Hohhot Plain, lying in the front of the Yingshan Mountains in inner Mongolia, isbounded by the mountain north, the Yellow River south, the Manhan Mountain east andloess hills southeast. Being 986 to 1100 meters above ...Hohhot Plain, lying in the front of the Yingshan Mountains in inner Mongolia, isbounded by the mountain north, the Yellow River south, the Manhan Mountain east andloess hills southeast. Being 986 to 1100 meters above ses level, the plain generally slopesdown to the southwest, just in accordance with the flowing direction of the Great Heihe Riv-er and the Small Heihe River.展开更多
In order to solve the problems including pipe corrosion, scaling and microbial growth, which severely threat safe op-eration of circulating cooling water system, this paper proposes ion exchange softening and alkaliza...In order to solve the problems including pipe corrosion, scaling and microbial growth, which severely threat safe op-eration of circulating cooling water system, this paper proposes ion exchange softening and alkalization process to solve these problems and carries out a series of studies to study the feasibility of ion exchange softening and alkaliza-tion process in the simulation process of circulating cooling water system. The studies include product water quality of ion exchange softening and alkalization process, effect on the performance of carbon steel and brass, and the inhibition that suppresses microbial growth. The results indicate that ion exchange softening and alkalization process is feasible to prevent the circulating cooling water system from scaling, pipe corrosion, and microbial growth without any other chemicals. Thus circulating cooling water system can achieve zerodischarge of wastewater.展开更多
Furfural residue, an industrial waste, is a kind of strongly acidic organic materials. Its comprehensive utilization in agriculture showed a significant effect on control of soil alkalization, amelioration of solonetz...Furfural residue, an industrial waste, is a kind of strongly acidic organic materials. Its comprehensive utilization in agriculture showed a significant effect on control of soil alkalization, amelioration of solonetz and increase of crop yields. In detail it may adjust pH, depress alkalinity, reduce bulk density and compactness and increase water permeability and retention ability of the soil. Meanwhile agricultural use of furfural residue provided an effective way to avoid its pollution of the soil, Water and air.展开更多
The novel calcium-silicate-hydrate(C-S-H)/paraffin composite phase change materials were synthesized using a discontinuous two-step nucleation method.Initially,the C-S-H precursor is separated and dried,followed by im...The novel calcium-silicate-hydrate(C-S-H)/paraffin composite phase change materials were synthesized using a discontinuous two-step nucleation method.Initially,the C-S-H precursor is separated and dried,followed by immersion in an aqueous environment to transform it into C-S-H.This two-step nucleation approach results in C-S-H with a specific surface area of 497.2 m^(2)/g,achieved by preventing C-S-H foil overlapping and refining its pore structure.When impregnated with paraffin,the novel C-S-H/paraffin composite exhibits superior thermal properties,such as a higher potential heat value of 148.3 J/g and an encapsulation efficiency of 81.6%,outperforming conventional C-S-H.Moreover,the composite material demonstrates excellent cyclic performance,indicating its potential for building thermal storage compared to other paraffin-based composites.Compared with the conventional method,this simple technology,which only adds conversion and centrifugation steps,does not negatively impact preparation costs,the environment,and resource consumption.This study provides valuable theoretical insights for designing thermal storage concrete materials and advancing building heat management.展开更多
A considerable efficiency gap exists between large-area perovskite solar modules and small-area perovskite solar cells.The control of forming uniform and large-area film and perovskite crystallization is still the mai...A considerable efficiency gap exists between large-area perovskite solar modules and small-area perovskite solar cells.The control of forming uniform and large-area film and perovskite crystallization is still the main obstacle restricting the efficiency of PSMs.In this work,we adopted a solid-liquid two-step film formation technique,which involved the evaporation of a lead iodide film and blade coating of an organic ammonium halide solution to prepare perovskite films.This method possesses the advantages of integrating vapor deposition and solution methods,which could apply to substrates with different roughness and avoid using toxic solvents to achieve a more uniform,large-area perovskite film.Furthermore,modification of the NiO_(x)/perovskite buried interface and introduction of Urea additives were utilized to reduce interface recombination and regulate perovskite crystallization.As a result,a large-area perovskite film possessing larger grains,fewer pinholes,and reduced defects could be achieved.The inverted PSM with an active area of 61.56 cm^(2)(10×10 cm^(2)substrate)achieved a champion power conversion efficiency of 20.56%and significantly improved stability.This method suggests an innovative approach to resolving the uniformity issue associated with large-area film fabrication.展开更多
Multiplicative noise removal problems have attracted much attention in recent years.Unlike additive noise,multiplicative noise destroys almost all information of the original image,especially for texture images.Motiva...Multiplicative noise removal problems have attracted much attention in recent years.Unlike additive noise,multiplicative noise destroys almost all information of the original image,especially for texture images.Motivated by the TV-Stokes model,we propose a new two-step variational model to denoise the texture images corrupted by multiplicative noise with a good geometry explanation in this paper.In the first step,we convert the multiplicative denoising problem into an additive one by the logarithm transform and propagate the isophote directions in the tangential field smoothing.Once the isophote directions are constructed,an image is restored to fit the constructed directions in the second step.The existence and uniqueness of the solution to the variational problems are proved.In these two steps,we use the gradient descent method and construct finite difference schemes to solve the problems.Especially,the augmented Lagrangian method and the fast Fourier transform are adopted to accelerate the calculation.Experimental results show that the proposed model can remove the multiplicative noise efficiently and protect the texture well.展开更多
