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Alkali Vapor Corrosion of Different Refractories at High Temperatures
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作者 FAN Muxu HOU Xiaojing +3 位作者 FENG Zhiyuan WANG Han LIU Pengcheng SHI Gan 《China's Refractories》 CAS 2023年第2期24-30,共7页
Commercial high purity corundum brick,corundum-mullite brick,mullite brick,calcium hexaaluminate brick and calcium hexaaluminate-corundum brick were studied to investigate their reaction state and alkali vapor corrosi... Commercial high purity corundum brick,corundum-mullite brick,mullite brick,calcium hexaaluminate brick and calcium hexaaluminate-corundum brick were studied to investigate their reaction state and alkali vapor corrosion mechanism at 1370 and 1500℃.The results show that:(1)served in hot alkali vapor,the high-purity corundum brick has no obvious slag layer but expands dramatically;(2)the corundum-mullite brick shows obvious reactive expansion at 1370℃and melting corrosion happens at 1500℃;(3)at 1370℃alkali vapor and mullite brick react and form a slag layer without volume effect;when the temperature increases to 1500℃,the reaction melting corrosion intensifies;(4)the calcium hexaaluminate brick and the calcium hexaaluminate-corundum brick form a thin slag layer in alkali vapor,and the sample surface absorbs Na+to form a dense layer with small volume effect. 展开更多
关键词 alkali vapor corrosion sodium carbonate calcium hexaaluminate CORUNDUM MULLITE
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Water vapor corrosion behaviors of high-entropy pyrosilicates 被引量:3
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作者 Zeyu Chen Chucheng Lin +3 位作者 Wei Zheng Caifen Jiang Yi Zeng Xuemei Song 《Journal of Materiomics》 SCIE 2022年第5期992-1000,共9页
In this study,the water vapor corrosion resistance of two types of high-entropy pyrosilicates((Yb_(0.2)Y_(0.2)Lu_(0.2)Ho_(0.2)Er_(0.2))_(2)Si_(2)O_(7)((5RE1/5)_(2)Si_(2)O_(7))and(Yb_(0.2)5Lu_(0.2)5Ho_(0.2)5Er_(0.2)5)_... In this study,the water vapor corrosion resistance of two types of high-entropy pyrosilicates((Yb_(0.2)Y_(0.2)Lu_(0.2)Ho_(0.2)Er_(0.2))_(2)Si_(2)O_(7)((5RE1/5)_(2)Si_(2)O_(7))and(Yb_(0.2)5Lu_(0.2)5Ho_(0.2)5Er_(0.2)5)_(2)Si_(2)O_(7)((4RE_(1/4))_(2)Si_(2)O_(7)))and two single-component pyrosilicates(Yb_(2)Si_(2)O_(7) and Lu_(2)Si_(2)O_(7))were evaluated at 1350℃ for 50e100 h,and the initial corrosion behaviors of these pyrosilicates were studied.The results showed that the final corrosion products of the four types of pyrosilicates were all X2-type monosilicates,exhibiting similar corrosion phenomena.However,(4RE_(1/4))_(2)Si_(2)O_(7) generated many nanoscale monosilicate grains during corrosion.The corrosion resistance of Lu_(2)Si_(2)O_(7) was clearly better than those of the others,and(4RE_(1/4))_(2)Si_(2)O_(7) exhibited the worst corrosion resistance.The corrosion mechanism of the pyrosilicate blocks was analyzed from the perspectives of grain size,bulk hydrophobicity,and binding energy.This study potentially provides a theoretical basis for the preparation of high-entropy pyrosilicates with different atomic ratios according to the different properties of the various rare earth elements. 展开更多
关键词 Environmental barrier coatings High-entropy pyrosilicates Water vapor corrosion
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