Three long-term fixed acoustic Doppler current profilers were first used for investigating the vertical structure of tidal currents in Xuliujing Section of Changjiang River Estuary.Moreover,three different periods(spr...Three long-term fixed acoustic Doppler current profilers were first used for investigating the vertical structure of tidal currents in Xuliujing Section of Changjiang River Estuary.Moreover,three different periods(spring,summer and fall)were also considered for investigating seasonal variations.The semi-diurnal tides were the most energetic,with along-channel speed of up to 80 cm/s for M_(2)constituent,which dominates at all stations with percent energy up to 65%–75%during seasons.The shape of tidal ellipses of the most energetic semi-diurnal constituent M_(2)showed obvious polarization of the flow paralleling to the riverbank,with the minor semi-axis being generally less than 20%of the major one.The maximum velocity of mean current is appeared in top layers at all the three stations,and the velocity decreased with the depth.The seasonal variations of direction are also observed,which is probably caused by complex local topography since the erosion and deposition in riverbed.Observed vertical variation of four parameters of M_(2)ellipses,agreed well with the optimally fit frictional solutions in top and middle layers.However,there was an obvious difference between frictional model and observed data in the lower water column.Discrepancies are probably on account of stratification,which strengthens in summer and fall due to the freshening influence of the Changjiang River Estuary outflow.展开更多
ABSTRACT The abilities of BCC-AGCM2.1 and BCC_AGCM2.2 to simulate the annual-mean cloud vertical structure (CVS) were evaluated through comparison with GCM-Oriented CALIPSO Cloud Product (CALIPSO-GOCCP) data. BCC...ABSTRACT The abilities of BCC-AGCM2.1 and BCC_AGCM2.2 to simulate the annual-mean cloud vertical structure (CVS) were evaluated through comparison with GCM-Oriented CALIPSO Cloud Product (CALIPSO-GOCCP) data. BCC-AGCM2.2 has a dynamical core and physical processes that are consistent with BCC-AGCM2.1, but has a higher horizontal resolution. Results showed that both BCC-AGCM versions underestimated the global-mean total cloud cover (TCC), middle cloud cover (MCC) and low cloud cover (LCC), and that BCC_AGCM2.2 underestimated the global-mean high cloud cover (HCC). The global-mean cloud cover shows a systematic decrease from BCCA-GCM2.1 to BCC_AGCM2.2, especially for HCC. Geographically, HCC is significantly overestimated in the tropics, particularly by BCC_AGCM2,1, while LCC is generally overestimated over extra-tropical lands, but significantly underestimated over most of the oceans, especially for subtropical marine stratocumulus clouds. The leading EOF modes of CVS were extracted. The BCC_AGCMs perform well in reproducing EOF1, but with a larger variance explained. The two models also capture the basic features of EOF3, except an obvious deficiency in eigen- vector peaks. EOF2 has the largest simulation biases in both position and strength of eigenvector peaks. Furthermore, we investigated the effects of CVS on relative shortwave and longwave cloud radiative forcing (RSCRF and RLCRF). Both BCC_AGCM versions successfully reproduce the sign of regression coefficients, except for RLCRF in PC1. However, the RSCRF relative contributions from PC1 and PC2 are overestimated, while the relative contribution from PC3 is underes timated in both BCC_AGCM versions. The RLCRF relative contribution is underestimated for PC2 and overestimated for PC3.展开更多
This study investigates the vertical structure of variability in the cross-equatorial flows(CEFs)over the Maritime Continent and Indian Ocean in boreal summer,based on three reanalysis datasets:ERA-Interim,JRA-55 and ...This study investigates the vertical structure of variability in the cross-equatorial flows(CEFs)over the Maritime Continent and Indian Ocean in boreal summer,based on three reanalysis datasets:ERA-Interim,JRA-55 and NCEP-2.The results show a high consistency in the interannual variability among the reanalysis datasets,especially between ERAInterim and JRA-55,while great uncertainty exists in the decadal or long-term changes of CEFs.Further analyses on the interannual variability in CEFs indicate that there is a significant negative relationship between the upper-and lower-level CEFs over the Maritime Continent—that is,the northerlies at the upper level and southerlies at the lower level are both enhanced or weakened.This seesaw pattern is also significantly related to the CEFs over the Indian Ocean at the upper level and lower level(i.e.,the Somali jet).This close relationship between the upper-and lower-level CEFs and between the Maritime Continent and Indian Ocean is manifested as the leading mode of equatorial meridional winds in the vertical-zonal section over the Maritime Continent and Indian Ocean.Finally,it is found that ENSO is closely related to the vertical leading mode,and to all the CEFs at the upper and lower levels over the Maritime Continent and Indian Ocean.展开更多
The algebraic solitary wave and its associated eigenvalue problem in a deep stratified fluid with a free surface and a shallow upper layer were studied. And its vertical structure was examined. An exact solution for t...The algebraic solitary wave and its associated eigenvalue problem in a deep stratified fluid with a free surface and a shallow upper layer were studied. And its vertical structure was examined. An exact solution for the derived 2D Benjamin-Ono equation was obtained, and physical explanation was given with the corresponding dispersion relation. As a special case, the vertical structure of the weakly nonlinear internal wave for the Holmboe density distribution was numerically investigated, and the propagating mechanism of the internal wave was studied by using the ray theory.展开更多
Cloud profiling radar(CPR) onboard Cloud Sat allows for deep penetration into dense clouds/precipitation. In this study, tropical cyclones(TCs) are classified into three stages as developing, mature, and decaying. The...Cloud profiling radar(CPR) onboard Cloud Sat allows for deep penetration into dense clouds/precipitation. In this study, tropical cyclones(TCs) are classified into three stages as developing, mature, and decaying. The circular TC area with the radius of 500 km is divided into five regions. The vertical structure characteristics of 94 Western Pacific TCs at different stages in different regions from June 2006 to February 2014 are statistically quantified using the Cloud Sat tropical cyclone overpass product(the CSTC Product). Contoured frequency by altitude diagrams(CFADs) of radar reflectivity show an arc-like feature and exhibit opposite distributions with a boundary at 5 km. Bright bands are found at this altitude, indicating melting layers. Deep convective(DC) clouds have the largest occurrence probability in the inner region, while Ci clouds occur more frequently in the outer region at 10-15 km. As clouds have the second largest vertical scale after DC clouds. Distributions of Ac, Cu, and Ns clouds at different stages have few distinctions.As the altitude increases, the ice effective radius and the distribution width parameter decrease while the particle number concentration increases. Moist static energy(MSE), cloud thickness(CT), liquid water path(LWP), ice water path(IWP), water vapor(WV), and rain rate(RR) all diminish along the radial direction and are significantly larger at the mature stage. The average value of MSE at the developing stage is larger than that at the decaying stage.展开更多