In this work,a two-step metal organic chemical vapor deposition(MOCVD)method was applied for growingβ-Ga_(2)O_(3) film on c-plane sapphire.Optimized buffer layer growth temperature(T_(B))was found at 700℃ and theβ-...In this work,a two-step metal organic chemical vapor deposition(MOCVD)method was applied for growingβ-Ga_(2)O_(3) film on c-plane sapphire.Optimized buffer layer growth temperature(T_(B))was found at 700℃ and theβ-Ga_(2)O_(3) film with full width at half maximum(FWHM)of 0.66°was achieved.A metal−semiconductor−metal(MSM)solar-blind photodetector(PD)was fabricated based on theβ-Ga_(2)O_(3) film.Ultrahigh responsivity of 1422 A/W@254 nm and photo-to-dark current ratio(PDCR)of 10^(6) at 10 V bias were obtained.The detectivity of 2.5×10^(15) Jones proved that the photodetector has outstanding performance in detecting weak signals.Moreover,the photodetector exhibited superior wavelength selectivity with rejection ratio(R_(250 nm)/R_(400 nm))of 105.These results indicate that the two-step method is a promising approach for preparation of high-qualityβ-Ga_(2)O_(3)films for high-performance solar-blind photodetectors.展开更多
Inconel 718 is the most popular nickel-based superalloy and is extensively used in aerospace,automotive,and energy indus-tries owing to its extraordinary thermomechanical properties.The effects of different two-step s...Inconel 718 is the most popular nickel-based superalloy and is extensively used in aerospace,automotive,and energy indus-tries owing to its extraordinary thermomechanical properties.The effects of different two-step solid solution treatments on microstructure andδphase precipitation of Inconel 718 alloy were studied,and the transformation mechanism fromγ″metastable phase toδphase was clarified.The precipitates were statistically analyzed by X-ray diffractometry.The results show that theδphase content firstly increased,and then decreased with the temperature of the second-step solid solution.The changes in microstructure andδphase were studied by scanning electron microscopy and transmission electron microscopy.An intragranularδphase formed in Inconel 718 alloy at the second-[100]_(δ)[011]γ step solid solution temperature of 925℃,and its orientation relationship withγmatrix was determined as//and(010)_(δ)//(111)γ.Furthermore,the Vickers hardness of different heat treatment samples was measured,and the sample treated by second-step solid solution at 1010℃ reached the maximum hardness of HV 446.84.展开更多
Diamonds on the Earth mainly occur in volcanic rocks such as kimberlites and lamproites^([1-8]),but can also be found in ultrahigh-pressure metamorphic rocks^([9-10]),meteorites^([11])and alluvial deposits^([12]).In r...Diamonds on the Earth mainly occur in volcanic rocks such as kimberlites and lamproites^([1-8]),but can also be found in ultrahigh-pressure metamorphic rocks^([9-10]),meteorites^([11])and alluvial deposits^([12]).In recent years,diamonds have been recovered from ophiolites^([13-16])and alkalic dolerites^([17-18]).The discovery of ophiolitic diamonds and alkalic dolerites diamonds has drawn significant research interests to explore the origin of this new class of diamond source and to infer the evolution of their hosting rocks[^(19-21)].This new type of diamond had been initially considered as a result of contamination.However,more and more evidences either directly or indirectly demonstrate that these diamonds are of natural origin^([16,18,19,22-24]).During a geological survey from 2012 to 2015,the geologists from Nanjing Centre of China Geological Survey discovered a large number of yellow microdiamonds in the Langan area in northern Anhui Province^([18,25-29]).The diamond-bearing rocks of these microdiamonds mainly include dolerite and olivine basalt.From 2016 to 2018,four microdiamonds in basic rocks were recovered again in the prospecting work for primary diamond deposits in the Tashan and Zhangji areas in Xuzhou,which is geographically close to Langan[30].All these microdiamonds are similar in colour and shape to ophiolite type diamonds^([31]),and show different characteristics of kimberlite and lamproite type diamonds.Cai,et al.(2019)reported the petrological characteristics of the diamondiferous rocks^([17,21,30]).In this paper,the morphology,infrared spectrum,and carbon isotope compositions of microdiamonds were analysed and discussed by Fourier infrared spectroscopy and carbon isotope test.The types of microdiamonds found in the North China Craton,the age of mantle occurrence,and the source of carbon isotopes were revealed.In the past,many deposits of macro-diamonds,mostly of TypeⅠa orⅡa,were found in the North China Craton,and they have been extensively studied.Microdiamonds recovered from the alkalic dolerites of the North China Craton were studied by FTIR and carbon isotopic.These diamonds are usually light yellow to yellow,with a few colourless,and cubic,octahedral or rhomboidal dodecahedron,and octahedron in shape.The surface characteristics of diamonds,such as dissolution,can be observed.The overall N concentration is not high,with an average of 173×10^(-6).The infrared spectra show that most of these diamonds are TypeⅠb,and C centres are found at 1344 cm^(-1).Three diamond samples are classified as TypeⅠa/Ⅰb,because of A centres and C centres in these diamonds.Two diamonds are classified as typeⅠaAB because B,B′and A centres are found co-existing.FTIR microscopic measurements from the core to the edge of the TypeⅠaAB diamond suggest a mantle residence time of approximately 550 Ma.The C isotopic analysis reveals that these diamonds are strongly depleted in 13 C.These lowδ^(13) C values of dolerites-hosted diamonds overlap with the lower ends of peridotitic diamonds and metamorphic diamonds,and the upper end of the ophiolitic diamonds.Additionally,the reason for the strong deficitδ^(13) C shown by the carbon isotope should be studied in the future.展开更多
In order to improve the bio-oxidation efficiency of Axi refractory gold concentrate, a two-step process including a high temperature chemical oxidation and a subsequent bio-oxidation, combined with p H control during ...In order to improve the bio-oxidation efficiency of Axi refractory gold concentrate, a two-step process including a high temperature chemical oxidation and a subsequent bio-oxidation, combined with p H control during the bio-oxidation step was used. The results revealed that the optimum mode was to maintain solution p H at 1.0-1.2 during the biological oxidation stage. Under this condition, the activity of mixed culture could be sustained and the formation of jarosite could be diminished, thus the oxidation efficiency was improved. The oxidation levels of iron and sulfur were improved by 12.50% and 15.49%, and the gold recovery was increased by 21.02%. Therefore, the two-step process combined with p H control is an effective method for oxidizing the biohydrometallurgical process of Axi gold concentrate, and it will have a broad prospect of application in dealing with complex refractory gold concentrate.展开更多
