Eu^(2+)在磷酸镧中的发光及Ce^(3+)→Eu^(2+)的能量传递

采用高温固相反应合成了LaPO4∶Eu2+和LaPO4∶Ce3+,Eu2+样品,报道了Eu2+在LaPO4中的发光性质和Ce3+→Eu2+的能量传递现象。文中探讨了Ce3+→Eu2+的能量传递机理,根据Dexter电多极相互作用的理论证明其为偶极子 偶极子相互作用的共振能量传递。

Gd_(2)ZnTiO_(6):Sm^(3+)荧光粉的制备及发光性能研究

通过溶胶-凝胶法制备出一系列Gd_(2-2x)ZnTiO_(6):xSm^(3+)(x=0,0.01,0.03,0.05,0.07,0.09,0.11)橙红色荧光粉,并对样品的晶体结构、微观形貌及荧光性能进行了测试和研究。结果表明:所制Gd_(2)ZnTiO_(6):Sm^(3+)(GZT:Sm^(3+))荧光粉均为双钙钛矿结构,属于单斜晶系(空间群:P2_(1)/n),由几十微米大小无规则形状的颗粒堆积而成。在407nm近紫外光激发下,GZT:Sm^(3+)的发射光谱展示出两个较弱的发射峰(^(4)G_(5/2)→_(6)H_(5/2),566nm;^(4)G_(5/2)→^(6)H_(9/2),650nm)和一个较强的发射峰(^(4)G_(5/2)→^(6)H_(7/2),603nm)。当Sm^(3+)离子摩尔浓度为5%时,GZT:Sm^(3+)样品发生浓度淬灭现象;基于Dexter的理论,浓度淬灭效应机制为电偶极子-电偶极子(d-d)相互作用。Sm^(3+)离子掺杂浓度较低时,样品呈现橙红色,随着掺杂浓度增加,荧光粉发光颜色逐渐向黄橙色区域偏移,其中Gd_(1.98)ZnTiO_(6):0.02Sm^(3+)荧光粉CIE色坐标为(0.6155,0.3835)与标准红光色坐标(0.670,0.330)较为接近,是很有潜力的LED用橙红色荧光粉。

Spontaneous Formation of Anti-ferromagnetic Vortex Lattice in a Fast Rotating BEC with Dipole Interactions

When a Bose-Einstein condensate is set to rotate, superfluid vortices will be formed, which finally condense into a vortex lattice as the rotation frequency further increases. We show that the dipole-dipole interactions renormalize the short-range interaction strength and result in a distinction between interactions of parallel-polarized atoms and interactions of antiparallel-polarized atoms. This effect may lead to a spontaneous breakdown of the rapidly rotating Bose condensate into a novel anti-ferromagnetic-like vortex lattice. The upward-polarized Bose condensate forms a vortex lattice, which is staggered against a downward-polarized vortex lattice. A phase diagram related to the coupling strength is obtained.

Entanglement Properties Between Two Spatially Separated Atoms with Cascade Configuration in Free Space

We investigate the entanglement properties between two identical atoms with cascade configuration through the retarded dipole-dipole interaction in free space when their spatial separation is on the order of radiation wavelength or less. We analyze the function of Hamiltonian induced by dipole-dipole interaction. By solving master equation, we show that the spontaneous emission induce entanglement and destroy entanglement too. We also show the long life time of entanglement within cascade configuration.

LINKAGE BETWEEN INDIAN OCEAN DIPOLE AND TWO TYPES OF El NI?O AND ITS POSSIBLE MECHANISMS

After compositing three representative ENSO indices,El Nio events have been divided into an eastern pattern(EP) and a central pattern(CP).By using EOF,correlation and composite analysis,the relationship and possible mechanisms between Indian Ocean Dipole(IOD) and two types of El Nio were investigated.IOD events,originating from Indo-Pacific scale air-sea interaction,are composed of two modes,which are associated with EP and CP El Ni o respectively.The IOD mode related to EP El Nio events(named as IOD1) is strongest at the depth of 50 to 150 m along the equatorial Indian Ocean.Besides,it shows a quasi-symmetric distribution,stronger in the south of the Equator.The IOD mode associated with CP El Nio(named as IOD2) has strongest signal in tropical southern Indian Ocean surface.In terms of mechanisms,before EP El Nio peaks,anomalous Walker circulation produces strong anomalous easterlies in equatorial Indian Ocean,resulting in upwelling in the east,decreasing sea temperature there;a couple of anomalous anticyclones(stronger in the south) form off the Equator where warm water accumulates,and thus the IOD1 occurs.When CP El Nio develops,anomalous Walker circulation is weaker and shifts its center to the west,therefore anomalous easterlies in equatorial Indian Ocean is less strong.Besides,the anticyclone south of Sumatra strengthens,and the southerlies east of it bring cold water from higher latitudes and northerlies west of it bring warm water from lower latitudes to the 15° to 25°S zone.Meanwhile,there exists strong divergence in the east and convergence in the west part of tropical southern Indian Ocean,making sea temperature fall and rise separately.Therefore,IOD2 lies farther south.