The tidal current is generally predominant in China's offshore areas. The vertical structure of the observedtidal current is quite complicated with the presence of seasonal thermocline. The observed tidal current ...The tidal current is generally predominant in China's offshore areas. The vertical structure of the observedtidal current is quite complicated with the presence of seasonal thermocline. The observed tidal current may be divided into two parts, an averaged barotropic tide current and a variation tide current. A method for studying the vertical structure of tidal current is developed from the constitution and distribution of energy, and the vertical structure of the observed tide current in the North Huanghai Sea is studied on the basis of the method. The result shows that the reason why the energy of the tidal current is concentrated on the neighbourhood of the thermocline mainly lies in the internal tides i under certain conditions, the fact that the direction of the internal tide current above the thermocline is opposite to the one below the thermocline will be able to cause the rotary directions of the observed tidal current above and below the thermocline to be in opposite. The interaction between the averaged barotropic and the variation tide current plays an important role in forming the vertical structure of the tidal current, and it is mainly the interaction that results in the inho-mogeneous distribution of the tide current energy in the entire water column ; the ratio between the total energies of the internal tide current above the thermocline and the variation tide current in the entire water column is greater than the ratio between the total energies of that below the thermocline and the variation's. In a strong internal tide area such as the neighbourhood of Station L4, at diurnal tide frequency, the above-mentioned corresponding ratios are about 38. 82% and 29. 88%, respectively, and the energy of the internal tide current is about 68. 70%of the energy of the variation tide current; at semidiurnal tide frequency, the above-mentioned corresponding ratios are about 26. 61 % and 19. 73% , respectively, and the total internal tide current energy is about 46. 36% of the total variation tide current energy.展开更多
The development of efficient perovskite light-emitting diodes(PeLEDs)relies strongly on the fabrication of perovskite films with rationally designed structures(grain size,composition,surface,etc.).Therefore,an underst...The development of efficient perovskite light-emitting diodes(PeLEDs)relies strongly on the fabrication of perovskite films with rationally designed structures(grain size,composition,surface,etc.).Therefore,an understanding of structure-performance relationships is of vital importance for developing high-performance perovskite devices,particularly for devices with in-situ fabricated perovskite nanocrystal films.In this study,we reveal the vertical structure of an in-situ fabricated quasi-two-dimensional perovskite film.By combining time-of-flight secondary ion mass spectrometry,energy dispersive spectroscopy,grazing incidence wide-angle X-ray scattering(GIWAXS),and low-temperature photoluminescence spectra,we illustrate that the resulting in-situ fabricated DPPA_(2)Cs_(n-1)Pb_(n)(Br_(0.3)I_(0.7))_(3n+1)(DPPA^(+):3,3-diphenylpropylammonium)film has a gradient structure with a very thin layer of ligands on the surface,predominantly small-n domains at the top,and predominantly large-n domains at the bottom owing to the solubility difference of the precursors.In addition,GIWAXS measurements show that the domain of n=2 on the top layer has an ordered in-plane alignment.Based on the understanding of the film structure,we developed an in-situ fabrication process with ligand exchange to achieve efficient pure red PeLEDs at 638 nm with an average external quantum efficiency(EQE)of 7.4%.The optimized device had a maximum luminance of 623 cd/m^(2) with a peak EQE of 9.7%.展开更多
Turbulence in the nocturnal boundary layer(NBL)is still not well characterized,especially over complex underlying surfaces.Herein,gradient tower data and eddy covariance data collected by the Beijing 325-m tower were ...Turbulence in the nocturnal boundary layer(NBL)is still not well characterized,especially over complex underlying surfaces.Herein,gradient tower data and eddy covariance data collected by the Beijing 325-m tower were used to better understand the differentiating characteristics of turbulence regimes and vertical turbulence structure of urban the NBL.As for heights above the urban canopy layer(UCL),the relationship between turbulence velocity scale(VTKE)and wind speed(V)was consistent with the“HOckey-Stick”(HOST)theory proposed for a relatively flat area.Four regimes have been identified according to urban nocturnal stable boundary layer.Regime 1 occurs where local shear plays a leading role for weak turbulence under the constraint that the wind speed V<VT(threshold wind speed).Regime 2 is determined by the existence of strong turbulence that occurs when V>VT and is mainly driven by bulk shear.Regime 3 is identified by the existence of moderate turbulence when upside-down turbulence sporadic bursts occur in the presence of otherwise weak turbulence.Regime 4 is identified as buoyancy turbulence,when V>VT,and the turbulence regime is affected by a combination of local wind shear,bulk shear and buoyancy turbulence.The turbulence activities demonstrated a weak thermal stratification dependency in regime 1,for which within the UCL,the turbulence intensity was strongly affected by local wind shear when V<VT.This study further showed typical examples of different stable boundary layers and the variations between turbulence regimes by analyzing the evolution of wind vectors.Partly because of the influence of large-scale motions,the power spectral density of vertical velocity for upsidedown structure showed an increase at low frequencies.The upside-down structures were also characterized by the highest frequency of the stable stratifications in the higher layer.展开更多
Mêdog County,with its mountains and valleys,is located in the southeastern Tibetan Plateau(TP)and at the lower reaches of the Yarlung Zangbo River.This area has the highest annual rainfall amount over the TP,and ...Mêdog County,with its mountains and valleys,is located in the southeastern Tibetan Plateau(TP)and at the lower reaches of the Yarlung Zangbo River.This area has the highest annual rainfall amount over the TP,and in situ measurements are very scarce due to frequent debris flows and transportation difficulties.A monitoring campaign focused on cloud and precipitation observations was established in Mêdog in 2019 as a part of the Second Tibetan Plateau Scientific Expedition and Research Program.This paper evaluates the accuracy of micro rain radar(MRR)measurements and investigates the variations in precipitation vertical structure in Mêdog using observations collected from the MRR,disdrometer,and rain gauges in summer 2021.The measurements from the three instruments show a strong consistency,with correlation coefficients exceeding 0.93.Although the profiles of integral rain parameters for different rain rate categories in Mêdog are similar to those in other regions,the vertical evolution of raindrop size distributions shows significant differences.For lightest rain,the evaporation of small raindrops and breakup of large raindrops are clear during their descent.For the rainfall rate category of 0.2–2.0 mm h−1(2.0–20.0 mm h−1),concentrations of small and medium(large)drops show almost uniform vertical structures,while the large(medium)drop number displays a positive(negative)gradient.A disturbance at height of 1.5–2.0 km above ground level(AGL)is observed in the heavy rainfall due to strong updrafts.In general,the MRR measurements in Mêdog are robust.The raindrop breakup process is more apparent in Mêdog than in other regions,resulting in high concentration of sizelimited raindrops.In addition,it is found that the interaction between steep terrain and Mêdog convective rain causes the strong updrafts between 1.5 and 2.0 km AGL.展开更多