[Objective] For preparing the biopesticide of Bacillus subtilis B579 with high spore concentration,the sporulation conditions were optimized.[Method] Two-step fermentation control strategy was used,in which,the first ...[Objective] For preparing the biopesticide of Bacillus subtilis B579 with high spore concentration,the sporulation conditions were optimized.[Method] Two-step fermentation control strategy was used,in which,the first phase(0-10 h)was to improve cell growth,and the second phase(10-30 h)was to promote spore formation.Four factors including initial glucose concentration,fermentation pH,temperature(in the second phase)and shaking speed(in the second phase)were optimized using the methods of single factor test and orthogonal experiment.[Result] The initial glucose concentration showed a significant effect on sporulation.The optimal conditions for the spore formation of B.subtilis B579 were as follows:initial glucose concentration 5 g/L,fermentation pH 7.0,the temperature for the first phase 37 ℃,and the shaking speed for the first phase 180 r/min,the temperature for the second phase 40 ℃,and the shaking speed for the second phase 200 r/min;in addition,the first phase was 10 h and the second phase of fermentation was conducted for 30 h.Under such conditions,the spore concentration and spore formation rate could reach 9.43×108 CFU/ml and 90.99%,respectively,which represented 6.70-fold and 2.43-fold increase compared with those before optimization.[Conclusion] The spores concentration of biocontrol agent was improved using two-step control strategy,which provided the basis for biopesticide production in large scale.展开更多
The accelerating factor (AF) method is a simple and appropriate way to investigate the atomic long-time deep diffusion at solid-solid interface. In the framework of AF hyperdynamics (HD) simulation, the relationsh...The accelerating factor (AF) method is a simple and appropriate way to investigate the atomic long-time deep diffusion at solid-solid interface. In the framework of AF hyperdynamics (HD) simulation, the relationship between the diffusion coefficient along the direction of z-axis which is normal to the Mg/Zn interface and temperature was investigated, and the AF's impact on the diffusion constant (D0) and activation energy (Q^*) was studied. Then, two steps were taken to simulate the atomic diffusion process and the formation of new phases: one for acceleration and the other for equilibration. The results show that: the Arrhenius equation works well for the description of Dz with different accelerating factors; the AF has no effect on the diffusion constant Do in the case of no phase transition; and the relationship between Q* and Q conforms to Q^*=Q/A. Then, the new Arrhenius equation for AFHD is successfully constructed as Dz=Doexp[-Q/(ART)]. Meanwhile, the authentic equilibrium conformations at any dynamic moment can only be reproduced by the equilibration simulation of the HD-simulated configurations. Key words: accelerating factor method; Arrhenius equation; two-steps scheme; Mg/Zn interface; hyperdynamic simulation展开更多
Using Object-oriented design and a new programming language JAVA, a physically-based model was built to simulate the hydrological, alkalization/de-alkalization and salinization/desalinization processes in soil. Furthe...Using Object-oriented design and a new programming language JAVA, a physically-based model was built to simulate the hydrological, alkalization/de-alkalization and salinization/desalinization processes in soil. Furthermore, a process-based model was built to evaluate the dynamics of four herbaceous ecosystems (including dynamics of above-ground biomass, below-ground biomass, and litter biomass), each dominated by Aneurolepidium chinense (Trin.) Kitag., Chloris virgata Sw., Puccinellia tenuiflora (Turcz.) Scribn. et Merr. and Suaeda glauca Bunge. This model is a daily-time step model, suitable for simulating hydrological, alkalization/de-alkalization and salinization/desalinization processes of heterogeneous soil, and growth dynamics of different grassland communities. With climatic data and experimental data of Changling Experimental Site in Jilin Province, the soil moisture content (in 1991, 1996, 1997 and 1998), soil salt concentration, exchangeable cation percentage and pH in soil and growth dynamics of these four sorts of grassland communities (in 1991) were simulated and the results were verified to be in accord with observed data.展开更多
We propose a two-step quantum secure direct communication (QSDC) protocol with hyperentanglement in both the spatial-mode and the polarization degrees of freedom of photon pairs which can in principle be produced wi...We propose a two-step quantum secure direct communication (QSDC) protocol with hyperentanglement in both the spatial-mode and the polarization degrees of freedom of photon pairs which can in principle be produced with a beta barium borate crystal. The secret message can be encoded on the photon pairs with unitary operations in these two degrees of freedom independently. This QSDC protocol has a higher capacity than the original two-step QSDC protocol as each photon pair can carry 4 bits of information. Compared with the QSDC protocol based on hyperdense coding, this QSDC protocol has the immunity to Trojan horse attack strategies with the process for determining the number of the photons in each quantum signal as it is a one-way quantum communication protocol.展开更多
The effects of the two-step ageing parameters (temperature and time) on the mechanical properties and electrical conductivity of 7B04 (A1-Zn-Mg-Cu) pre-stretched thick plates were studied. The results reveal that ...The effects of the two-step ageing parameters (temperature and time) on the mechanical properties and electrical conductivity of 7B04 (A1-Zn-Mg-Cu) pre-stretched thick plates were studied. The results reveal that the initial T1 ageing contributes a major increase of the tensile strength, and the 0.2% proof stress value reaches 482 MPa after ageing for 7 h at 115℃. Behavioral differences in the tensile properties of the alloy after the two-step ageing treatment were less with the first-step ageing at 115~C for different time periods (7, 14, and 21 h). The effects of the second ageing parameters on the properties and microstructure of the 7B04 alloy were remarkable. TEM analysis of the samples aged at Temper I (7 h at 115℃ + 12 h at 160℃) and Temper II (7 h at 115℃ + 16 h at 165℃) indicates that two kinds of phases, i.e. 11' and 11 phases, precipitate from the matrix and efficiently improve the tensile strength of the alloy, and the grain boundary precipitates are coarse and discrete. There are obvious precipitate free zones (PFZs) along the grain boundary in the microstructure of the alloy after the two-step ageing treatment.展开更多
