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MOLAR RATIOS OF C,N,P OF PARTICULATE MATTER AND THEIR VERTICAL FLUXES IN THE YELLOW SEA 被引量:3
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作者 王保栋 战闰 徐明德 《Chinese Journal of Oceanology and Limnology》 SCIE CAS CSCD 2002年第1期91-96,共6页
The vertical fluxes and molar ratios of carbon, nitrogen and phosphorus of suspended particulate matter in the Yellow Sea were studied based on the analysis of suspended particulate matter, sediments and sinking parti... The vertical fluxes and molar ratios of carbon, nitrogen and phosphorus of suspended particulate matter in the Yellow Sea were studied based on the analysis of suspended particulate matter, sediments and sinking particles obtained by use of moored sediment traps. The POC:PON ratios indicate that most of the particulate organic matter in the Yellow Sea water column comes from marine life rather than the continent. The vertical fluxes of SPM, POC, PON and POP in the Yellow Sea are much higher than those in other seas over the world, and present a typical pattern in shallow epicontinental seas. The estimated residence time of the bioactive elements showed that the speed of the biogeochemical process of materials in the Yellow Sea is much shorter than that in the open ocean as there was high primary productivity in this region. 展开更多
关键词 vertical flux Redfield ratio particulate matter the Yellow Sea
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Chemical characteristics and estimation on the vertical flux of N,P,Si in upwelling area of Taiwan Strait 被引量:1
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作者 Chen Shuitu and Ruan Wuqi(Fujian Institute of Oceanology, Xiamen 361012, China) 《Acta Oceanologica Sinica》 SCIE CAS CSCD 1995年第3期383-392,共10页
Based on the data obtained from oceanographic surveys at the central and northern parts of the TaiwanStrait during the period from 1983 to 1988, it is showed that the nutrient content in the coastal and bottom waters ... Based on the data obtained from oceanographic surveys at the central and northern parts of the TaiwanStrait during the period from 1983 to 1988, it is showed that the nutrient content in the coastal and bottom waters isrelatively high with an upward and offward decrease, and that the upwelling in the Fujian coastal area controls the distribution of nutrients in summer.The upwelling water is characterized by 2. 29 μmol/dm ̄3 of nitrate; 2. 83 μmol/dm ̄3of silicate; 0. 20 μmol/dm ̄3 of dissolved inorganic phosphate,respectively. Significant correlation between nutrientsand dissolved oxygen content and its degree of saturation, temperature, and salinity, respectively are found in the upweiling area. Average of N/P ratio in the area(15. 9) approaches to Redfield ratio. Their vertical flux is estimated tobe 23. 6 mg/(m ̄2·d) for - P, 223 mg/(m ̄2·d) for NO-N, 302 mg/(m ̄2·d) for SiO-Si, respectively,which is the main source Of nutients in the areas in summer. The mean of the flux of P and NO-N is about86 % and 73% necessary for phytoplankton in the euphotic zone. 展开更多
关键词 UPWELLING the Taiwan Strait nutrients distribution vertical flux
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On the variability of vertical eddy heat flux in the upper ocean
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作者 Tianshi Du Peiran Yang Zhao Jing 《Acta Oceanologica Sinica》 SCIE CAS CSCD 2022年第10期94-99,共6页
Ocean eddies produce strong vertical heat flux(VHF)in the upper ocean,exerting profound influences on the climate and ecosystem.Currently,mooring array provides a standard way to estimate the eddy-induced VHF(EVHF)bas... Ocean eddies produce strong vertical heat flux(VHF)in the upper ocean,exerting profound influences on the climate and ecosystem.Currently,mooring array provides a standard way to estimate the eddy-induced VHF(EVHF)based on the adiabatic potential density equation.Apart from the validity of adiabatic assumption,it remains unclear to what extent the estimated EVHF at a single location within a limited time period is representative of its climatological mean value.In this study,we analyzed the above issue by systematically evaluating the variability of EVHF simulated by a 1-km ocean model configured over the Kuroshio Extension.It is found that the EVHF at a single location exhibits pronounced variability.Even averaged over one year that is comparable to the current maintenance capacity of mooring array,the EVHF still deviates significantly from its climatological mean value.For more than 49%of locations in our computational domain(31°-40°N,149°-166°E),the discrepancy between the one-year mean EVHF and its climatological mean value at the peaking depth is larger than the climatological mean itself.The mesoscale eddies play a dominant role in the variability of EVHF but contribute little to the climatological mean EVHF;the opposite is true for submesoscale eddies.Our findings indicate that nested mooring array allowing for isolating the effects of submesoscale eddies will be useful to obtain climatological mean EVHF. 展开更多