In this paper, the characteristics of the atmospheric boundary layer(ABL) vertical structure over the North China Plain(NCP) during a comprehensive observation experiment conducted during 15–21 December 2018 were inv...In this paper, the characteristics of the atmospheric boundary layer(ABL) vertical structure over the North China Plain(NCP) during a comprehensive observation experiment conducted during 15–21 December 2018 were investigated. Observational data were obtained with a large tethered balloon, Doppler wind lidar, and ground-level instruments. The maximum concentration of PM_(2.5) exceeded 200 μg m^(-3), and the ratio of PM_(2.5)/PM_(10) was approximately 0.4(its maxi-mum was approximately 0.8) during the whole observation period, indicating the explosive growth of dominant fine-mode aerosols in the winter heating season. Elevated concentrations of pollutants decreased the solar irradiance received by the ground, resulting in lower temperature at ground level. Our results illustrate three distinct types of vertical profiles: Type 1(convective state)—the concentration of PM_(2.5) decreased nearly linearly with increase of the height below approximately 600 m;Type 2(stable state)—the PM_(2.5) concentration sharply decreased from the ground to approximately 200 m;and Type 3(multilayer structure)—some pollutants were suspended aloft in the upper air layer. Diurnal evolution of the vertical profiles of PM_(2.5) and their relationship with the changes in meteorological factors were identified. From daytime to nighttime, the vertical profiles evolved from Type 1 to Type 2 or Type 3. All the 33 vertical PM_(2.5) profiles that we obtained showed a strong relationship with elements of the ABL structure, such as the distributions of winds, the inversion layer, and turbulence activities. A light-wind layer and weak turbulence activity, especially within the inversion layer, contributed greatly to the accumulation of pollutants.Vertical PM_(2.5) concentration patterns were also greatly affected by local ground-level emission sources and regional transport processes.展开更多
In June 2013,a field experiment was conducted in Southeast Tibet in which the air temperature,moisture,and wind were measured by using a GPS sounding system.In the present study,based on these observations and ERA-Int...In June 2013,a field experiment was conducted in Southeast Tibet in which the air temperature,moisture,and wind were measured by using a GPS sounding system.In the present study,based on these observations and ERA-Interim reanalysis data,the vertical structures of these atmospheric properties and the possible influence of the South Asian summer monsoon(SASM) were investigated.On average,the temperature had a lapse rate of 6.8℃ km^(-1) below the tropopause of 18.0 km.A strong moisture inversion occurred at the near-surface,with a strength of 1.7 g kg^(-1)(100 m)^(-1) for specific humidity.During the observation period,the SASM experienced a south phase and a north phase in the middle and by the end of June,respectively.The monsoon's evolution led to large changes in convection and circulation over Southeast Tibet,which further affected the local thermal,moisture,and circulation conditions.The strong convection resulted in an elevated tropopause height over Southeast Tibet during the north phase of the SASM,and the large-scale warm and wet air masses delivered by the monsoon caused high local temperature and moisture conditions.展开更多
Agroforests are man-made ecosystems in which crops are associated with a main perennial species like Robusta Coffee Agroforests (RCAs), which is counted among the main modes of perennial crops production in Cameroon. ...Agroforests are man-made ecosystems in which crops are associated with a main perennial species like Robusta Coffee Agroforests (RCAs), which is counted among the main modes of perennial crops production in Cameroon. Despite the rich ecosystem services provided, the diversity of Associated Species (AS) found in these RCAs and the structure of the landscapes they form remain little known in Cameroon. The current study aimed to inventory AS and characterize the structure of RCAs in four sites (Ayos, Malantouen, Melong and Nkongsamba) belonging to three robusta coffee production basins in Cameroon. A systematic inventory with dendrometric measurements of the wood AS and coffee trees was carried out on 120 one-hectare plot unit, i.e. 30 plots per site. The results showed that 102 AS belonging to 83 genera and 41 families were identified in these RCAs. The RCAs of Ayos in the dense rainforest zone with bimodal rainfall pattern were the most diverse with 71 species, followed by those of Melong and Nkongsamba with respectively 39 and 33 species respectively in the dense rainforest zone with monomodal rainfall pattern, and Malantouen with 33 species in the high savannahs of the west. Structurally, average coffee tree and AS densities founded ranged from 1208 - 1456 plants/ha and 71 - 214 stems/ha and those of basal area from 7.29 - 17.40 m<sup>2</sup>/ha for coffee trees and 7.97 - 16.14 m<sup>2</sup>/ha for AS in function of site. Basis on the vertical stratification, the proportion of the 3 - 6 m stratum, which is mainly represented by introduced AS, varied from 38% - 62% depending on the site. The results of this study showed that RCAs contribute to the conservation of plant biodiversity, given the specific richness identified in these ecosystems.展开更多
The sensitive area of targeted observations for short-term(7 d)prediction of vertical thermal structure(VTS)in summer in the Yellow Sea was investigated.We applied the Conditional Nonlinear Optimal Perturbation(CNOP)m...The sensitive area of targeted observations for short-term(7 d)prediction of vertical thermal structure(VTS)in summer in the Yellow Sea was investigated.We applied the Conditional Nonlinear Optimal Perturbation(CNOP)method and an adjoint-free algorithm with the Regional Ocean Modeling System(ROMS).We used vertical integration of CNOP-type temperature errors to locate the sensitive areas,where reduction of initial errors is expected to yield the greatest improvement in VTS prediction for the selected verification area.The identified sensitive areas were northeast−southwest orientated northeast to the verification area,which were possibly related to the southwestward background currents.Then,we performed a series of sensitivity experiments to evaluate the effectiveness of the identified sensitive areas.Results show that initial errors in the identified sensitive areas had the greatest negative effect on VTS prediction in the verification area compared to errors in other areas(e.g.,the verification area and areas to its east and northeast).Moreover,removal of initial errors through deploying simulated observations in the identified sensitive areas led to more refined prediction than correction of initial conditions in the verification area itself.Our results suggest that implementation of targeted observation in the CNOP-based sensitive areas is an effective method to improve short-term prediction of VTS in summer in the Yellow Sea.展开更多
In this paper, on the basis of the heat conduction equation without consideration of the advection and turbulence effects, one-dimensional model for describing surface sea temperature ( T1), bottom sea temperature ( T...In this paper, on the basis of the heat conduction equation without consideration of the advection and turbulence effects, one-dimensional model for describing surface sea temperature ( T1), bottom sea temperature ( Tt ) and the thickness of the upper homogeneous layer ( h ) is developed in terms of the dimensionless temperature θT and depth η and self-simulation function θT - f(η) of vertical temperature profile by means of historical temperature data.The results of trial prediction with our one-dimensional model on T, Th, h , the thickness and gradient of thermocline are satisfactory to some extent.展开更多
Based on L-band sounding data,threshold method of relative humidity was used to analyze vertical distribution characteristics of precipitation cloud system in Tianjin region.The results showed that main precipitation ...Based on L-band sounding data,threshold method of relative humidity was used to analyze vertical distribution characteristics of precipitation cloud system in Tianjin region.The results showed that main precipitation cloud system affecting Tianjin is cold and warm mixed cloud,followed by cold cloud,and precipitation of warm cloud is less.During May-November,precipitation of cold and warm mixed cloud is dominant,and it is dominant by precipitation of cold cloud from January to April.In four seasons,the precipitation frequency of double-layer cloud is the most,and precipitation of single-layer cloud mainly appears during March-November,and peak is in June.Peak of cloud system with three or more layers all appears in July and August.The cold cloud and warm cloud catalysts should be selected respectively for artificial precipitation enhancement in Tianjin.In winter,cold cloud catalyst operation is selected;in spring,summer and autumn,the cold cloud catalyst is spread in the cold cloud area,and the warm cloud catalyst is distributed in the warm cloud area according to the conditions of cloud layer.展开更多