Gametophytes of Laminaria japonica were cryopreserved in liquid nitrogen using encapsulation-dehydration with two-step cooling method. Gametophytes cultured at 10℃ and under continuous irradiance of 30 μmol m^-2 s^-...Gametophytes of Laminaria japonica were cryopreserved in liquid nitrogen using encapsulation-dehydration with two-step cooling method. Gametophytes cultured at 10℃ and under continuous irradiance of 30 μmol m^-2 s^-1 for 3 weeks were encapsulated in calcium alginate beads. The beads were dehydrated in 0.4 molLl sucrose prepared with seawater for 6 h, desiccated in an incubator set at 10℃ and 70% relative humidity for 4 h, pre-frozen at either -40℃ or -60℃ for 30 min, and stored in liquid nitrogen for 〉24 h. As high as 43% of survival rate was observed when gametophytes were thawed by placing the beads in 40℃ seawater and re-hydrated in 0.05 molL^-1 citrate sodium prepared using 30‰ NaCl 7 d later. More cells of male gametophytes survived the whole procedure in comparison with female gametophytes. The cells of gametophytes surviving the preservation were able to grow asexually and produce morphologically normal sporophytes.展开更多
Temperature-dependent photoluminescence characteristics of organic-inorganic halide perovskite CH3NH3Pb I3-xClx films prepared using a two-step method on ZnO/FTO substrates were investigated. Surface morphology and ab...Temperature-dependent photoluminescence characteristics of organic-inorganic halide perovskite CH3NH3Pb I3-xClx films prepared using a two-step method on ZnO/FTO substrates were investigated. Surface morphology and absorption characteristics of the films were also studied. Scanning electron microscopy revealed large crystals and substrate coverage. The orthorhombic-to-tetragonal phase transition temperature was-140 K. The films' exciton binding energy was 77.6 ± 10.9 meV and the energy of optical phonons was 38.8 ± 2.5 meV. These results suggest that perovskite CH3NH3Pb I(3-x)Clx films have excellent optoelectronic characteristics which further suggests their potential usage in perovskitebased optoelectronic devices.展开更多
The design of the two-step gear reducer is a tedious and time-consuming process. For the purpose of improving the efficiency and intelligence of design process, case-based reasoning(CBR) technology was applied to th...The design of the two-step gear reducer is a tedious and time-consuming process. For the purpose of improving the efficiency and intelligence of design process, case-based reasoning(CBR) technology was applied to the design of the two-step gear reducer. Firstly, the current design method for the two-step gear reducer was analyzed and the principle of CBR was described. Secondly, according to the characteristics of the reducer, three key technologies of CBR were studied and the corresponding methods were provided, which are as follows: (a) an object-oriented knowledge representation method, (b) a retrieval method combining the nearest neighbor with the induction indexing, and (c) a case adaptation algorithm combining the revision based on rule with artificial revision. Also, for the purpose of improving the credibility of case retrieval, a new method for determining the weights of characteristics and a similarity formula were presented, which is a combinatorial weighting method with the analytic hierarchy process(AHP) and roughness set theory. Lastly, according to the above analytic results, a design system of the two-step gear reducer on CBR was developed by VC++, UG and Access 2003. A new method for the design of the two-step gear reducer is provided in this study. If the foregoing developed system is applied to design the two-step gear reducer, design efficiency is improved, which enables the designer to release from the tedious design process of the gear reducer so as to put more efforts on innovative design. The study result fully reflects the feasibility and validity of CBR technology in the process of the design of the mechanical parts.展开更多
Utilizing both the general quantum teleportation and the two-step protocol, a new method is presented by which multi-qubit quantum information can be teleported in a much easier way from a sender Alice to a receiver B...Utilizing both the general quantum teleportation and the two-step protocol, a new method is presented by which multi-qubit quantum information can be teleported in a much easier way from a sender Alice to a receiver Bob via the control of many agents in a network than by Yang et al's method. In this method, only all the agents collaborate with Bob can the unknown states in Alice's qubits be fully reconstructed in Bob's qubits. Comparisons between the method and Yang et al's method are made. Results show that, in this method, the preparation difficulty of initial states and the identification difficulty of entangled states are considerably reduced, new method is more feasible in technique, and Hadamard operations are not needed at all.展开更多
CeO2 oxygen carrier was prepared by precipitation method and tested by two-step steam reforming of methane (SRM). Two-step SRM for hydrogen and syngas generation is investigated in a fixed-bed reactor. Methane is di...CeO2 oxygen carrier was prepared by precipitation method and tested by two-step steam reforming of methane (SRM). Two-step SRM for hydrogen and syngas generation is investigated in a fixed-bed reactor. Methane is directly converted to syngas at a H2/CO ratio close to 2 : 1 at a high temperature (above 750 °C) by the lattice oxygen of CeO2; methane cracking is found when the reduction degree of CeO2 was above 5.0% at 850 °C in methane isothermal reaction. CeO2?δ obtained from methane isothermal reaction can split water to generate CO-free hydrogen and renew its lattice oxygen at 700 °C; simultaneously, deposited carbon is selectively oxidized to CO2 by steam following the reaction (C+2H2O→CO2+2H2). Slight deactivation in terms of amounts of desired products (syngas and hydrogen) is observed in ten repetitive two-step SRM process due to the carbon deposition on CeO2 surface as well as sintering of CeO2.展开更多
文摘Hohhot Plain, lying in the front of the Yingshan Mountains in inner Mongolia, isbounded by the mountain north, the Yellow River south, the Manhan Mountain east andloess hills southeast. Being 986 to 1100 meters above ses level, the plain generally slopesdown to the southwest, just in accordance with the flowing direction of the Great Heihe Riv-er and the Small Heihe River.
