We report the fabrication and optical characterization of spherical whispering gallery mode(WGM) resonators made from ultraviolet(UV)-curable adhesive. The fabricated microspheres have good sphericity and surface smoo...We report the fabrication and optical characterization of spherical whispering gallery mode(WGM) resonators made from ultraviolet(UV)-curable adhesive. The fabricated microspheres have good sphericity and surface smoothness, and can directly adhere to the tip of half-tapered fibers for easy manipulation. WGMs are e?ciently excited in the microsphere using an evanescent field of the tapered silica optical fibers. Resonances with quality factors of 1.3×10 5 are observed. The dependence of wavelength shifts of WGM resonances on the input light powers shows that the resonant wavelength of the proposed microsphere resonators can be tuned thermo-optically.展开更多
Conventionally, metallic nanostructures are used for surface-enhanced Raman spectroscopy(SERS), but recently there has been increasing interest in the enhancement of Raman scattering from dielectric substrates due to ...Conventionally, metallic nanostructures are used for surface-enhanced Raman spectroscopy(SERS), but recently there has been increasing interest in the enhancement of Raman scattering from dielectric substrates due to their improved stability and biocompatibility compared with metallic substrates. Here, we report the observation of enhanced Raman scattering from rhodamine 6 G molecules coated on silica microspheres. We excite the whispering gallery modes(WGMs) supported in the microspheres with a tapered fiber coupler for efficient WGM excitation, and the Raman enhancement can be attributed to the WGM mechanism. Strong resonance enhancement in pump laser intensity and modified Raman emission from the Purcell effect in the microsphere resonator are observed from the experiment and compared with theoretical results. A total Raman enhancement factor of 1.4 × 10~4 is observed, with contribution mostly from the enhancement in pump laser intensity. Our results show that, with an efficient pumping scheme, dielectric microspheres are a viable alternative to metallic SERS substrates.展开更多
Optical whispering gallery microcavities with high-quality factors have shown great potential toward achieveing ultrahigh-sensitivity sensing up to a single molecule or nanoparticle, which raises a huge demand on a de...Optical whispering gallery microcavities with high-quality factors have shown great potential toward achieveing ultrahigh-sensitivity sensing up to a single molecule or nanoparticle, which raises a huge demand on a deep theoretical insight into the crucial phenomena such as the mode shift, mode splitting, and mode broadening in sensing experiments. Here we propose an intuitive model to analyze these phenomena from the viewpoint of the nanoparticle-induced multiple scattering of the azimuthally propagating mode(APM). The model unveils explicit relations between these phenomena and the phase change and energy loss of the APM when scattered at the nanoparticle; the model also explains the observed polarization-dependent preservation of one resonance and the particle-dependent redshift or blueshift. The model indicates that the particle-induced coupling between the pair of unperturbed degenerate whispering gallery modes(WGMs) and the coupling between the WGMs and the free-space radiation modes, which are widely adopted in current theoretical formalisms, are realized via the reflection and scattering-induced free-space radiation of the APM, respectively, and additionally exhibits the contribution of cross coupling between the unperturbed WGMs and other different WGMs to forming the splittingresonant modes, especially for large particles.展开更多
基金supported by the National Natural Science Foundation of China(No.61275050)the Specialized Research Fund for the Doctoral Program of Higher Education(No.20120121110034)the Fundamental Research Funds for the Central Universities of Xiamen University(Nos.2010121059 and 2011121048)
文摘We report the fabrication and optical characterization of spherical whispering gallery mode(WGM) resonators made from ultraviolet(UV)-curable adhesive. The fabricated microspheres have good sphericity and surface smoothness, and can directly adhere to the tip of half-tapered fibers for easy manipulation. WGMs are e?ciently excited in the microsphere using an evanescent field of the tapered silica optical fibers. Resonances with quality factors of 1.3×10 5 are observed. The dependence of wavelength shifts of WGM resonances on the input light powers shows that the resonant wavelength of the proposed microsphere resonators can be tuned thermo-optically.
基金National Science Foundation(NSF)(CBET1264750,CBET 1264997)Army Research Office(ARO)(W911NF-16-1-0339)
文摘Conventionally, metallic nanostructures are used for surface-enhanced Raman spectroscopy(SERS), but recently there has been increasing interest in the enhancement of Raman scattering from dielectric substrates due to their improved stability and biocompatibility compared with metallic substrates. Here, we report the observation of enhanced Raman scattering from rhodamine 6 G molecules coated on silica microspheres. We excite the whispering gallery modes(WGMs) supported in the microspheres with a tapered fiber coupler for efficient WGM excitation, and the Raman enhancement can be attributed to the WGM mechanism. Strong resonance enhancement in pump laser intensity and modified Raman emission from the Purcell effect in the microsphere resonator are observed from the experiment and compared with theoretical results. A total Raman enhancement factor of 1.4 × 10~4 is observed, with contribution mostly from the enhancement in pump laser intensity. Our results show that, with an efficient pumping scheme, dielectric microspheres are a viable alternative to metallic SERS substrates.
基金National Key Basic Research Program of China(2013CB328701)National Natural Science Foundation of China(NSFC)(61322508,11504270)
文摘Optical whispering gallery microcavities with high-quality factors have shown great potential toward achieveing ultrahigh-sensitivity sensing up to a single molecule or nanoparticle, which raises a huge demand on a deep theoretical insight into the crucial phenomena such as the mode shift, mode splitting, and mode broadening in sensing experiments. Here we propose an intuitive model to analyze these phenomena from the viewpoint of the nanoparticle-induced multiple scattering of the azimuthally propagating mode(APM). The model unveils explicit relations between these phenomena and the phase change and energy loss of the APM when scattered at the nanoparticle; the model also explains the observed polarization-dependent preservation of one resonance and the particle-dependent redshift or blueshift. The model indicates that the particle-induced coupling between the pair of unperturbed degenerate whispering gallery modes(WGMs) and the coupling between the WGMs and the free-space radiation modes, which are widely adopted in current theoretical formalisms, are realized via the reflection and scattering-induced free-space radiation of the APM, respectively, and additionally exhibits the contribution of cross coupling between the unperturbed WGMs and other different WGMs to forming the splittingresonant modes, especially for large particles.
