By means of improved ligand-field theory, the "pure electronic" pressure-induced shifts (PS's) and the PS's due to electron-phonon interaction (EPI) of R1 line and R2 line of YAG:Cr^3+ have been calculated, ...By means of improved ligand-field theory, the "pure electronic" pressure-induced shifts (PS's) and the PS's due to electron-phonon interaction (EPI) of R1 line and R2 line of YAG:Cr^3+ have been calculated, respectively. The calculated results are in very good agreement with the experimental data. It is demonstrated that the admixture of │t^2 2(^3T1)e^4T2〉 and │t^3 2 ^2E〉 bases in the wavefunction of RI level of YAG:Crs+ and its change with pressure play a key role for the PS of RI line. The behaviors of the "pure electronic" PS of RI line and the PS of RI line due to EPI are different. It is the combined eEect of them that gives rise to the total PS of R1 line, which has satisfactorily explained the experimental results. The systematic analyses and comparisons between the feature of R1-line PS of YAG:Cr^3+ and the ones of three laser crystals (GSGG:Cr^3+, GGG:Cr^3+ and ruby) have been made, and the origin of the difference between them has been revealed.展开更多
The recent discovery and realizations of higher-order topological insulators enrich the fundamental studies on topological phases.Here,we report three-dimensional(3D)wave-steering capabilities enabled by topological b...The recent discovery and realizations of higher-order topological insulators enrich the fundamental studies on topological phases.Here,we report three-dimensional(3D)wave-steering capabilities enabled by topological boundary states at three different orders in a 3D phononic crystal with nontrivial bulk topology originated from the synergy of mirror symmetry of the unit cell and a non-symmorphic glide symmetry of the lattice.The multitude of topological states brings diverse possibilities of wave manipulations.Through judicious engineering of the boundary modes,we experimentally demonstrate two functionalities at different dimensions:2D negative refraction of sound wave enabled by a firstorder topological surface state with negative dispersion,and a 3D acoustic interferometer leveraging on second-order topological hinge states.Our work showcases that topological modes at different orders promise diverse wave steering applications across different dimensions.展开更多
文摘By means of improved ligand-field theory, the "pure electronic" pressure-induced shifts (PS's) and the PS's due to electron-phonon interaction (EPI) of R1 line and R2 line of YAG:Cr^3+ have been calculated, respectively. The calculated results are in very good agreement with the experimental data. It is demonstrated that the admixture of │t^2 2(^3T1)e^4T2〉 and │t^3 2 ^2E〉 bases in the wavefunction of RI level of YAG:Crs+ and its change with pressure play a key role for the PS of RI line. The behaviors of the "pure electronic" PS of RI line and the PS of RI line due to EPI are different. It is the combined eEect of them that gives rise to the total PS of R1 line, which has satisfactorily explained the experimental results. The systematic analyses and comparisons between the feature of R1-line PS of YAG:Cr^3+ and the ones of three laser crystals (GSGG:Cr^3+, GGG:Cr^3+ and ruby) have been made, and the origin of the difference between them has been revealed.
基金supported by the King Abdullah University of Science and Technology (KAUST) Office of Sponsored Research (OSR) under Award No. OSR-2016-CRG5-2950KAUST Baseline Research Fund BAS/1/1626-01-01+3 种基金supported by the Hong Kong Research Grants Council (GRF 12302420, 12300419, ECS 22302718, CRF C6013-18G)the National Natural Science Foundation of China via the Excellent Young Scientist Scheme (Hong Kong & Macao) (#11922416)the Youth Program (#11802256)Hong Kong Baptist University (RC-SGT2/18-19/ SCI/006)。
文摘The recent discovery and realizations of higher-order topological insulators enrich the fundamental studies on topological phases.Here,we report three-dimensional(3D)wave-steering capabilities enabled by topological boundary states at three different orders in a 3D phononic crystal with nontrivial bulk topology originated from the synergy of mirror symmetry of the unit cell and a non-symmorphic glide symmetry of the lattice.The multitude of topological states brings diverse possibilities of wave manipulations.Through judicious engineering of the boundary modes,we experimentally demonstrate two functionalities at different dimensions:2D negative refraction of sound wave enabled by a firstorder topological surface state with negative dispersion,and a 3D acoustic interferometer leveraging on second-order topological hinge states.Our work showcases that topological modes at different orders promise diverse wave steering applications across different dimensions.