文摘In order to solve the problems including pipe corrosion, scaling and microbial growth, which severely threat safe op-eration of circulating cooling water system, this paper proposes ion exchange softening and alkalization process to solve these problems and carries out a series of studies to study the feasibility of ion exchange softening and alkaliza-tion process in the simulation process of circulating cooling water system. The studies include product water quality of ion exchange softening and alkalization process, effect on the performance of carbon steel and brass, and the inhibition that suppresses microbial growth. The results indicate that ion exchange softening and alkalization process is feasible to prevent the circulating cooling water system from scaling, pipe corrosion, and microbial growth without any other chemicals. Thus circulating cooling water system can achieve zerodischarge of wastewater.
文摘Furfural residue, an industrial waste, is a kind of strongly acidic organic materials. Its comprehensive utilization in agriculture showed a significant effect on control of soil alkalization, amelioration of solonetz and increase of crop yields. In detail it may adjust pH, depress alkalinity, reduce bulk density and compactness and increase water permeability and retention ability of the soil. Meanwhile agricultural use of furfural residue provided an effective way to avoid its pollution of the soil, Water and air.
基金The National Natural Science Foundation of China(No.52122802,52078126)Jiangsu Provincial Department of Science and Technology Innovation Support Program(No.BK20222004,BZ2022036).
文摘The novel calcium-silicate-hydrate(C-S-H)/paraffin composite phase change materials were synthesized using a discontinuous two-step nucleation method.Initially,the C-S-H precursor is separated and dried,followed by immersion in an aqueous environment to transform it into C-S-H.This two-step nucleation approach results in C-S-H with a specific surface area of 497.2 m^(2)/g,achieved by preventing C-S-H foil overlapping and refining its pore structure.When impregnated with paraffin,the novel C-S-H/paraffin composite exhibits superior thermal properties,such as a higher potential heat value of 148.3 J/g and an encapsulation efficiency of 81.6%,outperforming conventional C-S-H.Moreover,the composite material demonstrates excellent cyclic performance,indicating its potential for building thermal storage compared to other paraffin-based composites.Compared with the conventional method,this simple technology,which only adds conversion and centrifugation steps,does not negatively impact preparation costs,the environment,and resource consumption.This study provides valuable theoretical insights for designing thermal storage concrete materials and advancing building heat management.
基金the financial support from Shanxi Province Science and Technology Department(20201101012,202101060301016)the support from the APRC Grant of the City University of Hong Kong(9380086)+5 种基金the TCFS Grant(GHP/018/20SZ)MRP Grant(MRP/040/21X)from the Innovation and Technology Commission of Hong Kongthe Green Tech Fund(202020164)from the Environment and Ecology Bureau of Hong Kongthe GRF grants(11307621,11316422)from the Research Grants Council of Hong KongGuangdong Major Project of Basic and Applied Basic Research(2019B030302007)Guangdong-Hong Kong-Macao Joint Laboratory of Optoelectronic and Magnetic Functional Materials(2019B121205002).
文摘A considerable efficiency gap exists between large-area perovskite solar modules and small-area perovskite solar cells.The control of forming uniform and large-area film and perovskite crystallization is still the main obstacle restricting the efficiency of PSMs.In this work,we adopted a solid-liquid two-step film formation technique,which involved the evaporation of a lead iodide film and blade coating of an organic ammonium halide solution to prepare perovskite films.This method possesses the advantages of integrating vapor deposition and solution methods,which could apply to substrates with different roughness and avoid using toxic solvents to achieve a more uniform,large-area perovskite film.Furthermore,modification of the NiO_(x)/perovskite buried interface and introduction of Urea additives were utilized to reduce interface recombination and regulate perovskite crystallization.As a result,a large-area perovskite film possessing larger grains,fewer pinholes,and reduced defects could be achieved.The inverted PSM with an active area of 61.56 cm^(2)(10×10 cm^(2)substrate)achieved a champion power conversion efficiency of 20.56%and significantly improved stability.This method suggests an innovative approach to resolving the uniformity issue associated with large-area film fabrication.
文摘Multiplicative noise removal problems have attracted much attention in recent years.Unlike additive noise,multiplicative noise destroys almost all information of the original image,especially for texture images.Motivated by the TV-Stokes model,we propose a new two-step variational model to denoise the texture images corrupted by multiplicative noise with a good geometry explanation in this paper.In the first step,we convert the multiplicative denoising problem into an additive one by the logarithm transform and propagate the isophote directions in the tangential field smoothing.Once the isophote directions are constructed,an image is restored to fit the constructed directions in the second step.The existence and uniqueness of the solution to the variational problems are proved.In these two steps,we use the gradient descent method and construct finite difference schemes to solve the problems.Especially,the augmented Lagrangian method and the fast Fourier transform are adopted to accelerate the calculation.Experimental results show that the proposed model can remove the multiplicative noise efficiently and protect the texture well.