Vertical differential structural deformation(VDSD),one of the most significant structural characteristics of strike-slip fault zones(SSFZs)in the Shunbei area,is crucial for understanding deformation in the SSFZ and i...Vertical differential structural deformation(VDSD),one of the most significant structural characteristics of strike-slip fault zones(SSFZs)in the Shunbei area,is crucial for understanding deformation in the SSFZ and its hydrocarbon accumulation significance.Based on drilling data and high-precision 3-D seismic data,we analyzed the geometric and kinematic characteristics of the SSFZs in the Shunbei area.Coupled with the stratification of the rock mechanism,the structural deformations of these SSFZs in different formations were differentiated and divided into four deformation layers.According to comprehensive structural interpretations and comparisons,three integrated 3-D structural models could describe the VDSD of these SSFZs.The time-space coupling of the material basis(rock mechanism stratification),changing dynamic conditions(e.g.,changing stress-strain states),and special deformation mechanism of the en echelon normal fault array uniformly controlled the formation of the VDSD in the SSFZs of the Shunbei area.The VDSD of the SSFZs in this area controlled the entire hydrocarbon accumulation process.Multi-stage structural superimposing deformation influenced the hydrocarbon migration,accumulation,distribution,preservation,and secondary adjustments.展开更多
This study evaluates the vertical profiles of aerosol and cloud optical properties in 40 dominated dust and smoke regions in Western-Northern Africa (WNA) and Central-Southern Africa (CSA), respectively, from the surf...This study evaluates the vertical profiles of aerosol and cloud optical properties in 40 dominated dust and smoke regions in Western-Northern Africa (WNA) and Central-Southern Africa (CSA), respectively, from the surface to 10km and from 2008 to 2011 based on LIVAS (LIdar climatology of Vertical Aerosol Structure for space-based lidar simulation studies). Aerosol extinction (AE), aerosol backscatter (AB), and aerosol depolarization (AD) generally increase from the surface to 1.2 km and decrease from 1.2 km to the upper layers in both WNA and CSA. AE and AB in CSA (maximum of 0.13 km<sup>-1</sup>, 0.14 km<sup>-1</sup>, 0.0021 km<sup>-1</sup>‧sr<sup>-1</sup>, 0.0033 km<sup>-1</sup>‧sr<sup>-1</sup>) are higher than in WNA (maximum of 0.07 km<sup>-1</sup>, 0.08 km<sup>-1</sup>, 0.0017 km<sup>-1</sup>‧sr<sup>-1</sup>, 0.0015 km<sup>-1</sup>‧sr<sup>-1</sup>) at 532 and 1064 nm respectively. AD in WNA (maximum of 0.25) is significantly higher than in CSA (maximum of 0.05). There is a smooth change with the height of cloud extinction and backscatter in WNA and CSA, while there is a remarkable increase of cloud depolarization with height, whereby it is high in CSA and low in WNA due to high and low fraction of cirrus respectively. Altocumulus has the highest extinction in NA (0.0139 km<sup>-1</sup>), CA (0.058 km<sup>-1</sup>), WA (0.013 km<sup>-1</sup>), while low overcast transparent (0.76 km<sup>-1</sup>) below 1 km in SA. The major findings of this study may contribute to the improvement of our understanding of aerosol-cloud interaction studies in dominated dust and smoke aerosol regions.展开更多
A n-type small molecule DC-IDT2E with 4,4,9,9-tetrakis(4-hexylphenyl)-indaceno[1,2-b:5,6-bt]dithiophene as a central building block, furan as rr-bridges, and 1,1 -dicyanomethylene-3-indanone as end acceptor groups,...A n-type small molecule DC-IDT2E with 4,4,9,9-tetrakis(4-hexylphenyl)-indaceno[1,2-b:5,6-bt]dithiophene as a central building block, furan as rr-bridges, and 1,1 -dicyanomethylene-3-indanone as end acceptor groups, was synthesized and used as an electron acceptor in solution-processed organic solar cells (OSCs). DC-IDT2F exhibited good thermal stability, broad and strong absorption in 500-850 rim, a narrow bandgap of 1.54 eV, LUMO of-3.88 eV, HOMO of-5.44 eV and an electron mobility of 6.5 × 10-4 cm2/(V.s). DC-IDT2F-based OSCs with conventional and inverted structures exhibited power conversion efficiencies of 2.26 and 3.08% respec- tively. The effect of vertical phase separation and morphology of the active layer on the device performance in the two structures was studied.展开更多
The spatial distribution and seasonal variations of the hypoxic zone in the eastern equatorial Indian Ocean were investigated using survey data collected from four cruises from 2013 to 2018.Results showed that hypoxic...The spatial distribution and seasonal variations of the hypoxic zone in the eastern equatorial Indian Ocean were investigated using survey data collected from four cruises from 2013 to 2018.Results showed that hypoxic zone occurred all year round in the eastern equatorial Indian Ocean,and it spread southward in the shape of a double tongue at two depths with one at subsurface centered at a depth of 150 m and the other in intermediate water centered at a depth of 800 m.The southward expansion and maximum thickness of the hypoxic zone were greatest in the spring inter-monsoon and least in the summer monsoon.The hypoxic zone originated from the southward expansion of the hypoxic water in the Bay of Bengal and its spatial distribution was driven by southward output flux of mid-deep(100–1000 m)hypoxic water from the Bay of Bengal.The hypoxia southward expansion was blocked near the equator in the subsurface layer,because of mixing with multiple zonal circulations(e.g.,Wyrtki Jets and the equatorial undercurrent),which meant that the hypoxic zone extended over a smaller area than in the intermediate water.These new findings will contribute to an improved understanding of the hypoxic zone and will contribute to circulation research,particularly about intermediate circulation in the eastern equatorial Indian Ocean.展开更多
The accuracies of three instruments in measuring atmospheric column humidity were assessed during an upper troposphere and lower stratosphere observation campaign conducted from 7 to 13 August 2009 in Kunming, China. ...The accuracies of three instruments in measuring atmospheric column humidity were assessed during an upper troposphere and lower stratosphere observation campaign conducted from 7 to 13 August 2009 in Kunming, China. The three instruments are a cryogenic frost-point hygrometer (CFH), a Vaisala RS80 radiosonde (RS80), and a GTS1 radiosonde (GTS1). The accuracy of relative humidity (RH) measurements made by the CFH, GTS1, and RS80 was similar between the surface and 500 hPa (~5.5 km above sea level). However, above 500 hPa, the errors in RH measurements made by the RS80, relative to measurements made by the CFH, are much less than those detected with the GTS1. Three different retrieval methods for determining cloud boundaries from CFH, RS80, and GTS1 measurements were developed and take into account the differences in accuracy among the three instruments. The method for the CFH is based on RH thresholds at all levels, which demands high accuracy. Given that the accuracy of RH measurements decreases at higher altitudes, the cloud detection methods for RS80 and GTS1 are different for different altitude ranges. Below 5 km, the methods for the RS80 and the GTS1 are similar to that of the CFH; above 5 km, the methods for the RS80 and the GTS1 are both developed based on the second-order derivatives of temperature and RH with respect to height, but with different criteria applied. Comparisons of cloud-layer retrievals derived from the three measurements are also made.展开更多
基金The National Natural Science Foundation of China under contract Nos 41806114 and 42266006the Jiangxi Provincial Natural Science Foundation under contract Nos 20202ACBL214019,20181BAB216031 and 20212BBE53031+2 种基金the Technological Innovation and Application Development in Chongqing under contract No.CSTB2022TIAD-GPX0016the Incentive and Guidance Project of Scientific Research Performance for Scientific Research Institutes in Chongqing under contract No.cstc2021jxjl120017the Open Fund of the Key Laboratory of Marine Environmental Survey Technology and Application of Ministry of Natural Resources under contract Nos MESTA-2020-A002 and MESTA-2021-B001.
