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High-throughput compositional mapping of triple-cation tin-lead perovskites for high-efficiency solar cells 被引量:1
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作者 Rajendra Kumar Gunasekaran Jina Jung +8 位作者 Sung Woong Yang Jungchul Yun Yeonghun Yun Devthade Vidyasagar Won Chang Choi Chang-Lyoul Lee Jun Hong Noh Dong Hoe Kim Sangwook Lee 《InfoMat》 SCIE CSCD 2023年第4期25-38,共14页
Mixed tin-ead perovskites suffer from structural instability and rapid tin oxidation;thus,the investigation of their optimal composition ranges is important to address these inherent weaknesses.The critical role of tr... Mixed tin-ead perovskites suffer from structural instability and rapid tin oxidation;thus,the investigation of their optimal composition ranges is important to address these inherent weaknesses.The critical role of triple cations in mixed Sn–Pb iodides is studied by performing a wide range of compositional screenings over mechanochemically synthesized bulk and solution-processed thin films.A ternary phase map of FA(Sn_(0.6)Pb_(0.4))I_(3),MA(Sn_(0.6)Pb_(0.4))I_(3),and Cs(Sn_(0.6)Pb_(0.4))I_(3)is formed,and a promising composition window of(FA_(0.6-x)MA_(0.4)Cs_(x))Sn_(0.6)Pb_(0.4)I_(3)(0≤x≤0.1)is demonstrated through phase,photoluminescence,and stability evaluations.Solar cell performance and chemical stability across the targeted compositional space are investigated,and FA_(0.55)MA_(0.4)Cs_(0.05)Sn_(0.6)Pb_(0.4)I_(3)with strain-relaxed lattices,reduced defect densities,and improved oxidation stability is demonstrated.The inverted perovskite solar cells with the optimal composition demonstrate a power conversion efficiency of over 22%with an open-circuit voltage of 0.867 V,which corresponds to voltage loss of 0.363 V,promising for the development of narrow-bandgap perovskite solar cells. 展开更多
关键词 compositional engineering mixed tin-ead iodides narrow-bandgap perovskites perovskite solar cells strain relaxation ternary phase mapping
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