基金This work was supported by the National Key Research and Development Program of China(Grant No.2020YFB2206103)。
文摘In this work,a two-step metal organic chemical vapor deposition(MOCVD)method was applied for growingβ-Ga_(2)O_(3) film on c-plane sapphire.Optimized buffer layer growth temperature(T_(B))was found at 700℃ and theβ-Ga_(2)O_(3) film with full width at half maximum(FWHM)of 0.66°was achieved.A metal−semiconductor−metal(MSM)solar-blind photodetector(PD)was fabricated based on theβ-Ga_(2)O_(3) film.Ultrahigh responsivity of 1422 A/W@254 nm and photo-to-dark current ratio(PDCR)of 10^(6) at 10 V bias were obtained.The detectivity of 2.5×10^(15) Jones proved that the photodetector has outstanding performance in detecting weak signals.Moreover,the photodetector exhibited superior wavelength selectivity with rejection ratio(R_(250 nm)/R_(400 nm))of 105.These results indicate that the two-step method is a promising approach for preparation of high-qualityβ-Ga_(2)O_(3)films for high-performance solar-blind photodetectors.
基金supported by the National Natural Science Foundation of China(Nos.52201203 and 52171107)the Hebei Provincial Natural Science Foundation,China(No.E2021501026)+1 种基金the National Natural Science Foundation of China-Joint Fund of Iron and Steel Research(No.U1960204)the“333”Talent Project of Hebei Province,China(No.B20221001).
文摘Inconel 718 is the most popular nickel-based superalloy and is extensively used in aerospace,automotive,and energy indus-tries owing to its extraordinary thermomechanical properties.The effects of different two-step solid solution treatments on microstructure andδphase precipitation of Inconel 718 alloy were studied,and the transformation mechanism fromγ″metastable phase toδphase was clarified.The precipitates were statistically analyzed by X-ray diffractometry.The results show that theδphase content firstly increased,and then decreased with the temperature of the second-step solid solution.The changes in microstructure andδphase were studied by scanning electron microscopy and transmission electron microscopy.An intragranularδphase formed in Inconel 718 alloy at the second-[100]_(δ)[011]γ step solid solution temperature of 925℃,and its orientation relationship withγmatrix was determined as//and(010)_(δ)//(111)γ.Furthermore,the Vickers hardness of different heat treatment samples was measured,and the sample treated by second-step solid solution at 1010℃ reached the maximum hardness of HV 446.84.
文摘Diamonds on the Earth mainly occur in volcanic rocks such as kimberlites and lamproites^([1-8]),but can also be found in ultrahigh-pressure metamorphic rocks^([9-10]),meteorites^([11])and alluvial deposits^([12]).In recent years,diamonds have been recovered from ophiolites^([13-16])and alkalic dolerites^([17-18]).The discovery of ophiolitic diamonds and alkalic dolerites diamonds has drawn significant research interests to explore the origin of this new class of diamond source and to infer the evolution of their hosting rocks[^(19-21)].This new type of diamond had been initially considered as a result of contamination.However,more and more evidences either directly or indirectly demonstrate that these diamonds are of natural origin^([16,18,19,22-24]).During a geological survey from 2012 to 2015,the geologists from Nanjing Centre of China Geological Survey discovered a large number of yellow microdiamonds in the Langan area in northern Anhui Province^([18,25-29]).The diamond-bearing rocks of these microdiamonds mainly include dolerite and olivine basalt.From 2016 to 2018,four microdiamonds in basic rocks were recovered again in the prospecting work for primary diamond deposits in the Tashan and Zhangji areas in Xuzhou,which is geographically close to Langan[30].All these microdiamonds are similar in colour and shape to ophiolite type diamonds^([31]),and show different characteristics of kimberlite and lamproite type diamonds.Cai,et al.(2019)reported the petrological characteristics of the diamondiferous rocks^([17,21,30]).In this paper,the morphology,infrared spectrum,and carbon isotope compositions of microdiamonds were analysed and discussed by Fourier infrared spectroscopy and carbon isotope test.The types of microdiamonds found in the North China Craton,the age of mantle occurrence,and the source of carbon isotopes were revealed.In the past,many deposits of macro-diamonds,mostly of TypeⅠa orⅡa,were found in the North China Craton,and they have been extensively studied.Microdiamonds recovered from the alkalic dolerites of the North China Craton were studied by FTIR and carbon isotopic.These diamonds are usually light yellow to yellow,with a few colourless,and cubic,octahedral or rhomboidal dodecahedron,and octahedron in shape.The surface characteristics of diamonds,such as dissolution,can be observed.The overall N concentration is not high,with an average of 173×10^(-6).The infrared spectra show that most of these diamonds are TypeⅠb,and C centres are found at 1344 cm^(-1).Three diamond samples are classified as TypeⅠa/Ⅰb,because of A centres and C centres in these diamonds.Two diamonds are classified as typeⅠaAB because B,B′and A centres are found co-existing.FTIR microscopic measurements from the core to the edge of the TypeⅠaAB diamond suggest a mantle residence time of approximately 550 Ma.The C isotopic analysis reveals that these diamonds are strongly depleted in 13 C.These lowδ^(13) C values of dolerites-hosted diamonds overlap with the lower ends of peridotitic diamonds and metamorphic diamonds,and the upper end of the ophiolitic diamonds.Additionally,the reason for the strong deficitδ^(13) C shown by the carbon isotope should be studied in the future.
基金Project(2010CB630901)supported by the National Basic Research Program of ChinaProject(2013M531814)supported by the 53rd China Postdoctoral Science Foundation
文摘In order to improve the bio-oxidation efficiency of Axi refractory gold concentrate, a two-step process including a high temperature chemical oxidation and a subsequent bio-oxidation, combined with p H control during the bio-oxidation step was used. The results revealed that the optimum mode was to maintain solution p H at 1.0-1.2 during the biological oxidation stage. Under this condition, the activity of mixed culture could be sustained and the formation of jarosite could be diminished, thus the oxidation efficiency was improved. The oxidation levels of iron and sulfur were improved by 12.50% and 15.49%, and the gold recovery was increased by 21.02%. Therefore, the two-step process combined with p H control is an effective method for oxidizing the biohydrometallurgical process of Axi gold concentrate, and it will have a broad prospect of application in dealing with complex refractory gold concentrate.