文摘Three long-term fixed acoustic Doppler current profilers were first used for investigating the vertical structure of tidal currents in Xuliujing Section of Changjiang River Estuary.Moreover,three different periods(spring,summer and fall)were also considered for investigating seasonal variations.The semi-diurnal tides were the most energetic,with along-channel speed of up to 80 cm/s for M_(2)constituent,which dominates at all stations with percent energy up to 65%–75%during seasons.The shape of tidal ellipses of the most energetic semi-diurnal constituent M_(2)showed obvious polarization of the flow paralleling to the riverbank,with the minor semi-axis being generally less than 20%of the major one.The maximum velocity of mean current is appeared in top layers at all the three stations,and the velocity decreased with the depth.The seasonal variations of direction are also observed,which is probably caused by complex local topography since the erosion and deposition in riverbed.Observed vertical variation of four parameters of M_(2)ellipses,agreed well with the optimally fit frictional solutions in top and middle layers.However,there was an obvious difference between frictional model and observed data in the lower water column.Discrepancies are probably on account of stratification,which strengthens in summer and fall due to the freshening influence of the Changjiang River Estuary outflow.
基金jointly supported by the National Natural Science Foundation of China (Grant Nos.41275077 and 41105054)the National Basic Research Program of China (973 Program:2010CB951902)+1 种基金the China Meteorological Administration (Grant Nos.GYHY201106022 and GYHY201306048)the Sun Yat-sen University "985 Project", Phase 3
文摘ABSTRACT The abilities of BCC-AGCM2.1 and BCC_AGCM2.2 to simulate the annual-mean cloud vertical structure (CVS) were evaluated through comparison with GCM-Oriented CALIPSO Cloud Product (CALIPSO-GOCCP) data. BCC-AGCM2.2 has a dynamical core and physical processes that are consistent with BCC-AGCM2.1, but has a higher horizontal resolution. Results showed that both BCC-AGCM versions underestimated the global-mean total cloud cover (TCC), middle cloud cover (MCC) and low cloud cover (LCC), and that BCC_AGCM2.2 underestimated the global-mean high cloud cover (HCC). The global-mean cloud cover shows a systematic decrease from BCCA-GCM2.1 to BCC_AGCM2.2, especially for HCC. Geographically, HCC is significantly overestimated in the tropics, particularly by BCC_AGCM2,1, while LCC is generally overestimated over extra-tropical lands, but significantly underestimated over most of the oceans, especially for subtropical marine stratocumulus clouds. The leading EOF modes of CVS were extracted. The BCC_AGCMs perform well in reproducing EOF1, but with a larger variance explained. The two models also capture the basic features of EOF3, except an obvious deficiency in eigen- vector peaks. EOF2 has the largest simulation biases in both position and strength of eigenvector peaks. Furthermore, we investigated the effects of CVS on relative shortwave and longwave cloud radiative forcing (RSCRF and RLCRF). Both BCC_AGCM versions successfully reproduce the sign of regression coefficients, except for RLCRF in PC1. However, the RSCRF relative contributions from PC1 and PC2 are overestimated, while the relative contribution from PC3 is underes timated in both BCC_AGCM versions. The RLCRF relative contribution is underestimated for PC2 and overestimated for PC3.
基金supported by the National Natural Science Foundation of China (Grant No. 41721004)
文摘This study investigates the vertical structure of variability in the cross-equatorial flows(CEFs)over the Maritime Continent and Indian Ocean in boreal summer,based on three reanalysis datasets:ERA-Interim,JRA-55 and NCEP-2.The results show a high consistency in the interannual variability among the reanalysis datasets,especially between ERAInterim and JRA-55,while great uncertainty exists in the decadal or long-term changes of CEFs.Further analyses on the interannual variability in CEFs indicate that there is a significant negative relationship between the upper-and lower-level CEFs over the Maritime Continent—that is,the northerlies at the upper level and southerlies at the lower level are both enhanced or weakened.This seesaw pattern is also significantly related to the CEFs over the Indian Ocean at the upper level and lower level(i.e.,the Somali jet).This close relationship between the upper-and lower-level CEFs and between the Maritime Continent and Indian Ocean is manifested as the leading mode of equatorial meridional winds in the vertical-zonal section over the Maritime Continent and Indian Ocean.Finally,it is found that ENSO is closely related to the vertical leading mode,and to all the CEFs at the upper and lower levels over the Maritime Continent and Indian Ocean.
文摘The algebraic solitary wave and its associated eigenvalue problem in a deep stratified fluid with a free surface and a shallow upper layer were studied. And its vertical structure was examined. An exact solution for the derived 2D Benjamin-Ono equation was obtained, and physical explanation was given with the corresponding dispersion relation. As a special case, the vertical structure of the weakly nonlinear internal wave for the Holmboe density distribution was numerically investigated, and the propagating mechanism of the internal wave was studied by using the ray theory.
基金National Natural Science Foundation of China(41076118)Young Scientists Fund of National Natural Science Foundation of China Grant(41005018)
文摘Cloud profiling radar(CPR) onboard Cloud Sat allows for deep penetration into dense clouds/precipitation. In this study, tropical cyclones(TCs) are classified into three stages as developing, mature, and decaying. The circular TC area with the radius of 500 km is divided into five regions. The vertical structure characteristics of 94 Western Pacific TCs at different stages in different regions from June 2006 to February 2014 are statistically quantified using the Cloud Sat tropical cyclone overpass product(the CSTC Product). Contoured frequency by altitude diagrams(CFADs) of radar reflectivity show an arc-like feature and exhibit opposite distributions with a boundary at 5 km. Bright bands are found at this altitude, indicating melting layers. Deep convective(DC) clouds have the largest occurrence probability in the inner region, while Ci clouds occur more frequently in the outer region at 10-15 km. As clouds have the second largest vertical scale after DC clouds. Distributions of Ac, Cu, and Ns clouds at different stages have few distinctions.As the altitude increases, the ice effective radius and the distribution width parameter decrease while the particle number concentration increases. Moist static energy(MSE), cloud thickness(CT), liquid water path(LWP), ice water path(IWP), water vapor(WV), and rain rate(RR) all diminish along the radial direction and are significantly larger at the mature stage. The average value of MSE at the developing stage is larger than that at the decaying stage.
