The physical absorption of CO2 in water containing different types of particles was studied in a micro-channel operated under Taylor flow. The maximum enhancement factors of 1.43-2.15 were measured for activated carb...The physical absorption of CO2 in water containing different types of particles was studied in a micro-channel operated under Taylor flow. The maximum enhancement factors of 1.43-2.15 were measured for activated carbon （AcC） particles. The analysis shows that the enhancement effect can be attributed to the shuttle mechanism. Considering the separate contributions of mass transfer from bubble cap and liquid film, a heterogeneous enhance- ment model is developed. According to this model, the enhancement factors Ecap, EFilm and Eov are mainly determined by mass transfer coefficient gL （gL Cap and KL Film）, adsorptive capacity of particles m, and coverage fraction of particles at gas-liquid interface （. With both effects of particle-to-interface adhesion and apparent viscosity included, the model nredicts the enhancement effect of AcC varticles reasonably well.展开更多
This paper studies the mass transfer performance of structured packings in the absorption of CO2 from air with aqueous Na OH solution. The Eight structured packings tested are sheet metal ones with corrugations of dif...This paper studies the mass transfer performance of structured packings in the absorption of CO2 from air with aqueous Na OH solution. The Eight structured packings tested are sheet metal ones with corrugations of different geometry parameters. Effective mass transfer area and overall gas phase mass transfer coefficient have been measured in an absorption column of 200 mm diameter under the conditions of gas F-factor in 0.38–1.52 Pa0.5and aqueous Na OH solution concentration of 0.10–0.15 kmol·m-3. The effects of gas/liquid phase flow rates and packing geometry parameters are also investigated. The results show that the effective mass transfer area changes not only with packing geometry parameters and liquid load, but also with gas F-factor. A new effective mass transfer area correlation on the gas F-factor and the liquid load was proposed, which is found to fit experiment data very well.展开更多
Marangoni convection and its influence on the mass transter in the liquid phase were investigated. Marangoni convection was visualized using laser Schlieren technique, Orderly polygonal convection patterns and random ...Marangoni convection and its influence on the mass transter in the liquid phase were investigated. Marangoni convection was visualized using laser Schlieren technique, Orderly polygonal convection patterns and random interfacial turbulence were observed. The effect of Marangoni convection on the mass transfer rate was studied by desorbing ethanol from aqneous solution in the falling film. The experimental results show that Marangoni convection can speed up the surface real and enhance the mass transfer rate in the liquid phase.The liquid mass transfer coefficient can be enhanced by as much as 3 folds. The corresponding empirical correlations are given in terms of the mass transfer enhancement factor. Furthermore, in considering the Marangoni effect, the conventional mass transfer correlation was modified, The differences between the values predicted by the correlation and the experimental data are within ±8.2% and the average difference is 4.2%.展开更多
基金Supported by the National＇Natural Science Foundation of China （20706041, 20876109）, and the Natural Science Foundation of Tianjin, China （09JCYBJC06500）.
文摘The physical absorption of CO2 in water containing different types of particles was studied in a micro-channel operated under Taylor flow. The maximum enhancement factors of 1.43-2.15 were measured for activated carbon （AcC） particles. The analysis shows that the enhancement effect can be attributed to the shuttle mechanism. Considering the separate contributions of mass transfer from bubble cap and liquid film, a heterogeneous enhance- ment model is developed. According to this model, the enhancement factors Ecap, EFilm and Eov are mainly determined by mass transfer coefficient gL （gL Cap and KL Film）, adsorptive capacity of particles m, and coverage fraction of particles at gas-liquid interface （. With both effects of particle-to-interface adhesion and apparent viscosity included, the model nredicts the enhancement effect of AcC varticles reasonably well.
基金Supported by the National Natural Science Foundation of China(51134017)and Petro China(2011E-24-09)
文摘This paper studies the mass transfer performance of structured packings in the absorption of CO2 from air with aqueous Na OH solution. The Eight structured packings tested are sheet metal ones with corrugations of different geometry parameters. Effective mass transfer area and overall gas phase mass transfer coefficient have been measured in an absorption column of 200 mm diameter under the conditions of gas F-factor in 0.38–1.52 Pa0.5and aqueous Na OH solution concentration of 0.10–0.15 kmol·m-3. The effects of gas/liquid phase flow rates and packing geometry parameters are also investigated. The results show that the effective mass transfer area changes not only with packing geometry parameters and liquid load, but also with gas F-factor. A new effective mass transfer area correlation on the gas F-factor and the liquid load was proposed, which is found to fit experiment data very well.
基金Supported by National Natural Science Foundation of China(No.20136010).
文摘Marangoni convection and its influence on the mass transter in the liquid phase were investigated. Marangoni convection was visualized using laser Schlieren technique, Orderly polygonal convection patterns and random interfacial turbulence were observed. The effect of Marangoni convection on the mass transfer rate was studied by desorbing ethanol from aqneous solution in the falling film. The experimental results show that Marangoni convection can speed up the surface real and enhance the mass transfer rate in the liquid phase.The liquid mass transfer coefficient can be enhanced by as much as 3 folds. The corresponding empirical correlations are given in terms of the mass transfer enhancement factor. Furthermore, in considering the Marangoni effect, the conventional mass transfer correlation was modified, The differences between the values predicted by the correlation and the experimental data are within ±8.2% and the average difference is 4.2%.