关键词 vertical eddy heat flux SUBMESOSCALE MESOSCALE climatological value pseudo-observation experiment
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Re-evaluating the vertical mass-flux profiles of aeolian sediment at the southern fringe of the Taklimakan Desert, China
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作者 XUE Jie LEI Jiaqiang +3 位作者 LI Shengyu GUI Dongwei MAO Donglei ZHOU Jie 《Journal of Arid Land》 SCIE CSCD 2015年第6期765-777,共13页
Reliable estimation of the mass-flux profiles of aeolian sediment is essential for predicting sediment transport rates accurately and designing measures to cope with wind-erosion. Vertical mass-flux profiles from seve... Reliable estimation of the mass-flux profiles of aeolian sediment is essential for predicting sediment transport rates accurately and designing measures to cope with wind-erosion. Vertical mass-flux profiles from seventeen wind-erosion events were re-evaluated using five typical models based on observed data obtained from a smooth bare field at the southern fringe of the Taklimakan Desert, China. The results showed that the exponential-function model and the logarithmic-function model exhibited the poorest fit between observed and predicted mass-flux profiles. The power-function model and the modified power-function model improved the fit to field data to an equivalent extent, while the five-parameter combined-function model with a scale constant(σ) of 0.00001 m(different from the σ value proposed by Fryear, which represented the height above which 50% of the total mass flux occurred) was verified as the best for describing the vertical aeolian sediment mass-flux profiles using goodness of fit(R2) and the Akaike Information Criterion(AIC) values to evaluate model performance. According to relationships among model parameters, the modified power model played a prominent explanatory role in describing the vertical profiles of the observed data, whereas the exponential model played a coordinating role. In addition, it was found that the vertical profiles could not be extrapolated using the five selected models or easily estimated using an efficient model without field observations by a near-surface sampler at 0 to 0.05 m. 展开更多
关键词 vertical profile mass flux aeolian sediment wind erosion Taklimakan Desert
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Sediment flux and source in northern Yellow Sea by ^(210)Pb technique 被引量:7
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作者 李凤业 李学刚 +3 位作者 宋金明 王桂芝 程鹏 高抒 《Chinese Journal of Oceanology and Limnology》 SCIE CAS CSCD 2006年第3期255-263,共9页
Sedimentation of fine-grained deposits on coastal zones and continental shelves are important because of the association with chemical pollutants, and the implication to the impact on biological processes, the stratig... Sedimentation of fine-grained deposits on coastal zones and continental shelves are important because of the association with chemical pollutants, and the implication to the impact on biological processes, the stratigraphic correlations, and changes in sedimentary environments. The Yellow Sea continental shelf receives large quantities of sediment from the Huanghe (Yellow) River. Unfortunately, little attention has been yet paid to the sedimentation on the shallow shelf and its features, and the vertical sediment flux in the area is poorly understood. In this study, nine cores were collected in northern Yellow Sea by the R/V Science 1 in September, 1998 and 1999 to examine the sedimentation rate, sediment flux and the provenance with ^210Pb analysis. The 2^210Pb activity profiles showed that the vertical sediment flux ranged from 0.06 to 1.18 g/cm^2·a in the region. In central part of the area, there was a patch of fine-grained mud, with the flux below 0.33 g/cm^2·a. Most profiles were featured in two-segment model. Differences in the profiles reflected spatial and temporal variations in hydrodynamic and sedimentary processes. In order to determine the provenance and sedimentary setting in the area, the geochemistry of Ca, Fe, Sr, Cu, Ti and Rb in 11 surficial sediment samples were studied, which showed that in the central northern Yellow Sea, the mud deposit was from multi-source but mainly from the Huanghe River. 展开更多
关键词 ^210PB vertical sediment flux Sediment source The Yellow Sea
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Observations of turbulent mixing and vertical diff usive salt fl ux in the Changjiang Diluted Water 被引量:1
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作者 Baisu ZHU Wei YANG +2 位作者 Chengfei JIANG Tao WANG Hao WEI 《Journal of Oceanology and Limnology》 SCIE CAS CSCD 2022年第4期1349-1360,共12页