基金Supported by the Natural Science Foundation of Tianjin(09JCZDJC19100)Scientific Research Fund of Tianjin Scienceand Technology University(20090403)~~
文摘[Objective] For preparing the biopesticide of Bacillus subtilis B579 with high spore concentration,the sporulation conditions were optimized.[Method] Two-step fermentation control strategy was used,in which,the first phase(0-10 h)was to improve cell growth,and the second phase(10-30 h)was to promote spore formation.Four factors including initial glucose concentration,fermentation pH,temperature(in the second phase)and shaking speed(in the second phase)were optimized using the methods of single factor test and orthogonal experiment.[Result] The initial glucose concentration showed a significant effect on sporulation.The optimal conditions for the spore formation of B.subtilis B579 were as follows:initial glucose concentration 5 g/L,fermentation pH 7.0,the temperature for the first phase 37 ℃,and the shaking speed for the first phase 180 r/min,the temperature for the second phase 40 ℃,and the shaking speed for the second phase 200 r/min;in addition,the first phase was 10 h and the second phase of fermentation was conducted for 30 h.Under such conditions,the spore concentration and spore formation rate could reach 9.43×108 CFU/ml and 90.99%,respectively,which represented 6.70-fold and 2.43-fold increase compared with those before optimization.[Conclusion] The spores concentration of biocontrol agent was improved using two-step control strategy,which provided the basis for biopesticide production in large scale.
基金Project (2012CB722805) supported by the National Basic Research Program of ChinaProjects (50974083, 51174131) supported by the National Natural Science Foundation of China+1 种基金Project (50774112) supported by the Joint Fund of NSFC and Baosteel, ChinaProject(07QA4021) supported by the Shanghai "Phosphor" Science Foundation, China
文摘The accelerating factor (AF) method is a simple and appropriate way to investigate the atomic long-time deep diffusion at solid-solid interface. In the framework of AF hyperdynamics (HD) simulation, the relationship between the diffusion coefficient along the direction of z-axis which is normal to the Mg/Zn interface and temperature was investigated, and the AF's impact on the diffusion constant (D0) and activation energy (Q^*) was studied. Then, two steps were taken to simulate the atomic diffusion process and the formation of new phases: one for acceleration and the other for equilibration. The results show that: the Arrhenius equation works well for the description of Dz with different accelerating factors; the AF has no effect on the diffusion constant Do in the case of no phase transition; and the relationship between Q* and Q conforms to Q^*=Q/A. Then, the new Arrhenius equation for AFHD is successfully constructed as Dz=Doexp[-Q/(ART)]. Meanwhile, the authentic equilibrium conformations at any dynamic moment can only be reproduced by the equilibration simulation of the HD-simulated configurations. Key words: accelerating factor method; Arrhenius equation; two-steps scheme; Mg/Zn interface; hyperdynamic simulation
文摘Using Object-oriented design and a new programming language JAVA, a physically-based model was built to simulate the hydrological, alkalization/de-alkalization and salinization/desalinization processes in soil. Furthermore, a process-based model was built to evaluate the dynamics of four herbaceous ecosystems (including dynamics of above-ground biomass, below-ground biomass, and litter biomass), each dominated by Aneurolepidium chinense (Trin.) Kitag., Chloris virgata Sw., Puccinellia tenuiflora (Turcz.) Scribn. et Merr. and Suaeda glauca Bunge. This model is a daily-time step model, suitable for simulating hydrological, alkalization/de-alkalization and salinization/desalinization processes of heterogeneous soil, and growth dynamics of different grassland communities. With climatic data and experimental data of Changling Experimental Site in Jilin Province, the soil moisture content (in 1991, 1996, 1997 and 1998), soil salt concentration, exchangeable cation percentage and pH in soil and growth dynamics of these four sorts of grassland communities (in 1991) were simulated and the results were verified to be in accord with observed data.
基金supported by the Natural Science Foundation of Jiangsu Provincial Universities, China (Grant No. 10KJB180004)
文摘We propose a two-step quantum secure direct communication (QSDC) protocol with hyperentanglement in both the spatial-mode and the polarization degrees of freedom of photon pairs which can in principle be produced with a beta barium borate crystal. The secret message can be encoded on the photon pairs with unitary operations in these two degrees of freedom independently. This QSDC protocol has a higher capacity than the original two-step QSDC protocol as each photon pair can carry 4 bits of information. Compared with the QSDC protocol based on hyperdense coding, this QSDC protocol has the immunity to Trojan horse attack strategies with the process for determining the number of the photons in each quantum signal as it is a one-way quantum communication protocol.
基金the National High-Tech Research Development Program of China (No. 2003AA331100).
文摘The effects of the two-step ageing parameters (temperature and time) on the mechanical properties and electrical conductivity of 7B04 (A1-Zn-Mg-Cu) pre-stretched thick plates were studied. The results reveal that the initial T1 ageing contributes a major increase of the tensile strength, and the 0.2% proof stress value reaches 482 MPa after ageing for 7 h at 115℃. Behavioral differences in the tensile properties of the alloy after the two-step ageing treatment were less with the first-step ageing at 115~C for different time periods (7, 14, and 21 h). The effects of the second ageing parameters on the properties and microstructure of the 7B04 alloy were remarkable. TEM analysis of the samples aged at Temper I (7 h at 115℃ + 12 h at 160℃) and Temper II (7 h at 115℃ + 16 h at 165℃) indicates that two kinds of phases, i.e. 11' and 11 phases, precipitate from the matrix and efficiently improve the tensile strength of the alloy, and the grain boundary precipitates are coarse and discrete. There are obvious precipitate free zones (PFZs) along the grain boundary in the microstructure of the alloy after the two-step ageing treatment.
