Two dimensional Fourier transforrn electronic spectroscopy (2DES) in the visible region enables direct observation of complex dynamics of molecules including quantum coherence in the condensed phase. This review aim...Two dimensional Fourier transforrn electronic spectroscopy (2DES) in the visible region enables direct observation of complex dynamics of molecules including quantum coherence in the condensed phase. This review aims to provide a bridge between the principles and intuitive physical description of 2DES for tutorial purpose. Special emphasis is laid upon how 2DES circumvents the restrictions from both uncertainty principle and the wave-packet collapse during the coherent detection, leading to the successful detection of the coherence in terms of energy difference between the eigenstates showing as the quantum beats; then upon the possible mixing among the pure electronic transition, single-rnode and multi-mode coupled vibronic transition leading to the observed beating phenomena. Finally, recent ad- vances in experimentally distinguishing between the electronic coherence and the vibrational coherence are briefly discussed.展开更多
Diversity in the neurons and noise are inevitable in the real neuronal network.In this paper,parameter diversity induced spiral waves and multiple spatial coherence resonances in a two-dimensional neuronal network wit...Diversity in the neurons and noise are inevitable in the real neuronal network.In this paper,parameter diversity induced spiral waves and multiple spatial coherence resonances in a two-dimensional neuronal network without or with noise are simulated.The relationship between the multiple resonances and the multiple transitions between patterns of spiral waves are identified.The coherence degrees induced by the diversity are suppressed when noise is introduced and noise density is increased.The results suggest that natural nervous system might profit from both parameter diversity and noise,provided a possible approach to control formation and transition of spiral wave by the cooperation between the diversity and noise.展开更多
基金supported by the National Natural Science Foundation of China (No.21227003, No.21433014, No.11721404)
文摘Two dimensional Fourier transforrn electronic spectroscopy (2DES) in the visible region enables direct observation of complex dynamics of molecules including quantum coherence in the condensed phase. This review aims to provide a bridge between the principles and intuitive physical description of 2DES for tutorial purpose. Special emphasis is laid upon how 2DES circumvents the restrictions from both uncertainty principle and the wave-packet collapse during the coherent detection, leading to the successful detection of the coherence in terms of energy difference between the eigenstates showing as the quantum beats; then upon the possible mixing among the pure electronic transition, single-rnode and multi-mode coupled vibronic transition leading to the observed beating phenomena. Finally, recent ad- vances in experimentally distinguishing between the electronic coherence and the vibrational coherence are briefly discussed.
基金Supported by National Natural Science Foundation of China under Grant Nos.11072135 and 10772101the Fundamental Research Funds for the Central Universities under Grant No.GK200902025
文摘Diversity in the neurons and noise are inevitable in the real neuronal network.In this paper,parameter diversity induced spiral waves and multiple spatial coherence resonances in a two-dimensional neuronal network without or with noise are simulated.The relationship between the multiple resonances and the multiple transitions between patterns of spiral waves are identified.The coherence degrees induced by the diversity are suppressed when noise is introduced and noise density is increased.The results suggest that natural nervous system might profit from both parameter diversity and noise,provided a possible approach to control formation and transition of spiral wave by the cooperation between the diversity and noise.