Based on microstructure measurements from a repeated sampling station southwest of the Jeju Island during summer,we studied the hydrography,pycnocline turbulence,and vertical salt fl ux in the Changjiang Diluted Water... Based on microstructure measurements from a repeated sampling station southwest of the Jeju Island during summer,we studied the hydrography,pycnocline turbulence,and vertical salt fl ux in the Changjiang Diluted Water(CDW).The water column was well stratifi ed with the CDW occupied the surface~20 m.Most of the large turbulent kinetic energy dissipation rate(ε)were found in the bottom boundary layer.Interestingly,intermittent strong turbulence(ε>10^(-6) W/kg)occurred in the pycnocline,which may induce strong mixing events and increase the vertical diff usive salt fl ux at the base of CDW by one order of magnitude.The daily-mean vertical diff usive salt fl ux could reach 4.3(2.1,8.9)×10^(-6) m/s.Both moored velocity measurements and associated wavelet analysis showed the presence of velocity fl uctuations when there was strong pycnocline turbulence.The moderate resolution imaging spectroradiometer(MODIS)satellite images further suggest that the velocity fl uctuations are induced by the prevailing internal solitary waves(ISWs)which are mainly generated at the shelf break of the East China Sea or the topographic features surrounding Jeju Island.The calculated gradient Richardson number denote the occurrence of shear instability in the pycnocline when strong turbulence presents.The presented results have strong implications for the importance of ISWs in infl uencing the vertical diff usion of CDW and changes in other properties. 展开更多
关键词 TURBULENCE vertical salt flux internal solitary wave Changjiang River plume
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Estimates of global M_2 internal tide energy fluxes using TOPEX/POSEIDON altimeter data
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作者 张艳伟 梁鑫峰 +1 位作者 田纪伟 杨丽芬 《Chinese Journal of Oceanology and Limnology》 SCIE CAS CSCD 2009年第1期129-134,共6页
TOPEX/POSEIDON altimeter data from October 1992 to June 2002 are used to calculate the global barotropic M2 tidal currents using long-term tidal harmonic analysis. The tides calculated agree well with ADCP data obtain... TOPEX/POSEIDON altimeter data from October 1992 to June 2002 are used to calculate the global barotropic M2 tidal currents using long-term tidal harmonic analysis. The tides calculated agree well with ADCP data obtained from the South China Sea (SCS). The maximum tide velocities along the semi-major axis and semi-minor axis can be computed from the tidal ellipse. The global distribution of M2 internal tide vertical energy flux from the sea bottom is calculated based on a linear internal wave generation model. The global vertical energy flux of M2 internal tide is 0.96 TW, with 0.36 TW in the Pacific, 0.31 TW in the Atlantic and 0.29 TW in the Indian Ocean, obtained in this study. The total horizontal energy flux of M2 internal tide radiating into the open ocean from the lateral boundaries is 0.13 TW, with 0.06 TW in the Pacific, 0.04TW in the Atlantic, and 0.03 TW in the Indian Ocean. The result shows that the principal lunar semi-diurnal tide Me provides enough energy to maintain the large-scale thermohaline circulation of the ocean. 展开更多
关键词 TOPEX/POSEIDON altimeter M2 internal tide vertical energy flux horizontal energy flux
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Oceanic vertical mixing of the lower halocline water in the Chukchi Borderland and Mendeleyev Ridge
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作者 Long Lin Hailun He +3 位作者 Yong Cao Tao Li Yilin Liu Mingfeng Wang 《Acta Oceanologica Sinica》 SCIE CAS CSCD 2021年第11期39-49,共11页
Oceanic vertical mixing of the lower halocline water(LHW)in the Chukchi Borderland and Mendeleyev Ridge was studied based on in situ hydrographic and turbulent observations.The depth-averaged turbulent dissipation rat... Oceanic vertical mixing of the lower halocline water(LHW)in the Chukchi Borderland and Mendeleyev Ridge was studied based on in situ hydrographic and turbulent observations.The depth-averaged turbulent dissipation rate of LHW demonstrates a clear topographic dependence,with a mean value of 1.2×10^(-9) W/kg in the southwest of Canada Basin,1.5×10^(-9) W/kg in the Mendeleyev Abyssal Plain,2.4×10^(-9) W/kg on the Mendeleyev Ridge,and2.7×10^(-9) W/kg on the Chukchi Cap.Correspondingly,the mean depth-averaged vertical heat flux of the LHW is0.21 W/m^(2) in the southwest Canada Basin,0.30 W/m^(2) in the Mendeleyev Abyssal Plain,0.39 W/m^(2) on the Mendeleyev Ridge,and 0.46 W/m^(2) on the Chukchi Cap.However,in the presence of Pacific Winter Water,the upward heat released from Atlantic Water through the lower halocline can hardly contribute to the surface ocean.Further,the underlying mechanisms of diapycnal mixing in LHW—double diffusion and shear instability—was investigated.The mixing in LHW where double diffusion were observed is always relatively weaker,with corresponding dissipation rate ranging from 1.01×10^(-9) W/kg to 1.57×10^(-9) W/kg.The results also show a strong correlation between the depth-average dissipation rate and strain variance in the LHW,which indicates a close physical linkage between the turbulent mixing and internal wave activities.In addition,both surface wind forcing and semidiurnal tides significantly contribute to the turbulent mixing in the LHW. 展开更多