基金The project supported by National Natural science Foundation of China
文摘The tidal current is generally predominant in China's offshore areas. The vertical structure of the observedtidal current is quite complicated with the presence of seasonal thermocline. The observed tidal current may be divided into two parts, an averaged barotropic tide current and a variation tide current. A method for studying the vertical structure of tidal current is developed from the constitution and distribution of energy, and the vertical structure of the observed tide current in the North Huanghai Sea is studied on the basis of the method. The result shows that the reason why the energy of the tidal current is concentrated on the neighbourhood of the thermocline mainly lies in the internal tides i under certain conditions, the fact that the direction of the internal tide current above the thermocline is opposite to the one below the thermocline will be able to cause the rotary directions of the observed tidal current above and below the thermocline to be in opposite. The interaction between the averaged barotropic and the variation tide current plays an important role in forming the vertical structure of the tidal current, and it is mainly the interaction that results in the inho-mogeneous distribution of the tide current energy in the entire water column ; the ratio between the total energies of the internal tide current above the thermocline and the variation tide current in the entire water column is greater than the ratio between the total energies of that below the thermocline and the variation's. In a strong internal tide area such as the neighbourhood of Station L4, at diurnal tide frequency, the above-mentioned corresponding ratios are about 38. 82% and 29. 88%, respectively, and the energy of the internal tide current is about 68. 70%of the energy of the variation tide current; at semidiurnal tide frequency, the above-mentioned corresponding ratios are about 26. 61 % and 19. 73% , respectively, and the total internal tide current energy is about 46. 36% of the total variation tide current energy.
基金supported by the National Natural Science Foundation of China(61735004).
文摘The development of efficient perovskite light-emitting diodes(PeLEDs)relies strongly on the fabrication of perovskite films with rationally designed structures(grain size,composition,surface,etc.).Therefore,an understanding of structure-performance relationships is of vital importance for developing high-performance perovskite devices,particularly for devices with in-situ fabricated perovskite nanocrystal films.In this study,we reveal the vertical structure of an in-situ fabricated quasi-two-dimensional perovskite film.By combining time-of-flight secondary ion mass spectrometry,energy dispersive spectroscopy,grazing incidence wide-angle X-ray scattering(GIWAXS),and low-temperature photoluminescence spectra,we illustrate that the resulting in-situ fabricated DPPA_(2)Cs_(n-1)Pb_(n)(Br_(0.3)I_(0.7))_(3n+1)(DPPA^(+):3,3-diphenylpropylammonium)film has a gradient structure with a very thin layer of ligands on the surface,predominantly small-n domains at the top,and predominantly large-n domains at the bottom owing to the solubility difference of the precursors.In addition,GIWAXS measurements show that the domain of n=2 on the top layer has an ordered in-plane alignment.Based on the understanding of the film structure,we developed an in-situ fabrication process with ligand exchange to achieve efficient pure red PeLEDs at 638 nm with an average external quantum efficiency(EQE)of 7.4%.The optimized device had a maximum luminance of 623 cd/m^(2) with a peak EQE of 9.7%.
基金supported by the National Natural Science Foundation of China (Grant No. 42105093 and 41975018)the China Postdoctoral Science Foundation (Grant No. 2020M670420)the Special Research Assistant Project。
文摘Turbulence in the nocturnal boundary layer(NBL)is still not well characterized,especially over complex underlying surfaces.Herein,gradient tower data and eddy covariance data collected by the Beijing 325-m tower were used to better understand the differentiating characteristics of turbulence regimes and vertical turbulence structure of urban the NBL.As for heights above the urban canopy layer(UCL),the relationship between turbulence velocity scale(VTKE)and wind speed(V)was consistent with the“HOckey-Stick”(HOST)theory proposed for a relatively flat area.Four regimes have been identified according to urban nocturnal stable boundary layer.Regime 1 occurs where local shear plays a leading role for weak turbulence under the constraint that the wind speed V<VT(threshold wind speed).Regime 2 is determined by the existence of strong turbulence that occurs when V>VT and is mainly driven by bulk shear.Regime 3 is identified by the existence of moderate turbulence when upside-down turbulence sporadic bursts occur in the presence of otherwise weak turbulence.Regime 4 is identified as buoyancy turbulence,when V>VT,and the turbulence regime is affected by a combination of local wind shear,bulk shear and buoyancy turbulence.The turbulence activities demonstrated a weak thermal stratification dependency in regime 1,for which within the UCL,the turbulence intensity was strongly affected by local wind shear when V<VT.This study further showed typical examples of different stable boundary layers and the variations between turbulence regimes by analyzing the evolution of wind vectors.Partly because of the influence of large-scale motions,the power spectral density of vertical velocity for upsidedown structure showed an increase at low frequencies.The upside-down structures were also characterized by the highest frequency of the stable stratifications in the higher layer.
基金Supported by the Second Tibetan Plateau Scientific Expedition and Research(STEP)Program(2019QZKK0105)National Key Research and Development Program of China(2018YFC1505702).
文摘Mêdog County,with its mountains and valleys,is located in the southeastern Tibetan Plateau(TP)and at the lower reaches of the Yarlung Zangbo River.This area has the highest annual rainfall amount over the TP,and in situ measurements are very scarce due to frequent debris flows and transportation difficulties.A monitoring campaign focused on cloud and precipitation observations was established in Mêdog in 2019 as a part of the Second Tibetan Plateau Scientific Expedition and Research Program.This paper evaluates the accuracy of micro rain radar(MRR)measurements and investigates the variations in precipitation vertical structure in Mêdog using observations collected from the MRR,disdrometer,and rain gauges in summer 2021.The measurements from the three instruments show a strong consistency,with correlation coefficients exceeding 0.93.Although the profiles of integral rain parameters for different rain rate categories in Mêdog are similar to those in other regions,the vertical evolution of raindrop size distributions shows significant differences.For lightest rain,the evaporation of small raindrops and breakup of large raindrops are clear during their descent.For the rainfall rate category of 0.2–2.0 mm h−1(2.0–20.0 mm h−1),concentrations of small and medium(large)drops show almost uniform vertical structures,while the large(medium)drop number displays a positive(negative)gradient.A disturbance at height of 1.5–2.0 km above ground level(AGL)is observed in the heavy rainfall due to strong updrafts.In general,the MRR measurements in Mêdog are robust.The raindrop breakup process is more apparent in Mêdog than in other regions,resulting in high concentration of sizelimited raindrops.In addition,it is found that the interaction between steep terrain and Mêdog convective rain causes the strong updrafts between 1.5 and 2.0 km AGL.