A Position-Dependent Two-Atom Entanglement in Real-Time Cavity QED System

We study a special two-atom entanglement case in assumed cavity QED experiment in which only one atom effectively exchanges a single photon with a cavity mode. We compute two-atom entanglement under position-dependent atomic resonant dipole-dipole interaction （RDDI） for large interatomic separation limit. We show that the RDDI, even t, hat which is much smaller than the maximal atomic Rabi frequency, can induce distinct diatom entanglement. The peak entanglement reaches a maximum when RDDI strength can compare with the Rabi frequency of an atom.

The Interacting Boson Model of Dipole—Octupole Strong Correlations in SU（3） Limit for Positive Parity States

Within the framework of the Usdpf(16) interacting boson model (IBM), the effects of strong correlations of the dipole (p?-boson) and the octupole (f?-boson) degree of freedom on the positive-parity states of even-even nuclei in SU(3) limit are discussed. It is shown that configurations of an even number of many p- and f-bosons can not only be incorporated into the usual low-lying collective rotational bands, such as the ground state band, β- and γ-vibrational bands, but also naturally form the rotational bands, etc. These results are similar to that of Usdg(15)-IBM and in good agreement with the experimental data of the nucleus. Besides, several intraband E2 transition probabilities are given, which are consistent with that of Usd(6)-IBM.

The Role of the Dipole Interaction of Molecules with Charged Particles in the Polar Stratosphere

Our analysis of published results of experiments in the Polar Regions substantiates and further develops our new approach to the photochemical processes in the polar stratosphere involving the charged particles. The dipole interaction of molecules with charged particles, primarily with ions, leads to the adhesion and disintegration of a number of molecules including ozone. Molecules acquire additional energy on the surface of the charged particles, enabling reactions that are not possible in space. Galactic cosmic rays are the main source of ions in the polar stratosphere, their equilibrium concentration at altitudes of 15 to 25 km can reach up ~ （1-5） ~ 103 ions/cm3. Estimations show that if the ozone destruction in the regime of＂collision＂ with ions then the lifetime of ozone will vary from 10 days to 2 months. We suppose that alongside with the chlorine mechanism of ozone destruction there is a mechanism of ozone decay on a charged particle which can act also at those latitudes and altitudes where chlorine oxide CIO is absent, as well as in the night conditions. Here, we demonstrated the close connection of photochemical processes with the dynamic, electrical and condensational phenomena in the stratosphere, in particular, with the accumulation of unipolar charged particles on the upper and lower boundaries of the polar stratospheric clouds and aerosol layers as a result of the activity of the global electric circuit.

经典驱动Tavis-Cummings模型中原子纠缠特性的研究

研究了受经典场驱动的两个二能级原子与单模腔场相互作用系统中两原子的纠缠动力学行为。该工作主要是对原子间的偶极子-偶极子(偶偶)相互作用和经典场驱动同时存在的Tavis-Cummings模型进行了研究,采用数值计算的方法,详细分析了经典场的驱动强度、原子间的偶偶相互作用强度和原子与腔场之间的失谐量对原子纠缠特性的影响。同时讨论了原子与腔场共振和非共振两种情况下,原子间偶偶相互作用和经典场驱动强度的最优参数区域。结果表明,适当调节经典场的驱动强度,原子间的偶偶相互作用强度和原子与腔场之间的失谐量,可以使原子的纠缠突然死亡现象得到抑制。

C-NOT gate based on ultracold Rydberg atom interactions

The Rydberg states of neutral atoms are strongly polarisable and possess long lifetimes because of high energies which can lead to strong and long range dipole-dipole interactions.The energy levels corresponding to these states are shifted because of dipole-dipole interactions and can be used to block transitions of more than one excitation in the Rydberg regime.This reputed Rydberg blockade is obtained when the excitation is shifted out of resonance by these interactions.Electromagnetically induced transparency(EIT)is sensitive to a small detuning.At large distances,up to several micrometers,the interactions can interrupt the EIT consequence.Herein we investigate a novel scheme based on EIT and Rydberg blockade and performed a simulation of a controlled-NOT(C-NOT)quantum gate which is critical for quantum computation by using neutral atoms.

