This study investigates changes in summer water vapor transport(WVT) over East Asia under 1.5°C and 2.0°C global warming(GW) for the +4.5 and +8.5 W m-2 Representative Concentration Pathway(RCP) scenarios(RC...This study investigates changes in summer water vapor transport(WVT) over East Asia under 1.5°C and 2.0°C global warming(GW) for the +4.5 and +8.5 W m-2 Representative Concentration Pathway(RCP) scenarios(RCP4.5 and RCP8.5, respectively). Of the 27 models used, 18 show better skill in simulating the climatological summer WVT over East Asia of the present day. Of those 18, 13 reach 1.5°C and 2.0°C GW for the two RCPs. Based on these 13 models, results show that — relative to the present day-th e summer WVT is enhanced over East Asia under 1.5°C and 2.0°C GW for RCP4.5 and RCP8.5. The inte r-model consistency is higher under 2.0°C GW. Increased water vapor content favors the enhanced WVT over both southern and northern East Asia, while lower-level circulation contributes to the enhanced WVT over southern East Asia. Compared to 1.5°C GW, th e summer WVT under 2.0°C GW is further enhanced over most of East Asia for RCP4.5. For RCP8.5, the summer WVT is also further enhanced over southern East Asia, while this is not the case over northern East Asia. Under the additional 0.5°C GW, the changes in summer WVT, with low in ter-model consistency, are closely related to anomalous lower-level circulation. Precipitation increases over the East China Sea to southern Japan, the Korean Peninsula, and North China, for both RCP4.5 and RCP8.5. However, the changes in precipitation over the South China Sea and Northeast China are different for the two RCPs. This is connected to the difference in the changes of WVT divergence.展开更多
The outputs of 17 models in the Coupled Model Intercomparison Project Phase 5 (CMIP5) are employed to investigate the temporal and spatial features of 2.0°C warming of the surface temperature over the globe and C...The outputs of 17 models in the Coupled Model Intercomparison Project Phase 5 (CMIP5) are employed to investigate the temporal and spatial features of 2.0°C warming of the surface temperature over the globe and China under the Representative Concentration Pathways (RCP) 4.5 scenario. The simulations of the period 1860-1899 in the "historical" experiment are chosen as the baseline. The simulations for the 21st century in the RCP4.5 experiment are chosen as the future project. The multi-model ensemble mean (MME) shows that the global mean temperature would cross the 2.0°C warming threshold in 2047. Warming in most of the models would cross the threshold during 2030-2060. For local warming, high-latitude areas in the Northern Hemisphere show the fastest warming over the globe. Land areas warm substantially faster than the oceans. Most of the southern oceans would not exceed the 2.0°C warming threshold within the 21st century. Over China, surface warming is substantially faster than the global mean. The area-averaged warming would cross the 2.0°C threshold in 2034. Locally, Northwest China shows the fastest warming trend, followed by Central North China and Northeast China. Central China, East China, and South China are the last to cross the 2.0°C warming threshold. The diversity of the models is also estimated in this study. Generally, the spread among the models increases with time, and there is smaller spread among the models for the areas with the faster warming.展开更多
The oxidation behavior of Hastelloy C-2000 alloy was investigated in air at 800 °C and 1000 °C for 100 h, respectively. Oxidation kinetics and oxide scales morphologies were examined by mass gain measurement...The oxidation behavior of Hastelloy C-2000 alloy was investigated in air at 800 °C and 1000 °C for 100 h, respectively. Oxidation kinetics and oxide scales morphologies were examined by mass gain measurement, scanning electron microscopy（SEM）, X-ray diffraction（XRD） and X-ray photoelectron spectroscopy（XPS）. The oxidation behavior of the alloy approximately follows a parabolic rate law. Moreover, annealing twins defect structure in matrix deteriorates the oxidation resistance of alloy due to the improvement of diffusion rates for alloying elements and oxygen atoms. At 800 °C, the microstructure is primarily composed of Ni O and Cr1.3Fe0.7O6 and the initial annealing twins structure is visible and Mo-rich phases are emerged to approach boundary of oxide scales. At 1000 °C, however, the morphology microstructure of oxide scales consists of oxide particle with fine Cr oxides and large Ni oxides by inlaying each other, whilst Mo-rich phases hardly appear closing to the interface of oxide scales.展开更多
化工、纺织印染与农药化肥等产业的蓬勃发展推动着人类社会的进步,但同时也给环境治理带来了巨大难题。目前,光催化降解局限于在特定波长下针对单一有机污染物进行降解,然而现实中的情况往往更复杂。因此,开发一种多功能光催化材料用于...化工、纺织印染与农药化肥等产业的蓬勃发展推动着人类社会的进步,但同时也给环境治理带来了巨大难题。目前,光催化降解局限于在特定波长下针对单一有机污染物进行降解,然而现实中的情况往往更复杂。因此,开发一种多功能光催化材料用于光催化降解不同有机污染物显得尤为重要。采用一步无模板溶剂热法合成了核壳结构的C-TiO_(2)复合材料前驱体,并在氩气气氛下煅烧得到高结晶度的C-TiO_(2)复合光催化材料。运用SEM、TEM、XRD和TG等表征手段对材料进行表征,结论如下:550℃煅烧时的样品为包含少量碳的高结晶度的锐钛矿相TiO 2,且550℃煅烧时的样品依然保持了完整的核壳结构。此外,C-TiO_(2)复合材料的比表面积高达85.69 m 2·g^(-1),平均孔径为16.4 nm以及孔体积为0.423 m 3·g^(-1)。在UV-Vis光照射下,C-TiO_(2)复合材料分别对罗丹明B(RhB)、亚甲基蓝(MB)和刚果红(CR)3种染料显示出增强的光催化降解活性。展开更多