关键词 oceanic vertical mixing lower halocline water dissipation rate vertical heat flux
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ANALYSIS OF RAINSTORMS ASSOCIATED WITH SIMILAR TRACK TROPICAL CYCLONES HAITANG (0505) AND BILIS (0604) 被引量:1
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作者 余贞寿 陈宣淼 +2 位作者 倪东鸿 冀春晓 谢海华 《Journal of Tropical Meteorology》 SCIE 2009年第1期111-115,共5页
It is generally thought that the influence of comparable track typhoons is approximately similar, but in fact their wind and especially their rainstorm distribution are often very different. Therefore, a contrastive a... It is generally thought that the influence of comparable track typhoons is approximately similar, but in fact their wind and especially their rainstorm distribution are often very different. Therefore, a contrastive analysis of rainstorms by tropical cyclones (TCs) Haitang (0505) and Bilis (0604), which are of a similar track, is designed to help understand the mechanism of the TC rainstorm and to improve forecasting skills. The daily rainfall of TC Haitang (0505) and Bilis (0604) is diagnosed and compared. The result indicates that these two TCs have similar precipitation distribution before landfall but different precipitation characteristics after landfall. Using NCEP/GFS analysis data, the synoptic situation is analyzed; water vapor transportation is discussed regarding the calculated water vapor flux and divergence. The results show that the heavy rainfall in the Zhejiang and Fujian Provinces associated with Haitang (0505) and Bilis (0604) before landfall results from a peripheral easterly wind, a combination of the tropical cyclone and the terrain. After landfall and moving far inland of the storm, the precipitation of Haitang is caused by water vapor convergence carried by its own circulation; it is much weaker than that in the coastal area. One of the important contributing factors to heavy rainstorms in southeast Zhejiang is a southeast jet stream, which is maintained over the southeast coast. In contrast, the South China Sea monsoon circulation transports large amounts of water vapor into Bilis – when a water-vapor transport belt south of the tropical cyclone significantly strengthens – which strengthens the transport. Then, it causes water vapor flux to converge on the south side of Bilis and diverge on the north side. Precipitation is much stronger on the south side than that on the north side. After Bilis travels far inland, the cold air guided by a north trough travels into the TC and remarkably enhances precipitation. In summary, combining vertical wind shear with water vapor transportation is a good way to predict rainstorms associated with landing tropical cyclones. 展开更多
关键词 weather forecast tropical cyclones typhoon rainstorms similar tracks water vapor flux vertical wind shear
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Effect of seasonal barrier layer on mixed-layer heat budget in the Bay of Bengal
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作者 Gayan Pathirana Dongxiao Wang +2 位作者 Gengxin Chen M.K.Abeyratne Tilak Priyadarshana 《Acta Oceanologica Sinica》 SCIE CAS CSCD 2022年第9期38-49,共12页
Time series measurements (2010–2017) from the Research Moored Array for African–Asian–Australian Monsoon Analysis and Prediction (RAMA) moorings at 15°N,90°E and 12°N,90°E are used to investigat... Time series measurements (2010–2017) from the Research Moored Array for African–Asian–Australian Monsoon Analysis and Prediction (RAMA) moorings at 15°N,90°E and 12°N,90°E are used to investigate the effect of the seasonal barrier layer (BL) on the mixed-layer heat budget in the Bay of Bengal (BoB).The mixed-layer temperature tendency (?T/?t) is primarily controlled by the net surface heat flux that remains in the mixed layer(Q’) from March to October,while both Q’and the vertical heat flux at the base of the mixed layer (Q_(h)),estimated as the residual of the mixed-layer heat budget,dominate during winter (November–February).An inverse relation is observed between the BL thickness and the mixed-layer temperature (MLT).Based on the estimations at the moorings,it is suggested that when the BL thickness is≥25 m,it exerts a considerable influence on ?T/?t through the modulation of Q_(h) (warming) in the BoB.The cooling associated with Q_(h) is strongest when the BL thickness is≤10 m with the MLT exceeding 29°C,while the contribution from Q_(h) remains nearly zero when the BL thickness varies between 10 m and 25 m.Temperature inversion is evident in the BoB during winter when the BL thickness remains≥25 m with an average MLT<28.5°C.Furthermore,Q_(h) follows the seasonal cycle of the BL at these RAMA mooring locations,with r>0.72 at the 95%significance level. 展开更多