Fe3O4 Octahedral Colloidal Crystals

We present a facile and controllable method for the large-scale fabrication of highly-ordered octahedral Fe3O4 colloidal ＂single crystals＂ without the assistance of a substrate. Oleic acid is used to reduce the solubility of the nano-building blocks in colloidal solution and to induce a ＂crystallization＂ process. Our colloidal crystals are of multimicron size and show typical crystallographic characteristics. They have a very robust structure and can serve as a novel ordered magnetic mesoporous material with a relatively narrow pore size distribution. The sample possesses an extremely high Verwey transition temperature （Tv） of 100 K and a high saturation magnetization （Ms） of 86 emu/g at 5 K based on its good crystallinity, as well as the interparticle dipolar interaction behavior arising from its unique structure. Electrochemical measurements have demonstrated the excellent capacity of the mesoporous colloidal crystals when used in lithium-ion batteries.

Interaction-Induced Chiral Quantum States of the Ultracold Polar Molecules

The ultracold polar molecules with the tunable dipole-dipole interaction, not only would enable explorations of a large class of exotic many-body physics phenomena, but also could be used for quantum information processing. In the present paper we demonstrate that this dipole-dipole interaction can generate the degenerate chiral quantum states acting as a qubit robust against noise when the ultracold polar molecules are confined by a triangular lattice. Moreover, we also find two first-order quantum phase transitions by controlling an external driving t^eld. One is the transition with the change of the different degenerate chiral quantum states. The other is the transition with the breaking of the degenerate quantum chirAL states to the nondegenerate state. In experiment, these first-order quantum phase transitions can be detected by measuring the collective molecular population.

Efficient Excitation of a Symmetric Collective Atomic State with a Single-Photon Through Dipole Blockade

In the famous quantum communication scheme developed by Duan et al.[L.M.Duan,M.D.Lukin,J.I.Cirac,and P.Zoller,Nature(London) 414(2001) 413],the probability of successful generating a symmetric collective atomic state with a single-photon emitted have to be far smaller than 1 to obtain an acceptable entangled state.Based on strong dipole-dipole interaction between two Rydberg atoms,two simultaneous excitations in an atomic ensemble are greatly suppressed,which makes it possible to excite a mesoscopic cold atomic ensemble into a near-ideal singly-excited symmetric collective state accompanied by a signal-photon with near unity success probability.

Dynamic Structure Factor of an Optically Trapped Dipolar Bose–Einstein Condensate

Motivated by the recent experimental achievements in using the Bragg spectroscopy to measure the excitation spectrum of an ultra-cold atomic system with long-range interactions, we investigate the dynamic structure factor of a cigar-shaped dipolar Bose condensate trapped in a one-dimensional optical lattices. Our results show that the Bogoliubov bands of the system, particularly the lowest one, can be significantly influenced when one tunes the dipole orientation. Consequently, the calculated static structure factor of an optically trapped dipolar Bose gas shows marked difference from the non-dipolar one. Moreover, we show that the effects of dipole-dipole interaction on the dynamic structure factor is also strongly affected by the strength of the optical confinement.

Quantum Interference of Dual-Channel Excited Magnons in Spin-1 Bose-Einstein Condensates Atomic Chain

We investigate the quantum interference of spin wave excitations of a spin-1 atomic Bose condensate confined in an optical lattice. Single-channel and dual-channel interactions are employed in our system, and their induced excitations are compared. Also we consider the interplay of magneto-optical excitations, which leads to a constructive or destructive effect for the creation of magnons based on background excitations. The population distributions of excited magnons can be well controlled by steering the long-range dipole-dipole interactions. Such a scheme can be used to demonstrate conventional quantum-optical phenomena like dynamical Casimir effect at finite temperatures.