium-ion battery management.

Transfer learning from synthetic data for open-circuit voltage curve reconstruction and state of health estimation of lithium-ion batteries from partial charging segments

Data-driven models for battery state estimation require extensive experimental training data,which may not be available or suitable for specific tasks like open-circuit voltage(OCV)reconstruction and subsequent state of health(SOH)estimation.This study addresses this issue by developing a transfer-learning-based OCV reconstruction model using a temporal convolutional long short-term memory(TCN-LSTM)network trained on synthetic data from an automotive nickel cobalt aluminium oxide(NCA)cell generated through a mechanistic model approach.The data consists of voltage curves at constant temperature,C-rates between C/30 to 1C,and a SOH-range from 70%to 100%.The model is refined via Bayesian optimization and then applied to four use cases with reduced experimental nickel manganese cobalt oxide(NMC)cell training data for higher use cases.The TL models’performances are compared with models trained solely on experimental data,focusing on different C-rates and voltage windows.The results demonstrate that the OCV reconstruction mean absolute error(MAE)within the average battery electric vehicle(BEV)home charging window(30%to 85%state of charge(SOC))is less than 22 mV for the first three use cases across all C-rates.The SOH estimated from the reconstructed OCV exhibits an mean absolute percentage error(MAPE)below 2.2%for these cases.The study further investigates the impact of the source domain on TL by incorporating two additional synthetic datasets,a lithium iron phosphate(LFP)cell and an entirely artificial,non-existing,cell,showing that solely the shifting and scaling of gradient changes in the charging curve suffice to transfer knowledge,even between different cell chemistries.A key limitation with respect to extrapolation capability is identified and evidenced in our fourth use case,where the absence of such comprehensive data hindered the TL process.

State-of-health estimation for fast-charging lithium-ion batteries based on a short charge curve using graph convolutional and long short-term memory networks

A fast-charging policy is widely employed to alleviate the inconvenience caused by the extended charging time of electric vehicles. However, fast charging exacerbates battery degradation and shortens battery lifespan. In addition, there is still a lack of tailored health estimations for fast-charging batteries;most existing methods are applicable at lower charging rates. This paper proposes a novel method for estimating the health of lithium-ion batteries, which is tailored for multi-stage constant current-constant voltage fast-charging policies. Initially, short charging segments are extracted by monitoring current switches,followed by deriving voltage sequences using interpolation techniques. Subsequently, a graph generation layer is used to transform the voltage sequence into graphical data. Furthermore, the integration of a graph convolution network with a long short-term memory network enables the extraction of information related to inter-node message transmission, capturing the key local and temporal features during the battery degradation process. Finally, this method is confirmed by utilizing aging data from 185 cells and 81 distinct fast-charging policies. The 4-minute charging duration achieves a balance between high accuracy in estimating battery state of health and low data requirements, with mean absolute errors and root mean square errors of 0.34% and 0.66%, respectively.

Data-driven strategy for state of health prediction and anomaly detection in lithium-ion batteries

This study addresses the crucial challenge of monitoring the State of Health(SOH)of Lithium-Ion Batteries(LIBs)in response to the escalating demand for renewable energy systems and the imperative to reduce CO2 emissions.The research introduces deep learning(DL)models,namely Encoder-Long Short-Term Memory(E-LSTM)and Convolutional Neural Network-LSTM(CNN–LSTM),each designed to forecast battery SOH.E-LSTM integrates an encoder for dimensionality reduction and an LSTM model to capture data dependencies.CNN–LSTM,on the other hand,employs CNN layers for encoding followed by LSTM layers for precise SOH estimation.Significantly,we prioritize model explainability by employing a game-theoretic approach known as SHapley Additive exPlanations(SHAP)to elucidate the output of our models.Furthermore,a method based on pattern mining was developed,synergizing with the model,to identify patterns contributing to abnormal SOH decrease.These insights are presented through informative plots.The proposed approach relies on the battery dataset from the Massachusetts Institute of Technology(MIT)and showcases promising results in accurately estimating SOH values,in which the E-LSTM model outperformed the CNN–LSTM model with a Mean Absolute Error(MAE)of less than 1%.

Enhanced vision-transformer integrating with semi-supervised transfer learning for state of health and remaining useful life estimation of lithium-ion batteries

The state of health(SOH)and remaining useful life(RUL)of lithium-ion batteries are crucial for health management and diagnosis.However,most data-driven estimation methods heavily rely on scarce labeled data,while traditional transfer learning faces challenges in handling domain shifts across various battery types.This paper proposes an enhanced vision-transformer integrating with semi-supervised transfer learning for SOH and RUL estimation of lithium-ion batteries.A depth-wise separable convolutional vision-transformer is developed to extract local aging details with depth-wise convolutions and establishes global dependencies between aging information using multi-head attention.Maximum mean discrepancy is employed to initially reduce the distribution difference between the source and target domains,providing a superior starting point for fine-tuning the target domain model.Subsequently,the abundant aging data of the same type as the target battery are labeled through semi-supervised learning,compensating for the source model's limitations in capturing target battery aging characteristics.Consistency regularization incorporates the cross-entropy between predictions with and without adversarial perturbations into the gradient backpropagation of the overall model.In particular,across the experimental groups 13–15 for different types of batteries,the root mean square error of SOH estimation was less than 0.66%,and the mean relative error of RUL estimation was 3.86%.Leveraging extensive unlabeled aging data,the proposed method could achieve accurate estimation of SOH and RUL.