关键词 barrier layer vertical heat flux temperature inversion Bay of Bengal
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Three-Dimensional Wave-Induced Current Model Equations and Radiation Stresses
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作者 XIA Hua-yong 《China Ocean Engineering》 SCIE EI CSCD 2017年第4期418-427,共10页
After the approach by Mellor (2003, 2008), the present paper reports on a repeated effort to derive the equations for three-dimensional wave-induced current. Via the vertical momentum equation and a proper coordinat... After the approach by Mellor (2003, 2008), the present paper reports on a repeated effort to derive the equations for three-dimensional wave-induced current. Via the vertical momentum equation and a proper coordinate transformation, the phase-averaged wave dynamic pressure is well treated, and a continuous and depth-dependent radiation stress tensor, rather than the controversial delta Dirac function at the surface shown in Mellor (2008), is provided. Besides, a phase-averaged vertical momentum flux over a sloping bottom is introduced. All the inconsistencies in Mellor (2003, 2008), pointed out by Ardhuin et al. (2008) and Bennis and Ardhuin (2011), are overcome in the presently revised equations. In a test case with a sloping sea bed, as shown in Ardhuin et al. (2008), the wave-driving forces derived in the present equations are in good balance, and no spurious vertical circulation occurs outside the surf zone, indicating that Airy’s wave theory and the approach of Mellor (2003, 2008) are applicable for the derivation of the wave-induced current model. 展开更多
关键词 sea surface wave wave-induced current radiation stress vertical wave momentum flux
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What Determines the Amplitude of ENSO Events?
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作者 WANG Yu-Xing YANG Hai-Jun Tore FUREVIK 《Atmospheric and Oceanic Science Letters》 CSCD 2013年第2期90-96,共7页
In this paper, the dynamic effect of oceanic upwelling on the intensity of E1 Nifio-Southern Oscilla tion (ENSO) is studied using a simple coupled model (Zebiak-Cane Model). The term balance analysis in the temper... In this paper, the dynamic effect of oceanic upwelling on the intensity of E1 Nifio-Southern Oscilla tion (ENSO) is studied using a simple coupled model (Zebiak-Cane Model). The term balance analysis in the temperature variability equation shows that the anomalous upwelling of the mean vertical temperature gradient and the mean advection of the anomalous meridional tem perature gradient are the two of most important factors that determine the intensity of ENSO events, in which the "vertical oceanic heat flux" in the eastern equatorial Pa cific (EEP) is the primary influencing factor. The lag cor relation between "vertical heat flux (VHF)" and ENSO intensity shows that the highest correlation occurs when the former leads the latter by one to two weeks. The VHF is positively correlated with the background thermocline strength in the EEP, and an increase of both could result in strong ENSO variability. Comparison of the forced and coupled experiments suggests that the coupled process can affect both the intensity and freauencv of ENSO. 展开更多
关键词 ENSO amplitude vertical heat flux thermo-cline strength
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Contrasting Regional Responses of Indian Summer Monsoon Rainfall to Exhausted Spring and Concurrently Emerging Summer El Nino Events
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作者 E.K.KRISHNA KUMAR S.ABHILASH +3 位作者 SANKAR SYAM P.VIJAYKUMAR K.R.SANTOSH A.V.SREENATH 《Advances in Atmospheric Sciences》 SCIE CAS CSCD 2023年第4期697-710,共14页
The inverse relationship between the warm phase of the El Nino Southern Oscillation(ENSO)and the Indian Summer Monsoon Rainfall(ISMR)is well established.Yet,some El Nino events that occur in the early months of the ye... The inverse relationship between the warm phase of the El Nino Southern Oscillation(ENSO)and the Indian Summer Monsoon Rainfall(ISMR)is well established.Yet,some El Nino events that occur in the early months of the year(boreal spring)transform into a neutral phase before the start of summer,whereas others begin in the boreal summer and persist in a positive phase throughout the summer monsoon season.This study investigates the distinct influences of an exhausted spring El Nino(springtime)and emerging summer El