基金Supported by the National Key Research and Development Program of China (2017YFC0209605)National Natural Science Foundation of China (41975108)General Financial Grant from the China Postdoctoral Science Foundation (2020M670420)。
文摘In this paper, the characteristics of the atmospheric boundary layer(ABL) vertical structure over the North China Plain(NCP) during a comprehensive observation experiment conducted during 15–21 December 2018 were investigated. Observational data were obtained with a large tethered balloon, Doppler wind lidar, and ground-level instruments. The maximum concentration of PM_(2.5) exceeded 200 μg m^(-3), and the ratio of PM_(2.5)/PM_(10) was approximately 0.4(its maxi-mum was approximately 0.8) during the whole observation period, indicating the explosive growth of dominant fine-mode aerosols in the winter heating season. Elevated concentrations of pollutants decreased the solar irradiance received by the ground, resulting in lower temperature at ground level. Our results illustrate three distinct types of vertical profiles: Type 1(convective state)—the concentration of PM_(2.5) decreased nearly linearly with increase of the height below approximately 600 m;Type 2(stable state)—the PM_(2.5) concentration sharply decreased from the ground to approximately 200 m;and Type 3(multilayer structure)—some pollutants were suspended aloft in the upper air layer. Diurnal evolution of the vertical profiles of PM_(2.5) and their relationship with the changes in meteorological factors were identified. From daytime to nighttime, the vertical profiles evolved from Type 1 to Type 2 or Type 3. All the 33 vertical PM_(2.5) profiles that we obtained showed a strong relationship with elements of the ABL structure, such as the distributions of winds, the inversion layer, and turbulence activities. A light-wind layer and weak turbulence activity, especially within the inversion layer, contributed greatly to the accumulation of pollutants.Vertical PM_(2.5) concentration patterns were also greatly affected by local ground-level emission sources and regional transport processes.
基金Supported by the China Meteorological Administration Special Public Welfare Research Fund(GYHY201206041)Project of Comprehensive Evaluation of Polar Areas on Global and Regional Climate Changes(CHINARE2016-04-04)Polar Environment Comprehensive Investigation and Assessment(CHINARE2016-02-03)
文摘In June 2013,a field experiment was conducted in Southeast Tibet in which the air temperature,moisture,and wind were measured by using a GPS sounding system.In the present study,based on these observations and ERA-Interim reanalysis data,the vertical structures of these atmospheric properties and the possible influence of the South Asian summer monsoon(SASM) were investigated.On average,the temperature had a lapse rate of 6.8℃ km^(-1) below the tropopause of 18.0 km.A strong moisture inversion occurred at the near-surface,with a strength of 1.7 g kg^(-1)(100 m)^(-1) for specific humidity.During the observation period,the SASM experienced a south phase and a north phase in the middle and by the end of June,respectively.The monsoon's evolution led to large changes in convection and circulation over Southeast Tibet,which further affected the local thermal,moisture,and circulation conditions.The strong convection resulted in an elevated tropopause height over Southeast Tibet during the north phase of the SASM,and the large-scale warm and wet air masses delivered by the monsoon caused high local temperature and moisture conditions.
文摘Agroforests are man-made ecosystems in which crops are associated with a main perennial species like Robusta Coffee Agroforests (RCAs), which is counted among the main modes of perennial crops production in Cameroon. Despite the rich ecosystem services provided, the diversity of Associated Species (AS) found in these RCAs and the structure of the landscapes they form remain little known in Cameroon. The current study aimed to inventory AS and characterize the structure of RCAs in four sites (Ayos, Malantouen, Melong and Nkongsamba) belonging to three robusta coffee production basins in Cameroon. A systematic inventory with dendrometric measurements of the wood AS and coffee trees was carried out on 120 one-hectare plot unit, i.e. 30 plots per site. The results showed that 102 AS belonging to 83 genera and 41 families were identified in these RCAs. The RCAs of Ayos in the dense rainforest zone with bimodal rainfall pattern were the most diverse with 71 species, followed by those of Melong and Nkongsamba with respectively 39 and 33 species respectively in the dense rainforest zone with monomodal rainfall pattern, and Malantouen with 33 species in the high savannahs of the west. Structurally, average coffee tree and AS densities founded ranged from 1208 - 1456 plants/ha and 71 - 214 stems/ha and those of basal area from 7.29 - 17.40 m<sup>2</sup>/ha for coffee trees and 7.97 - 16.14 m<sup>2</sup>/ha for AS in function of site. Basis on the vertical stratification, the proportion of the 3 - 6 m stratum, which is mainly represented by introduced AS, varied from 38% - 62% depending on the site. The results of this study showed that RCAs contribute to the conservation of plant biodiversity, given the specific richness identified in these ecosystems.
基金The National Natural Science Foundation of China under contract Nos 41705081 and 41906005the Innovation Special Zone Project under contract No.18-H863-05-ZT-001-012-06the Open Project Fund of the Laboratory for Regional Oceanography and Numerical Modeling,Pilot National Laboratory for Marine Science and Technology(Qingdao)under contract No.2019A05.
文摘The sensitive area of targeted observations for short-term(7 d)prediction of vertical thermal structure(VTS)in summer in the Yellow Sea was investigated.We applied the Conditional Nonlinear Optimal Perturbation(CNOP)method and an adjoint-free algorithm with the Regional Ocean Modeling System(ROMS).We used vertical integration of CNOP-type temperature errors to locate the sensitive areas,where reduction of initial errors is expected to yield the greatest improvement in VTS prediction for the selected verification area.The identified sensitive areas were northeast−southwest orientated northeast to the verification area,which were possibly related to the southwestward background currents.Then,we performed a series of sensitivity experiments to evaluate the effectiveness of the identified sensitive areas.Results show that initial errors in the identified sensitive areas had the greatest negative effect on VTS prediction in the verification area compared to errors in other areas(e.g.,the verification area and areas to its east and northeast).Moreover,removal of initial errors through deploying simulated observations in the identified sensitive areas led to more refined prediction than correction of initial conditions in the verification area itself.Our results suggest that implementation of targeted observation in the CNOP-based sensitive areas is an effective method to improve short-term prediction of VTS in summer in the Yellow Sea.
文摘In this paper, on the basis of the heat conduction equation without consideration of the advection and turbulence effects, one-dimensional model for describing surface sea temperature ( T1), bottom sea temperature ( Tt ) and the thickness of the upper homogeneous layer ( h ) is developed in terms of the dimensionless temperature θT and depth η and self-simulation function θT - f(η) of vertical temperature profile by means of historical temperature data.The results of trial prediction with our one-dimensional model on T, Th, h , the thickness and gradient of thermocline are satisfactory to some extent.
基金Supported by Open Research Fund Project of Key Laboratory of Meteorology and Ecological Environment of Hebei Province(Z202001Z,Z201602Z)Science and Technology Collaborative Innovation Fund Project in Bohai Rim Region(QYXM202004)Key Projects of Tianjin Meteorological Bureau(201801zdxm01)。
文摘Based on L-band sounding data,threshold method of relative humidity was used to analyze vertical distribution characteristics of precipitation cloud system in Tianjin region.The results showed that main precipitation cloud system affecting Tianjin is cold and warm mixed cloud,followed by cold cloud,and precipitation of warm cloud is less.During May-November,precipitation of cold and warm mixed cloud is dominant,and it is dominant by precipitation of cold cloud from January to April.In four seasons,the precipitation frequency of double-layer cloud is the most,and precipitation of single-layer cloud mainly appears during March-November,and peak is in June.Peak of cloud system with three or more layers all appears in July and August.The cold cloud and warm cloud catalysts should be selected respectively for artificial precipitation enhancement in Tianjin.In winter,cold cloud catalyst operation is selected;in spring,summer and autumn,the cold cloud catalyst is spread in the cold cloud area,and the warm cloud catalyst is distributed in the warm cloud area according to the conditions of cloud layer.