基金jointly supported by the National Key R&D Program of China [grant number 2017YFA0603802]the National Natural Science Foundation of China [grant numbers 41421004,41325018,and 41805062]
文摘This study investigates changes in summer water vapor transport(WVT) over East Asia under 1.5°C and 2.0°C global warming(GW) for the +4.5 and +8.5 W m-2 Representative Concentration Pathway(RCP) scenarios(RCP4.5 and RCP8.5, respectively). Of the 27 models used, 18 show better skill in simulating the climatological summer WVT over East Asia of the present day. Of those 18, 13 reach 1.5°C and 2.0°C GW for the two RCPs. Based on these 13 models, results show that — relative to the present day-th e summer WVT is enhanced over East Asia under 1.5°C and 2.0°C GW for RCP4.5 and RCP8.5. The inte r-model consistency is higher under 2.0°C GW. Increased water vapor content favors the enhanced WVT over both southern and northern East Asia, while lower-level circulation contributes to the enhanced WVT over southern East Asia. Compared to 1.5°C GW, th e summer WVT under 2.0°C GW is further enhanced over most of East Asia for RCP4.5. For RCP8.5, the summer WVT is also further enhanced over southern East Asia, while this is not the case over northern East Asia. Under the additional 0.5°C GW, the changes in summer WVT, with low in ter-model consistency, are closely related to anomalous lower-level circulation. Precipitation increases over the East China Sea to southern Japan, the Korean Peninsula, and North China, for both RCP4.5 and RCP8.5. However, the changes in precipitation over the South China Sea and Northeast China are different for the two RCPs. This is connected to the difference in the changes of WVT divergence.
基金supported by the National Basic Research Program of China(Grant No.2009CB421407)
文摘The outputs of 17 models in the Coupled Model Intercomparison Project Phase 5 (CMIP5) are employed to investigate the temporal and spatial features of 2.0°C warming of the surface temperature over the globe and China under the Representative Concentration Pathways (RCP) 4.5 scenario. The simulations of the period 1860-1899 in the "historical" experiment are chosen as the baseline. The simulations for the 21st century in the RCP4.5 experiment are chosen as the future project. The multi-model ensemble mean (MME) shows that the global mean temperature would cross the 2.0°C warming threshold in 2047. Warming in most of the models would cross the threshold during 2030-2060. For local warming, high-latitude areas in the Northern Hemisphere show the fastest warming over the globe. Land areas warm substantially faster than the oceans. Most of the southern oceans would not exceed the 2.0°C warming threshold within the 21st century. Over China, surface warming is substantially faster than the global mean. The area-averaged warming would cross the 2.0°C threshold in 2034. Locally, Northwest China shows the fastest warming trend, followed by Central North China and Northeast China. Central China, East China, and South China are the last to cross the 2.0°C warming threshold. The diversity of the models is also estimated in this study. Generally, the spread among the models increases with time, and there is smaller spread among the models for the areas with the faster warming.
基金Project(2013AA031004)supported by the National High-tech Research and Development Program of China
文摘The oxidation behavior of Hastelloy C-2000 alloy was investigated in air at 800 °C and 1000 °C for 100 h, respectively. Oxidation kinetics and oxide scales morphologies were examined by mass gain measurement, scanning electron microscopy（SEM）, X-ray diffraction（XRD） and X-ray photoelectron spectroscopy（XPS）. The oxidation behavior of the alloy approximately follows a parabolic rate law. Moreover, annealing twins defect structure in matrix deteriorates the oxidation resistance of alloy due to the improvement of diffusion rates for alloying elements and oxygen atoms. At 800 °C, the microstructure is primarily composed of Ni O and Cr1.3Fe0.7O6 and the initial annealing twins structure is visible and Mo-rich phases are emerged to approach boundary of oxide scales. At 1000 °C, however, the morphology microstructure of oxide scales consists of oxide particle with fine Cr oxides and large Ni oxides by inlaying each other, whilst Mo-rich phases hardly appear closing to the interface of oxide scales.
文摘化工、纺织印染与农药化肥等产业的蓬勃发展推动着人类社会的进步,但同时也给环境治理带来了巨大难题。目前,光催化降解局限于在特定波长下针对单一有机污染物进行降解,然而现实中的情况往往更复杂。因此,开发一种多功能光催化材料用于光催化降解不同有机污染物显得尤为重要。采用一步无模板溶剂热法合成了核壳结构的C-TiO_(2)复合材料前驱体,并在氩气气氛下煅烧得到高结晶度的C-TiO_(2)复合光催化材料。运用SEM、TEM、XRD和TG等表征手段对材料进行表征,结论如下:550℃煅烧时的样品为包含少量碳的高结晶度的锐钛矿相TiO 2,且550℃煅烧时的样品依然保持了完整的核壳结构。此外,C-TiO_(2)复合材料的比表面积高达85.69 m 2·g^(-1),平均孔径为16.4 nm以及孔体积为0.423 m 3·g^(-1)。在UV-Vis光照射下,C-TiO_(2)复合材料分别对罗丹明B(RhB)、亚甲基蓝(MB)和刚果红(CR)3种染料显示出增强的光催化降解活性。