Nino(summertime)on the regional variability of ISMR.The two ENSO categories were formulated based on the time of occurrence of positive SST anomalies over the Nino-3.4 region in the Pacific.The ISMR’s dynamical and thermodynamical responses to such events were investigated using standard metrics such as the Walker and Hadley circulations,vertically integrated moisture flux convergence(VIMFC),wind shear,and upper atmospheric circulation.The monsoon circulation features are remarkably different in response to the exhausted spring El Nino and emerging summer El Nino phases,which distinctly dictate regional rainfall variability.The dynamic and thermodynamic responses reveal that exhausted spring El Nino events favor excess monsoon rainfall over eastern peninsular India and deficit rainfall over the core monsoon regions of central India.In contrast,emerging summer El Nino events negatively impact the seasonal rainfall over the country,except for a few regions along the west coast and northeast India. 展开更多
关键词 exhausted spring El Nino emerging summer El Nino Indian Summer Monsoon Hadley and Walker circulation tropical easterly jet vertical integrated moisture flux convergence
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VERTICAL STRUCTURE OF SECOND-MOMENT TURBULENT VARIABLES
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作者 AL-JIBOORI.M.H. 徐玉貌 钱永甫 《Acta meteorologica Sinica》 SCIE 2001年第2期218-232,共15页
Two kinds of observational data,fluctuation and mean profile measurements,from a 325 m meteorological tower in Beijing,China,are used to evaluate local scales of velocity and temperature for higher heights by flux-gra... Two kinds of observational data,fluctuation and mean profile measurements,from a 325 m meteorological tower in Beijing,China,are used to evaluate local scales of velocity and temperature for higher heights by flux-gradient mean profiles and eddy-correlation techniques.A comparison of these methods each other was made in terms of vertical turbulence fluxes for momentum and beat at the same heigbt.The vertical profiles of non-dimensional second moments. such as vertical turbulent fluxes of momentum and heat.velocity and temperature standard deviations,were derived by local similarity theory.The local similarity relations expressed that the vertical distributions of non-dimensional second moment variables were found to be functions of z/Λ and z/h in the stable boundary layer and the function of z/Z_i for the convective boundary layer,where A the local Monin Obukhov(M-O)length.h the height of stable boundary layer and Z_i the height of mixed-layer.These relations are shown to agree well with the observational data. 展开更多
关键词 vertical turbulence fluxes local similarity theory standard deviations of velocity and temperature
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Historical records of polycyclic aromatic hydrocarbon deposition in a shallow eutrophic lake:Impacts of sources and sedimentological conditions 被引量:6
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作者 Chaocan Li Shouliang Huo +5 位作者 Zhiqiang Yu Wei Guo Beidou Xi Zhuoshi He Xiangying Zeng Fengchang Wu 《Journal of Environmental Sciences》 SCIE EI CAS CSCD 2016年第3期261-269,共9页
Sediment core samples collected from Lake Chaohu were analyzed for 15 priority polycyclic aromatic hydrocarbons(PAHs)to assess the spatial and temporal distributions of the PAHs during lacustrine sedimentary process... Sediment core samples collected from Lake Chaohu were analyzed for 15 priority polycyclic aromatic hydrocarbons(PAHs)to assess the spatial and temporal distributions of the PAHs during lacustrine sedimentary processes and regional economic development.Assessing the PAH sedimentary records over an approximately 100-year time span,we identified two stages in the PAH inputs and sources(before the 1970 s and after the 1970s)in the eastern lake region near a village,whereas three stages(before the 1950 s,1950s–1990s and after the1990s)were identified in the western lake region near urban and industrial areas.Rapid increases in the PAH depositional fluxes occurred during the second stage due to increased human activities in the Lake Chaohu basin.The composition and isomeric ratios of the PAHs revealed that pyrolysis is the main source of PAHs in this lake.Strong positive relationships between PAH concentration and the total organic carbon concentration,sediment grain size(〈 4 μm),as well as the local population and Gross Domestic Product indicated that the sedimentary conditions impact the depositional characteristics of the PAHs;simultaneously,socioeconomic activities,such as energy consumption and the levels of urban industrialization and civilization,affect both the composition and abundance of the PAHs. 展开更多
关键词 PAHs vertical distribution flux Sedimentological impact Socioeconomic
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