基金financially supported by the China Petroleum&Chemical Corporation(SINOPEC)(Grant No.P18047-2)the National Natural Science Foundation of China(Grant No.U19B6003-01)the National Key Research and Development Program of China(Grant No.2017YFC0601405)。
文摘Vertical differential structural deformation(VDSD),one of the most significant structural characteristics of strike-slip fault zones(SSFZs)in the Shunbei area,is crucial for understanding deformation in the SSFZ and its hydrocarbon accumulation significance.Based on drilling data and high-precision 3-D seismic data,we analyzed the geometric and kinematic characteristics of the SSFZs in the Shunbei area.Coupled with the stratification of the rock mechanism,the structural deformations of these SSFZs in different formations were differentiated and divided into four deformation layers.According to comprehensive structural interpretations and comparisons,three integrated 3-D structural models could describe the VDSD of these SSFZs.The time-space coupling of the material basis(rock mechanism stratification),changing dynamic conditions(e.g.,changing stress-strain states),and special deformation mechanism of the en echelon normal fault array uniformly controlled the formation of the VDSD in the SSFZs of the Shunbei area.The VDSD of the SSFZs in this area controlled the entire hydrocarbon accumulation process.Multi-stage structural superimposing deformation influenced the hydrocarbon migration,accumulation,distribution,preservation,and secondary adjustments.
文摘This study evaluates the vertical profiles of aerosol and cloud optical properties in 40 dominated dust and smoke regions in Western-Northern Africa (WNA) and Central-Southern Africa (CSA), respectively, from the surface to 10km and from 2008 to 2011 based on LIVAS (LIdar climatology of Vertical Aerosol Structure for space-based lidar simulation studies). Aerosol extinction (AE), aerosol backscatter (AB), and aerosol depolarization (AD) generally increase from the surface to 1.2 km and decrease from 1.2 km to the upper layers in both WNA and CSA. AE and AB in CSA (maximum of 0.13 km<sup>-1</sup>, 0.14 km<sup>-1</sup>, 0.0021 km<sup>-1</sup>‧sr<sup>-1</sup>, 0.0033 km<sup>-1</sup>‧sr<sup>-1</sup>) are higher than in WNA (maximum of 0.07 km<sup>-1</sup>, 0.08 km<sup>-1</sup>, 0.0017 km<sup>-1</sup>‧sr<sup>-1</sup>, 0.0015 km<sup>-1</sup>‧sr<sup>-1</sup>) at 532 and 1064 nm respectively. AD in WNA (maximum of 0.25) is significantly higher than in CSA (maximum of 0.05). There is a smooth change with the height of cloud extinction and backscatter in WNA and CSA, while there is a remarkable increase of cloud depolarization with height, whereby it is high in CSA and low in WNA due to high and low fraction of cirrus respectively. Altocumulus has the highest extinction in NA (0.0139 km<sup>-1</sup>), CA (0.058 km<sup>-1</sup>), WA (0.013 km<sup>-1</sup>), while low overcast transparent (0.76 km<sup>-1</sup>) below 1 km in SA. The major findings of this study may contribute to the improvement of our understanding of aerosol-cloud interaction studies in dominated dust and smoke aerosol regions.
基金supported by the National Natural Science Foundation of China(91433114,51261130582,21025418)the 973 Program(2011CB808401)the Chinese Academy of Sciences
文摘A n-type small molecule DC-IDT2E with 4,4,9,9-tetrakis(4-hexylphenyl)-indaceno[1,2-b:5,6-bt]dithiophene as a central building block, furan as rr-bridges, and 1,1 -dicyanomethylene-3-indanone as end acceptor groups, was synthesized and used as an electron acceptor in solution-processed organic solar cells (OSCs). DC-IDT2F exhibited good thermal stability, broad and strong absorption in 500-850 rim, a narrow bandgap of 1.54 eV, LUMO of-3.88 eV, HOMO of-5.44 eV and an electron mobility of 6.5 × 10-4 cm2/(V.s). DC-IDT2F-based OSCs with conventional and inverted structures exhibited power conversion efficiencies of 2.26 and 3.08% respec- tively. The effect of vertical phase separation and morphology of the active layer on the device performance in the two structures was studied.
基金supported by the National Natural Science Foundation of China(No.41806099)the Global Change and Air-Sea Interaction Project of China(No.GASI-04-HYST-06).
文摘The spatial distribution and seasonal variations of the hypoxic zone in the eastern equatorial Indian Ocean were investigated using survey data collected from four cruises from 2013 to 2018.Results showed that hypoxic zone occurred all year round in the eastern equatorial Indian Ocean,and it spread southward in the shape of a double tongue at two depths with one at subsurface centered at a depth of 150 m and the other in intermediate water centered at a depth of 800 m.The southward expansion and maximum thickness of the hypoxic zone were greatest in the spring inter-monsoon and least in the summer monsoon.The hypoxic zone originated from the southward expansion of the hypoxic water in the Bay of Bengal and its spatial distribution was driven by southward output flux of mid-deep(100–1000 m)hypoxic water from the Bay of Bengal.The hypoxia southward expansion was blocked near the equator in the subsurface layer,because of mixing with multiple zonal circulations(e.g.,Wyrtki Jets and the equatorial undercurrent),which meant that the hypoxic zone extended over a smaller area than in the intermediate water.These new findings will contribute to an improved understanding of the hypoxic zone and will contribute to circulation research,particularly about intermediate circulation in the eastern equatorial Indian Ocean.
基金supported by National Natural Science Foundation of China (GrantNo 40830102)the program "The Multi-scale Comprehensive Observation and Study of Spatial-Temporal Properties of Aerosol Project (MOSTap)" of National Basic Research Program of China (973 Program Grant No 2010CB950804)
文摘The accuracies of three instruments in measuring atmospheric column humidity were assessed during an upper troposphere and lower stratosphere observation campaign conducted from 7 to 13 August 2009 in Kunming, China. The three instruments are a cryogenic frost-point hygrometer (CFH), a Vaisala RS80 radiosonde (RS80), and a GTS1 radiosonde (GTS1). The accuracy of relative humidity (RH) measurements made by the CFH, GTS1, and RS80 was similar between the surface and 500 hPa (~5.5 km above sea level). However, above 500 hPa, the errors in RH measurements made by the RS80, relative to measurements made by the CFH, are much less than those detected with the GTS1. Three different retrieval methods for determining cloud boundaries from CFH, RS80, and GTS1 measurements were developed and take into account the differences in accuracy among the three instruments. The method for the CFH is based on RH thresholds at all levels, which demands high accuracy. Given that the accuracy of RH measurements decreases at higher altitudes, the cloud detection methods for RS80 and GTS1 are different for different altitude ranges. Below 5 km, the methods for the RS80 and the GTS1 are similar to that of the CFH; above 5 km, the methods for the RS80 and the GTS1 are both developed based on the second-order derivatives of temperature and RH with respect to height, but with different criteria applied. Comparisons of cloud-layer retrievals derived from the three measurements are also made.