文摘Gametophytes of Laminaria japonica were cryopreserved in liquid nitrogen using encapsulation-dehydration with two-step cooling method. Gametophytes cultured at 10℃ and under continuous irradiance of 30 μmol m^-2 s^-1 for 3 weeks were encapsulated in calcium alginate beads. The beads were dehydrated in 0.4 molLl sucrose prepared with seawater for 6 h, desiccated in an incubator set at 10℃ and 70% relative humidity for 4 h, pre-frozen at either -40℃ or -60℃ for 30 min, and stored in liquid nitrogen for 〉24 h. As high as 43% of survival rate was observed when gametophytes were thawed by placing the beads in 40℃ seawater and re-hydrated in 0.05 molL^-1 citrate sodium prepared using 30‰ NaCl 7 d later. More cells of male gametophytes survived the whole procedure in comparison with female gametophytes. The cells of gametophytes surviving the preservation were able to grow asexually and produce morphologically normal sporophytes.
基金supported by the International Science and Technology Cooperation Program of Science and Technology Bureau of Changchun City,China(Grant No.12ZX68)
文摘Temperature-dependent photoluminescence characteristics of organic-inorganic halide perovskite CH3NH3Pb I3-xClx films prepared using a two-step method on ZnO/FTO substrates were investigated. Surface morphology and absorption characteristics of the films were also studied. Scanning electron microscopy revealed large crystals and substrate coverage. The orthorhombic-to-tetragonal phase transition temperature was-140 K. The films' exciton binding energy was 77.6 ± 10.9 meV and the energy of optical phonons was 38.8 ± 2.5 meV. These results suggest that perovskite CH3NH3Pb I(3-x)Clx films have excellent optoelectronic characteristics which further suggests their potential usage in perovskitebased optoelectronic devices.
基金This project is supported by National Hi-tech Research and Development Program of China (863 Program, Grant No. 2008AA04Z115)Science and Technology Program of the Ministry of Construction of China (Grant No. 2008-K8-2)+1 种基金Jiangsu Provincial Natural Science Foundation of China (Grant No. BK2007042)Open Fund of State Key Lab of CAD&CG, Zhejiang University, China (Grant No. A0914)
文摘The design of the two-step gear reducer is a tedious and time-consuming process. For the purpose of improving the efficiency and intelligence of design process, case-based reasoning(CBR) technology was applied to the design of the two-step gear reducer. Firstly, the current design method for the two-step gear reducer was analyzed and the principle of CBR was described. Secondly, according to the characteristics of the reducer, three key technologies of CBR were studied and the corresponding methods were provided, which are as follows: (a) an object-oriented knowledge representation method, (b) a retrieval method combining the nearest neighbor with the induction indexing, and (c) a case adaptation algorithm combining the revision based on rule with artificial revision. Also, for the purpose of improving the credibility of case retrieval, a new method for determining the weights of characteristics and a similarity formula were presented, which is a combinatorial weighting method with the analytic hierarchy process(AHP) and roughness set theory. Lastly, according to the above analytic results, a design system of the two-step gear reducer on CBR was developed by VC++, UG and Access 2003. A new method for the design of the two-step gear reducer is provided in this study. If the foregoing developed system is applied to design the two-step gear reducer, design efficiency is improved, which enables the designer to release from the tedious design process of the gear reducer so as to put more efforts on innovative design. The study result fully reflects the feasibility and validity of CBR technology in the process of the design of the mechanical parts.
基金Project supported by the National Natural Science Foundation of China (Grant No 10304022).
文摘Utilizing both the general quantum teleportation and the two-step protocol, a new method is presented by which multi-qubit quantum information can be teleported in a much easier way from a sender Alice to a receiver Bob via the control of many agents in a network than by Yang et al's method. In this method, only all the agents collaborate with Bob can the unknown states in Alice's qubits be fully reconstructed in Bob's qubits. Comparisons between the method and Yang et al's method are made. Results show that, in this method, the preparation difficulty of initial states and the identification difficulty of entangled states are considerably reduced, new method is more feasible in technique, and Hadamard operations are not needed at all.
基金supported by the National Natural Science Foundation of China (NO. 51004060)the Natural Science Foundation of Yunnan Province (NO. 2008E030M, 2010ZC108)+2 种基金the Research Foundation for the Doctoral Program of Higher Education of China (NO. 20095314120005)the Analysis and Test Foundation of Kunming University of Science and Technology (KUST)the 2010 Innovation Foundation of KUST
文摘CeO2 oxygen carrier was prepared by precipitation method and tested by two-step steam reforming of methane (SRM). Two-step SRM for hydrogen and syngas generation is investigated in a fixed-bed reactor. Methane is directly converted to syngas at a H2/CO ratio close to 2 : 1 at a high temperature (above 750 °C) by the lattice oxygen of CeO2; methane cracking is found when the reduction degree of CeO2 was above 5.0% at 850 °C in methane isothermal reaction. CeO2?δ obtained from methane isothermal reaction can split water to generate CO-free hydrogen and renew its lattice oxygen at 700 °C; simultaneously, deposited carbon is selectively oxidized to CO2 by steam following the reaction (C+2H2O→CO2+2H2). Slight deactivation in terms of amounts of desired products (syngas and hydrogen) is observed in ten repetitive two-step SRM process due to the carbon deposition on CeO2 surface as well as sintering of CeO2.